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1. 发明申请

US20070275852A1 Molecular Sieve With Mfi Structure Containing Phosphorus and Metal Components, Preparation Process and Use Thereof 有权
标题翻译：含有磷和金属成分的Mfi结构的分子筛，其制备方法和用途
公开(公告)号：US20070275852A1
公开(公告)日：2007-11-29
申请号：US10577672
申请日：2004-10-28
申请人： Yibin Luo , Ying Ouyang , Xingtian Shu , Mingyuan He , Dianzhong Wang , Baoning Zong , Minggang Li
发明人： Yibin Luo , Ying Ouyang , Xingtian Shu , Mingyuan He , Dianzhong Wang , Baoning Zong , Minggang Li
IPC分类号： C01B39/38
CPC分类号： C01B39/026 , B01J29/084 , B01J29/405 , B01J29/46 , B01J29/48 , B01J29/80 , B01J2229/18 , B01J2229/42 , C10G11/02
摘要： A MFI-structured molecular sieve containing phosphorus and metal components has a formula expressed in anhydrous form and on the basis of oxide weight, as follows: (0˜0.3) Na2O (0.5˜5.5) Al2O3 (1.3˜10) P2O5 (0.7˜15) MlxOy (0.01˜5) M2mOn (70˜97) SiO2, wherein M1 is one of transition metals selected from the group consisting of Fe, Co and Ni, and M2 is any one of metals selected from the group consisting of Zn, Mn, Ga and Sn. Preparation processes and uses of the instant molecular sieve are also provided. The molecular sieve has an excellent performance for increasing the yield of lower olefins and increasing the aromatics content in gasoline, and can be used as a shape-selective active component for the catalytic cracking catalyst of petroleum hydrocarbons or its additives.
摘要翻译：含有磷和金属组分的MFI结构分子筛具有以无水形式和氧化物重量表示的式如下：（0〜0.3）Na 2 O（0.5〜5.5）Al （1.3〜10）P 2 O 5（0.7〜15）M 1 x 3 （0.01〜5）M 2 O（70〜97）SiO 2 N（O）其中，M1是选自Fe，Co和Ni中的过渡金属中的一种，M2是选自Zn，Mn，Ga和Sn中的任何一种金属。还提供了即时分子筛的制备方法和用途。该分子筛具有优异的提高低级烯烃的产率和提高汽油中芳烃含量的性能，可用作石油烃或其添加剂的催化裂化催化剂的形状选择性活性成分。

2. 发明授权

US07758847B2 Molecular sieve with MFI structure containing phosphorus and metal components, preparation process and use thereof 有权
标题翻译：具有含磷和金属成分的MFI结构的分子筛，其制备方法和用途
公开(公告)号：US07758847B2
公开(公告)日：2010-07-20
申请号：US10577672
申请日：2004-10-28
申请人： Yibin Luo , Ying Ouyang , Xingtian Shu , Mingyuan He , Dianzhong Wang , Baoning Zong , Minggang Li
发明人： Yibin Luo , Ying Ouyang , Xingtian Shu , Mingyuan He , Dianzhong Wang , Baoning Zong , Minggang Li
IPC分类号： C01B39/10 , C01B39/38 , B01J29/072 , B01J29/46
CPC分类号： C01B39/026 , B01J29/084 , B01J29/405 , B01J29/46 , B01J29/48 , B01J29/80 , B01J2229/18 , B01J2229/42 , C10G11/02
摘要： A MFI-structured molecular sieve containing phosphorus and metal components has a formula expressed in anhydrous form and on the basis of oxide weight, as follows: (0˜0.3) Na2O (0.5˜5.5) Al2O3 (1.3˜10) P2O5 (0.7˜15) M1xOy (0.01˜5) M2mOn (70˜97) SiO2, wherein M1 is one of transition metals selected from the group consisting of Fe, Co and Ni, and M2 is any one of metals selected from the group consisting of Zn, Mn, Ga and Sn. Preparation processes and uses of the instant molecular sieve are also provided. The molecular sieve has an excellent performance for increasing the yield of lower olefins and increasing the aromatics content in gasoline, and can be used as a shape-selective active component for the catalytic cracking catalyst of petroleum hydrocarbons or its additives.
摘要翻译：含有磷和金属组分的MFI结构分子筛具有无水形式和氧化物重量的表达式：（0〜0.3）Na 2 O（0.5〜5.5）Al 2 O 3（1.3〜10）P 2 O 5（0.7〜 15）M1xOy（0.01〜5）M2mOn（70〜97）SiO2，其中M1是选自Fe，Co和Ni中的过渡金属之一，M2是选自Zn， Mn，Ga和Sn。还提供了即时分子筛的制备方法和用途。该分子筛具有优异的提高低级烯烃的产率和提高汽油中芳烃含量的性能，可用作石油烃或其添加剂的催化裂化催化剂的形状选择性活性成分。

3. 发明授权

US07713904B2 Composition for desulfurization 有权
标题翻译：脱硫组成
公开(公告)号：US07713904B2
公开(公告)日：2010-05-11
申请号：US10562965
申请日：2004-06-24
申请人： Baoning Zong , Jinyu Zheng , Wenhua Xie , Yong Xu , Xuhong Mu , Yibin Luo , Minggang Li , Xingtian Shu
发明人： Baoning Zong , Jinyu Zheng , Wenhua Xie , Yong Xu , Xuhong Mu , Yibin Luo , Minggang Li , Xingtian Shu
IPC分类号： B01J27/195 , B01J29/06
CPC分类号： B01J29/84 , B01J29/084 , B01J29/088 , B01J29/40 , B01J29/405 , B01J29/80 , B01J2229/42 , C10G45/12 , C10G47/20
摘要： This invention relates to a composition with desulfurization property, in which the desulfurization component is a kind of molecular sieves with incorporation of vanadium into the skeleton. The composition has high hydrothermal stability and the vanadium is hard to lose.
摘要翻译：本发明涉及具有脱硫性质的组合物，其中脱硫组分是一种将钒掺入骨架中的分子筛。该组合物具有很高的水热稳定性，钒难以失去。

4. 发明申请

US20070060468A1 Composition for desulfurization 有权
标题翻译：脱硫组成
公开(公告)号：US20070060468A1
公开(公告)日：2007-03-15
申请号：US10562965
申请日：2004-06-24
申请人： Baoning Zong , Jinyu Zheng , Wenhua Xie , Yong Xu , Xuhong Mu , Yibin Luo , Minggang Li , Xingtian Shu
发明人： Baoning Zong , Jinyu Zheng , Wenhua Xie , Yong Xu , Xuhong Mu , Yibin Luo , Minggang Li , Xingtian Shu
IPC分类号： B01J29/04
CPC分类号： B01J29/84 , B01J29/084 , B01J29/088 , B01J29/40 , B01J29/405 , B01J29/80 , B01J2229/42 , C10G45/12 , C10G47/20
摘要： This invention relates to a composition with desulfurization property, in which the desulfurization component is a kind of molecular sieves with incorporation of vanadium into the skeleton. The composition has high hydrothermal stability and the vanadium is hard to lose.
摘要翻译：本发明涉及具有脱硫性质的组合物，其中脱硫组分是一种将钒掺入骨架中的分子筛。该组合物具有很高的水热稳定性，钒难以失去。

5. 发明申请

US20080261803A1 Modified Zeolite Beta 有权
标题翻译：改性沸石Beta
公开(公告)号：US20080261803A1
公开(公告)日：2008-10-23
申请号：US11915765
申请日：2006-05-31
申请人： Yibin Luo , Zhijian Da , Ying Ouyang , Li Zhuang , Jun Long , Xingtian Shu , Baoning Zong
发明人： Yibin Luo , Zhijian Da , Ying Ouyang , Li Zhuang , Jun Long , Xingtian Shu , Baoning Zong
IPC分类号： B01J21/04
CPC分类号： C01B39/10 , B01J29/7057 , B01J29/7615 , B01J29/7815 , B01J29/85 , B01J2229/18 , C01B39/06 , C10G11/05
摘要： A modified zeolite beta having an anhydrous chemical formula, by weight % of the oxides, of (0-0.3)Na2O.(0.5-10)Al2O3.(1.3-10)P2O5.(0.7-15)MxOy.(70-97)SiO2, wherein M is one or more transition metal(s) selected from the group consisting of Fe, Co, Ni, Cu, Mn, Zn and Sn, x is the number of the atoms of said transition metal M, and y is a number that meets with the requirement of the oxidation state of said transition metal M, is disclosed. The modified zeolite beta can be used as an active component of a cracking catalyst or additive for catalytic cracking of petroleum hydrocarbons.
摘要翻译：具有无水化学式的改性沸石β，其重量百分比为（0-0.3）Na 2 O（0.5-10）Al 2 O 3，（1.3-10）P 5 （0.7-15）M＆lt; x＆lt; （70-97）SiO 2，其中M是一种或多种选自Fe，Co，Ni，Cu，Mn，Zn的过渡金属和 Sn，x是所述过渡金属M的原子数，y是满足所述过渡金属M的氧化态的要求的数。改性沸石β可用作裂化催化剂或石油烃催化裂化添加剂的活性组分。

6. 发明授权

US07767611B2 Modified zeolite beta 有权
标题翻译：改性沸石β
公开(公告)号：US07767611B2
公开(公告)日：2010-08-03
申请号：US11915765
申请日：2006-05-31
申请人： Yibin Luo , Zhijian Da , Ying Ouyang , Li Zhuang , Jun Long , Xingtian Shu , Baoning Zong
发明人： Yibin Luo , Zhijian Da , Ying Ouyang , Li Zhuang , Jun Long , Xingtian Shu , Baoning Zong
IPC分类号： B01J29/06 , B01J29/072
CPC分类号： C01B39/10 , B01J29/7057 , B01J29/7615 , B01J29/7815 , B01J29/85 , B01J2229/18 , C01B39/06 , C10G11/05
摘要： A modified zeolite beta having an anhydrous chemical formula, by weight % of the oxides, of (0-0.3)Na2O.(0.5-10)Al2O3.(1.3-10)P2O5.(0.7-15)MxOy.(70-97)SiO2, wherein M is one or more transition metal(s) selected from the group consisting of Fe, Co, Ni, Cu, Mn, Zn and Sn, x is the number of the atoms of said transition metal M, and y is a number that meets with the requirement of the oxidation state of said transition metal M, is disclosed. The modified zeolite beta can be used as an active component of a cracking catalyst or additive for catalytic cracking of petroleum hydrocarbons.
摘要翻译：（0-0.3）Na2O（0.5-10）Al2O3。（1.3-10）P2O5（0.7-15）MxOy（70-97）的氧化物的无水化学式的改性沸石β ）SiO 2，其中M是选自Fe，Co，Ni，Cu，Mn，Zn和Sn中的一种或多种过渡金属，x是所述过渡金属M的原子数，y是公开了满足所述过渡金属M的氧化态的要求的数量。改性沸石β可用作裂化催化剂或石油烃催化裂化添加剂的活性组分。

7. 发明授权

US06368996B1 Hydrogenation catalyst and its preparation 有权
标题翻译：氢化催化剂及其制备
公开(公告)号：US06368996B1
公开(公告)日：2002-04-09
申请号：US09560444
申请日：2000-04-28
申请人： Xuhong Mu , Baoning Zong , Enze Min , Xuan Wang , Ying Wang , Xiaoxin Zhang , Xingtian Shu
发明人： Xuhong Mu , Baoning Zong , Enze Min , Xuan Wang , Ying Wang , Xiaoxin Zhang , Xingtian Shu
IPC分类号： B01J2500
CPC分类号： C07D201/16 , B01J25/02
摘要： An amorphous alloy catalyst for hydrogenation and its preparation method are disclosed herein. The catalyst essentially consists of nickel ranging between 60 and 98 wt %, iron ranging between 0 and 20 wt %, one doping metal element selected from the group consisting of chromium, cobalt, molybdenum, manganese and tungsten ranging between 0 and 20 wt %, and aluminum ranging between 0.5 and 30 wt % based on the weight of said catalyst, wherein the weight percentages of iron and the doping metal element component may not be zero at the same time; and just one broad diffusion peak appears at about 2 &thgr;=45±1° on the XRD patterns of the catalyst within 2 &thgr; range from 20 to 80°. The catalyst herein can be used in processes for hydrogenation of unsaturated compounds such as olefin, alkyne, aromatics, nitro, carbonyl groups, nitrile and soon, and for hydrorefining of caprolactam in particular.
摘要翻译：本文公开了一种用于氢化的无定形合金催化剂及其制备方法。该催化剂基本上由在60至98重量％之间的镍范围内，铁范围在0至20重量％之间，1种掺杂金属元素选自铬，钴，钼，锰和钨，其范围为0至20重量％和铝的范围在0.5至30重量％之间，基于所述催化剂的重量，其中铁和掺杂金属元素组分的重量百分比可以不同时为零; 并且在20至80°的2θ范围内，在催化剂的XRD图上，在约2θ= 45±1°处仅出现一个宽的扩散峰。本文的催化剂可用于不饱和化合物如烯烃，炔烃，芳族化合物，硝基，羰基，腈和不久的氢化方法，特别是加氢精制己内酰胺。

8. 发明申请

US20080308455A1 Catalyst and a Method for Cracking Hydrocarbons 审中-公开
标题翻译：催化剂和烃类裂化方法
公开(公告)号：US20080308455A1
公开(公告)日：2008-12-18
申请号：US11813056
申请日：2005-12-28
申请人： Jun Long , Wenbin Jiang , Mingde Xu , Huiping Tian , Yibin Luo , Xingtian Shu , Jiushun Zhang , Beiyan Chen , Haitao Song
发明人： Jun Long , Wenbin Jiang , Mingde Xu , Huiping Tian , Yibin Luo , Xingtian Shu , Jiushun Zhang , Beiyan Chen , Haitao Song
IPC分类号： C10G11/05
CPC分类号： C10G11/05 , B01J27/1853 , B01J29/46 , B01J35/0006 , B01J35/002 , B01J2229/42 , C10G11/02 , C10G47/16 , C10G2300/4018 , C10G2400/02
摘要： The invention discloses a catalyst and a method for cracking hydrocarbons. The catalyst comprises, calculated by dry basis, 10˜65 wt % ZSM-5 zeolite, 0˜60 wt % clay, 15˜60 wt % inorganic oxide binder, 0.5˜15 wt % one or more metal additives selected from the metals of Group VIIIB and 2˜25 wt % P additive, in which the metal additive is calculated by metal oxide and the P additive is calculated by P2O5. The method for cracking hydrocarbons using this catalyst increases the yield of FCC liquefied petroleum gas (LPG) and the octane number of FCC gasoline, as well as it increases the concentration of propylene in LPG dramatically.
摘要翻译：本发明公开了一种催化剂和一种裂化烃的方法。催化剂包括以干基计，10〜65重量％的ZSM-5沸石，0〜60重量％的粘土，15〜60重量％的无机氧化物粘合剂，0.5〜15重量％的一种或多种金属添加剂， ⅦB族和2〜25wt％P添加剂，其中金属添加剂由金属氧化物计算，P添加剂通过P2O5计算。使用该催化剂裂化烃的方法提高了FCC液化石油气（LPG）的产率和FCC汽油的辛烷值，并且显着提高了LPG中丙烯的浓度。

9. 发明授权

US5951963A Phosphorous containing zeolite having MFI type structure 失效
标题翻译：含有MFI型结构的含磷沸石
公开(公告)号：US5951963A
公开(公告)日：1999-09-14
申请号：US46630
申请日：1998-03-24
申请人： Mingyuan He , Xiaoming Yang , Xingtian Shu , Jinge Luo
发明人： Mingyuan He , Xiaoming Yang , Xingtian Shu , Jinge Luo
IPC分类号： B01J29/85 , C01B39/10 , C01B39/46
CPC分类号： B01J29/85 , C01B39/10 , B01J2229/16 , B01J2229/183 , B01J2229/32 , Y10S423/22 , Y10S423/30
摘要： The present invention discloses a phosphorus-containing zeolite having MFI type structure. The anhydrous composition (based on the mole ratios of oxides) of the above zeolite is0.01-0.3Na.sub.2 O.Al.sub.2 O.sub.3.0.2-1.5P.sub.2 O.sub.5.30-90SiO.sub.2Said zeolite possesses a X-ray diffraction pattern listed in Table 1. The pore volume ratio of 1.0-10 nm mesopore to 10-membered ring pore is no less than 0.5. The crystal particle size of said zeolite is in the range of 0.8-2.0 micron. Said zeolite exhibits superior hydrothermal stability in catalytic conversion of hydrocarbons. Especially, when said zeolite is applied in catalytic cracking of hydrocarbons, it will enhance the crackability of large molecules, improve gasoline octane value and stability, and reduce the sulfur content in the gasoline as well.
摘要翻译：本发明公开了具有MFI型结构的含磷沸石。上述沸石的无水组成（基于氧化物的摩尔比）为0.01-0.3Na2O.Al2O3.0.2-1.5P2O5.30-90SiO2所述沸石具有表1中列出的X射线衍射图。孔体积 1.0-10nm中孔与10元环孔的比例不小于0.5。所述沸石的晶体粒度在0.8-2.0微米的范围内。所述沸石在烃的催化转化中表现出优异的水热稳定性。特别是当所述沸石用于烃的催化裂化时，会提高大分子的裂解性，提高汽油辛烷值和稳定性，并降低汽油中的硫含量。

10. 发明授权

US08716163B2 Hydrocarbon conversion catalyst 有权
标题翻译：烃转化催化剂
公开(公告)号：US08716163B2
公开(公告)日：2014-05-06
申请号：US12439315
申请日：2006-09-28
申请人： Yujian Liu , Huiping Tian , Xingtian Shu , Jun Long , Yibin Luo , Chaogang Xie , Zhenyu Chen , Liuzhou Zhao , Yuxia Zhu , Youbao Lu
发明人： Yujian Liu , Huiping Tian , Xingtian Shu , Jun Long , Yibin Luo , Chaogang Xie , Zhenyu Chen , Liuzhou Zhao , Yuxia Zhu , Youbao Lu
IPC分类号： B01J21/00 , B01J21/16 , B01J29/04 , B01J29/08 , B01J29/18
CPC分类号： B01J29/80 , B01J29/40 , B01J29/7007 , B01J29/7057 , B01J29/7615 , B01J29/7815 , B01J35/023 , B01J35/04 , B01J35/1076 , B01J35/1095 , B01J37/0045 , B01J37/0219 , B01J37/0234 , B01J2229/20 , B01J2229/42 , C04B35/18 , C04B2235/3201 , C04B2235/3262 , C04B2235/3272 , C04B2235/3275 , C04B2235/3279 , C04B2235/3281 , C04B2235/3284 , C04B2235/3293 , C04B2235/447 , C10G2400/20
摘要： A hydrocarbon conversion catalyst, which comprises, based on the total weight of the catalyst, 1-60 wt % of a zeolite mixture, 5-99 wt % of a thermotolerant inorganic oxide and 0-70 wt % of clay, wherein said zeolite mixture comprises, based on the total weight of said zeolite mixture, 1-75 wt % of a zeolite beta modified with phosphorus and a transition metal M, 25-99 wt % of a zeolite having a MFI structure and 0-74 wt % of a large pore zeolite, wherein the anhydrous chemical formula of the zeolite beta modified with phosphorus and the transition metal M is represented in the mass percent of the oxides as (0-0.3)Na2O.(0.5-10)Al2O3.(1.3-10)P2O5.(0.7-15)MxOy.(64-97)SiO2, in which the transition metal M is one or more selected from the group consisting of Fe, Co, Ni, Cu, Mn, Zn and Sn; x represents the atom number of the transition metal M, and y represents a number needed for satisfying the oxidation state of the transition metal M.
摘要翻译：一种烃转化催化剂，其基于催化剂的总重量包含1-60重量％的沸石混合物，5-99重量％的耐热无机氧化物和0-70重量％的粘土，其中所述沸石混合物包括基于所述沸石混合物的总重量，1-75重量％的用磷和过渡金属M改性的沸石β，25-99重量％的具有MFI结构的沸石和0-74重量％的大孔沸石，其中用磷改性的沸石β和过渡金属M的无水化学式以氧化物的质量百分比表示为（0-0.3）Na 2 O（0.5-10）Al 2 O 3（1.3-10） P2O5（0.7-15）MxOy（64-97）SiO2，其中过渡金属M是选自Fe，Co，Ni，Cu，Mn，Zn和Sn中的一种或多种; x表示过渡金属M的原子数，y表示满足过渡金属M的氧化态所需的数。

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