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1. 发明授权

US09486795B2 Catalytic cracking catalyst, its preparation and use 有权
标题翻译：催化裂化催化剂，其制备及应用
公开(公告)号：US09486795B2
公开(公告)日：2016-11-08
申请号：US12666711
申请日：2008-06-27
申请人： Jun Long , Yujian Liu , Huiping Tian , Liuzhou Zhao , Yuxia Zhu , Zhenyu Chen , Yun Xu , Jing Fan
发明人： Jun Long , Yujian Liu , Huiping Tian , Liuzhou Zhao , Yuxia Zhu , Zhenyu Chen , Yun Xu , Jing Fan
IPC分类号： C10G11/05 , B01J35/10 , B01J29/06 , B01J29/40 , B01J29/80 , B01J29/08 , B01J29/70
CPC分类号： B01J35/10 , B01J29/06 , B01J29/084 , B01J29/40 , B01J29/405 , B01J29/7007 , B01J29/7057 , B01J29/80 , B01J35/108 , B01J2229/42 , C10G11/05
摘要： A catalyst for catalytically cracking hydrocarbon oils contains a substrate comprising alumina and a molecular sieve, characterized in that the pore distribution of said catalyst is 5-70% of the
摘要翻译：用于催化裂化烃油的催化剂含有包含氧化铝和分子筛的底物，其特征在于所述催化剂的孔分布为<2nm孔的5-70％，2-4nm孔的5-70％ 4-6nm孔中的0-10％，6-20nm孔的20-80％，20-100nm孔中的0-40％，基于孔径不大的孔的孔体积超过100nm。本发明的催化剂具有大的BET孔体积，高重量油裂解能力和耐焦化能力。

2. 发明申请

US20100288675A1 CATALYST FOR CONVERTING ACID-CONTAINING INFERIOR CRUDE OIL AND PROCESS FOR MAKING AND USING THE SAME 有权
标题翻译：用于转化含酸的无水原油的催化剂及其制备和使用方法
公开(公告)号：US20100288675A1
公开(公告)日：2010-11-18
申请号：US12812148
申请日：2009-01-09
申请人： Jun Long , Jiushun Zhang , Huiping Tian , Yuxia Zhu
发明人： Jun Long , Jiushun Zhang , Huiping Tian , Yuxia Zhu
IPC分类号： B01J29/06 , C10G11/05
CPC分类号： C10G45/12 , B01J21/16 , B01J23/02 , B01J29/06 , B01J29/08 , B01J29/18 , B01J29/40 , B01J29/7007 , B01J29/80 , B01J35/1019 , B01J35/1042 , B01J35/1047 , B01J35/1061 , B01J37/0045 , B01J2229/42 , C10G11/05
摘要： The present invention relates to a catalyst for converting inferior acid-containing crude oil. Based on the total amount of the catalyst, said catalyst comprises from 1 to 50 wt % of a mesopore material, from 1 to 60 wt % of molecular sieves and from 5 to 98 wt % of thermotolerant inorganic oxides and from 0 to 70 wt % of clays. Said mesopore material is an amorphous material containing alkaline earth oxide, silica and alumina, and has an anhydrous chemical formula of (0-0.3)Na2O.(1-50)MO.(6-58)Al2O3.(40-92)SiO2, based on the weight percent of the oxides, wherein M is one or more selected from Mg, Ca and Ba. Said mesopore material has a specific surface area of 200-400 m2/g, a pore volume of 0.5-2.0 ml/g, an average pore diameter of 8-20 nm, and a most probable pore size of 5-15 nm. The catalyst provided in the present invention is suitable for the catalytic conversion of crude oil having a total acid number of greater than 0.5 mgKOH/g and for the removal of organic acids, carbon residues and metals in crude oil, and thus has very good economic benefits.
摘要翻译：本发明涉及用于转化劣质含酸原油的催化剂。基于催化剂的总量，所述催化剂包含1至50重量％的中孔材料，1至60重量％的分子筛和5至98重量％的耐热无机氧化物和0至70重量％的粘土。所述中孔材料是含有碱土金属氧化物，二氧化硅和氧化铝的无定形材料，具有无水化学式（0-0.3）Na2O（1-50）MO。（6-58）Al2O3。（40-92）SiO2 ，基于氧化物的重量百分数，其中M是选自Mg，Ca和Ba中的一种或多种。所述中孔材料的比表面积为200-400m2 / g，孔体积为0.5-2.0ml / g，平均孔径为8-20nm，最可能的孔径为5-15nm。本发明提供的催化剂适用于总酸值大于0.5mgKOH / g的原油的催化转化和用于去除原油中的有机酸，碳残余物和金属，因此具有非常好的经济性好处

3. 发明申请

US20090325786A1 HYDROCARBON CONVERSION CATALYST 有权
标题翻译：碳氢转化催化剂
公开(公告)号：US20090325786A1
公开(公告)日：2009-12-31
申请号：US12439315
申请日：2006-09-28
申请人： Yujian Liu , Huiping Tian , Xingtian Shu , Jun Long , Yibin Luo , Chaogang Xie , Zhenyu Chen , Liuzhou Zhao , Yuxia Zhu , Youbao Lu
发明人： Yujian Liu , Huiping Tian , Xingtian Shu , Jun Long , Yibin Luo , Chaogang Xie , Zhenyu Chen , Liuzhou Zhao , Yuxia Zhu , Youbao Lu
IPC分类号： B01J29/04 , B01J21/16 , B01J29/40 , B01J29/072 , B01J29/08 , B01J29/18
CPC分类号： B01J29/80 , B01J29/40 , B01J29/7007 , B01J29/7057 , B01J29/7615 , B01J29/7815 , B01J35/023 , B01J35/04 , B01J35/1076 , B01J35/1095 , B01J37/0045 , B01J37/0219 , B01J37/0234 , B01J2229/20 , B01J2229/42 , C04B35/18 , C04B2235/3201 , C04B2235/3262 , C04B2235/3272 , C04B2235/3275 , C04B2235/3279 , C04B2235/3281 , C04B2235/3284 , C04B2235/3293 , C04B2235/447 , C10G2400/20
摘要： A hydrocarbon conversion catalyst, which comprises, based on the total weight of the catalyst, 1-60 wt % of a zeolite mixture, 5-99 wt % of a thermotolerant inorganic oxide and 0-70 wt % of clay, wherein said zeolite mixture comprises, based on the total weight of said zeolite mixture, 1-75 wt % of a zeolite beta modified with phosphorus and a transition metal M, 25-99 wt % of a zeolite having a MFI structure and 0-74 wt % of a large pore zeolite, wherein the anhydrous chemical formula of the zeolite beta modified with phosphorus and the transition metal M is represented in the mass percent of the oxides as (0-0.3)Na2O.(0.5-10)Al2O3.(1.3-10)P2O5.(0.7-15)MxOy.(64-97)SiO2, in which the transition metal M is one or more selected from the group consisting of Fe, Co, Ni, Cu, Mn, Zn and Sn; x represents the atom number of the transition metal M, and y represents a number needed for satisfying the oxidation state of the transition metal M. The catalysts provided in the present invention have higher ability to convert petroleum hydrocarbons and higher yields for light olefins, particularly for propylene. The catalysts can be used for the selectively producing light olefins.
摘要翻译：一种烃转化催化剂，其基于催化剂的总重量包含1-60重量％的沸石混合物，5-99重量％的耐热无机氧化物和0-70重量％的粘土，其中所述沸石混合物包括基于所述沸石混合物的总重量，1-75重量％的用磷和过渡金属M改性的沸石β，25-99重量％的具有MFI结构的沸石和0-74重量％的大孔沸石，其中用磷和过渡金属M改性的沸石β的无水化学式以氧化物的质量百分比表示为（0-0.3）Na 2 O（0.5-10）Al 2 O 3（1.3-10） P2O5（0.7-15）MxOy（64-97）SiO2，其中过渡金属M是选自Fe，Co，Ni，Cu，Mn，Zn和Sn中的一种或多种; x表示过渡金属M的原子数，y表示满足过渡金属M的氧化态所需的数。本发明提供的催化剂具有较高的转化石油烃的能力和较高的轻质烯烃产率，特别是用于丙烯。催化剂可用于选择性生产轻质烯烃。

4. 发明申请

US20080289997A1 PROCESS FOR CRACKING HYDROCARBON OILS 有权
标题翻译：破碎油气的方法
公开(公告)号：US20080289997A1
公开(公告)日：2008-11-27
申请号：US12027123
申请日：2008-02-06
申请人： Jun Long , Yuxia Zhu , Huiping Tian , Yujian Liu , Zhenyu Chen , Yaoqing Guo , Zhijian Da , Jiushun Zhang , Mingyuan He
发明人： Jun Long , Yuxia Zhu , Huiping Tian , Yujian Liu , Zhenyu Chen , Yaoqing Guo , Zhijian Da , Jiushun Zhang , Mingyuan He
IPC分类号： C10G11/00
CPC分类号： C10G11/14 , C10G11/05 , C10G11/16 , C10G11/182 , C10G2300/205 , C10G2300/4006 , C10G2300/4012 , C10G2300/701 , C10G2400/04
摘要： A novel process for cracking olefins including contacting a hydrocarbon oil with a catalyst in a riser reactor having multiple reaction zones under cracking reaction conditions; separating reaction products and the catalyst; regenerating at least a part of spent catalyst obtained, contacting a part of the regenerated catalyst with the hydrocarbon in the first reaction zone; contacting the other part of the spent catalyst and/or regenerated catalyst in at least one reaction zone after the first reaction zone with the products obtained in previous reaction zones.
摘要翻译：一种用于裂化烯烃的新方法，包括在裂化反应条件下具有多个反应区的提升管反应器中使烃油与催化剂接触; 分离反应产物和催化剂; 再生至少一部分所获得的废催化剂，使部分再生催化剂与第一反应区中的烃接触; 在第一反应区之后的至少一个反应区与先前反应区中获得的产物接触废催化剂和/或再生催化剂的另一部分。

5. 发明授权

US07347930B2 Process for cracking hydrocarbon oils 有权
标题翻译：裂解烃油的工艺
公开(公告)号：US07347930B2
公开(公告)日：2008-03-25
申请号：US10964644
申请日：2004-10-15
申请人： Jun Long , Yuxia Zhu , Huiping Tian , Yujian Liu , Zhenyu Chen , Yaoqing Guo , Zhijian Da , Jiushun Zhang , Mingyuan He
发明人： Jun Long , Yuxia Zhu , Huiping Tian , Yujian Liu , Zhenyu Chen , Yaoqing Guo , Zhijian Da , Jiushun Zhang , Mingyuan He
IPC分类号： C10G11/00 , C10G29/04
CPC分类号： C10G11/14 , C10G11/05 , C10G11/16 , C10G11/182 , C10G2300/205 , C10G2300/4006 , C10G2300/4012 , C10G2300/701 , C10G2400/04
摘要： A novel process for cracking olefins including contacting a hydrocarbon oil with a catalyst in a riser reactor having multiple reaction zones under cracking reaction conditions; separating reaction products and the catalyst; regenerating at least a part of spent catalyst obtained, contacting a part of the regenerated catalyst with the hydrocarbon in the first reaction zone; contacting the other part of the spent catalyst and/or regenerated catalyst in at least one reaction zone after the first reaction zone with the products obtained in previous reaction zones.
摘要翻译：一种用于裂化烯烃的新方法，包括在裂化反应条件下具有多个反应区的提升管反应器中使烃油与催化剂接触; 分离反应产物和催化剂; 再生至少一部分所获得的废催化剂，使部分再生催化剂与第一反应区中的烃接触; 在第一反应区之后的至少一个反应区与先前反应区中获得的产物接触废催化剂和/或再生催化剂的另一部分。

6. 发明授权

US09611432B2 Catalytic cracking catalyst having a higher selectivity, processing method and use thereof 有权
公开(公告)号：US09611432B2
公开(公告)日：2017-04-04
申请号：US12822493
申请日：2010-06-24
申请人： Youhao Xu , Shouye Cui , Jun Long , Jianhong Gong , Zhijian Da , Jiushun Zhang , Yuxia Zhu , Yibin Luo , Jinlian Tang
发明人： Youhao Xu , Shouye Cui , Jun Long , Jianhong Gong , Zhijian Da , Jiushun Zhang , Yuxia Zhu , Yibin Luo , Jinlian Tang
IPC分类号： C10G11/18 , B01J29/06 , C10G11/05 , B01J29/08 , B01J35/00 , B01J37/04 , B01J37/10
CPC分类号： C10G11/05 , B01J29/06 , B01J29/084 , B01J29/088 , B01J29/90 , B01J35/002 , B01J37/0045 , B01J37/04 , B01J37/10 , B01J38/30 , B01J2229/16 , B01J2229/32 , B01J2229/36 , B01J2229/42 , C10G11/18
摘要： The present invention provides a catalytic cracking catalyst, processing method and use thereof. When the catalyst is added into a commercial catalytic cracking unit, it has an initial activity of not higher than 80, preferably not higher than 75, more preferably not higher than 70, a self-balancing time of 0.1-50 h, and an equilibrium activity of 35-60. Said method enables the activity and selectivity of the catalyst in the catalytic cracking unit to be more homogeneous and notably improves the selectivity of the catalytic cracking catalyst, so as to obviously reduce the dry gas and coke yields, to sufficiently use steam and to reduce the energy consumption of the FCC unit.

7. 发明授权

US08809216B2 Catalyst for converting acid-containing inferior crude oil and process for making and using the same 有权
标题翻译：用于转化含酸劣质原油的催化剂及其制备和使用方法
公开(公告)号：US08809216B2
公开(公告)日：2014-08-19
申请号：US12812148
申请日：2009-01-09
申请人： Jun Long , Jiushun Zhang , Huiping Tian , Yuxia Zhu
发明人： Jun Long , Jiushun Zhang , Huiping Tian , Yuxia Zhu
IPC分类号： B01J29/06 , C10G11/05
CPC分类号： C10G45/12 , B01J21/16 , B01J23/02 , B01J29/06 , B01J29/08 , B01J29/18 , B01J29/40 , B01J29/7007 , B01J29/80 , B01J35/1019 , B01J35/1042 , B01J35/1047 , B01J35/1061 , B01J37/0045 , B01J2229/42 , C10G11/05
摘要： The present invention relates to a catalyst for converting inferior acid-containing crude oil. Based on the total amount of the catalyst, said catalyst comprises from 1 to 50 wt % of a mesopore material, from 1 to 60 wt % of molecular sieves and from 5 to 98 wt % of thermotolerant inorganic oxides and from 0 to 70 wt % of clays. Said mesopore material is an amorphous material containing alkaline earth oxide, silica and alumina, and has an anhydrous chemical formula of (0-0.3)Na2O.(1-50)MO.(6-58)Al2O3.(40-92)SiO2, based on the weight percent of the oxides, wherein M is one or more selected from Mg, Ca and Ba. Said mesopore material has a specific surface area of 200-400 m2/g, a pore volume of 0.5-2.0 ml/g, an average pore diameter of 8-20 nm, and a most probable pore size of 5-15 nm. The catalyst provided in the present invention is suitable for the catalytic conversion of crude oil having a total acid number of greater than 0.5 mgKOH/g and for the removal of organic acids, carbon residues and metals in crude oil, and thus has very good economic benefits.
摘要翻译：本发明涉及用于转化劣质含酸原油的催化剂。基于催化剂的总量，所述催化剂包含1至50重量％的中孔材料，1至60重量％的分子筛和5至98重量％的耐热无机氧化物和0至70重量％的粘土。所述中孔材料是含有碱土金属氧化物，二氧化硅和氧化铝的无定形材料，具有无水化学式（0-0.3）Na2O（1-50）MO。（6-58）Al2O3。（40-92）SiO2 ，基于氧化物的重量百分数，其中M是选自Mg，Ca和Ba中的一种或多种。所述中孔材料的比表面积为200-400m2 / g，孔体积为0.5-2.0ml / g，平均孔径为8-20nm，最可能的孔径为5-15nm。本发明提供的催化剂适用于总酸值大于0.5mgKOH / g的原油的催化转化和用于去除原油中的有机酸，碳残余物和金属，因此具有非常好的经济性好处

8. 发明申请

US20070293714A1 Zeolite-Containing Hydrocarbon-Converting Catalyst, the Preparation Process Thereof, and a Process for Converting Hydrocarbon Oils with the Catalyst 有权
公开(公告)号：US20070293714A1
公开(公告)日：2007-12-20
申请号：US11547209
申请日：2005-03-31
申请人： Jun Long , Zhijian Da , Huiping Tian , Zhenyu Chen , Weilin Zhang , Xingtian Shu , Jiushun Zhang , Yuxia Zhu , Yujian Liu
发明人： Jun Long , Zhijian Da , Huiping Tian , Zhenyu Chen , Weilin Zhang , Xingtian Shu , Jiushun Zhang , Yuxia Zhu , Yujian Liu
IPC分类号： B01J29/42 , C10G11/05
CPC分类号： B01J29/42 , B01J29/084 , B01J29/40 , B01J29/405 , B01J29/48 , B01J29/80 , B01J2229/42 , C10G11/05 , C10G2300/807 , C10G2400/20
摘要： A catalyst for converting hydrocarbons includes, based on the weight of the catalyst, 1-60% by weight of a zeolite, 0.1-10% by weight of an assistant catalytic component, 5-98% by weight of a thermotolerant inorganic oxide, and 0-70% by weight of a clay in terms of the oxide. The zeolite is a MFI-structured zeolite-containing phosphor and transition metal(s) or a mixture of the zeolite and a macroporous zeolite, which comprises, based on the weight of the mixture, 75-100% by weight of said MFI-structured zeolite containing phosphor and transition metal(s) and 0-25% by weight of the macroporous zeolite. In terms of the mass of the oxide, the MFI-structured zeolite containing phosphor and transition metal(s) has the following anhydrous chemical formula: (0-0.3)Na2O.(0.3-5.5)Al2O3.(1.0-10)P2O5.(0.7-15)M1xOy.(0.01-5)M2mOn(0-10)RE2O3.(70-97)SiO2 I or (0-0.3)Na2O.(0.3-5)Al2O3.(1.0-10)P2O5.(0.7-15)MpOq.(0-10)RE2O3.(70-98)SiO2 II The assistant catalytic component is one or more selected from the group consisting of the alkali earth metals, Group IVB metals, non-noble metals of Group VIII, and rare earth metals of the Periodic Table of the Elements. This catalyst has a higher ability to convert petroleum hydrocarbons and higher yields for propylene, ethylene, and light aromatics.

9. 发明申请

US20050279670A1 Process for cracking hydrocarbon oils 有权
标题翻译：裂解烃油的工艺
公开(公告)号：US20050279670A1
公开(公告)日：2005-12-22
申请号：US10949298
申请日：2004-09-27
申请人： Jun Long , Huiping Tian , Yujian Liu , Yuxia Zhu , Zhenyu Chen , Yaoqing Guo , Zhijian Da , Jiushun Zhang , Mingyuan He
发明人： Jun Long , Huiping Tian , Yujian Liu , Yuxia Zhu , Zhenyu Chen , Yaoqing Guo , Zhijian Da , Jiushun Zhang , Mingyuan He
IPC分类号： C10G45/04 , C10G11/02 , C10G11/04 , C10G11/05 , C10G47/00
CPC分类号： C10G11/05 , C10G11/04
摘要： This invention relates to a process for cracking hydrocarbon oils. Said process comprises contacting a hydrocarbon oil with a catalyst that has contacted with an atmosphere containing a reducing gas, separating cracked products and the catalyst, regenerating the catalyst, contacting the regenerated catalyst with said atmosphere containing a reducing gas, wherein said catalyst is a cracking catalyst containing a metal component, or a catalyst mixture of a cracking catalyst containing a metal component and a cracking catalyst free of metal component, contacting said catalyst with the atmosphere containing a reducing gas at a temperature of 100 to 900° C. for at least 1 second, wherein the amount of the atmosphere containing a reducing gas is not less than 0.03 cubic meters of reducing gas per ton of the cracking catalyst containing a metal component per minute, at a pressure of 0.1-0.5 MPa in the reduction reactor. The process has higher ability of desulfurizing and cracking heavy oils.
摘要翻译：本发明涉及一种裂解烃油的方法。所述方法包括使烃油与与还原气体的气氛接触的催化剂，分离裂化产物和催化剂，再生催化剂，使再生催化剂与含有还原气体的气氛接触，其中所述催化剂是裂化含有金属成分的催化剂或含有金属成分的裂化催化剂和不含金属成分的裂化催化剂的催化剂混合物，使催化剂与含有还原气体的气氛在100〜900℃的温度下接触至少 1秒钟，其中含有还原气体的气氛量在还原反应器中的压力为0.1-0.5MPa时，每分钟含有每分钟金属组分的裂化催化剂的还原气体不少于0.03立方米。该工艺具有较高的脱硫脱硫重油能力。

10. 发明申请

US20050133419A1 Process for cracking hydrocarbon oils 有权
标题翻译：裂解烃油的工艺
公开(公告)号：US20050133419A1
公开(公告)日：2005-06-23
申请号：US10964644
申请日：2004-10-15
申请人： Jun Long , Yuxia Zhu , Huiping Tian , Yujian Liu , Zhenyu Chen , Yaoqing Guo , Zhijian Da , Jiushun Zhang , Mingyuan He
发明人： Jun Long , Yuxia Zhu , Huiping Tian , Yujian Liu , Zhenyu Chen , Yaoqing Guo , Zhijian Da , Jiushun Zhang , Mingyuan He
IPC分类号： C10G51/04 , C10G11/02 , C10G11/05 , C10G11/14 , C10G11/16 , C10G11/18
CPC分类号： C10G11/14 , C10G11/05 , C10G11/16 , C10G11/182 , C10G2300/205 , C10G2300/4006 , C10G2300/4012 , C10G2300/701 , C10G2400/04
摘要： A novel process for cracking olefins including contacting a hydrocarbon oil with a catalyst in a riser reactor having multiple reaction zones under cracking reaction conditions; separating reaction products and the catalyst; regenerating at least a part of spent catalyst obtained, contacting a part of the regenerated catalyst with the hydrocarbon in the first reaction zone; contacting the other part of the spent catalyst and/or regenerated catalyst in at least one reaction zone after the first reaction zone with the products obtained in previous reaction zones.
摘要翻译：一种用于裂化烯烃的新方法，包括在裂化反应条件下具有多个反应区的提升管反应器中使烃油与催化剂接触; 分离反应产物和催化剂; 再生至少一部分所获得的废催化剂，使部分再生催化剂与第一反应区中的烃接触; 在第一反应区之后的至少一个反应区与先前反应区中获得的产物接触废催化剂和/或再生催化剂的另一部分。

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