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1. 发明授权

US06391967B1 Flame retarding thermoplastic resin composition 有权
标题翻译：阻燃热塑性树脂组合物
公开(公告)号：US06391967B1
公开(公告)日：2002-05-21
申请号：US09502620
申请日：2000-02-11
申请人： Kuen-Yuan Hwang , Hong-Hsing Chen , Ying-Ling Liu , Wen-Tsai Tsai
发明人： Kuen-Yuan Hwang , Hong-Hsing Chen , Ying-Ling Liu , Wen-Tsai Tsai
IPC分类号： C08L6134
CPC分类号： C08L61/14 , C08L61/34 , C08L2666/18 , C08L2666/24
摘要： This invention discloses a flame retarding thermoplastic resin composition, which is comprised of (i) a thermoplastic resin and (ii) a phenolic resin compound as a flame retardant, wherein the phenolic resin compound contains a nitrogen-containing heterocycle and phosphorus. Since the flame retarding thermoplastic resin composition of this invention does not contain halogen, and has excellent flame retardant properties and high heat resistance, it is useful in producing parts and products in the fields of electronics, electricity and automobile.
摘要翻译：本发明公开了一种阻燃热塑性树脂组合物，其由（i）热塑性树脂和（ii）酚醛树脂化合物作为阻燃剂组成，其中酚醛树脂化合物含有含氮杂环和磷。由于本发明的阻燃性热塑性树脂组合物不含卤素，并且具有优异的阻燃性能和高耐热性，因此在电子，电力和汽车领域的制造零件和产品中是有用的。

2. 发明授权

US06432539B1 Phosphorus-containing polymer having phenolic units and uses thereof 有权
标题翻译：含酚单体的含磷聚合物及其用途
公开(公告)号：US06432539B1
公开(公告)日：2002-08-13
申请号：US09431435
申请日：1999-11-01
申请人： Kuen-Yuan Hwang , Hong-Hsing Chen , An-Pang Tu , Ying-Ling Liu
发明人： Kuen-Yuan Hwang , Hong-Hsing Chen , An-Pang Tu , Ying-Ling Liu
IPC分类号： C08L6304
CPC分类号： H01L23/293 , C08G8/28 , C08G59/3254 , C08G59/621 , C08G61/02 , C08G2261/1422 , C08G2261/312 , C08G2261/3325 , C08G2261/3424 , C08G2261/592 , C08L61/14 , C08L63/00 , C08L85/02 , H01L23/145 , H01L2924/0002 , H05K1/0326 , Y10T428/31511 , C08L61/04 , C08L2666/22 , H01L2924/00 , C08L65/00
摘要： A phosphorus-containing polymer having phenolic units and an epoxy rein composition are provided. The epoxy resin composition suitably comprises an epoxy resin and a hardener, wherein the epoxy resin may be obtained by reacting the polymer with epihalohydrin, and the polymer may further act as the hardener.
摘要翻译：提供了具有酚类单元和环氧树脂组合物的含磷聚合物。环氧树脂组合物合适地包含环氧树脂和硬化剂，其中环氧树脂可以通过使聚合物与表卤代醇反应获得，并且聚合物可以进一步用作硬化剂。

3. 发明授权

US07084194B2 Halogen-free resin composition 有权
标题翻译：无卤树脂组合物
公开(公告)号：US07084194B2
公开(公告)日：2006-08-01
申请号：US10633890
申请日：2003-08-04
申请人： Kuen-Yuan Hwang , An-Pang Tu , Chi-Yi Ju , Wen-Tsai Tsai
发明人： Kuen-Yuan Hwang , An-Pang Tu , Chi-Yi Ju , Wen-Tsai Tsai
IPC分类号： C08L63/00
CPC分类号： C08G59/4021 , C08G59/304 , C08G59/4064 , C08G59/686 , H05K1/0326 , H05K3/386
摘要： A halogen-free resin composition is provided, comprising: (A) one or more phosphorous-containing epoxy resins; (B) a hardener; and (C) a hardening accelerator, wherein the hardener of component (B) has the structure represented by the following formula (I): wherein, each symbol is defined as in the specification. The halogen-free resin composition of the present invention has excellent thermal resistance and flame retardant property, and is thereby suitably useful in the application of adhesives, composite materials, laminated plates, printed circuit boards, copper foil adhesives, inks used for build-up process, semiconductor packaging materials, and the like.
摘要翻译：提供无卤树脂组合物，其包含：（A）一种或多种含磷环氧树脂; （B）硬化剂; 和（C）硬化促进剂，其中组分（B）的硬化剂具有由下式（I）表示的结构：其中每个符号如说明书中所定义。本发明的无卤树脂组合物具有优异的耐热性和阻燃性，因此适用于粘合剂，复合材料，层压板，印刷电路板，铜箔粘合剂，用于堆积的油墨的应用工艺，半导体封装材料等。

4. 发明授权

US06660786B2 Flame retarded epoxy resin composition 失效
标题翻译：阻燃环氧树脂组合物
公开(公告)号：US06660786B2
公开(公告)日：2003-12-09
申请号：US09811948
申请日：2001-03-19
申请人： Kuen-Yuan Hwang , Hong-Hsing Chen , Tsung-Yu Chen , Ching Fu Kao
发明人： Kuen-Yuan Hwang , Hong-Hsing Chen , Tsung-Yu Chen , Ching Fu Kao
IPC分类号： C08L6310
CPC分类号： C08K5/5399 , H05K1/0326 , H05K1/0373 , Y10T428/31511 , Y10T428/31522 , Y10T428/31529 , C08L63/00
摘要： The present invention relates to a flame retarded epoxy resin composition, which is characterized by that said flame retarded epoxy resin composition comprising: (A) at least one type of epoxy resin; (B) a phosphorus-and-nitrogen-containing heterocyclic compound, said compound having a moiety which can react with the epoxy group of the epoxy resin, usedful as a hardening agent, and having a structure as shown by formula (I): wherein m is an integer of from 0 to 2, n is an integer of from 3 to 7, but at least one m is not 2. The epoxy resin composition consisting of the above components (A) and (B) has improved flame retarded property and thus is suitably used as the flame retarded material required for the parts of composite material, laminated plates, printed circuit boards, electronic products, electrical products, and the like. According to the range of applications, the composition can be selectively added with additives such as a hardening agent, which does not contain phosphorus, a hardening promoter, a solvent, and the like.
摘要翻译：本发明涉及一种阻燃型环氧树脂组合物，其特征在于所述阻燃环氧树脂组合物包含：（A）至少一种环氧树脂;（B）含磷和氮的杂环化合物，所述化合物具有可与作为硬化剂的环氧树脂的环氧基反应的部分，并且具有如式（I）所示的结构：其中m为0-2的整数，n为整数为3〜7，但至少1m不为2.由上述成分（A）和（B）组成的环氧树脂组合物具有改善的阻燃性，因此适合用作部件所需的阻燃材料复合材料，层压板，印刷电路板，电子产品，电气产品等。根据应用范围，组合物可以选择性地添加添加剂，例如不含磷的硬化剂，硬化促进剂，溶剂等。

5. 发明授权

US06617029B2 Nitrogen-containing flame retarding epoxy resin and an epoxy resin composition containing the same 有权
标题翻译：含氮阻燃环氧树脂和含有该阻燃环氧树脂的环氧树脂组合物
公开(公告)号：US06617029B2
公开(公告)日：2003-09-09
申请号：US10035238
申请日：2002-01-04
申请人： Kuen-Yuan Hwang , Hong-Hsing Chen , Chih-Fu Chen , Huan-Chang Chao
发明人： Kuen-Yuan Hwang , Hong-Hsing Chen , Chih-Fu Chen , Huan-Chang Chao
IPC分类号： B32B2738
CPC分类号： C08K5/34922 , H05K1/0326 , Y10T428/31511 , C08L63/00
摘要： The present invention relates to a nitrogen-containing epoxy resin of the following formula: wherein R's are the same or different and each represents a hydrogen atom or —R13—C6-10 aryl-(OR14)p, and the aryl group is optionally substituted with C1-6 alkyl group, in which R13 represents a C1-6 alkylene group or a phenylene —CH2— group optionally substituted with a hydroxy group, R14 represents a glycidyl group, and p is an integer of 1 or 2, provided that at least one R group is not a hydrogen atom; R1 represents a phenyl group or —N(R)2 group in which R is defined as above. The resin is produced from sequentially reacting melamine derivatives with aldehydes, phenolic compounds, and epihalohydrin. The nitrogen-containing epoxy resin, alone or as part of an epoxy resin composition, provides excellent flame-retardant and heat-resistant properties without using halogen or diantimony trioxide; hence, the resin and its composition are favorable as encapsulating materials for semiconductor applications.
摘要翻译：本发明涉及下式的含氮环氧树脂：其中R相同或不同，各自表示氢原子或-R13-C6-10芳基 - （OR14）p，并且芳基任选被取代具有C 1-6烷基，其中R 13表示C 1-6亚烷基或任选被羟基取代的亚苯基-CH 2 - 基，R 14表示缩水甘油基，p表示1或2的整数，条件是在至少一个R基团不是氢原子; R 1表示苯基或-N（R）2基团，其中R如上定义。树脂是通过使三聚氰胺衍生物与醛，酚类化合物和表卤代醇顺序反应制备的。单独或作为环氧树脂组合物的一部分的含氮环氧树脂在不使用卤素或二氧化锑的情况下提供优异的阻燃和耐热性能; 因此，树脂及其组合物作为用于半导体应用的封装材料是有利的。

6. 发明授权

US6034185A Epoxy resin composition containing polyalkyl phenol resins and/or polyalkyl phenol epoxy resins 失效
标题翻译：含有聚烷基酚醛树脂和/或聚烷基酚环氧树脂的环氧树脂组合物
公开(公告)号：US6034185A
公开(公告)日：2000-03-07
申请号：US944818
申请日：1997-10-06
申请人： Kuen-Yuan Hwang , Hong-Hsing Chen , Biing Lu Perng , Shang Wen Chen
发明人： Kuen-Yuan Hwang , Hong-Hsing Chen , Biing Lu Perng , Shang Wen Chen
IPC分类号： C08L63/00 , C08G59/52 , C08G59/62 , C08L63/04 , C08G65/48
CPC分类号： C08G59/621 , C08G59/52 , C08L63/04
摘要： This invention relates to an epoxy resin composition which comprises polyalkyl phenol resins or polyalkyl phenol epoxy resins or both, wherein the polyalkyl phenol resins are represented by formula (I): ##STR1## wherein Ra, Rb and Rc may be the same or different from each other and stand for C.sub.1-5 alkyl styryl or halogen respectively;n is an integer of 0 to 4;k is an integer of 0 to 3;l is an integer of 0 to 4; andm is an integer of 1 to 10;and the polyalkyl phenol epoxy resins, which are obtained by reacting polyalkyl phenol resins of formula (I) with epihalohydrins, are represented by formula (II): ##STR2## wherein G stands for ##STR3## while the other symbols are the same as those defined above. The epoxy resin composition of this invention is able to provide a reactivity at lower temperatures and provide lower viscosity when used as hardener resins, as compared with traditional phenolic novolacs. Excellent molding properties and excellent stress resistance in soldering are obtained accordingly when such composition is used in electronic packaging.
摘要翻译：本发明涉及包含聚烷基酚树脂或聚烷基酚环氧树脂或两者的环氧树脂组合物，其中聚烷基酚树脂由式（I）表示：其中Ra，Rb和Rc可以彼此相同或不同，分别代表C1-5烷基苯乙烯基或卤素; n为0〜4的整数。 k为0〜3的整数， l为0〜4的整数; m为1〜10的整数。和通过使式（I）的聚烷基酚树脂与表卤代醇反应得到的聚烷基酚环氧树脂由式（II）表示：其中G代表其它符号与上述定义相同。与传统酚醛清漆相比，本发明的环氧树脂组合物能够在较低温度下提供反应性，并且当用作固化剂树脂时提供较低的粘度。因此，当将这种组合物用于电子包装时，可获得优异的成型性能和优异的耐焊接性。

7. 发明授权

US06818307B2 Flame retarded epoxy resin composition 失效
标题翻译：阻燃环氧树脂组合物
公开(公告)号：US06818307B2
公开(公告)日：2004-11-16
申请号：US10618529
申请日：2003-07-10
申请人： Kuen-Yuan Hwang , Hong-Hsing Chen , Tsung-Yu Chen , Ching Fu Kao
发明人： Kuen-Yuan Hwang , Hong-Hsing Chen , Tsung-Yu Chen , Ching Fu Kao
IPC分类号： B32B2738
CPC分类号： C08K5/5399 , H05K1/0326 , H05K1/0373 , Y10T428/31511 , Y10T428/31522 , Y10T428/31529 , C08L63/00
摘要： The present invention relates to a flame retarded epoxy resin composition, which is characterized by that said flame retarded epoxy resin composition comprising: (A) at least one type of epoxy resin; (B) a phosphorus-and-nitrogen-containing heterocyclic compound, said compound having a moiety which can react with the epoxy group of the epoxy resin, usedful as a hardening agent, and having a structure as shown by formula (I): wherein m is an integer of from 0 to 2, n is an integer of from 3 to 7, but at least one m is not 2. The epoxy resin composition consisting of the above components (A) and (B) has improved flame retarded property and thus is suitably used as the flame retarded material required for the parts of composite material, laminated plates, printed circuit boards, electronic products, electrical products, and the like. According to the range of applications, the composition can be selectively added with additives such as a hardening agent, which does not contain phosphorus, a hardening promoter, a solvent, and the like.
摘要翻译：本发明涉及一种阻燃型环氧树脂组合物，其特征在于所述阻燃环氧树脂组合物包含：（A）至少一种环氧树脂;（B）含磷和氮的杂环化合物，所述化合物具有可与作为硬化剂的环氧树脂的环氧基反应的部分，并且具有如式（I）所示的结构：其中m为0-2的整数，n为整数为3〜7，但至少1m不为2.由上述成分（A）和（B）组成的环氧树脂组合物具有改善的阻燃性，因此适合用作部件所需的阻燃材料复合材料，层压板，印刷电路板，电子产品，电气产品等。根据应用范围，组合物可以选择性地添加添加剂，例如不含磷的硬化剂，硬化促进剂，溶剂等。

8. 发明授权

US06576690B1 Phosphorous-containing flame retarding epoxy resin and an epoxy resin composition containing the same 有权
标题翻译：含磷阻燃环氧树脂和含有这种阻燃环氧树脂的环氧树脂组合物
公开(公告)号：US06576690B1
公开(公告)日：2003-06-10
申请号：US10104567
申请日：2002-03-22
申请人： Kuen-Yuan Hwang , Hong-Hsing Chen , Chih-Fu Chen
发明人： Kuen-Yuan Hwang , Hong-Hsing Chen , Chih-Fu Chen
IPC分类号： C08K336
CPC分类号： C08G59/1422 , C08G59/4071 , H05K1/0326
摘要： The present invention relates to a phosphorous-containing flame retarding epoxy resin and their composition comprising the nitrogen-containing flame retarding epoxy resin. More specifically, the present invention relates to a flame retarding epoxy resin having a pendent phosphorous-containing functional group and their composition comprising the nitrogen-containing flame retarding epoxy resin. The flame retarding phosphorous-containing epoxy resin and the epoxy resin composition containing the same of the present invention possess excellent flame retarding property and heat resistance without containing halogen and diantimony trioxide. Therefore they are useful as an encapsulating material in the semiconductor industry and the cured article prepared from the composition exhibits excellent molding ability and excellent reliance.
摘要翻译：本发明涉及含磷阻燃环氧树脂及其组合物，其含有含氮阻燃环氧树脂。更具体地，本发明涉及具有含侧基的含磷官能团的阻燃性环氧树脂及其组合物，其包含含氮阻燃环氧树脂。含有阻燃性含磷环氧树脂和含有本发明的阻燃性含磷环氧树脂的环氧树脂组合物在不含卤素和三氧化二锑的情况下具有优异的阻燃性和耐热性。因此，它们可用作半导体工业中的封装材料，并且由该组合物制备的固化制品表现出优异的模塑能力和优异的依赖性。

9. 发明授权

US08222441B2 Phosphorus-containing compounds and their preparing process and use 有权
标题翻译：含磷化合物及其制备方法和用途
公开(公告)号：US08222441B2
公开(公告)日：2012-07-17
申请号：US12385573
申请日：2009-04-13
申请人： Ching-Hsuan Lin , Tsung Li Lin , Chia Wei Chang , Kuen-Yuan Hwang , An-Pang Tu , Fang-Hsien Su
发明人： Ching-Hsuan Lin , Tsung Li Lin , Chia Wei Chang , Kuen-Yuan Hwang , An-Pang Tu , Fang-Hsien Su
IPC分类号： C07F9/32 , C08L71/02
CPC分类号： C07F9/657172 , C08K5/5313 , C09K21/12
摘要： A series of novel phosphorus-containing compounds having the following formula are disclosed: wherein R1-R12, A, B, D, X, and Y are as defined in the specification. A process for the preparation of the compound of formula (1), a curing agent, and a flame resistant epoxy resin and a preparation process thereof are also provided.
摘要翻译：公开了一系列具有下式的新型含磷化合物：其中R1-R12，A，B，D，X和Y如说明书中所定义。还提供了制备式（1）化合物，固化剂和阻燃环氧树脂的方法及其制备方法。

10. 发明申请

US20080262127A1 FLAME RESISTANT RESIN COMPOSITION 审中-公开
标题翻译：耐火树脂组合物
公开(公告)号：US20080262127A1
公开(公告)日：2008-10-23
申请号：US12018099
申请日：2008-01-22
申请人： Kuen-Yuan Hwang , An-Pang Tu , Gai-Chi Chen , I-Cheng Hsu
发明人： Kuen-Yuan Hwang , An-Pang Tu , Gai-Chi Chen , I-Cheng Hsu
IPC分类号： C08K3/00 , C08K3/20 , C08K3/26
CPC分类号： C08G59/3218 , C08G59/621 , C08K3/013 , C08L63/00 , C08L2666/54
摘要： A flame resistant resin composition is provided, which includes: (A) at least an epoxy resin having a biphenylic unit or a naphthalenic unit; (B) phenolic resins used as a curing agent, the phenolic resins include at least a phenolic resin having a biphenylic moiety and a polyphenolic moiety, wherein the the at least a phenolic resin having a biphenylic moiety and a polyphenolic moiety is in an amount of 30 to 100 wt % of the total weight of the curing agents; (C) a curing-promoting agent; and (D) an inorganic filler material. The resin composition includes an epoxy resin having a biphenylic unit or a naphthalenic unit and the phenolic resin having a biphenylic moiety and a polyphenolic moiety as a curing agent, such that excellent flame resistance can be achieved without adding flame resistant agents. The resin composition also has a higher glass transition temperature to improve the water absorption issue after curing, and increases heat stability. Therefore, the resin composition is particularly useful in composite materials, forming materials or semiconductor packaging materials.
摘要翻译：提供了一种阻燃树脂组合物，其包括：（A）至少一种具有联苯单元或萘单元的环氧树脂; （B）用作固化剂的酚醛树脂，酚醛树脂至少包括具有联苯部分和多酚部分的酚醛树脂，其中至少一种具有联苯部分和多酚部分的酚醛树脂的量为 30至100重量％的固化剂总重量; （C）固化促进剂; 和（D）无机填料。树脂组合物包括具有联苯单元或萘单元的环氧树脂和具有联苯部分和多酚部分作为固化剂的酚醛树脂，使得可以在不添加阻燃剂的情况下实现优异的阻燃性。树脂组合物还具有较高的玻璃化转变温度，以改善固化后的吸水问题，并且增加热稳定性。因此，树脂组合物特别适用于复合材料，成型材料或半导体封装材料。

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