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1. 发明授权

US09284267B2 Process for the preparation of urethanes 有权
标题翻译：制备聚氨酯的方法
公开(公告)号：US09284267B2
公开(公告)日：2016-03-15
申请号：US12321995
申请日：2009-01-28
申请人： Andreas Jacob , Stefan Wershofen , Stephan Klein , Jörg Sundermeyer , Fuming Mei
发明人： Andreas Jacob , Stefan Wershofen , Stephan Klein , Jörg Sundermeyer , Fuming Mei
IPC分类号： C07C263/04 , C07C269/04 , C07C273/18
CPC分类号： C07C269/00 , B01J31/183 , B01J31/1835 , C07C263/04 , C07C269/04 , C07C273/18 , C07C273/1809 , C07C271/12 , C07C271/28 , C07C275/28
摘要： Urethanes are prepared by oxidative carbonylation of at least one amino compound in the presence of carbon monoxide, oxygen and organic, at least one hydroxyl-group-carrying compound. The carbonylation is carried out in the absence of halogen-containing promoters. The carbonylation is also carried out in the presence of a metal complex catalyst which contains neutral bidentate N-chelate ligands of the (N˜N) type, two monoanionic N,O-chelate ligands of the general type (N˜O)− or tetradentate dianionic chelate ligands (O˜N˜N˜O)2−.
摘要翻译：在一氧化碳，氧和有机物，至少一种含羟基化合物的存在下，通过氧化羰基化至少一种氨基化合物制备聚氨酯。在不含卤素促进剂的情况下进行羰基化。羰基化还可以在金属络合物催化剂的存在下进行，该催化剂含有（N〜N）型中性二齿N-螯合配体，一般类型（N〜O）的两个单阴离子N，O-螯合配体）或四齿二离子螯合配体（O〜N〜N〜O）2-。

2. 发明申请

US20140155562A1 HOMOLEPTIC RARE EARTH TRIARYL COMPLEXES 审中-公开
标题翻译： HOMOLEPTIC RARE EARTH TRIARYL复合材料
公开(公告)号：US20140155562A1
公开(公告)日：2014-06-05
申请号：US14235285
申请日：2012-08-02
申请人： Oliver Thomas , Jörg Sundermeyer
发明人： Oliver Thomas , Jörg Sundermeyer
IPC分类号： C07F9/53 , C08F136/08 , C07F9/535 , C08G63/84
CPC分类号： C07F9/5345 , C07F9/5352 , C08F4/52 , C08F4/545 , C08F36/08 , C08F136/08 , C08G63/00 , C08G63/823 , C08G63/84 , C08G69/00 , C08G69/14
摘要： The invention relates to chelate-stabilized homleptic triaryl compounds based on phenylphosphoranes, to methods for preparing same and to the use thereof as catalysts. According to the invention, the object is achieved by homleptic rare earth triaryl complexes of the general formula (I), where SE=Sc, Y, La, Ce, Pr, Nd, Pm, Sm, Eu, Gd, Tb, Dy, Ho, Er, Tm, Yb or Lu; X=O, CRR′; R1, R2=phenyl; R, R′=mutually independently H, alkyl with n=10 C atoms, phenyl or trimethylsilyl.
摘要翻译：本发明涉及基于苯基磷烷的螯合稳定的亲和三芳基化合物，其制备方法及其作为催化剂的用途。根据本发明，该目的通过通式（I）的亲水性稀土三芳基络合物实现，其中SE = Sc，Y，La，Ce，Pr，Nd，Pm，Sm，Eu，Gd，Tb，Dy， Ho，Er，Tm，Yb或Lu; X = O，CRR'; R1，R2 =苯基; R，R'=相互独立地为H，具有n = 10个C原子的烷基，苯基或三甲基甲硅烷基。

3. 发明申请

US20110034713A1 Ortho-metalated, chelate-stabilized benzylamines of the rare-earth metals (RE) Ar3RE 审中-公开
标题翻译：稀土金属（RE）Ar3RE的正金属化，螯合稳定的苄胺
公开(公告)号：US20110034713A1
公开(公告)日：2011-02-10
申请号：US12745057
申请日：2008-11-25
申请人： Jörg Sundermeyer , Alexander Petrov , Oliver Thomas
发明人： Jörg Sundermeyer , Alexander Petrov , Oliver Thomas
IPC分类号： C07F5/00
CPC分类号： C07D207/06 , C07F3/00
摘要： The present invention describes homoleptic, ortho-metalated, chelate-stabilized benzylamine complexes of the rare-earth metals. The rare-earth metals are selected from Sc, Y, La, Ce, Pr, Nd, Pm, Sm, Eu, Gd, Tb, Dy, Ho, Er, Tm, Yb, Lu. In the complexes according to the present invention, at least one benzylic proton of the benzylamine ligand is replaced by an alkyl or aryl group. Such complexes are preferred in which both benzylic protons of the benzylamine ligand are replaced by an alkyl- or aryl group. The complexes according to the present invention are produced by reaction of chelate-stabilized rare-earth metal halides with ortho-lithiated aryl ligands at room temperature under inert gas atmosphere. The complexes according to the present invention are thermally stable and suitable for being used as catalysts for the hydroamination of olefins.
摘要翻译：本发明描述了稀土金属的均聚，邻位金属化，螯合稳定的苄胺络合物。稀土金属选自Sc，Y，La，Ce，Pr，Nd，Pm，Sm，Eu，Gd，Tb，Dy，Ho，Er，Tm，Yb，Lu。在根据本发明的络合物中，苄胺配体的至少一个苄基质子被烷基或芳基取代。这种络合物是优选的，其中苄胺配体的两个苄基质子都被烷基或芳基取代。根据本发明的络合物通过螯合稳定的稀土金属卤化物与邻位锂化的芳基配体在室温下在惰性气体气氛下反应来制备。根据本发明的络合物是热稳定的并且适用于用作烯烃的水解的催化剂。

4. 发明授权

US07667038B2 Tantalum and niobium compounds 失效
标题翻译：钽和铌化合物
公开(公告)号：US07667038B2
公开(公告)日：2010-02-23
申请号：US12249463
申请日：2008-10-10
申请人： Knud Reuter , Daniel Gaess , Jörg Sundermeyer
发明人： Knud Reuter , Daniel Gaess , Jörg Sundermeyer
IPC分类号： C07F9/00 , C07D333/02
CPC分类号： C07F9/005 , H01L21/28556
摘要： The present invention relates to specific, novel tantalum and niobium compounds which can serve as starting materials for the preparation of chemical vapour deposition (CVD) precursors.
摘要翻译：本发明涉及可用作制备化学气相沉积（CVD）前体的起始材料的具体的新型钽和铌化合物。

5. 发明申请

US20100024133A1 TRIS(HETEROCYCLYL) METAL COMPLEXES, WASHING AND CLEANING AGENTS CONTAINING THE SAME, AND USE AS BLEACH CATALYSTS 有权
标题翻译：金属复合物，含有它们的洗涤和清洁剂，以及作为漂白催化剂使用的TRIS（杂环）金属络合物
公开(公告)号：US20100024133A1
公开(公告)日：2010-02-04
申请号：US12577442
申请日：2009-10-12
申请人： Andre Hätzelt , Anette Nordskog , Stefan Leopold , Peter Schmiedel , Wolfgang von Rybinski , Jörg Sundermeyer , Jan Döring
发明人： Andre Hätzelt , Anette Nordskog , Stefan Leopold , Peter Schmiedel , Wolfgang von Rybinski , Jörg Sundermeyer , Jan Döring
IPC分类号： D06L3/10 , C07F9/02
CPC分类号： C11D3/3932 , C11D3/168
摘要： Tris(heterocyclyl)-metal complexes and the use thereof as bleach catalysts are described.
摘要翻译：描述了三（杂环基） - 金属络合物及其作为漂白催化剂的用途。

6. 发明授权

US07442407B2 Tantalum and niobium compounds and their use for chemical vapour deposition (CVD) 失效
公开(公告)号：US07442407B2
公开(公告)日：2008-10-28
申请号：US11482397
申请日：2006-07-07
申请人： Knud Reuter , Jörg Sundermeyer , Alexei Merkoulov , Wolfgang Stolz , Kerstin Volz , Michael Pokoj , Thomas Ochs
发明人： Knud Reuter , Jörg Sundermeyer , Alexei Merkoulov , Wolfgang Stolz , Kerstin Volz , Michael Pokoj , Thomas Ochs
IPC分类号： B05D5/12 , C07F517/00
CPC分类号： C07F9/005 , C23C16/34 , Y10T428/12528
摘要： Tantalum and niobium compounds having the general formula (I) and their use for the chemical vapour deposition process are described: wherein M stands for Nb or Ta, R1 and R2 C1 to C12 alkyl, C5 to C12 cycloalkyl, C6 to C10 aryl radicals, 1-alkenyl, 2-alkenyl, 3-alkenyl, triorganosilyl radicals —SiR3, or amino radicals NR2 R3 is C1 to C8 alkyl, C5 to C10 cycloalkyl, C6 to C14 aryl radical, or SiR3 or NR2, R4 denotes Cl, Br, I, NIH—R5 where R5 is C1 to C8 alkyl, C5 to C10 cycloalkyl or C6 to C10 aryl radical, or O—R6 where R6=optionally substituted C1 to C11 alkyl, C5 to C10 cycloalkyl, C6 to C10 aryl radical, or —SiR3, or BH4, or an allyl radical, or an indenyl radical, or an benzyl radical, or an cyclopentadienyl radical, or —NIR—NR′R″ (hydrazido(-1), wherein R, R′ and R″ have the aforementioned meaning of R, or CH2SiMe3, pseudohalide, or silylamide —N(SiMe3)2, and R7 and R8 are H, C1 to C12 alkyl, C5 to C12 cycloalkyl or C6 to C10 aryl radicals.

7. 发明申请

US20140163187A1 CYCLOPENTADIENYLIDENE-PHOSPHORANE CONSTRAINED GEOMETRY COMPLEXES OF RARE EARTH METALS 审中-公开
标题翻译：稀土金属的环烯二烯基磷光体约束几何复合物
公开(公告)号：US20140163187A1
公开(公告)日：2014-06-12
申请号：US14235259
申请日：2012-08-02
申请人： Nina Hillesheim , Jörg Sundermeyer
发明人： Nina Hillesheim , Jörg Sundermeyer
IPC分类号： C08F4/52 , C08G63/84 , C07F9/54
CPC分类号： C08F4/52 , B01J31/0235 , B01J31/2265 , B01J31/2295 , B01J2531/0205 , B01J2531/36 , B01J2531/37 , B01J2531/38 , C07F9/5352 , C07F9/54 , C07F17/00 , C08F36/08 , C08F2420/02 , C08G63/823 , C08G63/84 , C08F136/08 , C08F4/545
摘要： The invention relates to η5:η1-cyclopentadienylidene-phosphorane constrained geometry complexes of rare earth metals, abbreviated to η5:η1-CpPC-CGC, method for production and use of same. The η5:η1-CpPC-CGCs correspond to the general formula (1), wherein SE=Sc, Y, La, Ce, Pr, Nd, Pm, Sm, Eu, Gd, Tb, Dy, Ho, Er, Tm, Yb or Lu; X=independently of one another, a mono-anionic diorganoamido-, bistrimethylsilylamido-, halogenido-, alkyl-, aryl-, alkoxo-, aryloxo- or alkylaluminate (AlR4−) substituent; L=neutral ligand (PR3, NR3, pyridine), solvent molecule (THF, ether, DMF, DMSO, HMPT, tetrahydropyran THP, tetrahydrothiofuran THT); R=alkyl with up to 1-10 C atoms or mono- or polycyclical aryl with 6 to 20 C atoms; R1, R4=independently of one another H or methyl; R2, R3=independently of one another, H or methyl or tertiary butyl or together a substituted cycloalkyl group; R5, R6=methyl, n-butyl, tertiary butyl or phenyl; R7, R8=independently of one another H, trimethylsilyl, alkyl with 1-10 C atoms or mono- or polycyclical aryl with 6 to 20 C atoms, and m=0, 1, 2 or 3.
摘要翻译：本发明涉及＆amp; 5＆gt;稀土金属的1-环戊二烯基 - 正磷烷约束几何配合物，缩写为＆amp; e＆gt; 1-CpPC-CGC，其生产和使用方法。其中SE = Sc，Y，La，Ce，Pr，Nd，Pm，Sm，Eu，Gd，Tb，Dy，Ho等于通式（1） Er，Tm，Yb或Lu; X =彼此独立，单阴离子二有机基酰胺基，双三甲基甲硅烷基氨基 - ，卤代 - ，烷基 - ，芳基 - ，烷氧基 - ，芳氧基 - 或烷基铝酸盐（AlR 4 - ）取代基; L =中性配体（PR3，NR3，吡啶），溶剂分子（THF，醚，DMF，DMSO，HMPT，四氢吡喃THP，四氢噻呋喃THT）; R =具有至多1-10个C原子的烷基或具有6至20个C原子的单环或多环芳基; R1，R4 =彼此独立地为H或甲基; R2，R3彼此独立地为H或甲基或叔丁基或一起取代的环烷基; R 5，R 6 =甲基，正丁基，叔丁基或苯基; R 7，R 8彼此独立地为H，三甲基甲硅烷基，具有1-10个C原子的烷基或具有6至20个C原子的单环或多环芳基，m = 0,1,2或3。

8. 发明申请

US20130303740A1 METHOD FOR PRODUCING URETHANES 有权
标题翻译：生产尿素的方法
公开(公告)号：US20130303740A1
公开(公告)日：2013-11-14
申请号：US13816526
申请日：2011-08-09
申请人： Felix Gärtner , Andreas Jacob , Jörg Sundermeyer , Stephan Klein , Stefan Wershofen
发明人： Felix Gärtner , Andreas Jacob , Jörg Sundermeyer , Stephan Klein , Stefan Wershofen
IPC分类号： C07C269/04 , C07C263/00
CPC分类号： C07C263/00 , B01J31/2243 , B01J2231/70 , B01J2531/0241 , B01J2531/16 , B01J2531/821 , B01J2531/822 , B01J2531/827 , B01J2531/828 , B01J2531/845 , B01J2531/847 , C07C245/08 , C07C251/24 , C07C269/04 , C07D213/30 , C07D215/26 , C07C271/28
摘要： The invention relates to a method for producing urethanes or ureas or mixtures of urethanes and ureas by oxidative carbonylation of organic amines in the presence of carbon monoxide, oxygen and a catalyst, where the catalyst used is a transition metal complex containing the structural feature: [Mn+(O˜N˜O)2−](n-2)+(L)m(Z−)n-2 and the method is carried out under halogen-free reaction conditions. The invention further relates to transition metal complexes containing said structural feature and also to the use of such transition metal complexes as catalysts in the production of urethanes or ureas or mixtures of urethanes and ureas.
摘要翻译：本发明涉及通过在一氧化碳，氧气和催化剂存在下通过有机胺的氧化羰基化制备氨基甲酸酯或脲或聚氨酯和脲的混合物的方法，其中使用的催化剂是含有结构特征的过渡金属络合物： Mn +（O〜N〜O）2 - ]（n-2）+（L）m（Z-）n-2，该方法在无卤素反应条件下进行。本发明进一步涉及含有所述结构特征的过渡金属络合物，以及在生产聚氨酯或脲或者聚氨酯和脲的混合物中使用这种过渡金属配合物作为催化剂。

9. 发明申请

US20100029540A1 BIHETEROARYL METAL COMPLEXES AS BLEACH CATALYSTS 有权
标题翻译： BIHETEROARYL金属复合材料作为漂白催化剂
公开(公告)号：US20100029540A1
公开(公告)日：2010-02-04
申请号：US12577489
申请日：2009-10-12
申请人： Andre Hätzelt , Anette Nordskog , Stefan Leopold , Peter Schmiedel , Wolfgang von Rybinski , Jörg Sundermeyer , Jan Döring
发明人： Andre Hätzelt , Anette Nordskog , Stefan Leopold , Peter Schmiedel , Wolfgang von Rybinski , Jörg Sundermeyer , Jan Döring
IPC分类号： C11D3/39 , C07D401/04 , C07D471/04
CPC分类号： C07D471/04 , C11D3/3932
摘要： Biheteroaryl metal complexes and the use thereof as bleach catalysts are described.
摘要翻译：描述了双杂芳基金属络合物及其作为漂白催化剂的用途。

10. 发明授权

US06846769B2 Vanadium-imido-phosphoraneiminato complexes for the polymerization of olefins 失效
标题翻译：用于烯烃聚合的亚氨基 - 亚膦酰亚胺络合物
公开(公告)号：US06846769B2
公开(公告)日：2005-01-25
申请号：US10216573
申请日：2002-08-09
申请人： Michael Arndt-Rosenau , Martin Hoch , Jörg Sundermeyer , Jennifer Kipke , Martin Lemke
发明人： Michael Arndt-Rosenau , Martin Hoch , Jörg Sundermeyer , Jennifer Kipke , Martin Lemke
IPC分类号： C07F9/00 , C07F9/50 , C07F9/535 , C07F19/00 , C08F4/68 , C08F10/00 , C08F210/18 , B01J31/24 , B01J31/00
CPC分类号： C07F9/5355 , C08F10/00 , C08F210/18 , C08F4/68 , C08F210/06 , C08F232/00 , C08F2500/25 , C08F2500/21
摘要： The present invention relates to vanadium-imido-phosphoraneiminato compounds, to compositions containing vanadium-imido-phosphoraneiminato compounds, which compositions are suitable especially as catalysts for the polymerization of olefins, especially for ethylene/propylene or ethylene/α-olefin copolymerization and the terpolymerization of those monomers with dienes.
摘要翻译：本发明涉及钒 - 亚氨基 - 亚膦酰亚胺化合物，含有含有亚氨基 - 亚膦酰亚胺化合物的组合物，该组合物特别适用于烯烃聚合的催化剂，特别是用于乙烯/丙烯或乙烯/α-烯烃共聚合的三元共聚的那些单体与二烯。

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