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    • 9. 发明申请
      US20140296455A1 MULTINUCLEAR METALLOCENE CATALYST COMPOUND FOR OLEFIN POLYMERISATION AND COPOLYMERISATION AND METHOD FOR MAKING THEREOF 审中-公开
    • MULTINUCLEAR METALLOCENE CATALYST COMPOUND FOR OLEFIN POLYMERISATION AND COPOLYMERISATION AND METHOD FOR MAKING THEREOF
    • US20140296455A1
    • 2014-10-02
    • US14353936
    • 2012-10-29
    • SAUDI BASIC INDUSTRIES CORPORATION
    • Haif Al-Shammari , Helmut G. Alt
    • C08F110/02
    • C08F110/02 , B01J31/1815 , B01J31/2295 , B01J2531/0205 , B01J2531/46 , B01J2531/48 , B01J2531/56 , B01J2531/847 , C08F4/65927 , C08F10/00 , C08F10/02 , C08F2410/03 , C08F4/65904 , C08F4/64013 , C08F4/7006 , C08F2500/04
    • The invention relates to a multinuclear metallocene catalyst compound according to Formula (1), wherein Y and Y′ are the same or different and independently selected from the group consisting of C1-20 linear, branched or cyclic hydrocarbyl groups, C1-30 aryl and substituted aryl groups; L and L′ are the same or different and are electron-donating groups independently selected from the elements of Group 15 of the Periodic Table; Q and Q′ are the same or different and independently selected from the group consisting of C1-30 alkylene groups; M″ is a metal selected from Groups 3, 4, 5, 6, 7, 8, 9 and 10 or from lanthanide series elements of the Periodic Table; Z is selected from the group consisting of hydrogen, a halogen and C1-20 hydrocarbyl, C1-20 alkoxy and C1-20 aryloxy groups; z is an integer from 1 to 4; n and n′ are independently 0 or 1, with 1≦(n+n′)≦2; B and B′ are the same or different and each is a metallocene compound, with B being represented by the compound of Formula (2) and B′ being represented by the compound of Formula (3), wherein Si is silicon; R and R′ are the same or different and independently a hydrogen or a C1-20 alkyl or aryl group; D, D′, E and E′ are independently ligand compounds having a cyclopentadienyl skeleton selected from cyclopentadienyl, substituted cyclopentadienyl, indenyl, substituted indenyl, fluorenyl and substituted fluorenyl; M and M′ are the same or different and each is independently selected from the group consisting of scandium, yttrium, lanthanoid series elements, titanium, zirconium, hafnium, vanadium, niobium, and tantalum; X and X′ are the same or different and each is selected from the group consisting of hydrogen, a halogen, a C1-20 hydrocarbyl group, C1-20 alkoxy group; and C1-20 aryloxy group; x and x′ are independently integers from 1 to 3. This invention also relates to a catalyst system comprising said multinuclear metallocene catalyst compound and a co-catalyst, to a method of making the multinuclear metallocene catalyst compound and to a process for the polymerisation and copolymerisation of an olefin in the presence of said catalyst system. The invention relates to a multinuclear metallocene catalyst compound according to Formula 1, wherein: Y and Y′ are the same or different and independently selected from the group consisting of C1-20 linear, branched or cyclic hydrocarbyl groups, C1-30 aryl and substituted aryl groups; L and U are the same or different and are electron-donating groups independently selected from the elements of Group 15 of the Periodic Table; Q and Q′ are the same or different and independently selected from the group consisting of Ci-3o alkylene groups; M″ is a metal selected from Groups 3, 4, 5, 6, 7, 8, 9 and 10 or from lanthanide series elements of the Periodic Table; Z is selected from the group consisting of hydrogen, a halogen and C1-20 hydrocarbyl, C1-20 alkoxy and C1-20 aryloxy groups; z is an integer from 1 to 4; n and n′ are independently 0 or 1, with 1
    • 基本信息 添加关注 加入工作空间 PDF全文 PDF下载 全文下载 相似专利 双屏查看 权利要求书 说明书全文 Global Dossier Espacenet 法律信息 同族专利 专利引用
    • 10. 发明申请
      US20140163187A1 CYCLOPENTADIENYLIDENE-PHOSPHORANE CONSTRAINED GEOMETRY COMPLEXES OF RARE EARTH METALS 审中-公开
    • CYCLOPENTADIENYLIDENE-PHOSPHORANE CONSTRAINED GEOMETRY COMPLEXES OF RARE EARTH METALS
    • 稀土金属的环烯二烯基磷光体约束几何复合物
    • US20140163187A1
    • 2014-06-12
    • US14235259
    • 2012-08-02
    • Nina Hillesheim , Jörg Sundermeyer
    • Nina Hillesheim , Jörg Sundermeyer
    • C08F4/52 , C08G63/84 , C07F9/54
    • C08F4/52 , B01J31/0235 , B01J31/2265 , B01J31/2295 , B01J2531/0205 , B01J2531/36 , B01J2531/37 , B01J2531/38 , C07F9/5352 , C07F9/54 , C07F17/00 , C08F36/08 , C08F2420/02 , C08G63/823 , C08G63/84 , C08F136/08 , C08F4/545
    • The invention relates to η5:η1-cyclopentadienylidene-phosphorane constrained geometry complexes of rare earth metals, abbreviated to η5:η1-CpPC-CGC, method for production and use of same. The η5:η1-CpPC-CGCs correspond to the general formula (1), wherein SE=Sc, Y, La, Ce, Pr, Nd, Pm, Sm, Eu, Gd, Tb, Dy, Ho, Er, Tm, Yb or Lu; X=independently of one another, a mono-anionic diorganoamido-, bistrimethylsilylamido-, halogenido-, alkyl-, aryl-, alkoxo-, aryloxo- or alkylaluminate (AlR4−) substituent; L=neutral ligand (PR3, NR3, pyridine), solvent molecule (THF, ether, DMF, DMSO, HMPT, tetrahydropyran THP, tetrahydrothiofuran THT); R=alkyl with up to 1-10 C atoms or mono- or polycyclical aryl with 6 to 20 C atoms; R1, R4=independently of one another H or methyl; R2, R3=independently of one another, H or methyl or tertiary butyl or together a substituted cycloalkyl group; R5, R6=methyl, n-butyl, tertiary butyl or phenyl; R7, R8=independently of one another H, trimethylsilyl, alkyl with 1-10 C atoms or mono- or polycyclical aryl with 6 to 20 C atoms, and m=0, 1, 2 or 3.
    • 本发明涉及＆amp; 5＆gt;稀土金属的1-环戊二烯基 - 正磷烷约束几何配合物，缩写为＆amp; e＆gt; 1-CpPC-CGC，其生产和使用方法。 其中SE = Sc，Y，La，Ce，Pr，Nd，Pm，Sm，Eu，Gd，Tb，Dy，Ho等于通式（1） Er，Tm，Yb或Lu; X =彼此独立，单阴离子二有机基酰胺基，双三甲基甲硅烷基氨基 - ，卤代 - ，烷基 - ，芳基 - ，烷氧基 - ，芳氧基 - 或烷基铝酸盐（AlR 4 - ）取代基; L =中性配体（PR3，NR3，吡啶），溶剂分子（THF，醚，DMF，DMSO，HMPT，四氢吡喃THP，四氢噻呋喃THT）; R =具有至多1-10个C原子的烷基或具有6至20个C原子的单环或多环芳基; R1，R4 =彼此独立地为H或甲基; R2，R3彼此独立地为H或甲基或叔丁基或一起取代的环烷基; R 5，R 6 =甲基，正丁基，叔丁基或苯基; R 7，R 8彼此独立地为H，三甲基甲硅烷基，具有1-10个C原子的烷基或具有6至20个C原子的单环或多环芳基，m = 0,1,2或3。
    • 基本信息 添加关注 加入工作空间 PDF全文 PDF下载 全文下载 相似专利 双屏查看 权利要求书 说明书全文 Global Dossier Espacenet 法律信息 同族专利 专利引用
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