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1. 发明专利

JP2009220101A Method for producing gas adsorbing material and carbon dioxide, and method for recovering carbon dioxide 审中-公开
标题翻译：用于生产气体吸附材料和二氧化碳的方法和用于回收二氧化碳的方法
公开(公告)号：JP2009220101A
公开(公告)日：2009-10-01
申请号：JP2009010000
申请日：2009-01-20
申请人： Ngk Insulators Ltd , 日本碍子株式会社
发明人： GOTO MASASHI , FURUKAWA MASAHIRO
IPC分类号： B01J20/22 , B01D53/02 , B01D53/04 , B01D53/62
CPC分类号： Y02A50/2342 , Y02C10/08
摘要： PROBLEM TO BE SOLVED: To enhance the sorptive property of carbon dioxide and to recover carbon dioxide efficiently. SOLUTION: A gas adsorbing material 10 is composed of a stacked unit wherein a plurality of monomers 20 provided with four complex nuclear metals 22 (for example, Zn) combined in a tetrahedron shape by oxygen, and a plurality of monocarboxylic acids 24 that are coordinated in the complex nuclear metals 22 so as to have interaction parts 25 (e.g., benzene ring) stacked with other structures by uncombined interaction and to surround the complex nuclear metals 22. When an adsorption gas (carbon dioxide) is present, the gas adsorbing material 10 undergoes phase transition to a structure having spaces each of which is larger in molecular size than the gas, so as to incorporate the adsorbed gas. When the pressure of adsorbed gas is further increased, it undergoes even greater structural phase transition to a structure capable of incorporating a larger amount of the adsorbed gas. The gas adsorbing material 10 undergoes such structural phase transition reversibly, so that it can achieve adsorption and desorption of carbon dioxide while exerting a high adsorption amount compared with methane, nitrogen, steam, or the like. COPYRIGHT: (C)2010,JPO&INPIT
摘要翻译：要解决的问题：提高二氧化碳的吸附性能并有效回收二氧化碳。气体吸附材料10由堆叠单元构成，其中多个单体20具有四个以氧为四面体结合的复合核金属22（例如Zn）和多个单羧酸24 其在复杂核金属22中协调，以便通过未结合的相互作用与其它结构堆叠的相互作用部分25（例如苯环）并且包围复合核金属22.当存在吸附气体（二氧化碳）时，气体吸附材料10经历相变到具有比气体分子尺寸大的空间的结构，从而结合吸附气体。当吸附气体的压力进一步增加时，其经历与能够引入更多吸附气体的结构更大的结构相变。气体吸附材料10可逆地进行这种结构相变，从而与甲烷，氮气，蒸汽等相比能够实现高吸附量的二氧化碳的吸附和解吸。版权所有（C）2010，JPO＆INPIT

2. 发明专利

JP2010202641A Method for producing ceramic precursor 审中-公开
标题翻译：生产陶瓷前体的方法
公开(公告)号：JP2010202641A
公开(公告)日：2010-09-16
申请号：JP2010011270
申请日：2010-01-21
申请人： Ngk Insulators Ltd , 日本碍子株式会社
发明人： FURUKAWA MASAHIRO , NANBA MASAHARU , SAKAMOTO MASAOMI , KURIHARA MASATO
IPC分类号： C07C51/41 , C01G25/00 , C07C55/07 , C07F5/00 , C07F7/00 , C07F19/00
摘要： PROBLEM TO BE SOLVED: To provide a method for producing a ceramic precursor obtained by more dispersing an addition component into the main component.
SOLUTION: In the method for producing a ceramic precursor, the total or a part of a first raw material including component (a), being the main component, and a second raw material including component (b), being an addition component, is made into complex ligands 12 and 14, each surrounded by bridging ligands; the first and second raw materials are added to a solvent including at least one of water, methanol and ethanol so that the total amount of the first and second raw materials is more excessive than the solubility of the solvent, thereby forming a suspending fluid; and the first and second raw materials each added in an excess amount are eluted and become to be in a high concentration state, thereby depositing the ceramic precursor 20 from the solvent.
COPYRIGHT: (C)2010,JPO&INPIT
摘要翻译：待解决的问题：提供通过将添加成分分散在主成分中而得到的陶瓷前体的制造方法。解决方案：在陶瓷前体的制造方法中，包含作为主要成分的组分（a）和包含组分（b）的第二原料的第一原料的总或一部分作为添加组分被制成复合配体12和14，每个被配位体包围; 将第一和第二原料加入到包含水，甲醇和乙醇中的至少一种的溶剂中，使得第一和第二原料的总量比溶剂的溶解度更大，从而形成悬浮液; 并且分别过量的第一和第二原料被洗脱并变成高浓度状态，从而从溶剂沉积陶瓷前体20。版权所有（C）2010，JPO＆INPIT

3. 发明专利

JP2004136216A Silicon carbide-based catalyst body and its production method 有权
公开(公告)号：JP2004136216A
公开(公告)日：2004-05-13
申请号：JP2002303923
申请日：2002-10-18
申请人： Ngk Insulators Ltd , 日本碍子株式会社
发明人： FURUKAWA MASAHIRO , MORIMOTO KENJI , KAWASAKI SHINJI
IPC分类号： B01D53/86 , B01D53/94 , B01J23/02 , B01J23/58 , B01J27/224 , B01J35/04 , B01J37/00 , B01J37/02 , C04B35/565 , C04B38/00 , C04B41/85
CPC分类号： C04B38/0012 , B01D53/9422 , B01D2255/1021 , B01D2255/2022 , B01J23/02 , B01J23/58 , B01J27/224 , B01J35/04 , B01J37/0009 , B01J37/0018 , B01J37/0215 , B01J37/0248 , C04B35/565 , C04B2111/0081 , C04B2235/3826 , C04B2235/422 , C04B2235/5436 , C04B2235/6021 , C04B2235/80
摘要： PROBLEM TO BE SOLVED: To provide a silicon carbide-based catalyst body which enables a catalyst, e.g. a NO x occlusion catalyst to retain its activity for a long time. SOLUTION: This silicon carbide-based catalyst body comprises a porous body with a specific shape and a catalyst carried thereby. The porous body is composed of a first bonded texture formed by bonding a large number of silicon carbide particles, as aggregates, to each other in such a state as to retain many pores, and carrys a catalyst containing an alkali metal and/or an alkaline earth metal. The catalyst is characterized in that it is carried via a crystalline oxide film formed so as to at least partially cover the surface of the silicon carbide particles constituting the first bonded texture. COPYRIGHT: (C)2004,JPO

4. 发明专利

JP2010260762A Method for producing metal compound oxide 审中-公开
标题翻译：生产金属化合物氧化物的方法
公开(公告)号：JP2010260762A
公开(公告)日：2010-11-18
申请号：JP2009112249
申请日：2009-05-01
申请人： Ngk Insulators Ltd , 日本碍子株式会社
发明人： NANBA MASAHARU , YAMADA NAOHITO , FURUKAWA MASAHIRO
IPC分类号： C01G51/00 , C01B13/32 , C01G49/00
摘要： PROBLEM TO BE SOLVED: To provide a method for producing a metal compound oxide, with which the metal compound oxide with a desired structure is obtained more efficiently at a lower temperature, while more retaining the atomic arrangement of a precursor, by making the same into ceramic.
SOLUTION: The method for producing the metal compound oxide comprises a firing stage where the precursor in which the atomic arrangement of two or more kinds of metallic atoms lies in the prescribed one is used, the precursor is fired under the conditions where the segregation of the metallic elements is suppressed, or the precursor is fired under the conditions where the temperature rising rate in a prescribed temperature range reaches the prescribed temperature rising rate or below. When, e.g. a metal compound oxide having a perovskite structure expressed by general formula ABO
3 is produced, when a precursor 30 is heated by the production method, the intermediate body 40 of the precursor and a calcined matter is produced, and further, when heating is continued, a calcined matter 50 is produced, and finally, while retaining the atomic arrangement of the components entering the A, B sites, the metal compound oxide 20 can be obtained at a lower temperature.
COPYRIGHT: (C)2011,JPO&INPIT
摘要翻译：要解决的问题：提供一种制备金属复合氧化物的方法，通过该方法可以在较低温度下更有效地获得具有所需结构的金属复合氧化物，同时通过制备前体的原子排列更多地保持陶瓷也一样。解决方案：制备金属复合氧化物的方法包括使用其中两种或更多种金属原子的原子排列位于规定的前体的前体的烧制阶段，前体在抑制金属元素的偏析，或者在规定温度范围内的升温速度达到规定的升温速度以下的条件下烧成前体。何时，例如当通过制备方法加热前体30时，产生具有由通式ABO 3 表示的钙钛矿结构的金属复合氧化物，制备前体的中间体40和煅烧物，此外，当继续加热时，产生煅烧物质50，最后，在保持进入A，B位点的成分的原子排列的同时，可以在较低的温度下获得金属复合氧化物20。版权所有（C）2011，JPO＆INPIT

5. 发明专利

JP2009227540A Method for producing ceramic precursor, ceramic precursor, method for producing ceramic, and ceramic 审中-公开
标题翻译：用于生产陶瓷前体的方法，陶瓷前体，用于生产陶瓷的方法和陶瓷
公开(公告)号：JP2009227540A
公开(公告)日：2009-10-08
申请号：JP2008077646
申请日：2008-03-25
申请人： Ngk Insulators Ltd , 日本碍子株式会社
发明人： YAMADA NAOHITO , FURUKAWA MASAHIRO , NANBA MASAHARU
IPC分类号： C04B35/48 , C01C3/11 , C01C3/14 , C01C3/20 , C01G25/00 , C04B35/626
摘要： PROBLEM TO BE SOLVED: To more satisfactorily disperse the additional component of a ceramic precursor into the main component. SOLUTION: The atom-configurated ceramic can be obtained by coordinating a ligand 21 having an easily coordinatable part 22 which can be coordinated into an a component as the main component and a b component as an additional component and a hardly coordinatable part 23 in which the coupling with the a component and the b component is suppressed into the a component and the b component, so as to produce an a complex ligand 24 and a b complex ligand 25, adding an ion or a complex comprising a c component which can be coupled with two or more hardly coordinatable parts 23 (a c component 26) to a solution comprising the a complex ligand 24 and the b complex ligand 25, so as to produce a precursor 28 and firing the produced precursor 28 under mild conditions. Upon the production of the precursor 28, in the b complex ligands 25, mutual coupling is suppressed by the hardly coordinatable parts 23, and the c component lies therebetween, thus the phenomenon that the b components as an additional component are made adjacent does not occur, and the adjoining presence of the b components can be sufficiently suppressed. COPYRIGHT: (C)2010,JPO&INPIT
摘要翻译：要解决的问题：为了使陶瓷前体的附加成分更均匀地分散到主要成分中。解决方案：原子构型陶瓷可以通过配位具有易配位的部分22的配位体21，其可以配位成作为主要成分的组分和作为附加组分的ab组分和难以配位的部分23 其与a组分和b组分的偶联被抑制到组分和b组分中，以便产生复合配体24和ab络合配体25，加入离子或包含交联组分的络合物，其可以偶联具有两个或多个难以配位的部分23（交流部件26）至包含络合配体24和b络合配体25的溶液，以便产生前体28并在温和条件下烧制所制备的前体28。在制备前体28时，在b络合配体25中，互不耦合部分被几乎不配合的部分23抑制，并且c部件位于它们之间，因此不会发生作为附加部件的b成分相邻的现象并且能够充分地抑制b成分的相邻存在。版权所有（C）2010，JPO＆INPIT

6. 发明专利

JP2009154129A Gas adsorbent and its using method 审中-公开
标题翻译：气体吸附及其使用方法
公开(公告)号：JP2009154129A
公开(公告)日：2009-07-16
申请号：JP2007337722
申请日：2007-12-27
申请人： Ngk Insulators Ltd , 日本碍子株式会社
发明人： FURUKAWA MASAHIRO , GOTO MASASHI
IPC分类号： B01J20/22 , C07C63/08 , C07F3/06
摘要： PROBLEM TO BE SOLVED: To enhance the gas adsorbing rate of a gas adsorbent constituted of an integrated body formed by integrating a plurality of structure bodies.
SOLUTION: The gas adsorbent 10 is constituted of the integrated body formed by integrating a plurality of monomers 20. The monomers 20 are provided with a plurality of complex nucleus metals 22 and a plurality of mono-carbonic acids 24 which possess an interaction part 25 integrated with other monomers 20 by non-bonding interaction (for example, π-π stacking) and which are coordinated to the complex nucleus metals 22 by surrounding the complex nucleus metals 22. The gas adsorbent 10 are formed in an average diameter of 10 μm or smaller and the plurality of monomers 20 move to form a space between the plurality of monomers 20 by the interaction part 25 so that adsorption gases are adsorbed. It is desirable to make the gas adsorbents 10 start adsorption of gases at 87K and complete the adsorption by lowering the temperature finally to 77k or lower.
COPYRIGHT: (C)2009,JPO&INPIT
摘要翻译：要解决的问题：提高由通过整合多个结构体而形成的一体体构成的气体吸附剂的气体吸附速率。气体吸附剂10由通过整合多个单体20而形成的一体体构成。单体20设置有多个复合核金属22和多个具有相互作用的多元碳酸24 部分25通过非结合相互作用（例如π-π堆叠）与其它单体20集成，并且通过围绕复核原子金属22而与复合核金属22配位。气体吸附剂10形成为平均直径多个单体20通过相互作用部分25移动以在多个单体20之间形成空间，从而吸附吸附气体。期望使气体吸附剂10开始吸附87K的气体，并通过将温度降至77k以下来完成吸附。版权所有（C）2009，JPO＆INPIT

7. 发明专利

JP2013219017A Method for restoring ion conductivity of solid electrolyte ceramic material 有权
标题翻译：恢复固体电解陶瓷材料离子电导率的方法
公开(公告)号：JP2013219017A
公开(公告)日：2013-10-24
申请号：JP2013029894
申请日：2013-02-19
申请人： Ngk Insulators Ltd , 日本碍子株式会社
发明人： FURUKAWA MASAHIRO , HONDA AKIHIKO , YAMAMOTO KAZUHIRO
IPC分类号： H01M10/0562 , H01M10/052
CPC分类号： Y02E60/122 , Y02T10/7011
摘要： PROBLEM TO BE SOLVED: To restore, in a solid electrolyte ceramic material having a lithium ion conductivity which consists of oxide synthetic powder or an oxide sintered compact having a garnet type or garnet-like type crystal structure constituted by at least Li, La, Zr and O, the ion conductivity having lowered to under that immediately after synthesis or sintering.SOLUTION: A method comprises: performing a thermal treatment in a temperature region of no lower than 650°C on a ceramic material with its ion conductivity having lowered to under that immediately after the synthesis of oxide synthetic powder or the sintering of an oxide sintered compact under at least one kind of atmosphere selected from an inert gas atmosphere, an oxygen atmosphere and a decompression atmosphere.
摘要翻译：要解决的问题：为了恢复由氧化物合成粉末或具有由至少Li，La，Zr构成的石榴石型或石榴石型晶体结构的氧化物烧结体构成的具有锂离子传导性的固体电解质陶瓷材料和O，离子电导率降低到合成或烧结后的离子电导率。解决方案：一种方法包括：在陶瓷材料上在不低于650℃的温度范围内进行热处理，其离子传导性降低到低于即在合成氧化物合成粉末之后立即进行或在选自惰性气体气氛，氧气氛和减压气氛中的至少一种气氛下烧结氧化物烧结体。

8. 发明专利

JP2012214364A HONEYCOMB STRUCTURE, Si-SiC BASED COMPOSITE MATERIAL, METHOD FOR MANUFACTURING HONEYCOMB STRUCTURE, AND METHOD FOR MANUFACTURING Si-SiC BASED COMPOSITE MATERIAL 审中-公开
标题翻译：蜂窝结构，Si-SiC基复合材料，制造蜂窝结构的方法和制造Si-SiC基复合材料的方法
公开(公告)号：JP2012214364A
公开(公告)日：2012-11-08
申请号：JP2012053090
申请日：2012-03-09
申请人： Ngk Insulators Ltd , 日本碍子株式会社
发明人： FURUKAWA MASAHIRO , SHINSHI MARIKO , MATSUDA KAZUYUKI
IPC分类号： C04B41/85 , B01J35/04 , B01J37/02 , B01J37/08 , C04B35/565 , C04B38/00 , C04B41/88
CPC分类号： C04B35/565 , B01D46/0001 , B01D46/2425 , B01D46/2429 , B01D46/2448 , B01J35/04 , C04B35/573 , C04B35/6316 , C04B41/009 , C04B41/5096 , C04B41/85 , C04B2111/0081 , C04B2235/3208 , C04B2235/3826 , C04B2235/402 , C04B2235/428 , C04B2235/442 , C04B2235/5436 , C04B2235/5445 , C04B2235/80 , C04B2235/96 , C04B41/4539 , C04B41/4572 , C04B41/5155 , C04B2103/001 , C04B38/0006
摘要： PROBLEM TO BE SOLVED: To more easily form electrode portions and further to reduce volume resistivity.SOLUTION: A honeycomb structure 20 includes a partition portion 22 constituting a plurality of cells 23 serving as flow paths of a fluid. This honeycomb structure 20 further includes: electrode portions 32 which are disposed as parts of the partition portion 22 and which have an SiC phase, an oxide phase containing an Si oxide, an Al oxide, and an alkaline-earth metal oxide, and a metal phase containing metal Si and metal Al, where the proportion of metal Al relative to the total amount of metal Si and metal Al is 0.001-20 mol%; and a heat generation portion 34 which is a part of the partition portion 22 and which has a volume resistivity higher than that of the electrode portion 32. This honeycomb structure is obtained by forming an impregnation base material containing metal Si and metal Al and an alkaline-earth metal compound on a part of the surface of a honeycomb base material having an SiC phase and an oxide phase containing an Si oxide and impregnating metal Si and metal Al into pores of the honeycomb base material through heating in an inert atmosphere.
摘要翻译：要解决的问题：为了更容易地形成电极部分并进一步减小体积电阻率。解决方案：蜂窝结构体20包括构成作为流体的流路的多个单元23的分隔部22。该蜂窝结构体20还具备：分隔部22的一部分配置有SiC相，含有氧化硅，氧化铝，碱土类金属氧化物的氧化物相和金属氧化物的电极部32，相中金属Si和金属Al的总量相对于金属Si和金属Al的比例为0.001-20摩尔％; 以及作为分隔部22的一部分并且具有比电极部32的体积电阻率高的体积电阻率的发热部34.该蜂窝结构体通过形成含有金属Si和金属Al的浸渍基材和碱 - 在通过在惰性气氛中加热的情况下，在具有SiC相和含有氧化硅的氧化物相的蜂窝状基材的表面的一部分上，将金属Si浸渍到蜂窝状基材的孔中。版权所有（C）2013，JPO＆INPIT

9. 发明专利

JP2010082544A Gas adsorbent 审中-公开
标题翻译：气体吸收
公开(公告)号：JP2010082544A
公开(公告)日：2010-04-15
申请号：JP2008254290
申请日：2008-09-30
申请人： Ngk Insulators Ltd , 日本碍子株式会社
发明人： GOTO MASASHI , FURUKAWA MASAHIRO
IPC分类号： B01J20/22 , C01B3/00 , C07C51/41 , C07C63/06 , C07F1/08 , C07F3/06
CPC分类号： Y02E60/327
摘要： PROBLEM TO BE SOLVED: To provide a novel gas adsorbent having enhanced structural stability and capable of adsorbing hydrogen in a greater amount.
SOLUTION: The gas adsorbent is structured by including a first material constituted of integrated bodies of a plurality of structures each including a plurality of nucleic metal atoms (Zn) of a complex and a plurality of monocarboxylic acids (benzoic acid) each of which monocarboxylic acids includes an interactive member (a benzene ring) capable of combining with another structure by virtue of nonbinding interaction, and coordinates to the plurality of the nucleic metal atoms (Zn) in a manner surrounding the same, and a second material including noble metal (Pt) as catalytic metal supported by an inorganic support (carbon). The ratio of the first material to the second material is 90:10 by weight. The gas adsorbent exhibits a greater volume of adsorbed hydrogen gas relative to a calculated value theoretically calculated from the volume of hydrogen gas to be adsorbed by each of the first material and the second material, which clearly indicates the presence of a synergetic effect of the first and the second materials.
COPYRIGHT: (C)2010,JPO&INPIT
摘要翻译：要解决的问题：提供具有增强的结构稳定性并能够更大量吸附氢的新型气体吸附剂。解决方案：气体吸附剂通过包括由多个结构的整体组成的第一材料构成，每个结构包括复合物的多个核酸金属原子（Zn）和多个单羧酸（苯甲酸）所述单羧酸包括能够通过非结合相互作用与其它结构结合的相互作用的成员（苯环），并以包围其的方式与所述多个核酸原子（Zn）配位，以及包含贵金属的第二材料金属（Pt）作为由无机载体（碳）负载的催化金属。第一材料与第二材料的重量比为90:10。气体吸附剂相对于由第一材料和第二材料中的每一种吸附的氢气的体积理论上计算出的计算值，显示出较大的吸附氢气体积，这清楚地表明存在第一和第二材料的协同作用和第二种材料。版权所有（C）2010，JPO＆INPIT

10. 发明专利

JP2009189993A Gas adsorbing material and method for producing neon 审中-公开
标题翻译：气体吸附材料和生产方法
公开(公告)号：JP2009189993A
公开(公告)日：2009-08-27
申请号：JP2008035495
申请日：2008-02-18
申请人： Ngk Insulators Ltd , 日本碍子株式会社
发明人： GOTO MASASHI , FURUKAWA MASAHIRO
IPC分类号： B01J20/22 , B01D53/02 , B01D53/04 , C01B23/00 , C07C63/08 , C07F3/06
摘要： PROBLEM TO BE SOLVED: To efficiently produce neon by enhancing adsorption property of neon. SOLUTION: A gas adsorbing material 10 is composed of an aggregate in which a plurality of monomers 20 are aggregated, wherein each of the monomers 20 includes: four complex-core metals 22 (for example, Zn) bonded tetragonally through oxygen; and a plurality of monocarboxylic acids 24 each of which has an interaction part 25 (for example, a benzene ring) for aggregating with another structure by the nonbonding interaction and which are coordinated with the complex-core metal to surround the complex-core metal. When a gas to be adsorbed (neon gas) exists, the gas adsorbing material 10 induces the phase transition to such a structure that an opening having the size larger than the molecular size of the gas to be adsorbed is formed to take therein the gas to be adsorbed. When the pressure of the gas to be adsorbed becomes higher, the gas adsorbing material induces the phase transition to a bigger structure to take therein plenty of the gas to be adsorbed. It is considered that the gas adsorbing material 10 induces reversible phase transition and adsorbs/desorbs neon gas of the adsorbed/desorbed amount higher than that of helium, nitrogen, oxygen, etc. COPYRIGHT: (C)2009,JPO&INPIT
摘要翻译：要解决的问题：通过增强氖的吸附性能来有效地生产氖。气体吸附材料10由多个单体20聚集的聚集体组成，其中每个单体20包括四个通过氧四方键合的复合核心金属22（例如Zn）; 和多个一元羧酸24，每个单羧酸24具有相互作用部分25（例如苯环），用于通过非键合相互作用与另一结构聚合并与复核芯金属配合以包围复合芯金属。当存在待吸附气体（氖气）时，气体吸附材料10引起相变，使得形成具有大于待吸附气体的分子尺寸的孔的开口，从而将气体吸入被吸附。当吸附气体的压力变高时，气体吸附材料会引起相变到较大的结构，从而吸收大量的待吸附气体。认为气体吸附材料10引起可逆相变和吸附/解吸附氦气的吸附/脱附量高于氦，氮，氧等。◎答案：（C）2009，JPO＆INPIT

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