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1. 发明申请

US20060172884A1 Supported, titanized chromium catalyst and its use for preparing homopolymers and copolymers of ethylene 有权
标题翻译：负载型，钛酸化铬催化剂及其制备乙烯均聚物和共聚物的用途
公开(公告)号：US20060172884A1
公开(公告)日：2006-08-03
申请号：US11330071
申请日：2006-01-12
申请人： Martin Schneider , Rainer Karer , Dieter Lilge , Volker Rauschenberger , Philipp Rosendorfer , Joachim Wulff-Doring , Gunther Schweier , Martin Lux , Peter Bauer
发明人： Martin Schneider , Rainer Karer , Dieter Lilge , Volker Rauschenberger , Philipp Rosendorfer , Joachim Wulff-Doring , Gunther Schweier , Martin Lux , Peter Bauer
IPC分类号： C08F4/02
CPC分类号： C08F210/16 , C08F2410/04 , C08F4/24 , C08F4/69 , C08F4/025 , C08F210/14 , C08F2500/12 , C08F2500/17 , C08F2500/04 , C08F2500/26
摘要： Novel supported, titanized chromium catalysts for the homopolymerization of ethylene and the copolymerization of ethylene with α-olefins, a process for preparing them and to their use for the polymerization of olefins.
摘要翻译：用于乙烯均聚和乙烯与α-烯烃的共聚合的新型负载的钛化铬催化剂，其制备方法及其用于烯烃聚合的方法。

2. 发明申请

US20080177013A1 SUPPORTED, TITANIZED CHROMIUM CATALYST AND ITS USE FOR PREPARING HOMOPOLYMERS AND COPOLYMERS OF ETHYLENE 审中-公开
标题翻译：支持的钛酸钡催化剂及其用于制备乙烯的共聚物和共聚物的用途
公开(公告)号：US20080177013A1
公开(公告)日：2008-07-24
申请号：US11972488
申请日：2008-01-10
申请人： Martin SCHNEIDER , Rainer Karer , Dieter Lilge , Volker Rauschenberger , Philipp Rosendorfer , Joachim Wulff-Doring , Gunther Schweier , Martin Lux , Peter Bauer
发明人： Martin SCHNEIDER , Rainer Karer , Dieter Lilge , Volker Rauschenberger , Philipp Rosendorfer , Joachim Wulff-Doring , Gunther Schweier , Martin Lux , Peter Bauer
IPC分类号： C08F4/22
CPC分类号： C08F210/16 , C08F2410/04 , C08F4/24 , C08F4/69 , C08F4/025 , C08F210/14 , C08F2500/12 , C08F2500/17 , C08F2500/04 , C08F2500/26
摘要： Novel supported, titanized chromium catalysts for the homopolymerization of ethylene and the copolymerization of ethylene with α-olefins, a process for preparing them and to their use for the polymerization of olefins.
摘要翻译：用于乙烯均聚和乙烯与α-烯烃的共聚合的新型负载的钛化铬催化剂，其制备方法及其用于烯烃聚合的方法。

3. 发明授权

US07348384B2 Supported, titanized chromium catalyst and its use for preparing homopolymers and copolymers of ethylene 有权
标题翻译：负载型，钛酸化铬催化剂及其制备乙烯均聚物和共聚物的用途
公开(公告)号：US07348384B2
公开(公告)日：2008-03-25
申请号：US11330071
申请日：2006-01-12
申请人： Martin Schneider , Rainer Karer , Dieter Lilge , Volker Rauschenberger , Philipp Rosendorfer , Joachim Wulff-Döring , Günther Schweier , Martin Lux , Peter Bauer
发明人： Martin Schneider , Rainer Karer , Dieter Lilge , Volker Rauschenberger , Philipp Rosendorfer , Joachim Wulff-Döring , Günther Schweier , Martin Lux , Peter Bauer
IPC分类号： C08F10/02 , C08F4/24 , C08F4/18
CPC分类号： C08F210/16 , C08F2410/04 , C08F4/24 , C08F4/69 , C08F4/025 , C08F210/14 , C08F2500/12 , C08F2500/17 , C08F2500/04 , C08F2500/26
摘要： Novel supported, titanized chromium catalysts for the homopolymerization of ethylene and the copolymerization of ethylene with α-olefins, a process for preparing them and to their use for the polymerization of olefins.
摘要翻译：用于乙烯均聚和乙烯与α-烯烃的共聚合的新型负载的钛化铬催化剂，其制备方法及其用于烯烃聚合的方法。

4. 发明授权

US07019089B2 Suspended chrome catalyst containing titanium and the use thereof for producing ethylene homopolymers and copolymers 有权
标题翻译：含有钛的悬浮铬催化剂及其用于生产乙烯均聚物和共聚物的用途
公开(公告)号：US07019089B2
公开(公告)日：2006-03-28
申请号：US10332045
申请日：2001-06-28
申请人： Martin Schneider , Rainer Karer , Dieter Lilge , Volker Rauschenberger , Philipp Rosendorfer , Joachim Wulff-Döring , Günther Schweier , Martin Lux , Peter Bauer
发明人： Martin Schneider , Rainer Karer , Dieter Lilge , Volker Rauschenberger , Philipp Rosendorfer , Joachim Wulff-Döring , Günther Schweier , Martin Lux , Peter Bauer
IPC分类号： C08F10/02 , C08F4/24 , C08F4/18
CPC分类号： C08F210/16 , C08F2410/04 , C08F4/24 , C08F4/69 , C08F4/025 , C08F210/14 , C08F2500/12 , C08F2500/17 , C08F2500/04 , C08F2500/26
摘要： Novel supported, titanized chromium catalysts can be used for the homopolymerization of ethylene and the copolymerization of ethylene with α-olefins.
摘要翻译：新型负载的钛化铬催化剂可用于乙烯的均聚和乙烯与α-烯烃的共聚合。

5. 发明授权

US06649709B1 Gas phase fluidized bed method and ethylene homo- and copolymers obtained using said method 有权
标题翻译：气相流化床法和使用所述方法获得的乙烯均聚物和共聚物
公开(公告)号：US06649709B1
公开(公告)日：2003-11-18
申请号：US09555594
申请日：2000-05-31
申请人： Peter Bauer , Armin Lange , Rainer Karer , Philipp Rosendorfer , Manfred Hecker , Günther Schweier , Wolfgang Micklitz , Kaspar Evertz , Hans-Jacob Feindt
发明人： Peter Bauer , Armin Lange , Rainer Karer , Philipp Rosendorfer , Manfred Hecker , Günther Schweier , Wolfgang Micklitz , Kaspar Evertz , Hans-Jacob Feindt
IPC分类号： C08F234
CPC分类号： C08F10/02 , C08F4/24 , C08F2/34
摘要： A continuous vapor-phase fluidized-bed process for the preparation of ethylene homopolymers and copolymers having a density of from 0.87 to 0.97 g/cm3 in which ethylene or mixtures of ethylene and C3-C8 a-monoolefins are (co)polymerized in the presence of a supported chromium catalyst in the polymerization zone of a vapor-phase fluidized-bed reactor under pressures ranging from 1 to 100 bar and at temperatures ranging from 30° to 125° C. in the vapor phase in an agitated bed of bulk material comprising particulate polymer, the resultant heat of polymerization is removed by cooling the recirculated reactor gas and the resulting (co)polymer is removed from the vapor-phase fluidized-bed reactor, wherein, for the preparation of a (co)polymer of a specific density d, the (co)polymerization is carried out at a temperature which is in a range restricted by an upper envelope defined by equation I T H = 171 + 6 ⁢ d ′ 0.84 - d ′ ( I ) and a lower envelope defined by equation II T L = 173 + 7.3 ⁢ d ′ 0.837 - d ′ , ( II ) in which the variables have the following meanings: TH is the highest reaction temperature in ° C.; TL is the lowest reaction temperature in ° C.; d′ is the numerical value of the density d of the (co)polymer to be synthesized.
摘要翻译：用于制备密度为0.87至0.97g / cm 3的乙烯均聚物和共聚物的连续气相流化床方法，其中乙烯或乙烯和C 3 -C 8α-单烯烃的混合物（共）聚合在负载的铬催化剂的存在下，在气相流化床反应器的聚合区域的存在下，在压力范围为1至100巴，温度范围为30至125℃，气相在搅拌床包含颗粒聚合物的散装材料，通过冷却再循环的反应器气体除去所得到的聚合热，并将所得（共）聚合物从气相流化床反应器中除去，其中，为制备（共）聚合物特定密度d，（共）聚合在由等式I定义的上包络限制的范围内进行，并且由等式IIin定义的下包络，其中变量具有以下含义：T H是最高的反应温度，单位°C; TL是最低反应温度（℃）; d'是待合成的（共）聚合物的密度d的数值。

6. 发明授权

US06849699B2 Vapor-phase fluidized-bed process and ethylene homopolymers and copolymers produced thereby 失效
标题翻译：气相流化床方法和由此制备的乙烯均聚物和共聚物
公开(公告)号：US06849699B2
公开(公告)日：2005-02-01
申请号：US10658916
申请日：2003-09-11
申请人： Peter Bauer , Armin Lange , Rainer Karer , Philipp Rosendorfer , Manfred Hecker , Günther Schweier , Wolfgang Micklitz , Kaspar Evertz , Hans-Jacob Feindt
发明人： Peter Bauer , Armin Lange , Rainer Karer , Philipp Rosendorfer , Manfred Hecker , Günther Schweier , Wolfgang Micklitz , Kaspar Evertz , Hans-Jacob Feindt
IPC分类号： C08J5/18 , C08F2/34 , C08F4/02 , C08F4/24 , C08F4/69 , C08F10/02 , C08F210/02
CPC分类号： C08F10/02 , C08F4/24 , C08F2/34
摘要： A continuous vapor-phase fluidized-bed process for the preparation of ethylene homopolymers and copolymers having a density of from 0.87 to 0.97 g/cm3 in which ethylene or mixtures of ethylene and C3-C8 a-monoolefins are (co)polymerized in the presence of a supported chromium catalyst in the polymerization zone of a vapor-phase fluidized-bed reactor under pressures ranging from 1 to 100 bar and at temperatures ranging from 30° to 125° C. in the vapor phase in an agitated bed of bulk material comprising particulate polymer, the resultant heat of polymerization is removed by cooling the recirculated reactor gas and the resulting (co)polymer is removed from the vapor-phase fluidized-bed reactor, wherein, for the preparation of a (co)polymer of a specific density d, the (co)polymerization is carried out at a temperature which is in a range restricted by an upper envelope defined by equation I T H = 171 + 6 ⁢ ⁢ d ′ 0.84 - d ′ ( I ) and a lower envelope defined by equation II T L = 173 + 7.3 ⁢ ⁢ d ′ 0.837 - d ′ , ( II ) in which the variables have the following meanings: TH is the highest reaction temperature in ° C.; TL is the lowest reaction temperature in ° C.; d′ is the numerical value of the density d of the (co)polymer to be synthesized.
摘要翻译：用于制备密度为0.87至0.97g / cm 3的乙烯均聚物和共聚物的连续气相流化床方法，其中乙烯或乙烯和C 3 -C 8α-单烯烃的混合物（共）聚合在负载的铬催化剂的存在下，在气相流化床反应器的聚合区域的存在下，在压力范围为1至100巴，温度范围为30至125℃，气相在搅拌床包含颗粒聚合物的散装材料，通过冷却再循环的反应器气体除去所得到的聚合热，并将所得（共）聚合物从气相流化床反应器中除去，其中，为制备（共）聚合物特定密度d，（共）聚合在由等式I定义的上包络限制的范围内进行，并且由等式IIin定义的下包络，其中变量具有以下含义：T H是最高的反应温度，单位°C; TL是最低反应温度（℃）; d'是待合成的（共）聚合物的密度d的数值。

7. 发明授权

US06180729B2 Continuous gas-phase polymerization process 有权
标题翻译：连续气相聚合法
公开(公告)号：US06180729B2
公开(公告)日：2001-01-30
申请号：US09201084
申请日：1998-11-30
申请人： Armin Lange , Wolfgang Micklitz , Rainer Karer , Kaspar Evertz , Shahram Mihan , Hans-Jacob Feindt , Manfred Hecker , Peter Bauer , Philipp Rosendorfer
发明人： Armin Lange , Wolfgang Micklitz , Rainer Karer , Kaspar Evertz , Shahram Mihan , Hans-Jacob Feindt , Manfred Hecker , Peter Bauer , Philipp Rosendorfer
IPC分类号： C08F240
CPC分类号： C08F10/00 , C08F2/005 , C08F210/16 , Y02P20/584 , C08F2/34 , C08F2/40 , C08F2/007 , C08F2/002 , C08F210/14 , C08F2500/12 , C08F2500/18
摘要： In a continuous gas-phase polymerization process for preparing ethylene and propene homopolymers and copolymers, in which ethylene, propene or a mixture of ethylene or propene and C3-C8-&agr;-monoolefins is polymerized in the polymerization zone of a gas-phase polymerization reactor at from 30 to 125° C. and a pressure of from 1 to 100 bar in the gas phase in a bed of finely divided polymer in the presence of a catalyst, where the reactor gas is circulated to remove the heat of polymerization, polymer deposits in the circulating gas line are prevented by metering a catalyst poison having a boiling point above the maximum temperature within the circulating gas line into this circulating gas line in at most such an amount that it does not significantly impair the productivity of the catalyst in the reactor.
摘要翻译：在用于制备乙烯和丙烯均聚物和共聚物的连续气相聚合方法中，其中乙烯，丙烯或乙烯或丙烯和C 3 -C 8-α-单烯烃的混合物在气相聚合反应器的聚合区中聚合在催化剂存在下，在细分散的聚合物床中的气相中，在30至125℃和1至100巴的压力下，其中反应器气体循环以除去聚合热，聚合物沉积物通过将沸点高于循环气体管线中的最高温度的催化剂毒物计量到该循环气体管线中，至多使其不显着损害反应器中催化剂的生产率的程度来防止循环气体管线。

8. 发明授权

US06297323B1 Polymer mixture 失效
标题翻译：聚合物混合物
公开(公告)号：US06297323B1
公开(公告)日：2001-10-02
申请号：US09424909
申请日：1999-12-01
申请人： Peter Bauer , Martin Lux , Dieter Lilge
发明人： Peter Bauer , Martin Lux , Dieter Lilge
IPC分类号： C08L2316
CPC分类号： C08L23/0815 , C08L23/06 , C08L2205/02 , C08L2666/04
摘要： Polymer blends contain at least 85% by weight of ethylene/&agr;-olefin copolymers (A) prepared by metallocene catalysis and from 1 to 15% by weight of essentially linear ethylene/&agr;-olefin copolymers (B) prepared using another catalyst, the percentages in each case being based on the total weight of the polymer blend.
摘要翻译：聚合物共混物包含至少85重量％的通过茂金属催化制备的乙烯/α-烯烃共聚物（A）和1至15重量％的使用另一种催化剂制备的基本上线性的乙烯/α-烯烃共聚物（B），百分比在每种情况下都是基于聚合物共混物的总重量。

9. 发明授权

US06180731B2 Polymerisates of ethylene with a high degree of resistance to stress crack, and a catalyst system for the production thereof 失效
标题翻译：具有高抗应力裂纹性的乙烯的聚合物，以及用于制备它的催化剂体系
公开(公告)号：US06180731B2
公开(公告)日：2001-01-30
申请号：US09000011
申请日：1997-01-22
申请人： Wolfgang Rohde , Roland Saive , Dieter Lilge , Martin Lux , Peter Bauer
发明人： Wolfgang Rohde , Roland Saive , Dieter Lilge , Martin Lux , Peter Bauer
IPC分类号： C08F442
CPC分类号： C08F10/00 , C08F4/61904 , C08F4/61912 , C08F4/61925 , C08F210/16 , Y10S526/943 , C08F210/14 , C08F2500/13 , C08F2500/12 , C08F2500/07 , C08F2500/26 , C08F4/63904 , C08F4/69
摘要： Polymers of ethylene are obtainable by polymerization of ethylene and, if desired, further comonomers in the presence of a catalyst system comprising as active constituents I) a Phillips catalyst, II) a solid which is different from I) and comprises a component which is derived from the metallocene complexes of the formula (A) in which the substituents and indices have the following meanings: R1 to R10 are hydrogen, C1-C10-alkyl, 5-to 7-membered cycloalkyl which may in turn bear C1-C6-alkyl groups as substituents, C6-C15-aryl or aryalkyl, where two adjacent radicals may also together form a cyclic group having from 4 to 15 carbon atoms, or Si(R11)3, where R11 is C1-C10-alkyl, C6-C15-aryl or C3-C10-cycloalkyl, or the radicals R4 and R9 together form a group —[Y(R12R13)]m—, where Y is silicon, germanium, tin or carbon, and R12, R13 are hydrogen C1-C10-alky, C3-C10-cycloalyl or C6-C15-aryl, M is a metal of transition groups IV to VIII or a metal of the lanthanide series, Z1, Z2 are fluorine, chlorine, bromine, iodine, hydrogen, C1-C20-alkyl or aryl, —OR14, —OOCR14, where R14 is hydrogen or C1-C20-alkyl; R15 is C1-C20-alkyl; m is 1,2,3 or 4; n is 0, or 2; r is 0, 1 or 2; the sum n+r is likewise 0, 1 or 2, and, if desired, III) an organometallic component selected from groups IA, IIA, IIB and IIIA of the Periodic Table of the Elements.
摘要翻译：乙烯的聚合物可以通过在包含作为活性成分的催化剂体系的存在下乙烯和如果需要的情况下进一步的共聚单体获得。I）菲利普斯催化剂，II）与I）不同的固体，并且包含衍生自式（A）的金属茂络合物，其中取代基和指数具有以下含义：R 1至R 10是氢，C 1 -C 10 - 烷基，5-至7-元环烷基，其也可以含有C 1 -C 6 - 烷基作为取代基，其中两个相邻基团也可以一起形成具有4至15个碳原子的环状基团的C 6 -C 15 - 芳基或芳烷基，或其中R 11是C 1 -C 10 - 烷基，C 6 -C 15 - 芳基或C 3 -C 10 - 环烷基，或基团R 4和R 9一起形成 - [Y（R 12 R 13）] m - 基团，其中Y是硅，锗，锡或碳，R 12，R 13是氢C1-C10-烷基 C 3 -C 10 - 环烷基或C 6 -C 15 - 芳基，M为Ⅳ〜Ⅷ族金属或镧系金属，Z 1，Z 2为氟，氯，溴，碘，氢，C 1 -C 20烷基或芳基，-OR 14，-OOCR 14，其中R 14是氢或C 1 -C 20烷基; R 15是C 1 -C 20 - 烷基; m为1,2,3或4; n为0或2; r为0,1或2; 总和n + r同样为0,1或2，如果需要，III）选自元素周期表的IA，IIA，IIB和IIIA族的有机金属组分。

10. 发明授权

US06350814B1 Polymer mixture with good workability 有权
标题翻译：聚合物混合物具有良好的加工性能
公开(公告)号：US06350814B1
公开(公告)日：2002-02-26
申请号：US09529188
申请日：2000-04-10
申请人： Peter Bauer , Martin Lux , Dieter Lilge , Uwe Faller
发明人： Peter Bauer , Martin Lux , Dieter Lilge , Uwe Faller
IPC分类号： C08F800
CPC分类号： C08J9/18 , C08J2323/16 , C08L23/0815 , C08L2205/02 , C08L2314/06 , C08L2666/04
摘要： A polymer mixture comprises at least 40 but less than 85% by weight of an ethylene copolymer (A) which has a density of from 0.91 to 0.93 g/cm3, an HLMFR (190° C./21.6 kg) of from 5 to 60 g/10 min and a molar mass distribution Mw/Mn≦3, and more than 15 but at most 60% by weight of an ethylene copolymer (B) which has a density of from 0.93 to 0.945 g/cm3, an HLMFR (190° C./21.6 kg) of from 8 to 20 g/10 min and a molar mass distribution Mw/Mn≧7, where the percentages by weight are in each case based on the total mass of the components (A) and (B).
摘要翻译：聚合物混合物包含密度为0.91至0.93g / cm 3的乙烯共聚物（A）的至少40重量％至85重量％，HLMFR（190℃/ 21.6kg）为5至60 g / 10分钟，摩尔质量分布Mw /Mn≤3，以及大于15但至多60重量％的密度为0.93至0.945g / cm3的乙烯共聚物（B），HLMFR（ 190℃/ 21.6kg）为8至20g / 10min，摩尔质量分布Mw / Mn> = 7，其中每种情况下的重量百分数都是基于组分（A）和（B）。

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