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1. 发明申请

WO2018133967A1 SYSTEM AND METHOD FOR CHEMICAL LOOPING 审中-公开
公开(公告)号：WO2018133967A1
公开(公告)日：2018-07-26
申请号：PCT/EP2017/078879
申请日：2017-11-10
申请人： GENERAL ELECTRIC TECHNOLOGY GMBH
发明人： VITSE, Frederic
IPC分类号： C10J3/72
CPC分类号： C10J3/725 , C01B3/02 , C01B3/344 , C01B2203/0255 , C01B2203/0425 , C01B2203/0485 , C01B2203/1241 , C01B2203/84 , C10J2300/093 , C10J2300/0983 , C10J2300/0996 , C10J2300/1807 , Y02P30/30
摘要： A method for chemical looping includes the steps of introducing a fuel and an oxygen carrier to a reducer, wherein in the reducer the fuel reacts with the oxygen carrier to produce a gas containing a sulfur-containing species, within the reducer, capturing the sulfur-containing species with the oxygen carrier, transporting the oxygen carrier with the sulfur-containing species to an oxidizer, within the oxidizer, releasing the sulfur-containing species via an oxidation reaction, within the oxidizer, recapturing the sulfur-containing species with the oxygen carrier, and transporting the oxygen carrier with the sulfur-containing species back to the reducer. The oxygen carrier is a blend comprising at least one metal oxide and at least one calcium-containing species.

2. 发明申请

WO2018081060A1 METHOD, APPARATUS, AND COMPUTER-READABLE MEDIA FOR VORTEX ARC REACTOR 审中-公开
标题翻译： VORTEX ARC反应器的方法，装置和计算机可读介质
公开(公告)号：WO2018081060A1
公开(公告)日：2018-05-03
申请号：PCT/US2017/057998
申请日：2017-10-24
申请人： ROGERS, Michael, W.
发明人： ROGERS, Michael, W.
IPC分类号： B01J19/26 , B01J8/14
CPC分类号： B01J19/2405 , B01J8/14 , B01J19/088 , B01J19/1806 , B01J19/26 , B01J2208/00867 , B01J2219/00119 , B01J2219/0805 , B01J2219/0875 , C01B3/32 , C01B3/36 , C01B2203/0255 , C01B2203/1223 , C01B2203/1241 , C07C2/80 , C07C2/82 , C10G50/00 , C10G2300/1025 , C10G2400/30
摘要： Vortex arc reactor apparatus and method provide a nozzle with converging, throat, and diverging portions. Input structure inputs a reactant and an oxidant into the converging portion. Ignition structure ignites the input reactant and oxidant. A vortex-creating structure creates a vortex of the ignited reactant and oxidant in the converging portion. The input structure, the vortex-creating structure, and the nozzle converging and throat portions are configured to provide a throat-portion-vortex of ignited reactant and oxidant that has an angular velocity which provides (i) negatively-charged particles in an exterior portion of the throat-portion-vortex, (ii) positively-charged particles in an interior portion of the throat-portion-vortex, and (iii) at least one arcing reaction between the positively- charged particles and the negatively-charged particles, to form syngas and at least one aromatic liquid in the nozzle diverging portion. Gas/liquid separation structure is preferably configured to separate the formed syngas from the at least one aromatic liquid.
摘要翻译：涡流电弧反应器装置和方法提供了具有会聚，喉部和发散部分的喷嘴。输入结构将反应物和氧化剂输入会聚部分。点火结构点燃输入反应物和氧化剂。涡流产生结构在会聚部分中产生点燃的反应物和氧化剂的涡流。输入结构，涡流产生结构以及喷嘴会聚部和喉部部分被配置为提供具有角速度的点燃的反应物和氧化剂的喉部涡流，所述角速度提供（i）外部中的带负电的粒子（ii）喉部涡流的内部中的带正电的粒子，和（iii）带正电的粒子与带负电的粒子之间的至少一次电弧反应，以及在喷嘴分叉部分中形成合成气和至少一种芳香液体。气/液分离结构优选构造成将所形成的合成气与至少一种芳香液体分离。

3. 发明申请

WO2018004723A1 REACTOR-SEPARATOR ELEMENTS 审中-公开
标题翻译：反应器 - 分离器元件
公开(公告)号：WO2018004723A1
公开(公告)日：2018-01-04
申请号：PCT/US2016/059700
申请日：2016-10-31
申请人： COORS, W. Grover
发明人： COORS, W. Grover
IPC分类号： C01B3/50 , B01D53/22
CPC分类号： C25B1/10 , B01D53/228 , B01D53/326 , B01D61/12 , B01D63/063 , B01D69/046 , B01D71/022 , B01D71/024 , B01D2053/221 , B01D2256/16 , B01D2257/502 , B01D2257/504 , C01B3/40 , C01B3/501 , C01B3/503 , C01B2203/0233 , C01B2203/0405 , C01B2203/1058 , C01B2203/1241 , C01C1/0494 , C07C2/80 , C07C2529/06 , C25B11/02 , C25B13/02 , H01M8/0618 , H01M8/0656 , Y02C10/10 , Y02E60/366 , Y02P20/152
摘要： Reactor/separator elements for performing the generation and/or separation of hydrogen gas with improved efficiency have a central core and a separation layer that, in combination, define at least one spiral gas flow channel extending from one end of the central core to the opposite end of the central core. In use, the reactor/separator element may be placed in a housing which constrains gas on the outside of the reactor/separator element into the spiral channel defined by the outside of the separation layer.
摘要翻译：用于以改善的效率执行氢气的产生和/或分离的反应器/分离器元件具有中心核心和分离层，所述中心核心和分离层组合地限定至少一个螺旋气体流动通道，所述螺旋气体流动通道从一个中央核心的末端到中央核心的另一端。在使用中，反应器/分离器元件可以放置在将反应器/分离器元件外部的气体限制在由分离层外部限定的螺旋通道中的外壳中。

4. 发明申请

WO2017148929A1 LOW STEAM/CARBON REVAMP OF A PLANT COMPRISING A STEAM REFORMING SECTION AND A WATER-GAS SHIFT SECTION 审中-公开
标题翻译：包括蒸汽转化段和水气转换段的设备的低蒸汽/碳改造
公开(公告)号：WO2017148929A1
公开(公告)日：2017-09-08
申请号：PCT/EP2017/054618
申请日：2017-02-28
申请人： HALDOR TOPSØE A/S
发明人： ROSTRUP-NIELSEN, Thomas , SCHJØDT, Niels Christian , SPETH, Christian Henrik , KRØLL, Annette E.
IPC分类号： C01B3/48
CPC分类号： C01B3/48 , C01B2203/0233 , C01B2203/0283 , C01B2203/0288 , C01B2203/0294 , C01B2203/068 , C01B2203/1041 , C01B2203/1076 , C01B2203/1241 , C01B2203/1247 , C01B2203/1264 , C01B2203/141 , C01B2203/142 , C01B2203/143
摘要： The present invention relates to a revamp method for increasing the front-end capacity of a plant comprising - a reforming section, wherein a feed is reformed in at least one reforming step to - a reformed stream comprising CH 4 , CO, CO 2 , H 2 and H 2 O - a shift section wherein the reformed stream is shifted in a shift reaction in at least a high temperature shift step, said method comprising the steps of - In the High temperature shift step exchanging an original Fe-based catalyst with a non-Fe-based catalyst - Increasing the feed flow to the reforming section, and - The HTS step is carried out at a reduced steam/dry-gas ratio (S/DG) compared to an original S/DG in the original HTS step with the original Fe-based catalyst.
摘要翻译：本发明涉及一种用于增加设备前端容量的改造方法，其包括 - 重整段，其中进料在至少一个重整步骤中重整为 - 包含CH的重整流 4，CO，CO 2，H 2和H 2 O的偏移部分，其中重组流是所述方法包括以下步骤： - 在高温变换步骤中，将原始的Fe基催化剂与非Fe基催化剂交换 - 增加进入重整的进料流量 - 与最初的铁基催化剂在原始HTS步骤中的原始S / DG相比，HTS步骤在降低的蒸汽/干气比（S / DG）下进行。

5. 发明申请

WO2017087188A1 HEAT-RESISTANT HYDROCARBON REFORMING CATALYST BASED ON RHODIUM ON A LANTHANUM-STABILISED THETA-ALUMINA 审中-公开
标题翻译：基于铑的耐热烃重整催化剂在镧稳定的四氧化六铝上的应用
公开(公告)号：WO2017087188A1
公开(公告)日：2017-05-26
申请号：PCT/US2016/060528
申请日：2016-11-04
申请人： EXXONMOBIL RESEARCH AND ENGINEERING COMPANY
发明人： IDE, Matthew, Scott , BRODY, John, F. , WU, Jianxin , ALLEN, Joshua, W. , HERSHKOWITZ, Frank , BEHKISH, Arsam , SHARMA, Arun, K. , SKOULIDAS, Anastasios, I.
IPC分类号： B01J23/63 , B01J23/83 , B01J23/89 , B01J35/00 , B01J35/10 , B01J38/02 , C01B3/40 , B01J37/02 , B01J37/08 , B01J37/00
CPC分类号： C01B3/40 , B01J8/0438 , B01J8/0442 , B01J8/0492 , B01J8/0496 , B01J23/10 , B01J23/464 , B01J23/63 , B01J23/83 , B01J23/894 , B01J35/0066 , B01J35/04 , B01J35/1014 , B01J35/1019 , B01J37/0009 , B01J37/0036 , B01J37/0201 , B01J37/0215 , B01J37/0228 , B01J37/08 , B01J37/088 , B01J38/02 , B01J2208/00309 , B01J2523/00 , C01B2203/0233 , C01B2203/0238 , C01B2203/1023 , C01B2203/1047 , C01B2203/1064 , C01B2203/1082 , C01B2203/1235 , C01B2203/1241 , C01B2203/14 , C01B2203/1623 , C01B2203/1671 , B01J2523/31 , B01J2523/3706 , B01J2523/822
摘要： A reforming catalyst with improved surface area is provided by using high surface area alumina doped with a stabilizer metal, namely lanthanum, as a catalyst support. The lanthanum-stabilized alumina comprises theta alumina. The surface area of the catalyst can be higher than a typical reforming catalyst, and the surface area can also be maintained under high temperature operation (> 1200 °C). This can allow use of the catalyst for reforming in a higher temperature environment while maintaining a higher surface area, which can allow for improved dispersion and/or activity of an active metal such as rhodium on the catalyst support. The catalyst can be suitable for production of syngas from natural gas or other hydrocarbon- containing feeds.
摘要翻译：通过使用掺杂有稳定剂金属（即镧）的高表面积氧化铝作为催化剂载体，提供具有改善的表面积的重整催化剂。镧稳定的氧化铝包含θ氧化铝。催化剂的表面积可以高于典型的重整催化剂，并且表面积也可以在高温操作（> 1200℃）下保持。这可以允许在更高温度的环境中使用该催化剂进行重整，同时保持较高的表面积，这可以允许活性金属如铑在催化剂载体上的改善的分散和/或活性。该催化剂可适用于从天然气或其他含烃的原料生产合成气。

6. 发明申请

WO2017087125A1 A CARBON EFFICIENT PROCESS FOR CONVERTING METHANE TO OLEFINS AND METHANOL BY OXIDATIVE COUPLING OF METHANE 审中-公开
标题翻译：利用甲烷氧化偶联法将甲烷转化为烯烃和甲醇的高效碳工艺
公开(公告)号：WO2017087125A1
公开(公告)日：2017-05-26
申请号：PCT/US2016/058470
申请日：2016-10-24
申请人： SABIC GLOBAL TECHNOLOGIES, B.V. , SARSANI, Vidya Sagar Reddy , MAMEDOV, Aghaddin , WEST, David , LIANG, Wugeng
发明人： SARSANI, Vidya Sagar Reddy , MAMEDOV, Aghaddin , WEST, David , LIANG, Wugeng
IPC分类号： C07C29/50 , C07C29/151 , C07C2/82 , C07C5/327
CPC分类号： C07C5/32 , C01B3/36 , C01B2203/0255 , C01B2203/061 , C01B2203/062 , C01B2203/1241 , C07C2/82 , C07C5/327 , C07C29/1518 , C07C31/04 , C07C11/04 , C07C9/06
摘要： A method for producing olefins and methanol comprising introducing a first reactant mixture comprising CH 4 and O 2 to a first reaction zone; allowing the first reactant mixture to react via an OCM reaction to form a first product mixture characterized by a first H 2 /CO molar ratio; introducing a second reactant mixture comprising the first product mixture and an ethane stream to a second reaction zone, wherein ethane of the second reactant mixture undergoes a cracking reaction to produce ethylene; recovering a second product mixture from the second reaction zone, wherein the second product mixture is characterized by a second H 2 /CO molar ratio, and wherein the second H 2 /CO molar ratio is greater than the first H 2 /CO molar ratio; recovering from the second product mixture a methanol production feed stream comprising methane, H 2 and CO; and introducing the methanol production feed stream to a third reaction zone to produce methanol.
摘要翻译：一种用于生产烯烃和甲醇的方法，其包括将包含CH 4和O 2的第一反应物混合物引入到第一反应区中; 使第一反应物混合物经由OCM反应反应以形成以第一H 2 / CO摩尔比为特征的第一产物混合物; 将包含第一产物混合物和乙烷物流的第二反应物混合物引入第二反应区，其中第二反应物混合物的乙烷经历裂化反应以产生乙烯; 从第二反应区中回收第二产物混合物，其中第二产物混合物的特征在于第二H 2 / CO摩尔比，并且其中第二H 2 / CO 摩尔比大于第一H 2 / CO摩尔比; 从第二产物混合物中回收包含甲烷，H 2和CO的甲醇生产进料流; 并将甲醇生产原料流引入第三反应区以生产甲醇。

7. 发明申请

WO2017006121A1 CHEMICAL LOOPING 审中-公开
标题翻译：化学循环
公开(公告)号：WO2017006121A1
公开(公告)日：2017-01-12
申请号：PCT/GB2016/052044
申请日：2016-07-07
申请人： UNIVERSITY OF NEWCASTLE UPON TYNE
发明人： METCALFE, Ian
IPC分类号： B01J8/02 , C01B3/12 , C01B3/34 , C01B3/58
CPC分类号： B01J8/0221 , B01J2208/00548 , C01B3/12 , C01B3/34 , C01B3/583 , C01B2203/0233 , C01B2203/0283 , C01B2203/044 , C01B2203/047 , C01B2203/1241
摘要： This invention relates to a method of chemical looping using non-stoichiometric materials with a variable degree of non-stoichiometry. One application of these methods is in the water gas shift reaction for H 2 production. The methods of the invention can overcome limitations, e.g. those associated with chemical equilibria, which prevent chemical processes from proceeding with complete conversion of starting materials to products.
摘要翻译：本发明涉及一种使用非化学计量的具有可变程度的非化学计量的化学循环的方法。这些方法的一个应用是在H2生产的水煤气变换反应中。本发明的方法可以克服限制，例如与化学平衡相关的那些，其防止化学过程进行原料完全转化为产物。

8. 发明申请

WO2016191678A1 HYDROGEN PRODUCTION VIA SORBENT ENHANCED REFORMING WITH ATMOSPHERIC CALCINATION 审中-公开
标题翻译：氢气生产通过大气增压改造与大气压力
公开(公告)号：WO2016191678A1
公开(公告)日：2016-12-01
申请号：PCT/US2016/034636
申请日：2016-05-27
申请人： GAS TECHNOLOGY INSTITUTE
发明人： MAYS, Jeffrey , RAVISHANKAR, Sreenivasan
IPC分类号： C01B3/34 , C01B3/56
CPC分类号： C01B3/24 , B01D53/04 , B01D53/047 , B01D2253/10 , B01D2256/16 , B01D2257/504 , B01D2259/40088 , C01B3/30 , C01B3/34 , C01B3/56 , C01B2203/0233 , C01B2203/0425 , C01B2203/043 , C01B2203/0475 , C01B2203/1241
摘要： Processes and systems for producing hydrogen gas utilizing a sorbent enhanced reformer in combination with a calciner operating at atmospheric pressure. Feed material is introduced into the sorbent enhanced reformer to produce carbon dioxide and hydrogen gas. Sorbent material within the reformer acts to absorb carbon dioxide and form a used sorbent. The used sorbent is introduced into the atmospheric calciner to heat the used sorbent to desorb carbon dioxide from the used sorbent to produce regenerated sorbent which can be recycled to the reformer.
摘要翻译：利用吸附剂增强重整器与在大气压力下操作的煅烧器组合来生产氢气的方法和系统。将进料引入吸附剂增强重整器中以产生二氧化碳和氢气。重整器内的吸附材料用于吸收二氧化碳并形成用过的吸附剂。将所使用的吸附剂引入到大气煅烧器中以加热所用的吸附剂以从所使用的吸附剂中解吸二氧化碳，以产生可再循环至重整器的再生吸附剂。

9. 发明申请

WO2016180701A1 PROCESS FOR PREPARING A SYNGAS AND SYNGAS COOLING DEVICE 审中-公开
标题翻译：制备SYNGAS和SYGAS冷却装置的方法
公开(公告)号：WO2016180701A1
公开(公告)日：2016-11-17
申请号：PCT/EP2016/059994
申请日：2016-05-04
申请人： SHELL INTERNATIONALE RESEARCH MAATSCHAPPIJ B.V. , SHELL OIL COMPANY
发明人： SCHMITZ-GOEB, Manfred, Heinrich , SMIT, Ruben
IPC分类号： C01B3/36 , C01B3/38
CPC分类号： C01B3/386 , C01B3/36 , C01B3/38 , C01B3/382 , C01B2203/0244 , C01B2203/025 , C01B2203/0255 , C01B2203/0261 , C01B2203/0883 , C01B2203/0894 , C01B2203/1241 , C01B2203/82 , F28D7/024 , F28D7/12
摘要： The invention relates to a process for the preparation of a syngas comprising hydrogen and carbon monoxide comprising the steps of: (a) reacting a preheated methane comprising gas with an oxidising gas to obtain a hot raw syngas comprising carbon monoxide and hydrogen; (b) cooling the hot raw syngas resulting from step (a) to obtain the syngas by indirect heat exchange against water to produce saturated steam; (c) further cooling the raw syngas obtained in step (b) by indirect heat exchange against a methane comprising gas to obtain a cooled raw syngas and the preheated methane comprising gas for use in step (a), wherein: (i) steps (b) and (c) take place in a single cooling device for combined indirect heat exchange against water and against the methane comprising gas; and (ii) the preheated methane comprising gas obtained in step (c) has a temperature between 400 and 650°C. The invention also relates to a cooling device which can be used as the single cooling device in the above process. The cooling device comprises an evaporation section for producing saturated steam, a gas heat exchange section for preheating the methane comprising feed used in step (a) against the raw syngas and a dry steam collection space. This dry steam collection space is separated from the evaporation section where wet saturated steam is formed.
摘要翻译：本发明涉及一种制备包含氢气和一氧化碳的合成气的方法，包括以下步骤：（a）使包含气体的预热甲烷与氧化气体反应，得到包含一氧化碳和氢气的热原料合成气; （b）冷却由步骤（a）产生的热原料合成气，通过与水的间接热交换获得合成气以产生饱和蒸汽; （c）通过与包含甲烷的气体的间接热交换来进一步冷却步骤（b）中获得的原料合成气，以获得冷却的原料合成气，并且预热的甲烷包含用于步骤（a）中的气体，其中：（i）步骤 b）和（c）在单个冷却装置中进行，用于与水和包含气体的甲烷的组合间接热交换; 和（ii）步骤（c）中获得的包含气体的预热甲烷的温度在400-650℃之间。本发明还涉及一种在上述方法中可用作单个冷却装置的冷却装置。冷却装置包括用于产生饱和蒸汽的蒸发部分，用于将包括步骤（a）中使用的甲烷的甲烷预热到原始合成气的干燥蒸汽收集空间的气体热交换部分。该干蒸汽收集空间与形成湿饱和蒸汽的蒸发部分分离。

10. 发明申请

WO2016150268A1 绝热式天然气催化氧化炉在线烘炉方法审中-公开
公开(公告)号：WO2016150268A1
公开(公告)日：2016-09-29
申请号：PCT/CN2016/074636
申请日：2016-02-26
申请人：武汉凯迪工程技术研究总院有限公司
发明人：陈义龙 , 张岩丰 , 蒯平宇 , 田文堂 , 王大祥
IPC分类号： C01B3/38 , C01B31/18
CPC分类号： C01B3/40 , C01B3/386 , C01B32/40 , C01B2203/0261 , C01B2203/1017 , C01B2203/1082 , C01B2203/1241 , C01B2203/1614 , C01B2203/169
摘要：本发明公开了一种绝热式天然气催化氧化炉在线烘炉方法，包括：1)向天然气催化氧化炉中同时充入氧气、天然气和能够降低反应升温速率的控温气体，控制氧气和天然气的摩尔比为0.3～0.6∶1，同时控制控温气体与由氧气和天然气组成的原料气的摩尔比为0.1～7∶1.3～1.6；2)对混合气体进行预热逐步提高温度，直至达氧化反应触发温度时停止预热；3)逐步降低控温气体与原料气的摩尔比例，使反应温度以符合设计烘炉曲线要求的升温速率上升，直至反应温度达到工作温度后停止充入控温气体。本发明解决了烘炉期间温度升高过快的问题，避免了绝热耐火材料因骤热而开裂，保护了天然气催化氧化炉，使其能够平稳地过渡到正常运转的状态。

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