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1. 发明申请

WO2009111026A3 CATALYTIC PYROLYSIS OF SOLID BIOMASS AND RELATED BIOFUELS, AROMATIC, AND OLEFIN COMPOUNDS 审中-公开
公开(公告)号：WO2009111026A3
公开(公告)日：2009-09-11
申请号：PCT/US2009/001382
申请日：2009-03-03
申请人： UNIVERSITY OF MASSACHUSETTS , HUBER, George, W. , VISPUTE, Tushar , CARLSON, Torren , JAE, Jungho , CHENG, Yu-Ting , TOMPSETT, Geoffrey
发明人： HUBER, George, W. , VISPUTE, Tushar , CARLSON, Torren , JAE, Jungho , CHENG, Yu-Ting , TOMPSETT, Geoffrey
IPC分类号： C10G11/18
摘要： This invention relates to compositions and methods for fluid hydrocarbon product, and more specifically, to compositions and methods for fluid hydrocarbon product via catalytic pyrolysis. Some embodiments relate to methods for the production of specific aromatic products (e.g., benzene, toluene, naphthalene, xylene, etc.) via catalytic pyrolysis. Some such methods may involve the use of a composition comprising a mixture of a solid hydrocarbonaceous material and a heterogeneous pyrolytic catalyst component. In some embodiments, the mixture may be pyrolyzed at high temperatures (e.g., between 500 °C and 1000 °C). The pyrolysis may be conducted for an amount of time at least partially sufficient for production of discrete, identifiable biofuel compounds. Some embodiments involve heating the mixture of catalyst and hydrocarbonaceous material at high rates (e.g., from about 50 °C per second to about 1000 0C per second). The methods described herein may also involve the use of specialized catalysts. For example, in some cases, zeolite catalysts may be used; optionally, the catalysts used herein may have high silica to alumina molar ratios. In some instances, the composition fed to the pyrolysis reactor may have a relatively high catalyst to hydrocarbonaceous material mass ratio (e.g., from about 5: 1 to about 20:1).

2. 发明申请

WO2007103858A2 STABLE, AQUEOUS-PHASE, BASIC CATALYSTS AND REACTIONS CATALYZED THEREBY 审中-公开
标题翻译：稳定，水相，碱催化剂及其催化反应
公开(公告)号：WO2007103858A2
公开(公告)日：2007-09-13
申请号：PCT/US2007063286
申请日：2007-03-05
申请人： WISCONSIN ALUMNI RES FOUND , DUMESIS JAMES A , HUBER GEORGE W , CHHEDA JUBEN N , BARRETT CHRISTOPHER J
发明人： DUMESIS JAMES A , HUBER GEORGE W , CHHEDA JUBEN N , BARRETT CHRISTOPHER J
IPC分类号： C07C1/247 , C07C9/14
CPC分类号： C07C9/14 , B01J21/10 , B01J23/44 , C07D307/12
摘要： A catalytic process for converting biomass-derived carbohydrates to liquid alkanes, alkenes, and/or ethers is described. The process uses combinations of self- and crossed-aldol condensation reactions, dehydration reactions, and hydrogenation reactions, over specified metal-containing catalysts, to yield alkane, alkene, and ether products from carbohydrate reactants.
摘要翻译：描述了将生物质衍生的碳水化合物转化为液体烷烃，烯烃和/或醚的催化方法。该方法在特定的含金属催化剂上使用自交联和交叉醛醇缩合反应，脱水反应和氢化反应的组合，从碳水化合物反应物中得到烷烃，烯烃和醚产物。

3. 发明申请

WO2010033789A2 PRODUCTION OF HYDROGEN, LIQUID FUELS, AND CHEMICALS FROM CATALYTIC PROCESSING OF BIO-OILS 审中-公开
标题翻译：从生物油催化加工生产氢，液体燃料和化学品
公开(公告)号：WO2010033789A2
公开(公告)日：2010-03-25
申请号：PCT/US2009/057459
申请日：2009-09-18
申请人： UNIVERSITY OF MASSACHUSETTS , HUBER, George W. , VISPUTE, Tushar P. , ROUTRAY, Kamalakanta
发明人： HUBER, George W. , VISPUTE, Tushar P. , ROUTRAY, Kamalakanta
IPC分类号： C01B3/38 , C01B3/26 , C10G45/04 , C10G65/02 , B01J23/46 , B01J23/42 , B01J21/12
CPC分类号： C01B3/323 , B01J23/002 , B01J27/1856 , B01J37/0205 , B01J2523/00 , C01B2203/1047 , C01B2203/1052 , C01B2203/1058 , C01B2203/1064 , C01B2203/107 , C01B2203/1264 , C01B2203/148 , C10G1/083 , C10G1/086 , C10G3/47 , C10G3/52 , C10G49/007 , C10G2300/1014 , C10G2400/02 , C10G2400/04 , Y02P20/52 , Y02P30/20 , B01J2523/48 , B01J2523/51 , B01J2523/828
摘要： Disclosed herein is a method of generating hydrogen from a bio-oil, comprising hydrogenating a water-soluble fraction of the bio-oil with hydrogen in the presence of a hydrogenation catalyst, and reforming the water-soluble fraction by aqueous-phase reforming in the presence of a reforming catalyst, wherein hydrogen is generated by the reforming, and the amount of hydrogen generated is greater than that consumed by the hydrogenating. The method can further comprise hydrocracking or hydrotreating a lignin fraction of the bio-oil with hydrogen in the presence of a hydrocracking catalyst wherein the lignin fraction of bio-oil is obtained as a water-insoluble fraction from aqueous extraction of bio-oil. The hydrogen used in the hydrogenating and in the hydrocracking or hydrotreating can be generated by reforming the water-soluble fraction of bio-oil.
摘要翻译：本文公开了一种从生物油产生氢的方法，包括在氢化催化剂存在下用氢气氢化生物油的水溶性馏分，并通过水相重整在水溶性馏分中重整重整催化剂的存在，其中通过重整生成氢，并且产生的氢的量大于通过氢化消耗的氢的量。该方法可以进一步包括在加氢裂化催化剂存在下用氢气加氢裂解或加氢处理生物油的木质素部分，其中生物油的木质素部分作为水不溶性部分从生物油的水提取物中获得。用于氢化和加氢裂化或加氢处理的氢气可以通过重整生物油的水溶性部分来产生。

4. 发明申请

WO2013032672A1 METHOD FOR PRODUCING FLUID HYDROCARBONS 审中-公开
标题翻译：生产流体烃的方法
公开(公告)号：WO2013032672A1
公开(公告)日：2013-03-07
申请号：PCT/US2012/050510
申请日：2012-08-13
申请人： UNIVERSITY OF MASSACHUSETTS , HUBER, George W. , ZHANG, Huiyan , CARLSON, Torren
发明人： HUBER, George W. , ZHANG, Huiyan , CARLSON, Torren
IPC分类号： C10G1/08 , C10B49/22 , C10B53/02 , C10B57/06 , C10G1/10
CPC分类号： C10B49/22 , C10B53/02 , C10B57/06 , C10G1/002 , C10G1/02 , C10G1/08 , C10G1/10 , C10G3/42 , C10G3/50 , C10G2300/1011 , Y02E50/14 , Y02E50/32 , Y02P20/582 , Y02P30/20
摘要： The invention relates to methods for producing fluid hydrocarbon products, and more specifically, to methods for producing fluid hydrocarbon product via catalytic pyrolysis. The reactants comprise solid hydrocarbonaceous materials, and hydrogen or a source of hydrogen (e.g., an alcohol). The products may include specific aromatic compounds (e.g., benzene, toluene, naphthalene, xylene, etc.).
摘要翻译：本发明涉及制备流体烃产品的方法，更具体地说，涉及通过催化裂解制备流化烃产物的方法。反应物包括固体含烃物质，氢气或氢源（例如醇）。产物可以包括特定的芳族化合物（例如苯，甲苯，萘，二甲苯等）。

5. 发明申请

WO2010033789A3 PRODUCTION OF HYDROGEN, LIQUID FUELS, AND CHEMICALS FROM CATALYTIC PROCESSING OF BIO-OILS 审中-公开
标题翻译：生物油催化加工生产氢，液体燃料和化学品
公开(公告)号：WO2010033789A3
公开(公告)日：2010-07-15
申请号：PCT/US2009057459
申请日：2009-09-18
申请人： UNIV MASSACHUSETTS , HUBER GEORGE W , VISPUTE TUSHAR P , ROUTRAY KAMALAKANTA
发明人： HUBER GEORGE W , VISPUTE TUSHAR P , ROUTRAY KAMALAKANTA
IPC分类号： C01B3/38 , B01J21/12 , B01J23/42 , B01J23/46 , C01B3/26 , C10G45/04 , C10G65/02
CPC分类号： C01B3/323 , B01J23/002 , B01J27/1856 , B01J37/0205 , B01J2523/00 , C01B2203/1047 , C01B2203/1052 , C01B2203/1058 , C01B2203/1064 , C01B2203/107 , C01B2203/1264 , C01B2203/148 , C10G1/083 , C10G1/086 , C10G3/47 , C10G3/52 , C10G49/007 , C10G2300/1014 , C10G2400/02 , C10G2400/04 , Y02P20/52 , Y02P30/20 , B01J2523/48 , B01J2523/51 , B01J2523/828
摘要： Disclosed herein is a method of generating hydrogen from a bio-oil, comprising hydrogenating a water-soluble fraction of the bio-oil with hydrogen in the presence of a hydrogenation catalyst, and reforming the water-soluble fraction by aqueous-phase reforming in the presence of a reforming catalyst, wherein hydrogen is generated by the reforming, and the amount of hydrogen generated is greater than that consumed by the hydrogenating. The method can further comprise hydrocracking or hydrotreating a lignin fraction of the bio-oil with hydrogen in the presence of a hydrocracking catalyst wherein the lignin fraction of bio-oil is obtained as a water-insoluble fraction from aqueous extraction of bio-oil. The hydrogen used in the hydrogenating and in the hydrocracking or hydrotreating can be generated by reforming the water-soluble fraction of bio-oil.
摘要翻译：本文公开了一种从生物油产生氢气的方法，包括在氢化催化剂存在下用氢气将生物油的水溶性部分氢化，并且通过在所述生物油中的水相重整使所述水溶性部分重整重整催化剂的存在，其中通过重整产生氢气，并且产生的氢气量大于氢化消耗的氢气量。该方法可以进一步包括在加氢裂化催化剂存在下用氢气对生物油的木质素部分进行加氢裂化或加氢处理，其中生物油的木质素部分作为来自生物油水提取物的水不溶部分获得。用于氢化和加氢裂化或加氢处理中的氢可以通过重整生物油的水溶性部分而产生。

6. 发明申请

WO2009111026A8 CATALYTIC PYROLYSIS OF SOLID BIOMASS AND RELATED BIOFUELS, AROMATIC, AND OLEFIN COMPOUNDS 审中-公开
标题翻译：固体生物质和相关生物燃料，芳香烃和烯烃化合物的催化热解
公开(公告)号：WO2009111026A8
公开(公告)日：2009-12-03
申请号：PCT/US2009001382
申请日：2009-03-03
申请人： UNIV MASSACHUSETTS , HUBER GEORGE W , VISPUTE TUSHAR , CARLSON TORREN , JAE JUNGHO , CHENG YU-TING , TOMPSETT GEOFFREY
发明人： HUBER GEORGE W , VISPUTE TUSHAR , CARLSON TORREN , JAE JUNGHO , CHENG YU-TING , TOMPSETT GEOFFREY
IPC分类号： C10G11/18
CPC分类号： C10G1/002 , C10G1/08 , C10G2300/1014 , C10G2300/1018 , C10G2300/305 , C10G2400/02 , C10G2400/20 , C10G2400/30 , Y02P30/42
摘要： This invention relates to compositions and methods for fluid hydrocarbon product, and more specifically, to compositions and methods for fluid hydrocarbon product via catalytic pyrolysis. Some embodiments relate to methods for the production of specific aromatic products (e.g., benzene, toluene, naphthalene, xylene, etc.) via catalytic pyrolysis. Some such methods may involve the use of a composition comprising a mixture of a solid hydrocarbonaceous material and a heterogeneous pyrolytic catalyst component. In some embodiments, the mixture may be pyrolyzed at high temperatures (e.g., between 500 °C and 1000 °C). The pyrolysis may be conducted for an amount of time at least partially sufficient for production of discrete, identifiable biofuel compounds. Some embodiments involve heating the mixture of catalyst and hydrocarbonaceous material at high rates (e.g., from about 50 °C per second to about 1000 0C per second). The methods described herein may also involve the use of specialized catalysts. For example, in some cases, zeolite catalysts may be used; optionally, the catalysts used herein may have high silica to alumina molar ratios. In some instances, the composition fed to the pyrolysis reactor may have a relatively high catalyst to hydrocarbonaceous material mass ratio (e.g., from about 5: 1 to about 20:1).
摘要翻译：本发明涉及用于流体烃产品的组合物和方法，更具体地说，涉及用于通过催化热解的流体烃产物的组合物和方法。一些实施方案涉及通过催化热解生产特定芳族产物（例如苯，甲苯，萘，二甲苯等）的方法。一些此类方法可涉及使用包含固体含烃材料和非均相热解催化剂组分的混合物的组合物。在一些实施方案中，该混合物可以在高温下（例如在500℃和1000℃之间）热解。热解可以进行至少部分足以产生分立的，可识别的生物燃料化合物的时间量。一些实施方案涉及以高速率（例如，从约每秒50℃至每秒约1000℃）加热催化剂和含烃材料的混合物。本文所述的方法还可以涉及使用专门的催化剂。例如，在一些情况下，可以使用沸石催化剂; 任选地，本文使用的催化剂可以具有高的二氧化硅/氧化铝摩尔比。在一些情况下，进料至热解反应器的组合物可具有相对高的催化剂与烃材料质量比（例如约5：1至约20：1）。

7. 发明申请

WO2008020048A3 PRODUCTION OF LINEAR ALKANES BY HYDROTREATING MIXTURES OF TRIGLYCERIDES WITH VACUUM GASOIL 审中-公开
标题翻译：真空气加氢处理甘油三元混合物生产线性烷烃
公开(公告)号：WO2008020048A3
公开(公告)日：2008-04-24
申请号：PCT/EP2007058468
申请日：2007-08-15
申请人： BIOECON INT HOLDING NV , O'CONNOR PAUL , STAMIRES DENNIS , CORMA CAMOS AVELINO AVELINO , HUBER GEORGE W
发明人： O'CONNOR PAUL , STAMIRES DENNIS , CORMA CAMOS AVELINO AVELINO , HUBER GEORGE W
IPC分类号： C10G3/00 , C07C5/02 , C07C9/22 , C10G45/02 , C10L1/08
CPC分类号： C10G3/50 , C10G3/46 , C10G2300/1011 , C10G2300/1014 , C10G2300/1059 , C10G2300/4012 , C10G2300/805 , C10G2400/04 , Y02P30/20
摘要： A process is disclosed for mild hydro-conversion of oxygenated hydrocarbon compounds. The oxygenated hydrocarbon compounds are contacted with a hydro- conversion catalyst material at a reaction pressure below 100 bar. Preferred oxygenated hydrocarbon compounds are those obtained by the liquefaction of biomass. In a specific embodiment the process is used for production of normal alkanes by hydrotreating mixtures of triglycerides (or compounds derived-from triglycerides, including free fatty acids) and vacuum gasoil.
摘要翻译：公开了用于含氧烃化合物的温和加氢转化的方法。含氧烃化合物在低于100巴的反应压力下与加氢转化催化剂材料接触。优选的含氧烃化合物是通过液化生物质获得的那些。在一个具体的实施方案中，该方法用于通过加氢处理甘油三酯（或来自甘油三酯，包括游离脂肪酸的化合物）和真空瓦斯油的混合物来生产正烷烃。

8. 发明申请

WO2008020047A3 FLUID CATALYTIC CRACKING OF OXYGENATED COMPOUNDS 审中-公开
标题翻译：含氧化合物的流体催化裂化
公开(公告)号：WO2008020047A3
公开(公告)日：2008-04-03
申请号：PCT/EP2007058467
申请日：2007-08-15
申请人： BIOECON INT HOLDING NV , O'CONNOR PAUL , HUBER GEORGE W , CORMA CAMOS AVELINO AVELINO , SAVANAUD LAURENT LOUIS ANDRE
发明人： O'CONNOR PAUL , HUBER GEORGE W , CORMA CAMOS AVELINO AVELINO , SAVANAUD LAURENT LOUIS ANDRE
IPC分类号： C10G3/00 , C10G11/02 , C10G11/18 , C10G51/02
CPC分类号： C10G3/57 , C10G3/46 , C10G3/47 , C10G3/49 , C10G11/18 , C10G51/026 , C10G2300/1011 , C10G2300/1074 , C10G2300/4006 , C10G2300/805 , Y02E50/10 , Y02E50/30 , Y02P30/20
摘要： A process is disclosed for fluid catalytic cracking of oxygenated hydrocarbon compounds such as glycerol and bio-oil. In the process the oxygenated hydrocarbon compounds are contacted with a fluid cracking catalyst material for a period of less than 3 seconds. In a preferred process a crude-oil derived material, such as VGO, is also contacted with the catalyst.
摘要翻译：公开了一种用于含氧化合物如甘油和生物油的流化催化裂化的方法。在该过程中，氧化烃化合物与流体裂解催化剂材料接触少于3秒的时间。在优选的方法中，原油衍生的材料，例如VGO，也与催化剂接触。

9. 发明申请

WO2008020048A2 PRODUCTION OF LINEAR ALKANES BY HYDROTREATING MIXTURES OF TRIGLYCERIDES WITH VACUUM GASOIL 审中-公开
标题翻译：通过用真空气体氢化混合物混合生产线性烷烃
公开(公告)号：WO2008020048A2
公开(公告)日：2008-02-21
申请号：PCT/EP2007/058468
申请日：2007-08-15
申请人： BIOECON INTERNATIONAL HOLDING N.V. , O'CONNOR, Paul , STAMIRES, Dennis , CORMA CAMOS AVELINO, Avelino , HUBER, George W.
发明人： O'CONNOR, Paul , STAMIRES, Dennis , CORMA CAMOS AVELINO, Avelino , HUBER, George W.
IPC分类号： C10G3/00 , C10G45/02
CPC分类号： C10G3/50 , C10G3/46 , C10G2300/1011 , C10G2300/1014 , C10G2300/1059 , C10G2300/4012 , C10G2300/805 , C10G2400/04 , Y02P30/20
摘要： A process is disclosed for mild hydro-conversion of oxygenated hydrocarbon compounds. The oxygenated hydrocarbon compounds are contacted with a hydro- conversion catalyst material at a reaction pressure below 100 bar. Preferred oxygenated hydrocarbon compounds are those obtained by the liquefaction of biomass. In a specific embodiment the process is used for production of normal alkanes by hydrotreating mixtures of triglycerides (or compounds derived-from triglycerides, including free fatty acids) and vacuum gasoil.
摘要翻译：公开了一种用于氧化烃化合物的轻度加氢转化的方法。氧化烃化合物在低于100巴的反应压力下与水力转化催化剂材料接触。优选的含氧烃化合物是通过液化生物质获得的化合物。在一个具体实施方案中，该方法用于通过加氢处理甘油三酯（或衍生自甘油三酸酯，包括游离脂肪酸的化合物）和真空气体油的混合物来生产正烷烃。

10. 发明申请

WO2007103858A3 STABLE, AQUEOUS-PHASE, BASIC CATALYSTS AND REACTIONS CATALYZED THEREBY 审中-公开
公开(公告)号：WO2007103858A3
公开(公告)日：2007-09-13
申请号：PCT/US2007/063286
申请日：2007-03-05
申请人： WISCONSIN ALUMNI RESEARCH FOUNDATION , DUMESIS, James, A. , HUBER, George, W. , CHHEDA, Juben, N. , BARRETT, Christopher, J.
发明人： DUMESIS, James, A. , HUBER, George, W. , CHHEDA, Juben, N. , BARRETT, Christopher, J.
IPC分类号： C07C1/247 , C07C9/14
摘要： A catalytic process for converting biomass-derived carbohydrates to liquid alkanes, alkenes, and/or ethers is described. The process uses combinations of self- and crossed-aldol condensation reactions, dehydration reactions, and hydrogenation reactions, over specified metal-containing catalysts, to yield alkane, alkene, and ether products from carbohydrate reactants.

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