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1. 发明申请

WO2012015909A2 HETEROCYCLE CATALYZED ELECTROCHEMICAL PROCESS 审中-公开
标题翻译：杂环催化电化学工艺
公开(公告)号：WO2012015909A2
公开(公告)日：2012-02-02
申请号：PCT/US2011/045521
申请日：2011-07-27
申请人： LIQUID LIGHT, INC. , PRINCETON UNIVERSITY , COLE, Emily, Barton , BOCARSLY, Andrew, B.
发明人： COLE, Emily, Barton , BOCARSLY, Andrew, B.
IPC分类号： C25B3/04
CPC分类号： C25B3/04 , C25B1/003 , C25B3/105
摘要： A method for heterocycle catalyzed electrochemical reduction of a carbonyl compound is disclosed. The method generally includes steps (A) to (C). Step (A) may introduce the carbonyl compound into a solution of an electrolyte and a heterocycle catalyst in a divided electrochemical cell. The divided electrochemical cell may include an anode in a first cell compartment and a cathode in a second cell compartment. The cathode generally reduces the carbonyl compound to at least one aldehyde compound. Step (B) may vary which of the aldehyde compounds is produced by adjusting one or more of (i) a cathode material, (ii) the electrolyte, (iii) the heterocycle catalyst, (iv) a pH level and (v) an electrical potential. Step (C) may separate the aldehyde compounds from the solution.
摘要翻译：公开了一种用于羰基化合物的杂环催化的电化学还原的方法。该方法通常包括步骤（A）至（C）。步骤（A）可以将羰基化合物引入电解质和杂环催化剂的溶液中。分隔的电化学电池可以包括第一电池室中的阳极和第二电池室中的阴极。阴极通常将羰基化合物还原成至少一种醛化合物。步骤（B）可以通过调节（i）阴极材料，（ii）电解质，（iii）杂环催化剂，（iv）pH水平和（v））中的一种或多种来改变哪种醛化合物的产生电位步骤（C）可以将醛化合物与溶液分离。

2. 发明申请

WO2013082362A1 HETEROCYCLE CATALYZED CARBONYLATION HYDROFORMYLATION WITH CARBON DIOXIDE 审中-公开
标题翻译：二氧化碳杂化催化羰化氢化
公开(公告)号：WO2013082362A1
公开(公告)日：2013-06-06
申请号：PCT/US2012/067197
申请日：2012-11-30
申请人： LIQUID LIGHT, INC. , SIVASANKAR, Narayanapa , TEAMEY, Kyle , COLE, Emily, Barton
发明人： SIVASANKAR, Narayanapa , TEAMEY, Kyle , COLE, Emily, Barton
IPC分类号： C25B1/00 , C25B3/00 , C25B9/00
CPC分类号： C25B3/02 , B01J2231/321 , C25B1/003 , C25B3/00 , C25B3/04
摘要： Methods and systems for heterocycle catalyzed carbonylation and hydroformylation with carbon dioxide are disclosed. A method may include, but is not limited to, steps (A) to (D). Step (A) may introduce water to a first compartment of an electrochemical cell. The first compartment may include an anode. Step (B) may introduce carbon dioxide to a second compartment of the electrochemical cell. The second compartment may include a solution of an electrolyte, a heterocyclic catalyst, and a cathode. Step (C) may introduce a second reactant to the second compartment of the electrochemical cell. Step (D) may apply an electrical potential between the anode and the cathode in the electrochemical cell sufficient to induce liquid phase carbonylation or hydroformylation to form a product mixture.
摘要翻译：公开了用二氧化碳进行杂环催化羰基化和加氢甲酰基化的方法和系统。方法可以包括但不限于步骤（A）至（D）。步骤（A）可以将水引入电化学电池的第一隔室。第一隔室可包括阳极。步骤（B）可以将二氧化碳引入电化学电池的第二隔室。第二隔室可以包括电解质，杂环催化剂和阴极的溶液。步骤（C）可以将第二反应物引入电化学电池的第二隔室。步骤（D）可以在电化学电池中的阳极和阴极之间施加足以引起液相羰基化或加氢甲酰化以形成产物混合物的电势。

3. 发明申请

WO2012015909A3 HETEROCYCLE CATALYZED ELECTROCHEMICAL PROCESS 审中-公开
标题翻译：杂环催化电化学工艺
公开(公告)号：WO2012015909A3
公开(公告)日：2013-08-08
申请号：PCT/US2011045521
申请日：2011-07-27
申请人： LIQUID LIGHT INC , UNIV PRINCETON , COLE EMILY BARTON , BOCARSLY ANDREW B
发明人： COLE EMILY BARTON , BOCARSLY ANDREW B
IPC分类号： C25B3/04
CPC分类号： C25B3/04 , C25B1/003 , C25B3/105
摘要： A method for heterocycle catalyzed electrochemical reduction of a carbonyl compound is disclosed. The method generally includes steps (A) to (C). Step (A) may introduce the carbonyl compound into a solution of an electrolyte and a heterocycle catalyst in a divided electrochemical cell. The divided electrochemical cell may include an anode in a first cell compartment and a cathode in a second cell compartment. The cathode generally reduces the carbonyl compound to at least one aldehyde compound. Step (B) may vary which of the aldehyde compounds is produced by adjusting one or more of (i) a cathode material, (ii) the electrolyte, (iii) the heterocycle catalyst, (iv) a pH level and (v) an electrical potential. Step (C) may separate the aldehyde compounds from the solution.
摘要翻译：公开了一种用于羰基化合物的杂环催化的电化学还原的方法。该方法通常包括步骤（A）至（C）。步骤（A）可以将羰基化合物引入电解质和杂环催化剂的溶液中。分隔的电化学电池可以包括第一电池室中的阳极和第二电池室中的阴极。阴极通常将羰基化合物还原成至少一种醛化合物。步骤（B）可以通过调节（i）阴极材料，（ii）电解质，（iii）杂环催化剂，（iv）pH水平和（v））中的一种或多种来改变哪种醛化合物的产生电位步骤（C）可以将醛化合物与溶液分离。

4. 发明申请

WO2013006711A1 REDUCTION OF CARBON DIOXIDE TO CARBOXYLIC ACIDS, GLYCOLS, AND CARBOXYLATES 审中-公开
标题翻译：将二氧化碳还原成羧酸，甘油和羧酸酯
公开(公告)号：WO2013006711A1
公开(公告)日：2013-01-10
申请号：PCT/US2012/045578
申请日：2012-07-05
申请人： LIQUID LIGHT, INC. , COLE, Emily, Barton , TEAMEY, Kyle , BOCARSLY, Andrew, B. , SIVASANKAR, Narayanappa
发明人： COLE, Emily, Barton , TEAMEY, Kyle , BOCARSLY, Andrew, B. , SIVASANKAR, Narayanappa
IPC分类号： C25B3/04
CPC分类号： C25B11/04 , C25B3/04
摘要： Methods and systems for electrochemical conversion of carbon dioxide to carboxylic acids, glycols, and carboxylates are disclosed. A method may include, but is not limited to, steps (A) to (D). Step (A) may introduce water to a first compartment of an electrochemical cell. The first compartment may include an anode. Step (B) may introduce carbon dioxide to a second compartment of the electrochemical cell. The second compartment may include a solution of an electrolyte and a cathode. Step (C) may apply an electrical potential between the anode and the cathode in the electrochemical cell sufficient to reduce the carbon dioxide to a carboxylic acid intermediate. Step (D) may contact the carboxylic acid intermediate with hydrogen to produce a reaction product.
摘要翻译：公开了将二氧化碳电化学转化成羧酸，二醇和羧酸盐的方法和系统。方法可以包括但不限于步骤（A）至（D）。步骤（A）可以将水引入电化学电池的第一隔室。第一隔室可包括阳极。步骤（B）可以将二氧化碳引入电化学电池的第二隔室。第二隔室可以包括电解质和阴极的溶液。步骤（C）可以在电化学电池中的阳极和阴极之间施加足以将二氧化碳还原成羧酸中间体的电位。步骤（D）可以将羧酸中间体与氢接触以产生反应产物。

5. 发明申请

WO2012015905A1 REDUCING CARBON DIOXIDE TO PRODUCTS 审中-公开
标题翻译：减少二氧化碳产品
公开(公告)号：WO2012015905A1
公开(公告)日：2012-02-02
申请号：PCT/US2011/045515
申请日：2011-07-27
申请人： LIQUID LIGHT, INC. , COLE, Emily, Barton , SIVASANKAR, Narayanappa , BOCARSLY, Andrew, B. , TEAMEY, Kyle , KRISHNA, Nety
发明人： COLE, Emily, Barton , SIVASANKAR, Narayanappa , BOCARSLY, Andrew, B. , TEAMEY, Kyle , KRISHNA, Nety
IPC分类号： C25B3/04 , C25B1/00
CPC分类号： C25B3/04 , C25B1/003
摘要： A method for reducing carbon dioxide to one or more products is disclosed. The method may include steps (A) to (C). Step (A) may bubble the carbon dioxide into a solution of an electrolyte and a catalyst in a divided electrochemical cell. The divided electrochemical cell may include an anode in a first cell compartment and a cathode in a second cell compartment. The cathode generally reduces the carbon dioxide into the products. Step {B} may vary at least one of (i) which of the products is produced and (ii) a faradaic yield of the products by adjusting one or more of (a) a cathode material and (b) a surface morphology of the cathode. Step (C) may separate the products from the solution.
摘要翻译：公开了一种将二氧化碳还原成一种或多种产品的方法。该方法可以包括步骤（A）至（C）。步骤（A）可以使二氧化碳在电解槽中分解成电解质和催化剂的溶液。分隔的电化学电池可以包括第一电池室中的阳极和第二电池室中的阴极。阴极通常将二氧化碳减少到产品中。步骤{B}可以改变以下至少一个：（i）产生哪种产品;（ii）通过调整（a）阴极材料和（b）表面形态的一种或多种产品的法拉第产量阴极。步骤（C）可以将产品与溶液分开。

6. 发明申请

WO2012015921A1 ELECTROCHEMICAL PRODUCTION OF SYNTHESIS GAS FROM CARBON DIOXIDE 审中-公开
标题翻译：二氧化碳合成气的电化学生产
公开(公告)号：WO2012015921A1
公开(公告)日：2012-02-02
申请号：PCT/US2011/045534
申请日：2011-07-27
申请人： LIQUID LIGHT, INC. , SIVASANKAR, Narayanappa , COLE, Emily, Barton , TEAMEY, Kyle
发明人： SIVASANKAR, Narayanappa , COLE, Emily, Barton , TEAMEY, Kyle
IPC分类号： C25B3/00
CPC分类号： C25B1/02 , B01D53/326 , B01D2256/12 , B01D2257/504 , C25B1/00 , C25B1/003 , Y02E60/366 , Y02P20/152
摘要： A method for electrochemical production of synthesis gas from carbon dioxide is disclosed. The method generally includes steps (A) to (C). Step (A) may bubble the carbon dioxide into a solution of an electrolyte and a catalyst in a divided electrochemical cell. The divided electrochemical cell may include an anode in a first cell compartment and a cathode in a second cell compartment. The cathode generally reduces the carbon dioxide into a plurality of components. Step (B) may establish a molar ratio of the components in the synthesis gas by adjusting at least one of (i) a cathode material and (ii) a surface morphology of the cathode. Step (C) may separate the synthesis gas from the solution.
摘要翻译：公开了一种从二氧化碳电化学生产合成气的方法。该方法通常包括步骤（A）至（C）。步骤（A）可以使二氧化碳在电解槽中分解成电解质和催化剂的溶液。分隔的电化学电池可以包括第一电池室中的阳极和第二电池室中的阴极。阴极通常将二氧化碳减少为多个组分。步骤（B）可以通过调节（i）阴极材料和（ii）阴极的表面形态中的至少一个来建立合成气中的组分的摩尔比。步骤（C）可将合成气与溶液分离。

7. 发明申请

WO2010088524A3 CONVERSION OF CARBON DIOXIDE TO ORGANIC PRODUCTS 审中-公开
标题翻译：二氧化碳转化为有机产品
公开(公告)号：WO2010088524A3
公开(公告)日：2011-03-10
申请号：PCT/US2010022594
申请日：2010-01-29
申请人： UNIV PRINCETON , BOCARSLY ANDREW B , COLE EMILY BARTON
发明人： BOCARSLY ANDREW B , COLE EMILY BARTON
IPC分类号： C07C27/26
CPC分类号： C25B3/04 , C25B1/003 , C25B9/08 , Y02P20/134 , Y02P20/135
摘要： The invention relates to various embodiments of an environmentally beneficial method for reducing carbon dioxide. The methods in accordance with the invention include electrochemically or photoelectrochemically reducing the carbon dioxide in a divided electrochemical cell that includes an anode, e.g., an inert metal counterelectrode, in one cell compartment and a metal or p-type semiconductor cathode electrode in another cell compartment that also contains an aqueous solution of an electrolyte and a catalyst of one or more substituted or unsubstituted aromatic amines to produce therein a reduced organic product.
摘要翻译：本发明涉及减少二氧化碳的环境有益的方法的各种实施方案。根据本发明的方法包括电化学或光电化学还原分离的电化学电池中的二氧化碳，其包括在一个电池室中的阳极，例如惰性金属反电极，以及另一电池室中的金属或p型半导体阴极电极其还含有电解质的水溶液和一种或多种取代或未取代的芳族胺的催化剂，以在其中产生还原的有机产物。

8. 发明申请

WO2010088524A2 CONVERSION OF CARBON DIOXIDE TO ORGANIC PRODUCTS 审中-公开
标题翻译：二氧化碳转化为有机产品
公开(公告)号：WO2010088524A2
公开(公告)日：2010-08-05
申请号：PCT/US2010/022594
申请日：2010-01-29
申请人： PRINCETON UNIVERSITY , BOCARSLY, Andrew, B. , COLE, Emily Barton
发明人： BOCARSLY, Andrew, B. , COLE, Emily Barton
IPC分类号： C25B3/00 , C25B9/00
CPC分类号： C25B3/04 , C25B1/003 , C25B9/08 , Y02P20/134 , Y02P20/135
摘要： The invention relates to various embodiments of an environmentally beneficial method for reducing carbon dioxide. The methods in accordance with the invention include electrochemically or photoelectrochemically reducing the carbon dioxide in a divided electrochemical cell that includes an anode, e.g., an inert metal counterelectrode, in one cell compartment and a metal or p-type semiconductor cathode electrode in another cell compartment that also contains an aqueous solution of an electrolyte and a catalyst of one or more substituted or unsubstituted aromatic amines to produce therein a reduced organic product.
摘要翻译：本发明涉及减少二氧化碳的环境有益的方法的各种实施方案。根据本发明的方法包括电化学或光电化学还原分离的电化学电池中的二氧化碳，其包括在一个电池室中的阳极，例如惰性金属反电极，以及另一电池室中的金属或p型半导体阴极电极其还含有电解质的水溶液和一种或多种取代或未取代的芳族胺的催化剂，以在其中产生还原的有机产物。

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