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1. 发明申请

WO2008147546A1 CATALYST FOR CONVERSION OF HYDROCARBONS, PROCESS OF MAKING AND PROCESS OF USING THEREOF - INCORPORATION-2 审中-公开
标题翻译：碳氢化合物转化催化剂，其制备方法及其使用方法 - INCORPORATION-2
公开(公告)号：WO2008147546A1
公开(公告)日：2008-12-04
申请号：PCT/US2008/006638
申请日：2008-05-23
申请人： SAUDI BASIC INDUSTRIES CORPORATION , MITCHELL, Scott, F. , KHANMAMEDOVA, Alla, K. , STEVENSON, Scott, A. , VARTULI, Jim
发明人： MITCHELL, Scott, F. , KHANMAMEDOVA, Alla, K. , STEVENSON, Scott, A. , VARTULI, Jim
IPC分类号： B01J29/04
CPC分类号： B01J29/89 , B01J29/047 , B01J29/064 , B01J29/068 , B01J29/072 , B01J29/405 , B01J29/42 , B01J29/44 , B01J29/46 , B01J29/48 , B01J29/82 , B01J29/83 , B01J29/84 , B01J29/85 , B01J29/86 , B01J29/88 , B01J2229/18 , B01J2229/186 , C07C1/20 , C07C2/24 , C07C2/66 , C07C2/76 , C07C6/123 , C07C6/126 , C07C2529/44 , C10G3/47 , C10G3/49 , C10G11/05 , C10G25/03 , C10G35/065 , C10G35/085 , C10G45/10 , C10G45/12 , C10G45/62 , C10G45/64 , C10G47/16 , C10G47/18 , C10G50/00 , C10G2300/1081 , C10G2300/1088 , C10G2400/20 , C10G2400/30 , C07C15/02
摘要： This Invention is for a catalyst for conversion of hydrocarbons. The catalyst contains a zeolite with one element from Group 13, Group 14, or the first series transition metals and, optionally, germanium and/or aluminum In the zeolite framework. At least one Group 10 metal, such as platinum, Is deposited on the zeolite. Examples of the elements in the framework are tin, boron, iron or titanium. The catalyst is prepared by synthesizing a zeolite with one element from Group 13, Group 14, or the first series transition metals and, optionally, germanium and/or aluminum in the zeolite framework; depositing the metal; and calcining after preparation of the zeolite and before or after depositing the metal.
摘要翻译：本发明是用于烃转化的催化剂。该催化剂含有沸石，该沸石具有来自组13，组14或第一系列过渡金属以及任选的锗和/或铝的一种元素。在沸石上沉积至少一种第10族金属，例如铂。框架中的元素的实例是锡，硼，铁或钛。通过在沸石骨架中合成具有来自第13族，第14族或第一系列过渡金属和任选的锗和/或铝的一种元素的沸石来制备催化剂; 沉积金属; 并在制备沸石之后和在沉积金属之前或之后煅烧。

2. 发明申请

WO2008147543A1 CATALYST FOR CONVERSION OF HYDROCARBONS, PROCESS OF MAKING AND PROCESS OF USING THEREOF - INCORPORATION-1 审中-公开
标题翻译：碳氢化合物转化催化剂，其制备方法及其使用方法 - INCORPORATION-1
公开(公告)号：WO2008147543A1
公开(公告)日：2008-12-04
申请号：PCT/US2008/006631
申请日：2008-05-23
申请人： SAUDI BASIC INDUSTRIES CORPORATION , KHANMAMEDOVA, Alla, K. , STEVENSON, Scott, A. , MITCHELL, Scott, F. , FARMER, Dustin, B. , VARTULI, Jim
发明人： KHANMAMEDOVA, Alla, K. , STEVENSON, Scott, A. , MITCHELL, Scott, F. , FARMER, Dustin, B. , VARTULI, Jim
IPC分类号： B01J29/04
CPC分类号： C07C1/20 , B01J29/047 , B01J29/405 , B01J29/44 , B01J29/86 , B01J2229/183 , B01J2229/186 , C07C2/24 , C07C2/66 , C07C2/76 , C07C6/08 , C07C6/123 , C07C6/126 , C07C2521/02 , C07C2523/04 , C07C2523/14 , C07C2523/58 , C07C2523/62 , C07C2529/44 , C07C2529/86 , C10G1/04 , C10G11/05 , C10G25/03 , C10G35/085 , C10G35/095 , C10G45/00 , C10G45/10 , C10G45/12 , C10G45/62 , C10G45/64 , C10G47/18 , C10G50/00 , C10G2400/20 , C10G2400/30 , Y02P30/42 , C07C15/02
摘要： This invention is for a catalyst for conversion of hydrocarbons. The catalyst contains a zeolite having germanium and at least one selected from the group consisting of tin and boron incorporated into the zeolite framework and at least one metal selected from Group 10 deposited on the zeolite. The catalyst is prepared by synthesizing a zeolite having germanium and at least one selected from the group consisting of tin and boron incorporated into the zeolite framework; depositing the metal; and calcining after preparation of the zeolite and before or after depositing the metal. The catalyst may be used in a process for the conversion of hydrocarbons, such as propane to aromatics, by contacting the catalyst with alkanes having 2 to 12 carbon atoms per molecule and recovering the product.
摘要翻译：本发明是用于烃转化的催化剂。催化剂含有具有锗的沸石和选自掺入沸石骨架中的锡和硼中的至少一种和选自沉积在沸石上的组10中的至少一种金属。催化剂通过合成具有锗的沸石和掺入沸石骨架中的选自锡和硼中的至少一种来制备; 沉积金属; 并在制备沸石之后和在沉积金属之前或之后煅烧。催化剂可用于通过使催化剂与每分子具有2至12个碳原子的烷烃接触并回收产物来将烃类如丙烷转化成芳族化合物的方法。

3. 发明申请

WO2008091593A1 PROCESS OF USING ZEOLITE CATALYST FOR HYDROCARBON CONVERSION 审中-公开
标题翻译：使用沸石催化剂进行碳氢转化的方法
公开(公告)号：WO2008091593A1
公开(公告)日：2008-07-31
申请号：PCT/US2008/000807
申请日：2008-01-22
申请人： SAUDI BASIC INDUSTRIES CORPORATION , JUTTU, Gopalakrishnan, G. , SMITH, Robert, Scott
发明人： JUTTU, Gopalakrishnan, G. , SMITH, Robert, Scott
IPC分类号： B01J29/42
CPC分类号： B01J29/04 , B01J2229/20 , B01J2229/42 , C07C2/76 , C07C2529/74 , C07C15/00
摘要： This invention is for a catalyst for conversion of a hydrocarbonaceous feed. The catalyst is a zeolite aluminosilicate with a silicon to aluminum molar ratio from about 70: 1 to about 100: 1 on which a noble metal has been deposited. The zeolite catalyst may contain other optional tetravalent and trivalent elements in the zeolite framework. The zeolite structure may be MFI, FAU, TON, MFL, VPI, MEL, AEL, AFI, MWW or MOR. The catalyst is synthesized by preparing a zeolite containing aluminum, silicon and, optionally, other elements, such as germanium, in the framework, depositing a noble metal, such as platinum, on the zeolite and calcining the zeolite. The catalyst may be used for aromatization of alkanes to aromatics. One embodiment is a MFI zeolite catalyst which may be used for the aromatization of alkanes having two to six carbon atoms per molecule to aromatics, such as benzene, toluene and xylenes.
摘要翻译：本发明是用于烃类进料转化的催化剂。该催化剂是一种硅铝酸盐沸石，其硅与铝的摩尔比为约70:1至约100:1，其上沉积有贵金属。沸石催化剂可以在沸石骨架中含有其它任选的四价和三价元素。沸石结构可以是MFI，FAU，TON，MFL，VPI，MEL，AEL，AFI，MWW或MOR。通过在骨架中制备含有铝，硅和任选的其它元素如锗的沸石来合成催化剂，在沸石上沉积贵金属如铂，并煅烧沸石。催化剂可用于将烷烃芳构化成芳族化合物。一个实施方案是MFI沸石催化剂，其可用于每分子具有2-6个碳原子的芳族化合物与芳族化合物如苯，甲苯和二甲苯的芳族化。

4. 发明申请

WO2007130142A1 PROCESS FOR SYNTHESIZING A HETEROPOLY ACID CATALYST FOR OXIDATION OF UNSATURATED ALDEHYDES TO UNSATURATED CARBOXYLIC ACID 审中-公开
标题翻译：合成用于将不饱和醛类氧化成不饱和羧酸的异戊酸催化剂的方法
公开(公告)号：WO2007130142A1
公开(公告)日：2007-11-15
申请号：PCT/US2006/049374
申请日：2006-12-28
申请人： SAUDI BASIC INDUSTRIES CORPORATION , KAUFFMAN, James, W. , CAI, Lixia , LIANG, Wugeng
发明人： KAUFFMAN, James, W. , CAI, Lixia , LIANG, Wugeng
IPC分类号： C07C51/235 , B01J27/192
CPC分类号： B01J37/031 , B01J27/192 , B01J27/199 , C07C51/252 , C07C57/04
摘要： The present invention is for a process for making a heteropoly acid compound catalyst for oxidation of unsaturated aldehydes, such as methacrolein, to unsaturated carboxylic acids, such as methacrylic acid, said catalyst containing oxides of molybdenum, phosphorus, and M', wherein M' is cesium, potassium, rubidium, or sodium and bismuth. The process is a synthesis of the catalyst with specific process conditions for addition of the bismuth compound as an aqueous slurry without nitric acid. A catalyst precursor is formed by removing the water and drying the solid particles. The heteropoly acid compound catalyst is formed by calcination of the catalyst precursor.
摘要翻译：本发明涉及制备用于将不饱和醛如甲基丙烯醛氧化的杂多酸化合物催化剂转化为不饱和羧酸如甲基丙烯酸，所述催化剂含有钼，磷和M'的氧化物的方法，其中M' 是铯，钾，铷或钠和铋。该方法是具有特定工艺条件的催化剂的合成，用于加入铋化合物作为无硝酸的含水浆液。通过除去水并干燥固体颗粒来形成催化剂前体。通过煅烧催化剂前体形成杂多酸化合物催化剂。

5. 发明申请

WO2007014207A2 CATALYST FOR METHACROLEIN OXIDATION AND METHOD FOR MAKING AND USING SAME 审中-公开
标题翻译：甲基丙烯酸氧化催化剂及其制备和使用方法
公开(公告)号：WO2007014207A2
公开(公告)日：2007-02-01
申请号：PCT/US2006/028819
申请日：2006-07-25
申请人： SAUDI BASIC INDUCTRIES CORPORATION , STEVENSON, Scott, A. , LIANG, Wugeng , KAUFFMAN, James, W. , CAI, Lixia , MCGUFFEY, Angie , LINZER, Joseph, R.
发明人： STEVENSON, Scott, A. , LIANG, Wugeng , KAUFFMAN, James, W. , CAI, Lixia , MCGUFFEY, Angie , LINZER, Joseph, R.
IPC分类号： B01J27/00 , B01J27/198 , B01J27/188 , B01J27/19 , C07C51/16
CPC分类号： B01J27/188 , B01J23/002 , B01J27/199 , B01J35/10 , B01J35/1061 , B01J35/1066 , B01J2523/00 , C07C51/252 , C07C57/04 , B01J2523/15 , B01J2523/17 , B01J2523/305 , B01J2523/51 , B01J2523/53 , B01J2523/54 , B01J2523/55 , B01J2523/68
摘要： A catalyst for oxidation of unsaturated and/or saturated aldehyde to unsaturated acids is disclosed where the catalyst including at least molybdenum (Mo), phosphorus (P), vanadium (V), bismuth (Bi), and a first component selected from the group consisting of potassium (K), rubidium (Rb), cesium (Cs), thallium (Tl), or mixtures or combinations thereof, where the catalyst has at least 57% medium pores and a nitric acid to molybdenum mole ratio of at least 0.5:1 or at least 6.0:1 moles of HNO 3 per mole of Mo 12- Methods for making and using such catalysts are also disclosed.
摘要翻译：公开了至少包含钼（Mo），磷（P），钒（V），铋（Bi），氧化铋和选自钾（K），铷（Rb），铯（Cs），铊（Tl）或其混合物或组合的第一组分，其中催化剂具有至少57％的中孔和硝酸与钼摩尔比至少为0.5:1或至少为6.0:1摩尔HNO 3 /摩尔Mo 12 - 还公开了制备和使用这种催化剂的方法

6. 发明申请

WO2006004840A3 PROCESS FOR THE SELECTIVE CONVERSION OF ALKANES TO UNSATURATED CARBOXYLIC ACIDS 审中-公开
公开(公告)号：WO2006004840A3
公开(公告)日：2006-01-12
申请号：PCT/US2005/023121
申请日：2005-06-30
申请人： SAUDI BASIC INDUSTRIES CORPORATION , HAZIN, Paulette, N.
发明人： HAZIN, Paulette, N.
IPC分类号： C07C51/16
摘要： The invention disclosed is a process for the selective conversion of an alkane to an unsaturated carboxylic acid in a one-step process with a mixed metal oxide catalyst composition having the general formula: MOV a Nb b Te c Sb d M e O X wherein M is optional and may be one or more selected from silver, silicon, sulfur, zirconium, titanium, aluminum, copper, lithium, sodium, potassium, rubidium, cesium, gallium, phosphorus, iron, rhenium, cobalt, chromium, manganese, arsenic, indium, thallium, bismuth, germanium, tin, cerium or lanthanum. This catalyst may be prepared by co-precipitation of metal compounds which are calcined to form a mixed metal oxide catalyst.

7. 发明申请

WO2005094506A2 CATALYST COMPOSITION FOR THE SELECTIVE CONVERSION OF ALKANES TO UNSATURATED CARBOXYLIC ACIDS, METHOD OF MAKING AND METHOD OF USING THEREOF 审中-公开
标题翻译：烷基羧酸选择性转化为不饱和羧酸的催化剂组合物，制备方法及其使用方法
公开(公告)号：WO2005094506A2
公开(公告)日：2005-10-13
申请号：PCT/US2005/009732
申请日：2005-03-23
申请人： SAUDI BASIC INDUSTRIES CORPORATION , HAZIN, Paulette, N. , ELLIS, Paul, E., Jr.
发明人： HAZIN, Paulette, N. , ELLIS, Paul, E., Jr.
IPC分类号： B01J23/00 , B01J23/08 , B01J23/18 , B01J23/20 , B01J23/28 , B01J23/30 , B01J23/31 , B01J23/68 , B01J37/00 , B01J37/02 , C07C51/215 , C07C253/24 , C07C255/08
CPC分类号： B01J23/002 , B01J23/08 , B01J23/18 , B01J23/20 , B01J23/28 , B01J23/30 , B01J23/31 , B01J23/686 , B01J37/0036 , B01J37/0045 , B01J37/009 , B01J37/0236 , B01J2523/00 , C07C51/215 , C07C253/24 , Y02P20/52 , C07C57/04 , C07C255/08 , B01J2523/18 , B01J2523/53 , B01J2523/55 , B01J2523/56 , B01J2523/68 , B01J2523/32 , B01J2523/54 , B01J2523/69 , B01J2523/19
摘要： A catalyst comp sition having the formula: MO l V a Sb b Nb c M d O X wherein M is galliu , bismuth, silver or gold, a is 0.01 to 1, b is 0.01 to c is 0.01 to 1, d is 0.01 to 1 and x is determined by t e valence requirements of the other components. Other metals, such as tantalum, titanium, aluminum, zirconium, chromium, manganese, iron, ruthenium, cobalt, rhodium, nickel, platinum, boron, arsenic, lithium, sodium, po assium, rubidium, calcium, beryllium, magnesium, cerium, strontium, hafnium, phosphorus, europium, gadolin um, dysprosium, holmium, erbium, thulium, terbium, ytterbium, lutetium, lanthanum, scandium, palladiu praseodymium, neodymium, yttrium, thorium, tungsten, esium, zinc, tin, germanium, silicon, lead, barium or th llium may also be components of the catalyst. This ca alyst is prepared by co-precipitation of metal compounds which are calcined to form a mixed metal oxide catalys that can be used for the selective conversion of an al ane to an unsaturated carboxylic acid in a one-step process.
摘要翻译：具有下式的催化剂组成：其中M为胆酸，铋，银或金的MO1VaSbbNbcMdOX，a为0.01至1，b为0.01至c为0.01至1，d为0.01至1，x为其他组件。其他金属如钽，钛，铝，锆，铬，锰，铁，钌，钴，铑，镍，铂，硼，砷，锂，钠，锑，铷，钙，铍，镁，铈，锶，铪，磷，铕，钆，镝，钬，铒，ium，铽，镱，镥，镧，钪，铊，钕，钇，钍，钨，铈，锡，锗，铅，钡或铊也可以是催化剂的组分。金属化合物的共沉淀制备，其被煅烧以形成可用于在一步法中将醛与不饱和羧酸选择性转化的混合金属氧化物催化剂。

8. 发明申请

WO2005085157A1 CATALYST FOR AROMATIZATION OF ALKANES, PROCESS OF MAKING AND USING THEREOF 审中-公开
标题翻译：烷烃芳构化催化剂，制备方法及其用途
公开(公告)号：WO2005085157A1
公开(公告)日：2005-09-15
申请号：PCT/US2005/007403
申请日：2005-03-03
申请人： SAUDI BASIC INDUSTRIES CORPORATION , JUTTU, Gopalakrishnan, G. , SMITH, Robert, Scott
发明人： JUTTU, Gopalakrishnan, G. , SMITH, Robert, Scott
IPC分类号： C07C2/52
CPC分类号： B01J29/87 , B01J23/42 , B01J2229/20 , C07C2/76 , C07C2529/44 , C10G2400/30
摘要： A catalyst of a gallium zeolite on which platinum (Pt/Ga-ZSM-5) has been deposited may be used for aromatization of alkanes having two to six carbon atoms per molecule, such as ethane, propane, butane, etc., to aromatics, such as benzene, toluene and xylenes (BTX). The gallium zeolite contains gallium and silicon in the framework of the zeolite structure. The zeolite structure may be of MFI, FAU, TON, MFL, VPI, MEL, AEL, AFI, MWW or MOR, but preferably, the zeolite has a MFI structure, more preferably is ZSM-5 MFI zeolite. According to the IUPAC recommendations, an example of the sodium form of the zeolite would be represented as: |Na x . (H 2 O) z |[Ga x si y o 2y + 3x/2 ]-MFI where x=0.1-25; y=60-100; and z=0.1-10. Platinum may be deposited on the gallium zeolite by ion exchange or impregnation.
摘要翻译：可以使用其上沉积有铂（Pt / Ga-ZSM-5）的镓沸石的催化剂用于将每分子具有2-6个碳原子的烷烃如乙烷，丙烷，丁烷等芳构化成芳族化合物，如苯，甲苯和二甲苯（BTX）。镓沸石在沸石结构的框架中含有镓和硅。沸石结构可以是MFI，FAU，TON，MFL，VPI，MEL，AEL，AFI，MWW或MOR，但优选沸石具有MFI结构，更优选ZSM-5MFI沸石。根据IUPAC的建议，钠形式的沸石的例子将被表示为：|| Nax。（H2O）z || [Gax siyo2y + 3x / 2] -MFI其中x = 0.1-25; Y = 60-100; z = 0.1-10。铂可以通过离子交换或浸渍沉积在镓沸石上。

9. 发明申请

WO2011044037A1 PHOSPHORUS-CONTAINING ZEOLITE CATALYSTS AND THEIR METHOD OF PREPARATION 审中-公开
标题翻译：含磷的沸石催化剂及其制备方法
公开(公告)号：WO2011044037A1
公开(公告)日：2011-04-14
申请号：PCT/US2010/051309
申请日：2010-10-04
申请人： SAUDI BASIC INDUSTRIES CORPORATION , GHOSH, Ashim, Kumar , KULKARNI, Neeta , HARVEY, Pamela
发明人： GHOSH, Ashim, Kumar , KULKARNI, Neeta , HARVEY, Pamela
IPC分类号： B01J29/00 , B01J29/04 , B01J29/06
CPC分类号： B01J37/28 , B01J29/06 , B01J29/40 , B01J35/1038 , B01J37/0009 , B01J37/0201 , B01J37/04 , B01J37/06 , B01J37/10 , B01J2229/36 , B01J2229/37 , B01J2229/42 , C07C2/864 , C07C2529/40 , Y02P20/52 , C07C15/08
摘要： A zeolite catalyst that may be used in aromatic alkylation is prepared by treating a zeolite with a phosphorus compound. The phosphorus-treated zeolite is calcined and contacted with liquid water, whereby an amount of phosphorus is removed from the phosphorus-treated zeolite. The phosphorus -treated zeolite is then heated. A method of preparing an aromatic product may also be carried out by contacting the prepared zeolite catalyst with an aromatic alkylation feed of an aromatic compound and an alkylating agent under reaction conditions suitable for aromatic alkylation.
摘要翻译：可用于芳族烷基化的沸石催化剂通过用磷化合物处理沸石来制备。将磷处理的沸石煅烧并与液态水接触，由此从磷处理的沸石中除去一定量的磷。然后加热磷处理的沸石。制备芳香族产物的方法也可以通过使制备的沸石催化剂与芳族化合物和烷基化剂的芳族烷基化进料在适于芳族烷基化反应的条件下接触来进行。

10. 发明申请

WO2010121006A1 A PROCESS FOR PRODUCING AN UNSATURATED CARBOXYLIC ACID FROM AN ALKANE 审中-公开
标题翻译：一种从烷烃生产不饱和羧酸的方法
公开(公告)号：WO2010121006A1
公开(公告)日：2010-10-21
申请号：PCT/US2010/031206
申请日：2010-04-15
申请人： SAUDI BASIC INDUSTRIES CORPORATION , HAZIN, Paulette, N. , GALLOWAY, Frederick, Merrill , LEDFORD, John, S. , NUYEN, Andy, H.
发明人： HAZIN, Paulette, N. , GALLOWAY, Frederick, Merrill , LEDFORD, John, S. , NUYEN, Andy, H.
IPC分类号： C07C51/16
CPC分类号： B01J23/002 , B01J23/686 , B01J27/0576 , B01J37/0045 , B01J2523/00 , C07C51/215 , Y02P20/582 , C07C57/04 , B01J2523/53 , B01J2523/55 , B01J2523/56 , B01J2523/64 , B01J2523/68 , B01J2523/18
摘要： A one-step vapor phase oxidation process produces an unsaturated carboxylic acid, such as acrylic acid or methacrylic acid, from an alkane, such as propane or isobutane, with a mixed metal oxide catalyst and an excess of alkane relative to oxygen. The unreacted alkane and the byproduct alkene are recycled to the reaction zone without separation. Overall yield and productivity of the unsaturated carboxylic improves for such a process. An analogous method for the preparation of unsaturated nitrites is also disclosed.
摘要翻译：一步气相氧化法由烷烃如丙烷或异丁烷与混合的金属氧化物催化剂和过量的烷烃相对于氧气产生不饱和羧酸，如丙烯酸或甲基丙烯酸。未反应的烷烃和副产物烯烃不分离地再循环到反应区。对于这种方法，不饱和羧酸的总产率和生产率提高。还公开了用于制备不饱和亚硝酸盐的类似方法。

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