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1. 发明授权

US09938144B2 Process for producing synthesis gas and electrical energy 有权
公开(公告)号：US09938144B2
公开(公告)日：2018-04-10
申请号：US14827496
申请日：2015-08-17
申请人： LINDE AKTIENGESELLSCHAFT , BASF SE
发明人： Hans-Jurgen Maass , Otto Machhammer , Andreas Bode , Grigorios Kolios
IPC分类号： C01B3/30 , C01B31/18 , C01B3/24 , C01B3/28 , C10J3/18 , C10J3/20 , C10K3/02
CPC分类号： C01B3/30 , C01B3/24 , C01B3/28 , C01B32/40 , C01B2203/0216 , C01B2203/0272 , C01B2203/061 , C01B2203/062 , C01B2203/0822 , C01B2203/0838 , C01B2203/085 , C01B2203/1235 , C01B2203/148 , C01B2203/84 , C10J3/18 , C10J3/20 , C10K3/026 , Y02P20/128 , Y02P20/129 , Y02P20/146
摘要： The invention relates to a process for producing synthesis gas, in which carbon and hydrogen are obtained from hydrocarbon by thermal decomposition. At least a portion of the carbon obtained by the thermal decomposition is reacted, and at least a portion of the hydrogen obtained is reacted with carbon dioxide by a reverse water-gas shift reaction to give carbon monoxide and water. Carbon obtained by the thermal hydrocarbon decomposition is used as fuel in a power plant operation wherein the carbon is combusted to produce electrical power, and carbon dioxide formed in the combustion of the carbon is used in the reverse water-gas shift reaction.

2. 发明申请

US20150321912A1 METHOD FOR PERFORMING ENDOTHERMIC PROCESSES 审中-公开
标题翻译：执行内热过程的方法
公开(公告)号：US20150321912A1
公开(公告)日：2015-11-12
申请号：US14651862
申请日：2013-12-12
申请人： BASF SE , LINDE AG
发明人： Otto MACHHAMMER , Wolfgang Alois HORMUTH , Christian SCHNEIDER , Andreas BODE , Volker GOEKE , Hans-Juergen MASS , Matthias KERN , Dirk KLINGLER , Rene KOENIG , Philipp BRUEGGEMANN , Jens BERNNAT , Grigorios KOLIOS
IPC分类号： C01B3/28
CPC分类号： C01B3/28 , B01J8/00 , B01J19/00 , B01J2208/00415 , B01J2219/00135 , C01B2203/0272 , C01B2203/0866
摘要： The invention relates to a method of carrying out heat-consuming processes, wherein the total energy required averaged over a year for the heat-consuming process originates from at least two different energy sources, where one of the energy sources is an electric energy source whose power varies in the range from 0 to 100% of the total power required, and three different energy modes can individually provide the total power required for the heat-consuming process: (i) exclusively electric energy, (ii) a mixture of electric energy and at least one further nonelectric energy source or (iii) exclusively nonelectric energy, where the changeover time in which the change from one energy mode to another energy mode is completed is not more than 30 minutes.
摘要翻译：本发明涉及一种进行耗热过程的方法，其中对于耗热过程而言，平均一年以上的总能量源自至少两个不同的能源，其中一个能量源是电能源，功率在所需总功率的0至100％的范围内变化，并且三种不同的能量模式可以单独地提供耗散过程所需的总功率：（i）专用电能，（ii）电能的混合和至少一个另外的非电能源，或者（iii）唯一的非电能，其中从一个能量模式到另一个能量模式的改变的转换时间不超过30分钟。

3. 发明申请

US20070111051A1 Thermocatalytic process for CO2-free production of hydrogen and carbon from hydrocarbons 有权
标题翻译：用于从碳氢化合物中无CO2生产氢和碳的热催化过程
公开(公告)号：US20070111051A1
公开(公告)日：2007-05-17
申请号：US11648453
申请日：2006-12-29
申请人： Nazim Muradov
发明人： Nazim Muradov
IPC分类号： H01M8/06 , C01B3/26 , B01J19/00 , B01J8/02 , B01J8/00
CPC分类号： H01M8/0631 , B01J8/0055 , B01J8/24 , B01J8/26 , B01J8/28 , B01J8/388 , B01J19/2475 , B01J21/18 , B01J2208/00176 , B01J2208/00256 , B01J2208/00274 , B01J2219/00006 , C01B3/26 , C01B3/28 , C01B3/30 , C01B3/50 , C01B3/501 , C01B3/506 , C01B3/52 , C01B3/56 , C01B32/05 , C01B2203/0277 , C01B2203/04 , C01B2203/0405 , C01B2203/0415 , C01B2203/047 , C01B2203/0475 , C01B2203/048 , C01B2203/066 , C01B2203/0811 , C01B2203/0827 , C01B2203/10 , C01B2203/1041 , C01B2203/1241 , C01B2203/1247 , C01B2203/148 , H01M8/0612 , H01M8/0618 , H01M2008/1095 , Y02P20/584
摘要： This invention relates to a novel process for sustainable CO2-free production of hydrogen and carbon by thermocatalytic decomposition (or dissociation, pyrolysis, cracking) of hydrocarbon fuels over carbon-based catalysts in the absence of air and/or water. The process is applicable to any hydrocarbon fuel, including sulfurous fuels. Combination of a catalytic reactor with a gas separation unit allows to produce high purity hydrogen (at least, 99.0 v%) completely free of carbon oxides. In a preferred embodiment, sustainable continuous production of hydrogen and carbon is achieved by both internal and external activation of carbon catalysts. Internal activation of carbon catalyst is accomplished by recycling of hydrogen-depleted gas containing unsaturated and aromatic hydrocarbons back to the reactor. External activation can be achieved via surface gasification of carbon catalysts by hot combustion gases during catalyst heating. The process can conveniently be integrated with any type of fuel cell.
摘要翻译：本发明涉及一种通过在不存在空气的情况下通过碳基催化剂的烃燃料的热分解（或解离，裂解，裂化）来生产氢和碳的可持续的无CO 2的新方法，以及 /或水。该方法适用于任何碳氢燃料，包括含硫燃料。催化反应器与气体分离单元的组合允许产生完全不含碳氧化物的高纯度氢（至少99.0v％）。在优选的实施方案中，通过碳催化剂的内部和外部活化来实现可持续的氢和碳的连续生产。碳催化剂的内部活化是通过将含有不饱和烃和芳族烃的贫氢气回流回反应器来完成的。可以通过在催化剂加热期间通过热燃烧气体的碳催化剂的表面气化来实现外部活化。该方法可以方便地与任何类型的燃料电池集成。

4. 发明授权

US07157167B1 Thermocatalytic process for CO2-free production of hydrogen and carbon from hydrocarbons 有权
标题翻译：用于从碳氢化合物中无CO2生产氢和碳的热催化过程
公开(公告)号：US07157167B1
公开(公告)日：2007-01-02
申请号：US10683603
申请日：2003-10-10
申请人： Nazim Z. Muradov
发明人： Nazim Z. Muradov
IPC分类号： H01M8/18 , B01J8/00 , C01B3/26
CPC分类号： H01M8/0631 , B01J8/0055 , B01J8/24 , B01J8/26 , B01J8/28 , B01J8/388 , B01J19/2475 , B01J21/18 , B01J2208/00176 , B01J2208/00256 , B01J2208/00274 , B01J2219/00006 , C01B3/26 , C01B3/28 , C01B3/30 , C01B3/50 , C01B3/501 , C01B3/506 , C01B3/52 , C01B3/56 , C01B32/05 , C01B2203/0277 , C01B2203/04 , C01B2203/0405 , C01B2203/0415 , C01B2203/047 , C01B2203/0475 , C01B2203/048 , C01B2203/066 , C01B2203/0811 , C01B2203/0827 , C01B2203/10 , C01B2203/1041 , C01B2203/1241 , C01B2203/1247 , C01B2203/148 , H01M8/0612 , H01M8/0618 , H01M2008/1095 , Y02P20/584
摘要： A novel process and apparatus are disclosed for sustainable CO2-free production of hydrogen and carbon by thermocatalytic decomposition (dissociation, pyrolysis, cracking) of hydrocarbon fuels over carbon-based catalysts in the absence of air and/or water. The apparatus and thermocatalytic process improve the activity and stability of carbon catalysts during the thermocatalytic process and produce both high purity hydrogen (at least, 99.0 volume %) and carbon, from any hydrocarbon fuel, including sulfurous fuels. In a preferred embodiment, production of hydrogen and carbon is achieved by both internal and external activation of carbon catalysts. Internal activation of carbon catalyst is accomplished by recycling of hydrogen-depleted gas containing unsaturated and aromatic hydrocarbons back to the reactor. External activation of the catalyst can be achieved via surface gasification with hot combustion gases during catalyst heating. The process and apparatus can be conveniently integrated with any type of fuel cell to generate electricity.
摘要翻译：公开了一种新颖的方法和装置，用于在不存在空气和/或气体的情况下通过碳基催化剂的碳氢化合物燃料的热分解（解离，热解，裂化）来生产氢和碳，从而可持续地不产生CO 2，或水。该装置和热催化方法提高了碳催化剂在热催化过程中的活性和稳定性，并且从任何烃燃料（包括亚硫燃料）产生高纯度氢（至少99.0体积％）和碳。在优选的实施方案中，氢和碳的生产通过碳催化剂的内部和外部活化来实现。碳催化剂的内部活化是通过将含有不饱和烃和芳族烃的贫氢气回流回反应器来完成的。催化剂的外部活化可以通过在催化剂加热期间用热燃烧气体进行表面气化来实现。该方法和设备可以方便地与任何类型的燃料电池集成以发电。

5. 发明申请

US20040253168A1 System and method for hydrocarbon processing 审中-公开
标题翻译：烃加工的系统和方法
公开(公告)号：US20040253168A1
公开(公告)日：2004-12-16
申请号：US10830594
申请日：2004-04-23
发明人： Xi Chu
IPC分类号： C01B031/02 , B32B005/02 , F28D001/00 , G01N033/00 , G01N027/00
CPC分类号： H01M4/624 , B01J21/18 , B01J35/0013 , B82Y30/00 , B82Y40/00 , C01B3/26 , C01B3/28 , C01B3/386 , C01B32/15 , C01B2203/0261 , C01B2203/0277 , C01B2203/066 , C01B2203/085 , C01B2203/1041 , H01M4/587 , H01M8/0643 , H01M8/1009 , H01M10/0525 , Y02P20/134 , Y02P20/52
摘要： This patent discloses a system and method of producing nanostructured carbon and carbon monoxide-free hydrogen through the decomposition of hydrocarbons in a spouted bed reactor. The process is precisely controlled in such a way that the carbon particles generated in reaction has a unique nanostructure so their surfaces can act as catalytic sites for the decomposition of hydrocarbons. The process produces hydrogen stream containing no carbon monoxide, and The CO-free hydrogen is ideal fuel for fuel cells (especially the PEM) and many industrial chemical syntheses. The generated nanostructured carbon can be used as catalyst for the processing of hydrocarbons such as hydrogenation, dehydrogenation and partial oxidation of hydrocarbon chemicals. In addition, the nanostructured carbon produced can be used as electrode material for electrochemical energy conversation and storage and industrial electrochemical processes, fuel for the direct carbon fuel cell, and fillers of medical implants and components.
摘要翻译：该专利公开了一种通过喷射床反应器中的烃的分解来生产纳米结构碳和一氧化碳的氢的系统和方法。该方法被精确控制，使得反应中产生的碳颗粒具有独特的纳米结构，使得它们的表面可以作为烃分解的催化位点。该过程产生不含一氧化碳的氢气流，而无CO的燃料是燃料电池（特别是PEM）和许多工业化学合成的理想燃料。生成的纳米结构碳可用作烃类加工的催化剂，如烃类化学品的氢化，脱氢和部分氧化。另外，所生产的纳米结构碳可用作电化学能量对话和存储以及工业电化学工艺的电极材料，用于直接碳燃料电池的燃料，以及医疗植入物和组分的填料。

6. 发明授权

US3284161A Method for hydrogen production by catalytic decomposition of a gaseous hydrocarbon stream 失效
标题翻译：通过气态烃流的催化分解制氢的方法
公开(公告)号：US3284161A
公开(公告)日：1966-11-08
申请号：US25308563
申请日：1963-01-22
申请人： UNIVERSAL OIL PROD CO
发明人： POHLENZ JACK B , SCOTT NORMAN H
IPC分类号： C01B3/28 , C01B3/30 , C01B3/40 , C01B3/42 , C01B3/44
CPC分类号： C01B3/42 , C01B3/28 , C01B3/30 , C01B3/40 , C01B3/44 , C01B2203/0277 , C01B2203/0465 , C01B2203/0811 , C01B2203/1047 , C01B2203/1052 , C01B2203/1241

7. 发明授权

US09359200B2 Method for the parallel production of hydrogen and carbon-containing products 有权
标题翻译：并联生产氢和含碳产品的方法
公开(公告)号：US09359200B2
公开(公告)日：2016-06-07
申请号：US14131124
申请日：2012-07-05
申请人： Hans-Juergen Maass , Volker Goeke , Otto Machhammer , Marcus Guzmann , Christian Schneider , Wolfgang Alois Hormuth , Andreas Bode , Dirk Klingler , Matthias Kern , Grigorios Kolios
发明人： Hans-Juergen Maass , Volker Goeke , Otto Machhammer , Marcus Guzmann , Christian Schneider , Wolfgang Alois Hormuth , Andreas Bode , Dirk Klingler , Matthias Kern , Grigorios Kolios
IPC分类号： C01B3/24 , C01B31/02 , C01B3/28 , C01B3/30 , C10B57/00
CPC分类号： C01B3/24 , C01B3/28 , C01B3/30 , C01B32/05 , C01B2203/0272 , C01B2203/04 , C01B2203/0425 , C01B2203/0485 , C01B2203/049 , C01B2203/06 , C01B2203/0805 , C01B2203/0811 , C01B2203/0822 , C01B2203/0827 , C01B2203/0866 , C01B2203/1235 , C01B2203/1258 , C10B57/005 , Y02P20/128
摘要： The invention relates to a process for parallel preparation of hydrogen and one or more carbonaceous products, in which hydrocarbons are introduced into a reaction space (R) and decomposed thermally to carbon and hydrogen in the presence of carbon-rich pellets (W). It is a feature of the invention that at least a portion of the thermal energy required for the hydrocarbon decomposition is introduced into the reaction space (R) by means of a gaseous heat carrier.
摘要翻译：本发明涉及氢和一种或多种碳质产物的并行制备方法，其中在富含碳的颗粒（W）的存在下，将烃引入反应空间（R）并热分解成碳和氢。本发明的一个特征是烃分解所需的热能的至少一部分通过气态热载体引入反应空间（R）。

8. 发明申请

US20020007594A1 Thermocatalytic process for CO2-free production of hydrogen and carbon from hydrocarbons 失效
标题翻译：用于从碳氢化合物中无CO2生产氢和碳的热催化过程
公开(公告)号：US20020007594A1
公开(公告)日：2002-01-24
申请号：US09824437
申请日：2001-04-02
发明人： Nazim Z. Muradov
IPC分类号： B01J007/00 , C01B031/02 , B01J003/00 , C10J003/00
CPC分类号： H01M8/0631 , B01J8/0055 , B01J8/24 , B01J8/26 , B01J8/28 , B01J8/388 , B01J19/2475 , B01J21/18 , B01J2208/00176 , B01J2208/00256 , B01J2208/00274 , B01J2219/00006 , C01B3/26 , C01B3/28 , C01B3/30 , C01B3/50 , C01B3/501 , C01B3/506 , C01B3/52 , C01B3/56 , C01B32/05 , C01B2203/0277 , C01B2203/04 , C01B2203/0405 , C01B2203/0415 , C01B2203/047 , C01B2203/0475 , C01B2203/048 , C01B2203/066 , C01B2203/0811 , C01B2203/0827 , C01B2203/10 , C01B2203/1041 , C01B2203/1241 , C01B2203/1247 , C01B2203/148 , H01M8/0612 , H01M8/0618 , H01M2008/1095 , Y02P20/584
摘要： This invention relates to a novel process for sustainable CO2-free production of hydrogen and carbon by thermocatalytic decomposition (or dissociation, pyrolysis, cracking) of hydrocarbon fuels over carbon-based catalysts in the absence of air and/or water. The process is applicable to any hydrocarbon fuel, including sulfurous fuels. Combination of a catalytic reactor with a gas separation unit allows to produce high purity hydrogen (at least, 99.0 v %) completely free of carbon oxides. In a preferred embodiment, sustainable continuous production of hydrogen and carbon is achieved by both internal and external activation of carbon catalysts. Internal activation of carbon catalyst is accomplished by recycling of hydrogen-depleted gas containing unsaturated and aromatic hydrocarbons back to the reactor. External activation can be achieved via surface gasification of carbon catalysts by hot combustion gases during catalyst heating. The process can conveniently be integrated with any type of fuel cell.
摘要翻译：本发明涉及一种用于在不存在空气和/或水的情况下通过碳基催化剂的碳氢化合物燃料的热分解（或解离，热解，裂解）来可持续地无碳氧化生产氢和碳的新方法。该方法适用于任何碳氢燃料，包括含硫燃料。催化反应器与气体分离单元的组合允许产生完全不含碳氧化物的高纯度氢（至少99.0v％）。在优选的实施方案中，通过碳催化剂的内部和外部活化来实现可持续的氢和碳的连续生产。碳催化剂的内部活化是通过将含有不饱和烃和芳族烃的贫氢气回流回反应器来完成的。可以通过在催化剂加热期间通过热燃烧气体的碳催化剂的表面气化来实现外部活化。该方法可以方便地与任何类型的燃料电池集成。

9. 发明授权

US3306707A Hydrogen producing system with hydrocarbon stripping of regenerated catalyst 失效
标题翻译：氢再生催化剂烃生产系统
公开(公告)号：US3306707A
公开(公告)日：1967-02-28
申请号：US29161063
申请日：1963-07-01
申请人： UNIVERSAL OIL PROD CO
发明人： HARDISON LESLIE C
IPC分类号： C01B3/28
CPC分类号： C01B3/28 , C10G11/00 , C10G11/18 , Y02P20/584

10. 发明授权

US3129060A Control of conversion in a catalytic hydrogen producing unit 失效
标题翻译：控制催化氢生产装置中的转化率
公开(公告)号：US3129060A
公开(公告)日：1964-04-14
申请号：US18681762
申请日：1962-04-03
申请人： UNIVERSAL OIL PROD CO
发明人： POHLENZ JACK B
IPC分类号： C01B3/28 , C01B3/42
CPC分类号： C01B3/28 , C01B3/42 , C01B2203/0277 , C01B2203/0465 , C01B2203/0811 , C01B2203/1047 , C01B2203/1052 , C01B2203/1082 , C01B2203/1241 , C01B2203/16 , C01B2203/1623 , C01B2203/1695

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