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1. 发明授权

US5759709A Polymeric fluorescent substance and organic electroluminescence device 失效
标题翻译：聚合物荧光物质和有机电致发光器件
公开(公告)号：US5759709A
公开(公告)日：1998-06-02
申请号：US397489
申请日：1995-03-02
申请人： Shuji Doi , Takanobu Noguchi , Toshihiro Ohnishi , Masamitsu Ishitobi
发明人： Shuji Doi , Takanobu Noguchi , Toshihiro Ohnishi , Masamitsu Ishitobi
IPC分类号： C08G61/00 , C09K11/06 , H01L51/30 , H01L51/50 , H05B33/14
CPC分类号： H05B33/14 , C08G61/00 , C09K11/06 , H01L51/0035 , H01L51/0038 , H01L51/0043 , H01L51/5012 , Y10S428/917 , Y10T428/31504 , Y10T428/31678
摘要： An organic electroluminescence device having at least a light emitting layer between the electrodes consisting of one pair of an anode and a cathode, at least one of which electrodes is transparent or semi-transparent, wherein said light emitting layer comprises a polymeric fluorescent substance which emits a fluorescence in a solid state, is soluble in solvents and comprises at least one kind of repeating unit represented by the following formula (1) and at least one kind of repeating unit represented by the following formula (2) with the number of the formula (1) repeating units being 2-50% of the total number of all the repeating units: --Ar.sub.1 -- (1) --Ar.sub.2 -- (2) wherein Ar.sub.1 and Ar.sub.2 are each a bifunctional group forming a carbon--carbon bond with each of two adjacent groups, in the chemical structure of Ar.sub.1, the number of the consecutive atoms present in the shortest path between the two carbon atoms bonding to said two adjacent groups is 1, 3 or 5, and in the chemical structure of Ar.sub.2, the total number of the carbon and nitrogen atoms present in the shortest path between the two carbon atoms bonding to said two adjacent groups is an even number, and a novel polymeric fluorescent substance used in the above device.
摘要翻译：一种有机电致发光器件，其至少在由一对阳极和阴极组成的电极之间具有至少一个发光层，其中至少一个电极是透明或半透明的，其中所述发光层包括发射的聚合物荧光物质固体荧光可溶于溶剂，并且包含由下式（1）表示的至少一种重复单元和由下式（2）表示的至少一种重复单元，式（1）重复单元占全部重复单元总数的2-50％：-Ar1-（1）-Ar2-（2）其中Ar1和Ar2分别是形成碳 - 碳键的双官能团，两个相邻基团，在Ar1的化学结构中，键合到所述两个相邻基团的两个碳原子之间的最短路径中存在的连续原子的数目是1,3或5，并且在Ar2的化学结构中存在于键合到所述两个相邻基团的两个碳原子之间的最短路径中的碳原子数和氮原子数为偶数，并且在上述装置中使用新颖的聚合物荧光物质。

2. 发明授权

US5980781A Polymeric fluorescent substance and organic electroluminescence device 失效
标题翻译：聚合物荧光物质和有机电致发光器件
公开(公告)号：US5980781A
公开(公告)日：1999-11-09
申请号：US36023
申请日：1998-03-06
申请人： Shuji Doi , Takanobu Noguchi , Toshihiro Ohnishi , Masamitsu Ishitobi
发明人： Shuji Doi , Takanobu Noguchi , Toshihiro Ohnishi , Masamitsu Ishitobi
IPC分类号： C08G61/00 , C09K11/06 , H01L51/30 , H01L51/50 , H05B33/14
CPC分类号： H05B33/14 , C08G61/00 , C09K11/06 , H01L51/0035 , H01L51/0038 , H01L51/0043 , H01L51/5012 , Y10S428/917 , Y10T428/31504 , Y10T428/31678
摘要： Disclosed are an organic electroluminescence device having at least a light emitting layer between the electrodes consisting of one pair of an anode and a cathode, at least one of which electrodes is transparent or semi-transparent, wherein said light emitting layer comprises a polymeric fluorescent substance which emits a fluorescence in a solid state, is soluble in solvents and comprises at least one kind of repeating unit represented by the following formula (1) and at last one kind of repeating unit represented by the following formula (2) with the number of the formula (1) repeating units being 2-50% of the total number of all the repeating units:--Ar.sub.1 -- (1)--Ar.sub.2 -- (2)wherein Ar.sub.1 and Ar.sub.2 are each a bifunctional group forming a carbon--carbon bond with each of two adjacent groups, in the chemical structure of Ar.sub.1, the number of the consecutive atoms present in the shortest path between the two carbon atoms bonding to said two adjacent groups is 1, 3 or 5, and in the chemical structure of Ar.sub.2, the total number of the carbon and nitrogen atoms present in the shortest path between the two carbon atoms bonding to said two adjacent groups is an even number, and a novel polymeric fluorescent substance used in the above device.
摘要翻译：公开了一种有机电致发光器件，其具有在由一对阳极和阴极组成的电极之间的至少一个发光层，其中至少一个电极是透明或半透明的，其中所述发光层包含聚合物荧光物质其发出固体荧光，可溶于溶剂中，并且包含由下式（1）表示的至少一种重复单元和最后一种由下式（2）表示的重复单元，其数目为式（1）重复单元是全部重复单元总数的2-50％：-Ar1-（1）-Ar2-（2）其中Ar1和Ar2分别是形成碳 - 碳键的双官能团，两个相邻基团中的每一个在Ar1的化学结构中，键合到所述两个相邻基团的两个碳原子之间的最短路径中存在的连续原子的数目是1,3或5，并且在化学结构 Ar2中，键合到所述两个相邻基团的两个碳原子之间的最短路径中存在的碳和氮原子的总数为偶数，并且在上述装置中使用的新颖的聚合物荧光物质。

3. 发明授权

US06994921B2 Polymeric fluorescent substance and polymer light emitting device 有权
标题翻译：聚合物荧光物质和聚合物发光装置
公开(公告)号：US06994921B2
公开(公告)日：2006-02-07
申请号：US09928348
申请日：2001-08-14
申请人： Takanobu Noguchi , Masato Ueda , Masamitsu Ishitobi
发明人： Takanobu Noguchi , Masato Ueda , Masamitsu Ishitobi
IPC分类号： H05B33/14 , C09K11/06 , C08G61/00
CPC分类号： H01L51/0038 , C08G61/02 , C08G61/12 , C09K11/06 , H01L51/0035 , H01L51/0052 , H01L51/0094 , H01L51/5012 , Y10S428/917
摘要： A polymeric fluorescent substance exhibiting strong visible fluorescence in solid state. The substance has a polystyrene reduced number-average molecular weight of 1×103 to 1×108, and contains repeating units represented by formula (1), —Ar1—(CR1═CR2)m— (1) in the formula, Ar1 represents an arylene group having a specific substituent. By using the polymeric fluorescent substance, a high performance polymer LED can be prepared easily.
摘要翻译：在固体状态下表现出强烈可见荧光的聚合物荧光物质。该物质的聚苯乙烯换算的数均分子量为1×10 3至1×10 8，并含有由式

4. 发明授权

US06403237B1 Polymeric fluorescent substance and organic electroluminescence device 失效
标题翻译：聚合物荧光物质和有机电致发光器件
公开(公告)号：US06403237B1
公开(公告)日：2002-06-11
申请号：US09327501
申请日：1999-06-08
申请人： Takanobu Noguchi , Masamitsu Ishitobi , Makoto Kitano
发明人： Takanobu Noguchi , Masamitsu Ishitobi , Makoto Kitano
IPC分类号： H05B3314
CPC分类号： H05B33/14 , C08G61/02 , C09K11/06 , H01L51/0038 , H01L51/0052 , H01L51/5012 , H01L2251/308 , Y10S428/917
摘要： Provided is a high heat-resistant polymeric fluorescent substance having a divalent condensed polycyclic aromatic group of specific size having a bonding part at specific position shows fluorescence at a long wave length from orange to red, which is useful for fabricating an organic EL device having excellent properties by a coating method.
摘要翻译：提供具有特定尺寸的二价稠合多环芳族基团的具有特定位置的结合部分的高耐热性聚合物荧光物质，其显示从橙色到红色的长波长的荧光，其可用于制造具有优异的有机EL器件性能通过涂布法。

5. 发明授权

US07135579B2 Dibenzothiophene oxide compound, and process for producing the same 有权
标题翻译：二苯并噻吩氧化物，及其制造方法
公开(公告)号：US07135579B2
公开(公告)日：2006-11-14
申请号：US10873211
申请日：2004-06-23
申请人： Chizu Sekine , Masamitsu Ishitobi , Koichi Fujisawa , Kazunori Iwakura , Masayoshi Minai
发明人： Chizu Sekine , Masamitsu Ishitobi , Koichi Fujisawa , Kazunori Iwakura , Masayoshi Minai
IPC分类号： C07D333/76
CPC分类号： C09K19/3059 , C07D333/76 , C09K19/18 , C09K19/3491 , C09K19/42 , C09K2019/0448 , C09K2019/0496 , C09K2019/188 , Y10T428/10
摘要： There are disclosed novel compounds, liquid crystal compositions, polymers, optically anisotropic producgs, and optical or liquid crystal elements that have large refractive index anisotropy, mix easily with other liquid crystals, have advantageous stability against light, and exhibit absorption at practically short wavelength in the ultraviolet region. The compounds are represented by the formula (1) and have a phenylacetylene structure, wherein difference ΔE in energy of HOMO of parts (1-1), (1-2) and (1-3) calculated by the method of molecular orbitals is not less than 0.3 electronvolt, and the polarizability anisotropy Δα of a molecule represented by the formula (1) calculated in the same way is not lower than 500 A.U.: P1—H (1-2) P2—H (1-3) (A1 to A4: H, F, alkyl or alkoxy group of C1 to C10 optionally substituted with F; P1, P2: structure fulfilling the conditions of HOMO energy and polarizability).
摘要翻译：公开了具有大的折射率各向异性，容易与其他液晶混合的新型化合物，液晶组合物，聚合物，光学各向异性产物和光学或液晶元件，对光具有有利的稳定性，并且在实际短波长下表现出吸收紫外线区域。化合物由式（1）表示并具有苯乙炔结构，其中通过分子轨道方法计算的部分（1-1），（1-2）和（1-3）的HOMO的能量差ΔE为不小于0.3电子伏特，并且以相同方式计算的由式（1）表示的分子的极化率各向异性Δalpha不低于500AU：<？in-line-formula description =“In-line Formulas”end = “lead”？> P <1> H（1-2）<？in-line-formula description =“In-line Formulas”end =“tail”？> <？in-line-formula 描述=“在线公式”end =“lead”？> P <2> -H（1-3）<？in-line-formula description =“In-line Formulas”end =“tail （A 1至A 4）：任选被F取代的C至C 10的H，F，烷基或烷氧基; P 1，，满足HOMO能量和极化率条件的结构）。

6. 发明申请

US20110311899A1 POLYMER, POLYARYLENE BLOCK COPOLYMER, POLYELECTROLYTE, POLYELECTROLYTE MEMBRANE, AND FUEL CELL 审中-公开
标题翻译：聚合物，聚烯烃嵌段共聚物，聚电解质，聚电解质膜和燃料电池
公开(公告)号：US20110311899A1
公开(公告)日：2011-12-22
申请号：US12993675
申请日：2009-05-21
申请人： Toru Onodera , Taisuke Nakamura , Sho Kanesaka , Arihiro Yashiro , Takashi Yamada , Masamitsu Ishitobi , Shigeru Sasaki , Isao Kaito , Akira Kaito , Yuko Kaito
发明人： Toru Onodera , Taisuke Nakamura , Sho Kanesaka , Arihiro Yashiro , Takashi Yamada , Masamitsu Ishitobi , Shigeru Sasaki , Isao Kaito , Akira Kaito , Yuko Kaito
IPC分类号： B01J39/18 , H01M8/10
CPC分类号： C08J5/2256 , C08G61/12 , C08G2261/1452 , C08G2261/312 , C08G2261/3444 , C08G2261/354 , C08G2261/412 , C08G2261/516 , C08J2365/00 , H01B1/122 , H01M8/1027 , H01M8/1032 , H01M8/1039 , H01M2008/1095 , H01M2300/0082
摘要： The polymer electrolyte membrane according to the present invention comprises a polymer electrolyte having ion-exchange groups, wherein Sp and Snp satisfy a relationship expressed by the following expression (I): Sp/Snp≦0.42 (I) where Sp represents the total of peak areas obtained by measurement of a 13C-solid state nuclear magnetic resonance spectrum of the polymer electrolyte membrane, the polymer electrolyte membrane having been subjected to a first immersion treatment comprising immersing the polymer electrolyte membrane in 5 mmol/L iron (II) chloride tetrahydrate aqueous solution at 25° C. for 1 hour, and thereafter drying the polymer electrolyte membrane at 25° C. at 10 hPa or lower for 12 hours; and Snp represents the total of peak areas obtained by measurement of a 13C-solid state nuclear magnetic resonance spectrum of the polymer electrolyte membrane, the polymer electrolyte membrane before the first immersion treatment having been subjected to a second immersion treatment comprising immersing the polymer electrolyte membrane in water at 25° C. for 1 hour, and thereafter drying the polymer electrolyte membrane at 25° C. at 10 hPa or lower for 12 hours.
摘要翻译：本发明的高分子电解质膜包含具有离子交换基团的高分子电解质，其中，Sp和Snp满足由下式（I）表示的关系：Sp / Snp＆nlE; 0.42（I）其中Sp表示峰的总和通过测量聚合物电解质膜的13 C-固态核磁共振谱获得的区域，已经进行了第一次浸渍处理的聚合物电解质膜，包括将聚合物电解质膜浸入5mmol / L氯化铁（II）四水合物水溶液溶液在25℃下搅拌1小时，然后在10小时或更低温度下在25℃下干燥高分子电解质膜12小时; Snp表示通过测定高分子电解质膜的13 C-固体核磁共振谱得到的峰面积的总和，第一浸渍处理前的高分子电解质膜进行了第二浸渍处理，包括浸渍聚合物电解质膜在25℃的水中1小时，然后将聚合物电解质膜在25℃，10hPa以下干燥12小时。

7. 发明申请

US20100136459A1 ELECTROLYTE CONTAINING OXOCARBON MOLECULE AND USE THEREOF 审中-公开
标题翻译：电解液含有奥克兰分子及其用途
公开(公告)号：US20100136459A1
公开(公告)日：2010-06-03
申请号：US11917373
申请日：2006-06-19
申请人： Ken Yoshimura , Masamitsu Ishitobi
发明人： Ken Yoshimura , Masamitsu Ishitobi
IPC分类号： C08G10/00 , C07C49/15 , H01M8/10
CPC分类号： H01M10/0565 , C08K5/07 , C08K5/375 , H01B1/122 , H01M8/1009 , H01M8/1048 , H01M10/052 , H01M10/0567 , H01M2300/0082
摘要： The present invention provides, as an electrolyte which is useful as a material for a proton conductive membrane in a solid polymer fuel cell utilizing a gas fuel such as hydrogen gas or a liquid fuel such as methanol or dimethyl ether and which has higher proton conductivity than the conventional electrolytes do, an electrolyte characterized by containing an oxocarbon molecule, wherein the oxocarbon molecule has a difference in heat of formation ΔE defined as: ΔE=E2−E1 (kcal/mol) satisfying the range of: ΔE
摘要翻译：本发明提供一种电解质，其可用作利用气体燃料如氢气或液体燃料如甲醇或二甲醚的固体聚合物燃料电池中的质子传导膜的材料，并且具有比质子传导性更高的质子传导性常规的电解质是电解质，其特征在于含有氧化碳分子，其中氧化碳分子的形成热量Dgr; E定义为：＆Dgr; E = E2-E1（kcal / mol），满足以下范围：＆Dgr; E <-70（kcal / mol），其中E1（kcal / mol）是在氢离子不解离的状态下的形成热，E2（kcal / mol）是形成热，在分子离子中具有最低解离能的氢解离，两者都是根据分子轨道方法计算的稳定分子结构。

8. 发明申请

US20090325026A1 POLYMER ELECTROLYTE MEMBRANE AND PRODUCING METHOD THEREOF, MEMBRANE-ELECTRODE ASSEMBLY AND FUEL CELL USING THE POLYMER ELECTROLYTE MEMBRANE, AND EVALUATION ION METHOD OF IONIC CONDUCTIVITY OF THE POLYMER ELECTROLYTE MEMBRANE 审中-公开
标题翻译：聚合物电解质膜及其制造方法，使用聚合物电解质膜的膜电极组件和燃料电池，以及聚合物电解质膜的离子电导率的评价方法
公开(公告)号：US20090325026A1
公开(公告)日：2009-12-31
申请号：US12309395
申请日：2007-07-19
申请人： Masamitsu Ishitobi , Mitsunori Nodono , Yasuhiro Yamashita
发明人： Masamitsu Ishitobi , Mitsunori Nodono , Yasuhiro Yamashita
IPC分类号： H01M8/10 , H01M8/00 , B05D3/02
CPC分类号： C08J5/2287 , C08J5/2256 , C08J2365/02 , C08J2387/00 , H01B1/122 , H01M8/1023 , H01M8/1025 , H01M8/1027 , H01M8/1032 , H01M8/1067 , H01M8/1081 , H01M2300/0082 , Y02P70/56 , Y10T29/49108
摘要： A producing method of a polymer electrolyte membrane is provided in which a polymer electrolyte membrane can be easily obtained having excellent ion conductivity in the thickness direction.The preferred producing method of the polymer electrolyte membrane of the present invention is a producing method of the polymer electrolyte membrane having a micro phase separation structure, including an evaporating step of evaporating a solvent from a solution containing the polymer electrolyte having an ion conductive group, wherein a time from start to completion of the evaporation of the solvent is 60 minutes or less in the evaporating step.
摘要翻译：提供一种聚合物电解质膜的制造方法，其中可以容易地获得在厚度方向上具有优异的离子传导性的聚合物电解质膜。本发明的高分子电解质膜的优选制造方法是具有微相分离结构的高分子电解质膜的制造方法，其特征在于，包括从含有离子导电性基团的聚合物电解质的溶液中蒸发溶剂的蒸发工序，其中在蒸发步骤中从溶剂蒸发开始到完成的时间为60分钟以下。

9. 发明授权

US09011994B2 Gas-barrier multilayer film 有权
标题翻译：阻气性多层膜
公开(公告)号：US09011994B2
公开(公告)日：2015-04-21
申请号：US13263278
申请日：2010-04-08
申请人： Akira Hasegawa , Toshiya Kuroda , Masamitsu Ishitobi , Takashi Sanada , Toshihiko Tanaka
发明人： Akira Hasegawa , Toshiya Kuroda , Masamitsu Ishitobi , Takashi Sanada , Toshihiko Tanaka
IPC分类号： C09K19/00 , C23C16/54 , C23C16/40 , C23C16/505 , B32B15/08 , B32B27/32 , B32B27/36 , H01L51/44 , H01L51/52
CPC分类号： C23C16/545 , B32B15/08 , B32B27/281 , B32B27/302 , B32B27/306 , B32B27/32 , B32B27/325 , B32B27/34 , B32B27/36 , B32B27/365 , B32B2255/10 , B32B2255/20 , B32B2307/306 , B32B2307/31 , B32B2307/412 , B32B2307/7242 , B32B2307/732 , B32B2439/40 , B32B2439/60 , B32B2553/00 , C23C16/401 , C23C16/505 , H01L51/448 , H01L51/5237 , H01L51/5253 , Y10T428/10 , Y10T428/1064 , Y10T428/1068 , Y10T428/1317 , Y10T428/26 , Y10T428/265
摘要： A gas-barrier multilayer film including: a base member; and at least one thin film layer formed on at least one surface of the base member, wherein at least one layer of the thin film layer(s) satisfies at least one of requirements (A) and (B).
摘要翻译：一种阻气性多层膜，包括：基材; 以及形成在所述基底构件的至少一个表面上的至少一个薄膜层，其中所述薄膜层的至少一层满足要求（A）和（B）中的至少一个。

10. 发明申请

US20080139824A1 DIBENZOTHIOPHENE OXIDE COMPOUND, AND PROCESS FOR PRODUCING THE SAME 审中-公开
标题翻译：二苯氧基氧化物化合物及其制备方法
公开(公告)号：US20080139824A1
公开(公告)日：2008-06-12
申请号：US11943433
申请日：2007-11-20
申请人： Chizu Sekine , Masamitsu Ishitobi , Koichi Fujisawa , Kazunori Iwakura , Masayoshi Minai
发明人： Chizu Sekine , Masamitsu Ishitobi , Koichi Fujisawa , Kazunori Iwakura , Masayoshi Minai
IPC分类号： C07D333/76
CPC分类号： C09K19/3059 , C07D333/76 , C09K19/18 , C09K19/3491 , C09K19/42 , C09K2019/0448 , C09K2019/0496 , C09K2019/188 , Y10T428/10
摘要： There are disclosed novel compounds, liquid crystal compositions, polymers, optically anisotropic products, and optical or liquid or liquid crystal elements that have large refractive index anisotropy, mix easily with other liquid crystals, have advantageous stability against light, and exhibit absorption at practically short wavelength in the ultraviolet region. The compounds are represented by the formula (1) and have a phenylacetylene structure, wherein difference ΔE in energy of HOMO of parts (1-1), (1-2) and (1-3) calculated by the method of molecular orbitals is not less than 0.3 electronvolt, and the polarizability anisotropy Δα of a molecule represented by the formula (1) calculated in the same way is not lower than 500 A.U.: (A1 to A4: H, F, alkyl or alkoxy group of C1 to C10 optionally substituted with F; P1, P2; structure fulfilling the conditions of HOMO energy and polarizability).
摘要翻译：公开了新型化合物，液晶组合物，聚合物，光学各向异性产物，具有大的折射率各向异性的光学或液体或液晶元件，与其它液晶容易混合，对光具有有利的稳定性，并在几乎短时间内呈现吸收波长在紫外线区域。化合物由式（1）表示并具有苯乙炔结构，其中通过分子轨道方法计算的部分（1-1），（1-2）和（1-3）的HOMO的能量差ΔE为不小于0.3电子伏特，并且以相同方式计算的由式（1）表示的分子的极化率各向异性Δα不低于500AU：（A <1> 1 < H，F，任选被F取代的C 1至C 10的烷基或烷氧基; P 1，P 2;满足HOMO能量和极化率条件的结构）。

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