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1. 发明申请

US20050075453A1 Method for producing aqueous polymer dispersions containing colorants 失效
标题翻译：含有着色剂的聚合物水分散体的制备方法
公开(公告)号：US20050075453A1
公开(公告)日：2005-04-07
申请号：US10629552
申请日：2003-07-30
申请人： Klemens Mathauer , Arno Bohm , Walter Machtle , Peter Rossmanith , Sabine Kielhorn-Bayer , Klaus Mullen , Ulrike Rohr , Friedrich-Wilhelm Raulfs , Ulrike Schlosser , Wolfgang Schrof , Harutyun Hanciogullari , Karl Siemensmeyer , Paul Delavier , Rudiger Sens , Torsten Freund , Takahiro Ikeda , Takanori Wakebe
发明人： Klemens Mathauer , Arno Bohm , Walter Machtle , Peter Rossmanith , Sabine Kielhorn-Bayer , Klaus Mullen , Ulrike Rohr , Friedrich-Wilhelm Raulfs , Ulrike Schlosser , Wolfgang Schrof , Harutyun Hanciogullari , Karl Siemensmeyer , Paul Delavier , Rudiger Sens , Torsten Freund , Takahiro Ikeda , Takanori Wakebe
IPC分类号： C07D221/18 , C07C69/54 , C07C271/12 , C07D213/85 , C08F2/22 , C08F2/32 , C08F2/44 , C09B69/10 , C09D5/02 , C09D5/03 , C09D11/00 , D21H19/00
CPC分类号： C08F2/32 , C08F2/44 , C08K3/00 , C09B69/102
摘要： The present invention relates to a process for preparing dye-comprising aqueous polymer dispersions by free-radical aqueous emulsion polymerization of ethylenically unsaturated monomers in the presence of free-radical initiators, in which at least some of the monomers are employed in the form of an oil-in-water emulsion E1 whose disperse phase comprises at least one oil-soluble dye, wherein the disperse phase of E1 is formed essentially of dye-comprising monomer droplets having a diameter
摘要翻译：本发明涉及一种在自由基引发剂存在下通过烯键式不饱和单体的自由基水乳液聚合制备含染料的聚合物水分散体的方法，其中至少一些单体以水包油乳液E1，其分散相包含至少一种油溶性染料，其中E1的分散相基本上由具有直径<500nm的含染料的单体液滴形成。本发明还涉及如权利要求35所述的式III的苝染料。本发明除了含有染料的制剂外，还包括本发明的含染料的聚合物和着色剂，其包含本发明包括荧光增白剂。

2. 发明授权

US5986099A Substituted quaterrylene tetracarboxylic acid diimides 失效
标题翻译：取代的四亚甲基四羧酸二酰亚胺
公开(公告)号：US5986099A
公开(公告)日：1999-11-16
申请号：US860928
申请日：1997-07-21
申请人： Klaus Mullen , Heribert Quante , Arno Bohm
发明人： Klaus Mullen , Heribert Quante , Arno Bohm
IPC分类号： C07D221/18 , C07D471/06 , C09B5/62 , C09B57/08
CPC分类号： C07D221/18 , C09B5/62
摘要： Quaterrylenetetracarboxylic diimides I ##STR1## where R is hydrogen;C.sub.1 -C.sub.30 -alkyl whose carbon chain may be interrupted by one or e of --O--, --S--, --NR.sup.1 --, --CO-- and/or --SO.sub.2 -- and which may be monosubstituted or polysubstituted by cyano, C.sub.1 -C.sub.6 -alkoxy or a 5-, 6- or 7-membered heterocyclic radical which is attached via a nitrogen atom and which may contain further heteroatoms and may be aromatic, whereR.sup.1 is hydrogen or C.sub.1 -C.sub.6 -alkyl;C.sub.5 -C.sub.8 -cycloalkyl whose carbon skeleton may be interrupted by one or more of --O--, --S-- and/or --NR.sup.1 --;aryl or hetaryl, which may each be monosubstituted or poly-substituted by C.sub.1 -C.sub.18 -alkyl, C.sub.1 -C.sub.6 -alkoxy, cyano, --CONHR.sup.2, --NHCOR.sup.2 and/or aryl- or hetaryl-azo, which may each be substituted by C.sub.1 -C.sub.10 -alkyl, C.sub.1 -C.sub.6 -alkoxy or cyano, whereR.sup.2 is hydrogen; C.sub.1 -C.sub.18 -alkyl; aryl or hetaryl, which may each be substituted by C.sub.1 -C.sub.6 -alkyl, C.sub.1 -C.sub.6 -alkoxy, halogen or cyano;X is halogen; C.sub.1 -C.sub.18 -alkyl; aryloxy, arylthio, hetaryloxy or hetarylthio, which may each be substituted by C.sub.1 -C.sub.4 -alkyl or C.sub.1 -C.sub.4 -alkoxy;n is from 2 to 12,their preparation and use as pigments or fluorescent dyes.
摘要翻译： PCT No.PCT / EP96 / 00118 Sec。 371日期1997年7月21日 102（e）日期1997年7月21日PCT 1996年1月12日PCT PCT。公开号WO96 / 22332 日期：1996年7月25日四氢四羧酸二酰亚胺其中R为氢; 其碳链可以被-O - ， - S - ， - NR 1 - ， - CO - 和/或-SO 2 - 中的一个或多个中断的C 1 -C 30 - 烷基，并且其可以被氰基，C 1 -C 6单取代或多取代 - 烷氧基或5-，6-或7-元杂环基，其通过氮原子连接并且可以含有另外的杂原子并且可以是芳族的，其中R 1是氢或C 1 -C 6 - 烷基; 碳骨架可被-O - ， - S-和/或-NR1-中的一个或多个中断的C 5 -C 8 - 环烷基; 芳基或杂芳基，其可以各自被C1-C18-烷基，C1-C6-烷氧基，氰基，-CONHR2，-NHCOR2和/或芳基 - 或杂芳基 - 偶氮基单取代或多取代，其可以各自被C1 C 1-10 - 烷基，C 1 -C 6 - 烷氧基或氰基，其中R 2是氢; C1-C18-烷基; 芳基或杂芳基，其各自可被C 1 -C 6 - 烷基，C 1 -C 6 - 烷氧基，卤素或氰基取代; X是卤素; C1-C18-烷基; 芳氧基，芳硫基，杂芳氧基或杂芳硫基，其各自可被C 1 -C 4 - 烷基或C 1 -C 4 - 烷氧基取代; n为2至12，它们的制备和用作颜料或荧光染料。

3. 发明申请

US20060075585A1 Rylene dyes 失效
标题翻译：二烯染料
公开(公告)号：US20060075585A1
公开(公告)日：2006-04-13
申请号：US10522990
申请日：2003-07-25
申请人： Matthias Krieger , Arno Bohm , Lorenz Siggel , Stefan Becker , Klaus Mullen , Christopher Kohl
发明人： Matthias Krieger , Arno Bohm , Lorenz Siggel , Stefan Becker , Klaus Mullen , Christopher Kohl
IPC分类号： C09B49/00
CPC分类号： C09B5/62
摘要： Rylene dyes of the general formula I where the variables are defined as follows: R is hydrogen; optionally substituted C1-C30-alkyl, C5-C8-cycloalkyl, aryl or hetaryl; R′ is bromine; cyano; —NR32; optionally substituted aryloxy, arylthio, hetaryloxy or hetarylthio; optionally substituted C3-C18-alk-1-ynyl; X, Y are both hydrogen or together are a radical of the formula Ia n is 2, 3, 4 or additionally 1 when X and Y are a radical of the formula Ia; n′ is from 1 to 4; m is from 0 to 6.
摘要翻译：通式I的Rylene染料，其中变量定义如下：R是氢; 芳基或杂芳基;任选取代的C 1 -C 30 - 烷基，C 5 -C 8 - 环烷基，芳基或杂芳基; R'是溴; 氰基; -NR 3 3; 任选取代的芳氧基，芳硫基，杂芳氧基或杂芳硫基; 任选取代的C 3 -C 18 - 烷-1-基; 当X和Y是式Ia的基团时，X，Y都是氢或一起是式Ia n的基团是2,3,4或另外1， n'为1至4; m为0〜6。

4. 发明申请

US20070155968A1 Method for the production of terylene-3,4:11,12-tetracarboxydiimides by direct synthesis 失效
标题翻译：通过直接合成制备涤纶3,4：11,12-四羧酰亚胺的方法
公开(公告)号：US20070155968A1
公开(公告)日：2007-07-05
申请号：US10586133
申请日：2005-01-15
申请人： Martin Konemann , Arno Bohm , Willi Helfer , Jurgen Romeis , Jianqiang Qu , Klaus Mullen
发明人： Martin Konemann , Arno Bohm , Willi Helfer , Jurgen Romeis , Jianqiang Qu , Klaus Mullen
IPC分类号： C07D471/02
CPC分类号： C07D221/18 , C07D221/14 , C07D471/06
摘要： A process for preparing terylene-3,4:11,12-tetracarboximides I where the variables are each defined as follows: R, R′ are each independently hydrogen; if desired substituted alkyl or cycloalkyl; R1 is hydrogen or alkyl; R2 is hydrogen; alkyl; if desired substituted aryl or hetaryl, by reacting a perylene-3,4-dicarboximide II in the presence of a base-stable, high-boiling organic solvent and of an alkali metal or alkaline earth metal base, with a naphthalene-1,8-dicarboximide III in which X is hydrogen, bromine or chlorine.
摘要翻译：制备三苯醚-3,4：11,12-四甲酰亚胺I的方法，其中各变量各自定义如下：R，R'各自独立地为氢; 如果需要，取代的烷基或环烷基; R 1是氢或烷基; R 2是氢; 烷基; 如果需要取代的芳基或杂芳基，通过在碱稳定的高沸点有机溶剂和碱金属或碱土金属碱的存在下使苝-3,4-二甲酰亚胺II与萘-1,8 二甲酰亚胺III，其中X是氢，溴或氯。

5. 发明申请

US20090023937A1 9-CYANO-SUBSTITUTED PERYLENE-3,4-DICARBOXYLIC ACID MONOIMIDES 失效
标题翻译： 9-氰基取代的亚戊基-3,4-二羧酸单体
公开(公告)号：US20090023937A1
公开(公告)日：2009-01-22
申请号：US12239173
申请日：2008-09-26
申请人： Arno Bohm , Peter Blaschka , Willi Helfer , Dirk Hammel , Peter Schlichting , Klaus Mullen
发明人： Arno Bohm , Peter Blaschka , Willi Helfer , Dirk Hammel , Peter Schlichting , Klaus Mullen
IPC分类号： C07D311/02
CPC分类号： C09D11/328 , C07D221/18 , C07D311/78 , C09B5/62 , C09D11/037 , G03G5/0637
摘要： The current invention relates to a perylene-3,4-dicarboxylic anhydride, substituted in the 9-position, of the general formula III wherein Z is bromine or cyano, and processes for preparing 9-bromoperylene-3,4-dicarboxylic anhydride and 9-cyanoperylene-3,4-dicarboxylic anhydride.
摘要翻译：本发明涉及在9-位被取代的通式Ⅲ其中Z为溴或氰基的苝-3,4-二羧酸酐，以及制备9-溴戊烯-3,4-二羧酸酐和9 - 氰基-3,4-二羧酸酐。

6. 发明申请

US20060058330A1 Rylene derivatives and their use as dyes 有权
标题翻译：二烯衍生物及其作为染料的用途
公开(公告)号：US20060058330A1
公开(公告)日：2006-03-16
申请号：US10985942
申请日：2004-11-12
申请人： Matthias Krieger , Arno Bohm , Erik Reuther , Klaus Mullen
发明人： Matthias Krieger , Arno Bohm , Erik Reuther , Klaus Mullen
IPC分类号： A61K31/473 , C07D221/18
CPC分类号： C07D491/06 , C07D221/18 , C07D471/06 , C09B5/62
摘要： Rylene derivatives of the general formula I where the variables have the following meanings: R is hydrogen or substituted or unsubstituted C1-C30-alkyl, aryl or hetaryl; R1 is hydrogen or bromine; R2 is hydrogen or C1-C6-alkyl; R3 is hydrogen, C1-C18-alkyl or substituted or unsubstituted aryl or hetaryl; and n is 2 or 3.
摘要翻译：通式I的亚芳基衍生物

7. 发明申请

US20050222416A1 1,6,9,14-teltrasubstituted terrylene tetracarboxylic diimides 有权
公开(公告)号：US20050222416A1
公开(公告)日：2005-10-06
申请号：US10514568
申请日：2003-06-04
申请人： Arno Bohm , Matthias Krieger , Erik Reuther , Klaus Mullen
发明人： Arno Bohm , Matthias Krieger , Erik Reuther , Klaus Mullen
IPC分类号： C07D471/06 , C09B5/62 , C09K11/06 , C07D471/02
CPC分类号： C07D471/06 , C09B5/62
摘要： The invention relates to 1,6,9,14-tetrasubstituted terrylene tetracarboxylic acid diimides of general formula (I), in which the variables are defined as follows: X, Y independently of one another represent bromium; cyano; aryloxy, arylthio, hetaryloxy or hetarylthio, which can respectively be mono- or polysubstituted by C1-C12 alkyl, C1-C12 alkoxy, —COOR1, —SO3R1, halogen, hydroxy, carboxy, cyano, —CONHR2 and/or —NHCOR2; a group of formula -L-R3; a group of formula —NR22; R, R′ independently of one another represent hydrogen; C1-C30 alkyl, whose carbon chain can be interrupted by one or more groupings —O—, —S—, —NR1—, —CO— and/or —SO2— and which can be mono- or polysubstituted by cyano, C1-C6 alkoxy, aryl, which may be substituted by C1-C18 alkyl or C1-C6 alkoxy and/or a 5- to 7-membered heterocyclic group that is bonded by means of a nitrogen atom and that can contain additional heteroatoms and be aromatic; C5-C8 cycloalkyl, whose carbon skeleton can be interrupted by one or more groupings —O—, —S— and/or —NR1— and/or which can be mono- or polysubstituted by C1-C6 alkyl; aryl or hetaryl, which can be mono- or polysubstituted by C1-C18 alkyl, C1-C6 alkoxy, cyano, —CONHR2, —NHCOR2 and/or aryl- or hetarylazo, which can be respectively substituted by C1-C10 alkyl, C1-C6 alkoxy or cyano; and L represents 1,2-ethylene, 1,2-ethenylene or 1,2-ethynylene.

8. 发明授权

US5712361A Conjugated polymers containing ANSA substructures and their use as electroluminescence materials 失效
标题翻译：含有ANSA亚结构的共轭聚合物及其作为电致发光材料的用途
公开(公告)号：US5712361A
公开(公告)日：1998-01-27
申请号：US496202
申请日：1995-06-28
申请人： Roland Stern , Donald Lupo , Josef Salbeck , Hermann Schenk , Thomas Stehlin , Klaus Mullen , Ullrich Scherf , Joachim Huber
发明人： Roland Stern , Donald Lupo , Josef Salbeck , Hermann Schenk , Thomas Stehlin , Klaus Mullen , Ullrich Scherf , Joachim Huber
IPC分类号： C08G61/00 , C08G61/02 , C09K11/06 , H01L51/50 , H05B33/14 , C08G61/12
CPC分类号： H05B33/14 , C08G61/02 , C09K11/06 , Y10S428/917
摘要： Conjugated polymers containing ansa substructures and their use as electroluminescence materials. Conjugated polymers containing ansa substructures, which contain aromatic groups and in which adjacent aromatic groups are connected to one another in such a way that one ring atom of one aromatic group is directly linked to one ring atom of the other aromatic group and any further linkages of these two aromatic groups are possible only via a bridge containing at least one tetravalent carbon atom and/or heteroatom. The polymers of the invention having ansa substructures are outstandingly suitable as electroluminescence materials, since they have a very high color purity.
摘要翻译：含有ansa亚结构的共轭聚合物及其作为电致发光材料的用途。含有芳族基团的共轭聚合物，其中相邻芳族基团彼此连接，其中一个芳族基团的一个环原子直接与另一个芳族基团的一个环原子连接，这两个芳族基团仅通过含有至少一个四价碳原子和/或杂原子的桥可能。具有ansa子结构的本发明的聚合物非常适合作为电致发光材料，因为它们具有非常高的色纯度。

9. 发明授权

US5376507A Method to produce nonlinear optical microcomponents 失效
标题翻译：制造非线性光学微元件的方法
公开(公告)号：US5376507A
公开(公告)日：1994-12-27
申请号：US2822
申请日：1993-01-08
申请人： Wolfgang Ehrfeld , Herbert O. Moser , Klaus Mullen , Christoph Bubeck , Hans-Dieter Bauer
发明人： Wolfgang Ehrfeld , Herbert O. Moser , Klaus Mullen , Christoph Bubeck , Hans-Dieter Bauer
IPC分类号： G02F1/35 , G02F1/065 , G03F7/00 , G03F7/20 , G02B6/10
CPC分类号： G03F7/00 , G02F1/065 , G03F7/2039 , Y10S430/168
摘要： A method to produce nonlinear optical microcomponents is described which employs hitherto not yet used material combinations. Not only waveguide structures are produced by means of X-ray depth lithography, but also microcell structures, into which materials having nonlinear optical properties are introduced. The microstructure is produced as a positive mold part, from which there is subsequently generated, by means of electroforming, a mold insert, a negative of which is made using a polymer material. After the molding operation the microstructure is applied to a substrate, and nonlinear optical material, covered by a cover plate if needed or desired, is introduced into the microcell structure.
摘要翻译：描述了一种生产非线性光学微元件的方法，该方法采用迄今未使用的材料组合。不仅通过X射线深度光刻产生波导结构，而且还引入了具有非线性光学特性的材料的微单元结构。微结构作为正模具部件生产，随后通过电铸产生模具插入件，模具插件的负极由聚合物材料制成。在模制操作之后，将微结构施加到基板上，并且如果需要或期望，则由盖板覆盖的非线性光学材料被引入到微单元结构中。

10. 发明授权

US5728480A Poly(4,5,9,10-tetrahydropyrene-2,7-diyl) derivatives and their use as electroluminescence materials 失效
标题翻译：聚（4,5,9,10-四氢芘-2,7-二基）衍生物及其作为电致发光材料的用途
公开(公告)号：US5728480A
公开(公告)日：1998-03-17
申请号：US521263
申请日：1995-08-30
申请人： Roland Stern , Donald Lupo , Josef Salbeck , Hermann Schenk , Thomas Stehlin , Klaus Mullen , Martin Kreyenschmidt , Ullrich Scherf
发明人： Roland Stern , Donald Lupo , Josef Salbeck , Hermann Schenk , Thomas Stehlin , Klaus Mullen , Martin Kreyenschmidt , Ullrich Scherf
IPC分类号： C07C25/22 , C07B61/00 , C07C17/12 , C08G61/00 , C08G61/10 , C09K11/06 , H01L51/30 , H01L51/50 , H05B33/12 , H05B33/14
CPC分类号： C09K11/06 , C07C17/12 , C08G61/10 , H01L51/0035 , C07C2103/50 , C09K2211/1408 , C09K2211/1416 , H01L51/0052 , Y10S428/917 , Y10T428/31504 , Y10T428/31678
摘要： Poly(4,5,9,10-tetrahydropyrene-2,7-diyl) derivatives of the formula (I) ##STR1## where the symbols R.sup.1 to R.sup.4 have the following meanings: R.sup.1, R.sup.2, R.sup.3, R.sup.4 are identically or variously H, a straight-chain or branched alkyl chain containing 1 to 22 carbon atoms, it being possible for one or more nonadjacent CH.sub.2 groups also to be replaced by --O--, --COO--, --OOC-- and/or phenylene, aryl or aryloxy groups, it being possible for the aromatic to be substituted by C.sub.1 -C.sub.22 -alkyl, C.sub.1 -C.sub.22 -alkoxy, Br, Cl, F, CN, and/or NO.sub.2, Br, Cl, F, CN, NO.sub.2, or carboalkoxy containing 2 to 23 carbon atoms; n is 10 to 150, are suitable as electroluminescence materials.
摘要翻译：式（I）的（4,5,9,10-四氢苯-2,7-二基）衍生物其中符号R1至R4具有下列含义：R1，R2，R3，R4分别为同样或各种H，含有1至22个碳原子的直链或支链烷基链，一个或多个不相邻的CH 2基团也可以被-O - ， - COO - ， - OOC-和/或亚苯基代替芳基或芳氧基，芳香族可以被C 1 -C 22 - 烷基，C 1 -C 22 - 烷氧基，Br，Cl，F，CN和/或NO 2，Br，Cl，F，CN，NO 2 或含有2至23个碳原子的烷氧羰基; n为10〜150，适合作为电致发光材料。

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