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1. 发明授权

US5728480A Poly(4,5,9,10-tetrahydropyrene-2,7-diyl) derivatives and their use as electroluminescence materials 失效
标题翻译：聚（4,5,9,10-四氢芘-2,7-二基）衍生物及其作为电致发光材料的用途
公开(公告)号：US5728480A
公开(公告)日：1998-03-17
申请号：US521263
申请日：1995-08-30
申请人： Roland Stern , Donald Lupo , Josef Salbeck , Hermann Schenk , Thomas Stehlin , Klaus Mullen , Martin Kreyenschmidt , Ullrich Scherf
发明人： Roland Stern , Donald Lupo , Josef Salbeck , Hermann Schenk , Thomas Stehlin , Klaus Mullen , Martin Kreyenschmidt , Ullrich Scherf
IPC分类号： C07C25/22 , C07B61/00 , C07C17/12 , C08G61/00 , C08G61/10 , C09K11/06 , H01L51/30 , H01L51/50 , H05B33/12 , H05B33/14
CPC分类号： C09K11/06 , C07C17/12 , C08G61/10 , H01L51/0035 , C07C2103/50 , C09K2211/1408 , C09K2211/1416 , H01L51/0052 , Y10S428/917 , Y10T428/31504 , Y10T428/31678
摘要： Poly(4,5,9,10-tetrahydropyrene-2,7-diyl) derivatives of the formula (I) ##STR1## where the symbols R.sup.1 to R.sup.4 have the following meanings: R.sup.1, R.sup.2, R.sup.3, R.sup.4 are identically or variously H, a straight-chain or branched alkyl chain containing 1 to 22 carbon atoms, it being possible for one or more nonadjacent CH.sub.2 groups also to be replaced by --O--, --COO--, --OOC-- and/or phenylene, aryl or aryloxy groups, it being possible for the aromatic to be substituted by C.sub.1 -C.sub.22 -alkyl, C.sub.1 -C.sub.22 -alkoxy, Br, Cl, F, CN, and/or NO.sub.2, Br, Cl, F, CN, NO.sub.2, or carboalkoxy containing 2 to 23 carbon atoms; n is 10 to 150, are suitable as electroluminescence materials.
摘要翻译：式（I）的（4,5,9,10-四氢苯-2,7-二基）衍生物其中符号R1至R4具有下列含义：R1，R2，R3，R4分别为同样或各种H，含有1至22个碳原子的直链或支链烷基链，一个或多个不相邻的CH 2基团也可以被-O - ， - COO - ， - OOC-和/或亚苯基代替芳基或芳氧基，芳香族可以被C 1 -C 22 - 烷基，C 1 -C 22 - 烷氧基，Br，Cl，F，CN和/或NO 2，Br，Cl，F，CN，NO 2 或含有2至23个碳原子的烷氧羰基; n为10〜150，适合作为电致发光材料。

2. 发明授权

US5712361A Conjugated polymers containing ANSA substructures and their use as electroluminescence materials 失效
标题翻译：含有ANSA亚结构的共轭聚合物及其作为电致发光材料的用途
公开(公告)号：US5712361A
公开(公告)日：1998-01-27
申请号：US496202
申请日：1995-06-28
申请人： Roland Stern , Donald Lupo , Josef Salbeck , Hermann Schenk , Thomas Stehlin , Klaus Mullen , Ullrich Scherf , Joachim Huber
发明人： Roland Stern , Donald Lupo , Josef Salbeck , Hermann Schenk , Thomas Stehlin , Klaus Mullen , Ullrich Scherf , Joachim Huber
IPC分类号： C08G61/00 , C08G61/02 , C09K11/06 , H01L51/50 , H05B33/14 , C08G61/12
CPC分类号： H05B33/14 , C08G61/02 , C09K11/06 , Y10S428/917
摘要： Conjugated polymers containing ansa substructures and their use as electroluminescence materials. Conjugated polymers containing ansa substructures, which contain aromatic groups and in which adjacent aromatic groups are connected to one another in such a way that one ring atom of one aromatic group is directly linked to one ring atom of the other aromatic group and any further linkages of these two aromatic groups are possible only via a bridge containing at least one tetravalent carbon atom and/or heteroatom. The polymers of the invention having ansa substructures are outstandingly suitable as electroluminescence materials, since they have a very high color purity.
摘要翻译：含有ansa亚结构的共轭聚合物及其作为电致发光材料的用途。含有芳族基团的共轭聚合物，其中相邻芳族基团彼此连接，其中一个芳族基团的一个环原子直接与另一个芳族基团的一个环原子连接，这两个芳族基团仅通过含有至少一个四价碳原子和/或杂原子的桥可能。具有ansa子结构的本发明的聚合物非常适合作为电致发光材料，因为它们具有非常高的色纯度。

3. 发明授权

US5856434A Use of polymers containing isolated chromophores as electroluminescence materials 失效
标题翻译：使用含有分离发色团的聚合物作为电致发光材料
公开(公告)号：US5856434A
公开(公告)日：1999-01-05
申请号：US596198
申请日：1996-02-16
申请人： Roland Stern , Hermann Schenk , Josef Salbeck , Thomas Stehlin , Ullrich Scherf , Klaus Mullen , Gunther Leising
发明人： Roland Stern , Hermann Schenk , Josef Salbeck , Thomas Stehlin , Ullrich Scherf , Klaus Mullen , Gunther Leising
IPC分类号： C09B69/10 , C08G61/00 , C08G61/10 , C08G61/12 , C09K11/06 , H01L51/30 , H01L51/50 , H05B33/14 , C08G65/22
CPC分类号： H01L51/0044 , C08G61/10 , C08G61/12 , C09K11/06 , H01L51/0039 , H01L51/0062 , H01L51/5012
摘要： Use in electrooptical switching and display devices of a polymer comprising conjugatively linked chromophore segments whose emission properties are determined by the emission properties of the individual chromophore segments.Electroluminescence devices comprising the polymers of the present invention have, inter alia, a high color purity. The polymers used according to the present invention enable, in particular, blue and white electroluminescence to also be achieved.
摘要翻译： PCT No.PCT / EP94 / 02899 Sec。 371日期1996年2月16日 102（e）日期1996年2月16日PCT 1994年9月1日PCT公布。公开号WO95 / 07955 日期1995年3月23日使用包含共轭连接的发色团片段的聚合物的电光切换和显示装置，其发射性质由单个发色团片段的发射性质决定。包含本发明聚合物的电致发光器件尤其具有高色纯度。根据本发明使用的聚合物尤其能够实现蓝色和白色电致发光。

4. 发明授权

US5679760A Ladder polymers containing conjugated double bonds 失效
标题翻译：含共轭双键的梯形聚合物
公开(公告)号：US5679760A
公开(公告)日：1997-10-21
申请号：US410004
申请日：1995-03-21
申请人： Klaus Mullen , Ullrich Scherf
发明人： Klaus Mullen , Ullrich Scherf
IPC分类号： C08G61/02 , H01B1/12 , C08G6/00
CPC分类号： H01B1/128 , C08G61/02 , H01B1/127
摘要： The present invention relates to polymers with an extended system of conjugated double bonds constructed as homo and/or heterocyclic rings which are interlinked in pairs so that one ring is joined to the neighboring one at two adjacent atoms in the ring, in which one of these connections is made by a chemical bond to a ring atom of the neighboring ring and the other via a carbon, nitrogen, oxygen or sulphur atom to an atom of the neighboring ring adjacent said ring atom, their production and use in electrical, electronic and opto-electronic components.
摘要翻译：本发明涉及具有构建为成对互连的均聚双环和/或杂环的扩展系统的聚合物，使得一个环在环中的两个相邻原子处连接到相邻的一个环，其中这些之一通过与相邻环的环原子的化学键连接，另一个通过碳，氮，氧或硫原子连接到邻近所述环原子的相邻环的原子，它们在电气，电子和光电中的使用 -电子元器件。

5. 发明授权

US5986099A Substituted quaterrylene tetracarboxylic acid diimides 失效
标题翻译：取代的四亚甲基四羧酸二酰亚胺
公开(公告)号：US5986099A
公开(公告)日：1999-11-16
申请号：US860928
申请日：1997-07-21
申请人： Klaus Mullen , Heribert Quante , Arno Bohm
发明人： Klaus Mullen , Heribert Quante , Arno Bohm
IPC分类号： C07D221/18 , C07D471/06 , C09B5/62 , C09B57/08
CPC分类号： C07D221/18 , C09B5/62
摘要： Quaterrylenetetracarboxylic diimides I ##STR1## where R is hydrogen;C.sub.1 -C.sub.30 -alkyl whose carbon chain may be interrupted by one or e of --O--, --S--, --NR.sup.1 --, --CO-- and/or --SO.sub.2 -- and which may be monosubstituted or polysubstituted by cyano, C.sub.1 -C.sub.6 -alkoxy or a 5-, 6- or 7-membered heterocyclic radical which is attached via a nitrogen atom and which may contain further heteroatoms and may be aromatic, whereR.sup.1 is hydrogen or C.sub.1 -C.sub.6 -alkyl;C.sub.5 -C.sub.8 -cycloalkyl whose carbon skeleton may be interrupted by one or more of --O--, --S-- and/or --NR.sup.1 --;aryl or hetaryl, which may each be monosubstituted or poly-substituted by C.sub.1 -C.sub.18 -alkyl, C.sub.1 -C.sub.6 -alkoxy, cyano, --CONHR.sup.2, --NHCOR.sup.2 and/or aryl- or hetaryl-azo, which may each be substituted by C.sub.1 -C.sub.10 -alkyl, C.sub.1 -C.sub.6 -alkoxy or cyano, whereR.sup.2 is hydrogen; C.sub.1 -C.sub.18 -alkyl; aryl or hetaryl, which may each be substituted by C.sub.1 -C.sub.6 -alkyl, C.sub.1 -C.sub.6 -alkoxy, halogen or cyano;X is halogen; C.sub.1 -C.sub.18 -alkyl; aryloxy, arylthio, hetaryloxy or hetarylthio, which may each be substituted by C.sub.1 -C.sub.4 -alkyl or C.sub.1 -C.sub.4 -alkoxy;n is from 2 to 12,their preparation and use as pigments or fluorescent dyes.
摘要翻译： PCT No.PCT / EP96 / 00118 Sec。 371日期1997年7月21日 102（e）日期1997年7月21日PCT 1996年1月12日PCT PCT。公开号WO96 / 22332 日期：1996年7月25日四氢四羧酸二酰亚胺其中R为氢; 其碳链可以被-O - ， - S - ， - NR 1 - ， - CO - 和/或-SO 2 - 中的一个或多个中断的C 1 -C 30 - 烷基，并且其可以被氰基，C 1 -C 6单取代或多取代 - 烷氧基或5-，6-或7-元杂环基，其通过氮原子连接并且可以含有另外的杂原子并且可以是芳族的，其中R 1是氢或C 1 -C 6 - 烷基; 碳骨架可被-O - ， - S-和/或-NR1-中的一个或多个中断的C 5 -C 8 - 环烷基; 芳基或杂芳基，其可以各自被C1-C18-烷基，C1-C6-烷氧基，氰基，-CONHR2，-NHCOR2和/或芳基 - 或杂芳基 - 偶氮基单取代或多取代，其可以各自被C1 C 1-10 - 烷基，C 1 -C 6 - 烷氧基或氰基，其中R 2是氢; C1-C18-烷基; 芳基或杂芳基，其各自可被C 1 -C 6 - 烷基，C 1 -C 6 - 烷氧基，卤素或氰基取代; X是卤素; C1-C18-烷基; 芳氧基，芳硫基，杂芳氧基或杂芳硫基，其各自可被C 1 -C 4 - 烷基或C 1 -C 4 - 烷氧基取代; n为2至12，它们的制备和用作颜料或荧光染料。

6. 发明授权

US5376507A Method to produce nonlinear optical microcomponents 失效
标题翻译：制造非线性光学微元件的方法
公开(公告)号：US5376507A
公开(公告)日：1994-12-27
申请号：US2822
申请日：1993-01-08
申请人： Wolfgang Ehrfeld , Herbert O. Moser , Klaus Mullen , Christoph Bubeck , Hans-Dieter Bauer
发明人： Wolfgang Ehrfeld , Herbert O. Moser , Klaus Mullen , Christoph Bubeck , Hans-Dieter Bauer
IPC分类号： G02F1/35 , G02F1/065 , G03F7/00 , G03F7/20 , G02B6/10
CPC分类号： G03F7/00 , G02F1/065 , G03F7/2039 , Y10S430/168
摘要： A method to produce nonlinear optical microcomponents is described which employs hitherto not yet used material combinations. Not only waveguide structures are produced by means of X-ray depth lithography, but also microcell structures, into which materials having nonlinear optical properties are introduced. The microstructure is produced as a positive mold part, from which there is subsequently generated, by means of electroforming, a mold insert, a negative of which is made using a polymer material. After the molding operation the microstructure is applied to a substrate, and nonlinear optical material, covered by a cover plate if needed or desired, is introduced into the microcell structure.
摘要翻译：描述了一种生产非线性光学微元件的方法，该方法采用迄今未使用的材料组合。不仅通过X射线深度光刻产生波导结构，而且还引入了具有非线性光学特性的材料的微单元结构。微结构作为正模具部件生产，随后通过电铸产生模具插入件，模具插件的负极由聚合物材料制成。在模制操作之后，将微结构施加到基板上，并且如果需要或期望，则由盖板覆盖的非线性光学材料被引入到微单元结构中。

7. 发明申请

US20060075585A1 Rylene dyes 失效
标题翻译：二烯染料
公开(公告)号：US20060075585A1
公开(公告)日：2006-04-13
申请号：US10522990
申请日：2003-07-25
申请人： Matthias Krieger , Arno Bohm , Lorenz Siggel , Stefan Becker , Klaus Mullen , Christopher Kohl
发明人： Matthias Krieger , Arno Bohm , Lorenz Siggel , Stefan Becker , Klaus Mullen , Christopher Kohl
IPC分类号： C09B49/00
CPC分类号： C09B5/62
摘要： Rylene dyes of the general formula I where the variables are defined as follows: R is hydrogen; optionally substituted C1-C30-alkyl, C5-C8-cycloalkyl, aryl or hetaryl; R′ is bromine; cyano; —NR32; optionally substituted aryloxy, arylthio, hetaryloxy or hetarylthio; optionally substituted C3-C18-alk-1-ynyl; X, Y are both hydrogen or together are a radical of the formula Ia n is 2, 3, 4 or additionally 1 when X and Y are a radical of the formula Ia; n′ is from 1 to 4; m is from 0 to 6.
摘要翻译：通式I的Rylene染料，其中变量定义如下：R是氢; 芳基或杂芳基;任选取代的C 1 -C 30 - 烷基，C 5 -C 8 - 环烷基，芳基或杂芳基; R'是溴; 氰基; -NR 3 3; 任选取代的芳氧基，芳硫基，杂芳氧基或杂芳硫基; 任选取代的C 3 -C 18 - 烷-1-基; 当X和Y是式Ia的基团时，X，Y都是氢或一起是式Ia n的基团是2,3,4或另外1， n'为1至4; m为0〜6。

8. 发明授权

US5376506A Method to produce nonlinear optical microcomponents 失效
标题翻译：制造非线性光学微元件的方法
公开(公告)号：US5376506A
公开(公告)日：1994-12-27
申请号：US1194
申请日：1993-01-07
申请人： Wolfgang Ehrfeld , Herbert O. Moser , Klaus Mullen , Christoph Bubeck , Hans-Dieter Bauer
发明人： Wolfgang Ehrfeld , Herbert O. Moser , Klaus Mullen , Christoph Bubeck , Hans-Dieter Bauer
IPC分类号： G02B6/12 , G02B6/13 , G02F1/065 , G02F1/35 , G03F7/00 , G02B6/10
CPC分类号： G02B6/13 , G02F1/065 , G03F7/0005 , G02B2006/12069 , Y10S430/168
摘要： A method to produce nonlinear optical microcomponents is described which makes it possible to employ material combinations not yet used to date. By means of X-ray depth lithography not only waveguide structures, but also microcell structures are produced, into which subsequently material of nonlinear optical properties is placed. By means of X-ray depth lithography and micromolding techniques a mold insert with a waveguide structure is produced as a positive mold, and the waveguide structure is impressed into a polymer base material by means of the mold insert. Then the impressed waveguide structure is filled with optically linear material, and after the filling operation at least one microcell structure is produced, at least in the areas of the optically linear material, into which microcell structure optically nonlinear material is placed. The microcell structure may also be impressed by means of another mold insert.
摘要翻译：描述了一种产生非线性光学微元件的方法，其使得可能采用迄今尚未使用的材料组合。通过X射线深度光刻，不仅产生波导结构，而且产生微孔结构，随后放置非线性光学性质的材料。通过X射线深度光刻和显微成像技术，制造具有波导结构的模具插件作为正模，并且通过模具插入件将波导结构压入聚合物基体材料。然后用光学线性材料填充印制的波导结构，并且在填充操作之后，至少在光学线性材料的区域中产生至少一个微单元结构，微孔结构光学非线性材料被放置到该区域中。微孔结构也可以通过另一个模具插入物来施加压力。

9. 发明申请

US20100187482A1 Highly Conductive, Transparent Carbon Films as Electrode Materials 审中-公开
标题翻译：高导电，透明碳膜作为电极材料
公开(公告)号：US20100187482A1
公开(公告)日：2010-07-29
申请号：US12596478
申请日：2008-04-18
申请人： Klaus Mullen , Xuan Wang , Linjie Zhi
发明人： Klaus Mullen , Xuan Wang , Linjie Zhi
IPC分类号： H01B1/04 , B05D5/12
CPC分类号： C09D5/24 , B82Y10/00 , G01N27/305 , H01L31/022466 , H01L31/1884 , H01L51/444 , H01L51/5206 , Y02E10/549 , Y02P70/521
摘要： The present invention relates to an optically transparent conductive carbon-based film which is suitable for use as an electrode in optoelectronic devices etc. Further, the invention relates to a process for the production of the transparent conductive carbon film and the use thereof in electronic devices. Organic solar cells using transparent conductive carbon film as electrode display comparable performance with cells using ITO. These carbon films show high thermal and chemical stability, ultra-smooth surface, and good adhesion to substrates.
摘要翻译：本发明涉及适合用作光电子器件等中的电极的光学透明导电性碳基膜。此外，本发明涉及一种用于制造透明导电性碳膜的方法及其在电子设备中的应用。使用透明导电碳膜作为电极的有机太阳能电池显示与使用ITO的电池相当的性能。这些碳膜显示出高的热和化学稳定性，超光滑的表面和对基材的良好粘合性。

10. 发明申请

US20080188660A1 Hexarylene and Pentarylene Tetracarboxylic Acid Diimides 有权
标题翻译：六亚甲基和五亚甲基四羧酸二酰亚胺
公开(公告)号：US20080188660A1
公开(公告)日：2008-08-07
申请号：US11910944
申请日：2006-04-13
申请人： Neil Gregory Pschirer , Christopher Kohl , Klaus Mullen
发明人： Neil Gregory Pschirer , Christopher Kohl , Klaus Mullen
IPC分类号： C07D221/18
CPC分类号： C09B5/62 , C07D471/06
摘要： Rylenetetracarboximides of the general formula I in which the variables are defined as follows: R are identical or different radicals: hydrogen; alkyl, cycloalkyl, aryl or hetaryl, each substituted if desired; R′ are identical or different radicals: hydrogen; aryloxy, arylthio, hetaryloxy or hetarylthio, each substituted if desired; n is 1 or 2, and also a process for preparing the rylenetetracarboximides I and their use for coloring high molecular weight organic and inorganic materials, for preparing aqueous polymer dispersions which absorb in the near infrared region of the electromagnetic spectrum, for producing markings and inscriptions which absorb infrared light and are invisible to the human eye, as infrared absorbers for heat management, as IR laser beam-absorbing materials in fusion treatment of plastics parts, and also as active components in photovoltaics.
摘要翻译：其中变量定义如下：通式I的Ryl tetracarboximides：R是相同或不同的基团：氢; 烷基，环烷基，芳基或杂芳基，如果需要，各自被取代; R'是相同或不同的基团：氢; 芳氧基，芳硫基，杂芳氧基或杂芳硫基，如果需要，各自被取代; n为1或2，也是制备四环四甲酰亚胺I的方法及其用于着色高分子量有机和无机材料的用途，用于制备在电磁谱的近红外区域吸收的聚合物分散体，用于产生标记和铭文其吸收红外光并且对于人眼是不可见的，作为用于热管理的红外吸收剂，作为用于塑料部件的熔融处理的IR激光束吸收材料，以及作为光伏的有源组件。

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