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1. 发明授权

US5728480A Poly(4,5,9,10-tetrahydropyrene-2,7-diyl) derivatives and their use as electroluminescence materials 失效
标题翻译：聚（4,5,9,10-四氢芘-2,7-二基）衍生物及其作为电致发光材料的用途
公开(公告)号：US5728480A
公开(公告)日：1998-03-17
申请号：US521263
申请日：1995-08-30
申请人： Roland Stern , Donald Lupo , Josef Salbeck , Hermann Schenk , Thomas Stehlin , Klaus Mullen , Martin Kreyenschmidt , Ullrich Scherf
发明人： Roland Stern , Donald Lupo , Josef Salbeck , Hermann Schenk , Thomas Stehlin , Klaus Mullen , Martin Kreyenschmidt , Ullrich Scherf
IPC分类号： C07C25/22 , C07B61/00 , C07C17/12 , C08G61/00 , C08G61/10 , C09K11/06 , H01L51/30 , H01L51/50 , H05B33/12 , H05B33/14
CPC分类号： C09K11/06 , C07C17/12 , C08G61/10 , H01L51/0035 , C07C2103/50 , C09K2211/1408 , C09K2211/1416 , H01L51/0052 , Y10S428/917 , Y10T428/31504 , Y10T428/31678
摘要： Poly(4,5,9,10-tetrahydropyrene-2,7-diyl) derivatives of the formula (I) ##STR1## where the symbols R.sup.1 to R.sup.4 have the following meanings: R.sup.1, R.sup.2, R.sup.3, R.sup.4 are identically or variously H, a straight-chain or branched alkyl chain containing 1 to 22 carbon atoms, it being possible for one or more nonadjacent CH.sub.2 groups also to be replaced by --O--, --COO--, --OOC-- and/or phenylene, aryl or aryloxy groups, it being possible for the aromatic to be substituted by C.sub.1 -C.sub.22 -alkyl, C.sub.1 -C.sub.22 -alkoxy, Br, Cl, F, CN, and/or NO.sub.2, Br, Cl, F, CN, NO.sub.2, or carboalkoxy containing 2 to 23 carbon atoms; n is 10 to 150, are suitable as electroluminescence materials.
摘要翻译：式（I）的（4,5,9,10-四氢苯-2,7-二基）衍生物其中符号R1至R4具有下列含义：R1，R2，R3，R4分别为同样或各种H，含有1至22个碳原子的直链或支链烷基链，一个或多个不相邻的CH 2基团也可以被-O - ， - COO - ， - OOC-和/或亚苯基代替芳基或芳氧基，芳香族可以被C 1 -C 22 - 烷基，C 1 -C 22 - 烷氧基，Br，Cl，F，CN和/或NO 2，Br，Cl，F，CN，NO 2 或含有2至23个碳原子的烷氧羰基; n为10〜150，适合作为电致发光材料。

2. 发明授权

US5712361A Conjugated polymers containing ANSA substructures and their use as electroluminescence materials 失效
标题翻译：含有ANSA亚结构的共轭聚合物及其作为电致发光材料的用途
公开(公告)号：US5712361A
公开(公告)日：1998-01-27
申请号：US496202
申请日：1995-06-28
申请人： Roland Stern , Donald Lupo , Josef Salbeck , Hermann Schenk , Thomas Stehlin , Klaus Mullen , Ullrich Scherf , Joachim Huber
发明人： Roland Stern , Donald Lupo , Josef Salbeck , Hermann Schenk , Thomas Stehlin , Klaus Mullen , Ullrich Scherf , Joachim Huber
IPC分类号： C08G61/00 , C08G61/02 , C09K11/06 , H01L51/50 , H05B33/14 , C08G61/12
CPC分类号： H05B33/14 , C08G61/02 , C09K11/06 , Y10S428/917
摘要： Conjugated polymers containing ansa substructures and their use as electroluminescence materials. Conjugated polymers containing ansa substructures, which contain aromatic groups and in which adjacent aromatic groups are connected to one another in such a way that one ring atom of one aromatic group is directly linked to one ring atom of the other aromatic group and any further linkages of these two aromatic groups are possible only via a bridge containing at least one tetravalent carbon atom and/or heteroatom. The polymers of the invention having ansa substructures are outstandingly suitable as electroluminescence materials, since they have a very high color purity.
摘要翻译：含有ansa亚结构的共轭聚合物及其作为电致发光材料的用途。含有芳族基团的共轭聚合物，其中相邻芳族基团彼此连接，其中一个芳族基团的一个环原子直接与另一个芳族基团的一个环原子连接，这两个芳族基团仅通过含有至少一个四价碳原子和/或杂原子的桥可能。具有ansa子结构的本发明的聚合物非常适合作为电致发光材料，因为它们具有非常高的色纯度。

3. 发明授权

US5840217A Spiro compounds and their use as electroluminescence materials 失效
标题翻译：螺环化合物及其作为电致发光材料的用途
公开(公告)号：US5840217A
公开(公告)日：1998-11-24
申请号：US417390
申请日：1995-04-05
申请人： Donald Lupo , Josef Salbeck , Hermann Schenk , Thomas Stehlin , Roland Stern , Arno Wolf
发明人： Donald Lupo , Josef Salbeck , Hermann Schenk , Thomas Stehlin , Roland Stern , Arno Wolf
IPC分类号： C07D307/79 , C07C13/72 , C07C211/61 , C07D213/06 , C07D263/32 , C07D263/56 , C07D271/10 , C07D271/107 , C07D307/80 , C09K11/06 , H01L51/30 , H01L51/50 , H05B33/14 , G02F1/00 , H01B1/00 , H01J1/62
CPC分类号： H01L51/0052 , C07C13/72 , C07D271/107 , C07D307/80 , C09B69/105 , C09B69/109 , C09K11/06 , H01L51/0062 , H05B33/14 , C07C2103/18 , C07C2103/94 , H01L2251/308 , H01L51/0059 , H01L51/0069 , H01L51/007 , H01L51/0071 , H01L51/0073
摘要： Use of spiro compounds of the formula (I) ##STR1## where K.sup.1 and K.sup.2 are, independently of one another, conjugated systems, in electroluminescence devices. Preferred compounds of the formula (I) are 9,9'-spirobifluorene derivatives of the formula (II) ##STR2## where the benzo groups can be substituted independently of one another. Compounds of the formula (I) have a good solubility in customary organic solvents, improved film-forming properties and a significantly reduced tendency to crystallize. The production of electroluminescence devices is thereby made easier and their service life is increased.
摘要翻译：在电致发光器件中使用式（I）的化合物（I）其中K1和K2彼此独立地是共轭体系。优选的式（I）化合物是式（Ⅱ）的9,9'-螺二芴衍生物，其中苯并基可彼此独立地取代。式（I）化合物在常规有机溶剂中具有良好的溶解性，改善的成膜性能和显着降低的结晶倾向。因此，电致发光器件的制造变得更容易并且其使用寿命增加。

4. 发明授权

US5621131A Conjugated polymers having spiro centers and their use as electroluminescence materials 失效
标题翻译：具有螺旋中心的共轭聚合物及其作为电致发光材料的用途
公开(公告)号：US5621131A
公开(公告)日：1997-04-15
申请号：US541237
申请日：1995-10-12
申请人： Willi Kreuder , Donald Lupo , Josef Salbeck , Hermann Schenk , Thomas Stehlin
发明人： Willi Kreuder , Donald Lupo , Josef Salbeck , Hermann Schenk , Thomas Stehlin
IPC分类号： C07C17/35 , C07C25/22 , C07C69/00 , C08G61/00 , C08G61/02 , C09K11/06 , H01L51/30 , H01L51/50 , H05B33/14 , C07C22/00 , C08G59/00
CPC分类号： H05B33/14 , C07C17/35 , C07C25/22 , C07C69/00 , C08G61/00 , C09B69/101 , C09B69/102 , C09B69/105 , C09B69/109 , C09K11/06 , H01L51/0035 , H01L51/0036 , H01L51/0039 , H01L51/0043 , C07C2103/00 , H01L51/0052 , H01L51/0062 , H01L51/5012
摘要： Conjugated polymers comprising recurring units of the formula (I), ##STR1## A, B, C, D are identical or different and are each from one to fifteen identical or different arylene and/or heteroarylene and/or vinylene groups which, like the spirobifluorene skeleton itself, may be unsubstituted or substituted;S are identical or different substituents;m, n are 0 or 1.The polymers of the invention having the formula (I) are suitable as electroluminescence materials and have, in particular, a high color purity of the emission.
摘要翻译：包含式（I），（I）A，B，C，D的重复单元的共轭聚合物是相同或不同的，各自为1至15个相同或不同的亚芳基和/或亚杂芳基和/或亚乙烯基，如螺二芴骨架本身，可以是未取代的或取代的; S是相同或不同的取代基; m，n为0或1.具有式（I）的本发明的聚合物适合作为电致发光材料，特别是发光的高色纯度。

5. 发明授权

US5741921A Conjugated polymers containing hetero-spiro atoms and their use as electroluminescence materials 失效
标题翻译：含有杂 - 螺原子的共轭聚合物及其作为电致发光材料的用途
公开(公告)号：US5741921A
公开(公告)日：1998-04-21
申请号：US817376
申请日：1997-04-17
申请人： Willi Kreuder , Donald Lupo , Josef Salbeck , Hermann Schenk , Thomas Stehlin
发明人： Willi Kreuder , Donald Lupo , Josef Salbeck , Hermann Schenk , Thomas Stehlin
IPC分类号： H01L51/50 , C07F7/08 , C07F7/22 , C07F7/30 , C08G61/00 , C09K11/06 , H01L51/00 , H01L51/30
CPC分类号： C09K11/06 , C08G61/00 , H01L51/0035 , H01L51/0036 , H01L51/0043 , H01L51/0094 , H01L51/0052 , H01L51/0059 , H01L51/0062 , H01L51/007
摘要： Conjugated polymers comprising recurring units of the formula (I), ##STR1## where the symbols and indices have the following meanings: .psi. is an element of the 4th main group of the Periodic Table with the exception of carbon; D, E, F, G are identical or different and are each, for example, --O-- or a chemical bond; U is, for example, a chemical bond; V is, for example, as defined for U or is --O--; A are identical or different and are each, for example, H or a C.sub.1 -C.sub.20 -hydrocarbon radical; T is, for example, --O-- or --CA.dbd.CA--, where A is as defined above; K, L, M, Q are identical or different and are hydrocarbon radicals which can contain heteroatoms and have conjugated electron systems; m, n are identical or different and are 0, 1, 2, 3 or 4; are suitable as electroluminescence materials.
摘要翻译： PCT No.PCT / EP95 / 04594 371日期1997年04月17日 102（e）日期1997年4月17日PCT提交1995年11月22日PCT公布。公开号WO96 / 17036 日期1996年6月6日共轭聚合物包括式（I）的重复单元，其中符号和指数具有以下含义：psi是元素周期表第4主要元素的元素，碳; D，E，F，G相同或不同，各自为例如-O-或化学键; U是例如化学键; V例如为U定义或为-O-; A相同或不同，各自为例如H或C 1 -C 20烃基; T是例如-O-或-CA = CA-，其中A如上所定义; K，L，M，Q相同或不同，是可以含有杂原子并具有共轭电子系统的烃基; m，n相同或不同，为0,1,2,3或4; 适合用作电致发光材料。

6. 发明授权

US06329082B1 Hetero-spiro compounds and their use as electroluminescence materials 失效
标题翻译：杂环化合物及其作为电致发光材料的用途
公开(公告)号：US06329082B1
公开(公告)日：2001-12-11
申请号：US08836956
申请日：1997-05-22
申请人： Willi Kreuder , Donald Lupo , Josef Salbeck , Hermann Schenk , Thomas Stehlin
发明人： Willi Kreuder , Donald Lupo , Josef Salbeck , Hermann Schenk , Thomas Stehlin
IPC分类号： H05B3314
CPC分类号： H05B33/14 , C07F7/081 , C07F7/0812 , C07F7/30 , C08G61/00 , C09K11/06 , H01L51/0052 , H01L51/0059 , H01L51/0069 , H01L51/007 , H01L51/0094 , H01L2251/308 , Y10S428/917
摘要： Hetero-spiro compounds of the formula (I), where &PSgr; is an element of the 4th main group of the Periodic Table with the exception of carbon, preferably Sn, Ge or Si, particularly preferably Ge or Si, and K1 and K2 are, independently of one another, conjugated systems, for use in electroluminescence devices. The compounds of the formula (I) have a good solubility in customary organic solvents, improved film-forming properties and a significantly reduced tendency to crystallize.
摘要翻译：式（I）的杂 - 螺化合物，其中＆PSgr; 是元素周期表的第4主要元素，除了碳，优选Sn，Ge或Si，特别优选Ge或Si，并且K 1和K 2彼此独立地是用于电致发光器件的共轭体系。式（I）的化合物在常规有机溶剂中具有良好的溶解性，改善的成膜性能和显着降低的结晶倾向。

7. 发明授权

US5859211A Conjugated polymers containing heterospiro atoms and their use as electroluminescence materials 失效
标题翻译：含有杂环原子的共轭聚合物及其作为电致发光材料的用途
公开(公告)号：US5859211A
公开(公告)日：1999-01-12
申请号：US840843
申请日：1997-04-17
申请人： Willi Kreuder , Donald Lupo , Josef Salbeck , Hermann Schenk , Thomas Stehlin
发明人： Willi Kreuder , Donald Lupo , Josef Salbeck , Hermann Schenk , Thomas Stehlin
IPC分类号： C08G61/00 , C08G61/12 , C08G73/06 , C09K11/06 , H01L51/50 , H05B33/10 , C08G59/00
CPC分类号： H01L51/0043 , C08G61/00 , C08G73/0672 , C08G73/0688 , C09K11/06 , H01L51/5012
摘要： A conjugated polymer comprising repeating units of the formula (I), ##STR1## where the symbols and indices have the following meanings: .PSI. is an element of the 4th main group of the Periodic Table with the exception of carbon;D, E, F, G are identical or different and are --CR.sup.1 R.sup.2 --, --O--, --S--, --NR.sup.3 -- or a chemical bond;U is --CR.sup.4 .dbd.CR.sup.5 -- or a chemical bond;V is as defined for U or is --CR.sup.1 R.sup.2 --, --O--, --S--, --NR.sup.3 --, --SiR.sup.1 R.sup.2 --, --SO.sub.2 --, --O--, --CO--;A are identical or different and are H, a C.sub.1 --C.sub.20 -hydrocarbon radical which can also contain heteroatoms;T is --O--, --S--, --NR.sup.3 --, --CR.sup.1 R.sup.2 --, --CH.dbd.N--, --CA.dbd.CA--, --CH.dbd.CA--, --CH.dbd.CF-- or --CF.dbd.CF--;K, Q are identical or different hydrocarbon radicals which can contain heteroatoms and have conjugated electron systems;M, L are H or a straight-chain or branched alkyl group having from 1 to 22 carbon atoms, Br, Cl, F, CN, NO.sub.2 or CF.sub.3 ;m, n are identical or different and are 0, 1, 2, 3 or 4; and wherein said polymer is suitable as an electroluminescence material.
摘要翻译：包含式（I），（I）的重复单元的共轭聚合物，其中符号和指数具有以下含义：PSI是元素周期表第4主要组分的元素，除了碳; D，E，F，G相同或不同，为-CR1R2-，-O - ， - S-，-NR3-或化学键; U是-CR4 = CR5-或化学键; V如对于U或为-CR 1 R 2 - ， - O - ， - S - ， - NR 3 - ， - SiR 1 R 2 - ， - SO 2 - ， - O - ， - CO- A相同或不同，为H，也可含有杂原子的C 1 -C 20烃基; T是-O - ， - S - ， - NR 3 - ， - CR 1 R 2 - ， - CH = N-，-CA = CA-，-CH = CA-，-CH = CF-或-CF = CF-; K，Q是可以含有杂原子并具有共轭电子系统的相同或不同的烃基; M，L是H或具有1至22个碳原子的直链或支链烷基，Br，Cl，F，CN，NO 2或CF 3; m，n相同或不同，为0,1,2,3或4; 并且其中所述聚合物适合作为电致发光材料。

8. 发明授权

US5885368A Photovoltaic cell 失效
标题翻译：光伏电池
公开(公告)号：US5885368A
公开(公告)日：1999-03-23
申请号：US712426
申请日：1996-09-11
申请人： Donald Lupo , Josef Salbeck
发明人： Donald Lupo , Josef Salbeck
IPC分类号： H01L31/04 , C07C13/72 , C07C17/12 , C07C25/22 , H01L31/0256 , H01L31/06 , H01L51/00 , H01L51/30 , H01M14/00
CPC分类号： H01L51/0058 , C07C17/12 , C07C25/22 , H01L51/0094 , H01L51/4226 , C07C2103/18 , C07C2103/94 , H01L2251/306 , H01L51/0035 , H01L51/0059 , H01L51/007 , H01L51/0084 , Y02E10/549 , Y02P70/521
摘要： A photovoltaic cell having a charge transport layer comprising a hole conductor material is disclosed and claimed. The photovoltaic cell comprising a light absorbing layer having a semiconductor material with a bassed gap of at least 3.0 Ev, the surface of the semiconductor having a roughness of >20, optionally a sensitizer layer, a charge transport layer comprising one or more spiro compounds of the formula (I) as a hole conductor material ##STR1## where .PSI. is C, Si, Ge or Sn, andK.sup.1 and K.sup.2, independently of one another, are conjugated systems,and a counter electrode.
摘要翻译：公开并要求具有包含空穴导体材料的电荷传输层的光伏电池。该光伏电池包括具有至少3.0Ve的低音间隙的半导体材料的光吸收层，半导体的表面粗糙度> 20，任选的敏化剂层，电荷传输层，其包含一个或多个螺环化合物作为空穴导体材料（I）的式（I），其中PSI为C，Si，Ge或Sn，K1和K2彼此独立地为共轭体系和对电极。

9. 发明授权

US06335480B1 Photovoltaic cell 有权
标题翻译：光伏电池
公开(公告)号：US06335480B1
公开(公告)日：2002-01-01
申请号：US09381192
申请日：1999-11-24
申请人： Udo Bach , Michael Grätzel , Josef Salbeck , Frank Weissörtel , Donald Lupo
发明人： Udo Bach , Michael Grätzel , Josef Salbeck , Frank Weissörtel , Donald Lupo
IPC分类号： H01L3100
CPC分类号： H01L51/0058 , H01L51/0052 , H01L51/0054 , H01L51/0055 , H01L51/0059 , H01L51/006 , H01L51/0062 , H01L51/0064 , H01L51/007 , H01L51/0072 , H01L51/008 , H01L51/0086 , H01L51/0094 , H01L51/4226 , H01L2251/306 , Y02E10/549 , Y02P70/521
摘要： A photovoltaic cell comprising an electrolyte which comprises a hole conductor compound as redox system.
摘要翻译：一种包含电解质的光伏电池，其包含作为氧化还原体系的空穴导体化合物。

10. 发明授权

US06504042B1 Use of spiro compounds as materials in non-linear optics 失效
标题翻译：在非线性光学中使用螺状化合物作为材料
公开(公告)号：US06504042B1
公开(公告)日：2003-01-07
申请号：US08728780
申请日：1996-10-10
申请人： Donald Lupo , Josef Salbeck
发明人： Donald Lupo , Josef Salbeck
IPC分类号： G02F135
CPC分类号： G02F1/3617 , G02F1/3619
摘要： Spiro compounds of the formula I in which &psgr; is C, Si, Ge or Sn and K1 and K2 independently of one another are conjugated systems, are suitable as materials in nonlinear optics.
摘要翻译：其中psi是C，Si，Ge或Sn以及K1和K2彼此独立的式Iin的螺环化合物是共轭体系，适合作为非线性光学中的材料。

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