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1. 发明授权

US07015292B2 Silicon-containing olefin copolymer, crosslinkable rubber composition thereof, and use thereof 失效
标题翻译：含硅烯烃共聚物，其可交联橡胶组合物及其用途
公开(公告)号：US07015292B2
公开(公告)日：2006-03-21
申请号：US10499122
申请日：2002-12-26
申请人： Keiji Okada , Hidetatsu Murakami , Takashi Hakuta , Masaaki Kawasaki
发明人： Keiji Okada , Hidetatsu Murakami , Takashi Hakuta , Masaaki Kawasaki
IPC分类号： C08F130/08 , C08F10/00
CPC分类号： C08F210/18 , C08F210/02 , C08F210/06 , C08F210/16 , C08L23/0823 , C08L2666/02 , C08F232/00 , C08F2500/25 , C08F2500/17 , C08F2500/09 , C08F236/20 , C08F2500/03
摘要： A silicon-containing olefin copolymer is provided which comprises (a) a constituent unit derived from —CH2—CH2— such as ethylene, (b) a constituent unit derived from —CH2—CHR— where R is a hydrocarbon group of 1 to 18 carbon atoms, and (c) a constituent unit containing a specific silicon-containing group. A silicon-containing olefin copolymer is also provided which is obtainable by co-polymerizing ethylene, an a-olefin of 3 to 20 carbon atoms and a specific silicon-containing ethylene monomer.
摘要翻译：提供含硅烯烃共聚物，其包含（a）衍生自-CH 2 -CH 2 - 的结构单元，例如乙烯，（b）衍生自 -CH 2 - ，其中R是1至18个碳原子的烃基，和（c）含有特定含硅基团的构成单元。还提供了可通过使乙烯，3-20个碳原子的α-烯烃和特定的含硅乙烯单体共聚获得的含硅烯烃共聚物。

2. 发明申请

US20050038214A1 Silicon-containing olefin copolymer, crosslinkable rubber composition thereof, and use thereof 失效
标题翻译：含硅烯烃共聚物，其可交联橡胶组合物及其用途
公开(公告)号：US20050038214A1
公开(公告)日：2005-02-17
申请号：US10499122
申请日：2002-12-26
申请人： Keiji Okada , Hidetatsu Murakami , Takashi Hakuta , Masaaki Kawasaki
发明人： Keiji Okada , Hidetatsu Murakami , Takashi Hakuta , Masaaki Kawasaki
IPC分类号： C08F210/02 , C08F210/06 , C08F210/16 , C08F210/18 , C08L23/08 , C08F30/08
CPC分类号： C08F210/18 , C08F210/02 , C08F210/06 , C08F210/16 , C08L23/0823 , C08L2666/02 , C08F232/00 , C08F2500/25 , C08F2500/17 , C08F2500/09 , C08F236/20 , C08F2500/03
摘要： The first silicon-containing olefin copolymer of the present invention comprises (a) a constituent unit derived from —CH2—CH2—, (b) a constituent unit derived from —CH2—CHR— [R is a hydrocarbon group of 1 to 18 carbon atoms], and (c) a constituent unit containing a specific silicon-containing group, and has a molar ratio [(a)/(b)] of the constituent units (a) to the constituent units (b) of from 99/1 to 30/70, a content of the constituent unit (c) of from 0.1 to 10 mol % based on 100 mol % of the total amounts of the constituent units (a), (b) and (c), and a branching index of not less than 0.70. The second silicon-containing olefin copolymer of the present invention is obtainable by copolymerizing ethylene, an α-olefin of 3 to 20 carbon atoms and a specific silicon-containing ethylene monomer, and has a molar ratio of ethylene to α-olefin of from 99/1 to 30/70, an intrinsic viscosity, as measured in decalin at 135° C., of from 0.1 to 10 dl/g, a content of the ethylene monomer of from 0.1 to 10 mol % based on 100 mol % of the total amounts of ethylene, α-olefin and the ethylene monomer. These copolymers may be cross-linked and then submitted to use, and have a high cross-linking rate, excellent productivity, heat ageing properties, weathering resistance. They, further, can provide a rubber composition capable of preparing molded articles having excellent properties such as scratch resistance, resistance to compression set, electric properties and strength. They furthermore can provide sealing materials, potting materials, coating materials and adhesives made from the composition and also provide cross-linked articles of the composition.
摘要翻译：本发明的第一含硅烯烃共聚物包含（a）衍生自-CH 2 -CH 2 - 的构成单元，（b）衍生自-CH 2 -CHR-的结构单元[R是1至18碳的烃基原子]，（c）含有特定含硅基团的构成单元，构成单元（a）与构成单元（b）的摩尔比[（a）/（b）]为99 / 1〜30/70，构成单元（c）的含量相对于构成单元（a），（b）和（c）的总量的100摩尔％为0.1〜10摩尔％，分支指数不低于0.70。本发明的第二含硅烯烃共聚物可通过使乙烯，3-20个碳原子的α-烯烃和特定的含硅乙烯单体共聚而获得，并且乙烯与α-烯烃的摩尔比为99 / 1〜30/70，在135℃萘烷中测定的特性粘度为0.1〜10dl / g，乙烯单体的含量相对于100摩尔％为0.1〜10摩尔％乙烯，α-烯烃和乙烯单体的总量。这些共聚物可以交联，然后使用，具有高的交联速度，优异的生产率，热老化性能，耐候性。它们还可以提供能够制备具有优异性能如耐刮擦性，耐压缩变形性，电性能和强度的模制品的橡胶组合物。它们还可以提供由组合物制成的密封材料，灌封材料，涂料和粘合剂，并且还提供组合物的交联物品。

3. 发明申请

US20070219320A1 Process for Producing Rubber Composition, Rubber Composition and use Thereof 审中-公开
标题翻译：生产橡胶组合物，橡胶组合物的方法及用途
公开(公告)号：US20070219320A1
公开(公告)日：2007-09-20
申请号：US11587756
申请日：2005-04-28
申请人： Kotaro Ichino , Masao Kunizane , Yuji Ishii , Kunihide Hiraoka , Masaaki Kawasaki , Hidetatsu Murakami , Keiji Okada
发明人： Kotaro Ichino , Masao Kunizane , Yuji Ishii , Kunihide Hiraoka , Masaaki Kawasaki , Hidetatsu Murakami , Keiji Okada
IPC分类号： C08F8/00
CPC分类号： C08L21/00 , B60C1/0016 , C08K5/0016 , C08L9/00 , C08L23/16 , C08L2666/06 , C08L2666/08
摘要： A process for producing a rubber composition containing a nonconjugated polyene copolymer (A), a softener (B) and a diene rubber (C), comprising: a step of mixing a copolymer composition (I), said copolymer composition (I) comprising 100 parts by weight of a nonconjugated polyene copolymer (A), said nonconjugated polyene copolymer (A) being a random copolymer containing 96 to 70 mol % of the structural units derived from α-olefin (A1) and 4 to 30 mol % of the structural units derived from nonconjugated polyene (A2) and having a glass transition temperature (Tg) of −25 to 20° C., and 1 to 100 parts by weight of the softener (B); the diene rubber (C); and optionally further the softener (B). A tire tread using the rubber composition and a tire having the tire tread.
摘要翻译：一种制备含有非共轭多烯共聚物（A），软化剂（B）和二烯橡胶（C）的橡胶组合物的方法，包括：将共聚物组合物（I），所述共聚物组合物（I）重量份的非共轭多烯共聚物（A），所述非共轭多烯共聚物（A）是含有96-70％（摩尔）衍生自α-烯烃（A1）的结构单元和4-30％（摩尔）结构衍生自非共轭多烯（A2）并且玻璃化转变温度（Tg）为-25至20℃的单元和1至100重量份的软化剂（B）; 二烯橡胶（C）; 和任选地进一步的软化剂（B）。使用橡胶组合物的轮胎胎面和具有轮胎胎面的轮胎。

4. 发明授权

US06303727B1 Linear triene compound and copolymer 失效
标题翻译：线性三烯化合物和共聚物
公开(公告)号：US06303727B1
公开(公告)日：2001-10-16
申请号：US09320838
申请日：1999-05-26
申请人： Ken Maeda , Masaaki Yasuda , Terunori Fujita , Keiji Okada , Makoto Kamimura , Kazuyuki Takimoto , Hidetatsu Murakami , Masaaki Kawasaki , Keiji Watanabe
发明人： Ken Maeda , Masaaki Yasuda , Terunori Fujita , Keiji Okada , Makoto Kamimura , Kazuyuki Takimoto , Hidetatsu Murakami , Masaaki Kawasaki , Keiji Watanabe
IPC分类号： C08F13600
CPC分类号： C08F236/22 , C07C2/04 , C07C11/21 , C07C2527/24 , C07C2531/14
摘要： A novel and useful linear triene compound represented by the following formula (1) is co-polymerized with an &agr;-olefin to obtain an ethylenically unsaturated copolymer which is superior in weather-ability, heat resitance and fastness to ozone, together with superior scorch stability and vulcanizability at high velocity in which R1, R2, R3, R4, R5 and R6 stand each, independently of each other, for hydrogen atom or an alkyl having 1-3 carbon atoms, R7 represents an alkyl having 1-3 carbon atoms and n is an integer of 0-5, with the proviso that each of R4s or of R5s may be identical with or different from each other, respectively, when n is 2 or greater.
摘要翻译：由下式（1）表示的新型有用的线性三烯化合物与α-烯烃共聚，得到耐候性，耐热性和耐臭氧性优异的烯属不饱和共聚物，以及优异的焦烧稳定性和R 1，R 2，R 3，R 4，R 5和R 6各自独立地表示氢原子或具有1-3个碳原子的烷基的高速度下的硫化性，R7表示具有1-3个碳原子的烷基，n表示是0-5的整数，条件是当n为2或更大时，R 4或R 5中的每一个可以分别彼此相同或不同。

5. 发明申请

US20080188621A1 Rubber Composition and Use Thereof 审中-公开
标题翻译：橡胶组合物及其用途
公开(公告)号：US20080188621A1
公开(公告)日：2008-08-07
申请号：US11587904
申请日：2005-04-28
申请人： Kotaro Ichino , Masao Kunizane , Yuji Ishit , Kunihide Hiraoka , Masaaki Kawasaki , Hidetatsu Murakami , Keiji Okada
发明人： Kotaro Ichino , Masao Kunizane , Yuji Ishit , Kunihide Hiraoka , Masaaki Kawasaki , Hidetatsu Murakami , Keiji Okada
IPC分类号： C08L9/02
CPC分类号： C08L21/00 , B60C1/0016 , C08L9/00 , C08L9/02 , C08L23/16 , C08L53/00 , C08L2666/02 , C08L2666/08
摘要： Provided is a rubber composition which can give a tire excellent in braking performance and fuel consumption and which is excellent in mechanical strength and fatigue resistance, and a use thereof.The rubber composition of the present invention contains a (A) 60 to 0.1 parts by weight of a nonconjugated polyene copolymer, which is a random copolymer containing 96 to 70 mol % of the structural units derived from α-olefin (A1) and 4 to 30 mol % of the structural units derived from a nonconjugated polyene (A2), and has a glass transition temperature (Tg) of −25 to 20° C., (B) 40 to 99.9 parts by weight of a diene rubber and (C) at least one selected from the group consisting of specific polymers.
摘要翻译：提供一种橡胶组合物，其能够赋予制动性能和燃料消耗优异并且机械强度和耐疲劳性优异的轮胎及其用途。本发明的橡胶组合物含有（A）60〜0.1重量份的非共轭多烯共聚物，其是含有96〜70摩尔％的来自α-烯烃（A1）的结构单元和4〜衍生自非共轭多烯（A2）的结构单元的30摩尔％，玻璃化转变温度（Tg）为-25〜20℃，（B）为40〜99.9重量份的二烯系橡胶，（C ）选自由特定聚合物组成的组中的至少一种。

6. 发明授权

US06787623B1 Unconjugated cyclopolyene copolymer, rubber composition, and use 失效
标题翻译：未结合的环戊烯共聚物，橡胶组合物及用途
公开(公告)号：US06787623B1
公开(公告)日：2004-09-07
申请号：US09787890
申请日：2001-03-26
申请人： Hidetatsu Murakami , Keiji Okada , Masaaki Kawasaki , Kotaro Ichino
发明人： Hidetatsu Murakami , Keiji Okada , Masaaki Kawasaki , Kotaro Ichino
IPC分类号： C08F23620
CPC分类号： C08L21/00 , B60C1/0016 , C08F210/02 , C08F210/18 , C08L23/08 , C08L23/0823 , Y10T152/10495 , C08L2666/06 , C08L2666/04 , C08F236/20 , C08F2500/25 , C08F2500/17 , C08F210/06
摘要： A tire provided with a tire tread made from a rubber composition comprising (A) a random copolymer based on non-conjugated cyclic polyene comprising structural units originated from one or more &agr;-olefins (A1) and originated from one or more non-conjugated cyclic polyene (A2), the said random copolymer having a content of the structural unit(s) originated from one or more &agr;-olefins (A1) in the range of 93 to 70 mole %; a content of the structural unit originated from one or more non-conjugated cyclic polyene (A2) in the range of 7 to 30 mole %; an intrinsic viscosity [&eegr;], determined in decalin at 135° C., in the range of 0.01 to 20 dl/g; a glass transition temperature (Tg) of not higher than 40° C.; and an iodine value in the range of 50 to 150, and (B) a rubber based on diene, in a weight proportion of {the random copolymer based on non-conjugated cyclic polyene (A)} versus {the rubber based on diene (B)} in the range from 60/40 to 0.1/99.9 exhibits a superior braking performance and, compatible therewith, a superior driving fuel cost aspect.
摘要翻译：本发明提供一种轮胎胎面，其由橡胶组合物制成，该轮胎胎面由（A）基于非共轭环状多烯的无规共聚物构成，所述非共轭环多烯包含源自一种或多种α-烯烃（A1）的结构单元，并且源于一种或多种非共轭环多烯（A2），所述无规共聚物具有来源于一种或多种α-烯烃（A1）的结构单元的含量在93-70摩尔％范围内; 来自一种或多种7-30摩尔％的非共轭环状多烯（A2）的结构单元的含量; 在135℃的萘烷中测定的特性粘度η在0.01至20dl / g的范围内; 玻璃化转变温度（Tg）不高于40℃; 碘值在50〜150范围内，（B）基于二烯的橡胶，以{非共轭环状多烯（A）}为基准的无规共聚物）与{基于二烯的橡胶 B）}在60/40至0.1 / 99.9的范围内表现出优异的制动性能，并且与其兼容，具有优异的驱动燃料成本方面。

7. 发明申请

US20080064818A1 Nonconjugated Polyene Copolymer, Rubber Composition and Uses Thereof 审中-公开
标题翻译：非共轭多烯共聚物，橡胶组合物及其用途
公开(公告)号：US20080064818A1
公开(公告)日：2008-03-13
申请号：US11587755
申请日：2005-04-11
申请人： Hidetatsu Murakami , Keiji Okada , Kotaro Ichino , Masaaki Kawasaki , Hiroki Ebata , Yasuhiro Hasada , Shigenobu Ikenaga
发明人： Hidetatsu Murakami , Keiji Okada , Kotaro Ichino , Masaaki Kawasaki , Hiroki Ebata , Yasuhiro Hasada , Shigenobu Ikenaga
IPC分类号： C08L19/00 , C08F10/00
CPC分类号： C08F210/18 , B60C1/0016 , C08F236/20 , C08L21/00 , C08L23/145 , C08L23/16 , C08L2666/06 , C08F210/06 , C08F2500/25 , C08F2500/17
摘要： Disclosed are a conjugated polyene copolymer comprising a random copolymer having structural units derived from α-olefin (A1) of 2 to 20 carbon atoms and structural units derived from nonconjugated polyene (A2), said nonconjugated polyene copolymer having a glass transition temperature (Tg) of −25 to 20 □ and Mooney viscosity of [ML(1+4)100□] of 5 to 190; a rubber composition comprising the nonconjugated polyene copolymer and a diene-based rubber (B); a modifier for tires comprising the copolymer; a rubber material for tires comprising the rubber composition; a tire tread obtained from the rubber material for tires; and a tire having the tire tread.
摘要翻译：公开了包含具有衍生自2-20个碳原子的α-烯烃（A1）和来自非共轭多烯（A2）的结构单元的结构单元的无规共聚物的共轭多烯共聚物，所述非共轭多烯共聚物具有玻璃化转变温度（Tg） -25〜20□，门尼粘度[ML（1 + 4）100□]为5〜190; 包含非共轭多烯共聚物和二烯基橡胶（B）的橡胶组合物; 用于包含所述共聚物的轮胎的改性剂; 一种用于轮胎的橡胶材料，包括橡胶组合物; 从轮胎用橡胶材料获得的轮胎胎面; 以及具有轮胎胎面的轮胎。

8. 发明申请

US20070015893A1 Curable composition and its use 审中-公开
公开(公告)号：US20070015893A1
公开(公告)日：2007-01-18
申请号：US11515318
申请日：2006-09-05
申请人： Takashi Hakuta , Masaaki Kawasaki , Yoshiharu Kikuchi , Mitsunao Arino , Mitsuko Nagai , Hiroaki Sakaguchi , Masaki Sugawara , Masao Kishi , Kaoru Ueno , Takashi Abe , Michio Sekine
发明人： Takashi Hakuta , Masaaki Kawasaki , Yoshiharu Kikuchi , Mitsunao Arino , Mitsuko Nagai , Hiroaki Sakaguchi , Masaki Sugawara , Masao Kishi , Kaoru Ueno , Takashi Abe , Michio Sekine
IPC分类号： C08G77/60
CPC分类号： C09D123/16 , B32B17/1055 , C08F210/18 , C08F230/08 , C08L23/16 , C08L83/00 , C08L83/04 , C08L2312/08 , C09J123/16 , C08F210/06 , C08F2500/25 , C08F2500/21
摘要： The curable composition of the present invention contains (A1) a silyl-containing ethylene/α-olefin/non-conjugated polyene random copolymer rubber which has a structural unit derived from a norbornene compound as the non-conjugated polyene with at least one specific vinyl group at the terminal and contains a specific hydrolyzable silyl group, and (B) a compound, other than the rubber (A1), having a hydroxyl group and/or a hydrolyzable group, e.g., (B1) a compound having a silanol group and/or a compound which can react with moisture to form a compound having a silanol group in the molecule. This compound improves elongation of the cured product and residual surface tackiness, and, at the same time, is high in curing speed and capable of giving the cured product of high resistance to weather. It is suitable for, e.g., adhesives, tackifiers, paints, sealants, waterproof materials, spray materials, shaping materials and casting rubber materials.

9. 发明授权

US06864315B1 Crosslinkable rubber compositions and use thereof 有权
标题翻译：可交联橡胶组合物及其用途
公开(公告)号：US06864315B1
公开(公告)日：2005-03-08
申请号：US09673608
申请日：2000-03-14
申请人： Takashi Hakuta , Masaaki Kawasaki , Yoshiharu Kikuchi , Hidenari Nakahama , Taku Koda , Hiroshi Kameda , Shuichi Nonaka , Mikio Hosoya , Yuji Ishii , Mitsunao Arino , Tsutomu Nakamura , Satao Hirabayashi , Takeo Yoshida
发明人： Takashi Hakuta , Masaaki Kawasaki , Yoshiharu Kikuchi , Hidenari Nakahama , Taku Koda , Hiroshi Kameda , Shuichi Nonaka , Mikio Hosoya , Yuji Ishii , Mitsunao Arino , Tsutomu Nakamura , Satao Hirabayashi , Takeo Yoshida
IPC分类号： C08K5/00 , C08L23/16 , C08L83/04 , C08L47/00
CPC分类号： C08K5/0025 , C08L23/16 , C08L83/04 , C08L2312/08 , C08L2314/02 , C08L83/00
摘要： The crosslinkable rubber composition of the invention is crosslinkable by hot air, and a hot-air crosslinked rubber sheet thereof has no scratch on the surface in a hardness test using a pencil of HB and has a compression set of not more than 70% after a heat treatment at 150° C. for 22 hours. The rubber composition comprises an ethylene/α-olefin/non-conjugated polyene random copolymer rubber comprising a specific vinyl end group-containing norbornene compound, a SiH group-containing compound having at least two SiH groups in one molecule, and if necessary, an addition reaction catalyst comprising a platinum group element and a reaction inhibitor. The automobile weatherstrip, hose, rubber vibration insulator, belt, sealing material, expanded product, covered electric wire, electric wire joint, electric insulating part and household rubber product according to the invention comprise the above-mentioned rubber composition. The rubber composition has a high crosslinking rate and excellent productivity to produce crosslinked rubber molded products, is capable of undergoing hot-air crosslinking such as HAV or UHF and is capable of providing crosslinked rubber molded products having excellent compression set resistance, strength properties, heat resistance, weathering resistance and abrasion resistance.
摘要翻译：本发明的交联性橡胶组合物可以通过热风进行交联，在使用HB的铅笔的硬度试验中，热风交联橡胶片在表面没有刮痕，并且在a后的压缩永久变形为70％以上在150℃下热处理22小时。该橡胶组合物包含一个乙烯/α-烯烃/非共轭多烯无规共聚物橡胶，其包含特定的含乙烯基端基的降冰片烯化合物，在一个分子中具有至少两个SiH基团的含SiH基化合物，如果需要，包含铂族元素和反应抑制剂的加成反应催化剂。根据本发明的汽车密封条，软管，橡胶振动绝缘子，带，密封材料，膨胀产品，包覆电线，电线接头，电绝缘部件和家用橡胶制品包括上述橡胶组合物。橡胶组合物具有高交联率和优异的生产交联橡胶成型体的生产率，能够进行热风交联如HAV或UHF，并且能够提供具有优异的耐压缩变形性，强度性能，热性能的交联橡胶模制产品耐电阻，耐候性和耐磨性。

10. 发明授权

US6140441A Ethylenic random copolymer, process for preparing the same, and rubber composition 失效
标题翻译：乙烯无规共聚物，其制备方法和橡胶组合物
公开(公告)号：US6140441A
公开(公告)日：2000-10-31
申请号：US983636
申请日：1998-03-30
申请人： Takashi Hakuta , Mikio Hosoya , Tetsuo Tojo , Masaaki Kawasaki
发明人： Takashi Hakuta , Mikio Hosoya , Tetsuo Tojo , Masaaki Kawasaki
IPC分类号： C08F4/68 , C08F210/18
CPC分类号： C08F210/18
摘要： A process for preparing an ethylene/.alpha.-olefin/norbornene nonconjugated polyene random copolymer, comprising preparing an ethylene random copolymer simultaneously meeting the following requirements (1) to (5):(1) the molar ratio of ethylene (a) to an .alpha.-olefin (b) having 3 to 20 carbon atoms ranges from 40:60 to 95:5;(2) a given amount of non conjugated polyene (c) has a norbornene skeleton;(3) the available network chain density .nu. is not less than 1.5.times.10.sup.20 /cm.sup.3 after press cross-linking of the copolymer using a dicumyl peroxyde;(4) the ratio of the rate .gamma.1 of shear showing a shearing stress of 0.4.times.10.sup.6 dyn/cm.sup.2 as determined from the melt flow curve at 100.degree. C. and the rate .gamma.2 of shear showing a shearing stress of 2.4.times.10.sup.6 dyn/cm.sup.2, that is .gamma.2/.gamma.1 and the available network chain density .nu. has a relationship represented by the following general formula: 0.04.times.10.sup.-19 .ltoreq.Log(.gamma.2/.gamma.1)/.nu..ltoreq.0.20.times.10.sup.-19 ; and(5) the intrinsic viscosity [.eta.] ranges from 0.5 to 10 dl/g as measured in decalin at 135.degree. C. The copolymer has excellent cross-linkability, can be cross-linked with a small amount of a peroxide or the like, and a cross-linked rubber composition prepared using this copolymer has excellent heat aging resistance, mechanical strength, weather resistance, and oxone resistance.
摘要翻译： PCT No.PCT / JP97 / 01815 Sec。 371日期1998年3月30日 102（e）1998年3月30日PCT PCT 1997年5月28日PCT公布。公开号WO97 / 45466 日期1997年12月4日制备乙烯/α-烯烃/降冰片烯非共轭多烯无规共聚物的方法，包括同时制备满足以下要求（1）至（5）的乙烯无规共聚物：（1）乙烯 a）具有3至20个碳原子的α-烯烃（b）的范围为40:60至95:5; （2）给定量的非共轭多烯（c）具有降冰片烯骨架; （3）使用二枯基过氧化物压制交联共聚物后，可用的网络链密度nu不小于1.5×10 20 / cm 3; （4）从100℃的熔体流动曲线确定的剪切应力为剪切应力为0.4×10 6 dyn / cm 2的剪切速率γ1与剪切应力为2.4×10 6 dyn / cm 2，即γ2 /γ1，可用的网络链密度nu具有由以下通式表示的关系：0.04×10-19

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