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1. 发明授权

US07799956B2 Process for producing phenol and methyl ethyl ketone 失效
标题翻译：苯酚和甲基乙基酮的制备方法
公开(公告)号：US07799956B2
公开(公告)日：2010-09-21
申请号：US11660065
申请日：2005-08-05
申请人： Jane Chi-ya Cheng , John S. Buchanan , Doron Levin , Michael A. Steckel , Jihad M. Dakka , James P. Stokes , John L. Robbins , Jon E. Stanat , Charles M. Smith , José G. Santiesteban
发明人： Jane Chi-ya Cheng , John S. Buchanan , Doron Levin , Michael A. Steckel , Jihad M. Dakka , James P. Stokes , John L. Robbins , Jon E. Stanat , Charles M. Smith , José G. Santiesteban
IPC分类号： C07C45/00 , C07C37/08
CPC分类号： C07C37/08 , C07C45/53 , C07C409/08 , C07C2529/70 , Y02P20/127 , Y02P20/52 , C07C49/10 , C07C39/04
摘要： A process for producing phenol and methyl ethyl ketone comprises contacting benzene with a C4 alkylating agent under alkylation conditions with catalyst comprising zeolite beta or a molecular sieve having an X-ray diffraction pattern including d-spacing maxima at 12.4±0.25, 6.9±0.15, 3.57±0.07 and 3.42±0.07 Angstrom to produce an alkylation effluent comprising sec-butylbenzene. The sec-butylbenzene is then oxidized to produce a hydroperoxide and the hydroperoxide is decomposed to produce phenol and methyl ethyl ketone.
摘要翻译：一种生产苯酚和甲基乙基酮的方法包括在烷基化条件下使苯与C4烷基化剂与包含β沸石的催化剂或具有包含d-间距最大值的X射线衍射图的分子筛在12.4±0.25,6.9±0.15， 3.57±0.07和3.42±0.07埃，以产生包含仲丁基苯的烷基化流出物。然后将仲丁基苯氧化生成氢过氧化物，氢过氧化物分解生成苯酚和甲基乙基酮。

2. 发明授权

US5346871A Catalyst for dehydrogenation of paraffins 失效
标题翻译：石蜡脱氢催化剂
公开(公告)号：US5346871A
公开(公告)日：1994-09-13
申请号：US28442
申请日：1993-03-09
申请人： John L. Robbins , Elise Marucchi-Soos , Jack W. Johnson , John F. Brody
发明人： John L. Robbins , Elise Marucchi-Soos , Jack W. Johnson , John F. Brody
IPC分类号： B01J23/60 , B01J23/62 , B01J29/04 , C07C5/32 , C07C5/333 , B01J21/16 , B01J23/06 , B01J23/08
CPC分类号： B01J29/049 , B01J23/60 , B01J23/62 , C07C5/325 , C07C5/3337
摘要： The present invention is directed to a novel catalyst composition and its use in the dehydrogenation of paraffins to olefins. The catalyst comprises an alloy of a Group VIII noble metal and a metal selected from the group consisting of zinc and gallium on a support selected from the group consisting of silica, zinc oxide modified silica and zinc oxide modified silica-pillared clays when said alloy is a zinc alloy, and silica, gallium oxide modified silica and gallium oxide modified silica-pillared clays when said alloy is a gallium alloy. The instant catalyst is an active and selective catalyst for the catalytic dehydrogenation of paraffins to olefins, especially gaseous paraffins, having the added benefit of retaining high activity and selectivity even following repeated regeneration by calcination in oxygen containing gas at temperatures of 450.degree. C. to 650.degree. C., preferably 450.degree. C. to 500.degree. C.
摘要翻译：本发明涉及新型催化剂组合物及其在链烷烃脱氢成烯烃中的应用。所述催化剂包含由选自二氧化硅，氧化锌改性二氧化硅和氧化锌改性二氧化硅柱状粘土的载体上的第八族贵金属和选自锌和镓的金属的合金，当所述合金为锌合金，二氧化硅，氧化镓改性二氧化硅和氧化镓改性二氧化硅柱状粘土。本催化剂是用于将链烷烃催化脱氢成烯烃，特别是气态烷烃的活性和选择性催化剂，具有保持高活性和选择性的附加益处，即使在含氧气体中通过在450℃至450℃的温度下煅烧反复再生， 650℃，优选450℃至500℃

3. 发明申请

US20100083575A1 Co-gasification process for hydrocarbon solids and biomass 有权
标题翻译：烃固体和生物质的共同气化过程
公开(公告)号：US20100083575A1
公开(公告)日：2010-04-08
申请号：US12586872
申请日：2009-09-29
申请人： Ramesh Varadaraj , John L. Robbins , Michael Siskin
发明人： Ramesh Varadaraj , John L. Robbins , Michael Siskin
IPC分类号： C10J3/00
CPC分类号： C10J3/72 , C10J3/466 , C10J3/54 , C10J3/66 , C10J2300/092 , C10J2300/0926 , C10J2300/093 , C10J2300/0943 , C10J2300/0993 , C10J2300/1884 , Y02E50/32 , Y02P20/145 , Y02T50/678
摘要： A process for the co-gasification of carbonaceous solids (coal, coke) and biomass in which the biomass material is pyrolyzed to provide a biomass pyrolysis oil and biomass char or coke which are then mixed with the carbonaceous solid to form a slurry. This slurry is then heated if necessary to achieve a viscosity which can be processed conveniently in the gasifier. The heat required for pyrolyzing the biomass can conveniently be obtained from the heat exchanger used to cool the hot synthesis gas product emerging from the gasifier.
摘要翻译：一种用于碳质固体（煤，焦炭）和生物质的共同气化的方法，其中生物质材料被热解以提供生物质热解油和生物质焦炭或焦炭，然后将其与碳质固体混合以形成浆料。如果需要，则将该浆料加热以达到可在气化器中方便地加工的粘度。热解生物质所需的热量可以方便地从用于冷却从气化器出来的热合成气产品的热交换器获得。

4. 发明授权

US5137620A Reforming process using a pretreated catalyst 失效
标题翻译：使用预处理催化剂的重整工艺
公开(公告)号：US5137620A
公开(公告)日：1992-08-11
申请号：US703310
申请日：1991-05-20
申请人： John L. Robbins , Elise Marucchi-Soos , Ming Chow , William E. Gates , Shun C. Fung , Joseph P. Boyle
发明人： John L. Robbins , Elise Marucchi-Soos , Ming Chow , William E. Gates , Shun C. Fung , Joseph P. Boyle
IPC分类号： B01J23/42 , B01J23/40 , B01J23/44 , B01J23/46 , B01J23/62 , B01J23/656 , B01J29/068 , C10G35/085 , C10G35/09 , C10G35/095
CPC分类号： C10G35/095 , B01J23/40 , B01J29/068 , C10G35/085
摘要： A reforming process using a Supported Group VIII noble metal reforming catalyst which has been pretreated with an unsaturated aliphatic hydrocarbon at elevated temperatures, thereby lowering activity during initial reforming operations and reducing gas production during the initial operation.
摘要翻译：使用在高温下用不饱和脂肪烃预处理的负载VIII族贵金属重整催化剂的重整方法，从而降低初始重整操作期间的活性并降低初始操作期间的气体产量。

5. 发明授权

US5051384A Method for pretreating a reforming catalyst 失效
标题翻译：改性催化剂的预处理方法
公开(公告)号：US5051384A
公开(公告)日：1991-09-24
申请号：US497170
申请日：1990-03-22
申请人： John L. Robbins , Elise Marucchi-Soos , Ming Chow , William E. Gates , Shun C. Fung
发明人： John L. Robbins , Elise Marucchi-Soos , Ming Chow , William E. Gates , Shun C. Fung
IPC分类号： B01J23/40 , B01J29/068 , B01J29/62 , B01J37/08 , B01J38/04 , B01J38/10 , C07B61/00 , C10G35/085 , C10G35/095
CPC分类号： C10G35/095 , B01J29/068 , C10G35/085 , Y10S502/521
摘要： Supported Group VIII noble metal reforming catalysts are pretreated with an unsaturated aliphatic hydrocarbon at elevated temperatures, thereby lower activity during initial reforming operation and reducing gas production during the initial operation.

6. 发明授权

US09057031B2 Co-gasification process for hydrocarbon solids and biomass 有权
标题翻译：烃固体和生物质的共同气化过程
公开(公告)号：US09057031B2
公开(公告)日：2015-06-16
申请号：US12586872
申请日：2009-09-29
申请人： Ramesh Varadaraj , John L. Robbins , Michael Siskin
发明人： Ramesh Varadaraj , John L. Robbins , Michael Siskin
IPC分类号： C01B3/36 , C10J3/72 , C10J3/46 , C10J3/54 , C10J3/66
CPC分类号： C10J3/72 , C10J3/466 , C10J3/54 , C10J3/66 , C10J2300/092 , C10J2300/0926 , C10J2300/093 , C10J2300/0943 , C10J2300/0993 , C10J2300/1884 , Y02E50/32 , Y02P20/145 , Y02T50/678
摘要： A process for the co-gasification of carbonaceous solids (coal, coke) and biomass in which the biomass material is pyrolyzed to provide a biomass pyrolysis oil and biomass char or coke which are then mixed with the carbonaceous solid to form a slurry. This slurry is then heated if necessary to achieve a viscosity which can be processed conveniently in the gasifier. The heat required for pyrolyzing the biomass can conveniently be obtained from the heat exchanger used to cool the hot synthesis gas product emerging from the gasifier.
摘要翻译：一种用于碳质固体（煤，焦炭）和生物质的共同气化的方法，其中生物质材料被热解以提供生物质热解油和生物质焦炭或焦炭，然后将其与碳质固体混合以形成浆料。如果需要，则将该浆料加热以达到可在气化器中方便地加工的粘度。热解生物质所需的热量可以方便地从用于冷却从气化器出来的热合成气产品的热交换器获得。

7. 发明授权

US5604047A Carbon monoxide removal method based on adsorption/steam desorption cycle 失效
标题翻译：基于吸附/蒸汽脱附循环的一氧化碳去除方法
公开(公告)号：US5604047A
公开(公告)日：1997-02-18
申请号：US494206
申请日：1995-06-23
申请人： Richard J. Bellows , John L. Robbins
发明人： Richard J. Bellows , John L. Robbins
IPC分类号： B01D53/02 , C01B3/56 , H01M8/06 , H01M8/18 , H01M8/04
CPC分类号： C01B3/56 , H01M8/0662 , C01B2203/043 , C01B2203/047
摘要： The present invention comprises a method for lowering the carbon monoxide content of a CO-containing hydrogen rich gas stream by contacting the gas stream with an adsorbent capable of preferentially adsorbing the carbon monoxide in the gas stream, the adsorbent being selected from the group consisting of platinum, palladium, ruthenium, rhenium, iridium, the carbides and nitrides of tungsten, molybdenum, vanadium, chromium, tantalum, and mixtures thereof whereby a substantially CO free, hydrogen rich gas stream is obtained. Preferably the absorbent will have a surface area from 0.5 to about 200 m.sup.2 /gm.
摘要翻译：本发明包括通过使气流与能够优先吸附气流中的一氧化碳的吸附剂接触来降低含CO的富氢气流的一氧化碳含量的方法，所述吸附剂选自铂，钯，钌，铼，铱，钨，钼，钒，铬，钽及其混合物的碳化物和氮化物，由此得到基本上不含CO的富氢气流。优选地，吸收剂的表面积为0.5至约200m 2 / gm。

8. 发明授权

US5476982A Catalyst for dehydrogenation of paraffins 失效
标题翻译：石蜡脱氢催化剂
公开(公告)号：US5476982A
公开(公告)日：1995-12-19
申请号：US259717
申请日：1994-06-14
申请人： John L. Robbins , Elise Marucchi-Soos , Jack W. Johnson , John F. Brody
发明人： John L. Robbins , Elise Marucchi-Soos , Jack W. Johnson , John F. Brody
IPC分类号： B01J23/60 , B01J23/62 , B01J29/04 , C07C5/32 , C07C5/333
CPC分类号： B01J29/049 , B01J23/60 , B01J23/62 , C07C5/325 , C07C5/3337
摘要： The present invention is directed to a novel catalyst composition and its use in the dehydrogenation of paraffins to olefins. The catalyst comprises an alloy of a Group VIII noble metal and a metal selected from the group consisting of zinc and gallium on a support selected from the group consisting of silica, zinc oxide modified silica and zinc oxide modified silica-pillared clays when said alloy is a zinc alloy, and silica, gallium oxide modified silica and gallium oxide modified silica-pillared clays when said alloy is a gallium alloy. The instant catalyst is an active and selective catalyst for the catalytic dehydrogenation of paraffins to olefins, especially gaseous paraffins, having the added benefit of retaining high activity and selectivity even following repeated regeneration by calcination in oxygen containing gas at temperatures of 450.degree. C. to 650.degree. C., preferably 450.degree. C. to 500.degree. C.
摘要翻译：本发明涉及新型催化剂组合物及其在链烷烃脱氢成烯烃中的应用。所述催化剂包含由选自二氧化硅，氧化锌改性二氧化硅和氧化锌改性二氧化硅 - 柱状粘土的载体上的第八族贵金属和选自锌和镓的金属的合金，当所述合金为锌合金，二氧化硅，氧化镓改性二氧化硅和氧化镓改性二氧化硅柱状粘土。本催化剂是用于将链烷烃催化脱氢成烯烃，特别是气态烷烃的活性和选择性催化剂，具有保持高活性和选择性的附加益处，即使在含氧气体中通过在450℃至450℃的温度下煅烧反复再生， 650℃，优选450℃至500℃

9. 发明授权

US5324363A Method for carbonaceous deposit removal and for reducing engine octane requirement using an aqueous base 失效
标题翻译：使用含水基质除去碳质沉积物并减少发动机辛烷值要求的方法
公开(公告)号：US5324363A
公开(公告)日：1994-06-28
申请号：US914730
申请日：1992-07-20
申请人： John L. Robbins , Robert S. Lunt
发明人： John L. Robbins , Robert S. Lunt
IPC分类号： C10L10/06 , F02B77/04 , F02M63/00 , B08B3/10
CPC分类号： F02B77/04 , C10L10/06
摘要： Accumulation of carbonaceous deposits on the combustion chamber surfaces of internal combustion engines is responsible for increased fuel octane requirement to prevent knock. Treatment of these carbonaceous deposits with weak bases, such as aqueous ethylenediamine, aids in their removal and thereby reduces the octane requirement of an internal combustion engine. The method is also applicable for removal of carbonaceous deposits from metal surfaces generally.
摘要翻译：内燃机燃烧室表面积碳沉积物负责增加燃料辛烷值以防止爆震。用弱碱（如乙二胺水溶液）处理这些碳质沉积物有助于其去除，从而降低内燃机的辛烷值。该方法也适用于通常从金属表面除去碳质沉积物。

10. 发明授权

US5070064A Catalyst pretreatment method 失效
标题翻译：催化预处理方法
公开(公告)号：US5070064A
公开(公告)日：1991-12-03
申请号：US389916
申请日：1989-08-07
申请人： Edward C. Hsu , John L. Robbins
发明人： Edward C. Hsu , John L. Robbins
IPC分类号： B01J21/06 , B01J23/889 , B01J35/02 , B01J37/00 , B01J37/06 , B03B5/00 , C07B61/00 , C07C1/06 , C10G2/00
CPC分类号： C10G2/332 , B01J23/8896 , B01J35/023 , B01J37/00 , B01J37/009 , B01J37/06 , B03B5/00 , C07C1/066 , B01J21/063 , C07C2523/75
摘要： An improved pretreatment method for preparing powdered catalysts with well controlled particle size distributions that are free of sub 1 micron particles comprising dispersion of the powdered catalyst in liquid comprised of either a) a hydrocarbon containing low levels of a surfactant or, b) a surfactant containing polar protic solvent, followed by decantation of the suspended finely divided sub 1 micron particles and repeating said sequence until essentially 90% of the sub 1 micron particles have been removed.

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