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1. 发明授权

US5137620A Reforming process using a pretreated catalyst 失效
标题翻译：使用预处理催化剂的重整工艺
公开(公告)号：US5137620A
公开(公告)日：1992-08-11
申请号：US703310
申请日：1991-05-20
申请人： John L. Robbins , Elise Marucchi-Soos , Ming Chow , William E. Gates , Shun C. Fung , Joseph P. Boyle
发明人： John L. Robbins , Elise Marucchi-Soos , Ming Chow , William E. Gates , Shun C. Fung , Joseph P. Boyle
IPC分类号： B01J23/42 , B01J23/40 , B01J23/44 , B01J23/46 , B01J23/62 , B01J23/656 , B01J29/068 , C10G35/085 , C10G35/09 , C10G35/095
CPC分类号： C10G35/095 , B01J23/40 , B01J29/068 , C10G35/085
摘要： A reforming process using a Supported Group VIII noble metal reforming catalyst which has been pretreated with an unsaturated aliphatic hydrocarbon at elevated temperatures, thereby lowering activity during initial reforming operations and reducing gas production during the initial operation.
摘要翻译：使用在高温下用不饱和脂肪烃预处理的负载VIII族贵金属重整催化剂的重整方法，从而降低初始重整操作期间的活性并降低初始操作期间的气体产量。

2. 发明授权

US5051384A Method for pretreating a reforming catalyst 失效
标题翻译：改性催化剂的预处理方法
公开(公告)号：US5051384A
公开(公告)日：1991-09-24
申请号：US497170
申请日：1990-03-22
申请人： John L. Robbins , Elise Marucchi-Soos , Ming Chow , William E. Gates , Shun C. Fung
发明人： John L. Robbins , Elise Marucchi-Soos , Ming Chow , William E. Gates , Shun C. Fung
IPC分类号： B01J23/40 , B01J29/068 , B01J29/62 , B01J37/08 , B01J38/04 , B01J38/10 , C07B61/00 , C10G35/085 , C10G35/095
CPC分类号： C10G35/095 , B01J29/068 , C10G35/085 , Y10S502/521
摘要： Supported Group VIII noble metal reforming catalysts are pretreated with an unsaturated aliphatic hydrocarbon at elevated temperatures, thereby lower activity during initial reforming operation and reducing gas production during the initial operation.

3. 发明授权

US07033971B2 Method for using stabilizing catalyst activity during MTO unit operation 有权
标题翻译：在MTO单元运行期间使用稳定催化剂活性的方法
公开(公告)号：US07033971B2
公开(公告)日：2006-04-25
申请号：US10774859
申请日：2004-02-09
申请人： Shun C. Fung , Richard B. Hall , Hafedh Kochkar , Karl G. Strohmaier , Nicolas P. Coute , Kenneth R. Clem
发明人： Shun C. Fung , Richard B. Hall , Hafedh Kochkar , Karl G. Strohmaier , Nicolas P. Coute , Kenneth R. Clem
IPC分类号： B01J27/182 , B01J21/20
CPC分类号： B01J29/90 , B01J38/12 , C10G3/48 , C10G3/49 , C10G3/62 , C10G2300/708 , C10G2300/802 , C10G2300/805 , C10G2400/20 , Y02P30/20
摘要： A method for maintaining the activity of silicoaluminophosphate (SAPO) molecular sieve catalyst particles during oxygenate to olefin conversion reactions. After regeneration of SAPO catalyst particles, the regenerated particles are mixed with particles having coke on their surface in a manner that maintains their catalytic activity at a predetermined level.
摘要翻译：一种在含氧化合物转化成烯烃转化反应期间维持硅铝磷酸盐（SAPO）分子筛催化剂颗粒的活性的方法。在SAPO催化剂颗粒再生后，将再生颗粒与其表面上具有焦炭的颗粒以保持其催化活性在预定水平的方式混合。

4. 发明授权

US06518475B2 Process for making ethylene and propylene 失效
标题翻译：制备乙烯和丙烯的方法
公开(公告)号：US06518475B2
公开(公告)日：2003-02-11
申请号：US09785409
申请日：2001-02-16
申请人： Shun C. Fung , Chunshe Cao , Teng Xu
发明人： Shun C. Fung , Chunshe Cao , Teng Xu
IPC分类号： C07C100
CPC分类号： C07C1/20 , C07C2529/85 , Y02P20/52 , Y02P20/584 , Y02P30/42 , Y10S585/904 , C07C11/04 , C07C11/06
摘要： A process for increasing the ethylene selectivity of a silicoaluminophosphate molecular sieve catalyst by using acetone in an oxygenate conversion process. Acetone can be added with the oxygenate feed at a concentration from about 1% to about 15% by weight, preferably about 1% to about 8% by weight, more preferably about 2% to about 5% by weight. Alternatively, acetone can be added as a pre-feed to the molecular sieve catalyst, particularly regenerated and fresh catalyst, in an contact zone. The pre-feed contacted catalyst is then directed to an oxygenate conversion zone. The acetone concentration in the pre-feed is from about 1% to about 99% by weight, preferably about 30% to about 70% by weight.
摘要翻译：一种通过在含氧化合物转化方法中使用丙酮来提高硅铝磷酸盐分子筛催化剂的乙烯选择性的方法。丙酮可以以约1％至约15％重量，优选约1％至约8％重量，更优选约2％至约5％重量的浓度加入含氧化合物进料。或者，可以在接触区中将丙酮作为预进料加入到分子筛催化剂，特别是再生和新鲜的催化剂中。然后将预进料接触的催化剂导入含氧化合物转化区。预进料中的丙酮浓度为约1重量％至约99重量％，优选约30重量％至约70重量％。

5. 发明授权

US06437208B1 Making an olefin product from an oxygenate 有权
标题翻译：从含氧化合物制备烯烃产物
公开(公告)号：US06437208B1
公开(公告)日：2002-08-20
申请号：US09481364
申请日：2000-01-11
申请人： Keith H. Kuechler , Marcel J. G. Janssen , Stephen N. Vaughn , Shun C. Fung , Nicolas P. Coute , Jeffrey Scott Smith , James R. Lattner , Jeffrey L. White , Teng Xu , William L. Kuechler, Sr. , Machteld M. Mertens , Cornelius W. M. Van Oorschot
发明人： Keith H. Kuechler , Marcel J. G. Janssen , Stephen N. Vaughn , Shun C. Fung , Nicolas P. Coute , Jeffrey Scott Smith , James R. Lattner , Jeffrey L. White , Teng Xu , William L. Kuechler, Sr. , Machteld M. Mertens , Cornelius W. M. Van Oorschot
IPC分类号： C07C120
CPC分类号： C10G50/00 , B01J29/85 , B01J29/90 , B01J35/0006 , B01J2229/123 , C10G3/49 , C10G3/57 , C10G3/62 , C10G2300/1022 , C10G2300/1029 , C10G2300/4018 , C10G2300/708 , C10G2400/02 , C10G2400/20 , C10G2400/22 , Y02P30/42
摘要： Disclosed is a method for making olefin product from an oxygenate-containing feedstock. In the method, a silicoaluminophosphate molecular sieve catalyst is contacted with the oxygenate-containing feedstock in a reactor at an average catalyst feedstock exposure index of at least 1.0. The method produces lower coke yield and provides an olefin product which is low in C1-C4 paraffin content. The invention is particularly effective in producing an olefin product having a very low propane content.
摘要翻译：公开了一种从含氧化合物的原料制备烯烃产物的方法。在该方法中，将硅铝磷酸盐分子筛催化剂在反应器中与含氧化合物的原料接触，平均催化剂原料暴露指数为至少1.0。该方法产生较低的焦炭产量，并提供C1-C4链烷烃含量低的烯烃产物。本发明在生产丙烷含量非常低的烯烃产物方面特别有效。

6. 发明授权

US5763348A Method of regenerating deactivated catalyst 失效
标题翻译：再生失活催化剂的方法
公开(公告)号：US5763348A
公开(公告)日：1998-06-09
申请号：US474922
申请日：1995-06-07
申请人： Shun C. Fung , Samuel J. Tauster , Jay Y. Koo
发明人： Shun C. Fung , Samuel J. Tauster , Jay Y. Koo
IPC分类号： B01J20/34 , B01J29/62 , B01J29/90 , B01J38/44 , C10G35/095 , B01J38/42
CPC分类号： C10G35/095 , B01J29/62 , B01J29/90 , B01J38/44 , B01J2229/26 , B01J2229/36 , B01J2229/40 , B01J2229/42
摘要： A deactivated reforming catalyst comprising a type L zeolite containing a Group VIII noble metal may be regenerated and have enhanced dispersion by a method involving contacting the catalyst with oxygen and water at elevated temperatures, contacting the catalyst at elevated temperatures with a source of chlorine such as HCl or Cl.sub.2, and preferably oxygen and water, contacting the catalyst at elevated temperatures with oxygen and optionally water, and contacting the catalyst at elevated temperatures with hydrogen and optionally water to reduce the catalyst. Preferably the noble metal is platinum.
摘要翻译：包含含有VIII族贵金属的L型沸石的失活重整催化剂可以再生，并且通过包括使催化剂在高温下与氧和水接触的方法得到增强的分散，使高温下的催化剂与氯源接触，例如 HCl或Cl 2，优选氧和水，使催化剂在升高的温度下与氧和任选的水接触，并将催化剂在升高的温度下与氢气和任选的水接触以还原催化剂。贵金属优选为铂。

7. 发明授权

US4648960A Bound zeolite catalyst and process for using said catalyst 失效
标题翻译：结合沸石催化剂和使用所述催化剂的方法
公开(公告)号：US4648960A
公开(公告)日：1987-03-10
申请号：US837780
申请日：1986-03-10
申请人： Kenneth R. Poeppelmeier , Walter G. Funk , John J. Steger , Shun C. Fung , Virginia R. Cross , Jar-Lin Kao
发明人： Kenneth R. Poeppelmeier , Walter G. Funk , John J. Steger , Shun C. Fung , Virginia R. Cross , Jar-Lin Kao
IPC分类号： B01J29/62 , C10G35/06 , C10G35/095
CPC分类号： C10G35/095 , B01J29/62 , B01J2229/26 , B01J2229/42
摘要： A class of bound catalysts which exhibit superior activity maintenance in dehydrocyclization reactions are defined as a type L zeolite having exchangeable cations of which at least 75% are selected from Group IA and calcium and barium cations and containing well dispersed particles of at least one Group VIII noble metal where at least 90% of the noble metal thereof is dispersed in the form of particles having a diameter less than 7 .ANG.. The catalysts may also be identified as type L zeolites loaded with at least one Group VIII noble metal which have a terminal cracking index (as a measure of production of pentanes versus butanes from hexane) of at least 1.5.
摘要翻译：在脱氢环化反应中表现出优异的活性维持性的一类结合的催化剂定义为具有可交换阳离子的L型沸石，其中至少75％选自IA族和钙和钡阳离子，并且含有至少一种VIII族的良好分散的颗粒贵金属，其中至少90％的贵金属以直径小于7安士的颗粒形式分散。催化剂也可以被鉴定为负载有至少一种VIII族贵金属的L型沸石，其具有至少1.5的末端裂解指数（作为戊烷与己烷的丁烷的生成量的量度）。

8. 发明授权

US4492767A Low temperature decoking process for reactivating iridium and selenium containing catalysts 失效
标题翻译：用于再生铱和含硒催化剂的低温脱焦工艺
公开(公告)号：US4492767A
公开(公告)日：1985-01-08
申请号：US548218
申请日：1983-11-02
申请人： Shun C. Fung
发明人： Shun C. Fung
IPC分类号： B01J23/96 , B01J27/30 , C10G35/09 , B01J27/02 , C10G35/085
CPC分类号： C10G35/09 , B01J23/96 , B01J27/30
摘要： A process is disclosed for reactivating a coked and agglomerated iridium and selenium containing catalyst and particularly platinum-iridium-selenium on alumina reforming catalysts. The process includes a low temperature decoking step to achieve partial decoking while minimizing agglomeration, a reducing step involving contacting the decoked agglomerated catalyst with a reducing gas such as hydrogen to reduce agglomerated iridium oxides to the free metal, a halide pretreatment step to increase the chloride level of the catalyst to about 1.3 weight percent and above, and a halogen redispersion step. The redispersion step is performed with a mixture of elemental halogen and water vapor.
摘要翻译：公开了一种用于在氧化铝重整催化剂上重新激活焦化和附聚的铱和含硒催化剂，特别是铂 - 铱 - 硒的方法。该方法包括低温脱焦步骤以实现部分除焦同时最小化聚集，还原步骤包括使经过去除的附聚催化剂与还原气体如氢接触以将附聚的氧化铱降低至游离金属，卤化物预处理步骤以增加氯化物催化剂的水平为约1.3重量％以上，以及卤素再分散步骤。再分散步骤用元素卤素和水蒸气的混合物进行。

9. 发明授权

US4467045A Redispersion of Ir catalysts by low temperature reduction step 失效
标题翻译：通过低温还原步骤对Ir催化剂进行再分散
公开(公告)号：US4467045A
公开(公告)日：1984-08-21
申请号：US428927
申请日：1982-09-30
申请人： Shun C. Fung
发明人： Shun C. Fung
IPC分类号： B01J23/96 , B01J23/46 , C10G35/085 , C10G35/09
CPC分类号： B01J23/96
摘要： A process is described for the redispersion of iridium-containing catalysts involving a low temperature hydrogen reduction step, i.e., from 190.degree. C. up to about 250.degree. C. after a coke burn-off. The low temperature reduction step allows milder conditions during subsequent halogen redispersion.
摘要翻译：描述了一种涉及低温氢还原步骤的含铱催化剂再分散的方法，即焦炭燃烧后的190℃至约250℃。低温降温步骤在随后的卤素再分散过程中允许更温和的条件。

10. 发明授权

US06110857A Method of minimizing iron contamination during catalyst regeneration processes 失效
公开(公告)号：US06110857A
公开(公告)日：2000-08-29
申请号：US925364
申请日：1997-09-08
申请人： Shun C. Fung , Walter S. Kmak
发明人： Shun C. Fung , Walter S. Kmak
IPC分类号： B01J23/46 , B01J23/656 , B01J23/96 , B01J38/10 , B01J38/12 , B01J38/42 , B01J38/44 , B01J20/34
CPC分类号： B01J38/44 , B01J23/96 , B01J23/468 , B01J23/6567 , B01J38/10 , B01J38/12 , B01J38/42
摘要： The present invention is directed toward improved processes for the regeneration of noble metal-containing catalysts wherein iron contamination of the catalyst during regeneration is significantly diminished. It has been found that maintenance of any iron present in contact with the catalyst in the oxidized state (e.g., as Fe.sub.2 O.sub.3 or Fe.sub.3 O.sub.4) during contact of the catalyst with a source of halogen in the regeneration haliding step results in a marked decrease in the degree of catalyst contamination by iron species.

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