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1. 发明授权

US08017693B2 Polyolefin functional at each end 有权
标题翻译：聚烯烃在每端有功能
公开(公告)号：US08017693B2
公开(公告)日：2011-09-13
申请号：US10569475
申请日：2004-08-27
申请人： Haruyuki Makio , Terunori Fujita
发明人： Haruyuki Makio , Terunori Fujita
IPC分类号： C08F10/00 , C08F4/44
CPC分类号： C08F10/00 , C08F8/00 , C08F8/20 , C08F110/02 , C08F110/06 , C08F4/64048
摘要： A telechelic polyolefin represented by the following general formula (I): X—P—Y (1) wherein X and Y are each a group containing at least one element selected from oxygen, sulfur, nitrogen, phosphorus and halogens, X and Y may be the same or different, P represents a chain made mainly of an olefin composed only of carbon and hydrogen atoms, and X and Y are bonded to both terminals of P, wherein the molecular weight distribution (Mw/Mn) obtained by gel permeation chromatography (GPC) is from 1.0 to 1.5, is useful for various purposes.
摘要翻译：由以下通式（I）表示的遥爪聚烯烃：X-P-Y（1）其中X和Y各自为含有选自氧，硫，氮，磷和卤素中的至少一种元素的基团，X和Y可以相同或不同，P表示主要由仅由碳和氢原子组成的烯烃，X和Y键合到P的两个末端的链，其中通过凝胶渗透色谱法获得的分子量分布（Mw / Mn）（GPC）为1.0〜1.5，适用于各种用途。

2. 发明授权

US08129475B2 Telechelic polyolefin 有权
标题翻译：远端聚烯烃
公开(公告)号：US08129475B2
公开(公告)日：2012-03-06
申请号：US13085816
申请日：2011-04-13
申请人： Haruyuki Makio , Terunori Fujita
发明人： Haruyuki Makio , Terunori Fujita
IPC分类号： C08F10/00 , C08F4/44
CPC分类号： C08F10/00 , C08F8/00 , C08F8/20 , C08F110/02 , C08F110/06 , C08F4/64048
摘要： A process of preparing a telechelic polyolefin is disclosed by performing steps 1a, 2, and 1b in this order in the presence of an olefin polymerizing catalyst and subsequently performing step 3 if necessary. Step 1a involves reacting the olefin polymerizing catalyst with a polar-group-containing olefin (C). Step 2 involves reacting the resultant compound of step 1a with at least one olefin (D) selected from ethylene and olefins having 3 to 20 carbon atoms n times wherein n is an integer of 1 or more, provided that when n is an integer of 2 or more, the olefins (D) used in the respective contact operations are different in kind or composition. Step 1b involves reacting the resultant compound of step 2 with the same or different polar-group-containing olefin (C). Step 3 involves chemically converting the Y′ group in the general formula (II) to a different group.
摘要翻译：通过在烯烃聚合催化剂的存在下依次进行步骤1a，2和1b来公开制备遥爪聚烯烃的方法，随后如果需要进行步骤3。步骤1a包括使烯烃聚合催化剂与含极性基团的烯烃（C）反应。步骤2包括使步骤1a的所得化合物与选自乙烯和碳原子数3〜20的烯烃的至少一种烯烃（D）反应n次，其中n为1以上的整数，条件是当n为2的整数时或更多，各接触操作中使用的烯烃（D）的种类或组成不同。步骤1b包括使所得到的步骤2的化合物与相同或不同的含极性基团的烯烃（C）反应。步骤3涉及将通式（II）中的Y'基团化学转化为不同的基团。

3. 发明申请

US20050124771A1 Olefin polymerization catalysts, transition metal compounds, processes for olefin polymerization, and alpha-olefin/conjugated diene copolymers 有权
标题翻译：烯烃聚合催化剂，过渡金属化合物，烯烃聚合方法和α-烯烃/共轭二烯共聚物
公开(公告)号：US20050124771A1
公开(公告)日：2005-06-09
申请号：US11028923
申请日：2005-01-05
申请人： Terunori Fujita , Yasushi Tohi , Makoto Mitani , Shigekazu Matsui , Junji Saito , Masatoshi Nitabaru , Kiyoaki Sugi , Haruyuki Makio , Toshiyuki Tsutsui
发明人： Terunori Fujita , Yasushi Tohi , Makoto Mitani , Shigekazu Matsui , Junji Saito , Masatoshi Nitabaru , Kiyoaki Sugi , Haruyuki Makio , Toshiyuki Tsutsui
IPC分类号： C08F210/04 , C07F7/00 , C07F7/08 , C07F9/00 , C08F4/602 , C08F110/02 , C08F110/06 , C08F210/02 , C08F210/12 , C08F210/16 , C08F4/44
CPC分类号： C08F210/02 , C07F7/003 , C07F7/0803 , C07F9/005 , C08F10/00 , C08F110/02 , C08F110/06 , C08F210/16 , C08F2500/17 , C08F2500/01 , C08F2500/03 , C08F236/06 , C08F210/06 , C08F4/64189 , C08F4/64048 , C08F4/7022 , C08F4/6812
摘要： The invention provides a process using olefin polymerization catalysts exhibiting excellent polymerization activities. The olefin polymerization catalysts of the invention contain a transition metal compound of and at least one of an organometallic compound, an organoaluminum oxy-compound or a compound which reacts with said transition metal compound to form an ion pair. The process using the inventive catalysts is useful in producing α-olefin/conjugated diene copolymers having specific properties.
摘要翻译：本发明提供一种使用显示优异聚合活性的烯烃聚合催化剂的方法。本发明的烯烃聚合催化剂含有有机金属化合物，有机铝氧化合物或与所述过渡金属化合物反应形成离子对的化合物中的至少一种的过渡金属化合物。使用本发明催化剂的方法可用于制备具有特定性质的α-烯烃/共轭二烯共聚物。

4. 发明授权

US06875718B2 Olefin polymerization catalysts, transition metal compounds, processes for olefin polymerization, and α-olefin/conjugated diene copolymers 有权
标题翻译：烯烃聚合催化剂，过渡金属化合物，烯烃聚合方法和α-烯烃/共轭二烯共聚物
公开(公告)号：US06875718B2
公开(公告)日：2005-04-05
申请号：US09942706
申请日：2001-08-31
申请人： Terunori Fujita , Yasushi Tohi , Makoto Mitani , Shigekazu Matsui , Junji Saito , Masatoshi Nitabaru , Kiyoaki Sugi , Haruyuki Makio , Toshiyuki Tsutsui
发明人： Terunori Fujita , Yasushi Tohi , Makoto Mitani , Shigekazu Matsui , Junji Saito , Masatoshi Nitabaru , Kiyoaki Sugi , Haruyuki Makio , Toshiyuki Tsutsui
IPC分类号： C08F210/04 , C07F7/00 , C07F7/08 , C07F9/00 , C08F4/602 , C08F110/02 , C08F110/06 , C08F210/02 , C08F210/12 , C08F210/16 , B01J31/00 , B01J37/00 , C08F4/02 , C08F4/60 , C08F4/44
CPC分类号： C08F210/02 , C07F7/003 , C07F7/0803 , C07F9/005 , C08F10/00 , C08F110/02 , C08F110/06 , C08F210/16 , C08F2500/17 , C08F2500/01 , C08F2500/03 , C08F236/06 , C08F210/06 , C08F4/64189 , C08F4/64048 , C08F4/7022 , C08F4/6812
摘要： The invention provides olefin polymerization catalysts exhibiting excellent polymerization activities, a process for olefin polymerization using the catalysts, a novel transition metal compound useful for the catalysts, and α-olefin/conjugated diene copolymers having specific properties. The olefin polymerization catalysts of the invention contain (A) a transition metal compound of formula (I), and (B) an organometallic compound, an organoaluminum oxy-compound or an ionizing ionic compound. The novel transition metal compounds of the invention are compounds of formula (I) wherein M is a transition metal atom of Group 3 or 4 of the periodic table; R1 is a hydrocarbon group, etc.; R2 to R5 are each H, a halogen, a hydrocarbon group, etc.; R6 is a halogen, a hydrocarbon group, etc.; n is a number satisfying a valence of M; and X is a halogen, a hydrocarbon group, etc
摘要翻译：本发明提供了表现出优异聚合活性的烯烃聚合催化剂，使用该催化剂的烯烃聚合方法，用于该催化剂的新型过渡金属化合物和具有特定性质的α-烯烃/共轭二烯共聚物。本发明的烯烃聚合催化剂含有（A）式（I）的过渡金属化合物和（B）有机金属化合物，有机铝氧化合物或离子化离子化合物。本发明的新型过渡金属化合物是式（I）的化合物，其中M是周期表第3或4族的过渡金属原子; R 1是烃基等; R 2〜R 5各自为H，卤素，烃基等; R 6是卤素，烃基等; n是满足M价的数; X为卤素，烃基等

5. 发明申请

US20070010639A1 Polyolefin functional at each end 有权
标题翻译：聚烯烃在每端有功能
公开(公告)号：US20070010639A1
公开(公告)日：2007-01-11
申请号：US10569475
申请日：2004-08-27
申请人： Haruyuki Makio , Terunori Fujita
发明人： Haruyuki Makio , Terunori Fujita
IPC分类号： C08F4/44
CPC分类号： C08F10/00 , C08F8/00 , C08F8/20 , C08F110/02 , C08F110/06 , C08F4/64048
摘要： A telechelic polyolefin represented by the following general formula (I): X—P—Y (1) wherein X and Y are each a group containing at least one element selected from oxygen, sulfur, nitrogen, phosphorus and halogens, X and Y may be the same or different, P represents a chain made mainly of an olefin composed only of carbon and hydrogen atoms, and X and Y are bonded to both terminals of P, wherein the molecular weight distribution (Mw/Mn) obtained by gel permeation chromatography (GPC) is from 1.0 to 1.5, is useful for various purposes.
摘要翻译：由以下通式（I）表示的遥爪聚烯烃：<？in-line-formula description =“In-line formula”end =“lead”？> XPY（1）<？in-line-formula description =“In 其中X和Y各自为含有选自氧，硫，氮，磷和卤素中的至少一种元素的基团，X和Y可以相同或不同，P代表链主要由仅由碳原子和氢原子组成的烯烃，X和Y键合到P的两个末端，其中通过凝胶渗透色谱法（GPC）获得的分子量分布（Mw / Mn）为1.0至1.5，为用于各种目的。

6. 发明授权

US06309997B1 Olefin polymerization catalysts, transition metal compounds, processes for olefin polymerization, and &agr;-olefin/conjugated diene copolymers 失效
标题翻译：烯烃聚合催化剂，过渡金属化合物，烯烃聚合方法和α-烯烃/共轭二烯共聚物
公开(公告)号：US06309997B1
公开(公告)日：2001-10-30
申请号：US09065593
申请日：1998-04-24
申请人： Terunori Fujita , Yasushi Tohi , Makoto Mitani , Shigekazu Matsui , Junji Saito , Masatoshi Nitabaru , Kiyoaki Sugi , Haruyuki Makio , Toshiyuki Tsutsui
发明人： Terunori Fujita , Yasushi Tohi , Makoto Mitani , Shigekazu Matsui , Junji Saito , Masatoshi Nitabaru , Kiyoaki Sugi , Haruyuki Makio , Toshiyuki Tsutsui
IPC分类号： B01J2106
CPC分类号： C08F210/02 , C07F7/003 , C07F7/0803 , C07F9/005 , C08F10/00 , C08F110/02 , C08F110/06 , C08F210/16 , C08F2500/17 , C08F2500/01 , C08F2500/03 , C08F236/06 , C08F210/06 , C08F4/64189 , C08F4/64048 , C08F4/7022 , C08F4/6812
摘要： The invention provides olefin polymerization catalyst exhibiting excellent polymerization activities, a process for olefin polymerization using the catalyst, a novel transition metal compound useful for the catalyst, and an &agr;-olefin/conjugated diene copolymer having specific properties. The olefin polymerization catalyst of the invention comprises (A) a transition metal compound of formula (I) or (II), and (B) an organometallic compound, an oranoaluminum oxy-compound or an ionizing ionic compound. The novel transition metal compound of the invention is a compound of formula (I) wherein M is a transition meal atom of Group 3 or 4 of the periodic table; m is an integer of 1 to 3; R1 is a hydrocarbon group, etc.; R2 to R5 are each H, a halogen, a hydrocarbon group, etc.; R6 is a halogen, a hydrocarbon group, etc.; n is a number satisfying a valence of M; and X is a halogen, a hydrocarbon group, etc.
摘要翻译：本发明提供了表现出优异聚合活性的烯烃聚合催化剂，使用该催化剂的烯烃聚合方法，用于催化剂的新型过渡金属化合物和具有特定性能的α-烯烃/共轭二烯共聚物。本发明的烯烃聚合催化剂包含（A）式（I）或（II）的过渡金属化合物和（B）有机金属化合物，或者是含有氧化铝的氧化合物或离子化离子化合物。本发明的新型过渡金属化合物是式（I）的化合物，其中M是周期表第3或4族的过渡膳食原子; m为1〜3的整数。 R1是烃基等; R2至R5各自为H，卤素，烃基等; R6是卤素，烃基等; n是满足M价的数; X为卤素，烃基等

7. 发明申请

US20110196118A1 TELECHELIC POLYOLEFIN 有权
公开(公告)号：US20110196118A1
公开(公告)日：2011-08-11
申请号：US13085816
申请日：2011-04-13
申请人： Haruyuki Makio , Terunori Fujita
发明人： Haruyuki Makio , Terunori Fujita
IPC分类号： C08F4/76
CPC分类号： C08F10/00 , C08F8/00 , C08F8/20 , C08F110/02 , C08F110/06 , C08F4/64048
摘要： A process of preparing a telechelic polyolefin is disclosed by performing steps 1a, 2, and 1b in this order in the presence of an olefin polymerizing catalyst and subsequently performing step 3 if necessary. Step 1a involves reacting the olefin polymerizing catalyst with a polar-group-containing olefin (C). Step 2 involves reacting the resultant compound of step 1a with at least one olefin (D) selected from ethylene and olefins having 3 to 20 carbon atoms n times wherein n is an integer of 1 or more, provided that when n is an integer of 2 or more, the olefins (D) used in the respective contact operations are different in kind or composition. Step 1b involves reacting the resultant compound of step 2 with the same or different polar-group-containing olefin (C). Step 3 involves chemically converting the Y′ group in the general formula (II) to a different group.
摘要翻译：通过在烯烃聚合催化剂的存在下依次进行步骤1a，2和1b来公开制备遥爪聚烯烃的方法，随后如果需要进行步骤3。步骤1a包括使烯烃聚合催化剂与含极性基团的烯烃（C）反应。步骤2包括使步骤1a的所得化合物与选自乙烯和碳原子数3〜20的烯烃的至少一种烯烃（D）反应n次，其中n为1以上的整数，条件是当n为2的整数时或更多，各接触操作中使用的烯烃（D）的种类或组成不同。步骤1b包括使所得到的步骤2的化合物与相同或不同的含极性基团的烯烃（C）反应。步骤3涉及将通式（II）中的Y'基团化学转化为不同的基团。

8. 发明授权

US07300903B2 Olefin polymerization catalysts, transition metal compounds, processes for olefin polymerization, and α-olefin/conjugated diene copolymers 有权
标题翻译：烯烃聚合催化剂，过渡金属化合物，烯烃聚合方法和α-烯烃/共轭二烯共聚物
公开(公告)号：US07300903B2
公开(公告)日：2007-11-27
申请号：US11028923
申请日：2005-01-05
申请人： Terunori Fujita , Yasushi Tohi , Makoto Mitani , Shigekazu Matsui , Junji Saito , Masatoshi Nitabaru , Kiyoaki Sugi , Haruyuki Makio , Toshiyuki Tsutsui
发明人： Terunori Fujita , Yasushi Tohi , Makoto Mitani , Shigekazu Matsui , Junji Saito , Masatoshi Nitabaru , Kiyoaki Sugi , Haruyuki Makio , Toshiyuki Tsutsui
IPC分类号： B01J31/00 , C08F4/06 , C08F4/44
CPC分类号： C08F210/02 , C07F7/003 , C07F7/0803 , C07F9/005 , C08F10/00 , C08F110/02 , C08F110/06 , C08F210/16 , C08F2500/17 , C08F2500/01 , C08F2500/03 , C08F236/06 , C08F210/06 , C08F4/64189 , C08F4/64048 , C08F4/7022 , C08F4/6812
摘要： The invention provides a process using olefin polymerization catalysts exhibiting excellent polymerization activities. The olefin polymerization catalysts of the invention contain a transition metal compound typified by formula (I) and at least one of an organometallic compound, an organoaluminum oxy-compound or a compound which reacts with said transition metal compound to form an ion pair. The process using the inventive catalysts is useful in producing α-olefin/conjugated diene copolymers having specific properties
摘要翻译：本发明提供一种使用显示优异聚合活性的烯烃聚合催化剂的方法。本发明的烯烃聚合催化剂含有式（I）代表的过渡金属化合物和有机金属化合物，有机铝氧化合物或与所述过渡金属化合物反应形成离子对的化合物中的至少一种。使用本发明催化剂的方法可用于制备具有特定性质的α-烯烃/共轭二烯共聚物

9. 发明申请

US20060270814A1 Polyolefin functional at one end 审中-公开
标题翻译：聚烯烃在一端有功能
公开(公告)号：US20060270814A1
公开(公告)日：2006-11-30
申请号：US10569604
申请日：2004-08-27
申请人： Haruyuki Makio , Terunori Fujita
发明人： Haruyuki Makio , Terunori Fujita
IPC分类号： C08F4/06
CPC分类号： C08F10/00 , C08F8/00 , C08F8/20 , C08F110/02 , C08F110/06 , C08F4/64048
摘要： A single-chain-end functionalized polyolefin, which is represented by the following general formula (I): P—X (I) wherein X is a group containing at least one element selected from oxygen, sulfur, nitrogen, phosphorus and halogens, P represents a polymer chain made mainly of an olefin composed only of carbon and hydrogen atoms, and X is bonded to a terminal of P, wherein the molecular weight distribution (Mw/Mn) obtained by gel permeation chromatography (GPC) is from 1.0 to 1.5.
摘要翻译：单链端官能化聚烯烃，其由以下通式（I）表示：<？in-line-formula description =“In-line Formulas”end =“lead”？> PX（I）<？in -line-formula description =“In-line Formulas”end =“tail”？>其中X是含有至少一个选自氧，硫，氮，磷和卤素的元素的基团，P代表主要由烯烃仅由碳和氢原子组成，X与P的末端键合，其中通过凝胶渗透色谱法（GPC）获得的分子量分布（Mw / Mn）为1.0至1.5。

10. 发明授权

US06770723B2 &agr;-olefin/conjugated diene copolymers 有权
标题翻译： α-烯烃/共轭二烯共聚物
公开(公告)号：US06770723B2
公开(公告)日：2004-08-03
申请号：US09942636
申请日：2001-08-31
申请人： Terunori Fujita , Yasushi Tohi , Makoto Mitani , Shigekazu Matsui , Junji Saito , Masatoshi Nitabaru , Kiyoaki Sugi , Haruyuki Makio , Toshiyuki Tsutsui
发明人： Terunori Fujita , Yasushi Tohi , Makoto Mitani , Shigekazu Matsui , Junji Saito , Masatoshi Nitabaru , Kiyoaki Sugi , Haruyuki Makio , Toshiyuki Tsutsui
IPC分类号： C08F23604
CPC分类号： C08F210/02 , C07F7/003 , C07F7/0803 , C07F9/005 , C08F10/00 , C08F110/02 , C08F110/06 , C08F210/16 , C08F2500/17 , C08F2500/01 , C08F2500/03 , C08F236/06 , C08F210/06 , C08F4/64189 , C08F4/64048 , C08F4/7022 , C08F4/6812
摘要： The invention provides olefin polymerization catalyst exhibiting excellent polymerization activities, a process for olefin polymerization using the catalyst, a novel transition metal compound useful for the catalyst, and an &agr;-olefin/conjugated diene copolymer having specific properties. The olefin polymerization catalyst of the invention comprises (A) a transition metal compound of formula (I) or (II), and (B) an organometallic compound, an oranoaluminum oxy-compound or an ionizing ionic compound. The novel transition metal compound of the invention is a compound of formula (I) wherein M is a transition meal atom of Group 3 or 4 of the periodic table; m is an integer of 1 to 3; R1 is a hydrocarbon group, etc.; R2 to R5 are each H, a halogen, a hydrocarbon group, etc.; R6 is a halogen, a hydrocarbon group, etc.; n is a number satisfying a valence of M; and X is a halogen, a hydrocarbon group, etc.
摘要翻译：本发明提供了表现出优异聚合活性的烯烃聚合催化剂，使用该催化剂的烯烃聚合方法，用于催化剂的新型过渡金属化合物和具有特定性能的α-烯烃/共轭二烯共聚物。本发明的烯烃聚合催化剂包含（A）式（I）或（II）的过渡金属化合物和（B）有机金属化合物，或者是含有氧化铝的氧化合物或离子化离子化合物。本发明的新型过渡金属化合物是式（I）的化合物，其中M是周期表第3或4族的过渡膳食原子; m为1〜3的整数。 R 1是烃基等; R 2〜R 5各自为H，卤素，烃基等; R 6是卤素，烃基等; n是满足M价的数; X为卤素，烃基等

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