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1. 发明授权

US08278256B2 Fluorinated lubricants 有权
标题翻译：氟化润滑剂
公开(公告)号：US08278256B2
公开(公告)日：2012-10-02
申请号：US12516158
申请日：2007-11-29
申请人： Giuseppe Marchionni , Pier Antonio Guarda , Marco Avataneo
发明人： Giuseppe Marchionni , Pier Antonio Guarda , Marco Avataneo
IPC分类号： C10M105/18
CPC分类号： C08G65/007 , C08L27/12 , C08L71/02 , C08L2205/05 , C10M107/38 , C10M2213/043 , C10M2213/0606 , C10N2230/06 , C10N2230/74 , C10N2250/10 , C08L2666/04
摘要： Polymers of formula Q-O-[A-B]z-[A-B′]z-A-Q′ (I) wherein: A=-(X)a—O-A′-(X′)b— with A′=perfluoropolyether chain and X, X′=—CF2—, —CF2CF2—; a, b=0.1 with the proviso that a=1 if A is linked to Q-O—; b=0 when A is linked to Q′; B derives from homopolymerizable olefins by radical route, of formula: —[(CR1R2—CR3R4)j(CR5R6—CR7R8)j′]— (Ia) wherein j is an integer from 1 to 30, j′ is an integer from 0 to 29 with the proviso that (j+j′) is higher than 2 and lower than 30; R1-R8 are halogen; H; C1-C6 (per)haloalkyl; C1-C6 alkyl; or C1-C6 oxy(per)fluoroalkyl; B′=B but at least one among R1-R8 has a meaning different from that in B; z, z′ are such that the number average molecular weight of the polymer of formula (I) is between 500 and 150,000; Q, Q′=C1-C3 (per)fluoroalkyl or functional end group —(CFW)-Dq-Tk; W=F, CF3; k and q are integers, k ranges from 1 to 4, q is an integer and is equal to 0 or 1; with the proviso that at least one of Q, Q′ is functional end group.
摘要翻译：具有式QO- [AB] z- [AB'] zAQ'（I）的聚合物其中：A = - （X）a-OA' - （X'）b-，其中A'=全氟聚醚链，X，X'= -CF 2 - ， - C 2 CF 2 - ; a，b = 0.1，条件是如果A连接到Q-O-，则a = 1; 当A连接到Q'时，b = 0; B通过自由基途径衍生自均聚烯烃，式为： - [（CR1R2-CR3R4）j（CR5R6-CR7R8）j'] - （Ia）其中j为1至30的整数，j'为0至 29，条件是（j + j'）高于2且低于30; R1-R8是卤素; H; C1-C6（全）卤代烷基; C1-C6烷基; 或C 1 -C 6氧基（全）氟代烷基; B'= B，但R1-R8中至少有一个与B不同; z，z'使得式（I）的聚合物的数均分子量在500和150,000之间; Q，Q'= C1-C3（全）氟烷基或官能端基 - （CFW）-Dq-Tk; W = F，CF3; k和q是整数，k的范围是1到4，q是整数，等于0或1; 条件是Q，Q'中的至少一个是官能端基。

2. 发明申请

US20100105584A1 Fluorinated Lubricants 有权
标题翻译：氟化润滑剂
公开(公告)号：US20100105584A1
公开(公告)日：2010-04-29
申请号：US12516048
申请日：2007-11-29
申请人： Marco Avataneo , Pier Antonio Guarda , Giuseppe Marchionni , Patrizia Maccone , Giovanni Boccaletti
发明人： Marco Avataneo , Pier Antonio Guarda , Giuseppe Marchionni , Patrizia Maccone , Giovanni Boccaletti
IPC分类号： C10M125/26 , C08F214/18 , C10M107/38 , C10M147/04 , C10M149/20
CPC分类号： C08F293/00 , C08F214/182 , C08F283/06 , C08F293/005 , C08L53/00 , C10M107/38 , C10M119/22 , C10M2201/0616 , C10M2201/1026 , C10M2201/1056 , C10M2203/045 , C10M2203/065 , C10M2203/1006 , C10M2203/1025 , C10M2203/1045 , C10M2205/0285 , C10M2207/1206 , C10M2207/2805 , C10M2209/1033 , C10M2213/043 , C10M2213/046 , C10M2213/0606 , C10M2213/0613 , C10M2213/0626 , C10M2215/121 , C10M2217/0456 , C10M2229/025 , C10N2210/01 , C10N2210/02 , C10N2220/021 , C10N2220/022 , C10N2230/06 , C10N2230/74 , C10N2240/06 , C10N2240/202 , C10N2250/10 , C10N2250/121 , C08L2666/02 , C08L2666/04
摘要： Fluorinated lubricants of formula: T-O[A-B]z-[A-B′]z′-A-T′ (I)wherein: A=—(X)a—O-A′-(X′)b wherein A′ is a perfluoropolyether chain comprising units (CF2O), (CF2CF2O), (CF2CF2CF2O), (CF2CF2CF2CF2O); X, X′═—CF2—, —CF2CF2—; a, b=0 or 1; B derives from olefins, of which at least one homopolymerizable by radical route, of formula: —[(CR1R2—CR3R4)j(CR5R6—CR7R8)j′]— (Ia) wherein j=1-5, j′=0-4 and 2
摘要翻译：氟化润滑剂，其结构式如下：TO [AB] z- [AB'] z'-AT'（I）其中：A = - （X）a-OA' - （X'）b其中A' （CF 2 CF 2 O），（CF 2 CF 2 CF 2 O），（CF 2 CF 2 CF 2 CF 2 O） X，X'= CF 2 - ， - CF 2 CF 2 - ; a，b = 0或1; B衍生自其中至少一种可通过自由基路线均聚的至少一种式： - [（CR1R2-CR3R4）j（CR5R6-CR7R8）j'] - （Ia）其中j = 1-5，j'= 0- 4和2 <（j + j'）<5; R1-R8 =卤素，H，C1-C6（全）卤代烷基，C1-C6烷基，C1-C6氧基（全） - 氟烷基; z≥2; z'为0或整数; z，z'使得式（I）的聚合物的数均分子量在500-500,000的范围内; B'=（Ia），但R 1 -R 8中的至少一个具有不同于B和2和nlE的含义;（j + j'）<5; T，T'= C 1 -C 3全氟烷基，C 1 -C 6烷基及其组合物。

3. 发明申请

US20100069275A1 Fluorinated lubricants 有权
标题翻译：氟化润滑剂
公开(公告)号：US20100069275A1
公开(公告)日：2010-03-18
申请号：US12516158
申请日：2007-11-29
申请人： Giuseppe Marchionni , Pier Antonio Guarda , Marco Avataneo
发明人： Giuseppe Marchionni , Pier Antonio Guarda , Marco Avataneo
IPC分类号： C10M147/04 , C08L27/12
CPC分类号： C08G65/007 , C08L27/12 , C08L71/02 , C08L2205/05 , C10M107/38 , C10M2213/043 , C10M2213/0606 , C10N2230/06 , C10N2230/74 , C10N2250/10 , C08L2666/04
摘要： Polymers of formula Q-O-[A-B]z-[A-B′]z-A-Q′ (I) wherein: A=-(X)a—O-A′-(X′)b— with A′=perfluoropolyether chain and X, X′=—CF2—, —CF2CF2—; a, b=0.1 with the proviso that a=1 if A is linked to Q-O—; b=0 when A is linked to Q′; B derives from homopolymerizable olefins by radical route, of formula: —[(CR1R2—CR3R4)j(CR5R6—CR7R8)j′]— (Ia) wherein j is an integer from 1 to 30, j′ is an integer from 0 to 29 with the proviso that (j+j′) is higher than 2 and lower than 30; R1-R8 are halogen; H; C1-C6 (per)haloalkyl; C1-C6 alkyl; or C1-C6 oxy(per)fluoroalkyl; B′=B but at least one among R1-R8 has a meaning different from that in B; z, z′ are such that the number average molecular weight of the polymer of formula (I) is between 500 and 150,000; Q, Q′=C1-C3 (per)fluoroalkyl or functional end group —(CFW)-Dq-Tk; W=F, CF3; k and q are integers, k ranges from 1 to 4, q is an integer and is equal to 0 or 1; with the proviso that at least one of Q, Q′ is functional end group.
摘要翻译：具有式QO- [AB] z- [AB'] zAQ'（I）的聚合物其中：A = - （X）a-OA' - （X'）b-，其中A'=全氟聚醚链，X，X'= -CF 2 - ， - C 2 CF 2 - ; a，b = 0.1，条件是如果A连接到Q-O-，则a = 1; 当A连接到Q'时，b = 0; B通过自由基途径衍生自均聚烯烃，式为： - [（CR1R2-CR3R4）j（CR5R6-CR7R8）j'] - （Ia）其中j为1至30的整数，j'为0至 29，条件是（j + j'）高于2且低于30; R1-R8是卤素; H; C1-C6（全）卤代烷基; C1-C6烷基; 或C 1 -C 6氧基（全）氟代烷基; B'= B，但R1-R8中至少有一个与B不同; z，z'使得式（I）的聚合物的数均分子量在500和150,000之间; Q，Q'= C1-C3（全）氟烷基或官能端基 - （CFW）-Dq-Tk; W = F，CF3; k和q是整数，k的范围是1到4，q是整数，等于0或1; 条件是Q，Q'中的至少一个是官能端基。

4. 发明授权

US08507642B2 (Per)fluorinated addition products 失效
标题翻译：（Per）氟化加成产物
公开(公告)号：US08507642B2
公开(公告)日：2013-08-13
申请号：US12921938
申请日：2009-03-13
申请人： Giuseppe Marchionni , Marco Avataneo , Pier Antonio Guarda
发明人： Giuseppe Marchionni , Marco Avataneo , Pier Antonio Guarda
IPC分类号： C08G65/22 , C08G73/24 , C08G65/00 , C08G73/00
CPC分类号： C08G65/007 , C08G65/3312 , C08G65/3331 , C08G65/337 , C08L2205/05
摘要： The invention pertains to a process for the addition of at least one (per)fluoropolyether peroxide comprising at least one peroxidic moiety and at least one fluoropolyoxyalkene chain (chain Rf) (i.e. a fluorocarbon segment comprising ether linkages in main chain) [peroxide (P)] onto a per(halo)fluorinated aromatic compound [compound (F)], so as to yield an addition compound of said compound (F), said addition compound [compound (A)] comprising at least one perfluorinated non-aromatic cyclic moiety having at least two substituents comprising a chain Rf and, optionally, conjugated or non conjugated double bond(s). Said addition compounds have been notably found useful as additives for (per)fluorinated fluids and lubricants or as base materials for the manufacture of gum and/or graft polymer compositions.
摘要翻译：本发明涉及添加至少一种（全）含氟聚醚过氧化物的方法，该过氧化物包含至少一个过氧化物部分和至少一个氟聚氧亚烷基链（链Rf）（即在主链中包含醚键的氟烃部分）[过氧化物（P ）]到全（卤）氟化芳族化合物[化合物（F）]]，得到所述化合物（F）的加成化合物，所述加成化合物[化合物（A）]包含至少一个全氟化非芳族环部分具有至少两个包含链R f的取代基和任选的共轭或非共轭双键。特别地，所述加成化合物可用作（全）氟化流体和润滑剂或用作制备胶和/或接枝聚合物组合物的基础材料的添加剂。

5. 发明授权

US08258090B2 Fluorinated lubricants 有权
标题翻译：氟化润滑剂
公开(公告)号：US08258090B2
公开(公告)日：2012-09-04
申请号：US12516048
申请日：2007-11-29
申请人： Marco Avataneo , Pier Antonio Guarda , Giuseppe Marchionni , Patrizia Maccone , Giovanni Boccaletti
发明人： Marco Avataneo , Pier Antonio Guarda , Giuseppe Marchionni , Patrizia Maccone , Giovanni Boccaletti
IPC分类号： C10M105/18
CPC分类号： C08F293/00 , C08F214/182 , C08F283/06 , C08F293/005 , C08L53/00 , C10M107/38 , C10M119/22 , C10M2201/0616 , C10M2201/1026 , C10M2201/1056 , C10M2203/045 , C10M2203/065 , C10M2203/1006 , C10M2203/1025 , C10M2203/1045 , C10M2205/0285 , C10M2207/1206 , C10M2207/2805 , C10M2209/1033 , C10M2213/043 , C10M2213/046 , C10M2213/0606 , C10M2213/0613 , C10M2213/0626 , C10M2215/121 , C10M2217/0456 , C10M2229/025 , C10N2210/01 , C10N2210/02 , C10N2220/021 , C10N2220/022 , C10N2230/06 , C10N2230/74 , C10N2240/06 , C10N2240/202 , C10N2250/10 , C10N2250/121 , C08L2666/02 , C08L2666/04
摘要： Fluorinated lubricants of formula: T-O-[A-B]z-[A-B′]z′-A-T′ (I) wherein: A=—(X)a—O-A′-(X′)b wherein A′ is a perfluoropolyether chain comprising units (CF2O), (CF2CF2O), (CF2CF2CF2O), (CF2CF2CF2CF2O); X, X′=—CF2—, —CF2CF2—; a, b=0 or 1; B derives from olefins, of which at least one homopolymerizable by radical route, of formula: —[(CR1R2—CR3R4)j(CR5R6—CR7R8)j′]— (Ia) wherein j=1-5, j′=0-4 and 2
摘要翻译：氟化润滑剂，其结构式为：TO- [AB] z- [AB'] z'-AT'（I）其中：A = - （X）a-OA' - （X'）b其中A'是全氟聚醚链，单元（CF 2 O），（CF 2 CF 2 O），（CF 2 CF 2 CF 2 O），（CF 2 CF 2 CF 2 CF 2 O） X，X'= -CF 2 - ， - CF 2 CF 2 - ; a，b = 0或1; B衍生自其中至少一种可通过自由基路线均聚的至少一种式： - [（CR1R2-CR3R4）j（CR5R6-CR7R8）j'] - （Ia）其中j = 1-5，j'= 0- 4和2 <（j + j'）<5; R1-R8 =卤素，H，C1-C6（全）卤代烷基，C1-C6烷基，C1-C6氧基（全） - 氟烷基; z≥2; z'为0或整数; z，z'使得式（I）的聚合物的数均分子量在500-500,000的范围内; B'=（Ia），但R 1 -R 8中的至少一个具有不同于B和2和nlE的含义;（j + j'）<5; T，T'= C 1 -C 3全氟烷基，C 1 -C 6烷基及其组合物。

6. 发明申请

US20110015107A1 (Per)Fluorinated addition products 失效
标题翻译：（Per）氟化加成产物
公开(公告)号：US20110015107A1
公开(公告)日：2011-01-20
申请号：US12921938
申请日：2009-03-13
申请人： Giuseppe Marchionni , Marco Avataneo , Pier Antonio Guarda
发明人： Giuseppe Marchionni , Marco Avataneo , Pier Antonio Guarda
IPC分类号： C10M145/22 , C08L71/00 , C08G65/00
CPC分类号： C08G65/007 , C08G65/3312 , C08G65/3331 , C08G65/337 , C08L2205/05
摘要： The invention pertains to a process for the addition of at least one (per)fluoropolyether peroxide comprising at least one peroxidic moiety and at least one fluoropolyoxyalkene chain (chain Rf) (i.e. a fluorocarbon segment comprising ether linkages in main chain) [peroxide (P)] onto a per(halo)fluorinated aromatic compound [compound (F)], so as to yield an addition compound of said compound (F), said addition compound [compound (A)] comprising at least one perfluorinated non-aromatic cyclic moiety having at least two substituents comprising a chain Rf and, optionally, conjugated or non conjugated double bond(s). Said addition compounds have been notably found useful as additives for (per)fluorinated fluids and lubricants or as base materials for the manufacture of gum and/or graft polymer compositions.
摘要翻译：本发明涉及添加至少一种（全）含氟聚醚过氧化物的方法，该过氧化物包含至少一个过氧化物部分和至少一个氟聚氧亚烷基链（链Rf）（即在主链中包含醚键的氟烃部分）[过氧化物（P ）]到全（卤）氟化芳族化合物[化合物（F）]]，得到所述化合物（F）的加成化合物，所述加成化合物[化合物（A）]包含至少一个全氟化非芳族环部分具有至少两个包含链R f的取代基和任选的共轭或非共轭双键。特别地，所述加成化合物可用作（全）氟化流体和润滑剂或用作制备胶和/或接枝聚合物组合物的基础材料的添加剂。

7. 发明授权

US08557952B2 Polyfunctional (per)fluoropolyethers 有权
标题翻译：多官能（全）氟聚醚
公开(公告)号：US08557952B2
公开(公告)日：2013-10-15
申请号：US13131240
申请日：2009-12-02
申请人： Giuseppe Marchionni , Silvia Petricci , Pier Antonio Guarda
发明人： Giuseppe Marchionni , Silvia Petricci , Pier Antonio Guarda
IPC分类号： C08G75/00 , C08G73/00
CPC分类号： C08G65/007
摘要： The invention pertains to novel (per)fluoropolyethers comprising at least one (per)fluoropolyoxyalkylene chain (chain Rf) comprising at least one recurring unit (R2) having formula: CF2—CF(CF2OSO2F)—O— (poly(fluorosulfate) PFPE) to a process for their manufacture, and to their use for providing functional (per)fluoropolyethers.
摘要翻译：本发明涉及包含至少一种（全）氟聚氧化烯链（链Rf）的新型（全）氟聚醚，其包含至少一个具有式CF 2 CF（CF 2 OSO 2 F）-O-（聚（氟硫酸酯）PFPE）的重复单元（R2）涉及其制造方法及其用于提供功能性（全）氟聚醚的用途。

8. 发明申请

US20130244131A1 Fuel cell modules 审中-公开
标题翻译：燃料电池模块
公开(公告)号：US20130244131A1
公开(公告)日：2013-09-19
申请号：US13989283
申请日：2011-11-28
申请人： Vincenzo Arcella , Giuseppe Marchionni , Ugo De Patto , Pier Antonio Guarda
发明人： Vincenzo Arcella , Giuseppe Marchionni , Ugo De Patto , Pier Antonio Guarda
IPC分类号： H01M8/10
CPC分类号： H01M8/1006 , H01M8/0232 , H01M8/0254 , H01M8/1004 , H01M2008/1095
摘要： A method for the preparation of corrugated fuel cell units from a composite laminate comprising an ion conductive membrane having first and second surface; a first electrocatalyst layer in contact with the first surface of the membrane; a second electrocatalyst layer in contact with the second surface of the membrane; a first metallic mesh in contact with said first electrocatalyst layer and a second metallic mesh in contact with said second electrocatalyst layer.
摘要翻译：一种由复合层压制备波纹燃料电池单元的方法，包括具有第一和第二表面的离子传导膜; 与膜的第一表面接触的第一电催化剂层; 与所述膜的第二表面接触的第二电催化剂层; 与所述第一电催化剂层接触的第一金属网和与所述第二电催化剂层接触的第二金属网。

9. 发明授权

US07629483B2 Peroxidic perfluoropolyethers 有权
标题翻译：过氧化全氟聚醚
公开(公告)号：US07629483B2
公开(公告)日：2009-12-08
申请号：US12099293
申请日：2008-04-08
申请人： Giuseppe Marchionni , Pier Antonio Guarda
发明人： Giuseppe Marchionni , Pier Antonio Guarda
IPC分类号： C07C309/06
CPC分类号： C08G65/32 , C08G65/007
摘要： Peroxidic perfluoropolyethers having formula: X1—O(CF2O)n1(CF2CF2O)m1(CF2(CF2)zCF2O)p1(O)h—X2 (I) wherein: X1 and X2, equal to or different from each other, are chain end groups selected among —CF2COF, —COF, —SO2F; n1, m1, p1 and h are integers such that the number average molecular weight is in the range 700-100,000; z=1 or 2; with the proviso that: the m1/n1 ratio is between 0.2 and 10; the p1/(n1+m1) ratio is lower than 0.05; the h/(n1+m1+p1) ratio is such that the PO content, defined as grams of active oxygen/100 g of compound, is in the range 0.8-4.5, preferably 1.4-3.8; the perfluorooxyalkylene units being statistically distributed along the polymeric chain.
摘要翻译：具有式：X1-O（CF2O）n1（CF2CF2O）m1（CF2（CF2）zCF2O）p1（O）h-X2（I）的过氧化全氟聚醚其中：X 1和X 2彼此相同或不同，为链末端 -CF 2 COF，-COF，-SO 2 F中选择的基团; n1，m1，p1和h是数均分子量在700-100,000范围内的整数; z = 1或2; 条件是：m1 / n1比在0.2和10之间; p1 /（n1 + m1）比低于0.05; h /（n1 + m1 + p1）的比例使得定义为活性氧克数/ 100g化合物的PO含量在0.8-4.5，优选1.4-3.8的范围内; 全氟氧化烯单元沿着聚合物链统计分布。

10. 发明申请

US20080194881A1 Peroxidic Perflouropolyethers 有权
标题翻译：过氧化物Perflouropolyethers
公开(公告)号：US20080194881A1
公开(公告)日：2008-08-14
申请号：US12099293
申请日：2008-04-08
申请人： Giuseppe MARCHIONNI , Pier Antonio Guarda
发明人： Giuseppe MARCHIONNI , Pier Antonio Guarda
IPC分类号： C07C43/17
CPC分类号： C08G65/32 , C08G65/007
摘要： Peroxidic perfluoropolyethers having formula: X1—O(CF2O)n1(CF2CF2O)m1(CF2(CF2)zCF2O)p1(O)h—X2 (I) wherein: X1 and X2, equal to or different from each other, are chain end groups selected among —CF2COF, —COF, —SO2F; n1, m1, p1 and h are integers such that the number average molecular weight is in the range 700-100,000; z=1 or 2; with the proviso that: the m1/n1 ratio is between 0.2 and 10; the p1/(n1+m1) ratio is lower than 0.05; the h/(n1+m1+p1) ratio is such that the PO content, defined as grams of active oxygen/100 g of compound, is in the range 0.8-4.5, preferably 1.4-3.8; the perfluorooxyalkylene units being statistically distributed along the polymeric chain.
摘要翻译：具有下式的过氧化全氟聚醚：<？in-line-formula description =“In-line Formulas”end =“lead”？> X 1 -O（CF 2 O）（CF 2）2（CF 2）2（CF 2）（CF 2）（CF 2）（O） > 2 <？in-line-formula description =“In-line Formulas”end =“tail”？>其中：X 1和X 2 < SUB>，彼此相同或不同，为选自-CF 2 COF，-COF，-SO 2 F的链端基; n1，m1，p1和h是数均分子量在700-100,000范围内的整数; z = 1或2; 条件是：m1 / n1比在0.2和10之间; p1 /（n1 + m1）比低于0.05; h /（n1 + m1 + p1）的比例使得定义为活性氧克数/ 100g化合物的PO含量在0.8-4.5，优选1.4-3.8的范围内; 全氟氧化烯单元沿着聚合物链统计分布。

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