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1. 发明授权

US08828734B2 Nitric oxide detection element and process for producing same 有权
标题翻译：一氧化氮检测元件及其制造方法
公开(公告)号：US08828734B2
公开(公告)日：2014-09-09
申请号：US13814155
申请日：2011-07-12
申请人： Kouichi Hiranaka , Toyofumi Nagamatsu , Yoshihiko Sadaoka , Yoshiteru Itagaki
发明人： Kouichi Hiranaka , Toyofumi Nagamatsu , Yoshihiko Sadaoka , Yoshiteru Itagaki
IPC分类号： G01N21/77 , G01N1/22 , G01N33/00 , G01N31/22 , G01N21/78
CPC分类号： G01N21/783 , G01N31/224 , G01N33/0037 , Y02A50/245 , Y10T436/177692 , Y10T436/25875
摘要： Provided are a nitric oxide detection element capable of detecting NO gas contained in a mixed gas at a high speed even when the amount thereof is a super trace amount of ten and several parts per billion; and a process for producing the element. In a nitric oxide detection element having a substrate 12 and a sensing film 11 formed on a surface of the substrate, the sensing film is composed of nitric oxide sensing particles and a polymer adhesive. The nitric oxide sensing particles are produced by adsorbing a dye having a porphyrin skeleton and having, as a central metal, divalent cobalt onto surfaces of inorganic particles.
摘要翻译：提供一种能够高速检测混合气体中所含的NO气体的一氧化氮检测元件，即使其量超过十倍和十亿分之一的超痕量，和该元件的制造方法。在具有形成在基板的表面上的基板12和感测膜11的一氧化氮检测元件中，感测膜由一氧化氮感测颗粒和聚合物粘合剂构成。一氧化氮感测颗粒是通过吸附具有卟啉骨架的染料和在无机颗粒的表面上具有二价钴作为中心金属来制备的。

2. 发明授权

US4985317A Lithium ion-conductive solid electrolyte containing lithium titanium phosphate 失效
标题翻译：含锂磷酸锂的锂离子导电固体电解质
公开(公告)号：US4985317A
公开(公告)日：1991-01-15
申请号：US372075
申请日：1989-06-28
申请人： Ginya Adachi , Nobuhito Imanaka , Hiromichi Aono , Eisuke Sugimoto , Yoshihiko Sadaoka , Naoshi Yasuda , Takeo Hara , Masaki Nagata
发明人： Ginya Adachi , Nobuhito Imanaka , Hiromichi Aono , Eisuke Sugimoto , Yoshihiko Sadaoka , Naoshi Yasuda , Takeo Hara , Masaki Nagata
IPC分类号： C01B25/45 , C01B33/20 , H01M6/18
CPC分类号： H01M6/185 , C01B25/45 , C01B33/20 , C04B35/16 , C04B35/447 , H01M6/18 , C04B2235/3203 , C04B2235/3217 , C04B2235/3224 , C04B2235/3225 , C04B2235/3227 , C04B2235/3232 , C04B2235/3272 , C04B2235/3418 , C04B2235/447 , C04B2235/77 , C04B2235/80
摘要： A lithium ion-conductive solid electrolyte consisting of a compound represented by the chemical formula, Li.sub.1+x M.sub.x Ti.sub.2-x (PO.sub.4).sub.3 (M is at least one element selected from the group consisting of Fe, Al and rare earth elements and x is a number of 0.1 to 1.9), a compound represented by the chemical formula, Li.sub.1+y Ti.sub.2 Si.sub.y P.sub.3-y O.sub.12 (Y is a number of 0.1 to 2.9), or a compound obtained by mixing a compound represented by the chemical formula, LiTi.sub.2 (PO.sub.4).sub.3 with a lithium compound other than LiTi.sub.2 (PO.sub.4).sub.3 and sintering the resulting mixture. Said lithium ion-conductive solid electrolyte can be produced by subjecting to solid phase reaction a mixture of a titanium oxide, a lithium salt, a phosphoric salt and M.sub.2 O.sub.3 (M is at least one element selected from the group consisting of Fe, Al and rare earth elements) or a silicon oxide or a mixture of LiTi.sub.2 (PO.sub.4).sub.3 and other lithium compound. Said lithium ion-conductive electrolyte can be used in the form of a lithium ion-conductive electrolyte sheet to prepare a structure suitable for solid electrochemical elements.
摘要翻译：由化学式Li1 + xMxTi2-x（PO4）3表示的化合物组成的锂离子传导性固体电解质（M为选自Fe，Al和稀土元素中的至少一种元素，x为数为0.1〜1.9），由化学式Li1 + yTi2SiyP3-yO12表示的化合物（Y为0.1〜2.9的数），或将化学式表示的化合物LiTi2（PO4）3 与LiTi 2（PO 4）3之外的锂化合物并烧结所得混合物。所述锂离子传导性固体电解质可以通过将氧化钛，锂盐，磷酸盐和M 2 O 3的混合物进行固相反应来制造（M为选自Fe，Al和稀土元素中的至少一种元素地球元素）或氧化硅或LiTi 2（PO 4）3与其它锂化合物的混合物。所述锂离子传导性电解质可以以锂离子传导电解质片的形式使用，以制备适用于固体电化学元件的结构。

3. 发明申请

US20110228276A1 NITROGEN OXIDE SENSING ELEMENT, NITROGEN OXIDE SENSOR, NITROGEN OXIDE CONCENTRATION DETERMINATION DEVICE USING SAME, AND METHOD FOR DETERMINING NITROGEN OXIDE CONCENTRATION 失效
标题翻译：氮氧化物传感元件，氮氧化物传感器，使用其的氮氧化物浓度测定装置以及用于测定氮氧化物浓度的方法
公开(公告)号：US20110228276A1
公开(公告)日：2011-09-22
申请号：US13131200
申请日：2009-11-06
申请人： Kouichi Hiranaka , Toyofumi Nagamatsu , Yoshihiko Sadaoka , Yoshiteru Itagaki
发明人： Kouichi Hiranaka , Toyofumi Nagamatsu , Yoshihiko Sadaoka , Yoshiteru Itagaki
IPC分类号： G01N21/00 , G01N7/00
CPC分类号： G01N21/77 , G01N21/7703 , G01N31/22 , G01N33/497 , G01N2021/7773 , G01N2021/7783
摘要： The nitrogen oxide sensing element of the present invention is such that a sensing film (11) is formed on the surface of a substrate (12a), the sensing film including a polymer containing as dispersed therein a porphyrin containing cobalt as a central metal, or a single derivative having a porphyrin skeleton containing cobalt as a central metal or a mixture of derivatives each having a porphyrin skeleton containing cobalt as a central metal; thus, this sensing element is capable of determining the concentration of NO with high sensitivity and satisfactory accuracy under the condition that the cobalt porphyrin is not affected by reaction inhibitors such as O2 and CO even in the atmosphere.
摘要翻译：本发明的氮氧化物感测元件使得在基板（12a）的表面上形成感测膜（11），该感测膜包括含有分散在其中的含有钴作为中心金属的卟啉的聚合物，或具有含有钴作为中心金属的卟啉骨架的单一衍生物或各自具有含有钴作为中心金属的卟啉骨架的衍生物的混合物; 因此，即使在大气中钴卟啉也不受反应抑制剂如O2和CO的影响，该感应元件能够以高灵敏度和令人满意的精度确定NO的浓度。

4. 发明授权

US5322612A Carbon dioxide gas detection element 失效
标题翻译：二氧化碳气体检测元件
公开(公告)号：US5322612A
公开(公告)日：1994-06-21
申请号：US930148
申请日：1992-08-13
申请人： Tooru Abe , Takaaki Kuroiwa , Yoshihiko Sadaoka
发明人： Tooru Abe , Takaaki Kuroiwa , Yoshihiko Sadaoka
IPC分类号： G01N27/406 , G01N27/407 , G01N27/416 , G01N33/00 , G01H27/26
CPC分类号： G01N27/4074 , G01N33/004
摘要： A carbon dioxide gas detection element includes a solid electrolyte of a sodium ion conductor made of a ceramic/glass composite material.
摘要翻译：一种二氧化碳气体检测元件包括由陶瓷/玻璃复合材料制成的钠离子导体的固体电解质。

5. 发明授权

US5952237A Method for detecting harmful gases which is applicable to broad gas concentration range 失效
公开(公告)号：US5952237A
公开(公告)日：1999-09-14
申请号：US728529
申请日：1996-10-09
申请人： Kazunari Tanaka , Chiaki Igarashi , Yoshihiko Sadaoka
发明人： Kazunari Tanaka , Chiaki Igarashi , Yoshihiko Sadaoka
IPC分类号： G01N31/00 , G01N21/31 , G01N21/77 , G01N21/78 , G01N31/22 , G01N31/16 , G01N21/79 , G01N21/80
CPC分类号： G01N21/3151 , G01N21/78 , G01N21/783 , Y10T436/15 , Y10T436/153333 , Y10T436/19 , Y10T436/20 , Y10T436/25875
摘要： The present invention provides a method by which harmful trace gases in a gaseous mixture containing as such harmful halogen gases, halogenated hydrogen gases, acid gases, oxidizing gases, basic gases, organic acid gases, especially halogen gases or halogenated hydrogen gases, are detected by using tetraphenylporphyrin (TPP) and quantitated from a calibration curve constructed therefrom, where the range of detectable concentration is made adjustable so that harmful gas can be detected and quantitated over a broad range of concentration. Furthermore, this invention also provides a method for extending the accessible range of gas concentration by adjusting the sensitivity of the detector material via control of tetraphenylporphyrin concentration in matrix polymer of the detector material, by controlling the gas concentration range via measurement at a specific wavelength(s), and by the use of a plurality of detector materials with pre-set assay sensitivity.

6. 发明授权

US4920451A Moisture-sensitive element 失效
标题翻译：水分敏感元素
公开(公告)号：US4920451A
公开(公告)日：1990-04-24
申请号：US353903
申请日：1989-05-18
申请人： Yoshiro Sakai , Yoshihiko Sadaoka , Takaai Kuroiwa , Tooru Abe , Tetsuya Miyagishi
发明人： Yoshiro Sakai , Yoshihiko Sadaoka , Takaai Kuroiwa , Tooru Abe , Tetsuya Miyagishi
IPC分类号： G01N27/22
CPC分类号： G01N27/225
摘要： A moisture-sensitive element includes a moisture-sensitive film consisting of a polymer prepared by polymerizing a methacrylate monomer not having a hydroxyl group. A humidity detector using the moisture-sensitive element is also disclosed.

7. 发明授权

US08508738B2 Nitrogen oxide sensing element, nitrogen oxide sensor, nitrogen oxide concentration determination device using same, and method for determining nitrogen oxide concentration 失效
标题翻译：氮氧化物感测元件，氮氧化物传感器，使用其的氮氧化物浓度测定装置以及氮氧化物浓度的测定方法
公开(公告)号：US08508738B2
公开(公告)日：2013-08-13
申请号：US13131200
申请日：2009-11-06
申请人： Kouichi Hiranaka , Toyofumi Nagamatsu , Yoshihiko Sadaoka , Yoshiteru Itagaki
发明人： Kouichi Hiranaka , Toyofumi Nagamatsu , Yoshihiko Sadaoka , Yoshiteru Itagaki
IPC分类号： G01N21/00
CPC分类号： G01N21/77 , G01N21/7703 , G01N31/22 , G01N33/497 , G01N2021/7773 , G01N2021/7783
摘要： The nitrogen oxide sensing element of the present invention is such that a sensing film (11) is formed on the surface of a substrate (12a), the sensing film including a polymer containing as dispersed therein a porphyrin containing cobalt as a central metal, or a single derivative having a porphyrin skeleton containing cobalt as a central metal or a mixture of derivatives each having a porphyrin skeleton containing cobalt as a central metal; thus, this sensing element is capable of determining the concentration of NO with high sensitivity and satisfactory accuracy under the condition that the cobalt porphyrin is not affected by reaction inhibitors such as O2 and CO even in the atmosphere.
摘要翻译：本发明的氮氧化物感测元件使得在基板（12a）的表面上形成感测膜（11），该感测膜包括含有分散在其中的含有钴作为中心金属的卟啉的聚合物，或具有含有钴作为中心金属的卟啉骨架的单一衍生物或各自具有含有钴作为中心金属的卟啉骨架的衍生物的混合物; 因此，即使在大气中钴卟啉也不受反应抑制剂如O2和CO的影响，该感应元件能够以高灵敏度和令人满意的精度确定NO的浓度。

8. 发明授权

US6096557A Gas detection method and apparatus using gas reactive pigment 失效
标题翻译：使用气体反应性颜料的气体检测方法和装置
公开(公告)号：US6096557A
公开(公告)日：2000-08-01
申请号：US910231
申请日：1997-08-13
申请人： Kazunari Tanaka , Chiaki Igarashi , Yoshihiko Sadaoka
发明人： Kazunari Tanaka , Chiaki Igarashi , Yoshihiko Sadaoka
IPC分类号： G01N21/25 , G01N21/77 , G01N21/78 , G01N31/22 , G01N33/00
CPC分类号： G01N31/223 , Y10T436/15 , Y10T436/153333 , Y10T436/177692 , Y10T436/19
摘要： This invention provides a method for determining the concentration of a gas to be detected by a gas detector using a gas reactive pigment, wherein the dynamic range of the detectable concentration can be controlled. The method comprising bringing a gas to be detected such as a halogen gas, a hydrogen halide gas or the like into contact with a gas detector placed in a detection area and comprising a gas reactive pigment tetraphenylporphyrin or a derivative thereof represented by the general formula (1) or a metal complex of tetraphenylporphyrin or a derivative thereof represented by the general formula (2); and irradiating said gas detector with a detection beam and measuring a color change in said gas detector to determine the concentration of said gas to be detected, wherein the measurement is carried out in the temperature range from 40 to 80.degree. C. of said detection area; and a detection apparatus for carrying out the said method are disclosed.
摘要翻译：本发明提供了一种用气体反应性颜料测定由气体检测器检测的气体的浓度的方法，其中可以控制可检测浓度的动态范围。所述方法包括使诸如卤素气体，卤化氢气体等的被检测气体与放置在检测区域中的气体检测器接触，并且包含由通式表示的气体反应性颜料四苯基卟啉或其衍生物（ 1）或由通式（2）表示的四苯基卟啉或其衍生物的金属络合物; 并用检测光束照射所述气体检测器，并测量所述气体检测器中的颜色变化，以确定所述待检测气体的浓度，其中所述测量在所述检测区域的40℃至80℃的温度范围内进行 ; 并且公开了一种用于执行所述方法的检测装置。

9. 发明授权

US5161085A Moisture sensitive element and method of manufacturing the same 失效
标题翻译：水分敏感元件及其制造方法
公开(公告)号：US5161085A
公开(公告)日：1992-11-03
申请号：US837059
申请日：1992-02-18
申请人： Yoshirou Sakai , Yoshihiko Sadaoka , Masanobu Matsuguchi , Takaaki Kuroiwa , Tooru Abe
发明人： Yoshirou Sakai , Yoshihiko Sadaoka , Masanobu Matsuguchi , Takaaki Kuroiwa , Tooru Abe
IPC分类号： G01N27/22
CPC分类号： G01N27/225
摘要： A moisture sensitive element includes a moisture sensitive film consisting of a polymer obtained by polymerizing and crosslinking a fluorine-containing polyimide oligomer or a polyisoimide oligomer having acetylene as a terminal group and its isomer. The moisture sensitive element also includes electrodes formed on upper and lower surfaces of the moisture sensitive film.
摘要翻译：湿敏元件包括由通过聚合和交联含氟聚酰亚胺低聚物或具有乙炔作为端基的聚异酰亚胺低聚物及其异构体获得的聚合物组成的湿敏膜。湿敏元件还包括形成在湿敏膜的上表面和下表面上的电极。

10. 发明申请

US20130137184A1 NITRIC OXIDE DETECTION ELEMENT AND PROCESS FOR PRODUCING SAME 有权
标题翻译：氮氧化物检测元件及其生产方法
公开(公告)号：US20130137184A1
公开(公告)日：2013-05-30
申请号：US13814155
申请日：2011-07-12
申请人： Kouichi Hiranaka , Toyofumi Nagamatsu , Yoshihiko Sadaoka , Yoshiteru Itagaki
发明人： Kouichi Hiranaka , Toyofumi Nagamatsu , Yoshihiko Sadaoka , Yoshiteru Itagaki
IPC分类号： G01N21/78
CPC分类号： G01N21/783 , G01N31/224 , G01N33/0037 , Y02A50/245 , Y10T436/177692 , Y10T436/25875
摘要： Provided are a nitric oxide detection element capable of detecting NO gas contained in a mixed gas at a high speed even when the amount thereof is a super trace amount of ten and several parts per billion; and a process for producing the element. In a nitric oxide detection element having a substrate 12 and a sensing film 11 formed on a surface of the substrate, the sensing film is composed of nitric oxide sensing particles and a polymer adhesive. The nitric oxide sensing particles are produced by adsorbing a dye having a porphyrin skeleton and having, as a central metal, divalent cobalt onto surfaces of inorganic particles.
摘要翻译：提供一种能够高速检测混合气体中所含的NO气体的一氧化氮检测元件，即使其量超过十倍和十亿分之一的超痕量，和该元件的制造方法。在具有形成在基板的表面上的基板12和感测膜11的一氧化氮检测元件中，感测膜由一氧化氮感测颗粒和聚合物粘合剂构成。一氧化氮感测颗粒是通过吸附具有卟啉骨架的染料和在无机颗粒的表面上具有二价钴作为中心金属来制备的。

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