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1. 发明授权

US5447702A Fluid bed desulfurization 失效
标题翻译：流化床脱硫
公开(公告)号：US5447702A
公开(公告)日：1995-09-05
申请号：US206569
申请日：1994-03-04
申请人： William M. Campbell , Gunnar B. Henningsen
发明人： William M. Campbell , Gunnar B. Henningsen
IPC分类号： B01D53/52 , B01D53/83 , C01B17/04 , C01B17/50 , C01B17/74 , C10J3/46 , C10J3/54 , C10J3/56 , C10J3/84 , C10K1/30 , C10K1/26
CPC分类号： B01D53/83 , B01D53/52 , C01B17/0408 , C01B17/508 , C01B17/74 , C10J3/00 , C10J3/54 , C10J3/56 , C10J3/84 , C10K1/004 , C10K1/026 , C10K1/30 , Y02E20/18
摘要： A method and apparatus for desulfurizing a gas and regenerating a sorbent is disclosed. The sulfur-containing feed gas which can be an effluent gas from a coal gasification reactor, for example, is desulfurized with a particulated metallic oxide sorbent in a transport riser. The sulfided sorbent is than separated from a desulfurized effluent gas and regenerated by contact with an oxygen-containing gas in a transport riser. The regenerated sorbent is separated from an SO.sub.2 containing offgas and recycled to the desulfurization step. The degree of sorbent conversion in the desulfurization step is held at a low level and the sorbent regeneration rate is increased to avoid excessive temperature rise in the regeneration step. In such manner, sorbent cooling can be substantially eliminated. The regeneration riser preferably comprises a once-through lift riser to minimize the riser transport gas requirements to just oxidant gas or oxidant gas mixed with a reduced amount of diluent gas. A reduction in use of diluent gas give a relatively high offgas SO.sub.2 concentration of as much as 15 mole percent, suitable for sulfuric acid manufacture and/or reduction to sulfur.
摘要翻译：公开了一种用于使气体脱硫和再生吸附剂的方法和装置。例如，可以将来自煤气化反应器的流出气体的含硫进料气体用运输提升管中的颗粒状金属氧化物吸附剂进行脱硫。硫化吸附剂不是从脱硫废气中分离出来的，而是通过与输送提升管中的含氧气体接触来再生。将再生的吸附剂与含SO 2的废气分离并再循环至脱硫步骤。脱硫步骤中的吸附剂转化度保持在低水平，并且增加吸附剂再生速率以避免再生步骤中过度的温度升高。以这种方式，可以基本上消除吸附剂冷却。再生提升管优选地包括一次通过的提升提升器，以使提升管输送气体的要求最小化为仅与减少量的稀释气体混合的氧化剂气体或氧化剂气体。稀释气体的使用的减少使得相对较高的废气SO 2浓度高达15摩尔％，适用于硫酸制造和/或还原为硫。

2. 发明授权

US5578093A Fluid bed desulfurization 失效
公开(公告)号：US5578093A
公开(公告)日：1996-11-26
申请号：US463442
申请日：1995-06-05
申请人： William M. Campbell , Gunnar B. Henningsen
发明人： William M. Campbell , Gunnar B. Henningsen
IPC分类号： B01D53/52 , B01D53/83 , C01B17/04 , C01B17/50 , C01B17/74 , C10J3/46 , C10J3/54 , C10J3/56 , C10J3/84 , C10K1/30 , C10K1/26
CPC分类号： B01D53/83 , B01D53/52 , C01B17/0408 , C01B17/508 , C01B17/74 , C10J3/00 , C10J3/54 , C10J3/56 , C10J3/84 , C10K1/004 , C10K1/026 , C10K1/30 , Y02E20/18
摘要： A method and apparatus for desulfurizing a gas and regenerating a sorbent is disclosed. The sulfur-containing feed gas which can be an effluent gas from a coal gasification reactor, for example, is desulfurized with a particulated metallic oxide sorbent in a transport riser. The sulfided sorbent is than separated from a desulfurized effluent gas and regenerated by contact with an oxygen-containing gas in a transport riser. The regenerated sorbent is separated from an SO.sub.2 containing offgas and recycled to the desulfurization step. The degree of sorbent conversion in the desulfurization step is held at a low level and the sorbent regeneration rate is increased to avoid excessive temperature rise in the regeneration step. In such manner, sorbent cooling can be substantially eliminated. The regeneration riser preferably comprises a once-through lift riser to minimize the riser transport gas requirements to just oxidant gas or oxidant gas mixed with a reduced amount of diluent gas. A reduction in use of diluent gas give a relatively high offgas SO.sub.2 concentration of as much as 15 mole percent, suitable for sulfuric acid manufacture and/or reduction to sulfur.

3. 发明授权

US5560900A Transport partial oxidation method 失效
标题翻译：运输部分氧化法
公开(公告)号：US5560900A
公开(公告)日：1996-10-01
申请号：US305241
申请日：1994-09-13
申请人： Eusebius A. Gbordzoe , Gunnar B. Henningsen , Darryl W. Hertz
发明人： Eusebius A. Gbordzoe , Gunnar B. Henningsen , Darryl W. Hertz
IPC分类号： C01B3/36 , B01J19/00 , C01B3/28 , C01B3/34 , C10G9/00 , C10L3/06 , C10L10/14 , C01B3/24 , C01B3/26
CPC分类号： C01B3/28 , C01B3/344 , Y02P20/124 , Y02P20/129
摘要： Disclosed are a process for converting low value hydrocarbon streams to hydrogen and/or synthesis gas products and a transport reactor useful in the conversion process. In the transport reactor, carbon produced is deposited on a circulating inert particulated carrier. The carbon deposited is partially oxidized to supply heat for the endothermic reactions. Reaction effluent gas leaving the transport reactor can be processed to remove particulate matter, sulfur compounds, and acid gases; condense the steam; and separate hydrogen from carbon monoxide to produce a purified hydrogen and/or syngas product. The present process has the flexibility to continuously handle all types of low value hydrocarbon feeds substantially without process disruption.
摘要翻译：公开了一种将低价值烃流转化为氢和/或合成气产物的方法以及在转化过程中有用的运输反应器。在运输反应器中，产生的碳沉积在循环惰性微粒载体上。沉积的碳被部分氧化以供给吸热反应的热量。可以处理离开运输反应器的反应废气以除去颗粒物，硫化合物和酸性气体; 冷凝蒸汽; 并从一氧化碳中分离出氢气以产生纯化的氢和/或合成气产物。本方法具有灵活性，可以连续处理所有类型的低价值烃进料，基本上没有过程中断。

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