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1. 发明申请

US20110160412A1 HYBRID ORGANIC-INORGANIC MATERIALS THAT CONTAIN STABILIZED CARBENE 有权
标题翻译：混合有机无机材料，含有稳定的碳
公开(公告)号：US20110160412A1
公开(公告)日：2011-06-30
申请号：US12812535
申请日：2009-01-23
申请人： Chloe Thieuleux , Christophe Coperet , Laurent Veyre , Robert Corriu , Catherine Reye , Ahmad Mehdi , Jean-Marie Basset , Tarun Maishal , Malika Boualleg , Lyad Karame , Jean-Michel Camus , Johan Alauzun
发明人： Chloe Thieuleux , Christophe Coperet , Laurent Veyre , Robert Corriu , Catherine Reye , Ahmad Mehdi , Jean-Marie Basset , Tarun Maishal , Malika Boualleg , Lyad Karame , Jean-Michel Camus , Johan Alauzun
IPC分类号： C07F1/10 , C07F15/00 , C07C45/68 , C08F4/58
CPC分类号： B01J31/2273 , B01J31/0295 , B01J31/181 , B01J2231/4211 , B01J2531/821 , B01J2531/827 , B01J2540/32
摘要： The present invention relates to materials and particularly “organometallic-organic-inorganic hybrid materials” that can be used as heterogeneous catalysts for selective catalytic reactions. More precisely this invention relates to organic-inorganic hybrid nanostructured materials comprising a regularly distributed stabilized carbene that binds strongly to a metal so as to form a stable organometallic-organic-inorganic hybrid material having high catalytic performances.
摘要翻译：本发明涉及可用作选择性催化反应的非均相催化剂的材料，特别是“有机金属 - 有机 - 无机杂化材料”。更确切地说，本发明涉及有机 - 无机混合纳米结构材料，其包含与金属强烈结合的规则分布稳定的卡宾，以形成具有高催化性能的稳定的有机金属 - 有机 - 无机杂化材料。

2. 发明授权

US06524372B1 Silica gel incorporating polyazacycloalkane structural units 有权
标题翻译：掺有多氮杂环烷结构单元的硅胶
公开(公告)号：US06524372B1
公开(公告)日：2003-02-25
申请号：US09600954
申请日：2000-07-25
申请人： Robert Corriu , Catherine Reye , Ahmad Mehdi , Gérard Dubois , Claude Chuit , Franck Denat , Bruno Roux-Fouillet , Roger Guilard , Gilles Lagrange , Stéphane Brandes
发明人： Robert Corriu , Catherine Reye , Ahmad Mehdi , Gérard Dubois , Claude Chuit , Franck Denat , Bruno Roux-Fouillet , Roger Guilard , Gilles Lagrange , Stéphane Brandes
IPC分类号： B01D5302
CPC分类号： C07F7/0896 , B01D53/02 , B01D2253/20 , B01D2253/202 , B01D2256/12 , B01D2257/104 , C01B13/0262 , C01B15/013 , C01B21/0455 , C01B2210/0045 , C01B2210/0046 , C07F7/1804
摘要： A novel compound which can be used in the field of separation and purification of gases is disclosed. The compound can be incorporated into a silica gel incorporating polyazacycloalkane structural units for separating a predetermined gas from a mixture of gases. The mixture of gases is brought into contact with a metallated hybrid gel under conditions which make possible the absorption of the gas to be separated, followed by a phase of desorption of the attached gas, and the recovery of the gas.
摘要翻译：公开了一种可用于气体分离和纯化领域的新型化合物。该化合物可以并入含有用于从气体混合物中分离预定气体的多氮杂环烷结构单元的硅胶中。使气体混合物与金属化混合凝胶接触，使得可能吸收待分离的气体，随后附着气体的解吸相和气体的回收。

3. 发明授权

US07452845B2 Mesoporous organic-inorganic hybrid materials for separating gases 有权
标题翻译：用于分离气体的介孔有机 - 无机杂化材料
公开(公告)号：US07452845B2
公开(公告)日：2008-11-18
申请号：US10472301
申请日：2002-03-21
申请人： Robert Corriu , Ahmad Mehdi , Catherine Reye , Henry Ledon , Roger Guilard , Stéphane Brandes , Chloé Thieuleux
发明人： Robert Corriu , Ahmad Mehdi , Catherine Reye , Henry Ledon , Roger Guilard , Stéphane Brandes , Chloé Thieuleux
IPC分类号： B01J20/00
CPC分类号： C07F1/005
摘要： The invention concerns a method for preparing organic-inorganic hybrid materials with controlled porosity and functionality comprising hydrolysis and condensation polymerization of a compound of formula (I): Z-R1—Si(OR)(OR′)(OR″), with an alkaline or alkaline-earth silicate in a mol ratio of (I)/(silicate)=1:9, in the presence of a non-ionic surfactant, to form a mesoporous silica represented by Z-R1—SiO1.5 9 SiO2, whereon is then anchored an organic compound, represented by (Δ)N—H, comprising a —NH— group capable of reacting with Z, to form a functionalized mesoporous silica represented by (Δ)N—R—SiO1.5 9 SiO2, which is optionally complexed with a metallic cation to form an organometallic complex. The invention also concerns the use of these materials to separate gases.
摘要翻译：本发明涉及一种制备具有受控孔隙率和功能性的有机 - 无机杂化材料的方法，包括式（I）化合物的水解和缩聚：ZR 1 -Si（OR）（OR'）（OR'） OR“），在非离子表面活性剂的存在下，以（I）/（硅酸盐）= 1:9的摩尔比的碱土金属或碱土金属硅酸盐形成由ZR

4. 发明授权

US4841084A New hexacoordinate silicon complexes, the process for their preparation and their application 失效
标题翻译：新的六配位硅复合物，其制备方法及其应用
公开(公告)号：US4841084A
公开(公告)日：1989-06-20
申请号：US813128
申请日：1985-12-24
申请人： Robert J. Corriu , Genevieve E. Cerveau , Claude G. Chuit , Catherine Reye
发明人： Robert J. Corriu , Genevieve E. Cerveau , Claude G. Chuit , Catherine Reye
IPC分类号： C07F7/02 , C07F7/04 , C07F7/08 , C07F7/12 , C07F7/18
CPC分类号： C07F7/0821 , C07F7/045 , C07F7/0807 , C07F7/0809 , C07F7/0896 , C07F7/123 , C07F7/1852
摘要： The present invention relates to new hexacoordinate silicon complexes, the process for their preparation and their application.These new complexes correspond to the general formula I: ##STR1## in which: A represents an alkali metal or alkaline earth metal except for magnesium, andn=0 or 1.
摘要翻译：本发明涉及新的六配位硅复合物，其制备方法及其应用。这些新配合物对应于通式I：其中：A代表除镁以外的碱金属或碱土金属，n = 0或1。

5. 发明授权

US07517512B2 Mesoporous organic-inorganic hybrid materials for separating gases 有权
标题翻译：用于分离气体的介孔有机 - 无机杂化材料
公开(公告)号：US07517512B2
公开(公告)日：2009-04-14
申请号：US12043486
申请日：2008-03-06
申请人： Robert Corriu , Ahmad Mehdi , Catherine Reye , Henry Ledon , Roger Guilard , Stéphane Brandes , Chloé Thieuleux
发明人： Robert Corriu , Ahmad Mehdi , Catherine Reye , Henry Ledon , Roger Guilard , Stéphane Brandes , Chloé Thieuleux
IPC分类号： B01D53/86
CPC分类号： C07F1/005
摘要： The invention concerns a method for preparing organic-inorganic hybrid materials with controlled porosity and functionality comprising hydrolysis and condensation polymerization of a compound of formula (I): Z-R1—Si(OR)(OR′)(OR″), with an alkaline or alkaline-earth silicate in a mol ratio of (I)/(silicate)=1:9, in the presence of a non-ionic surfactant, to form a mesoporous silica represented by Z-R1—SiO1.5 9 SiO2, whereon is then anchored an organic compound, represented by (Δ)N—H, comprising a —NH— group capable of reacting with Z, to form a functionalized mesoporous silica represented by (Δ)N—R—SiO1.5 9 SiO2, which is optionally complexed with a metallic cation to form an organometallic complex. The invention also concerns the use of these materials to separate gases.
摘要翻译：本发明涉及一种制备具有受控孔隙率和功能性的有机 - 无机杂化材料的方法，包括式（I）化合物：Z-R1-Si（OR）（OR'）（OR“）与水解和缩聚在非离子表面活性剂存在下，以（I）/（硅酸盐）= 1:9的摩尔比计的碱土金属或碱土金属硅酸盐，形成由Z-R1-SiO1.59SiO 2表示的介孔二氧化硅然后将其固定在由（Δ）NH表示的有机化合物中，该化合物包含能与Z反应的-NH-基团，形成由（Delta）NR-SiO 1.59SiO 2表示的官能化介孔二氧化硅，与金属阳离子络合形成有机金属络合物。本发明还涉及使用这些材料来分离气体。

6. 发明申请

US20080152561A1 MESOPOROUS ORGANIC-INORGANIC HYBRID MATERIALS FOR SEPARATING GASES 有权
标题翻译：用于分离气体的多孔有机无机混合材料
公开(公告)号：US20080152561A1
公开(公告)日：2008-06-26
申请号：US12043486
申请日：2008-03-06
申请人： Robert Corriu , Ahmad Mehdi , Catherine Reye , Henry Ledon , Roger Guilard , Stephane Brandes , Chloe Thieuleux
发明人： Robert Corriu , Ahmad Mehdi , Catherine Reye , Henry Ledon , Roger Guilard , Stephane Brandes , Chloe Thieuleux
IPC分类号： B01D53/46 , B01D53/38 , C01B13/02 , C07F7/02
CPC分类号： C07F1/005
摘要： The invention concerns a method for preparing organic-inorganic hybrid materials with controlled porosity and functionality comprising hydrolysis and condensation polymerization of a compound of formula (I): Z-R1—Si(OR)(OR′)(OR″), with an alkaline or alkaline-earth silicate in a mol ratio of (I)/(silicate)=1:9, in the presence of a non-ionic surfactant, to form a mesoporous silica represented by Z-R1—SiO1.5 9 SiO2, whereon is then anchored an organic compound, represented by (Δ)N—H, comprising a —NH— group capable of reacting with Z, to form a functionalized mesoporous silica represented by (Δ)N—R—SiO1.5 9 SiO2, which is optionally complexed with a metallic cation to form an organometallic complex. The invention also concerns the use of these materials to separate gases.
摘要翻译：本发明涉及一种制备具有受控孔隙率和功能性的有机 - 无机杂化材料的方法，包括式（I）化合物的水解和缩聚：ZR 1 -Si（OR）（OR'）（OR'） OR“），在非离子表面活性剂的存在下，以（I）/（硅酸盐）= 1:9的摩尔比的碱土金属或碱土金属硅酸盐形成由ZR

7. 发明授权

US4617413A Pentacoordinate silicon complexes, the process for their preparation and their application to the preparation of organosilanes 失效
标题翻译：五配位硅复合物，其制备方法及其在制备有机硅烷中的应用
公开(公告)号：US4617413A
公开(公告)日：1986-10-14
申请号：US813740
申请日：1985-12-24
申请人： Robert J. Corriu , Genevieve E. Cerveau , Claude G. Chuit , Catherine Reye
发明人： Robert J. Corriu , Genevieve E. Cerveau , Claude G. Chuit , Catherine Reye
IPC分类号： C07F7/08 , C07F7/18
CPC分类号： C07F7/1868 , C07F7/0809 , C07F7/0827 , C07F7/0836 , C07F7/0896
摘要： The present invention relates to new pentacoordinate silicon complexes, the process for their preparation and their application to the preparation of organosilanes.The pentacoordinate silicon complexes according to the invention correspond to the general formula I: ##STR1## in which: R denotes an alkyl, alkenyl, alkynyl, aryl, aralkyl, aralkenyl, aralkynyl or alkylaryl radical in which the aliphatic fragments are linear, branched or cyclic and contain from 1 to 20 carbon atoms,A represents an alkali metal or alkaline earth metal, with the proviso however that A represents neither sodium nor potassium when R is a phenyl radical, andn=1 or 2.
摘要翻译：本发明涉及新的五配位硅配合物，其制备方法及其在制备有机硅烷中的应用。根据本发明的五配位硅配合物对应于通式I：其中：R表示烷基，烯基，炔基，芳基，芳烷基，芳烯基，芳炔基或烷基芳基，其中脂族片段是线性的支链或环状且含有1至20个碳原子，A表示碱金属或碱土金属，但条件是当R为苯基时，A不表示钠或钾，n = 1或2。

8. 发明授权

US08871877B2 Hybrid organic-inorganic materials that contain stabilized carbene 有权
标题翻译：混合有机 - 无机材料，含有稳定的卡宾
公开(公告)号：US08871877B2
公开(公告)日：2014-10-28
申请号：US12812535
申请日：2009-01-23
申请人： Chloe Thieuleux , Christophe Coperet , Laurent Veyre , Robert Corriu , Catherine Reye , Ahmad Mehdi , Jean-Marie Basset , Tarun Maishal , Malika Boualleg , Iyad Karame , Jean-Michel Camus , Johan Alauzun
发明人： Chloe Thieuleux , Christophe Coperet , Laurent Veyre , Robert Corriu , Catherine Reye , Ahmad Mehdi , Jean-Marie Basset , Tarun Maishal , Malika Boualleg , Iyad Karame , Jean-Michel Camus , Johan Alauzun
IPC分类号： C07F1/10 , C07F15/00 , C07C45/68 , C08F4/58
CPC分类号： B01J31/2273 , B01J31/0295 , B01J31/181 , B01J2231/4211 , B01J2531/821 , B01J2531/827 , B01J2540/32
摘要： The present invention relates to materials and particularly “organometallic-organic-inorganic hybrid materials” that can be used as heterogeneous catalysts for selective catalytic reactions. More precisely this invention relates to organic-inorganic hybrid nanostructured materials comprising a regularly distributed stabilized carbene that binds strongly to a metal so as to form a stable organometallic-organic-inorganic hybrid material having high catalytic performances.
摘要翻译：本发明涉及可用作选择性催化反应的非均相催化剂的材料，特别是“有机金属 - 有机 - 无机杂化材料”。更确切地说，本发明涉及有机 - 无机混合纳米结构材料，其包含与金属强烈结合的规则分布稳定的卡宾，以形成具有高催化性能的稳定的有机金属 - 有机 - 无机杂化材料。

9. 发明授权

US4835316A New organomagnesium complexes in solid form, process for their preparation, and their use 失效
标题翻译：固体形式的新的有机镁络合物，其制备方法及其用途
公开(公告)号：US4835316A
公开(公告)日：1989-05-30
申请号：US103642
申请日：1987-10-02
申请人： Robert Corriu , Genevieve Cerveau , Claude Chuit , Catherine Reye , Alain Boudin
发明人： Robert Corriu , Genevieve Cerveau , Claude Chuit , Catherine Reye , Alain Boudin
IPC分类号： C07C45/00 , C07F3/02
CPC分类号： C07C45/004 , C07F3/02
摘要： Organgomagnesium complexes which correspond to the formula (I): ps(RMgX).sub.m /N[--CHR.sub.1 --CHR.sub.2 --O--(CHR.sub.3 --CHR.sub.4 --O).sub.n --R.sub.5 ].sub.3 (I)wherein:m is 1, 2, or 3;R denotes a substituted or unsubstituted group which is:linear or branched alkyl containing from 1 to 18 carbon atoms,alkenyl or alkynyl containing from 2 to 18 carbon atoms,cycloalkyl or cycloalkenyl containing from 3 to 12 carbon atoms,alkoxyalkyl, dialkoxyalkyl or alkylthiocarbonyl, aryl (which aryl may particularly be position-substituted by at least a halogen or an alkoxy, trifluoroemethyl, trifluoromethoxy or trifluromethoylthio group), oralkoxyaryl or alkylthioaryl;X denotes a chlorine, iodine or bromine atom;n is an integer ranging from 0 to about 10;R.sub.1, R.sub.2, R.sub.3 and R.sub.4, which are identical or di fferent, denote a hydrogen atom or an alkyl or cycloalkyl radical containing from 1 to 4 carbon atoms; andR.sub.5, which is identical or different in each of the three [--CHR.sub.1 --CHR.sub.2 --O--(CHR.sub.3 --CHR.sub.4 --O) hd n--R.sub.5 ] chains, denotes an alkyl or cycloalkyl radical containing 1 to 12 carbon atoms, a phenyl radical or a radical of formula --C.sub.p H.sub.2p --.phi. or C.sub.p H.sub.(2p+1) --.phi.--, wherein p ranges from 1 to about 12.
摘要翻译：对应于式（I）的络联络合物：ps（RMgX）m / N [-CHR1-CHR2-O-（CHR3-CHR4-O）n-R5] 3（I）其中：m为1,2或 3; R表示取代或未取代的基团，其为：含有1至18个碳原子的直链或支链烷基，含有2至18个碳原子的烯基或炔基，含有3至12个碳原子的环烷基或环烯基，烷氧基烷基，二烷氧基烷基或烷硫基羰基，芳基（该芳基可以特别被至少一个卤素或烷氧基，三氟甲基，三氟甲氧基或三氟甲硫基）位置取代）或烷氧基芳基或烷硫基芳基; X表示氯，碘或溴原子; n为0〜10的整数; 相同或不同的R 1，R 2，R 3和R 4表示氢原子或含有1至4个碳原子的烷基或环烷基; 和每个三个[-CHR1-CHR2-O-（CHR3-CHR4-O）hd n-R5]链相同或不同的R5表示含有1至12个碳原子的烷基或环烷基，苯基基团或式-CpH2p-phi或CpH（2p + 1） - phi - 的基团，其中p为1至约12。

10. 发明授权

US4665209A Process for the preparation of hydrogenosilanes or halogenosilanes 失效
标题翻译：制备氢硅烷或卤代硅烷的方法
公开(公告)号：US4665209A
公开(公告)日：1987-05-12
申请号：US813739
申请日：1985-12-24
申请人： Robert J. Corriu , Genevieve E. Cerveau , Claude G. Chuit , Catherine Reye
发明人： Robert J. Corriu , Genevieve E. Cerveau , Claude G. Chuit , Catherine Reye
IPC分类号： C07F7/18 , C07F7/08 , C07F7/12
CPC分类号： C07F7/123 , C07F7/0896
摘要： A process for the preparation of hydrogenosilanes or halogenosilanes corresponding to the general formula I:R--SiR'.sub.3
摘要翻译：对应于通式I的制备氢硅烷或卤代硅烷的方法：R-SiR'

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