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21. 发明申请

US20090208391A1 PROCESSES FOR THE RECOVERY OF CATALYTIC METAL AND CARBON NANOTUBES 有权
标题翻译：催化金属和碳纳米管的回收方法
公开(公告)号：US20090208391A1
公开(公告)日：2009-08-20
申请号：US12358772
申请日：2009-01-23
申请人： Jun Ma , Robert Hoch
发明人： Jun Ma , Robert Hoch
IPC分类号： C01G55/00 , D01F9/12 , B01J38/68
CPC分类号： B01J38/48 , B01J21/185 , B01J21/20 , B01J23/44 , B01J23/96 , B01J38/60 , B82Y30/00 , B82Y40/00 , C01B32/17 , Y02P20/584
摘要： A new method for recovering a catalytic metal and carbon nanotubes from a supported catalyst is provided. The carbon nanotube, including carbon nanotube structures, may serve as the support for the catalytic metal. The valence state of the catalytic metal, if not already in the positive state, is raised to a positive state by contacting the supported catalyst with a mild oxidizing agent under conditions which does not destroy the carbon nanotube. The supported catalyst is simultaneously or subsequently contacted with an acid solution to dissolve the catalytic metal without dissolving the carbon nanotube.
摘要翻译：提供了一种从负载催化剂中回收催化金属和碳纳米管的新方法。包括碳纳米管结构在内的碳纳米管可以用作催化金属的载体。在不破坏碳纳米管的条件下，通过使负载型催化剂与温和氧化剂接触，将催化金属的价态（如果尚未处于正态）升高至正态。负载的催化剂同时或随后与酸溶液接触以溶解催化金属而不溶解碳纳米管。

22. 发明申请

US20100086472A1 Single-walled carbon nanotube catalysts and method for preparing same 有权
标题翻译：单壁碳纳米管催化剂及其制备方法
公开(公告)号：US20100086472A1
公开(公告)日：2010-04-08
申请号：US11602136
申请日：2006-11-20
申请人： Jun Ma , David Moy
发明人： Jun Ma , David Moy
IPC分类号： D01F9/12
CPC分类号： D01F9/127 , B01J21/005 , B01J23/002 , B01J23/005 , B01J23/78 , B01J37/0236 , B01J37/031 , B01J37/08 , B01J37/18 , B01J2523/00 , B82Y30/00 , B82Y40/00 , C01B32/162 , C01B2202/02 , B01J2523/22 , B01J2523/842 , B01J2523/845 , B01J2523/41 , B01J2523/31
摘要： An activated catalyst capable of selectively growing single-walled carbon nanotubes when reacted with carbonaceous gas is provided. The activated catalyst is formed by reducing a catalyst that comprises a complex oxide. The complex oxide may be of formula Ax-wFwBy-vGvOz wherein x/y≦2; z/y≦4; 0≦w≦0.3x; 0≦v≦0.3y; A is a Group VIII element; F is an element that is different from A but has, in said composition, the same valence state as A; B is an element different from A and F, and is an element whose simple oxide, in which B is at the same valence state as in the complex oxide, is not reducible in the presence of hydrogen gas at a temperature less than about 900° C.; G is an element different from A, B and F, and is an element whose simple oxide, in which G is at the same valence state as in the complex oxide, is not reducible in the presence of hydrogen gas at a temperature less than about 900° C.; and O is oxygen. The complex oxide is reduced at a temperature less that 950° C. Methods of making, uses for and carbon fibril-containing product made with these activated catalysts are also provided.
摘要翻译：提供能够与碳质气体反应时能够选择性地生长单壁碳纳米管的活化催化剂。通过还原包含复合氧化物的催化剂形成活化的催化剂。复合氧化物可以具有式Ax-wFwBy-vGvOz，其中x / y＆nlE; 2; z / y＆nlE; 4; 0＆nlE; w＆nlE; 0.3x; 0＆nlE; v＆nlE; 0.3y; A是VIII族元素; F是与A不同的元素，在所述组合物中具有与A相同的价态; B是与A和F不同的元素，并且是其中B与复合氧化物处于相同价态的简单氧化物在氢气存在下在小于约900°的温度下不可还原的元素 C。; G是不同于A，B和F的元素，并且是其中G与复合氧化物处于相同价态的简单氧化物的元素在氢气存在下在小于约 900°C。而O是氧。复合氧化物在低于950℃的温度下还原。还提供了用这些活化的催化剂制备，用于含有原纤维的产物的方法。

23. 发明申请

US20090286679A1 SINGLE-WALLED CARBON NANOTUBE CATALYST 审中-公开
标题翻译：单壁碳纳米管催化剂
公开(公告)号：US20090286679A1
公开(公告)日：2009-11-19
申请号：US11841505
申请日：2007-08-20
申请人： Jun Ma , David Moy
发明人： Jun Ma , David Moy
IPC分类号： B01J23/00
CPC分类号： D01F9/127 , B01J21/005 , B01J23/002 , B01J23/005 , B01J23/78 , B01J37/0236 , B01J37/031 , B01J37/08 , B01J37/18 , B01J2523/00 , B82Y30/00 , B82Y40/00 , C01B32/162 , C01B2202/02 , B01J2523/22 , B01J2523/842 , B01J2523/845 , B01J2523/41 , B01J2523/31
摘要： An activated catalyst capable of selectively growing single-walled carbon nanotubes when reacted with carbonaceous gas is provided. The activated catalyst is formed by reducing a catalyst that comprises a complex oxide. The complex oxide may be of formula AxByOz, wherein x/y≦2 and z/y≦4, A being a Group VIII element and B being an element such that an oxide of element B is not reducible in the presence of hydrogen at a temperature less than or equal to about 900° C. Methods of making, uses for and carbon fibril-containing product made with these activated catalysts are also provided.
摘要翻译：提供能够与碳质气体反应时能够选择性地生长单壁碳纳米管的活化催化剂。通过还原包含复合氧化物的催化剂形成活化的催化剂。复合氧化物可以具有式AxByOz，其中x / y <= 2且z / y <= 4，A是VIII族元素，B是使元素B的氧化物在氢气存在下不可还原的元素在低于或等于约900℃的温度下，还提供了用这些活化的催化剂制备，使用和含碳原子纤维的产品的方法。

24. 发明授权

US07968489B2 Methods of preparing supported catalysts from metal loaded carbon nanotubes 失效
标题翻译：从负载碳纳米管的碳纳米管制备载体催化剂的方法
公开(公告)号：US07968489B2
公开(公告)日：2011-06-28
申请号：US11841359
申请日：2007-08-20
申请人： Jun Ma , David Moy , Asif Chishti , Jun Yang
发明人： Jun Ma , David Moy , Asif Chishti , Jun Yang
IPC分类号： B01J21/18 , B01J27/06 , B01J23/00 , B01J23/02 , B01J23/06 , B01J23/40 , B01J23/74
CPC分类号： C07C209/36 , B01J21/185 , B01J23/26 , B01J23/28 , B01J23/42 , B01J23/44 , B01J35/006 , B01J35/0066 , B01J35/06 , B01J37/0009 , B01J37/0207 , B01J37/06 , B01J37/20 , B01J37/30 , B82Y30/00 , B82Y40/00 , C01B32/174 , C01B2202/02 , C01B2202/06 , Y10S977/742 , Y10S977/745 , Y10S977/748 , Y10S977/75 , Y10S977/752 , C07C211/46
摘要： A new method for preparing a supported catalyst is herein provided. Carbon nanotubes are functionalized by contacting them with an oxidizing agent to form functionalized carbon nanotubes. A metal catalyst is then loaded or deposited onto the functionalized carbon nanotubes. The mixture is then extruded to form the supported catalyst comprising a carbon nanotube structure containing metal catalyst more evenly dispersed within the internal structure of the carbon nanotube structure.
摘要翻译：本文提供了一种制备负载型催化剂的新方法。通过使碳纳米管与氧化剂接触以形成官能化的碳纳米管来官能化。然后将金属催化剂负载或沉积到官能化的碳纳米管上。然后将混合物挤出以形成负载的催化剂，其包括更均匀地分散在碳纳米管结构的内部结构内的含有金属催化剂的碳纳米管结构。

25. 发明授权

US07576027B2 Methods of making carbide and oxycarbide containing catalysts 失效
标题翻译：制备含碳化碳和含碳氧化物的催化剂的方法
公开(公告)号：US07576027B2
公开(公告)日：2009-08-18
申请号：US11608359
申请日：2006-12-08
申请人： Jun Ma , David Moy
发明人： Jun Ma , David Moy
IPC分类号： B01J27/22 , B01J21/18 , B01J23/00
CPC分类号： B01J27/22 , B01J21/185 , B01J23/28 , B01J37/08 , B82Y30/00 , B82Y40/00 , C01B32/168 , C01B32/18 , C01B32/90 , Y10S977/742 , Y10S977/745 , Y10S977/748 , Y10S977/749 , Y10S977/788 , Y10S977/81 , Y10S977/811 , Y10S977/847
摘要： Methods for forming compositions including carbide-containing nanorods and/or oxycarbide-containing nanorods and/or carbon nanotubes bearing carbides and oxycarbides. Rigid porous structures including oxycarbide-containing nanorods and/or carbide containing nanorods and/or carbon nanotubes bearing modified carbides and oxycarbides and methods of making the same are also provided. The compositions and rigid porous structures of the invention can be used either as catalyst and/or catalyst supports in fluid phase catalytic chemical reactions. Processes for making supported catalyst for selected fluid phase catalytic reactions are also provided.
摘要翻译：用于形成包含含碳纳米棒和/或含碳氧化物的纳米棒和/或含有碳化物和碳氧化物的碳纳米管的组合物的方法。还提供了包括含有碳氧化物的纳米棒和/或包含纳米棒和/或含有改性碳化物和碳氧化物的碳纳米管的刚性多孔结构及其制备方法。本发明的组合物和刚性多孔结构可用作流化相催化化学反应中的催化剂和/或催化剂载体。还提供了用于制备选择的流化相催化反应的负载型催化剂的方法。

26. 发明申请

US20080039315A1 METHODS OF PREPARING SUPPORTED CATALYSTS FROM METAL LOADED CARBON NANOTUBES 失效
标题翻译：从金属负载碳纳米管制备支持催化剂的方法
公开(公告)号：US20080039315A1
公开(公告)日：2008-02-14
申请号：US11841359
申请日：2007-08-20
申请人： Jun Ma , David Moy , Asif Chishti , Jun Yang
发明人： Jun Ma , David Moy , Asif Chishti , Jun Yang
IPC分类号： B01J21/18
CPC分类号： C07C209/36 , B01J21/185 , B01J23/26 , B01J23/28 , B01J23/42 , B01J23/44 , B01J35/006 , B01J35/0066 , B01J35/06 , B01J37/0009 , B01J37/0207 , B01J37/06 , B01J37/20 , B01J37/30 , B82Y30/00 , B82Y40/00 , C01B32/174 , C01B2202/02 , C01B2202/06 , Y10S977/742 , Y10S977/745 , Y10S977/748 , Y10S977/75 , Y10S977/752 , C07C211/46
摘要： A new method for preparing a supported catalyst is herein provided. Carbon nanotubes are functionalized by contacting them with an oxidizing agent to form functionalized carbon nanotubes. A metal catalyst is then loaded or deposited onto the functionalized carbon nanotubes. The mixture is then extruded to form the supported catalyst comprising a carbon nanotube structure containing metal catalyst more evenly dispersed within the internal structure of the carbon nanotube structure.
摘要翻译：本文提供了一种制备负载型催化剂的新方法。通过使碳纳米管与氧化剂接触以形成官能化的碳纳米管来官能化。然后将金属催化剂负载或沉积到官能化的碳纳米管上。然后将混合物挤出以形成负载的催化剂，其包括更均匀地分散在碳纳米管结构的内部结构内的含有金属催化剂的碳纳米管结构。

27. 发明申请

US20070179050A1 Methods of Making Carbide And Oxycarbide Containing Catalysts 失效
标题翻译：制备含有催化剂的硬质合金和含氧化碳的方法
公开(公告)号：US20070179050A1
公开(公告)日：2007-08-02
申请号：US11608359
申请日：2006-12-08
申请人： Jun Ma , David Moy
发明人： Jun Ma , David Moy
IPC分类号： B01J21/18
CPC分类号： B01J27/22 , B01J21/185 , B01J23/28 , B01J37/08 , B82Y30/00 , B82Y40/00 , C01B32/168 , C01B32/18 , C01B32/90 , Y10S977/742 , Y10S977/745 , Y10S977/748 , Y10S977/749 , Y10S977/788 , Y10S977/81 , Y10S977/811 , Y10S977/847
摘要： Methods for forming compositions including carbide-containing nanorods and/or oxycarbide-containing nanorods and/or carbon nanotubes bearing carbides and oxycarbides. Rigid porous structures including oxycarbide-containing nanorods and/or carbide containing nanorods and/or carbon nanotubes bearing modified carbides and oxycarbides and methods of making the same are also provided. The compositions and rigid porous structures of the invention can be used either as catalyst and/or catalyst supports in fluid phase catalytic chemical reactions. Processes for making supported catalyst for selected fluid phase catalytic reactions are also provided.
摘要翻译：用于形成包含含碳纳米棒和/或含碳氧化物的纳米棒和/或含有碳化物和碳氧化物的碳纳米管的组合物的方法。还提供了包括含有碳氧化物的纳米棒和/或包含纳米棒和/或含有改性碳化物和碳氧化物的碳纳米管的刚性多孔结构及其制备方法。本发明的组合物和刚性多孔结构可用作流化相催化化学反应中的催化剂和/或催化剂载体。还提供了用于制备选择的流化相催化反应的负载型催化剂的方法。

28. 发明授权

US07169730B2 Modified carbide and oxycarbide containing catalysts and methods of making and using thereof 失效
标题翻译：含有改性碳化物和含碳氧化物的催化剂及其制备和使用方法
公开(公告)号：US07169730B2
公开(公告)日：2007-01-30
申请号：US10873739
申请日：2004-06-22
申请人： Jun Ma , David Moy
发明人： Jun Ma , David Moy
IPC分类号： B01J21/18 , C07C5/02 , C07C5/22 , C07C2/58 , C07C25/00
CPC分类号： B01J21/185 , B01J21/18 , B01J27/22 , B01J35/023 , B01J37/24 , B01J37/28 , B82Y30/00 , B82Y40/00 , C01B32/15 , C01B32/168 , C01B32/18 , C01B32/907 , C01B2202/34 , C01B2202/36 , C01P2002/72 , C01P2004/03 , C01P2004/04 , C01P2004/13 , C01P2004/50 , C01P2004/64 , C01P2004/80 , C01P2004/82 , C01P2006/10 , C01P2006/14 , C01P2006/60 , C01P2006/80 , C30B23/00 , C30B29/605 , D01F9/12 , D01F11/122 , Y10S977/788 , Y10T428/249962 , Y10T428/249967 , Y10T428/25 , Y10T428/2918 , Y10T428/292
摘要： Compositions including modified carbide-containing nanorods and/or modified oxycarbide-containing nanorods and/or modified carbon nanotubes bearing carbides and oxycarbides and methods of making the same are provided. Rigid porous structures including modified oxycarbide-containing nanorods and/or modified carbide containing nanorods and/or modified carbon nanotubes bearing modified carbides and oxycarbides and methods of making the same are also provided. The compositions and rigid porous structures of the invention can be used either as catalyst and/or catalyst supports in fluid phase catalytic chemical reactions. Processes for making supported catalyst for selected fluid phase catalytic reactions are also provided.
摘要翻译：提供了包含改性的含碳纳米棒和/或修饰的含碳氧化物的纳米棒和/或含有碳化物和碳氧化物的改性碳纳米管的组合物及其制备方法。还提供了包含改性含碳氧化物的纳米棒和/或含有纳米棒和/或改性碳纳米管的修饰碳纳米管和碳氧化物的刚性多孔结构及其制备方法。本发明的组合物和刚性多孔结构可用作流化相催化化学反应中的催化剂和/或催化剂载体。还提供了用于制备选择的流化相催化反应的负载型催化剂的方法。

29. 发明授权

US06841508B2 Carbide and oxycarbide based compositions, rigid porous structures including the same, methods of making and using the same 失效
标题翻译：基于碳化物和碳氧化物的组合物，包括其的刚性多孔结构，制备和使用它们的方法
公开(公告)号：US06841508B2
公开(公告)日：2005-01-11
申请号：US10170269
申请日：2002-06-11
申请人： David Moy , Chunming Niu , Jun Ma , James M. Willey
发明人： David Moy , Chunming Niu , Jun Ma , James M. Willey
IPC分类号： C04B38/00 , B01J21/18 , B01J27/22 , B01J27/224 , B01J35/02 , C01B31/02 , C01B31/30 , C07B61/00 , C07C5/03 , C07C5/27 , C07C7/163 , C07C9/06 , C07C9/12 , C07C9/22 , C10G35/04 , C10G45/04 , C10G45/44 , C10G45/58 , C10G47/02 , C30B23/00 , D01F9/12 , D01F11/12 , C01B35/10 , C04B35/52 , B32B5/24
CPC分类号： B82Y30/00 , B01J21/18 , B01J27/22 , B01J35/023 , B82Y40/00 , C01B32/168 , C01B32/907 , C01B2202/36 , C01P2002/72 , C01P2004/03 , C01P2004/04 , C01P2004/13 , C01P2004/50 , C01P2004/64 , C01P2004/80 , C01P2004/82 , C01P2006/10 , C01P2006/14 , C01P2006/60 , C01P2006/80 , C30B23/00 , C30B29/605 , D01F9/12 , D01F11/122 , Y10S977/737 , Y10S977/762 , Y10S977/895 , Y10T428/249962 , Y10T428/249967 , Y10T428/25 , Y10T428/2918 , Y10T428/292
摘要： Compositions including oxycarbide-based nanorods and/or carbide-based nanorods and/or carbon nanotubes bearing carbides and oxycarbides and methods of making the same are provided.Rigid porous structures including oxycarbide-based nanorods and/or carbide based nanorods and/or carbon nanotubes bearing carbides and oxycarbides and methods of making the same are also provided.The compositions and rigid porous structures of the invention can be used either as catalyst and/or catalyst supports in fluid phase catalytic chemical reactions. Processes for making supported catalyst for selected fluid phase catalytic reactions are also provided. The fluid phase catalytic reactions catalyzed include hydrogenation, hydrodesulfurisation, hydrodenitrogenation, hydrodemetallisation, hydrodeoxigenation, hydrodearomatization, dehydrogenation, hydrogenolysis, isomerization, alkylation, dealkylation and transalkylation.
摘要翻译：提供了包括基于碳氧化物的纳米棒和/或碳化物基纳米棒和/或碳纳米管和碳纳米管的组合物及其制备方法。包括基于碳氧化物的纳米棒和/或碳化物基纳米棒和/或碳纳米管的刚性多孔结构还提供了含碳化物和碳氧化物及其制备方法。本发明的组合物和刚性多孔结构可用作流化相催化化学反应中的催化剂和/或催化剂载体。还提供了用于制备选择的流化相催化反应的负载型催化剂的方法。催化的流相催化反应包括氢化，加氢脱硫，加氢脱氮，加氢脱金属，加氢脱氧，氢化脱氢，脱氢，氢解，异构化，烷基化，脱烷基化和烷基转移。

30. 发明授权

US06809229B2 Method of using carbide and/or oxycarbide containing compositions 失效
标题翻译：使用碳化物和/或含碳氧化物的组合物的方法
公开(公告)号：US06809229B2
公开(公告)日：2004-10-26
申请号：US10023618
申请日：2001-12-18
申请人： David Moy , Chunming Niu , Jun Ma , Jason M. Willey
发明人： David Moy , Chunming Niu , Jun Ma , Jason M. Willey
IPC分类号： C07C522
CPC分类号： B82Y30/00 , B01J21/18 , B01J27/22 , B01J35/023 , B82Y40/00 , C01B32/15 , C01B32/168 , C01B32/18 , C01B32/907 , C01B32/949 , C01B2202/34 , C01B2202/36 , C01P2002/72 , C01P2004/03 , C01P2004/04 , C01P2004/13 , C01P2004/50 , C01P2004/64 , C01P2004/80 , C01P2004/82 , C01P2006/10 , C01P2006/14 , C01P2006/60 , C01P2006/80 , C10G25/003 , C10G45/02 , C10G45/60 , C10G2300/1081 , C10G2300/1088 , C10G2300/202 , C30B23/00 , C30B29/605 , D01F9/12 , D01F11/122
摘要： Compositions including carbide-containing nanorods and/or oxycarbide-containing nanorods and/or carbon nanotubes bearing carbides and oxycarbides and methods of making the same are provided. Rigid porous structures including oxycarbide-containing nanorods and/or carbide containing nanorods and/or carbon nanotubes bearing carbides and oxycarbides and methods of making the same are also provided. The compositions and rigid porous structures of the invention can be used either as catalyst and/or catalyst supports in fluid phase catalytic chemical reactions. Processes for making supported catalyst for selected fluid phase catalytic reactions are also provided.
摘要翻译：提供了包括含碳纳米棒和/或含碳氧化物的纳米棒和/或含有碳化物和碳氧化物的碳纳米管的组合物及其制备方法。还提供了包括含有碳氧化物的纳米棒和/或碳纳米棒和/或含有碳化物和碳氧化物的碳纳米管的刚性多孔结构及其制备方法。本发明的组合物和刚性多孔结构可用作流化相催化化学反应中的催化剂和/或催化剂载体。还提供了用于制备选择的流化相催化反应的负载型催化剂的方法。

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