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1. 发明授权

US5030787A Catalytic disproportionation/transalkylation utilizing a C9+ aromatics feed 失效
标题翻译：使用C9 +芳族化合物进料的催化歧化/烷基转移
公开(公告)号：US5030787A
公开(公告)日：1991-07-09
申请号：US511145
申请日：1990-04-19
申请人： Robert P. L. Absil , Scott Han , David O. Marler , David S. Shihabi , James C. Vartuli , Philip Varghese
发明人： Robert P. L. Absil , Scott Han , David O. Marler , David S. Shihabi , James C. Vartuli , Philip Varghese
IPC分类号： C07C4/18
CPC分类号： C07C4/18 , C07C2529/70
摘要： A feedstock containing one or more C.sub.9 + aromatic compounds, and optionally benzene and/or toluene, undergoes conversion over a catalyst comprising a zeolite possessing a Constraint Index of from 1 to about 3 to provide a product containing a substantial amount of C.sub.6 -C.sub.8 aromatic compounds, e.g. benzene and xylene(s), predominantly the latter.
摘要翻译：含有一种或多种C 9+芳族化合物，以及任选的苯和/或甲苯的原料经由含有约1至约3约束指数的沸石的催化剂进行转化以提供含有大量C 6 -C 8芳族化合物，例如苯和二甲苯，主要是后者。

2. 发明授权

US4851604A Toluene disproportionation 失效
标题翻译：甲苯歧化
公开(公告)号：US4851604A
公开(公告)日：1989-07-25
申请号：US92842
申请日：1987-09-02
申请人： Robert P. L. Absil , Scott Han , David O. Marler , David S. Shihabi
发明人： Robert P. L. Absil , Scott Han , David O. Marler , David S. Shihabi
IPC分类号： B01J29/65 , B01J29/40 , C07B61/00 , C07C1/00 , C07C6/12 , C07C15/02 , C07C67/00
CPC分类号： C07C6/123 , C07C2529/40 , C07C2529/65 , C07C2529/70 , Y02P20/52
摘要： An improved process is provided for vapor-phase disproportionation of toluene over catalyst comprising a molecular sieve having a high lattice aluminum content whereby its silica/alumina mole ratio is less than 55 and a diffusion rate constant of less than about 150 sec.sup.-1.

3. 发明授权

US4962257A Process for the catalytic disproportionation of toluene 失效
标题翻译：甲苯催化歧化过程
公开(公告)号：US4962257A
公开(公告)日：1990-10-09
申请号：US469633
申请日：1990-01-24
申请人： Robert P. L. Absil , Scott Han , David O. Marler , David S. Shihabi
发明人： Robert P. L. Absil , Scott Han , David O. Marler , David S. Shihabi
IPC分类号： B01J29/04 , C07C2/12 , C07C6/12
CPC分类号： B01J29/04 , C07C2/12 , C07C6/123 , C07C2529/06 , C07C2529/70
摘要： A process is provided for the disproportionation of toluene which comprises contacting toluene under disproportionation conditions with a catalyst comprising a particular synthetic porous crystalline molecular sieve.
摘要翻译：提供了用于甲苯歧化的方法，其包括在歧化条件下将甲苯与包含特定的合成多孔结晶分子筛的催化剂接触。

4. 发明授权

US5085762A Catalytic cracking of hydrocarbons 失效
标题翻译：碳氢化合物的催化裂化
公开(公告)号：US5085762A
公开(公告)日：1992-02-04
申请号：US548349
申请日：1990-07-05
申请人： Robert P. L. Absil , Emmerson Bowes , Gary J. Green , David O. Marler , David S. Shihabi , Richard F. Socha
发明人： Robert P. L. Absil , Emmerson Bowes , Gary J. Green , David O. Marler , David S. Shihabi , Richard F. Socha
IPC分类号： B01J29/70 , B01J29/86 , C10G11/05
CPC分类号： B01J29/7038 , B01J29/86 , C10G11/05 , B01J2229/26 , B01J2229/36 , B01J2229/42
摘要： Emission of noxious nitrogen oxides with the flue gas from the regenerator of a fluid catalytic cracking plant are reduced by incorporating into the circulating inventory of cracking catalyst separate additive particles that contain a copper-loaded zeolite material having a characteristic structure with a defined X-ray diffraction pattern. The preferred material of this type is zeolite MCM-22. The copper may be exchanged onto the zeolite or impregnated into the catalyst. In addition, the catalyst may include titanium or zirconium to provide stability and further improvements in stability may be obtained with the addition of rareearth metal cations, especially cerium or yttrium. NOX and CO emissions from the regenerator are reduced, and the gasoline produced in the unit may have an improved octane number.
摘要翻译：流化催化裂化装置的再生器的废气中的有害氮氧化物的排放通过将含有具有特定结构的含铜负载沸石材料的裂化催化剂的分开的添加剂颗粒加入循环库存中来减少，所述添加剂颗粒具有规定的X射线衍射图案。这种类型的优选材料是沸石MCM-22。铜可以交换到沸石上或浸入催化剂中。此外，催化剂可以包括钛或锆以提供稳定性，并且通过添加乳剂金属阳离子，特别是铈或钇，可以获得稳定性的进一步改善。来自再生器的NO x和CO排放减少，并且在该单元中产生的汽油可能具有改善的辛烷值。

5. 发明授权

US5013422A Catalytic hydrocracking process 失效
标题翻译：催化加氢裂化工艺
公开(公告)号：US5013422A
公开(公告)日：1991-05-07
申请号：US479790
申请日：1990-02-14
申请人： Robert P. L. Absil , Thomas F. Degnan , Scott Han , David O. Marler , Richard F. Socha , Michael R. Stapleton
发明人： Robert P. L. Absil , Thomas F. Degnan , Scott Han , David O. Marler , Richard F. Socha , Michael R. Stapleton
IPC分类号： B01J29/04 , B01J29/14 , B01J29/16 , B01J29/70 , B01J29/74 , B01J29/80 , C07C2/12 , C10G47/16 , C10G65/10 , C10G65/12
CPC分类号： B01J29/7038 , B01J29/04 , B01J29/146 , B01J29/166 , B01J29/7088 , B01J29/7415 , B01J29/7815 , B01J29/7876 , B01J29/80 , B01J29/86 , C07C2/12 , C10G47/16 , C10G65/10 , C10G65/12 , B01J2229/16 , B01J2229/26 , B01J2229/42 , C07C2529/70
摘要： A hydrocracking process is provided comprising contacting a hydrocarbon stream under hydrocracking conditions and in the presence of hydrogen with a catalyst composition which comprises a synthetic porous crystalline zeolite having a particular X-ray diffraction pattern. An embodiment of the invention provides a process for reducing the pour point of a waxy component-containing hydrocarbon oil by hydrocracking and dewaxing. Another embodiment of the invention provides a dual-stage hydrocracking process to produce premium gasoline and distillate boiling range products.
摘要翻译：提供加氢裂化方法，包括在加氢裂化条件下和氢存在下使烃流与包含具有特定X射线衍射图的合成多孔结晶沸石的催化剂组合物接触。本发明的一个实施方案提供了通过加氢裂化和脱蜡来降低含蜡组分的烃油的倾点的方法。本发明的另一个实施方案提供了一种双级加氢裂化方法，用于生产高级汽油和馏出物沸点产物。

6. 发明授权

US5173461A Toluene disproportionation catalyst 失效
标题翻译：甲苯歧化催化剂
公开(公告)号：US5173461A
公开(公告)日：1992-12-22
申请号：US497046
申请日：1990-03-21
申请人： Robert P. Absil , Scott Han , David S. Shihabi , David O. Marler , Clarence D. Chang , Donna M. Mitko
发明人： Robert P. Absil , Scott Han , David S. Shihabi , David O. Marler , Clarence D. Chang , Donna M. Mitko
IPC分类号： B01J29/40 , C07C6/12
CPC分类号： B01J29/40 , C07C6/126 , B01J2229/12 , B01J2229/26 , B01J2229/32 , B01J2229/42 , C07C2529/40
摘要： A catalyst comprising a molecular sieve having a lattice aluminum content in which the silica/alumina framework mole ratio is less than 55, and having a diffusion rate constant of less than about 150 sec.sup.-1 .times.10.sup.-6 is particularly useful for vapor-phase disproportionation of toluene.
摘要翻译：包含具有格子铝含量的分子筛的催化剂，其二氧化硅/氧化铝骨架摩尔比小于55，并且具有小于约150秒-1×10 -6的扩散速率常数特别适用于气相歧化甲苯。

7. 发明授权

US5173278A Denitrification of flue gas from catalytic cracking 失效
标题翻译：烟气从催化裂化中脱氮
公开(公告)号：US5173278A
公开(公告)日：1992-12-22
申请号：US669821
申请日：1991-03-15
申请人： David O. Marler , Ajit V. Sapre , David S. Shihabi , Richard F. Socha , Scott A. Stevenson
发明人： David O. Marler , Ajit V. Sapre , David S. Shihabi , Richard F. Socha , Scott A. Stevenson
IPC分类号： B01D53/86 , C10G11/18
CPC分类号： B01D53/8625 , B01D53/8621 , C10G11/182 , B01D2257/408 , Y02P30/446
摘要： A flue gas that contains small amounts of both HCN and NO.sub.x, produced, for example, by catalyst regeneration in the fluid catalytic cracking of a petroleum gas oil, is readily denitrified by the catalyzed reaction that proceeds approximately according to:HCN+NO.fwdarw.N.sub.2 (gas)+CO+CO.sub.2 +H.sub.2 OIf the molar ratio of HCN to NO in the flue gas is about 1.0, e.g. in the range of about 0.8 to 1.2, effective denitrification is achieved without first changing the composition of the flue gas by contacting it with catalyst under conversion conditions including elevated temperature. If the molar ratio of HCN to NO exceeds 1.2, the ratio may be adjusted to about 1.0 to 1.1 by thermal or catalytic oxidation in the presence of oxygen gas, followed by catalytic denitrification. If the molar ratio is less than about 0.8, the effective molar ratio is adjusted to about 1.0 to 1.1 by adding NH.sub.3 gas, followed by denitirification. In all three instances an excessive content of carbon monoxide in the flue gas may be corrected by passing the denitrified flue gas to a CO-boiler.Catalysts for the denitrification reaction are described and exemplified by crystalline zeolites of the ZSM-5 type, and by vanadium oxide supported on titania.
摘要翻译：含有少量HCN和NOx的烟道气，例如通过在石油瓦斯油的流化催化裂化中的催化剂再生产生的烟气，可以通过大致按以下方式进行的催化反应脱氮：HCN + NO-> N2（气体）+ CO + CO2 + H2O如果烟气中HCN与NO的摩尔比为约1.0，在约0.8至1.2的范围内，无需首先在包括升高的温度的转化条件下将催化剂与催化剂接触，而不改变烟道气的组成，实现有效的脱氮。如果HCN与NO的摩尔比超过1.2，则在氧气存在下通过热或催化氧化将该比例调节至约1.0至1.1，然后进行催化反硝化。如果摩尔比小于约0.8，则通过加入NH 3气体将有效摩尔比调节至约1.0-1.1，然后进行脱硝。在所有三种情况下，可以通过将反硝化烟道气通过CO锅炉来校正烟道气中过量的一氧化碳。用于脱氮反应的催化剂通过ZSM-5型的结晶沸石和负载在二氧化钛上的氧化钒来描述和例示。

8. 发明授权

US06143261A Catalytic reduction of nitrogen oxide emissions with MCM-49 and MCM-56 失效
标题翻译：用MCM-49和MCM-56催化还原氮氧化物排放
公开(公告)号：US06143261A
公开(公告)日：2000-11-07
申请号：US990459
申请日：1997-12-15
申请人： Daria N. Lissy , David O. Marler , John P. McWilliams , David S. Shihabi , Sanjay B. Sharma
发明人： Daria N. Lissy , David O. Marler , John P. McWilliams , David S. Shihabi , Sanjay B. Sharma
IPC分类号： B01D53/86 , B01D53/94 , B01J29/03 , B01J29/04 , C01B21/00
CPC分类号： B01J29/042 , B01D53/8628 , B01D53/9418 , B01J29/0308 , B01J29/041 , B01J29/045 , B01D2251/2067 , B01D2255/202 , B01D2255/204 , B01D2255/20761 , Y02T10/24
摘要： MCM-56 and MCM-49 have been demonstrated to be effective catalysts for the reduction of nitrogen oxide (NO.sub.x) emissions in a net oxidizing environment such as Selective Catalytic Reduction or lean burn engine exhaust applications. MCM-56 and MCM-49 can be utilized as a component of a spherical or cylindrical catalyst particle or as a wash coat on a ceramic or metallic monolith. Optionally, a transition metal such as copper, can be added to the catalyst for improved activity.
摘要翻译： MCM-56和MCM-49已经被证明是在净氧化环境（如选择性催化还原或贫燃发动机排气应用）中减少氮氧化物（NOx）排放的有效催化剂。 MCM-56和MCM-49可用作球形或圆柱形催化剂颗粒的组分或作为陶瓷或金属整料上的洗涤涂层。任选地，可以将诸如铜的过渡金属加入到催化剂中以改善活性。

9. 发明授权

US5780703A Process for producing low aromatic diesel fuel with high cetane index 失效
标题翻译：具有高十六烷指数的低芳烃柴油的生产工艺
公开(公告)号：US5780703A
公开(公告)日：1998-07-14
申请号：US513107
申请日：1995-08-09
申请人： Clarence D. Chang , Stuart D. Hellring , David O. Marler , Jose G. Santiesteban , James C. Vartuli
发明人： Clarence D. Chang , Stuart D. Hellring , David O. Marler , Jose G. Santiesteban , James C. Vartuli
IPC分类号： B01J23/30 , B01J23/882 , B01J23/888 , B01J37/03 , C07C2/58 , C07C5/27 , C10G50/00 , C10G35/04
CPC分类号： C10G50/00 , B01J23/30 , B01J23/882 , B01J23/888 , C07C2/58 , C07C5/2772 , B01J37/03 , C07C2521/06 , C07C2523/30
摘要： A process for converting at least one olefin and at least one isoparaffin to a diesel fuel blending component comprising the steps of contacting the olefin and the isoparaffin with a catalyst comprising an acidic solid comprising a Group IVB metal oxide modified with an oxyanion of a Group VIB metal to provide a diesel fuel. Process conditions can be varied to favor the formation of gasoline, distillate, lube range products or mixtures thereof.
摘要翻译：一种将至少一种烯烃和至少一种异链烷烃转化为柴油燃料共混组分的方法，包括以下步骤：使烯烃和异链烷烃与包含酸性固体的催化剂接触，所述酸性固体包含用VIB族氧基反应改性的IVB族金属氧化物金属提供柴油。工艺条件可以变化以有利于形成汽油，馏出物，润滑剂产品或其混合物。

10. 发明授权

US5063038A Zeolite synthesis using an alcohol or like molecule 失效
标题翻译：使用醇或类似分子的沸石合成
公开(公告)号：US5063038A
公开(公告)日：1991-11-05
申请号：US91612
申请日：1987-08-31
申请人： Garry W. Kirker , Donald J. Klocke , James C. Vartuli , Pochen Chu , David O. Marler , John P. McWilliams
发明人： Garry W. Kirker , Donald J. Klocke , James C. Vartuli , Pochen Chu , David O. Marler , John P. McWilliams
IPC分类号： B01J29/40 , B01J29/65 , B01J29/70 , C01B39/48 , C07C2/66 , C07C4/18
CPC分类号： C07C4/18 , B01J29/40 , B01J29/65 , B01J29/7046 , C01B39/48 , C07C2/66 , B01J2229/20 , B01J2229/26 , B01J2229/36 , B01J2229/42 , C07C2529/65 , C07C2529/70 , Y10S423/35 , Y10S423/36
摘要： There is provided a method for preparing a zeolite other than ZSM-5 from a reaction mixture comprising a mixed organic directing agent which is a combination of (a) an organic nitrogen containing compound such as an amine or a quaternary ammonium compound and (b) an alcohol and/or diol. Particular zeolites synthesized by this method include ZSM-22 and ZSM-23. The use of an alcohol or a diol may inhibit the coformation of ZSM-5. Especially when used to prepare ZSM-23, this method enables the preparation of more catalytically active ZSM-23 of reduced crystallite size and also enables the use of lower crystallization temperatures. Particular mixed organic directing agents for the preparation of ZSM-23 are combination of (a) pyrrolidine and (b) ethanol or ethylene glycol. Other factors which enhance the activity of ZSM-23 include the use of the following in the reaction mixtures for preparing ZSM-23: potassium ions; precipitated silica particles as sources of silica; and spray dried precipitated silica/alumina particles as sources of silica and alumina. The catalytic stability of alumina bound ZSM-23 catalysts is especially enhanced by steaming. Particular reactions which can be catalyzed by ZSM-23 made according to methods described herein include the dealkylation of ethylbenzene and the alkylation of benzene with ethylene.
摘要翻译：提供了一种从含有（a）有机氮化合物如胺或季铵化合物的组合的混合有机导向剂的反应混合物制备ZSM-5以外的沸石的方法，（b）醇和/或二醇。通过该方法合成的特定沸石包括ZSM-22和ZSM-23。使用醇或二醇可能会抑制ZSM-5的共形。特别是当用于制备ZSM-23时，该方法能够制备更小的微晶尺寸的更具催化活性的ZSM-23，并且还能够使用较低的结晶温度。用于制备ZSM-23的特殊混合有机导向剂是（a）吡咯烷和（b）乙醇或乙二醇的组合。提高ZSM-23活性的其他因素包括在制备ZSM-23：钾离子的反应混合物中使用以下物质：沉淀二氧化硅颗粒作为二氧化硅来源; 和喷雾干燥的沉淀二氧化硅/氧化铝颗粒作为二氧化硅和氧化铝的来源。氧化铝结合的ZSM-23催化剂的催化稳定性通过蒸汽特别提高。根据本文所述方法制备的可以由ZSM-23催化的特定反应包括乙苯的脱烷基化和苯与乙烯的烷基化。

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