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1. 发明申请

WO2011141546A3 PROCESS FOR LIQUEFYING A CELLULOSIC MATERIAL 审中-公开
标题翻译：用于液化材料的方法
公开(公告)号：WO2011141546A3
公开(公告)日：2012-10-11
申请号：PCT/EP2011057695
申请日：2011-05-12
申请人： SHELL INT RESEARCH , VON HEBEL KLAAS LAMBERTUS , LANGE JEAN-PAUL
发明人： VON HEBEL KLAAS LAMBERTUS , LANGE JEAN-PAUL
IPC分类号： C08H8/00 , C10G1/06
CPC分类号： C10G1/002 , C08H8/00 , C10G1/065 , C10G3/50 , C10G2300/1014 , C10G2300/208 , C10G2300/44 , C10G2400/02 , C10G2400/04 , C10G2400/08 , C10L1/02 , C10L1/04 , C10L2200/0469 , C10L2290/544 , Y02E50/13 , Y02P30/20
摘要： A process for liquefying a cellulosic material to produce a liquefied product, which process comprises contacting the cellulosic material simultaneously with - an acid catalyst; - a solvent mixture containing water and a co-solvent, which co-solvent comprises one or more polar solvents and which co-solvent is present in an amount of more than or equal to 10% by weight and less than or equal to 95% by weight, based on the total weight of water and co-solvent; - a hydrogenation catalyst; and - a source of hydrogen. Products obtained from the above process and use of such products to prepare biofuels.
摘要翻译：一种用于液化纤维素材料以产生液化产物的方法，该方法包括使纤维素材料与酸催化剂同时接触; - 含有水和共溶剂的溶剂混合物，所述共溶剂包含一种或多种极性溶剂，并且所述助溶剂的存在量为大于或等于10重量％且小于或等于95重量％，基于水和助溶剂的总重量; - 氢化催化剂; 和 - 氢源。从上述方法获得的产品和使用这些产品制备生物燃料。

2. 发明申请

WO2011015645A3 PROCESS FOR PREPARING A HYDROXYACID OR HYDROXYESTER 审中-公开
标题翻译：制备羟肟酸或羟肟酸酯的方法
公开(公告)号：WO2011015645A3
公开(公告)日：2011-03-31
申请号：PCT/EP2010061461
申请日：2010-08-06
申请人： SHELL INT RESEARCH , HAAN RENE JOHAN , LANGE JEAN-PAUL
发明人： HAAN RENE JOHAN , LANGE JEAN-PAUL
IPC分类号： C07C51/377 , C07C53/126 , C07C67/31
CPC分类号： C07C51/377 , C07C67/03 , C07D307/33 , Y02P20/127 , C07C59/01 , C07C69/533
摘要： A process for preparing a hydroxyacid or hydroxyester from a reactant selected from (a) a carboxylic acid having an aldehyde or keto group; and (b) an ester of a carboxylic acid having an aldehyde or keto group; by contacting the reactant with a metal catalyst in the presence of hydrogen, wherein the metal catalyst is supported on a titanium dioxide or zirconium dioxide support.
摘要翻译：从选自（a）具有醛或酮基的羧酸的反应物制备羟基酸或羟基酯的方法; 和（b）具有醛或酮基的羧酸酯; 通过在氢的存在下使反应物与金属催化剂接触，其中金属催化剂负载在二氧化钛或二氧化锆载体上。

3. 发明申请

WO2011015385A1 PROCESS FOR PREPARING AN ESTER 审中-公开
标题翻译：制备ESTER的方法
公开(公告)号：WO2011015385A1
公开(公告)日：2011-02-10
申请号：PCT/EP2010/055862
申请日：2010-04-29
申请人： SHELL INTERNATIONALE RESEARCH MAATSCHAPPIJ B.V. , HAAN, Rene, Johan , LANGE, Jean-Paul
发明人： HAAN, Rene, Johan , LANGE, Jean-Paul
IPC分类号： C07C67/08
CPC分类号： C07C67/08 , C07C67/00 , C07C69/24
摘要： A process for preparing an ester of formula (I): R 3 CH 2 - (CR 1 R 2 ) n -CH 2 -O-CO-(CR 1 R 2 ) n -CH 2 R 3 (I) wherein n is 1-3 and R 1 and R 2 are each, independently, a hydrogen atom or a carbon-linked organic group and R 3 is a carbon-linked organic group, by hydrogenation of a reactant selected from: (a) a lactone of formula (II) wherein n is 1-3 and R 1 and R 2 are each, independently, a hydrogen atom or a carbon-linked organic group and R 3 is a carbon-linked organic group; (b) an ester of a carboxylic acid of formula (III) R 4 -O-CO- (CR 1 R 2 ) n -CO-R 3 (III) wherein n is 1-3 and R 1 and R 2 are each, independently, a hydrogen atom or a carbon-linked organic group and R 3 and R 4 are a carbon-linked organic group; and c) a carboxylic acid of formula (IV) H-O-CO- (CR 1 R 2 ) n -CO-R 3 (IV) wherein n is 1-3 and R 1 and R 2 are each, independently, a hydrogen atom or a carbon-linked organic group and R 3 is a carbon-linked organic group; which process involves contacting the reactant with a heterogeneous catalyst comprising a hydrogenating metal in the presence of hydrogen, wherein the catalyst is a zeolite-free heterogeneous catalyst comprising a hydrogenating metal supported on a metal oxide or a mixed oxide.
摘要翻译：制备式（I）的酯的方法：R 3 -CH 2 - （CR 1 R 2）n -CH 2 -O-CO-（CR 1 R 2）n -CH 2 R 3（I）其中n为1-3，并且R 1和R 2各自独立地为氢原子或碳连接的有机基团，并且R 3是碳连接的有机基团，通过氢化选自以下的反应物：（a）式（II）的内酯，其中n为1-3且R 1和R 2各自为氢，独立地是氢原子或碳连接的有机基团，并且R 3是碳连接的有机基团; （b）式（III）的羧酸R 4 -O-CO-（CR 1 R 2）n -CO-R 3（III）的酯，其中n为1-3，并且R 1和R 2各自独立地为氢原子或碳键的有机基团，R 3和R 4为碳键的有机基团; 和c）式（Ⅳ）HO-CO-（CR1R2）n-CO-R3（Ⅳ）的羧酸，其中n为1-3，R 1和R 2各自独立地为氢原子或碳键连接的有机基团和R 3是碳键的有机基团; 该方法包括在氢气存在下使反应物与包含氢化金属的多相催化剂接触，其中所述催化剂是不含沸石的多相催化剂，其包含负载在金属氧化物上的氢化金属或混合氧化物。

4. 发明申请

WO2010136436A1 GASOLINE COMPOSITIONS 审中-公开
标题翻译：汽油组合物
公开(公告)号：WO2010136436A1
公开(公告)日：2010-12-02
申请号：PCT/EP2010/057132
申请日：2010-05-25
申请人： SHELL INTERNATIONALE RESEARCH MAATSCHAPPIJ B.V. , FELIX-MOORE, Allison , LANGE, Jean-Paul , SMITH, Johanne
发明人： FELIX-MOORE, Allison , LANGE, Jean-Paul , SMITH, Johanne
IPC分类号： C10L1/02 , C10L1/18 , C10L10/08 , C10L10/10
CPC分类号： C10L10/08 , C10L1/023 , C10L1/19 , C10L10/10
摘要： An unleaded gasoline composition comprising: (i) a gasoline base fuel; and (ii) component A, wherein component A is an alkyl alkenoate compound, or a mixture of alkyl alkenoate compounds, selected from compounds of formula I: wherein R 1 is a linear alkenyl group containing 3 to 5 carbon atoms, optionally substituted by a methyl group, and R 2 is a linear or branched alkyl group containing 1 to 6 carbon atoms. The gasoline composition of the present invention exhibits good lubricity.
摘要翻译：一种无铅汽油组合物，包括：（i）汽油基燃料; 或（ii）成分A，其中组分A为烷基烯酸酯化合物，或选自式I化合物的烷基烯酸酯化合物的混合物：其中R 1为含有3至5个碳原子的直链烯基，任选被甲基并且R 2是含有1至6个碳原子的直链或支链烷基。本发明的汽油组合物表现出良好的润滑性。

5. 发明申请

WO2007023173A8 A PROCESS FOR THE CONVERSION OF FURFURYL ALCOHOL INTO LEVULINIC ACID OR ALKYL LEVULINATE 审中-公开
标题翻译：将糠醇转化为乙酰丙酸或乙酰丙酸的方法
公开(公告)号：WO2007023173A8
公开(公告)日：2007-09-07
申请号：PCT/EP2006065613
申请日：2006-08-24
申请人： SHELL INT RESEARCH , VAN DE GRAAF WOUTER DAVID , LANGE JEAN-PAUL
发明人： VAN DE GRAAF WOUTER DAVID , LANGE JEAN-PAUL
IPC分类号： C07C51/00 , C07C59/185
CPC分类号： C07C51/00 , C07C67/00 , C07C59/185 , C07C69/716
摘要： A process for the conversion of furfuryl alcohol into levulinic acid or alkyl levulinate comprising contacting furfuryl alcohol and water or an alkyl alcohol with a porous heterogeneous catalyst comprising strong acid ion exchange resin, wherein the catalyst has pores with an average pore diameter in the range of from 1 to 1000 nm.
摘要翻译：一种将糠醇转化为乙酰丙酸或乙酰丙酸烷基酯的方法，包括使糠醇和水或烷基醇与包含强酸离子交换树脂的多孔非均相催化剂接触，其中所述催化剂具有平均孔径为从1到1000nm。

6. 发明申请

WO2011015645A2 PROCESS FOR PREPARING A HYDROXYACID OR HYDROXYESTER 审中-公开
标题翻译：制备羟基酸或羟基酯的方法
公开(公告)号：WO2011015645A2
公开(公告)日：2011-02-10
申请号：PCT/EP2010/061461
申请日：2010-08-06
申请人： SHELL INTERNATIONALE RESEARCH MAATSCHAPPIJ B.V. , HAAN, Rene, Johan , LANGE, Jean-Paul
发明人： HAAN, Rene, Johan , LANGE, Jean-Paul
IPC分类号： C07C51/377 , C07D307/33 , C07C59/01
CPC分类号： C07C51/377 , C07C67/03 , C07D307/33 , Y02P20/127 , C07C59/01 , C07C69/533
摘要： A process for preparing a hydroxyacid or hydroxyester from a reactant selected from (a) a carboxylic acid having an aldehyde or keto group; and (b) an ester of a carboxylic acid having an aldehyde or keto group; by contacting the reactant with a metal catalyst in the presence of hydrogen, wherein the metal catalyst is supported on a titanium dioxide or zirconium dioxide support.
摘要翻译：从选自以下的反应物制备羟基酸或羟基酯的方法：（a）具有醛或酮基的羧酸; 和（b）具有醛或酮基的羧酸的酯; 通过在氢存在下使反应物与金属催化剂接触，其中金属催化剂负载在二氧化钛或二氧化锆载体上。

7. 发明申请

WO2009156439A1 PROCESS FOR THE HYDROGENOLYSIS OF FURFURYL DERIVATIVES 审中-公开
标题翻译：呋喃衍生物氢化方法
公开(公告)号：WO2009156439A1
公开(公告)日：2009-12-30
申请号：PCT/EP2009/057899
申请日：2009-06-24
申请人： SHELL INTERNATIONALE RESEARCH MAATSCHAPPIJ B.V. , LANGE, Jean-Paul
发明人： LANGE, Jean-Paul
IPC分类号： C07D307/36
CPC分类号： C07D307/36 , Y02P20/127
摘要： The present invention relates to a process for the hydrogenolysis of a furfuryl derivative to 2-methylfuran derivative, comprising: (a) contacting under liquid phase conditions a solution of the furfuryl derivative in a solvent having a boiling point above the boiling point of furfuryl derivative with hydrogen in the presence of a catalyst comprising a hydrogenation compound to form a 2-methylfuran derivative and water, at a temperature and pressure suitable to maintain the furfuryl derivative in the solvent in the liquid phase, and (b) continuously distilling the 2-methylfuran derivative from the reaction mixture.
摘要翻译：本发明涉及糠基衍生物氢解成2-甲基呋喃衍生物的方法，包括：（a）在液相条件下使糠基衍生物在沸点高于糠基衍生物的沸点的溶剂中接触在含有氢化化合物的催化剂存在下，使氢气在适于将糠基衍生物保持在溶剂中的温度和压力下形成2-甲基呋喃衍生物和水，和（b）连续蒸馏2- 甲基呋喃衍生物。

8. 发明申请

WO2008142127A1 PROCESS FOR CONVERTING LEVULINIC ACID INTO PENTANOIC ACID 审中-公开
标题翻译：将维生素酸转化成苦味酸的方法
公开(公告)号：WO2008142127A1
公开(公告)日：2008-11-27
申请号：PCT/EP2008/056293
申请日：2008-05-21
申请人： SHELL INTERNATIONALE RESEARCH MAATSCHAPPIJ B.V. , AYOUB, Paul Marie , LANGE, Jean-Paul
发明人： AYOUB, Paul Marie , LANGE, Jean-Paul
IPC分类号： C07C51/36 , C07C53/126
CPC分类号： C07C51/36 , C07C53/126
摘要： A process for converting levulinic acid into pentanoic acid, the process comprising the following steps: (a) contacting a feedstock comprising levulinic acid under hydrogenating conditions, in the presence of hydrogen, with a non-acidic heterogeneous hydrogenation catalyst comprising a hydrogenation metal supported on a solid catalyst carrier to obtain a first effluent comprising gamma valerolactone; (b) contacting at least part of the first effluent under hydrogenating conditions, in the presence of hydrogen, with a strongly acidic catalyst and a hydrogenation metal to obtain a second effluent comprising pentanoic acid, wherein step (b) is operated at a conversion per pass of at most 70 wt% to obtain the second effluent comprising pentanoic acid and unconverted gamma valerolactone, and wherein part of the unconverted gamma valerolactone is recycled to step (a) and/or step (b).
摘要翻译：一种将乙酰丙酸转化为戊酸的方法，该方法包括以下步骤：（a）在氢存在下，在氢化条件下，将包含乙酰丙酸的原料与非酸性非均相氢化催化剂接触，所述非酸性非均相氢化催化剂包含负载在固体催化剂载体，以获得包含γ-戊内酯的第一流出物; （b）在氢气条件下，在氢气存在下，与强酸性催化剂和氢化金属接触至少部分第一流出物以获得包含戊酸的第二流出物，其中步骤（b）以每转化率通过至多70重量％以获得包含戊酸和未转化的γ-戊内酯的第二流出物，并且其中部分未转化的γ-戊内酯再循环至步骤（a）和/或步骤（b）。

9. 发明申请

WO2006067171A1 A PROCESS FOR THE HYDROGENATION OF A LACTONE OR OF A CARBOXYLIC ACID OR AN ESTER HAVING A GAMMA-CARBONYL GROUP 审中-公开
标题翻译：一种柠檬酸或羧酸或具有氨基羰基的酯的加氢方法
公开(公告)号：WO2006067171A1
公开(公告)日：2006-06-29
申请号：PCT/EP2005/057009
申请日：2005-12-21
申请人： SHELL INTERNATIONALE RESEARCH MAATSCHAPPIJ B.V. , VAN DEN BRINK, Peter John , VON HEBEL, Klaas Lambertus , LANGE, Jean-Paul , PETRUS, Leonardus
发明人： VAN DEN BRINK, Peter John , VON HEBEL, Klaas Lambertus , LANGE, Jean-Paul , PETRUS, Leonardus
IPC分类号： C07C51/377 , C07C53/126
CPC分类号： C07C51/377 , C07C53/126
摘要： The invention provides a process for the hydrogenation of a reactant selected from the group consisting of : (a) a 5- or 6-membered lactone that is substituted at the ring-closing carbon atom and has a proton at a carbon atom adjacent to the ring-closing carbon atom; (b) an ester of a carboxylic acid having a gamma- carbonyl group and a proton at a carbon atom adjacent to the carbon atom of the carbonyl group; and (c) a carboxylic acid having a gamma-carbonyl group and a proton at a carbon atom adjacent to the carbon atom of the carbonyl group, wherein the reactant is contacted with a strongly acidic heterogeneous catalyst comprising a hydrogenating metal, in the presence of hydrogen, at a temperature in the range of from 100 to 350 °C and a pressure in the range of from 1 to 150 bar (absolute). The invention further provides a fuel composition, preferably a diesel composition, comprising di-alkyl 4-methylnonanedioate or di-alkyl 3-ethyl-4-methylheptanedioate.
摘要翻译：本发明提供了一种用于氢化反应物的方法，所述反应物选自：（a）在闭环碳原子处被取代并且在与碳原子相邻的碳原子处具有质子的5-或6-元内酯闭环碳原子; （b）在与羰基的碳原子相邻的碳原子处具有γ-羰基和质子的羧酸的酯; 和（c）在与羰基的碳原子相邻的碳原子处具有γ-羰基和质子的羧酸，其中反应物与包含氢化金属的强酸性多相催化剂在存在下，氢气，温度范围为100至350℃，压力范围为1至150巴（绝对）。本发明还提供一种燃料组合物，优选含有4-甲基壬二酸二烷基酯或3-乙基-4-甲基庚二酸二烷基酯的柴油组合物。

10. 发明申请

WO2006045765A1 REVERSE FLOW REACTOR WITH INTEGRATED SEPARATION AND PROCESS FOR THE EMPLOYING THIS REACTOR 审中-公开
标题翻译：具有集成分离的反向流动反应器和使用该反应器的方法
公开(公告)号：WO2006045765A1
公开(公告)日：2006-05-04
申请号：PCT/EP2005/055483
申请日：2005-10-24
申请人： SHELL INTERNATIONALE RESEARCH MAATSCHAPPIJ B.V. , BOS, Alouisius, Nicolaas, Renee , KABRA, Girish, Rajkumar , LANGE, Jean-Paul
发明人： BOS, Alouisius, Nicolaas, Renee , KABRA, Girish, Rajkumar , LANGE, Jean-Paul
IPC分类号： B01J8/04
CPC分类号： B01D51/10 , B01D53/02 , B01D2253/10 , B01D2253/202 , B01D2257/204 , B01D2257/30 , B01D2257/80 , B01J8/0446 , B01J2208/00106 , B01J2208/00699 , B01J2208/00707 , B01J2208/025
摘要： The present invention pertains to a reverse-flow reactor comprising at least one catalyst bed which is preceded and followed by at least one bed containing selectively adsorbing material, and its application for in a process for the removal of contaminants from a process stream.
摘要翻译：本发明涉及一种反流反应器，其包含至少一个催化剂床，其前面和后面是至少一个含有选择性吸附材料的床，以及其在从工艺流中除去污染物的方法中的应用。

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