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1. 发明申请

WO2007099111A1 A HYDROGENATION PROCESS FOR THE CONVERSION OF A CARBOXYLIC ACID OR AN ESTER HAVING A CARBONYL GROUP 审中-公开
标题翻译：用于转化羧酸或具有羰基的酯的氢化方法
公开(公告)号：WO2007099111A1
公开(公告)日：2007-09-07
申请号：PCT/EP2007/051879
申请日：2007-02-28
申请人： SHELL INTERNATIONALE RESEARCH MAATSCHAPPIJ B.V. , LANGE, Jean-Paul , PETRUS, Leonardus , HAAN, Rene Johan
发明人： LANGE, Jean-Paul , PETRUS, Leonardus , HAAN, Rene Johan
IPC分类号： C07C51/367 , C07C67/31 , C07D307/32 , C07D309/30
CPC分类号： C07D307/33 , C07C51/367 , C07D309/30 , C07C59/01
摘要： A hydrogenation process for the conversion of a reactant selected from the group consisting of a carboxylic acid having a carbonyl group and an ester of a carboxylic acid having a carbonyl group to form a carboxylic acid or an ester with a hydroxyl group or a lactone, wherein the reactant is contacted with a heterogeneous catalyst comprising a hydrogenating compound, in the presence of formic acid, at a temperature in the range of from 150 to 400 °C and a pressure in the range of from 1.0 to 150 bar (absolute).
摘要翻译：用于将选自具有羰基的羧酸和具有羰基的羧酸的酯的反应物转化以形成羧酸或具有羟基或内酯的酯的氢化方法，其中在甲酸存在下，反应物与包含氢化化合物的非均相催化剂在150-400℃的温度和1.0-150巴（绝对）范围内的压力下接触。

2. 发明申请

WO2011015643A1 PROCESS FOR HYDROGENATION 审中-公开
标题翻译：加氢方法
公开(公告)号：WO2011015643A1
公开(公告)日：2011-02-10
申请号：PCT/EP2010/061458
申请日：2010-08-06
申请人： SHELL INTERNATIONALE RESEARCH MAATSCHAPPIJ B.V. , HAAN, Rene, Johan , LANGE, Jean-Paul
发明人： HAAN, Rene, Johan , LANGE, Jean-Paul
IPC分类号： C07C51/377 , C07C53/126
CPC分类号： C07C51/377 , C07C53/126
摘要： A process for the hydrogenation of a reactant selected from: (a) a 5- or 6-membered lactone that is substituted at the ring-closing carbon atom and has a proton at a carbon atom adjacent to the ring-closing carbon atom; (b) an ester of a carboxylic acid having a gamma- carbonyl group and a proton at a carbon atom adjacent to the carbon atom of the carbonyl group; and (c) a carboxylic acid having a gamma-carbonyl group and a proton at a carbon atom adjacent to the carbon atom of the carbonyl group, which process involves contacting the reactant with a catalyst in the presence of hydrogen, at a temperature from 100 to 3500C and a pressure from 1 to 150 bar (absolute), provided the pressure is low enough to avoid condensation of the heaviest feed component at the temperature chosen, and wherein the catalyst is a weakly acidic heterogeneous catalyst comprising a hydrogenating metal.
摘要翻译：一种选自以下的反应物的氢化方法：（a）在闭环碳原子上被取代并在与闭环碳原子相邻的碳原子处具有质子的5-或6-元内酯; （b）在与羰基的碳原子相邻的碳原子处具有γ-羰基和质子的羧酸的酯; 和（c）在与羰基碳原子相邻的碳原子处具有γ-羰基和质子的羧酸，该方法包括在氢气存在下使反应物与催化剂接触，温度为100℃ 只要压力足够低以避免在所选择的温度下最重的进料组分的冷凝，并且其中催化剂是包含氢化金属的弱酸性非均相催化剂。

3. 发明申请

WO2011015645A3 PROCESS FOR PREPARING A HYDROXYACID OR HYDROXYESTER 审中-公开
标题翻译：制备羟肟酸或羟肟酸酯的方法
公开(公告)号：WO2011015645A3
公开(公告)日：2011-03-31
申请号：PCT/EP2010061461
申请日：2010-08-06
申请人： SHELL INT RESEARCH , HAAN RENE JOHAN , LANGE JEAN-PAUL
发明人： HAAN RENE JOHAN , LANGE JEAN-PAUL
IPC分类号： C07C51/377 , C07C53/126 , C07C67/31
CPC分类号： C07C51/377 , C07C67/03 , C07D307/33 , Y02P20/127 , C07C59/01 , C07C69/533
摘要： A process for preparing a hydroxyacid or hydroxyester from a reactant selected from (a) a carboxylic acid having an aldehyde or keto group; and (b) an ester of a carboxylic acid having an aldehyde or keto group; by contacting the reactant with a metal catalyst in the presence of hydrogen, wherein the metal catalyst is supported on a titanium dioxide or zirconium dioxide support.
摘要翻译：从选自（a）具有醛或酮基的羧酸的反应物制备羟基酸或羟基酯的方法; 和（b）具有醛或酮基的羧酸酯; 通过在氢的存在下使反应物与金属催化剂接触，其中金属催化剂负载在二氧化钛或二氧化锆载体上。

4. 发明申请

WO2011015385A1 PROCESS FOR PREPARING AN ESTER 审中-公开
标题翻译：制备ESTER的方法
公开(公告)号：WO2011015385A1
公开(公告)日：2011-02-10
申请号：PCT/EP2010/055862
申请日：2010-04-29
申请人： SHELL INTERNATIONALE RESEARCH MAATSCHAPPIJ B.V. , HAAN, Rene, Johan , LANGE, Jean-Paul
发明人： HAAN, Rene, Johan , LANGE, Jean-Paul
IPC分类号： C07C67/08
CPC分类号： C07C67/08 , C07C67/00 , C07C69/24
摘要： A process for preparing an ester of formula (I): R 3 CH 2 - (CR 1 R 2 ) n -CH 2 -O-CO-(CR 1 R 2 ) n -CH 2 R 3 (I) wherein n is 1-3 and R 1 and R 2 are each, independently, a hydrogen atom or a carbon-linked organic group and R 3 is a carbon-linked organic group, by hydrogenation of a reactant selected from: (a) a lactone of formula (II) wherein n is 1-3 and R 1 and R 2 are each, independently, a hydrogen atom or a carbon-linked organic group and R 3 is a carbon-linked organic group; (b) an ester of a carboxylic acid of formula (III) R 4 -O-CO- (CR 1 R 2 ) n -CO-R 3 (III) wherein n is 1-3 and R 1 and R 2 are each, independently, a hydrogen atom or a carbon-linked organic group and R 3 and R 4 are a carbon-linked organic group; and c) a carboxylic acid of formula (IV) H-O-CO- (CR 1 R 2 ) n -CO-R 3 (IV) wherein n is 1-3 and R 1 and R 2 are each, independently, a hydrogen atom or a carbon-linked organic group and R 3 is a carbon-linked organic group; which process involves contacting the reactant with a heterogeneous catalyst comprising a hydrogenating metal in the presence of hydrogen, wherein the catalyst is a zeolite-free heterogeneous catalyst comprising a hydrogenating metal supported on a metal oxide or a mixed oxide.
摘要翻译：制备式（I）的酯的方法：R 3 -CH 2 - （CR 1 R 2）n -CH 2 -O-CO-（CR 1 R 2）n -CH 2 R 3（I）其中n为1-3，并且R 1和R 2各自独立地为氢原子或碳连接的有机基团，并且R 3是碳连接的有机基团，通过氢化选自以下的反应物：（a）式（II）的内酯，其中n为1-3且R 1和R 2各自为氢，独立地是氢原子或碳连接的有机基团，并且R 3是碳连接的有机基团; （b）式（III）的羧酸R 4 -O-CO-（CR 1 R 2）n -CO-R 3（III）的酯，其中n为1-3，并且R 1和R 2各自独立地为氢原子或碳键的有机基团，R 3和R 4为碳键的有机基团; 和c）式（Ⅳ）HO-CO-（CR1R2）n-CO-R3（Ⅳ）的羧酸，其中n为1-3，R 1和R 2各自独立地为氢原子或碳键连接的有机基团和R 3是碳键的有机基团; 该方法包括在氢气存在下使反应物与包含氢化金属的多相催化剂接触，其中所述催化剂是不含沸石的多相催化剂，其包含负载在金属氧化物上的氢化金属或混合氧化物。

5. 发明申请

WO2009077606A3 GASOLINE COMPOSITION AND PROCESS FOR THE PREPARATION OF ALKYLFURFURYL ETHER 审中-公开
标题翻译：汽油组合物和制备碱金属氧化物的方法
公开(公告)号：WO2009077606A3
公开(公告)日：2009-10-08
申请号：PCT/EP2008067937
申请日：2008-12-18
申请人： SHELL INT RESEARCH , HAAN RENE JOHAN , LANGE JEAN-PAUL
发明人： HAAN RENE JOHAN , LANGE JEAN-PAUL
IPC分类号： C10L1/02 , C07D307/42 , C10L1/18
CPC分类号： C10L1/023 , C10L1/14 , C10L1/1824 , C10L1/1855 , C10L1/19 , C10L10/10
摘要： The invention provides a gasoline composition comprising in the range of from 0.1 to 30 wt% alkylfurfuryl ether with an alkyl group having 1 to 4 carbon atoms. The invention further provides a process for the preparation of a gasoline composition comprising blending the alkylfurfuryl ether in a gasoline base fuel, and a process for the preparation of an alkylfurfuryl ether wherein an alkyl alcohol having in the range of 1 to 4 carbon atoms is reacted with furfuryl alcohol by contacting a liquid phase comprising the alkyl alcohol and furfuryl alcohol with an acidic zeolite catalyst at a temperature in the range of from 50 to 200 °C.
摘要翻译：本发明提供一种汽油组合物，其含有0.1至30重量％的烷基糠醚与具有1至4个碳原子的烷基。本发明还提供一种制备汽油组合物的方法，其包括将烷基糠醚混合在汽油基燃料中，以及制备烷基糠基醚的方法，其中具有1至4个碳原子的烷基醇反应与糠醇通过使包含烷基醇和糠醇的液相与酸性沸石催化剂在50至200℃的温度下接触。

6. 发明申请

WO2009077606A2 GASOLINE COMPOSITION AND PROCESS FOR THE PREPARATION OF ALKYLFURFURYL ETHER 审中-公开
标题翻译：汽油组合物和制备烷基糠醇醚的方法
公开(公告)号：WO2009077606A2
公开(公告)日：2009-06-25
申请号：PCT/EP2008/067937
申请日：2008-12-18
申请人： SHELL INTERNATIONALE RESEARCH MAATSCHAPPIJ B.V. , HAAN, Rene Johan , LANGE, Jean-Paul
发明人： HAAN, Rene Johan , LANGE, Jean-Paul
IPC分类号： C10L1/02 , C10L1/18 , C07D307/42
CPC分类号： C10L1/023 , C10L1/14 , C10L1/1824 , C10L1/1855 , C10L1/19 , C10L10/10
摘要： The invention provides a gasoline composition comprising in the range of from 0.1 to 30 wt% alkylfurfuryl ether with an alkyl group having 1 to 4 carbon atoms. The invention further provides a process for the preparation of a gasoline composition comprising blending the alkylfurfuryl ether in a gasoline base fuel, and a process for the preparation of an alkylfurfuryl ether wherein an alkyl alcohol having in the range of 1 to 4 carbon atoms is reacted with furfuryl alcohol by contacting a liquid phase comprising the alkyl alcohol and furfuryl alcohol with an acidic zeolite catalyst at a temperature in the range of from 50 to 200 °C.
摘要翻译：本发明提供了一种汽油组合物，其包含0.1-30重量％的具有1-4个碳原子的烷基的烷基糠基醚。本发明进一步提供了一种制备汽油组合物的方法，该方法包括将烷基糠基醚在汽油基础燃料中混合，以及制备烷基糠基醚的方法，其中使具有1至4个碳原子的烷基醇反应与糠醇接触，其中包含烷基醇和糠醇的液相与酸性沸石催化剂在50-200℃的温度下接触。

7. 发明申请

WO2011015645A2 PROCESS FOR PREPARING A HYDROXYACID OR HYDROXYESTER 审中-公开
标题翻译：制备羟基酸或羟基酯的方法
公开(公告)号：WO2011015645A2
公开(公告)日：2011-02-10
申请号：PCT/EP2010/061461
申请日：2010-08-06
申请人： SHELL INTERNATIONALE RESEARCH MAATSCHAPPIJ B.V. , HAAN, Rene, Johan , LANGE, Jean-Paul
发明人： HAAN, Rene, Johan , LANGE, Jean-Paul
IPC分类号： C07C51/377 , C07D307/33 , C07C59/01
CPC分类号： C07C51/377 , C07C67/03 , C07D307/33 , Y02P20/127 , C07C59/01 , C07C69/533
摘要： A process for preparing a hydroxyacid or hydroxyester from a reactant selected from (a) a carboxylic acid having an aldehyde or keto group; and (b) an ester of a carboxylic acid having an aldehyde or keto group; by contacting the reactant with a metal catalyst in the presence of hydrogen, wherein the metal catalyst is supported on a titanium dioxide or zirconium dioxide support.
摘要翻译：从选自以下的反应物制备羟基酸或羟基酯的方法：（a）具有醛或酮基的羧酸; 和（b）具有醛或酮基的羧酸的酯; 通过在氢存在下使反应物与金属催化剂接触，其中金属催化剂负载在二氧化钛或二氧化锆载体上。

8. 发明申请

WO2005058793A1 A PROCESS FOR THE PREPARATION OF AN ALKYL ALKENOATE 审中-公开
标题翻译：一种制备阿尔卡尼酸酯的方法
公开(公告)号：WO2005058793A1
公开(公告)日：2005-06-30
申请号：PCT/EP2004/053536
申请日：2004-12-16
申请人： SHELL INTERNATIONALE RESEARCH MAATSCHAPPIJ B.V. , HAAN, Rene Johan , LANGE, Jean-Paul
发明人： HAAN, Rene Johan , LANGE, Jean-Paul
IPC分类号： C07C67/327
CPC分类号： C07C67/03 , C07C69/533
摘要： A process for the preparation of an alkyl alkenoate, wherein a lactone of the general molecular formula (I) wherein n is 1, 2 or 3, R 1 is a C 1 -C 4 alkyl group, and R 2 , R 3 and R 4 are, independently, a H atom or a C 1 -C 4 alkyl group, is reacted with a C 1 -C 4 alkyl alcohol in a liquid phase in the presence of a strong acid catalyst at transesterification conditions to form the alkyl alkenoate, wherein alkyl alkenoate and alcohol are continuously removed from the liquid phase by distillation.
摘要翻译：一种制备烷基链烯酸酯的方法，其中通式（I）的内酯，其中n为1,2或3，R 1为C 1 -C 4烷基，R 2，R 3和R 4独立地为在强酸催化剂的存在下，在酯交换反应条件下，将H原子或C1-C4烷基与C1-C4烷基醇反应，形成烷基链烯酸酯，其中烷基链烯酸酯和醇从液相通过蒸馏。

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