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1. 发明申请

WO2004101575A2 IMPLEMENTATION OF A STRATEGY FOR ACHIEVING EXTRAORDINARY LEVELS OF SURFACE AND POROSITY IN CRYSTALS 审中-公开
标题翻译：实现水晶表面和孔隙特征水平的策略
公开(公告)号：WO2004101575A2
公开(公告)日：2004-11-25
申请号：PCT/US2004/014465
申请日：2004-05-07
申请人： THE REGENTS OF THE UNIVERSITY OF MICHIGAN , YAGHI, Omar, M. , MATZGER, Adam, J. , ROWSELL, Jesse
发明人： YAGHI, Omar, M. , MATZGER, Adam, J. , ROWSELL, Jesse
IPC分类号： C07F3/00
CPC分类号： F17C11/005 , B01J20/22 , B01J20/226 , C07F3/003 , Y02E60/321
摘要： The present invention provides a metal-organic framework ("MOF”) comprising a plurality of metal clusters and a plurality of multidentate, linking ligands. Each metal of the plurality of metal clusters comprises one or more metal ions. Each ligand of the plurality of multidentate linking ligands connects adjacent metal clusters. The present invention also provides a method of forming the metalorganic framework. The method of the invention comprises combining a solution comprising one or metal ions with a multidentate linking ligand having a sufficient number of accessible sites for atomic or molecular adsorption that the surface area of the resulting metal-organic framework is greater than 2,900 M 2 /g.
摘要翻译：本发明提供了包含多个金属簇和多个多齿连接配体的金属 - 有机骨架（“MOF”）。多个金属簇中的每个金属包括一种或多种金属离子。多个多齿连接配体的每个配体连接相邻的金属簇。本发明还提供了形成金属有机骨架的方法。本发明的方法包括将包含一种或多种金属离子的溶液与具有足够数量的用于原子或分子吸附的可接近位点的多齿连接配体组合，使得所得金属 - 有机骨架的表面积大于2900M 2 /G。

2. 发明申请

WO2007101241A2 PREPARATION OF FUNCTIONALIZED ZEOLITIC FRAMEWORKS 审中-公开
标题翻译：功能化的ZEOLIIC框架的制备
公开(公告)号：WO2007101241A2
公开(公告)日：2007-09-07
申请号：PCT/US2007/062955
申请日：2007-02-28
申请人： THE REGENTS OF THE UNIVERSITY OF MICHIGAN , THE REGENTS OF THE UNIVERSITY OF CALIFORNIA , YAGHI, Omar, M. , HAYASHI, Hideki , BANERJEE, Rahul , PARK, Kyo, Sung , WANG, Bo , COTE, Adrien
发明人： YAGHI, Omar, M. , HAYASHI, Hideki , BANERJEE, Rahul , PARK, Kyo, Sung , WANG, Bo , COTE, Adrien
CPC分类号： B01J20/226 , B01J20/30 , B01J31/1691 , B01J31/1815 , B01J31/183 , B01J2531/0216 , B01J2531/26 , B01J2531/33 , B01J2531/845 , C01B39/00 , C01B39/02 , C07F3/00 , C07F3/003 , C07F3/06 , C07F15/00 , C07F15/065 , C07F19/005 , F17C11/005 , Y02C10/08
摘要： The disclosure provides zeolitic frameworks for gas separation, gas storage, catalysis and sensors. More particularly the disclosure provides zeolitic frameworks (ZIFs) The ZIF of the disclosure comprises any number of transition metals or a homogenous transition metal composition.
摘要翻译：本公开提供了用于气体分离，气体储存，催化和传感器的沸石框架。更具体地说，本公开提供了沸石骨架（ZIF）。本公开的ZIF包含任何数量的过渡金属或均匀的过渡金属组合物。

3. 发明申请

WO2007038508A2 METAL-ORGANIC FRAMEWORKS WITH EXCEPTIONALLY HIGH CAPACITY FOR STORAGE OF CARBON DIOXIDE AT ROOM-TEMPERATURE 审中-公开
标题翻译：金属有机框架具有极高的储存二氧化碳在室温下的高容量
公开(公告)号：WO2007038508A2
公开(公告)日：2007-04-05
申请号：PCT/US2006/037472
申请日：2006-09-26
申请人： THE REGENTS OF THE UNIVERSITY OF MICHIGAN , YAGHI, Omar, M.
发明人： YAGHI, Omar, M.
IPC分类号： B01D53/02
CPC分类号： B01D53/02 , B01D53/04 , B01D53/92 , B01D2253/20 , B01D2253/204 , B01D2253/306 , B01D2257/504 , B01D2258/01 , B01D2259/4525 , B01D2259/4566 , B01J20/226 , F01N3/0807 , F01N3/0857 , F17C11/00 , F17C2221/013 , F17C2227/0302 , F17C2227/0383 , Y02C10/08 , Y02T10/20 , Y10S95/903
摘要： A carbon dioxide storage system includes a container and a conduit attached to the container for introducing or removing a carbon dioxide-containing composition from the container. A carbon dioxide storage material is positioned within the container. The carbon dioxide-storage material includes a metal-organic framework, which has a sufficient surface area to store at least (10) carbon dioxide molecules per formula unit of the metal-organic framework at a temperature of about 25° C.
摘要翻译：二氧化碳储存系统包括容器和连接到容器的导管，用于从容器中引入或除去含二氧化碳的组合物。二氧化碳储存材料位于容器内。二氧化碳储存材料包括金属 - 有机骨架，其具有足够的表面积以在约25℃的温度下存储至少（10）个二氧化碳分子，每个金属 - 有机骨架的每个配方单位。

4. 发明申请

WO2006028479A1 METAL-ORGANIC POLYHEDRA 审中-公开
标题翻译：金属有机聚合物
公开(公告)号：WO2006028479A1
公开(公告)日：2006-03-16
申请号：PCT/US2004/040658
申请日：2004-12-03
申请人： THE REGENTS OF THE UNIVERSITY OF MICHIGAN , YAGHI, Omar, M. , SUDIK, Andrea, C
发明人： YAGHI, Omar, M. , SUDIK, Andrea, C
IPC分类号： C07F15/02
CPC分类号： C07F15/025
摘要： The present invention provides porous metal-organic polyhedra. The porous metal-organic polyhedra of the present invention comprises a plurality of metal clusters each of which have two or more metal ions, and a sufficient number of capping ligands to inhibit polymerization of the metal organic polyhedra. The porous metal-organic polyhedra further includes a plurality of multidentate linking ligands that connect adjacent metal clusters into a geometrical shape describable as a polyhedral with metal clusters positioned at one or more vertices of the polyhedron. The present invention also provides a method of making the porous metal-organic polyhedra in which a solution comprising a solvent, one or more ions, and a counterions that complexes to the porous metal-organic polyhedra as a capping ligand to inhibit polymerization of the metal organic polyhedra, with a multidentate linking ligand.
摘要翻译：本发明提供多孔金属有机多面体。本发明的多孔金属有机多面体包含多个金属簇，每个金属簇具有两个或更多个金属离子，以及足够数量的封端配体以抑制金属有机多面体的聚合。多孔金属 - 有机多面体还包括多个多齿连接配体，其将相邻金属簇连接成可描述为多面体的几何形状，其中金属簇位于多面体的一个或多个顶点。本发明还提供一种制备多孔金属 - 有机多面体的方法，其中包含溶剂，一种或多种离子和与作为封端配体的多孔金属有机多面体复合的抗衡离子的溶液以抑制金属的聚合有机多面体，具有多齿连接配体。

5. 发明申请

WO2005003622A1 NON CYLINDRICAL GAS STORAGE TANK USING ADSORDENT COMPRISING BIDENTATE ORGANIC COMPUND 审中-公开
标题翻译：非圆形气罐储存罐使用包含有机有机电脑
公开(公告)号：WO2005003622A1
公开(公告)日：2005-01-13
申请号：PCT/EP2004/007097
申请日：2004-06-30
申请人： BASF AKTIENGESELLSCHAFT , THE REGENTS OF THE UNIVERSITY OF MICHIGAN
发明人： MÜLLER, Ulrich , HESSE, Michael , HESS, Reinhard , SENK, Rainer , HÖLZLE, Markus , YAGHI, Omar, M.
IPC分类号： F17C11/00
CPC分类号： H01M8/04216 , B01J20/226 , C01B3/0015 , F17C11/005 , F17C2221/033 , F17C2223/035 , F17C2223/036 , F17C2270/0763 , H01M8/04208 , Y02C10/08 , Y02E60/321 , Y02E60/327 , Y02E60/328 , Y10S502/526
摘要： The present invention relates to a container such as a container having non-cylindrical geometry, for uptaking, or storing, or releasing, or uptaking and storing, or uptaking and releasing, or storing and releasing, or uptaking, storing and releasing at least one gas, comprising at least one opening for allowing the at least one gas to enter and exit or at least one opening for allowing the at least one gas to enter and at least one opening for allowing the at least one gas to exit said container, and a gas-tight mechanism capable of storing the at least one gas under a pressure of from 1 to 750 bar, especially preferably from 50 to 80 bar, inside the container, said container further comprising a metallo-organic framework material comprising pores and at least one metal ion and at least one at least bidentate organic compound which is bound to said metal ion, as well as to a storage system and a fuel cell comprising said container, and to a method of using said container or said fuel cell for supplying power to power plants, cars, trucks, busses, cell phones, and laptops.
摘要翻译：本发明涉及一种容器，例如具有非圆柱形几何形状的容器，用于吸收或储存或释放，吸收和储存，吸收和释放，或储存和释放或吸收储存和释放至少一个气体，包括用于允许至少一种气体进入和离开的至少一个开口或用于允许至少一种气体进入的至少一个开口和用于允许至少一种气体离开所述容器的至少一个开口，以及一种气密机构，其能够在所述容器内的1至750巴，特别优选50至80巴的压力下储存所述至少一种气体，所述容器还包括金属 - 有机骨架材料，所述金属 - 有机骨架材料至少包含孔一种金属离子和与所述金属离子结合的至少一种至少二齿有机化合物，以及包含所述容器的储存系统和燃料电池，以及使用所述容器或所述燃料的方法为电厂，汽车，卡车，公共汽车，手机和笔记本电脑供电的电池。

6. 发明申请

WO2005068474A1 ORGANOMETALLIC FRAMEWORK MATERIAL, PREPARATION AND USE 审中-公开
标题翻译：有机骨架材料，制备和使用
公开(公告)号：WO2005068474A1
公开(公告)日：2005-07-28
申请号：PCT/EP2005/000271
申请日：2005-01-13
申请人： BASF AKTIENGESELLSCHAFT , THE REGENTS OF THE UNIVERSITY OF MICHIGAN
发明人： MÜLLER, Ulrich , LIPPERT, Gerald , SCHUBERT, Olga , HESSE, Michael , HESS, Reinhard , STOESSER, Michael , YAGHI, Omar, M.
IPC分类号： C07F3/00
CPC分类号： C07F3/003 , B01J20/226
摘要： A process for preparing an organometallic framework material comprising reacting at least one metal salt with at least one at least bidentate compound capable of coordination to the metal ion of said metal salt, in the presence of an aqueous solvent system and at least one base wherein at least one bidentate compound comprises at least carboxy group and at least one further group which is not a carboxy group and which is capable of forming a hydrogen bridge linkage.
摘要翻译：一种制备有机金属骨架材料的方法，包括使至少一种金属盐与至少一种能够与所述金属盐的金属离子配位的至少二齿化合物在水性溶剂体系和至少一种碱的存在下反应，其中在至少一个二齿化合物至少包含羧基和至少一个不是羧基并且能够形成氢桥键的另外的基团。

7. 发明申请

WO2005003069A2 PROCESS FOR THE ALKOXYLATION OF MONOOLS IN THE PRESENCE OF METALLO-ORGANIC FRAMEWORK MATERIALS 审中-公开
标题翻译：金属有机骨架材料存在下单体烷基化的方法
公开(公告)号：WO2005003069A2
公开(公告)日：2005-01-13
申请号：PCT/EP2004/007143
申请日：2004-07-01
申请人： BASF AKTIENGESELLSCHAFT , THE REGENTS OF THE UNIVERSITY OF MICHIGAN
发明人： MÜLLER, Ulrich , METELKINA, Olga , HESSE, Michael , STÖßER, Michael , HAAS, Peter , YAGHI, Omar, M.
IPC分类号： C07C41/03
CPC分类号： C08G65/2606 , C07C41/03 , C08G18/283 , C08G65/2645 , C08G65/266 , C08G2101/00 , C07C43/11
摘要： The present invention relates to a process for the alkoxylation of a monool with at least one alkoxylating agent to an alkoxylated alcohol wherein a catalyst is employed which comprises a metallo-organic framework material of metal ions and at least bidentate coordinately bound organic ligands.
摘要翻译：本发明涉及使用至少一种烷氧基化剂将烷氧基化为烷氧基化醇的方法，其中使用包含金属离子的金属有机骨架材料和至少二齿配位结合的有机配体的催化剂。

8. 发明申请

WO2006050898A1 SHAPED BODIES CONTAINING METAL-ORGANIC FRAMEWORKS 审中-公开
标题翻译：包含金属有机框架的形状体
公开(公告)号：WO2006050898A1
公开(公告)日：2006-05-18
申请号：PCT/EP2005/011918
申请日：2005-11-08
申请人： BASF AKTIENGESELLSCHAFT , THE REGENTS OF THE UNIVERSITY OF MICHIGAN
发明人： HESSE, Michael , MÜLLER, Ulrich , YAGHI, Omar, M.
IPC分类号： B01J31/00 , C01B3/00 , F17C11/00
CPC分类号： F17C11/005 , B01J20/0244 , B01J20/226 , B01J20/28011 , B01J20/2803 , B01J20/28042 , B01J20/28057 , B01J20/3007 , B01J20/3035 , B01J20/3042 , B01J31/1691 , B01J35/1028 , B01J37/0009 , B01J2231/005 , B01J2531/26 , Y02E60/324 , Y10T428/249953 , Y10T428/249967 , Y10T428/24997 , Y10T428/25 , Y10T428/298
摘要： The present invention relates to shaped bodies containing a metal-organic framework material (MOF) as well as a process for the preparation thereof and their use especially as catalyst or storage medium.
摘要翻译：本发明涉及含有金属 - 有机骨架材料（MOF）的成型体以及其制备方法及其特别用作催化剂或储存介质的用途。

9. 发明申请

WO2004037895A1 PROCESS FOR PRODUCING POLYALKYLENE CARBONATES 审中-公开
标题翻译：生产聚亚烷基碳酸酯的方法
公开(公告)号：WO2004037895A1
公开(公告)日：2004-05-06
申请号：PCT/EP2003/011704
申请日：2003-10-22
申请人： BASF AKTIENGESELLSCHAFT , THE REGENTS OF THE UNIVERSITY OF MICHIGAN
发明人： MÜLLER, Ulrich , LUINSTRA, Gerrit , YAGHI, Omar, M. , METELKINA, Olga , STÖßER, Michael
IPC分类号： C08G64/34
CPC分类号： B01J31/1691 , B01J31/2239 , B01J2231/14 , B01J2531/16 , B01J2531/22 , B01J2531/26 , B01J2531/27 , B01J2531/38 , B01J2531/44 , B01J2531/72 , B01J2531/842 , B01J2531/845 , B01J2531/847 , C08G64/34
摘要： The present invention relates to a process for the preparation of polyalkylene carbonate, an alternating copolymer, obtainable from the ring opening of an alkene oxide or an alkene oxide precursor in the presence of carbon dioxide or any substance delivering carbon oxide, in the presence of at least one catalyst containing a metal-organic framework material, wherein said framework material comprises pores and a metal ion and an at least bidentate organic compound, said bidentate organic compound being coordinately bound to the metal ion.
摘要翻译：本发明涉及一种制备聚亚烷基碳酸酯的方法，一种交替共聚物，可在二氧化碳或任何物质输送碳氧化物的存在下，由烯烃氧化物或氧化烯前体的开环在有至少一种含有金属 - 有机骨架材料的催化剂，其中所述骨架材料包含孔和金属离子和至少二齿有机化合物，所述二齿有机化合物与金属离子配位结合。

10. 发明申请

WO2002088148A1 ISORETICULAR METAL-ORGANIC FRAMEWORKS, PROCESS FOR FORMING THE SAME, AND SYSTEMATIC DESIGN OF PORE SIZE AND FUNCTIONALITY THEREIN,WITH APPLICATION FOR GAS STORAGE 审中-公开
标题翻译：相关金属有机框架，其形成方法以及孔径尺寸和功能的系统设计，适用于气体存储
公开(公告)号：WO2002088148A1
公开(公告)日：2002-11-07
申请号：PCT/US2002/013763
申请日：2002-04-29
申请人： THE REGENTS OF THE UNIVERSITY OF MICHIGAN
发明人： YAGHI, Omar, M. , EDDAOUDI, Mohamed , LI, Hailian , KIM, Jaheon , ROSI, Nathaniel
IPC分类号： C07F3/00
CPC分类号： B01J20/2808 , B01J20/226 , B01J20/28011 , B01J20/28014 , B01J20/28069 , B01J20/28078 , B01J20/30 , B01J31/1691 , B01J2531/26 , C07F3/003 , F17C11/007 , Y02C10/08
摘要： The ability to design and construct solid-state materials with pre-determined structures is a grand challenge in chemistry. An inventive strategy based on reticulating metal ions and organic carboxylate links into extended networks has been advanced to a point that allows the design of porous structures in which pore size and functionality can be varied systematically. MOF-5, a prototype of a new class of porous materials and one that is constructed from octahedral Zn-O-C clusters and benzene links, was used to demonstrate that its 3-D porous system can be functionalized with the organic groups, -Br, -NH2, -OC 3 H 7 , -OC 5 H 11 , -H 4 C 2 and -H 4 C 4 , and its pore size expanded with the long molecular struts biphenyl, tetrahydropyrene, pyrene, and terphenyl. The ability to direct the formation of the octahedral clusters in the presence of a desired carboxylate link is an essential feature of this strategy, which resulted in the design of an isoreticular (having the same framework topology) series of sixteen well-defined materials whose crystals have open space representing up to 91.1% of the crystal volume, and homogeneous periodic pores that can be incrementally varied from 3.8 to 28.8 angstroms. Unlike the unpredictable nature of zeolite and other molecular sieve syntheses, the deliberate control exercised at the molecular level in the design of these crystals is expected to have tremendous implications on materials properties and future technologies. Indeed, data indicate that members of this series represent the first monocrystalline mesoporous organic/inorganic frameworks, and exhibit the highest capacity for methane storage (155 cm 3 /cm 3 at 36 atm) and the lowest densities (0.41 to 0.21 g/cm 3 ) attained to date for any crystalline material at room temperature.
摘要翻译：使用预定结构设计和构建固态材料的能力是化学领域的一大挑战。基于将金属离子和有机羧酸盐连接网络化成扩展网络的创新策略已经进展到允许孔径和功能性可以系统地变化的多孔结构的设计。 MOF-5是一种新型多孔材料的原型，由八面体Zn-OC簇和苯环构成的原型，用于证明其3-D多孔体系可以用有机基团-Br， -NH2，-OC3H7，-OC5H11，-H4C2和-H4C4，其孔径用长分子支链联苯，四氢苯乙烯，芘和三联苯扩展。在存在所需的羧酸酯键的情况下引导形成八面体簇的能力是该策略的基本特征，其导致设计了十六种明确定义的材料的晶体（具有相同的框架拓扑）系列，其晶体具有高达91.1％晶体体积的开放空间，并且均匀的周期性孔隙可以逐渐变化，从3.8到28.8埃。与沸石和其他分子筛合成的不可预知的性质不同，在分子水平上对这些晶体的设计进行有意的控制预计对材料性能和未来技术有巨大的影响。事实上，数据表明，这一系列的成员代表了第一个单晶介孔有机/无机骨架，并且表现出最高的甲烷储存能力（36 atm时为155 cm 3 / cm 3），最低密度为0.41〜0.21 g / cm 3）在室温下达到任何结晶物质。

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