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1. 发明申请

WO2018098455A2 PRECURSORS FOR DEPOSITION OF METAL, METAL NITRIDE AND METAL OXIDE BASED FILMS OF TRANSITION METALS 审中-公开
公开(公告)号：WO2018098455A2
公开(公告)日：2018-05-31
申请号：PCT/US2017/063355
申请日：2017-11-28
申请人： APPLIED MATERIALS, INC.
发明人： SCHMIEGE, Benjamin , ANTHIS, Jeffrey, W. , THOMPSON, David
IPC分类号： C07F5/00 , C23C16/18 , C23C16/455 , C23C16/34 , C23C16/40
CPC分类号： C07F15/045 , C07F5/00 , C07F15/025 , C07F15/06
摘要： Metal coordination complexes comprising a metal atom coordinated to at least one aza-allyl ligand having the structure represented by (1) where each R1 -R4 are independently selected from the group consisting of H, branched or unbranched C1 -C6 alkyl, branched or unbranched C1 -C6 alkenyl, branched or unbranched C1 -C6 alkynyl, cycloalkyl groups having in the range of 1 to 6 carbon atoms, silyl groups and halogens. Methods of depositing a film using the metal coordination complex and a suitable reactant are also described.

2. 发明申请

WO2017173362A1 SELECTIVE, ADSORBATE-INDUCED SPIN STATE CHANGES IN TRANSITION METAL-BASED METAL-ORGANIC FRAMEWORKS 审中-公开
标题翻译：过渡金属基有机骨架中选择性，吸附剂诱导的自旋态变化
公开(公告)号：WO2017173362A1
公开(公告)日：2017-10-05
申请号：PCT/US2017/025541
申请日：2017-03-31
申请人： THE REGENTS OF THE UNIVERSITY OF CALIFORNIA
发明人： LONG JR., Jeffrey R. , KEITZ, Benjamin K. , REED, Douglas
IPC分类号： C07F15/02 , B01J20/22
CPC分类号： B01J20/226 , B01D53/02 , B01D53/04 , B01D2253/204 , B01D2256/10 , B01D2256/16 , B01D2256/22 , B01D2256/24 , B01D2256/245 , B01D2257/102 , B01D2257/104 , B01D2257/502 , B01J20/28066 , B01J20/3425 , B01J20/3483 , B01J20/3491 , C01B3/56 , C01B32/40 , C01B2203/042 , C01B2203/047 , C01B2210/002 , C01B2210/0021 , C07F15/025
摘要： An adsorbate-selective metal organic framework includes a transition metal; and a plurality of organic molecules coordinated to the transition metal so as to preserve open coordination sites for selectively adsorbing molecules that have low-lying π* orbitals. The transition metal has a lowest energy spin state in the presence of the selectively adsorbed molecules that are strongly bonding to the transition metal through π-donating interactions which is different than the lowest energy spin state in the absence of these adsorbed molecules. The transition metal has also a lowest energy spin state in the presence of non-selected molecules that are weakly bonding to the transition metal through σ- and/or π-accepting and/or donating interactions.
摘要翻译：吸附物选择性金属有机骨架包含过渡金属; 和多个与过渡金属配位的有机分子，以保持开放的配位位置，以选择性地吸附具有低位π*轨道的分子。过渡金属在存在选择性吸附的分子时具有最低的能量自旋状态，所述分子通过π-供体相互作用与过渡金属强烈结合，这与不存在这些吸附分子时的最低能量自旋状态不同。过渡金属在存在未选择的分子时也具有最低的能量自旋状态，这些分子通过σ-和/或π-接受和/或捐赠相互作用与过渡金属弱结合。

3. 发明申请

WO2017066070A2 ACETATE COMPLEXES AND METHODS FOR ACETATE QUANTIFICATION 审中-公开
标题翻译：醋酸酯配合物和醋酸酯定量方法
公开(公告)号：WO2017066070A2
公开(公告)日：2017-04-20
申请号：PCT/US2016/055673
申请日：2016-10-06
申请人： GENERAL ELECTRIC COMPANY
发明人： LEACH, Andrew , CHEN, Rui , PALACIOS, Manuel
IPC分类号： C07F15/02 , A61K49/06
CPC分类号： G01N33/15 , C07F15/025 , G01N21/31
摘要： The present invention is directed to methods of acetate quantification and acetate complexes useful in the methods of acetate quantification. Such methods and complexes are useful for any application where acetate quantification is desired, including measuring of concentration of 13 C hyperpolarized acetate for imaging agent quality control in MRI and NMR spectroscopy. The disclosed acetate complexes may be prepared from acetate, Fe 3+ , and sulfosalicylic acid and from acetate, Fe 3+ , and salicylic acid.
摘要翻译：本发明涉及用于乙酸盐定量方法的乙酸盐定量方法和乙酸盐复合物。此类方法和复合物可用于需要进行醋酸盐定量的任何应用，包括测量13 C超极化醋酸盐的浓度以用于MRI和NMR光谱学中的成像剂质量控制。所公开的乙酸盐配合物可以由乙酸盐，Fe 3+和磺基水杨酸以及乙酸盐，Fe 3+和水杨酸来制备。

4. 发明申请

WO2015191505A1 POLYDENTATE LIGANDS AND THEIR COMPLEXES FOR MOLECULAR CATALYSIS 审中-公开
标题翻译：聚异氰酸酯配体及其用于分子催化的复合物
公开(公告)号：WO2015191505A1
公开(公告)日：2015-12-17
申请号：PCT/US2015/034793
申请日：2015-06-09
申请人： LOS ALAMOS NATIONAL SECURITY, LLC
发明人： DUB, Pavel, A. , GORDON, John, Cameron
IPC分类号： C07F15/00
CPC分类号： C07F15/025 , C07C323/25 , C07D295/13 , C07D333/20 , C07F1/08 , C07F9/5022 , C07F9/5027 , C07F9/5325 , C07F9/5329 , C07F9/655345 , C07F13/005 , C07F15/004 , C07F15/0053 , C07F15/045 , C07F15/065
摘要： The present invention relates generally to novel achiral and chiral sulfur-, nitrogen- and phosphorus-containing ligands, designated as NNS-type, P(0)NS-type, PNS-type, SNNS-type, SNNP(0)-type, or SNNP-type polydentate ligands and transition metal complexes of these ligands. The catalysts derived from these ligands and transition metal complexes may be used in a wide range of catalytic reactions, including hydrogenation and transfer hydrogenation of unsaturated organic compounds, dehydrogenation of alcohols and boranes, various dehydrogenative couplings, and other catalytic transformations.
摘要翻译：本发明一般涉及新型非手性和手性含硫，氮和磷的配体，称为NNS型，P（0）NS型，PNS型，SNNS型，SNNP（0）型，或SNNP型多齿配体和这些配体的过渡金属络合物。衍生自这些配体和过渡金属配合物的催化剂可用于广泛的催化反应，包括不饱和有机化合物的氢化和转移氢化，醇和硼烷的脱氢，各种脱氢偶联和其它催化转化。

5. 发明申请

WO2015177511A1 METHOD OF PREPARING A METAL ORGANIC FRAMEWORK 审中-公开
标题翻译：制备金属有机框架的方法
公开(公告)号：WO2015177511A1
公开(公告)日：2015-11-26
申请号：PCT/GB2015/051383
申请日：2015-05-11
申请人： THE TEXAS A&M UNIVERSITY SYSTEM , JASON, Ornstein
发明人： ZHOU, Hong-Cai , FENG, Dawei , WANG, Kecheng , TIAN, Jian
IPC分类号： C07F15/02 , C07D487/22 , C07F7/00 , C07F7/08 , C07C51/41 , C07C63/307
CPC分类号： C07F7/0818 , C07D487/22 , C07F7/006 , C07F15/025
摘要： The present invention relates to a method of preparing a metal organic framework comprising metal ions and carboxylate ligands; the method comprises: reacting (i) a source of metal ions, with (ii) a carboxylic acid precursor of a the carboxylate ligands, in an organic solvent consisting of one or more carboxylic acid solvents, at a temperature of about 75°C or greater, optionally in the presence of water. The present invention also relates to the same method for preparing monocrystalline metal organic frameworks as well as the metal organic frameworks obtained from such methods.
摘要翻译：本发明涉及一种制备包含金属离子和羧酸盐配体的金属有机骨架的方法; 该方法包括：（i）金属离子源与（ii）羧酸酯配体的羧酸前体在由一种或多种羧酸溶剂组成的有机溶剂中，在约75℃的温度或更大，任选地在水的存在下。本发明还涉及制备单晶金属有机骨架的相同方法以及由这些方法获得的金属有机骨架。

6. 发明申请

WO2015169763A1 PORPHYRIN MOLECULAR CATALYSTS FOR SELECTIVE ELECTROCHEMICAL REDUCTION OF CO2 INTO CO 审中-公开
标题翻译：用于选择性电化学还原二氧化碳的聚吡咯分子催化剂
公开(公告)号：WO2015169763A1
公开(公告)日：2015-11-12
申请号：PCT/EP2015/059746
申请日：2015-05-04
申请人： CENTRE NATIONAL DE LA RECHERCHE SCIENTIFIQUE (CNRS) , UNIVERSITE PARIS DIDEROT PARIS 7
发明人： COSTENTIN, Cyrille , ROBERT, Marc , DROUET, Samuel , PASSARD, Guillaume , SAVEANT, Jean-Michel , TATIN, Arnaud
IPC分类号： C07F15/02 , C07D487/22 , C25B3/04
CPC分类号： C25B1/00 , C01B32/40 , C07D487/22 , C07F15/025 , C25B9/00 , C25B11/12
摘要： The present invention relates to porphyrins of formula (I): wherein R 1 to R 6 , R 1' to R 6' , X, X' Y and Y' are as described in claim 1. The invention also relates to complexes of said porphyrins with transition metals, in particular iron, preferably as Fe(III) or Fe(0) complex, and salts thereof, use thereof as catalysts for the selective electrochemical reduction of CO 2 into CO, electrochemical cells comprising said complexes, and a method for selectively reducing electrochemically CO 2 into CO using said complexes.
摘要翻译：本发明涉及式（I）的卟啉：其中R 1至R 6，R 1'至R 6'，X，X'Y和Y'如权利要求1所述。本发明还涉及所述卟啉与过渡金属的络合物，特别是铁，优选为Fe（III）或Fe（O）络合物及其盐，其作为用于将CO 2选择性电化还原成CO的催化剂的用途，包含所述络合物的电化学电池以及选择性还原电化学CO 2的方法使用所述复合物进入CO。

7. 发明申请

WO2014028574A3 ADSORPTION SYSTEMS USING METAL-ORGANIC FRAMEWORKS 审中-公开
标题翻译：使用金属有机框架的吸附系统
公开(公告)号：WO2014028574A3
公开(公告)日：2015-05-21
申请号：PCT/US2013054863
申请日：2013-08-14
申请人： ARKEMA INC , BATTELLE MEMORIAL INSTITUTE
发明人： VAN HORN BRETT L , BERTELO CHRISTOPHER A , SILVERMAN GARY S , MCGRAIL B PETER , THALLAPALLY PRAVEEN K , MOTKURI RADHA K , JENKS JEROMY J
IPC分类号： F25B17/08 , B01D53/02 , C07F3/06
CPC分类号： C09K5/047 , B01D53/02 , B01D2253/204 , B01J20/226 , C01C3/11 , C07C63/28 , C07C63/307 , C07C65/03 , C07F1/005 , C07F3/003 , C07F11/005 , C07F15/025 , C07F15/045 , C07F15/065 , C07F19/005 , F25B15/006 , F25B2315/006
摘要： The present invention relates to sorbants such as metal-organic frameworks (MOFs), covalent organic frameworks (COFs), porous aromatic frameworks (PAFs) or porous polymer networks (PPNs) for separations of gases or liquids, gas storage, cooling, and heating applications, including, but not limited to, adsorption chillers.
摘要翻译：本发明涉及用于气体或液体分离的金属 - 有机骨架（MOF），共价有机骨架（COF），多孔芳族骨架（PAF）或多孔聚合物网络（PPN）等吸附剂，气体储存，冷却和加热应用，包括但不限于吸附式制冷机。

8. 发明申请

WO2015034814A1 ADDITIVE FOR A SILICONE ENCAPSULANT 审中-公开
标题翻译：加入硅胶
公开(公告)号：WO2015034814A1
公开(公告)日：2015-03-12
申请号：PCT/US2014/053672
申请日：2014-09-02
申请人： DOW CORNING CORPORATION
发明人： KLEYER, Donald, L. , SCHMIDT, Randall, G. , TOMASIK, Adam, C. , XU, Shengqing
IPC分类号： C08K5/5419 , C08K9/10
CPC分类号： C08K5/5419 , C07F15/025 , C08K5/5406 , H01L23/296 , H01L2924/0002 , C08L83/04 , H01L2924/00
摘要： An additive for a silicone encapsulant has the structure: Formula (I) wherein R 1 and R 2 are each -O-Si(R 4 )(R 5 )(R 6 ) and each of R 4 , R 5 , and R 6 is independently chosen from C 1 -C 10 hydrocarbyl groups, C 1 -C 10 alkyl groups, C 2 -C 10 alkenyl groups, and C 6 -C 10 aryl groups, and wherein R 3 is independently chosen from C 1 -C 10 hydrocarbyl groups, C 1 -C 10 alkyl groups, C 2 -C 10 alkenyl groups, and C 6 -C 10 aryl groups. The additive is formed using a method that includes the step of reacting iron metal or an iron (III) compound with a hydroxyl functional organosiloxane. An encapsulant includes the additive and a polyorganosiloxane. The encapsulant can be utilized to form a device that includes an electronic component and the encapsulant disposed on the electronic component. The device is formed using a method that includes the step of disposing the encapsulant on the electronic device.
摘要翻译：用于硅酮密封剂的添加剂具有以下结构：式（I）其中R 1和R 2各自为-O-Si（R 4）（R 5）（R 6），并且R 4，R 5和R 6各自独立地选自C 1 -C 10烃基基团，C 1 -C 10烷基，C 2 -C 10烯基和C 6 -C 10芳基，其中R 3独立地选自C 1 -C 10烃基，C 1 -C 10烷基，C 2 -C 10烯基和C 6 -C 10 芳基。使用包括使铁金属或铁（III）化合物与羟基官能的有机硅氧烷反应的步骤的方法形成添加剂。密封剂包括添加剂和聚有机硅氧烷。密封剂可用于形成包括电子部件和设置在电子部件上的密封剂的装置。该装置使用包括将密封剂设置在电子设备上的步骤的方法形成。

9. 发明申请

WO2014209412A1 N-ACETYL L-CYSTEINE CHELATES AND METHODS FOR MAKING AND USING THE SAME 审中-公开
标题翻译： N-乙酰基-L-胞嘧啶及其制备和使用方法
公开(公告)号：WO2014209412A1
公开(公告)日：2014-12-31
申请号：PCT/US2013/053440
申请日：2013-08-02
申请人： VIVA PHARMACEUTICAL, INC. , DANIELS, Rhett Sean
发明人： DANIELS, Rhett Sean , XIE, Xueju
IPC分类号： A01N37/12 , A01N37/44
CPC分类号： A61K31/315 , A23L33/165 , A23L33/175 , A23L33/18 , A23V2002/00 , A61K31/555 , C07F1/08 , C07F3/02 , C07F3/06 , C07F15/025 , A23V2200/30 , A23V2200/322 , A23V2200/324 , A23V2250/156 , A23V2250/1586 , A23V2250/1588 , A23V2250/1592 , A23V2250/1608 , A23V2250/161 , A23V2250/1612 , A23V2250/1626 , A23V2250/1642 , A23V2250/55
摘要： A nutritional supplement for a human, the supplement having a chelate comprised of an N-acetyl-L-cysteine ligand bonded to a metal to form a chelate ring. A method for preparing a chelate comprised of N-acetyl-L-cysteine ligand and a metal having the steps of: dissolving an amount of N-acetyl-L-cysteine in an aqueous solution, adding a metal to the aqueous solution, stirring and heating the aqueous solution, and removing the solvent under reduced pressure. A method of treating a human for one or more of oxidative stress, cardiovascular disease, cerebrovascular disease, neurodegenerative diseases, Alzheimer's disease, ADHD, bipolar, schizophrenia, autism, dementia, and HIV in a human comprising administering an effective amount of a composition having N-acetyl-L-cysteine in a chelate formation with a metal. A compound having a chelate formulation with a metal being chelated by an N-acetyl-L-cysteine ligand.
摘要翻译：一种人的营养补充剂，该补充物具有由与金属键合形成螯合环的N-乙酰基-L-半胱氨酸配体组成的螯合物。一种制备由N-乙酰基-L-半胱氨酸配体和金属组成的螯合物的方法，其步骤为：将一定量的N-乙酰基-L-半胱氨酸溶解在水溶液中，向该水溶液中加入金属，搅拌和加热水溶液，并在减压下除去溶剂。一种治疗人类患有氧化应激，心血管疾病，脑血管疾病，神经变性疾病，阿尔茨海默病，ADHD，双相，精神分裂症，孤独症，痴呆和HIV中的一种或多种的方法，包括给予有效量的具有 N-乙酰基-L-半胱氨酸与金属螯合形成。具有金属被N-乙酰基-L-半胱氨酸配体螯合的螯合剂的化合物。

10. 发明申请

WO2014182681A1 SATURATED AND UNSATURATED SILAHYDROCARBONS VIA IRON AND COBALT PYRIDINE DIIMINE CATALYZED OLEFIN SILYLATION 审中-公开
标题翻译：饱和和不饱和硅烷通过铁和钴吡啶二胺催化烯烃硅烷
公开(公告)号：WO2014182681A1
公开(公告)日：2014-11-13
申请号：PCT/US2014/036942
申请日：2014-05-06
申请人： MOMENTIVE PERFORMANCE MATERIALS INC. , PRINCETON UNIVERSTY
发明人： LEWIS, Kenrick, M. , ATIENZA, Crisita Carmen Hojilla , BOYER, Julie, L. , CHIRIK, Paul, J. , DELIS, Johannes, G.P. , ROY, Aroop, Kumar
IPC分类号： C07F7/08 , C07F15/02 , C07F15/06
CPC分类号： C07F7/0829 , C07F7/0809 , C07F7/0896 , C07F15/02 , C07F15/025 , C07F15/06 , C07F15/065
摘要： The present invention relates to processes for the synthesis of saturated and unsaturated silahydrocarbons using iron-containing or cobalt-containing catalysts. The processes of the invention can produce tetraalkylsilanes, phenyltrialkylsilanes, substituted phenyltrialkylsilanes and their mixtures, which are useful as lubricants and hydraulic fluids, as well as alkyl alkenylsilanes, phenyl alkenylsilanes and substituted phenyl alkenylsilanes and their mixtures, which are useful in the synthesis of saturated silahydrocarbons and other organofunctional silanes.
摘要翻译：本发明涉及使用含铁或含钴催化剂合成饱和和不饱和硅烷烃的方法。本发明的方法可以生产四烷基硅烷，苯基三烷基硅烷，取代的苯基三烷基硅烷及其混合物，其可用作润滑剂和液压流体，以及烷基烯基硅烷，苯基烯基硅烷和取代的苯基烯基硅烷及其混合物，其可用于合成饱和硅烷烃等有机官能硅烷。

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