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1. 发明申请

WO2010084112A1 PROCESS FOR THE HYDRO-DEMETALLIZATION OF HYDROCARBON FEEDSTOCKS 审中-公开
标题翻译：烃类进料水解的方法
公开(公告)号：WO2010084112A1
公开(公告)日：2010-07-29
申请号：PCT/EP2010/050560
申请日：2010-01-19
申请人： SHELL INTERNATIONALE RESEARCH MAATSCHAPPIJ B.V. , DE DEUGD, Ronald Martijn , HERBST, Brendan Michael , HUVE, Laurent Georges , LIN, Wencai
发明人： DE DEUGD, Ronald Martijn , HERBST, Brendan Michael , HUVE, Laurent Georges , LIN, Wencai
IPC分类号： B01J35/02 , C10G45/04 , C10G45/06 , C10G45/08
CPC分类号： B01J35/026 , B01J23/28 , B01J23/85 , B01J27/19 , B01J37/28 , C10G45/04 , C10G45/06 , C10G45/08 , C10G49/002
摘要： A process for the catalytic hydro-demetallization of a hydrocarbon feedstock over a fixed bed of hydro- demetallization catalyst particles, the process comprising contacting the heavy hydrocarbon oil and hydrogen at elevated temperature and elevated pressure with the catalyst particles in the fixed bed, the catalyst particles being extruded catalyst particles of one or more catalytically active metals on a porous carrier, the extruded particles comprising three protrusions each extending from and attached to a central position, wherein the central position is aligned along the longitudinal axis of the particle, the cross-section of the particle occupying the space encompassed by the outer edges of six circles around a central circle, each of the six circles touching two neighbouring circles whilst three alternating circles are equidistant to the central circle and may be attached to the central circle, minus the space occupied by the three remaining outer circles and including the six interstitial regions.
摘要翻译：一种用于在固定床上加氢脱金属催化剂颗粒的烃原料催化加氢脱金属的方法，该方法包括使重烃和氢在高温和高压下与固定床中的催化剂颗粒接触，催化剂颗粒是多孔载体上的一种或多种催化活性金属的挤出催化剂颗粒，所述挤出颗粒包括三个突起，每个突起从中心位置延伸并连接到中心位置，其中中心位置沿着颗粒的纵向轴线排列，占据由围绕中心圆的六个圆的外边缘包围的空间的颗粒的截面，六个圆中的每一个接触两个相邻的圆，而三个交替的圆与中心圆等距，并且可以附着到中心圆，减去其余三个外围占有空间，包括六个间隙区域。

2. 发明申请

WO2005118749A1 A PROCESS FOR DESULPHURISING AND DEWAXING A HYDROCARBON FEEDSTOCK BOILING IN THE GASOIL BOILING RANGE 审中-公开
标题翻译：一种在气体沸腾范围内进行脱硫和脱蜡的方法
公开(公告)号：WO2005118749A1
公开(公告)日：2005-12-15
申请号：PCT/EP2005/052542
申请日：2005-06-02
申请人： SHELL INTERNATIONALE RESEARCH MAATSCHAPPIJ B.V. , HUVE, Laurent Georges
发明人： HUVE, Laurent Georges
IPC分类号： C10G45/62
CPC分类号： C10G45/62 , C10G45/68 , C10G49/002 , C10G65/043 , C10G65/08
摘要： A process for desulphurising and dewaxing a hydrocarbon feedstock boiling in the gasoil boiling range to obtain a desulphurised and dewaxed gasoil fraction for use in an ultra low sulphur diesel fuel, comprising the following steps: (a) hydrodesulphurising the hydrocarbon feedstock boiling in the gasoil boiling range by contacting the feedstock in a hydrodesulphurisation reaction zone at elevated temperature and pressure, in the presence of hydrogen, with a hydrodesulphurisation catalyst and withdrawing a liquid hydrodesulphurisation effluent from the reaction zone; (b) catalytically dewaxing the liquid hydrodesulphurisation effluent to obtain a desulphurised and dewaxed gasoil fraction by contacting the liquid hydrodesulphurisation effluent, at elevated temperature and pressure in the presence of hydrogen, with a stacked bed of catalysts having a first upstream bed of noble metal containing hydrofinishing catalyst and a second downstream bed of noble metal containing dewaxing catalyst, wherein hydrogen and the liquid effluent are countercurrently supplied to the stacked bed of catalysts.
摘要翻译：一种用于在油烟沸点范围内沸腾的烃原料脱硫和脱蜡以获得用于超低硫柴油燃料的脱硫和脱蜡汽油部分的方法，包括以下步骤：（a）将在沸石沸腾沸腾的烃原料加氢脱硫通过在加氢脱硫反应区中在升高的温度和压力下，在氢的存在下与加氢脱硫催化剂接触原料并从反应区抽出液体加氢脱硫流出物; （b）将液体加氢脱硫流出物进行催化脱蜡以获得脱硫和脱蜡的汽油部分，通过在氢存在下，在高温和高压下使液体加氢脱硫流出物与具有第一上游贵金属上游床的层叠床接触，加氢精制催化剂和含贵金属的脱蜡催化剂的第二下游床，其中氢气和液体流出物逆流供应到催化剂层叠床。

3. 发明申请

WO2006032698A1 FAUJASITE ZEOLITE, ITS PREPARATION AND USE IN HYDROCRACKING 审中-公开
标题翻译： FAUJASITE ZEOLITE，其制备和使用在水力发电
公开(公告)号：WO2006032698A1
公开(公告)日：2006-03-30
申请号：PCT/EP2005/054774
申请日：2005-09-23
申请人： SHELL INTERNATIONALE RESEARCH MAATSCHAPPIJ B.V. , CREYGHTON, Edward Julius , HUVE, Laurent Georges , KLAZINGA, Aan Hendrik
发明人： CREYGHTON, Edward Julius , HUVE, Laurent Georges , KLAZINGA, Aan Hendrik
IPC分类号： B01J29/08
CPC分类号： C10G47/20 , B01J29/08 , B01J29/084 , B01J29/166 , B01J35/002 , B01J35/026 , B01J35/1023 , B01J37/0009 , B01J2229/16 , B01J2229/18 , B01J2229/20 , B01J2229/36 , B01J2229/37 , B01J2229/42 , C10G47/02 , C10G47/16
摘要： The invention provides a zeolite of the faujasite structure which has a unit cell size in the range of from 24.40 to 24.50 A; a bulk silica to alumina ratio (SAR) in th range of from 5 to 10; and an alkali metal content of less than 0.15 wt%. Such zeolites have been found to have a very useful naphtha selectivity in hydrocracking, particularly a selectivity to heavy naphtha. A preparation process for the zeolite, hydrocracking catalyst composition comprising the zeolite and its use in hydrocracking are also provided.
摘要翻译：本发明提供了八面沸石结构的沸石，其具有在24.40至24.50A范围内的晶胞尺寸; 体积二氧化硅与氧化铝的比例（SAR）在5至10的范围内; 碱金属含量小于0.15重量％。已经发现这种沸石在加氢裂化中具有非常有用的石脑油选择性，特别是重质石脑油的选择性。还提供了沸石的制备方法，包含沸石的加氢裂化催化剂组合物及其在加氢裂化中的用途。

4. 发明申请

WO2012055759A1 HYDROCARBON CONVERSION CATALYST COMPOSITION 审中-公开
标题翻译：碳氢转化催化剂组合物
公开(公告)号：WO2012055759A1
公开(公告)日：2012-05-03
申请号：PCT/EP2011/068345
申请日：2011-10-20
申请人： SHELL INTERNATIONALE RESEARCH MAATSCHAPPIJ B.V. , DOMOKOS, László , HUVE, Laurent Georges , JONGKIND, Hermanus , KLAZINGA, Aan Hendrik , RIGUTTO, Marcello Stefano
发明人： DOMOKOS, László , HUVE, Laurent Georges , JONGKIND, Hermanus , KLAZINGA, Aan Hendrik , RIGUTTO, Marcello Stefano
IPC分类号： B01J29/70
CPC分类号： B01J29/7446 , B01J23/42 , B01J23/44 , B01J23/755 , B01J29/70 , B01J29/703 , B01J29/7049 , B01J29/708 , B01J29/80 , B01J37/0201 , B01J2229/16 , B01J2229/37 , B01J2229/42 , C10G35/065 , C10G45/64 , C10G49/08 , C10G50/00 , C10G65/12
摘要： A hydrocarbon conversion catalyst composition which comprises ZSM-48 and/or EU-2 zeolite particles and refractory oxide binder essentially free of alumina in which the average aluminium concentration of the ZSM-48 and/or EU-2 zeolite particles is at least 1.3 times the aluminium concentration at the surface of the particles, processes for preparing such catalyst compositions and processes for converting hydrocarbon feedstock with the help of such compositions.
摘要翻译：烃转化催化剂组合物，其包含ZSM-48和/或EU-2沸石颗粒和基本上不含氧化铝的耐火氧化物粘合剂，其中ZSM-48和/或EU-2沸石颗粒的平均铝浓度为至少1.3倍颗粒表面的铝浓度，制备这种催化剂组合物的方法和借助于这些组合物转化烃原料的方法。

5. 发明申请

WO2012055755A1 HYDROCARBON CONVERSION CATALYST COMPOSITION 审中-公开
标题翻译：碳氢转化催化剂组合物
公开(公告)号：WO2012055755A1
公开(公告)日：2012-05-03
申请号：PCT/EP2011/068329
申请日：2011-10-20
申请人： SHELL INTERNATIONALE RESEARCH MAATSCHAPPIJ B.V. , DOMOKOS, László , HUVE, Laurent Georges , JONGKIND, Hermanus , KLAZINGA, Aan Hendrik , RIGUTTO, Marcello Stefano
发明人： DOMOKOS, László , HUVE, Laurent Georges , JONGKIND, Hermanus , KLAZINGA, Aan Hendrik , RIGUTTO, Marcello Stefano
IPC分类号： B01J29/70
CPC分类号： B01J29/7446 , B01J23/42 , B01J23/44 , B01J23/755 , B01J29/70 , B01J29/703 , B01J29/7049 , B01J29/708 , B01J29/80 , B01J37/0201 , B01J2229/16 , B01J2229/37 , B01J2229/42 , C10G35/065 , C10G45/64 , C10G49/08 , C10G50/00 , C10G65/12
摘要： A hydrocarbon conversion catalyst composition which comprises dealuminated ZSM-48 and/or EU-2 zeolite and a refractory oxide binder essentially free of alumina, processes for preparing such composition and processes for converting hydrocarbon feedstock with the help of such compositions.
摘要翻译：一种烃转化催化剂组合物，其包含脱铝的ZSM-48和/或EU-2沸石和基本上不含氧化铝的耐火氧化物粘合剂，用于制备此类组合物的方法和借助于这种组合物转化烃原料的方法。

6. 发明申请

WO2005085394A1 PROCESS TO CONTINUOUSLY PREPARE TWO OR MORE BASE OIL GRADES AND MIDDLE DISTILLATES 审中-公开
标题翻译：连续制备两种或多种基础油和中间馏分的方法
公开(公告)号：WO2005085394A1
公开(公告)日：2005-09-15
申请号：PCT/EP2005/050860
申请日：2005-03-01
申请人： SHELL INTERNATIONALE RESEARCH MAATSCHAPPIJ B.V. , ADAMS, Nicholas James , HEGGE, Harmannus Julius , HUVE, Laurent Georges , POLDER, Kevin John Anthony , STEENGE, Wiecher Derk Evert
发明人： ADAMS, Nicholas James , HEGGE, Harmannus Julius , HUVE, Laurent Georges , POLDER, Kevin John Anthony , STEENGE, Wiecher Derk Evert
IPC分类号： C10G65/12
CPC分类号： C10G65/12 , C10G45/64
摘要： Process to prepare simultaneously two or more base oil grades and middle distillates from a mineral crude derived feed, in particular a de-asphalted oil or a vacuum distillate feed or their mixtures, by performing the following steps: (a) hydrocracking the mineral crude derived feed, thereby obtaining an effluent; (b) distillation of the effluent as obtained in step (a) into one or more middle distillates and a full range residue boiling substantially above 340 ° C, (c) catalytically dewaxing the full range residue by contacting the residue with a dewaxing catalyst comprising a zeolite of the MTW type and a Group VIII metal, thereby obtaining a dewaxed oil; (d) isolating by means of distillation two or more base oil grades from the dewaxed oil obtained in step (c); and (e) isolating a dewaxed gas oil from the dewaxed-oil obtained in step (c); wherein the dewaxed oil as obtained in step (c) comprises between 10 and 40 wt% of a dewaxed heavy gas oil boiling for more than 70 wt% between 370 and 400 ° C.
摘要翻译：通过进行以下步骤同时制备来自矿物原油衍生的原料，特别是脱沥青油或真空馏分进料或其混合物的两种或更多种基础油级和中间馏分的方法：（a）加氢裂化衍生的矿物粗品进料，从而获得流出物; （b）将步骤（a）中获得的流出物蒸馏成一个或多个中间馏出物和基本上在340℃以上沸腾的全范围残余物，（c）通过使残余物与脱蜡相接触来催化脱蜡全部残余物包含MTW型沸石和VIII族金属的催化剂，从而得到脱蜡油; （d）通过蒸馏从步骤（c）中获得的脱蜡油中分离出两种或更多种基础油级; 和（e）从步骤（c）中获得的脱蜡油中分离脱蜡瓦斯油; 其中在步骤（c）中获得的脱蜡油包含10-40重量％的在370和400℃之间沸腾超过70重量％的脱蜡重质瓦斯油。

7. 发明申请

WO2014082985A1 HYDROTREATING AND DEWAXING PROCESS 审中-公开
标题翻译：加氢脱蜡工艺
公开(公告)号：WO2014082985A1
公开(公告)日：2014-06-05
申请号：PCT/EP2013/074695
申请日：2013-11-26
申请人： SHELL INTERNATIONALE RESEARCH MAATSCHAPPIJ B.V. , SHELL OIL COMPANY
发明人： HUVE, Laurent Georges , CHUA, Meng Loong
IPC分类号： C10G45/00 , C10G47/00 , C10G49/22 , C10G65/02
CPC分类号： C10G65/04 , C10G45/00 , C10G47/00 , C10G49/22 , C10G65/02
摘要： The invention provides a process for hydrotreating and dewaxing a hydrocarbon feedstock, comprising the steps of: (a) hydrotreating the feedstock under hydrotreating conditions in a first reaction zone to obtain a first stage hydrotreated effluent; and (b) introducing at least part of the first stage hydrotreated effluent into a second reaction zone in which the first stage hydrotreated effluent is subjected to a series of alternating dewaxing steps and hydrotreating steps, which dewaxing steps are carried out under catalytically dewaxing conditions and the hydrotreating steps are carried out under hydrotreating conditions, wherein the first step in the series of alternating dewaxing and hydrotreating steps is a dewaxing step and the last step of the series of alternating dewaxing and hydrotreating steps is a hydrotreating step, and the dewaxing steps are carried out with a dewaxing catalyst which comprises a Group VIII metal hydrogenation component, dealuminated aluminosilicate zeolite crystallites and a low acidity refractory oxide binder material which is essentially free of alumina.
摘要翻译：本发明提供了一种用于加氢处理和脱蜡烃原料的方法，包括以下步骤：（a）在加氢处理条件下在第一反应区加氢处理原料以获得第一阶段加氢处理的流出物; 和（b）将至少部分第一级加氢处理的流出物引入第二反应区，其中第一级加氢处理的流出物经受一系列的交替脱蜡步骤和加氢处理步骤，该脱蜡步骤在催化脱蜡条件下进行，加氢处理步骤在加氢处理条件下进行，其中一系列交替脱蜡和加氢处理步骤中的第一步是脱蜡步骤，并且一系列交替脱蜡和加氢处理步骤的最后一步是加氢处理步骤，脱蜡步骤为用脱蜡催化剂进行，该脱蜡催化剂包含第VIII族金属氢化组分，脱铝铝硅酸盐沸石微晶和基本上不含氧化铝的低酸度难熔氧化物粘合剂材料。

8. 发明申请

WO2014177424A2 PROCESS FOR PREPARING A HEAVY BASE OIL 审中-公开
标题翻译：制备重油基油的方法
公开(公告)号：WO2014177424A2
公开(公告)日：2014-11-06
申请号：PCT/EP2014/058144
申请日：2014-04-22
申请人： SHELL INTERNATIONALE RESEARCH MAATSCHAPPIJ B.V. , SHELL OIL COMPANY
发明人： HUVE, Laurent Georges , BARIC, John Joseph , BOUMENDJEL, Nariman , DUININCK, Jakob Willem , AARTS, Godfried Johannes
CPC分类号： C10G67/02 , C10G45/64 , C10G65/043 , C10G65/08 , C10G65/12 , C10G2300/202 , C10G2400/10
摘要： The invention provides a process for preparing a heavy base oil comprising the steps of: (a) providing a hydrocarbonaceous feedstock which contains at least 50% by weight of hydrocarbons boiling above 460 °C, nitrogen in amount in the range of from 800-2500 ppmw, and sulphur in an amount in the range of from 1.5-4.0 %wt ppmw; (b) hydrotreating the hydrocarbonaceous feedstock with a hydrotreating catalyst in the presence of a hydrogen- containing gas under hydrotreating conditions to obtain a hydrotreated product which contains nitrogen in an amount in the range of from 30-80 ppmw and sulphur in an amount in the range of from 200-450 ppmw; (c) removing at least 50% of the N¾ and ¾S which is present in the hydrotreated product as obtained in step (b); (d) catalytically dewaxing at least part of the hydrotreated product as obtained in step (c) with a dewaxing catalyst in the presence of a hydrogen- containing gas under catalytic dewaxing conditions to obtain a dewaxed product, which dewaxing catalyst comprises a Group VIII metal hydrogenation component, dealuminated aluminosilicate zeolite crystallites and a low acidity refractory oxide binder material which is essentially free of alumina; (e) hydrofinishing at least part of the dewaxed product as obtained in step (d) with a hydrofinishing catalyst in the presence of a hydrogen-containing gas under hydrofinishing conditions to obtain a heavy base oil; and (f) recovering the heavy base oil.
摘要翻译：本发明提供一种制备重质基础油的方法，包括以下步骤：（a）提供含烃原料，该原料含有至少50重量％沸点高于460℃的烃，其量为800-2500 ppmw和硫，其量为1.5-4.0重量ppmw; （b）在加氢处理条件下，在含氢气体存在下，用加氢处理催化剂对含烃原料进行加氢处理，得到加氢处理的产物，其含量范围为30-80ppmw，硫含量为范围为200-450 ppmw; （c）除去在步骤（b）中获得的加氢处理产物中存在的至少50％的N 3和S 3 S; （d）在催化脱蜡条件下，在含氢气体存在下，用脱蜡催化剂将步骤（c）中得到的加氢处理产物的至少一部分催化脱蜡以获得脱蜡产物，该脱蜡催化剂包含第Ⅷ族金属氢化组分，脱铝铝硅酸盐沸石微晶和基本上不含氧化铝的低酸度难熔氧化物粘合剂材料; （e）在加氢精制条件下，在含氢气体存在下，用加氢精制催化剂加氢精制步骤（d）得到的至少部分脱蜡产物，得到重质基础油; 和（f）回收重质基础油。

9. 发明申请

WO2014095813A1 PROCESS FOR PREPARING A HYDROWAX 审中-公开
标题翻译：制备HYDROWAX的方法
公开(公告)号：WO2014095813A1
公开(公告)日：2014-06-26
申请号：PCT/EP2013/076837
申请日：2013-12-17
申请人： SHELL INTERNATIONALE RESEARCH MAATSCHAPPIJ B.V. , SHELL OIL COMPANY
发明人： BARIC, John Joseph , VAN DIJK, Nicolaas , HUVE, Laurent Georges
IPC分类号： C10G65/12 , B01J21/12 , B01J23/888 , B01J37/20 , B01J29/08 , C10G73/44
CPC分类号： C10M101/025 , B01J23/882 , B01J29/076 , B01J29/166 , C10G47/16 , C10G65/12 , C10G73/44 , C10G2300/301
摘要： The invention provides a process for preparing a hydrowax comprising the steps of: (a) providing a hydrocarbonaceous feedstock which contains more than 4% by weight of hydrocarbons boiling in the range of from 550 to 800 °C; (b) hydrotreating the hydrocarbonaceous feedstock with a hydrotreating catalyst in the presence of a hydrogen- containing gas under hydrotreating conditions to obtain a hydrotreated product; (c) hydrocracking at least part of the hydrotreated product as obtained in step (b) with a hydrocracking catalyst in the presence of a hydrogen-containing gas under hydrocracking conditions to obtain a hydrocracked product, which hydrocracking catalyst contains a zeolitic component which is present in an amount of at least 14 wt%, based on the total weight of the hydrocracking catalyst, and wherein the volume ratio of the hydrotreating catalyst as used in step (b) and the hydrocracking catalyst is more than 1; and (d) recovering from the hydrocracked product as obtained in step (c) the hydrowax.
摘要翻译：本发明提供了一种制备水合物的方法，包括以下步骤：（a）提供含烃原料，其含有超过4重量％的沸点为550-800℃的烃; （b）在加氢处理条件下在含氢气体存在下，用加氢处理催化剂加氢处理含烃原料，得到加氢处理产物; （c）在加氢裂化条件下，在含氢气体存在下，用加氢裂化催化剂加氢裂化步骤（b）中得到的加氢处理产物的至少一部分，得到加氢裂化催化剂，该催化剂含有存在的沸石组分相对于加氢裂化催化剂的总重量为至少14重量％，其中步骤（b）中使用的加氢处理催化剂与加氢裂化催化剂的体积比大于1; 和（d）从在步骤（c）获得的加氢裂化产物中回收氢氟烃。

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