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1. 发明申请

WO2015038668A1 NOVEL CATALYST COMPLEX AND USE THEREOF IN ALKANE OLIGOMERIZATION 审中-公开
标题翻译：新型催化剂复合物及其在碱性低聚物中的应用
公开(公告)号：WO2015038668A1
公开(公告)日：2015-03-19
申请号：PCT/US2014/055027
申请日：2014-09-10
申请人： CHEVRON U.S.A. INC. , RUTGERS, THE STATE UNIVERSITY OF NEW JERSEY
发明人： GOLDMAN, Alan, Stuart , STIBRANY, Robert, Timothy , SAXTON, Robert, J. , MIRONOV, Oleg
IPC分类号： B01J31/02 , B01J31/16 , B01J31/28 , C07C5/333 , C07C11/00
CPC分类号： C07C5/03 , B01J31/0208 , B01J31/183 , B01J31/2409 , B01J2231/20 , B01J2231/766 , B01J2531/824 , B01J2531/827 , B01J2531/828 , C07C2/32 , C07C5/333 , C07C5/48 , C07C5/52 , C07C2531/02 , C07C2531/14 , C07C2531/22 , C07C2531/24 , C07C11/02 , C07C9/00
摘要： Provided is a Group 9 novel metal catalyst complex further comprising a ketone-containing cocatalyst. The metal catalyst complex is useful in generating olefins from alkanes with great efficiency. In one embodiment, provided is an iridium catalyst complex useful in the dehydrogenation of alkanes comprising a ketone-containing cocatalyst and iridium complexed with a tridentate ligand. Also provided is a novel dehydrogenation method which utilizes the catalyst composition. In other embodiments, a novel process for preparing oligomers from alkanes utilizing the catalyst composition is provided.
摘要翻译：提供了另外包含含酮助催化剂的第9族新型金属催化剂络合物。金属催化剂络合物可用于以高效率从烷烃产生烯烃。在一个实施方案中，提供了一种可用于含有酮的助催化剂和与三齿配体络合的铱的烷烃脱氢的铱催化剂络合物。还提供了一种利用催化剂组合物的新型脱氢方法。在其它实施方案中，提供了利用催化剂组合物从烷烃制备低聚物的新方法。

2. 发明申请

WO2015134663A1 ALKANE DEHYDROGENATION PROCESS 审中-公开
标题翻译：碱脱氢方法
公开(公告)号：WO2015134663A1
公开(公告)日：2015-09-11
申请号：PCT/US2015/018818
申请日：2015-03-04
申请人： CHEVRON U.S.A. INC. , RUTGERS, THE STATE UNIVERSITY OF NEW JERSEY
发明人： KUMAR, Akshai , MIRONOV, Oleg , SAXTON, Robert, J. , GOLDMAN, Alan, Stuart
IPC分类号： C07F15/00 , C07F9/02 , C07F9/00
CPC分类号： C07F15/0033 , B01J31/2409 , B01J2231/766 , B01J2531/0244 , B01J2531/827 , C07C5/52 , C07C2531/24 , C07C11/08 , C07C11/02 , C07C11/10
摘要： Disclosed herein are processes for dehydrogenation of an alkane to an alkene using an iridium pincer complex. In the dehydrogenation reactions, hydrogen that is co-formed during the process must be removed for the chemical reaction to proceed and to prevent the excess hydrogen from poisoning the catalyst. In one embodiment the process comprises providing an alkane feedstock comprising at least one alkane and contacting the alkane with an iridium pincer complex in the presence of a hydrogen acceptor selected from the group consisting of ethylene, propene, or mixtures to form an alkene product. The processes disclosed herein can accomplish facile, low-temperature transfer dehydrogenation of alkanes with unprecedented selectivities and TONs at a reasonable rate of conversion.
摘要翻译：本文公开了使用铱钳形复合物将烷烃脱氢成烯烃的方法。在脱氢反应中，必须除去在该过程中共同形成的氢，以进行化学反应并防止过量的氢中毒催化剂。在一个实施方案中，该方法包括提供包含至少一种烷烃的烷烃原料，并在选自乙烯，丙烯或其混合物的氢受体存在下与铱螯合物接触以形成烯烃产物。本文公开的方法可以以合理的转化速率，以前所未有的选择性和TON来实现烷烃的轻度，低温转移脱氢。

3. 发明申请

WO2011066150A2 HYDROPROCESSING BULK CATALYST AND METHODS OF MAKING THEREOF 审中-公开
标题翻译：加氢处理的本体催化剂及其制备方法
公开(公告)号：WO2011066150A2
公开(公告)日：2011-06-03
申请号：PCT/US2010/057031
申请日：2010-11-17
申请人： CHEVRON U.S.A. INC. , MIRONOV, Oleg , KUPERMAN, Alexander E. , HAN, Jinyi
发明人： MIRONOV, Oleg , KUPERMAN, Alexander E. , HAN, Jinyi
IPC分类号： B01J31/02 , B01J27/04 , B01J37/20 , C07C4/06 , C10G45/04
CPC分类号： C10G49/02 , B01J23/80 , B01J23/883 , B01J27/043 , B01J27/0515 , C10G49/12 , C10G2300/1037 , C10G2300/703 , C10G2300/80
摘要： A hydroprocessing bulk catalyst is provided. A process to prepare hydroprocessing bulk catalysts is also provided. The hydroprocessing catalyst has the formula (R p ) i (M t ) a (L u ) b (S v ) d (C w ) e (H x ) f (O y ) g (N z ) h , wherein M is at least a "d" block element metal; L is also at least a "d" block element metal, but different from M; t, u, v, w, x, y, z representing the total charge for each of the components (M, L, S, C, H, O and N, respectively); R is optional and in one embodiment, R is a lanthanoid element metal; 0 i pi+ta+ub+vd+we+xf+yg+zh=0; 0 . The catalyst has an X-ray powder diffraction pattern with at least three diffractions peak located at 2-θ angles of greater than 25°. In one embodiment, the catalyst is prepared by forming at least a sulfided catalyst precursors from at least two "d" block element metals; and mixing the catalyst precursor with a hydrocarbon compound to form the hydroprocessing catalyst composition. In another embodiment, the catalyst is prepared by the thermal decomposition of an oil dispersible sulfur containing organic metal precursor upon contact with a hydrocarbon oil, generating a slurry catalyst. In yet another embodiment, the catalyst is prepared from an in-situ or ex-situ sulfidation of "d block element metal precursors in a solvent carrier.
摘要翻译：提供加氢处理本体催化剂。还提供了制备加氢处理本体催化剂的方法。该加氢处理催化剂具有下式：（R p p）i（M t）a a（L u ）<子> b'/子>（S ^{v ）<子> d （C ^{瓦特）<子>电子（H ^{X ）<子>˚F（O ^{ý）<子>克（N ^{ž）其中M至少是一个“d” 块金属元素; L也至少是“d” 块元素金属，但不同于M; t，u，v，w，x，y，z分别表示每个分量（M，L，S，C，H，O和N）的总电荷; R是可选的并且在一个实施方案中，R是镧系元素金属; 0 <= i <= 1; PI + TA + UB + VD +我们+ XF + YG + ZH = 0; 0 < b; 0 < b / a =＆lt; 5; 0.5（a + b）≤d≤5（a + b）; 0 < e <= 11（a + b）; 0 < f <= 7（a + b）; 0 < g <= 5（a + b）; 0 < h <= 2（a + b）。该催化剂具有X射线粉末衍射图，其中至少三个衍射峰位于大于25℃的2-θ角处。在一个实施方案中，通过从至少两个“d”形成至少一种硫化催化剂前体来制备催化剂。块状元素金属; 并将催化剂前体与烃化合物混合以形成加氢处理催化剂组合物。在另一个实施方案中，所述催化剂通过在与烃油接触后热分解油分散性含硫有机金属前体来制备，从而产生浆料催化剂。在又一个实施方案中，所述催化剂由溶剂载体中的“d嵌段元素金属前体的原位或非原位硫化制备”。}}}}}

4. 发明申请

WO2009058861A2 HYDROPROCESSING BULK CATALYST AND USES THEREOF 审中-公开
标题翻译：氢化聚合物催化剂及其用途
公开(公告)号：WO2009058861A2
公开(公告)日：2009-05-07
申请号：PCT/US2008/081581
申请日：2008-10-29
申请人： CHEVRON U.S.A. INC. , BRAIT, Axel , KUPERMAN, Alexander E. , LOPEZ, Jaime , MIRONOV, Oleg , REYNOLDS, Bruce , CHEN, Kaidong
发明人： BRAIT, Axel , KUPERMAN, Alexander E. , LOPEZ, Jaime , MIRONOV, Oleg , REYNOLDS, Bruce , CHEN, Kaidong
IPC分类号： B01J23/16
CPC分类号： C10G47/04 , B01J23/24 , B01J23/28 , B01J23/85 , B01J23/882 , B01J23/883 , B01J23/8885 , B01J27/0515 , B01J35/002 , B01J35/023 , B01J35/1009 , B01J35/1014 , B01J35/1042 , B01J35/1047 , B01J37/0236 , B01J37/031 , B01J37/038 , B01J37/04 , B01J37/16 , B01J37/20 , B01J37/343 , C10G47/06 , C10G49/04 , C10G2300/107 , C10G2300/1077 , Y10S502/517
摘要： A hydroprocessing bulk catalyst is provided. A process to prepare hydroprocessing bulk catalysts is also provided. The use of the bulk catalyst in hydroprocessing oil feedstock is also provided. The hydroprocessing catalyst has the formula (M t ) a (L u ) b (S v ) d (C w ) e (H x ) f (O y ) g (N z ) h, , wherein M is at least one group VIB metal; promoter metal L is optional and if present, L is at least one Group VIII non-noble metal; t, u, v, w, x, y, z representing the total charge for each of the components (M, L, S, C, H, O and N, respectively); ta+ub+vd+we+xf+yg+zh=0; 0 =
摘要翻译：提供加氢处理体积催化剂。还提供了制备加氢处理大量催化剂的方法。还提供了在加氢处理油原料中使用本体催化剂。加氢处理催化剂具有式（Mt）a（Lu）b（Sv）d（Cw）e（Hx）f（Oy）g（Nz）h ,,其中M是至少一组VIB金属; 促进剂金属L是任选的，如果存在，L是至少一种第VIII族非贵金属; 表示各组分（M，L，S，C，H，O和N分别）的总电荷的t，u，v，w，x，y，z; TA + UB + VD +我们+ XF + YG + ZH = 0; 0 =

5. 发明申请

WO2012092006A2 HYDROPROCESSING CATALYSTS AND METHODS FOR MAKING THEREOF 审中-公开
标题翻译：氢化催化剂及其制备方法
公开(公告)号：WO2012092006A2
公开(公告)日：2012-07-05
申请号：PCT/US2011/066016
申请日：2011-12-20
申请人： CHEVRON U.S.A. INC. , KUPERMAN, Alexander E. , BRAIT, Axel , KOU, Bo , REYNOLDS, Bruce Edward , DUNCKLEY, Christopher Paul , MARIS, Erin P. , NGUYEN, Joseph V. , CHABOT, Julie , KWIK, Kenneth , JIAO, Ling , MIRONOV, Oleg , BHADURI, Rahul Shankar , YANG, Shuwu , KOTUN, Modinat
发明人： KUPERMAN, Alexander E. , BRAIT, Axel , KOU, Bo , REYNOLDS, Bruce Edward , DUNCKLEY, Christopher Paul , MARIS, Erin P. , NGUYEN, Joseph V. , CHABOT, Julie , KWIK, Kenneth , JIAO, Ling , MIRONOV, Oleg , BHADURI, Rahul Shankar , YANG, Shuwu , KOTUN, Modinat
IPC分类号： B01J23/28 , B01J23/30 , B01J23/755 , B01J35/10 , B01J19/24
CPC分类号： B01J23/883 , B01J23/24 , B01J23/85 , B01J23/8872 , B01J23/8873 , B01J27/051 , B01J27/0515 , B01J35/0073 , B01J35/1019 , B01J35/1023 , B01J35/1042 , B01J35/1047 , B01J35/1095 , B01J37/20 , C10G49/04 , C10G49/06 , C10G49/12 , C10G2300/107 , C10G2300/1077 , C10G2300/205 , C10G2300/301 , C10G2300/701 , C10G2300/703 , C10G2300/802
摘要： A process for preparing a slurry catalyst for the heavy oil upgrade is provided. The slurry catalyst has a BET total surface area of at least 100 m2?/g, a total pore volume of at least 0.5 cc/g and a polymodal pore distribution with at least 80% of pore sizes from 5 to 2,000 Angstroms. In one embodiment, a polar aprotic solvent is mixed with the metal precursor feed to form an oil-dispersible precursor. In another embodiment, the precursor feedstock is selected from any of a pressure leach solution from metal recovery, a rework material, a double metal salt precursor, a single metal precursor. In one embodiment, high shear mixing is employed to generate an emulsion. In another embodiment, sulfiding is carried out at least twice for enhanced sulfiding. In another embodiment, at least a metal precursor feedstock is split into portions for addition in various stages of the process.
摘要翻译：提供了一种制备用于重油升级的浆料催化剂的方法。浆料催化剂的BET总表面积为至少100m 2 / g，总孔体积至少为0.5cc / g，多孔模数孔隙分布为至少80％孔径从5至2000埃。在一个实施方案中，将极性非质子溶剂与金属前体进料混合以形成油分散性前体。在另一个实施方案中，前体原料选自金属回收的压力浸出溶液，返修材料，双金属盐前体，单一金属前体中的任一种。在一个实施方案中，采用高剪切混合来产生乳液。在另一个实施方案中，硫化进行至少两次以增强硫化。在另一个实施方案中，至少金属前体原料被分成用于在该方法的各个阶段中添加的部分。

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