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11. 发明申请

WO2014078014A2 PRODUCTION OF SALTS OF 4-HYDROXYBUTYRATE USING BIOBASED RAW MATERIALS 审中-公开
标题翻译：使用生物原料生产4-羟基丁酸盐
公开(公告)号：WO2014078014A2
公开(公告)日：2014-05-22
申请号：PCT/US2013/065916
申请日：2013-10-21
申请人： METABOLIX, INC.
发明人： PEOPLES, Oliver , SAMUELSON, Derek , SENECHAL, Max , PARK, Sung, Min , GREDDER, Joseph , MIRLEY, Christopher
IPC分类号： C07D307/06
CPC分类号： C07C59/01 , A61K9/28 , A61K47/34 , A61L17/105 , C07C51/41 , C07D307/06 , C07D307/33 , C08G63/06
摘要： Gamma-butyrolactone ("GBL") and Gamma-hydroxybutyrate ("GHB") having a unique carbon footprint as defined by the percent modern carbon (pmc) are described herein. The percent modern carbon can be controlled by varying the amounts of biobased, renewable starting materials and petroleum-based starting materials to prepare GBL or GHB having a defined pmc or by preparing mixtures of GBL or GHB prepared from biobased renewable starting materials and GBL or GHB prepared from petroleum-based starting materials.
摘要翻译：本文描述了由现代碳百分比（pmc）定义的具有独特碳足迹的γ-丁内酯（“GBL”）和γ-羟基丁酸酯（“GHB”）。现代碳的百分比可以通过改变生物基可再生原料和石油基原料的量来控制，以制备具有确定的pmc的GBL或GHB或通过制备由生物基可再生原料和GBL或GHB制备的GBL或GHB的混合物由石油基原材料制成。

12. 发明申请

WO2014028943A1 BIOBASED RUBBER MODIFIERS FOR POLYMER BLENDS 审中-公开
标题翻译：用于聚合物混合物的生物橡胶改性剂
公开(公告)号：WO2014028943A1
公开(公告)日：2014-02-20
申请号：PCT/US2013/055624
申请日：2013-08-19
申请人： METABOLIX, INC.
发明人： WEINLEIN, Roger , KANN, Yelena
IPC分类号： C08J5/18 , C08L27/06 , C08L33/12 , C08L59/02
CPC分类号： C08J5/18 , C08J2327/06 , C08J2333/12 , C08J2359/02 , C08J2467/04 , C08L27/06 , C08L33/12 , C08L67/04
摘要： Compositions of polymer blends of polyvinylchloride (PVC) or polymethylmethacrylate (PMMA) or polyoxymethylene (POM) and polyhydroxyalkanoate (PHA) are described. In certain embodiments, the PHA is a poly-3-hydroxybutyrate-co-4-hydroxybutyrate copolymer having a weight percent 4-hydroxybutyrate of 30-45%. In other embodiments the PHA is a multiphase P3HB-4HB copolymer blend having one phase fully amorphous. The PHA is mixed with the PVC or PMMA or POM to optimize its optical, thermal and mechanical properties. In certain embodiments, the polymer is branched with optionally additives that improve properties. Methods of making the compositions of the invention are also described. The invention also includes articles, films and laminates comprising the compositions.
摘要翻译：描述了聚氯乙烯（PVC）或聚甲基丙烯酸甲酯（PMMA）或聚甲醛（POM）和聚羟基链烷酸酯（PHA）的聚合物共混物的组合物。在某些实施方案中，PHA是具有30-45％重量百分比的4-羟基丁酸酯的聚-3-羟基丁酸酯 - 共-4-羟基丁酸酯共聚物。在其它实施方案中，PHA是具有一相完全无定形的多相P3HB-4HB共聚物共混物。 PHA与PVC或PMMA或POM混合，以优化其光学，热学和机械性能。在某些实施方案中，聚合物用可任意改进性质的添加剂进行支化。还描述了制备本发明组合物的方法。本发明还包括包含组合物的制品，薄膜和层压材料。

13. 发明申请

WO2013023140A1 POST PROCESS PURIFICATION FOR GAMMA-BUTYROLACTONE PRODUCTION 审中-公开
标题翻译：用于γ-丁内酯生产的后处理纯化
公开(公告)号：WO2013023140A1
公开(公告)日：2013-02-14
申请号：PCT/US2012/050337
申请日：2012-08-10
申请人： METABOLIX, INC. , VAN WALSEM, Johan , LICATA, John , ANDERSON, Erik , SPARKS, Kevin , FARMER, William , MIRLEY, Christopher , BICKMEIER, Jeffrey, A. , SKRALY, Frank, A. , RAMSEIER, Thomas, M. , D'AMBRUOSO, Ann , SIVASUBRAMANIAN, Melarkodes , SHABTAI, Yossef , SAMUELSON, Derek , HARRIS, Stephen
发明人： VAN WALSEM, Johan , LICATA, John , ANDERSON, Erik , SPARKS, Kevin , FARMER, William , MIRLEY, Christopher , BICKMEIER, Jeffrey, A. , SKRALY, Frank, A. , RAMSEIER, Thomas, M. , D'AMBRUOSO, Ann , SIVASUBRAMANIAN, Melarkodes , SHABTAI, Yossef , SAMUELSON, Derek , HARRIS, Stephen
IPC分类号： C12P7/62 , B01D3/00 , B01D3/14 , C07D307/33
CPC分类号： C07D307/33 , B01D1/18 , B01D1/20 , C12P7/625 , C12P17/04
摘要： Post purification processes and methods for making pure biobased gamma-butyrolactone from renewable carbon resources comprising filtration and/or distillation and/or peroxide treatment are described herein.
摘要翻译：本文描述了用于由可再生碳源制备纯生物基γ-丁内酯的后纯化方法和方法，包括过滤和/或蒸馏和/或过氧化物处理。

14. 发明申请

WO2012149162A2 GREEN PROCESS FOR PRODUCING POLYHYDROXYALKANOATES AND CHEMICALS USING A RENEWABLE FEEDSTOCK 审中-公开
标题翻译：生产聚羟基烷酸酯和化学品的绿色工艺使用可再生料
公开(公告)号：WO2012149162A2
公开(公告)日：2012-11-01
申请号：PCT/US2012/035217
申请日：2012-04-26
申请人： METABOLIX, INC. , ZHANG, Zhigang , MCCHALICHER, Christopher, W.J. , VAN WALSEM, Johan , PEOPLES, Oliver, P. , ENO, Richard, P. , RAMSEIER, Thomas, M.
发明人： ZHANG, Zhigang , MCCHALICHER, Christopher, W.J. , VAN WALSEM, Johan , PEOPLES, Oliver, P. , ENO, Richard, P. , RAMSEIER, Thomas, M.
IPC分类号： C12N1/20
CPC分类号： C12N15/63 , C12N1/20 , C12N15/52 , C12P7/04 , C12P7/18 , C12P7/24 , C12P7/46 , C12P7/625
摘要： Disclosed are organisms genetically engineered to make useful products when grown on ethanol as a carbon source. The organisms are genetically engineered to produce various useful products such as polyhydroxyalkanoates, diols, diacids, higher alcohols, and other useful chemicals.
摘要翻译：公开的是在乙醇作为碳源生长时被遗传工程化以制备有用产物的生物。生物体被遗传工程化以产生各种有用的产物，例如聚羟基链烷酸酯，二醇，二酸，高级醇和其它有用的化学品。

15. 发明申请

WO2012142100A1 BIODEGRADABLE COEXTRUDED MULTILAYER FILMS 审中-公开
标题翻译：生物可降解的多层薄膜
公开(公告)号：WO2012142100A1
公开(公告)日：2012-10-18
申请号：PCT/US2012/033040
申请日：2012-04-11
申请人： METABOLIX, INC. , KRISHNASWAMY, Rajendra, K.
发明人： KRISHNASWAMY, Rajendra, K.
IPC分类号： B32B27/30 , B32B27/36
CPC分类号： B32B27/08 , B32B7/12 , B32B27/306 , B32B27/36 , B32B37/182 , B32B2250/05 , B32B2250/24 , B32B2250/40 , B32B2270/00 , B32B2307/7163 , B32B2307/7244 , B32B2439/70 , Y10T428/31786 , Y10T428/31797
摘要： Described herein is a biobased, fully biodegradable multilayer film having gas barrier properties. Also included is a method of making such material.
摘要翻译：本文描述的是具有阻气性的生物基的完全可生物降解的多层膜。还包括制造这种材料的方法。

16. 发明申请

WO2011146484A2 TOUGHENING POLYLACTIC ACID WITH POLYHYDROXYALKANOATES 审中-公开
标题翻译：用聚羟基烷酸酯增韧多羟基酸
公开(公告)号：WO2011146484A2
公开(公告)日：2011-11-24
申请号：PCT/US2011036808
申请日：2011-05-17
申请人： METABOLIX INC , KRISHNASWAMY RAJENDRA K
发明人： KRISHNASWAMY RAJENDRA K
CPC分类号： C08L67/04 , B32B27/08 , B32B27/18 , B32B27/36 , B32B2307/716 , B32B2307/7163 , B32B2367/00 , C08G63/02 , C08G63/06 , C08G63/08 , C08G63/912 , C08J3/00 , C08J3/20 , C08J2367/04 , C08J2467/04 , C08K3/01 , C08K3/013 , C08K3/014 , C08K3/04 , C08K3/22 , C08K3/28 , C08K3/34 , C08K3/346 , C08K3/36 , C08K5/0008 , C08K5/0016 , C08K5/005 , C08K5/0083 , C08K5/09 , C08K5/14 , C08K5/16 , C08K5/52 , C08K5/521 , C08K2003/2206 , C08L23/08 , C08L23/0884 , C08L33/06 , C08L33/068 , C08L67/00 , C08L67/02 , C08L2201/06 , C08L2203/16 , Y10T428/265 , Y10T428/31786 , C08L2666/18
摘要： Compositions of polymer blends of polylactic acid (PLA) and polyhydroxyalkanoate are described. In certain embodiments, the PHA is a multiphase copolymer blend having one phase a fully amorphous phase with a glass transition temperature of below 20°C and is between about 5 to about 45% of the total PHA. Methods of making the compositions of the invention are also described. The invention also includes articles, films and laminates comprising the compositions.
摘要翻译：描述了聚乳酸（PLA）和聚羟基链烷酸酯的聚合物共混物的组合物。在某些实施方案中，PHA是具有一相的玻璃化转变温度低于20℃并且在总PHA的约5至约45％之间的完全无定形相的多相共聚物共混物。还描述了制备本发明组合物的方法。本发明还包括包含组合物的制品，薄膜和层压材料。

17. 发明申请

WO2011100601A1 PROCESS FOR GAMMA-BUTYROLACTONE PRODUCTION 审中-公开
标题翻译： γ-丁内酯生产方法
公开(公告)号：WO2011100601A1
公开(公告)日：2011-08-18
申请号：PCT/US2011/024612
申请日：2011-02-11
申请人： METABOLIX, INC. , VAN WALSEM, Johan , ANDERSON, Erik , LICATA, John , SPARKS, Kevin, A. , FARMER, William, R. , MIRLEY, Christopher , BICKMEIER, Jeffrey, A. , D'AMBRUOSO, Ann , SKRALY, Frank, A. , RAMSEIER, Thomas, M. , SIVASUBRAMANIAN, M.S.
发明人： VAN WALSEM, Johan , ANDERSON, Erik , LICATA, John , SPARKS, Kevin, A. , FARMER, William, R. , MIRLEY, Christopher , BICKMEIER, Jeffrey, A. , D'AMBRUOSO, Ann , SKRALY, Frank, A. , RAMSEIER, Thomas, M. , SIVASUBRAMANIAN, M.S.
IPC分类号： C07D307/33 , C12P7/62
CPC分类号： A45D40/0068 , C07C67/08 , C07C67/333 , C07D305/12 , C07D307/33 , C07D309/30 , C07D319/12 , C07D407/04 , C12P7/52 , C12P7/625 , C12P17/04 , C07C69/56 , C07C69/54
摘要： The application is directed to a process for the production of a biobased gamma -butyrolactone product, comprising combining a genetically engineered biomass comprising poly- 4 -hydroxy-butyrate and a catalyst, and heating the biomass with the catalyst to convert the poly- 4 -hydroxybutyrate to a gamma -butyrolactone product.
摘要翻译：本申请涉及用于生产生物基γ-丁内酯产物的方法，包括将包含聚-4-羟基丁酸酯和基质催化剂的基因工程生物质与催化剂组合，催化剂将聚-4-羟基丁酸酯转化为γ-丁内酯产物。

18. 发明申请

WO2010151811A3 BRANCHED ALIPHATIC-AROMATIC POLYESTER BLENDS 审中-公开
标题翻译：分散的脂肪 - 芳香族聚酯混合物
公开(公告)号：WO2010151811A3
公开(公告)日：2011-03-31
申请号：PCT/US2010040056
申请日：2010-06-25
申请人： METABOLIX INC , KRISHNASWAMY RAJENDRA K , SUN XIUDONG
发明人： KRISHNASWAMY RAJENDRA K , SUN XIUDONG
IPC分类号： C08L67/04 , C08G63/06 , C08G63/183 , C08J5/18 , C08K5/14 , C08L67/03
CPC分类号： C08L67/02 , B32B27/08 , B32B27/18 , B32B27/36 , B32B2270/00 , B32B2307/54 , B32B2307/558 , B32B2307/5825 , B32B2307/7145 , B32B2307/7163 , B32B2307/738 , B32B2410/00 , B32B2435/00 , B32B2439/00 , B32B2457/00 , B32B2509/00 , B32B2535/00 , B32B2553/00 , B32B2555/00 , B32B2605/00 , C08G63/91 , C08G63/912 , C08J5/18 , C08J2367/02 , C08J2367/04 , C08J2467/04 , C08L67/04 , C08L67/08 , Y10T428/31794
摘要： Compositions of PHAs with aromatic/aliphatic polyester are described and methods of making the same.
摘要翻译：描述了具有芳族/脂族聚酯的PHAs的组合物及其制备方法。

19. 发明申请

WO2010118041A1 METHOD OF IMPROVING FILM PROCESSING AND INJECTION MOLDING OF POLYHYDROXYALKANOATE POLYMERS 审中-公开
标题翻译：改进聚羟基烷基酯聚合物膜的加工和注塑成型的方法
公开(公告)号：WO2010118041A1
公开(公告)日：2010-10-14
申请号：PCT/US2010/030111
申请日：2010-04-06
申请人： METABOLIX, INC. , KRISHNASWAMY, Rajendra, K.
发明人： KRISHNASWAMY, Rajendra, K.
IPC分类号： C08G63/00 , C08K3/26
CPC分类号： C08J3/203 , C08J9/0066 , C08J2367/04 , C08K3/26 , C08K5/0083 , C08L67/02 , C08L67/04 , C08L2666/18
摘要： Processing and improvements in processing of polyhydroxyalkanoate polymer films, sheet, injection moldings, thermoforms, and blow moldings are provided, by use of particular types of calcium carbonate. Methods for using the calcium carbonates in processing of polyhydroxyalkanoate polymers are also disclosed, as well as polyhydroxyalkanoate polymer compositions comprising the calcium carbonates, and articles made therefrom.
摘要翻译：通过使用特定类型的碳酸钙提供加工和改进聚羟基链烷酸酯聚合物膜，片，注射成型品，热成型件和吹塑成型品的加工。还公开了在聚羟基链烷酸酯聚合物的加工中使用碳酸钙的方法，以及包含碳酸钙的聚羟基链烷酸酯聚合物组合物和由其制备的制品。

20. 发明申请

WO2010068953A3 GREEN PROCESS AND COMPOSITIONS FOR PRODUCING POLY(5HV) AND 5 CARBON CHEMICALS 审中-公开
标题翻译：用于生产聚（5HV）和5碳化合物的绿色方法和组合物
公开(公告)号：WO2010068953A3
公开(公告)日：2010-08-05
申请号：PCT/US2009067943
申请日：2009-12-14
申请人： METABOLIX INC , FARMER WILLIAM R , BICKMEIER JEFF , LU CHENFENG , CHANG DONG-EUN , SKRALY FRANK , RAMSEIER THOMAS MARTIN
发明人： FARMER WILLIAM R , BICKMEIER JEFF , LU CHENFENG , CHANG DONG-EUN , SKRALY FRANK , RAMSEIER THOMAS MARTIN
IPC分类号： C12N1/21 , C12N9/00 , C12N9/02 , C12N9/04 , C12N9/10 , C12N9/80 , C12N9/88 , C12N15/52 , C12P7/04 , C12P7/18 , C12P7/42 , C12P7/44 , C12P7/62
CPC分类号： C12N15/52 , C12N9/0006 , C12N9/0008 , C12N9/0069 , C12N9/10 , C12N9/1029 , C12N9/1096 , C12N9/80 , C12N9/88 , C12N9/93 , C12P7/04 , C12P7/18 , C12P7/42 , C12P7/44 , C12P7/625
摘要： Recombinant hosts for producing polyhydroxyalkanoates and methods of producing polyhydroxyalkanoates from renewable carbon substrates are provided. Certain recombinant hosts that produce 5 carbon chemicals such as 5-amino?entanoate (5AP), 5 -hydroxy valerate (5HV), glutarate, and 1,5 pentanediol (PDO) are also provided. One embodiment provides a recombinant host expressing a gene encoding a heterologous enzyme selected from the group consisting of a polyhydroxyalkanoate synthase and a 5-hydroxyvalerate-CoA (5HV-CoA) transferase, wherein the host produces a polymer containing 5-hydroxyvalerate. Preferably, the host expresses both a polyhydroxyalkanoate synthase and a 5HV-CoA transferase. The host can be prokaryotic or eukaryotic. A preferred prokaryotic host is E. coli. The polymers produced by the recombinant hosts can be homopolymers or copolymers of 5-hydroxyvalerate. A preferred copolymer is poly(3-hydroxybutyrate-co-5-hydroxyvalerate).
摘要翻译：提供了用于生产聚羟基链烷酸酯的重组宿主和从可再生碳底物生产聚羟基链烷酸酯的方法。还提供了产生5种碳化学物质的某些重组宿主，如5-氨基蓖麻酸酯（5AP），5-羟基戊酸酯（5HV），戊二酸酯和1,5-戊二醇（PDO）。一个实施方案提供了表达编码选自聚羟基链烷酸酯合酶和5-羟基戊酸酯-CoA（5HV-CoA）转移酶的异源酶的基因的重组宿主，其中所述宿主产生含有5-羟基戊酸酯的聚合物。优选地，宿主表达聚羟基链烷酸酯合成酶和5HV-CoA转移酶。宿主可以是原核生物或真核生物。优选的原核宿主是大肠杆菌。由重组宿主产生的聚合物可以是5-羟基戊酸酯的均聚物或共聚物。优选的共聚物是聚（3-羟基丁酸酯 - 共-5-羟基戊酸酯）。

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