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1. 发明授权

US07811962B2 Manufacture of exhaust articles for internal combustion engines 有权
标题翻译：制造内燃机排气制品
公开(公告)号：US07811962B2
公开(公告)日：2010-10-12
申请号：US12183365
申请日：2008-07-31
申请人： Zhicheng Hu , Patrick L. Burk , Shau-Lin F. Chen , Harold N. Rabinowitz , Christopher M. Minnella , Aaron N. Israel
发明人： Zhicheng Hu , Patrick L. Burk , Shau-Lin F. Chen , Harold N. Rabinowitz , Christopher M. Minnella , Aaron N. Israel
IPC分类号： B01J23/10
CPC分类号： B01D53/9454 , B01J23/63 , B01J23/8946 , B01J37/0244 , F01N3/2803 , F01N2510/06 , Y02T10/22
摘要： Provided are methods for manufacturing a base metal undercoat containing catalyst and an exhaust article containing the catalyst. The catalyst contains a base metal undercoat with an oxygen storage component, substantially free of platinum group metal components, and at least one catalytic layer.
摘要翻译：提供了制备含有催化剂的贱金属底涂层和含有该催化剂的排气制品的方法。催化剂含有基本不含铂族金属组分的氧储存组分的基底金属底涂层和至少一种催化剂层。

2. 发明授权

US07276212B2 Exhaust articles for internal combustion engines 有权
标题翻译：内燃机用排气制品
公开(公告)号：US07276212B2
公开(公告)日：2007-10-02
申请号：US09968192
申请日：2001-10-01
申请人： Zhicheng Hu , Patrick L. Burk , Shau-Lin F. Chen , Harold N. Rabinowitz , Christopher M. Minnella , Aaron N. Israel
发明人： Zhicheng Hu , Patrick L. Burk , Shau-Lin F. Chen , Harold N. Rabinowitz , Christopher M. Minnella , Aaron N. Israel
IPC分类号： B01D53/34 , F01N3/10
CPC分类号： B01D53/9454 , B01J23/63 , B01J23/8946 , B01J37/0244 , F01N3/2803 , F01N2510/06 , Y02T10/22
摘要： Provided is a base metal undercoat containing catalyst and an exhaust article containing the catalyst. The catalyst contains a base metal undercoat with an oxygen storage component, and at least one catalytic layer. Also provided are methods for preparing the catalyst and methods for monitoring the oxygen storage capacity of an exhaust article containing the catalyst.
摘要翻译：提供含有催化剂的贱金属底涂层和含有该催化剂的排气制品。催化剂含有具有储氧成分的贱金属底涂层和至少一个催化剂层。还提供了制备催化剂的方法和用于监测含有催化剂的排气制品的储氧能力的方法。

3. 发明申请

US20090042722A1 Manufacture of Exhaust Articles for Internal Combustion Engines 有权
标题翻译：内燃机尾气制造
公开(公告)号：US20090042722A1
公开(公告)日：2009-02-12
申请号：US12183365
申请日：2008-07-31
申请人： Zhicheng Hu , Patrick L. Burk , Shau-Lin F. Chen , Harold N. Rabinowitz , Christopher M. Minnella , Aaron N. Israel
发明人： Zhicheng Hu , Patrick L. Burk , Shau-Lin F. Chen , Harold N. Rabinowitz , Christopher M. Minnella , Aaron N. Israel
IPC分类号： B01J23/10
CPC分类号： B01D53/9454 , B01J23/63 , B01J23/8946 , B01J37/0244 , F01N3/2803 , F01N2510/06 , Y02T10/22
摘要： Provided are methods for manufacturing a base metal undercoat containing catalyst and an exhaust article containing the catalyst. The catalyst contains a base metal undercoat with an oxygen storage component, substantially free of platinum group metal components, and at least one catalytic layer.
摘要翻译：提供了制备含有催化剂的贱金属底涂层和含有该催化剂的排气制品的方法。催化剂含有基本不含铂族金属组分的氧储存组分的基底金属底涂层和至少一种催化剂层。

4. 发明授权

US6110862A Catalytic material having improved conversion performance 失效
标题翻译：催化材料具有改进的转化性能
公开(公告)号：US6110862A
公开(公告)日：2000-08-29
申请号：US74239
申请日：1998-05-07
申请人： Shau-Lin F. Chen , Harold N. Rabinowitz , Chong Kim
发明人： Shau-Lin F. Chen , Harold N. Rabinowitz , Chong Kim
IPC分类号： B01D53/94 , B01D53/86 , B01J23/40 , B01J32/00 , B01J35/10
CPC分类号： B01D53/865 , B01J23/40 , B01J35/1042 , B01J35/108 , Y02C20/10
摘要： A novel catalytic material is prepared by dispersing a catalytically active species, e.g., one or more platinum group metals, on a support phase that contains a high porosity, meso-pores high surface area (HPMPHSA) material. The HPMPHSA material has a porosity, measured in milliliters per gram of material, that is typically at least about 30 percent greater than that of a corresponding conventional material, preferably at least 50 percent greater. In a particular embodiment, the support phase of the catalytic material contains a HPMPHSA alumina having a porosity of about 0.9 ml/g, whereas a conventional alumina typically has a porosity of about 0.45 ml/g. The surface area is above 90, preferably above 100, more preferably equal or above 150 to 160 m.sup.2 /g. The support phase may be wholly composed of the HPMPHSA material or it may be composed of a mixture of the HPMPHSA material and a conventional material. Such a mixture preferably contains at least about 20 percent HPMPHSA material, by weight, e.g., 20 to 50 percent by weight.
摘要翻译：通过将催化活性物质，例如一种或多种铂族金属分散在含有高孔隙率，中孔高表面积（HPMPHSA）材料的载体相上来制备新的催化材料。 HPMPHSA材料具有以毫克/克材料测量的孔隙率，其通常比相应的常规材料的孔隙率至少大约30％，优选地至少大于50％。在一个具体实施方案中，催化材料的载体相含有孔隙率为约0.9ml / g的HPMPHSA氧化铝，而常规氧化铝通常具有约0.45ml / g的孔隙率。表面积大于90，优选大于100，更优选等于或高于150至160m2 / g。支撑相可以完全由HPMPHSA材料组成，或者它可以由HPMPHSA材料和常规材料的混合物组成。这种混合物优选含有至少约20％重量的HPMPHSA材料，例如20至50％重量。

5. 发明授权

US06727202B2 Enhanced NOx trap having increased durability 失效
标题翻译：增强的NOx捕集器具有增加的耐久性
公开(公告)号：US06727202B2
公开(公告)日：2004-04-27
申请号：US09933586
申请日：2001-08-21
申请人： Michel Deeba , Shau-Lin F. Chen , John K. Hochmuth , Patrick L. Burk , Xinyi Wei
发明人： Michel Deeba , Shau-Lin F. Chen , John K. Hochmuth , Patrick L. Burk , Xinyi Wei
IPC分类号： B01J3702
CPC分类号： F01N3/0842 , B01D53/9431 , B01J23/34 , B01J23/6562 , B01J23/92 , B01J37/0201 , B01J37/0242 , B01J37/0248 , F01N3/0814 , F01N2250/12 , F01N2370/02 , F01N2370/22 , Y02C20/10 , Y02T10/24
摘要： A catalytic trap disposed in an exhaust passage of an internal combustion engine which is operated with periodic alternations between lean and stoichiometric or rich conditions, for abatement of NOx in an exhaust gas stream which is generated by the engine. The trap comprises a catalytic trap material and a refractory carrier member on which the catalytic trap material is disposed. The catalytic trap material comprises: (i) a refractory metal oxide support; (ii) a catalytic component effective for promoting the reduction of NOx under stoichiometric or rich conditions; and (iii) a NOx sorbent effective for adsorbing the NOx under lean conditions and desorbing and reducing the NOx to nitrogen under stoichiometric or rich conditions. The NOx sorbent comprises a metal oxide selected from the group consisting of one or alkali metal oxides, alkaline earth metal oxides and mixtures of one or more alkali metal oxides and alkaline earth metal oxides. The manganese component is selected from the group consisting of: (1) a manganese oxide, (2) a mixed oxide of manganese and a transition metal and/or a rare earth metal, (3) a compound of an alkali metal and a manganese oxide, (4) a compound of an alkaline earth metal and a manganese oxide and (5) mixtures of the foregoing oxides and compounds.
摘要翻译：设置在内燃机的排气通道中的催化捕集器，其在稀薄和化学计量或富含条件之间的周期性变化下操作，以减少由发动机产生的废气流中的NOx。捕集器包括催化捕集材料和其上设置有催化捕集材料的耐火载体构件。催化捕集材料包括：（i）难熔金属氧化物载体; （ii）在化学计量或富含条件下有效促进NOx还原的催化组分; 和（iii）有效地在稀薄条件下吸附NOx的NOx吸附剂，并且在化学计量或富含条件下将NOx解吸并还原成氮。 NOx吸附剂包括选自一种或碱金属氧化物，碱土金属氧化物和一种或多种碱金属氧化物和碱土金属氧化物的混合物的金属氧化物。锰成分选自：（1）锰氧化物，（2）锰与过渡金属和/或稀土金属的混合氧化物，（3）碱金属和锰的化合物氧化物，（4）碱土金属和氧化锰的化合物和（5）上述氧化物和化合物的混合物。

6. 发明授权

US06239064B1 Catalytic compositions and methods for suppression of halogenation of organic compounds with oxidation products of halogenated organic compounds in gaseous emission streams 有权
标题翻译：催化组合物和用于在气体排放物流中用卤化有机化合物的氧化产物抑制有机化合物卤化的方法
公开(公告)号：US06239064B1
公开(公告)日：2001-05-29
申请号：US09195053
申请日：1998-11-18
申请人： Pascaline H. Nguyen , James M. Chen , Chung-Zong Wan , Shau-Lin F. Chen , Zhicheng Hu
发明人： Pascaline H. Nguyen , James M. Chen , Chung-Zong Wan , Shau-Lin F. Chen , Zhicheng Hu
IPC分类号： B01J2358
CPC分类号： B01J23/63 , B01D53/8662 , B01D53/8668
摘要： Methods and chemical compositions for treating a gas stream comprising non-halogenated and halogenated organic compounds while suppressing halogenation of the non-halogenated organic compounds with the oxidation products of the halogenated organic compounds in the gas stream are disclosed. The gas stream in the presence of oxygen is contacted with the catalyst compositions of the invention to oxidize the non-halogenated and the halogenated compounds to form water, carbon dioxide, and halogen molecules (Cl2, Br2, etc.) and/or halogen acids such as HCl, HBr, etc. An advantage of the present compositions and methods is that halogenation or of the treated emissions is suppressed over a process operating temperature range 400 to 550° C.
摘要翻译：公开了用于处理包含非卤化和卤化有机化合物的气流同时抑制非卤代有机化合物与气流中的卤代有机化合物的氧化产物的卤化反应的方法和化学组合物。在氧存在下的气流与本发明的催化剂组合物接触以氧化非卤化和卤化的化合物以形成水，二氧化碳和卤素分子（Cl 2，Br 2等）和/或卤素酸例如HCl，HBr等。本发明的组合物和方法的优点是在400至550℃的工艺操作温度范围内抑制了卤化或经处理的发射。

7. 发明授权

US08940242B2 Multi-zoned catalyst compositions 有权
标题翻译：多区催化剂组合物
公开(公告)号：US08940242B2
公开(公告)日：2015-01-27
申请号：US12761873
申请日：2010-04-16
申请人： Shau-Lin F. Chen , Dennis R. Anderson
发明人： Shau-Lin F. Chen , Dennis R. Anderson
IPC分类号： B01D50/00 , F23J11/00 , F02M25/06 , F01N3/28 , F01N3/08
CPC分类号： F01N3/2828 , F01N3/08 , F01N3/0814 , F01N3/0835 , F01N3/0864 , F01N2250/12 , F01N2330/06 , F01N2330/30 , F01N2330/60 , F01N2510/0682 , F01N2510/0684
摘要： Exhaust gas treatment substrates, and systems and methods including the same are provided. Catalyst substrates having flow properties where in configuring an outer, peripheral zone, more exhaust gas flows through a central zone as compared to the outer, peripheral zone. The outer, peripheral zone can have a trapping or adsorbing material on surfaces of its passages, or it can have a longer axial length as compared to the inner zone, or its passages can have smaller openings as compared to the inner zone. In one embodiment, an overcoat containing a trapping material such as a hydrocarbon trap is applied to an inlet end. In another embodiment, catalyst having an oxygen storage component is applied to an outlet end.
摘要翻译：提供废气处理基板，以及包括其的系统和方法。具有流动特性的催化剂衬底，其中在构造外部周边区域时，与外部周边区域相比，更多的废气流过中心区域。外部周边区域可以在其通道的表面上具有捕获或吸附材料，或者与内部区域相比可以具有更长的轴向长度，或者与内部区域相比，其通道可以具有较小的开口。在一个实施方案中，将包含捕获材料如烃阱的外涂层施加到入口端。在另一个实施方案中，将具有储氧组分的催化剂施加到出口端。

8. 发明授权

US06777370B2 SOx tolerant NOx trap catalysts and methods of making and using the same 有权
标题翻译： SOx耐受性NOx捕集催化剂及其制备和使用方法
公开(公告)号：US06777370B2
公开(公告)日：2004-08-17
申请号：US09834505
申请日：2001-04-13
申请人： Shau-Lin F. Chen
发明人： Shau-Lin F. Chen
IPC分类号： B01J2334
CPC分类号： B01D53/945 , B01D2255/1021 , B01D2255/1023 , B01D2255/1025 , B01D2255/206 , B01D2255/9022 , B01D2255/91 , B01J23/58 , B01J23/63 , B01J23/8892 , B01J35/0006 , B01J37/0248 , Y02T10/22
摘要： The present invention relates to a layered catalyst composite useful for reducing contaminants in exhaust gas streams, especially gaseous streams containing sulfur oxide contaminants. More specifically, the present invention is concerned with improved catalysts of the type generally referred to as “three-way conversion” catalysts. The layered catalysts trap sulfur oxide contaminants which tend to poison three-way conversion catalysts used to abate other pollutants in the stream. The layered catalyst composites of the present invention have a sulfur oxide absorbing layer before or above a nitrogen oxide absorbing layer. The layered catalyst composite comprises a first layer and a second layer. The first layer comprises a first support and at least one first platinum component. The second layer comprises a second support and a SOx sorbent component, wherein the SOx sorbent component is selected from the group consisting of MgAl2O4, MnO, MnO2, and Li2O. The sulfur oxide absorbing layer selectively and reversibly absorbs sulfur oxides over nitrogen oxides and prevents or alleviates sulfur oxide poisoning of the nitrogen oxide trap.
摘要翻译：本发明涉及一种用于减少废气流中污染物，特别是含有硫氧化物污染物的气流的层状催化剂复合物。更具体地，本发明涉及通常称为“三向转化”催化剂的改进的催化剂。分层催化剂捕获硫氧化物污染物，其倾向于毒化用于消除流中其它污染物的三元转化催化剂。本发明的层状催化剂复合体在氮氧化物吸收层之前或之上具有硫氧化物吸收层。层状催化剂复合材料包括第一层和第二层。第一层包括第一载体和至少一种第一铂组分。第二层包括第二载体和SOx吸附剂组分，其中SO x吸附剂组分选自MgAl 2 O 4，MnO，MnO 2和Li 2 O。硫氧化物吸收层选择性地且可逆地吸收氮氧化物上的硫氧化物并且防止或减轻氮氧化物阱的硫氧化物中毒。

9. 发明授权

US06923945B2 Layered SOX tolerant NOX trap catalysts and methods of making and using the same 有权
标题翻译：层状SOX耐受性NOX捕集催化剂及其制备和使用方法
公开(公告)号：US06923945B2
公开(公告)日：2005-08-02
申请号：US10766374
申请日：2004-01-28
申请人： Shau-Lin F. Chen
发明人： Shau-Lin F. Chen
IPC分类号： F01N3/10 , B01D53/94 , B01J23/58 , B01J23/63 , B01J23/656 , B01J23/889 , B01J35/00 , B01J37/02 , F01N3/28 , B01D53/50 , B01D53/56 , B01D53/60
CPC分类号： B01D53/945 , B01D2255/1021 , B01D2255/1023 , B01D2255/1025 , B01D2255/206 , B01D2255/9022 , B01D2255/91 , B01J23/58 , B01J23/63 , B01J23/8892 , B01J35/0006 , B01J37/0248 , Y02T10/22
摘要： The present invention relates to a layered catalyst composite useful for reducing contaminants in exhaust gas streams, especially gaseous streams containing sulfur oxide contaminants. More specifically, the present invention is concerned with improved catalysts of the type generally referred to as “three-way conversion” catalysts. The layered catalysts trap sulfur oxide contaminants which tend to poison three-way conversion catalysts used to abate other pollutants in the stream. The layered catalyst composites of the present invention have a sulfur oxide absorbing layer before or above a nitrogen oxide absorbing layer. The layered catalyst composite comprises a first layer and a second layer. The first layer comprises a first support and at least one first platinum component. The second layer comprises a second support and a SOx sorbent component having a free energy of formation from about 0 to about −90 Kcal/mole at 350° C. The sulfur oxide absorbing layer selectively and reversibly absorbs sulfur oxides over nitrogen oxides and prevents or alleviates sulfur oxide poisoning of the nitrogen oxide trap.
摘要翻译：本发明涉及一种用于减少废气流中污染物，特别是含有硫氧化物污染物的气流的层状催化剂复合物。更具体地，本发明涉及通常称为“三向转化”催化剂的改进的催化剂。分层催化剂捕获硫氧化物污染物，其倾向于毒化用于消除流中其它污染物的三元转化催化剂。本发明的层状催化剂复合体在氮氧化物吸收层之前或之上具有硫氧化物吸收层。层状催化剂复合材料包括第一层和第二层。第一层包括第一载体和至少一种第一铂组分。第二层包括在350℃下具有约0至约-90Kcal /摩尔的形成自由能的第二载体和SO x吸附剂组分。硫氧化物吸收层选择性地和可逆地吸收硫氧化物超过氮氧化物，并防止或减轻氮氧化物陷阱的硫氧化物中毒。

10. 发明申请

US20140031197A1 Catalyst Materials 有权
标题翻译：催化剂材料
公开(公告)号：US20140031197A1
公开(公告)日：2014-01-30
申请号：US13560096
申请日：2012-07-27
申请人： Gary A. Gramiccioni , Stephan Siemund , Shau-Lin F. Chen , Kenneth Brown
发明人： Gary A. Gramiccioni , Stephan Siemund , Shau-Lin F. Chen , Kenneth Brown
IPC分类号： B01J27/053
CPC分类号： B01J23/63 , B01D53/945 , B01D2255/1023 , B01D2255/2042 , B01D2255/2063 , B01D2255/2065 , B01D2255/2066 , B01D2255/20715 , B01D2255/2092 , B01D2255/902 , B01D2255/908 , B01J23/002 , B01J37/0242 , B01J37/0244 , B01J37/082 , B01J37/16 , Y02T10/22
摘要： A catalyst material including a catalyst carrier including a porous alumina support and a hindrance layer on the alumina support, the hindrance layer comprising one or more barium sulfate, strontium sulfate, zirconium sulfate, and calcium sulfate is described. The catalyst carrier further includes a rare earth oxide. The catalyst material can further comprise a platinum group metal oxide. The hindrance layer may prevent the rare earth oxide from forming a complex with the support. The catalyst material is useful for methods and systems of abating pollutants from automotive exhaust gas.
摘要翻译：描述了一种催化剂材料，其包括在氧化铝载体上包含多孔氧化铝载体和阻碍层的催化剂载体，所述阻碍层包含一种或多种硫酸钡，硫酸锶，硫酸锆和硫酸钙。催化剂载体还包括稀土氧化物。催化剂材料还可以包含铂族金属氧化物。阻碍层可以防止稀土氧化物与载体形成络合物。催化剂材料可用于减轻汽车尾气污染物的方法和系统。

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