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1. 发明授权

US5702827A Olefin thermoplastic elastomer and laminate thereof 失效
公开(公告)号：US5702827A
公开(公告)日：1997-12-30
申请号：US459804
申请日：1995-06-02
申请人： Yuichi Itoh , Kyoko Kobayashi , Akira Uchiyama , Toru Takehara
发明人： Yuichi Itoh , Kyoko Kobayashi , Akira Uchiyama , Toru Takehara
IPC分类号： B32B27/32 , C08L23/02 , C08L23/10 , C08L23/16 , C08L53/00 , C08L53/02 , B32B23/08
CPC分类号： C08L23/16 , B32B27/32 , C08L23/02 , C08L23/10 , C08L53/02 , C08L53/025 , C08L53/00 , Y10T428/31917 , Y10T428/31924 , Y10T428/31931 , Y10T428/31938
摘要： Olefin thermoplastic elastomers which comprise a partially crosslinked thermoplastic elastomer comprising a crystalline polyolefin resin (A), a block copolymer (B) which is composed of a polymer block of styrene or its derivative and a specific isoprene polymer block, and an olefin rubber (C), and thermoplastic elastomer laminates, having a substrate formed from a specific olefin thermoplastic elastomer or a crystalline polyolefin resin and a skin layer formed from the above-mentioned olefin thermoplastic elastomer, which are excellent in mechanical strength, heat resistance, heat aging resistance, weathering resistance and scratch resistance have been provided by the present invention.

2. 发明授权

US5596042A Olefin thermoplastic elastomer and laminate thereof 失效
标题翻译：烯烃热塑性弹性体及其层压材料
公开(公告)号：US5596042A
公开(公告)日：1997-01-21
申请号：US626900
申请日：1996-04-04
申请人： Yuichi Itoh , Kyoko Kobayashi , Akira Uchiyama , Toru Takehara
发明人： Yuichi Itoh , Kyoko Kobayashi , Akira Uchiyama , Toru Takehara
IPC分类号： B32B27/32 , C08L23/02 , C08L23/10 , C08L23/16 , C08L53/00 , C08L53/02 , C08L25/08
CPC分类号： C08L23/16 , B32B27/32 , C08L23/02 , C08L23/10 , C08L53/02 , C08L53/025 , C08L53/00 , Y10T428/31917 , Y10T428/31924 , Y10T428/31931 , Y10T428/31938
摘要： Olefin thermoplastic elastomers which comprise a partially crosslinked thermoplastic elastomer comprising a crystalline polyolefin resin (A), a block copolymer (B) which is composed of a polymer block of styrene or its derivative and a specific isoprene polymer block, and an olefin rubber (C), and thermoplastic elastomer laminates, having a substrate formed from a specific olefin thermoplastic elastomer or a crystalline polyolefin resin and a skin layer formed from the above-mentioned olefin thermoplastic elastomer, which are excellent in mechanical strength, heat resistance, heat aging resistance, weathering resistance and scratch resistance have been provided by the present invention.
摘要翻译：包含部分交联的热塑性弹性体的烯烃热塑性弹性体包括结晶聚烯烃树脂（A），由苯乙烯或其衍生物的聚合物嵌段和特定的异戊二烯聚合物嵌段组成的嵌段共聚物（B）和烯烃橡胶（C ）和热塑性弹性体层压体，其具有由特定烯烃热塑性弹性体或结晶聚烯烃树脂形成的基材和由上述烯烃热塑性弹性体形成的表层，其机械强度，耐热性，耐热老化性优异，本发明提供了耐候性和耐划伤性。

3. 发明授权

US06635705B2 Olefinic thermoplastic elastomer composition and method for producing the same 失效
标题翻译：烯烃类热塑性弹性体组合物及其制造方法
公开(公告)号：US06635705B2
公开(公告)日：2003-10-21
申请号：US09986477
申请日：2001-11-08
申请人： Yuichi Itoh , Kyoko Kobayashi , Akira Uchiyama , Masaaki Kawasaki
发明人： Yuichi Itoh , Kyoko Kobayashi , Akira Uchiyama , Masaaki Kawasaki
IPC分类号： C08L2316
CPC分类号： C08L23/02 , C08K5/01 , C08K5/02 , C08K5/14 , C08L23/0815 , C08L23/12 , C08L23/16 , C08L23/22 , C08L91/00 , C08L2205/02 , C08L2205/03 , C08L2207/04 , C08L2312/02 , C08L2314/06 , Y10S526/943 , C08L2666/04
摘要： The present invention relates to an olefinic thermoplastic elastomer composition which comprises a crystalline polyolefin resin (A), an ethylene-&agr;-olefin-non-conjugated polyene copolymer rubber (B) and at least on rubber (C) selected from polyisobutylene, butyl rubber and a propylene-ethylene copolymer rubber having a propylene content of 50 mol % or more or an ethylene-&agr;-olefin copolymer (D) having a density of 0.870 to 0.940 (g/cm3) and an ethylene content of 85 mol % or more, said ethylene-&agr;-olefin-non-conjugated polyene copolymer rubber (B) being crosslinked thermoplastic elastomer composition, being obtained by random copolymerization of ethylene, and &agr;-olefin having 3 to 20 carbon atoms and a non-conjugated polyene in the presence of a metallocene catalyst, (1) containing the unit (a) derived from the ethylene and the unit (b) derived from the &agr;-olefin in a molar ratio of 40/60 to 95/5 [(a)/(b)], (2) having an iodine value of 1 to 50 and (3) having an intrinsic viscosity [&eegr;] measured in decalin at 135° C. of 1.0 to 10 dl/g; and relates to a method for manufacturing the same.
摘要翻译：本发明涉及一种烯烃热塑性弹性体组合物，其包含结晶聚烯烃树脂（A），乙烯-α-烯烃 - 非共轭多烯共聚物橡胶（B）和至少在选自聚异丁烯，丁基橡胶丙烯含量为50摩尔％以上的丙烯 - 乙烯共聚物橡胶或密度为0.870〜0.940（g / cm 3），乙烯含量为85摩尔的乙烯-α-烯烃共聚物（D）％以上，所述乙烯-α-烯烃 - 非共轭多烯共聚物橡胶（B）为交联热塑性弹性体组合物，其通过乙烯的无规共聚和具有3-20个碳原子的α-烯烃和非共轭多烯在茂金属催化剂的存在下，（1）含有衍生自乙烯的单元（a）和衍生自α-烯烃的单元（b），摩尔比为40/60至95/5 [（a）/ （b）]，（2）碘值为1〜50，（3）具有内嵌在135℃萘烷中测得的粘度η为1.0-10dl / g; 涉及其制造方法。

4. 发明授权

US06723794B2 Olefin thermoplastic elastomer composition comprising crystalline polyolefin resin and ethylene/&agr;-olefin/nonconjugated polyene copolymer rubber 有权
标题翻译：包含结晶聚烯烃树脂和乙烯/α-烯烃/非共轭多烯共聚物橡胶的烯烃热塑性弹性体组合物
公开(公告)号：US06723794B2
公开(公告)日：2004-04-20
申请号：US10066575
申请日：2002-02-06
申请人： Masaaki Kawasaki , Keiji Okada , Tetsuo Tojo , Kyoko Kobayashi , Yuichi Itoh , Akira Uchiyama , Toshiyuki Tsutsui , Toshihiro Sagane
发明人： Masaaki Kawasaki , Keiji Okada , Tetsuo Tojo , Kyoko Kobayashi , Yuichi Itoh , Akira Uchiyama , Toshiyuki Tsutsui , Toshihiro Sagane
IPC分类号： C08L2302
CPC分类号： C08L23/02 , A61J1/03 , B65D23/003 , B65D51/28 , C08K5/14 , C08L23/0815 , C08L23/10 , C08L23/142 , C08L23/16 , C08L23/22 , C08L91/00 , C08L2205/03 , C08L2207/04 , C08L2312/00 , C08L2666/04
摘要： An olefin thermoplastic elastomer composition comprises a crystalline polyolefin resin (A) and an ethylene/&agr;-olefin/nonconjugated polyene copolymer rubber (B), and optionally a softener (C) and/or an inorganic filler (D), in a specific ratio. The copolymer rubber (B) is prepared by the use of a metallocene catalyst and comprises ethylene, an &agr;-olefin of 3 to 20 carbon atoms and a nonconjugated polyene. This composition ca provide molded products of more excellent tensile strength, elongation at break, elastomeric properties (elongation set, permanent compression set, etc.), heat resistance and low-temperature properties than the conventional non-crosslinked olefin thermoplastic elastomers, even if the composition is in the non-crosslinked form. The composition in the partially or completely crosslinked form can provided molded products of more excellent low-temperature properties, tensile strength, elongation at break and elastomeric properties than the conventional vulcanized rubbers.
摘要翻译：烯烃热塑性弹性体组合物包含结晶聚烯烃树脂（A）和乙烯/α-烯烃/非共轭多烯共聚物橡胶（B）和任选的软化剂（C）和/或无机填料（D）。共聚物橡胶（B）通过使用茂金属催化剂制备，包括乙烯，3-20个碳原子的α-烯烃和非共轭多烯。该组合物提供比常规非交联烯烃热塑性弹性体更优异的拉伸强度，断裂伸长率，弹性体性能（伸长率设定，永久压缩变形等），耐热性和低温性能的成型产品，即使组合物为非交联形式。部分或完全交联形式的组合物可以提供比常规硫化橡胶更优异的低温性能，拉伸强度，断裂伸长率和弹性体性能的成型产品。

5. 发明授权

US07094828B2 Olefin thermoplastic elastomer composition 有权
标题翻译：烯烃热塑性弹性体组合物
公开(公告)号：US07094828B2
公开(公告)日：2006-08-22
申请号：US10199066
申请日：2002-07-22
申请人： Kyoko Kobayashi , Hiroyasu Yamaoka , Yuichi Itoh , Akira Uchiyama
发明人： Kyoko Kobayashi , Hiroyasu Yamaoka , Yuichi Itoh , Akira Uchiyama
IPC分类号： C08J3/22
CPC分类号： C08L53/00 , C08L23/10 , C08L23/12 , C08L23/16 , C08L53/02 , C08L91/00 , C08L2207/04 , C08L2312/00 , C08L2666/24 , C08L2666/04 , C08L2666/02
摘要： An olefin thermoplastic elastomer composition which is superior in the resistance to oils, heat resistance, formability and flexibility is provided, said elestomer composition comprising the components(A) 40–90 parts by weight of a polypropylene resin having a melt flow rate (determined at 230 ° C. under a load of 2.16 kg according to ASTM D 1238) of 0.1–5 g/10 minutes,(B) 10–60 parts by weight of a copolymer rubber based on olefin, the contents of the components (A) and (B) summing up to 100 parts by weight, and(C) 20–150 parts by weight of a softener,wherein the composition is in such a cross-linked state that the gel content thereof amounts to 97% by weight or higher.
摘要翻译：提供了耐油性，耐热性，成形性和柔软性优异的烯烃热塑性弹性体组合物，所述组分（A）包含40-90重量份的具有熔体流动速率的聚丙烯树脂（在 230℃，根据ASTM D 1238的2.16kg负荷）为0.1-5g / 10分钟，（B）10-60重量份基于烯烃的共聚物橡胶，组分（A）的含量和（B）总计100重量份，和（C）20-150重量份的软化剂，其中组合物处于交联状态，其凝胶含量为97重量％以上。

6. 发明授权

US6146739A Glass run channel 失效
标题翻译：玻璃运行通道
公开(公告)号：US6146739A
公开(公告)日：2000-11-14
申请号：US27178
申请日：1998-02-20
申请人： Yuichi Itoh , Masato Karaiwa , Kyoko Kobayashi , Akira Uchiyama
发明人： Yuichi Itoh , Masato Karaiwa , Kyoko Kobayashi , Akira Uchiyama
IPC分类号： B60J10/00 , B60J10/04 , C08L23/06 , C08L23/12 , C08L23/16 , B32B27/08 , B32B27/32
CPC分类号： C08L23/06 , B60J10/17 , B60J10/27 , B60J10/74 , C08L23/12 , C08L23/16 , Y10T428/24198 , Y10T428/31917
摘要： A glass run channel comprising a glass run channel body composed of a bottom wall and side walls extending from two opposite edges of the bottom wall, the glass run channel body having a substantially U-shaped section and provided with a groove, and tonguelike draining parts protruding from vicinities of distal edges of the side walls toward the bottom wall of the glass run channel body so as to become proximate to each other. Each of the tonguelike draining parts has a window glass contact part composed of a surface to be brought into contact with a window glass, which comprises a layer of a thermoplastic elastomer and a layer of an ultrahigh molecular weight polyolefin composition. The layer of ultrahigh molecular weight polyolefin composition is arranged so as to contact a window glass. The ultrahigh molecular weight polyolefin composition comprises at least a polyolefin (composition) having a specified intrinsic viscosity and an olefinic thermoplastic elastomer. The glass run channel is excellent in the durability, tight contactability with a window glass exhibited when the window glass is held closed and supple slide exhibited when a window glass is closed or opened and, even when twisted or bent, is free from a creasing of the ultrahigh molecular weight polyolefin composition layer.
摘要翻译：一种玻璃导槽，包括由底壁和从底壁的两个相对边缘延伸的侧壁组成的玻璃导槽体，所述玻璃导槽体具有大致U形截面并设置有凹槽，并且舌状排液部分从侧壁的远侧边缘的附近向玻璃导槽体的底壁突出，以使彼此靠近。每个舌形排液部分具有由玻璃接触的表面组成的窗玻璃接触部分，其包括热塑性弹性体层和超高分子量聚烯烃组合物层。超高分子量聚烯烃组合物层布置成与窗玻璃接触。超高分子量聚烯烃组合物至少包含具有特定特性粘度的聚烯烃（组合物）和烯属热塑性弹性体。玻璃运行通道在窗玻璃闭合时呈现的窗玻璃的耐久性，与窗玻璃紧密接触的紧密接触性，并且当窗玻璃闭合或打开时呈现柔顺的滑动，并且即使扭曲或弯曲也不会起皱超高分子量聚烯烃组合物层。

7. 发明授权

US5856399A Thermoplastic elastomer composition 失效
标题翻译：热塑性弹性体组合物
公开(公告)号：US5856399A
公开(公告)日：1999-01-05
申请号：US635319
申请日：1996-04-19
申请人： Yuichi Itoh , Kyoko Kobayashi , Akira Uchiyama
发明人： Yuichi Itoh , Kyoko Kobayashi , Akira Uchiyama
IPC分类号： C08K5/00 , C08L23/00 , C08L23/02 , C08L23/10 , C08L23/16 , C08L25/00 , C08L53/00 , C08L53/02 , C08L91/00
CPC分类号： C08L23/02 , C08L23/16 , C08L2207/04 , C08L23/10 , C08L2312/00 , C08L53/02 , C08L91/00
摘要： The thermoplastic elastomer composition of the invention comprises a crystalline polyolefin resin (A), an olefin rubber (B), a hydrogenated styrene block copolymer (C), a softener (D), and optionally, a peroxide non-crosslinked type hydrocarbon rubber (E) in a specific amount of each, and has a gel content of not less than 97%. This composition may be mixed with a crystalline polyolefin resin. The thermoplastic elastomer composition has excellent moldability and is able to provide a molded product having excellent elastomeric properties, high resistance to permanent compression set and good appearance. In particular, a composition obtained by mixing this thermoplastic elastomer composition and a crystalline polyolefin resin shows excellent moldability.
摘要翻译：本发明的热塑性弹性体组合物包含结晶聚烯烃树脂（A），烯烃橡胶（B），氢化苯乙烯嵌段共聚物（C），软化剂（D）和任选的过氧化物非交联型烃橡胶 E），其凝胶含量不低于97％。该组合物可以与结晶聚烯烃树脂混合。热塑性弹性体组合物具有优异的成型性，能够提供具有优异的弹性性能，高耐永久压缩永久变形和良好外观的成型体。特别地，通过混合该热塑性弹性体组合物和结晶聚烯烃树脂获得的组合物显示出优异的成型性。

8. 发明授权

US07582352B2 Layered product olefin foam and use 失效
公开(公告)号：US07582352B2
公开(公告)日：2009-09-01
申请号：US10069603
申请日：2001-06-29
申请人： Kyoko Kobayashi , Akira Uchiyama
发明人： Kyoko Kobayashi , Akira Uchiyama
IPC分类号： B32B27/32 , B29C39/12
CPC分类号： B32B25/14 , B32B5/18 , B32B27/065 , B32B27/32 , B32B2266/025 , B32B2605/08 , Y10T428/249981 , Y10T428/249986 , Y10T428/249989 , Y10T428/249991 , Y10T428/249992 , Y10T428/249993
摘要： The foamed laminate based on olefin according to the present invention is composed of a substrate layer of a foamed body made of either an ethylenic thermoplastic elastomer comprising a polyethylene resin and an ethylene/α-olefin copolymer having a Mooney viscosity ML1+4 (100° C.) of 90-250 and an ethylene content of 70-95 mole % or an ethylenic thermoplastic elastomer composition comprising 100 parts by weight of an olefinic thermoplastic elastomer and 1-20 parts by weight of an olefinic thermoplastic resin and, under lamination thereon, a skin layer made of either an ultrahigh molecular weight polyolefin resin having an intrinsic viscosity of 3.5-8.3 dl/g or made of an olefinic thermoplastic elastomer composition comprising an olefinic thermoplastic elastomer and a lubricant. The foamed laminate according to the present invention is easy in recycled use, obtainable at a high foaming expansion ratio with soft hand touch and is superior in the appearance, abrasion resistance, durability and sliding performance.

9. 发明授权

US06221963B1 Thermoplastic elastomer based on olefin and process for producing the same 有权
标题翻译：基于烯烃的热塑性弹性体及其制备方法
公开(公告)号：US06221963B1
公开(公告)日：2001-04-24
申请号：US09340044
申请日：1999-06-28
申请人： Kyoko Kobayashi , Akira Uchiyama
发明人： Kyoko Kobayashi , Akira Uchiyama
IPC分类号： C08F800
CPC分类号： C08L23/06 , C08L23/04 , C08L23/12 , C08L23/16 , C08L2205/02 , C08L2207/04 , C08L2666/04
摘要： A thermoplastic elastomer based on olefin which can be produced simply by melt-kneading 5-60% by weight of a polyethylene resin (A) together with 40-95% by weight of an ethylene/&agr;-olefin copolymer (B) with optional subsidiary component(s) before the kneaded mass is molded into a formed product, the said elastomer being capable of recycling for reclamation and exhibiting the following characteristics {circle around (1)} to {circle around (3)} namnely, 9≦Y−0.43 X≦27 (1) {circle around (1)} in which X denotes the JIS A-hardness value (a dimensionless value) of the thermoplastic elastomer based on olefin determined according to the prescription of JIS K 6301 and Y represents the permanent compressive strain value (expressed by %) of the thermoplastic elastomer based on olefin determined according to the prescription of JIS K 6301 under a condition of 70° C.×22 hours, {circle around (2)} tensile strength in the raqnge from 5 to 30 MPa and {circle around (3)} a permanent elongation of 18% or less determined according to the prescription of JIS K 6301.
摘要翻译：一种基于烯烃的热塑性弹性体，其可以简单地通过将5-60重量％的聚乙烯树脂（A）与40-95重量％的乙烯/α-烯烃共聚物（B）与任选的附属物所述弹性体能够循环再造，并且具有以下特征（圆周（1）}到{圆周（3）}周围{圆周（ 1）}，其中X表示根据JIS K 6301的配方确定的基于烯烃的热塑性弹性体的JIS A硬度值（无量纲值），Y表示热塑性塑料的永久压缩应变值（以％表示）在70℃×22小时的条件下测定的基于烯烃的烯烃弹性体，在5〜30MPa的拉伸强度（{圆周（3）}周围的{圈（2）}周围）永久伸长率为18％以下根据JIS K 6301的处方。

10. 发明授权

US06803418B2 Thermoplastic olefin elastomer composition 有权
标题翻译：热塑性烯烃弹性体组合物
公开(公告)号：US06803418B2
公开(公告)日：2004-10-12
申请号：US10276242
申请日：2002-11-14
申请人： Kyoko Kobayashi , Yuichi Itou , Takayuki Onogi , Akira Uchiyama
发明人： Kyoko Kobayashi , Yuichi Itou , Takayuki Onogi , Akira Uchiyama
IPC分类号： C08L2300
CPC分类号： C08L23/10 , C08L23/142 , C08L23/16 , C08L91/00 , C08L2207/04 , C08L2666/04
摘要： The present invention relates to an olefinic thermoplastic elastomer composition obtainable by dynamically heat treating 5 to 50 parts by weight of a polypropylene resin (A) and 50 to 95 parts by weight of an &agr;-olefinic copolymer (B) having a Mooney viscosity ML1+4 (100° C.) of 60 to 250 in the absence of a crosslinking agent. The olefinic thermoplastic elastomer composition is characterized in that the glass transition temperature (Tg) in dynamic visco-elasticity measurement derived from the polypropylene resin (A) is lower than that of the polypropylene resin (A) itself and that the &agr;-olefinic copolymer (B) is at least one selected from the following (b-1) and (b-2): (b-1) ethylene-&agr;-olefinic copolymers which have an ethylene content of 51 to 60 mol % to the total amount of the ethylene-&agr;-olefinic copolymer-constituting ethylene and &agr;-olefin other than ethylene, (b-2) propylene-&agr;-olefinic copolymers which have a propylene content of 60 to 90 mol % to the total amount of the ethylene-&agr;-olefinic copolymer-constituting propylene and &agr;-olefin other than propylene.
摘要翻译：本发明涉及通过动态热处理5〜50重量份聚丙烯树脂（A）和50〜95重量份具有门尼粘度ML1 +的α-烯烃共聚物（B）的烯烃类热塑性弹性体组合物，在不存在交联剂的情况下，4（100℃）为60至250。烯属热塑性弹性体组合物的特征在于，由聚丙烯树脂（A）得到的动态粘弹性测定中的玻璃化转变温度（Tg）低于聚丙烯树脂（A）本身的玻璃化转变温度（Tg），α-烯烃共聚物 B）为选自以下（b-1）和（b-2）:( b-1）乙烯-α-烯烃共聚物中的至少一种：乙烯含量为51〜60摩尔％乙烯-α-烯烃共聚物构成乙烯和乙烯以外的α-烯烃，（b-2）丙烯-α-烯烃共聚物，丙烯含量为乙烯-α-烯烃共聚物总量的60-90％构成丙烯和丙烯以外的α-烯烃。

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