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1. 发明授权

US08686352B2 Systems and computer program products for mass spectrometry 有权
标题翻译：用于质谱的系统和计算机程序产品
公开(公告)号：US08686352B2
公开(公告)日：2014-04-01
申请号：US13468967
申请日：2012-05-10
申请人： Yohei Kawaguchi , Yuichiro Hashimoto , Masuyuki Sugiyama , Shun Kumano , Shuhei Hashiba , Masahito Togami
发明人： Yohei Kawaguchi , Yuichiro Hashimoto , Masuyuki Sugiyama , Shun Kumano , Shuhei Hashiba , Masahito Togami
IPC分类号： H01J49/26
CPC分类号： H01J49/0031 , H01J49/004
摘要： A mass spectrometry system is mounted with (1) an action planning module for determining a measurement schedule provided by a combination of an MS analysis and an MSn analysis (where n≧2) according to a measuring time provided previously; and (2) a mass spectrometry unit having a tandem mass spectrometry function for outputting a mass spectrum obtained by performing each measurement action constructing the measurement schedule.
摘要翻译：一种质谱系统安装有（1）动作计划模块，用于根据先前提供的测量时间确定由MS分析和MSn分析（其中n≥2）的组合提供的测量计划; 和（2）具有串联质谱分析功能的质谱分析装置，用于输出通过进行构成测定时间表的每个测定动作而得到的质谱。

2. 发明申请

US20120298852A1 SYSTEMS AND COMPUTER PROGRAM PRODUCTS FOR MASS SPECTROMETRY 有权
标题翻译：用于质谱分析的系统和计算机程序产品
公开(公告)号：US20120298852A1
公开(公告)日：2012-11-29
申请号：US13468967
申请日：2012-05-10
申请人： Yohei Kawaguchi , Yuichiro Hashimoto , Masuyuki Sugiyama , Shun Kumano , Shuhei Hashiba , Masahito Togami
发明人： Yohei Kawaguchi , Yuichiro Hashimoto , Masuyuki Sugiyama , Shun Kumano , Shuhei Hashiba , Masahito Togami
IPC分类号： H01J49/26
CPC分类号： H01J49/0031 , H01J49/004
摘要： A mass spectrometry system is mounted with (1) an action planning module for determining a measurement schedule provided by a combination of an MS analysis and an MSn analysis (where n≧2) according to a measuring time provided previously; and (2) a mass spectrometry unit having a tandem mass spectrometry function for outputting a mass spectrum obtained by performing each measurement action constructing the measurement schedule.
摘要翻译：一种质谱系统安装有（1）动作计划模块，用于根据先前提供的测量时间确定由MS分析和MSn分析（其中n≥2）的组合提供的测量计划; 和（2）具有串联质谱分析功能的质谱分析装置，用于输出通过进行构成测定时间表的每个测定动作而得到的质谱。

3. 发明授权

US09076638B2 Mass spectrometer method and mass spectrometer 有权
标题翻译：质谱仪和质谱仪
公开(公告)号：US09076638B2
公开(公告)日：2015-07-07
申请号：US13365355
申请日：2012-02-03
申请人： Masuyuki Sugiyama , Yuichiro Hashimoto , Hideki Hasegawa , Shuhei Hashiba , Shun Kumano
发明人： Masuyuki Sugiyama , Yuichiro Hashimoto , Hideki Hasegawa , Shuhei Hashiba , Shun Kumano
IPC分类号： H01J49/26 , H01J49/00
CPC分类号： H01J49/0031 , H01J49/0045
摘要： A variation in an ionization efficiency and the amount of sample which is introduced into an ion trap is corrected and quantified. Ions of an internal standard and ions of a sample are trapped in the ion trap at the same time, and a concentration of the sample is quantified according to an intensity of the ions of the internal standard which are mass-selectively ejected, and an intensity of fragment ions of the sample.
摘要翻译：电离效率的变化和引入离子阱的样品量被校正和量化。将内标的离子和样品的离子同时捕获在离子阱中，并且根据质量选择性地喷射的内标的离子的强度来量化样品的浓度，强度的样品的碎片离子。

4. 发明申请

US20120326022A1 MASS SPECTROMETER AND MASS ANALYZING METHOD 有权
标题翻译：质谱仪和质谱分析方法
公开(公告)号：US20120326022A1
公开(公告)日：2012-12-27
申请号：US13527627
申请日：2012-06-20
申请人： Shun KUMANO , Masuyuki Sugiyama , Yuichiro Hashimoto , Hideki Hasegawa , Masuyoshi Yamada , Hidetoshi Morokuma , Shuhei Hashiba
发明人： Shun KUMANO , Masuyuki Sugiyama , Yuichiro Hashimoto , Hideki Hasegawa , Masuyoshi Yamada , Hidetoshi Morokuma , Shuhei Hashiba
IPC分类号： H01J49/04
CPC分类号： H01J49/0409 , H01J49/0495
摘要： A mass spectrometer including a sample attaching member of attaching a sample, an ionizing chamber including an introductory port of the sample attaching member and an ionization source of generating a sample ion, a vacuumed chamber having a mass analyzer of analyzing the sample ion, and an opening/closing mechanism provided between the ionizing chamber and the vacuumed chamber, in which the opening/closing mechanism is controlled from a closed state to an open state after introducing the sample attaching member into the ionizing chamber to thereby enable to perform ionization with inconsiderable fragmentation at a high sensitivity with a high throughput
摘要翻译：一种质谱仪，包括附着样品的样品附着构件，包括样品附着构件的入口的电离室和产生样品离子的离子源，具有分析样品离子的质量分析器的真空室，以及设置在离子化室和真空室之间的开/关机构，其中将样品附着构件引入电离室之后，将开/关机构从关闭状态控制到打开状态，从而能够以不可分割的碎片进行电离灵敏度高，吞吐量高

5. 发明授权

US09184037B2 Mass spectrometer and mass analyzing method 有权
标题翻译：质谱仪和质量分析方法
公开(公告)号：US09184037B2
公开(公告)日：2015-11-10
申请号：US13527627
申请日：2012-06-20
申请人： Shun Kumano , Masuyuki Sugiyama , Yuichiro Hashimoto , Hideki Hasegawa , Masuyoshi Yamada , Hidetoshi Morokuma , Shuhei Hashiba
发明人： Shun Kumano , Masuyuki Sugiyama , Yuichiro Hashimoto , Hideki Hasegawa , Masuyoshi Yamada , Hidetoshi Morokuma , Shuhei Hashiba
IPC分类号： H01J49/00 , H01J49/04
CPC分类号： H01J49/0409 , H01J49/0495
摘要： A mass spectrometer including a sample attaching member of attaching a sample, an ionizing chamber including an introductory port of the sample attaching member and an ionization source of generating a sample ion, a vacuumed chamber having a mass analyzer of analyzing the sample ion, and an opening/closing mechanism provided between the ionizing chamber and the vacuumed chamber, in which the opening/closing mechanism is controlled from a closed state to an open state after introducing the sample attaching member into the ionizing chamber to thereby enable to perform ionization with inconsiderable fragmentation at a high sensitivity with a high throughput.
摘要翻译：一种质谱仪，包括附着样品的样品附着构件，包括样品附着构件的入口的电离室和产生样品离子的离子源，具有分析样品离子的质量分析器的真空室，以及设置在离子化室和真空室之间的开/关机构，其中将样品附着构件引入电离室之后，将开/关机构从关闭状态控制到打开状态，从而能够以不可分割的碎片进行电离灵敏度高，吞吐量高。

6. 发明授权

US08710430B2 Mass spectrometry method 有权
标题翻译：质谱法
公开(公告)号：US08710430B2
公开(公告)日：2014-04-29
申请号：US13527619
申请日：2012-06-20
申请人： Masuyuki Sugiyama , Yuichiro Hashimoto , Shun Kumano , Yohei Kawaguchi , Hidetoshi Morokuma
发明人： Masuyuki Sugiyama , Yuichiro Hashimoto , Shun Kumano , Yohei Kawaguchi , Hidetoshi Morokuma
IPC分类号： H01J49/42 , H01J49/26 , H01J49/00
CPC分类号： H01J49/4265 , H01J49/0009 , H01J49/0036
摘要： A mass spectrometry method that corrects the effects from space charge and that achieves both sensitivity and a dynamic range. The mass axis of the mass spectrum is corrected based on the counts of ions accumulated within the ion trap at the point in time each ion was extracted.
摘要翻译：一种校正空间电荷效应并实现灵敏度和动态范围的质谱法。基于在每个离子被提取的时间点内积聚在离子阱内的离子的计数校正质谱的质量轴。

7. 发明授权

US09543135B2 Mass spectrometer and mass analyzing method for efficiently ionizing a sample with less carry-over 有权
标题翻译：质谱分析方法，用于有效地离子化样品，携带较少
公开(公告)号：US09543135B2
公开(公告)日：2017-01-10
申请号：US13562435
申请日：2012-07-31
申请人： Shun Kumano , Masuyuki Sugiyama , Yuichiro Hashimoto , Hideki Hasegawa , Masuyoshi Yamada , Kazushige Nishimura , Hidetoshi Morokuma
发明人： Shun Kumano , Masuyuki Sugiyama , Yuichiro Hashimoto , Hideki Hasegawa , Masuyoshi Yamada , Kazushige Nishimura , Hidetoshi Morokuma
IPC分类号： H01J49/00 , H01J49/04
CPC分类号： H01J49/0431
摘要： A mass spectrometer for efficiently ionizing a sample with less carry-over. The ratio of the amount of sample gas to that of a whole headspace gas is increased by decreasing the pressure inside of a sample vessel in which the sample is sealed thereby efficiently ionizing the sample.
摘要翻译：一种用于有效地电离样品的质谱仪，其携带较少。样品气体与整个顶部空间气体的比例通过降低样品容器的内部压力而增加，其中样品被密封，从而有效地使样品电离。

8. 发明申请

US20140151543A1 ANALYSIS DEVICE AND ANALYSIS METHOD 有权
标题翻译：分析装置和分析方法
公开(公告)号：US20140151543A1
公开(公告)日：2014-06-05
申请号：US13884755
申请日：2011-11-08
申请人： Hisashi Nagano , Yasutaka Suzuki , Hideo Kashima , Yuichiro Hashimoto , Masuyuki Sugiyama , Masakazu Sugaya , Yasunori Doi , Koichi Terada
发明人： Hisashi Nagano , Yasutaka Suzuki , Hideo Kashima , Yuichiro Hashimoto , Masuyuki Sugiyama , Masakazu Sugaya , Yasunori Doi , Koichi Terada
IPC分类号： H01J49/00 , H01J49/04
CPC分类号： H01J49/0422 , G01N1/2211 , G01N1/2214 , G01N33/0057 , G01N2001/028 , H01J49/00 , H01J49/0036 , H01J49/04 , H01J49/0459 , H01J49/0468 , Y02A50/25
摘要： Provided is a technique of analyzing particles in real time while collecting and condensing the particles continuously. Gas and/or particles as a detection target substance that are attached to an authentication target 2 are removed by air flow from a blowing region 5. The removed sample is sucked and is condensed and sampled at a sampling region 10, and ions of the sample are generated at an ion source 21 and are then subjected to mass analysis at a mass analysis region 23. Determination of the obtained mass spectrum is made as to the presence or not of a mass spectrum derived from the detection target substance, and a monitor 27 displays a result thereof. Thereby, the detection target substance attached to the authentication target 2 can be detected continuously in real time, promptly and with a less error rate.
摘要翻译：提供了一种在连续收集和冷凝颗粒时实时分析颗粒的技术。作为检测对象物质的作为检测对象物质的气体和/或颗粒被从吹扫区域5的空气流除去。将取出的样品抽吸并在采样区域10被冷凝并取样，并且样品的离子在离子源21处产生，然后在质量分析区域23进行质量分析。对获得的质谱进行测定，确定是否存在从检测目标物质得到的质谱，以及监测器27 显示其结果。因此，可以实时，及时且误码率较小的连续检测附着于认证对象2的检测对象物质。

9. 发明授权

US07800058B2 Mass spectrometer and mass spectrometry method 有权
标题翻译：质谱仪和质谱法
公开(公告)号：US07800058B2
公开(公告)日：2010-09-21
申请号：US11979811
申请日：2007-11-08
申请人： Masuyuki Sugiyama , Yuichiro Hashimoto , Hideki Hasegawa , Izumi Waki
发明人： Masuyuki Sugiyama , Yuichiro Hashimoto , Hideki Hasegawa , Izumi Waki
IPC分类号： H01J49/00
CPC分类号： H01J49/4225 , H01J49/4215
摘要： A mass spectrometer that is switchable to operate as a linear trap or as a mass filter, and attaining both high ejection efficiency when operated as a linear trap and high mass resolving power when operated as a mass filter. A mass spectrometer includes an ion source for ionizing a sample, a linear trap quadrupole rod lens supplied with ionized ions, a trap electrode for forming a potential to trap the supplied ions between one end of the quadrupole lens and the other end, a control unit to regulate the trap lens voltage, and a mass analyzer or detector to detect ions ejected from the linear trap, and characterized in switching between an operation where the supplied ions are trapped in a section quadrupole rod lens and ejected by the controller unit regulating the trap electrode voltage; and an operation where ions are selective passed through according to their mass. The ejection efficiency when operated as an ion trap, and the mass resolving power when operated as a quadrupole mass filter are vastly improved compared to conventional methods.
摘要翻译：可以切换为线性捕集器或质量过滤器的质谱仪，当作为质量过滤器操作时，作为线性捕集器操作时获得高喷射效率和高质量分辨能力的质谱仪。质谱仪包括用于电离样品的离子源，提供有离子化离子的线性捕获四极杆透镜，用于形成用于捕获四极透镜的一端与另一端之间的供应离子的电位的捕获电极，控制单元调节陷波透镜电压，以及质量分析器或检测器，用于检测从线性阱捕获的离子，并且其特征在于，在所提供的离子被捕获在四极杆棒状透镜中并由调节阱的控制器单元喷射的操作之间进行切换电极电压; 以及根据其质量选择性地通过离子的操作。当作为离子阱操作时的喷射效率以及当作为四极质量过滤器操作时的质量分辨能力与常规方法相比大大提高。

10. 发明申请

US20080121795A1 Mass spectrometer and mass spectrometry method 有权
标题翻译：质谱仪和质谱法
公开(公告)号：US20080121795A1
公开(公告)日：2008-05-29
申请号：US11979811
申请日：2007-11-08
申请人： Masuyuki Sugiyama , Yuichiro Hashimoto , Hideki Hasegawa , Izumi Waki
发明人： Masuyuki Sugiyama , Yuichiro Hashimoto , Hideki Hasegawa , Izumi Waki
IPC分类号： H01J49/42
CPC分类号： H01J49/4225 , H01J49/4215
摘要： A mass spectrometer that is switchable to operate as a linear trap or as a mass filter, and attaining both high ejection efficiency when operated as a linear trap and high mass resolving power when operated as a mass filter. A mass spectrometer includes an ion source for ionizing a sample, a linear trap quadrupole rod lens supplied with ionized ions, a trap electrode for forming a potential to trap the supplied ions between one end of the quadrupole lens and the other end, a control unit to regulate the trap lens voltage, and a mass analyzer or detector to detect ions ejected from the linear trap, and characterized in switching between an operation where the supplied ions are trapped in a section quadrupole rod lens and ejected by the controller unit regulating the trap electrode voltage; and an operation where ions are selective passed through according to their mass. The ejection efficiency when operated as an ion trap, and the mass resolving power when operated as a quadrupole mass filter are vastly improved compared to conventional methods.
摘要翻译：可以切换为线性捕集器或质量过滤器的质谱仪，当作为质量过滤器操作时，作为线性捕集器操作时获得高喷射效率和高质量分辨能力的质谱仪。质谱仪包括用于电离样品的离子源，提供有离子化离子的线性捕获四极杆透镜，用于形成用于捕获四极透镜的一端与另一端之间的供应离子的电位的捕获电极，控制单元调节陷波透镜电压，以及质量分析器或检测器，用于检测从线性阱捕获的离子，并且其特征在于，在所提供的离子被捕获在四极杆棒状透镜中并由调节阱的控制器单元喷射的操作之间进行切换电极电压; 以及根据其质量选择性地通过离子的操作。当作为离子阱操作时的喷射效率以及当作为四极质量过滤器操作时的质量分辨能力与常规方法相比大大提高。

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