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1. 发明授权

US4868226A Process for producing filler-containing polypropylene resin composition 失效
标题翻译：用于生产含填料的聚丙烯树脂组合物的方法
公开(公告)号：US4868226A
公开(公告)日：1989-09-19
申请号：US180931
申请日：1988-04-13
申请人： Tatsuyuki Mitsuno , Hideo Shinonaga , Akio Daimon
发明人： Tatsuyuki Mitsuno , Hideo Shinonaga , Akio Daimon
IPC分类号： C08K3/00 , C08L23/08 , C08L23/10 , C08L51/06
CPC分类号： C08L23/10 , C08K3/0033 , C08L53/00 , C08L23/0869 , C08L51/06
摘要： A process for producing a filler-containing polypropylene resin composition is disclosed. The composition comprises (a) from 27 to 87% by weight of a polypropylene resin, (b) from 3 to 15% by weight of a modified polypropylene resin containing from 0.1 to 3 mol% of an unsaturated dicarboxylic acid anhydride repeating unit, (c) from 5 to 30% by weight of an ethylene copolymer composed of from 82 to 98.7 mol% of an ethylene repeating unit, from 1 to 15 mol% of an ester repeating unit selected from alkyl acrylates and alkyl methacrylates having from 1 to 8 carbon atoms in the alkyl moiety thereof, and from 0.3 to 3 mol% of an unsaturated dicarboxylic acid anhydride repeating unit, and (d) from 5 to 40% by weight of a filler. The process comprises melt-mixing the components (a), (b), and (d) and then melt-mixing the resulting mixture with the component (c). The resin compositon exhibits excellent finishing properties, such as adhesion, coating properties, and printability, as well as improved rigidity and thermal properties.

2. 发明授权

US4946896A Thermoplastic elastomer composition 失效
标题翻译：热塑性弹性体组合物
公开(公告)号：US4946896A
公开(公告)日：1990-08-07
申请号：US265845
申请日：1988-11-01
申请人： Tatsuyuki Mitsuno , Hideo Shinonaga , Akio Daimon
发明人： Tatsuyuki Mitsuno , Hideo Shinonaga , Akio Daimon
IPC分类号： C08L23/08 , C08L7/00 , C08L21/00 , C08L23/00 , C08L23/10 , C08L23/16 , C08L33/00 , C08L33/02 , C08L51/00 , C08L51/02 , C08L77/00 , C08L101/00
CPC分类号： C08L23/10 , C08L23/16 , B41M5/5254 , C08L2205/03 , C08L23/0869 , C08L2312/00
摘要： There is provided a thermoplastic elastomer composition having excellent surface processabilities such as adhesion, paintability and printability together with impact resistance. This composition comprises (A) 20-80% by weight of a polypropylene resin, (B) 5-38% by weight of an ethylene copolymer having 82-98.7 mol % of an ethylene unit, 1-15 mol % of an ester unit selected from alkyl acrylate and methacrylate having an alkyl group of 1-8 carbon atoms and 0.3-3 mol % of an unsaturated dicarboxylic acid anhydride unit and (C) 5-70% by weight of ethylene-propylene and/or ethylene-propylene-non-conjugated diene copolymer rubber which contain 50-85 mol % of an ethylene unit and have a Mooney viscosity at 100.degree. C. of 20-100 and an iodine value of 20 or less.
摘要翻译：提供了具有优异的表面加工性的热塑性弹性体组合物，例如粘合性，可着色性和可印性以及抗冲击性。该组合物包含（A）20-80重量％的聚丙烯树脂，（B）5-38重量％的具有82-98.7摩尔％乙烯单元的乙烯共聚物，1-15摩尔％的酯单元选自具有1-8个碳原子的烷基和0.3-3mol％的不饱和二羧酸酐单元的丙烯酸酯和甲基丙烯酸烷基酯和（C）5-70重量％的乙烯 - 丙烯和/或乙烯 - 丙烯 - 非共轭二烯共聚物橡胶，其包含50-85mol％的乙烯单元，并且在100℃下的门尼粘度为20-100，碘值为20或更小。

3. 发明授权

US4764546A Filler-containing polypropylene resin composition and process for producing the same 失效
标题翻译：含填料的聚丙烯树脂组合物及其制造方法
公开(公告)号：US4764546A
公开(公告)日：1988-08-16
申请号：US41514
申请日：1987-04-23
申请人： Tatsuyuki Mitsuno , Hideo Shinonaga , Akio Daimon
发明人： Tatsuyuki Mitsuno , Hideo Shinonaga , Akio Daimon
IPC分类号： C08K3/00 , C08L23/08 , C08L23/10 , C08L51/06 , C08K3/34 , C08K9/06 , C08L35/00
CPC分类号： C08L23/10 , C08K3/0033 , C08L53/00 , C08L23/0869 , C08L51/06
摘要： A filler-containing polypropylene resin composition and a process for producing the same are disclosed. The composition comprises (a) from 27 to 87% by weight of a polypropylene resin, (b) from 3 to 15% by weight of a modified polypropylene resin containing from 0.1 to 3 mol % of an unsaturated dicarboxylic acid anhydride repeating unit, (c) from 5 to 30% by weight of an ethylene copolymer composed of from 82 to 98.7 mol % of an ethylene repeating unit, from 1 to 15 mol % of an ester repeating unit selected from alkyl acrylates and alkyl methacrylates having from 1 to 8 carbon atoms in the alkyl moiety thereof, and from 0.3 to 3 mol % of an unsaturated dicarboxylic acid anhydride repeating unit, and (d) from 5 to 40% by weight of a filler. The process comprises melt-mixing the components (a), (b) and (d) and then melt-mixing the resulting mixture with the component (c). The resin composition exhibits excellent finishing properties, such as adhesion, coating properties, and printability, as well as improved rigidity and thermal properties.
摘要翻译：公开了一种含填料的聚丙烯树脂组合物及其制造方法。组合物包含（a）27〜87重量％的聚丙烯树脂，（b）3〜15重量％的含有0.1〜3摩尔％的不饱和二羧酸酐重复单元的改性聚丙烯树脂（ c）5〜30重量％的由82〜98.7摩尔％乙烯重复单元构成的乙烯共聚物，1〜15摩尔％的选自丙烯酸烷基酯和1〜8个碳酸甲基丙烯酸酯的酯重复单元其烷基部分为碳原子，0.3〜3摩尔％的不饱和二羧酸酐重复单元，（d）5〜40重量％的填料。该方法包括熔融混合组分（a），（b）和（d），然后将所得混合物与组分（c）熔融混合。树脂组合物表现出优异的整理性能，例如粘合性，涂布性能和可印刷性，以及改善的刚性和热性能。

4. 发明授权

US4902738A Thermoplastic elastomer composition and process for producing same 失效
标题翻译：热塑性弹性体组合物及其制备方法
公开(公告)号：US4902738A
公开(公告)日：1990-02-20
申请号：US277864
申请日：1988-11-30
申请人： Tatsuyuki Mitsuno , Hideo Shinonaga , Akio Daimon , Satoru Hosoda
发明人： Tatsuyuki Mitsuno , Hideo Shinonaga , Akio Daimon , Satoru Hosoda
IPC分类号： C08K5/00 , C08F255/00 , C08J3/24 , C08K5/14 , C08K5/34 , C08K5/35 , C08L23/00 , C08L23/02 , C08L23/16 , C08L89/00
CPC分类号： C08F255/00
摘要： A thermoplastic elastomer composition which is excellent in melt-flowability and is able to afford injection molded articles superior in appearance is provided, which is a mixture comprising (A) 20-50 parts by weight of an olefinic copolymer rubber, (B) 50-80 parts by weight of an olefinic plastic having a ratio of melt index M.sub.1 /M.sub.0 of 2-50 wherein M.sub.0 is a melt index of the plastic before subjected to thermal decomposition with organic peroxide and M.sub.1 is a melt index of the plastic after subjected to the thermal decomposition with the organic peroxide, sum of (A) and (B) being 100 parts by weight, (C) 5-25 parts by weight of a mineral oil and (D) 0.1-3 parts by weight of a bismaleimide compound, said mixture being dynamically heat treated with (E) an organic peroxide after bismaleimide compound (D) is homogeneously dispersed in the mixture.
摘要翻译：提供熔体流动性优异并且能够提供外观优异的注塑制品的热塑性弹性体组合物，其是包含（A）20-50重量份的烯烃共聚物橡胶，（B）50- 80重量份熔体指数M1 / M0比为2-50的烯烃塑料，其中M0是在用有机过氧化物进行热分解之前的塑料的熔体指数和M1是经受的塑料的熔体指数有机过氧化物的热分解（A）和（B）之和为100重量份，（C）5-25重量份矿物油和（D）0.1-3重量份双马来酰亚胺化合物，在双马来酰亚胺化合物（D）均匀分散在混合物中后，所述混合物用（E）有机过氧化物动态热处理。

5. 发明授权

US4686257A Polypropylene resin composition containing filler 失效
标题翻译：含有填料的聚丙烯树脂组合物
公开(公告)号：US4686257A
公开(公告)日：1987-08-11
申请号：US889533
申请日：1986-07-25
申请人： Tatsuyuki Mitsuno , Teruhisa Koyama , Hideo Shinonaga , Akio Daimon
发明人： Tatsuyuki Mitsuno , Teruhisa Koyama , Hideo Shinonaga , Akio Daimon
IPC分类号： C08L23/00 , C08K3/00 , C08K3/24 , C08K3/34 , C08K7/00 , C08K7/02 , C08L23/08 , C08L23/10 , C08L33/00 , C08L33/02 , C08L51/00 , C08L51/02 , C08L53/00 , C08L77/00 , C08L101/00 , C08L35/00 , C08L37/00
CPC分类号： C08K3/34 , C08L23/10 , C08L23/0869
摘要： A filler-containing polypropylene resin composition is disclosed, comprising (a) from 30 to 90% by weight of a polypropylene resin, (b) from 2.5 to 38% by weight of an ethylene copolymer composed of from 82 to 98.7 mol % of ethylene, from 1 to 15 mol % of an ester selected from alkyl acrylate and alkyl methacrylates having from 1 to 8 carbon atoms in the alkyl moiety thereof and from 0.3 to 3 mol % of an unsaturated dicarboxylic acid anhydride, and (c) from 5 to 50% by weight of a filler. Molded products obtained from the composition have improved finishing properties, such as adhesion, coating properties, printability, and the like.
摘要翻译：公开了一种含填料的聚丙烯树脂组合物，其包含（a）30至90重量％的聚丙烯树脂，（b）2.5至38重量％的由82至98.7摩尔％的乙烯组成的乙烯共聚物，1〜15摩尔％的选自丙烯酸烷基酯和其烷基部分具有1〜8个碳原子的甲基丙烯酸烷基酯和0.3〜3摩尔％的不饱和二羧酸酐的酯，和（c）5〜 50重量％的填料。从组合物获得的成型品具有改进的整理性能，例如粘合性，涂层性能，可印刷性等。

6. 发明授权

US5260366A Thermoplastic elastomer composition and process for producing same 失效
标题翻译：热塑性弹性体组合物及其制备方法
公开(公告)号：US5260366A
公开(公告)日：1993-11-09
申请号：US742499
申请日：1991-08-05
申请人： Tatsuyuki Mitsuno , Hideo Shinonaga , Masashi Yamamoto
发明人： Tatsuyuki Mitsuno , Hideo Shinonaga , Masashi Yamamoto
IPC分类号： C08L23/10 , C08L53/02 , C08K3/26
CPC分类号： C08L53/025 , C08L23/10 , C08L53/00 , C08L53/02 , C08L2205/03 , C08L2207/04 , C08L23/12 , C08L91/00
摘要： A thermoplastic elastomer composition superior in moldability and appearance, little in anisotropy of mechanical properties, especially, tensile strength and retaining low temperature impact strength, is obtained by previously melt-kneading an intermediate composition comprising (a) 100 parts by weight of a selectively hydrogenated block copolymer which has at least two mono-alkenyl or mono-alkenylidene aromatic hydrocarbon polymer blocks A having a number-average molecular weight of 25,000-35,000 and at least one partially or completely hydrogenated aliphatic conjugated diene hydrocarbon polymer block B having a number-average molecular weight of 100,000-150,000, (b) 50-150 parts by weight of an extender oil and (c) 0-50 parts by weight of polypropylene I, then adding, to the kneaded intermediate composition, (d) polypropylene II containing at least 35% by weight of a propylene-ethylene block copolymer having a melt flow rate of 10-30 g/10 min. and an ethylene content of 3-15% by weight in such amount that total amount of polypropylene I plus polypropylene II is 200-400 parts by weight per 100 parts by weight of block copolymer (a) and then further melt kneading the mixture. Further addition of a filler to the composition can afford a thermoplastic elastomer composition of small linear expansion coefficient with retaining the above properties.
摘要翻译：通过预先将包含（a）100重量份的选择性氢化的中间体组合物熔融捏合，得到成型性和外观优异的机械性能，特别是拉伸强度和保持低温冲击强度几何异形性的热塑性弹性体组合物嵌段共聚物，其具有至少两个数均分子量为25,000-35,000的单烯基或单亚烯基芳族烃聚合物嵌段A和至少一种部分或完全氢化的脂族共轭二烯烃聚合物嵌段B，其具有数均分子量分子量为100,000-150,000，（b）50-150重量份的增量油和（c）0-50重量份的聚丙烯I，然后向捏合的中间体组合物中加入（d）含有至少35重量％的熔体流动速率为10-30克/ 10分钟的丙烯 - 乙烯嵌段共聚物。并且乙烯含量为3-15重量％，其量使得每100重量份嵌段共聚物（a）的聚丙烯I加聚丙烯II的总量为200-400重量份，然后进一步熔融捏合该混合物。向组合物中进一步添加填料可以提供具有小的线膨胀系数的热塑性弹性体组合物，并保持上述性能。

7. 发明授权

US5077082A Method of treating surface of shaped body formed of polypropylene resin 失效
标题翻译：处理形成聚丙烯树脂的成型体表面的方法
公开(公告)号：US5077082A
公开(公告)日：1991-12-31
申请号：US506085
申请日：1990-04-09
申请人： Koichiroh Katoh , Tatasuyuki Mitsuno , Hideo Shinonaga , Akio Daimon
发明人： Koichiroh Katoh , Tatasuyuki Mitsuno , Hideo Shinonaga , Akio Daimon
IPC分类号： B05D3/06 , B05D3/10 , B05D7/02 , B05D7/24 , B29C35/08 , B29C59/16 , B29C65/48 , B29C71/00 , B29K23/00 , C08J7/00 , C08J7/02 , C08L23/16 , C08L53/00
CPC分类号： C08L23/16 , B29C59/16 , B29C71/0009 , C08L23/10 , C08L53/00 , B29C2035/0827
摘要： A shaped body formed of a polypropylene resin is surface-treated by a method which includes the steps of:providing a shaped body formed of a composition containing (A) 5-95% by weight of a specific propylene-ethylene block copolymer and (B) 5-95% by weight of a specific ethylene-propylene copolymer rubber;contacting a surface of the shaped body with a UV-ray absorbing liquid at a temperature and for a period of time sufficient to swell the surface; andirradiating UV rays having wavelengths of 300 nm or less on the swollen surface thereby increasing the surface energy of the surface of the shaped body. The thus treated shaped body is ready for coating with a coating material.
摘要翻译：由聚丙烯树脂形成的成形体通过包括以下步骤的方法进行表面处理：提供由包含（A）5-95重量％的特定丙烯 - 乙烯嵌段共聚物和（B ）5-95重量％的特定乙烯 - 丙烯共聚物橡胶; 在足以使表面膨胀的温度和一段时间内使成形体的表面与紫外线吸收液体接触; 并且在波长表面上照射波长为300nm以下的紫外线，从而增加成形体表面的表面能。如此处理的成形体准备涂覆涂层材料。

8. 发明授权

US5296273A Coating method for polypropylene resin moldings 失效
标题翻译：聚丙烯树脂模塑制品的涂布方法
公开(公告)号：US5296273A
公开(公告)日：1994-03-22
申请号：US794881
申请日：1991-11-20
申请人： Hiroomi Abe , Hideo Shinonaga , Kyoji Suzuki , Satoru Sogabe
发明人： Hiroomi Abe , Hideo Shinonaga , Kyoji Suzuki , Satoru Sogabe
IPC分类号： B05D7/02 , B05D3/06 , B05D7/00 , C08J7/00 , C08J7/04 , B05D1/36 , B05D3/02 , B05D7/26
CPC分类号： B05D7/52 , B05D3/063 , B05D3/065 , C08J7/047 , C08J2323/12
摘要： A method for coating a polypropylene resin molding is disclosed, comprising irradiating the surface of a molding of a polypropylene resin selected from a polypropylene and a propylene-ethylene block copolymer with an ultraviolet light having an irradiating wavelength in the region of 300 nm or less, coating the irradiated surface with a primer, and further coating the coated surface with a coating material. A method for coating a polypropylene resin molding is also disclosed, comprising coating the surface of a molding of a polypropylene resin selected from a polypropylene and a propylene-ethylene block copolymer with a primer, irradiating the coated surface with an ultraviolet light having an irradiating wavelength in the region of 300 nm or less, and further coating the irradiated surface with a coating material.
摘要翻译：公开了一种涂布聚丙烯树脂成型体的方法，包括用300nm以下的区域照射波长的紫外线照射选自聚丙烯和丙烯 - 乙烯嵌段共聚物的聚丙烯树脂的成型体的表面，用底漆涂覆照射的表面，并用涂料进一步涂覆涂覆的表面。还公开了一种用于涂布聚丙烯树脂模制品的方法，包括用引物涂布选自聚丙烯和丙烯 - 乙烯嵌段共聚物的聚丙烯树脂的模塑品的表面，用涂覆表面照射具有照射波长的紫外线在300nm以下的区域，进一步用被覆材料涂布被照射的面。

9. 发明授权

US4166079A Dyeable polyolefin composition 失效
标题翻译：可变聚烯烃组合物
公开(公告)号：US4166079A
公开(公告)日：1979-08-28
申请号：US866402
申请日：1977-12-30
申请人： Yoshiharu Tatsukami , Hazime Nishibara , Yasutoshi Kobayashi , Hideo Shinonaga
发明人： Yoshiharu Tatsukami , Hazime Nishibara , Yasutoshi Kobayashi , Hideo Shinonaga
IPC分类号： C08F8/32 , C08G59/14 , C08L23/02
CPC分类号： C08G59/1477 , C08F8/32 , C08G59/1433 , C08K5/17 , C08L23/02 , C08L23/10
摘要： A method for producing aminated copolymers by aminating ethylene-glycidyl acrylates copolymers, which comprises conducting the amination in a heterogeneous system using a mixed solvent of an amine and a lower alcohol, and a dyeable polyolefin composition comprising the said aminated copolymer and polyolefin.

10. 发明授权

US5585187A Methods for surface treating and paint-coating resin composition molded articles and paint-coated article obtained by said method for paint-coating 失效
标题翻译：表面处理和涂漆树脂组合物模塑制品的方法和通过所述涂料方法获得的涂料制品
公开(公告)号：US5585187A
公开(公告)日：1996-12-17
申请号：US440059
申请日：1995-05-12
申请人： Hideo Shinonaga , Satoru Sogabe
发明人： Hideo Shinonaga , Satoru Sogabe
IPC分类号： C08L53/00 , B32B9/00
CPC分类号： C08L53/00 , Y10T428/251 , Y10T428/31562 , Y10T428/31587 , Y10T428/31696 , Y10T428/31938
摘要： The present invention relates to;a method for surface treating a polypropylene resin composition molded article, which comprises irradiating a molded article with ultraviolet light having an irradiation wavelength of 300 nm or less, said molded article being obtained from a polypropylene resin composition which comprises:(A) 15-92% by weight of a crystalline propylene-ethylene block copolymer resin,(B) 5-40% by weight of an ethylene-propylene copolymer rubber,(C) 1-15% by weight of a hydroxyl group-containing propylene oligomer, and(D) 2-30% by weight of an inorganic filler;a method for paint-coating a polypropylene resin composition molded article, which comprises irradiating a molded article with ultraviolet light having an irradiation wavelength of 300 nm or less and coating the irradiated surface with a paint, said molded article being obtained from a polypropylene resin composition which comprises said components (A), (B), (C) and (D) above-mentioned; anda paint-coated article obtained by said method for paint-coating the polypropylene resin composition molded article.According to the present invention, the methods for surface treating and paint-coating the polypropylene resin composition molded article, which gives excellent paint-coatability and adhesion property of said molded article, and the paint-coated article, which is useful and suited especially for automotive exterior parts such as a bumper and an instrument panel, obtained by said method for paint-coating may be provided.
摘要翻译：本发明涉及一种用于表面处理聚丙烯树脂组合物模制品的方法，其包括用模制品照射具有300nm或更小的照射波长的紫外光，所述模制品由聚丙烯树脂组合物获得，所述聚丙烯树脂组合物包含：（A）15-92 （B）5-40重量％的乙烯 - 丙烯共聚物橡胶，（C）1-15重量％的含羟基丙烯低聚物和（ D）2-30重量％的无机填料; 一种涂布聚丙烯树脂组合物成型体的方法，其特征在于，包括用模制品对具有300nm以下的照射波长的紫外线照射并用涂料涂布所述照射面，所述成型体由聚丙烯树脂组合物其包含上述组分（A），（B），（C）和（D）; 以及通过所述涂布所述聚丙烯树脂组合物成型品的方法得到的涂漆制品。根据本发明，对聚丙烯树脂组合物成型体进行表面处理和涂漆的方法，其具有优异的所述成型体的涂漆性和粘合性，以及涂料制品，其特别适用于可以提供通过所述涂漆方法获得的汽车外部部件，例如保险杠和仪表板。

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