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1. 发明授权

US5677408A Propylene elastomer and process for preparation thereof 失效
标题翻译：丙烯弹性体及其制备方法
公开(公告)号：US5677408A
公开(公告)日：1997-10-14
申请号：US448502
申请日：1995-06-05
申请人： Takashi Ueda , Akira Mizuno , Masaaki Kawasaki , Daisuke Fukuoka , Yoshihisa Kiso , Tatsuya Tanizaki , Mikio Hashimoto , Masahiro Sugi , Toshiyuki Tsutsui
发明人： Takashi Ueda , Akira Mizuno , Masaaki Kawasaki , Daisuke Fukuoka , Yoshihisa Kiso , Tatsuya Tanizaki , Mikio Hashimoto , Masahiro Sugi , Toshiyuki Tsutsui
IPC分类号： C07C45/46 , C07C49/67 , C07C49/697 , C07F17/00 , C08F4/619 , C08F4/6192 , C08F4/639 , C08F4/6392 , C08F4/642 , C08F4/659 , C08F4/6592 , C08F10/00 , C08F10/06 , C08F110/06 , C08F210/06 , C08F210/16 , C08F210/08
CPC分类号： C08F210/16 , C07C45/46 , C07C49/67 , C07C49/697 , C07F17/00 , C08F10/00 , C08F10/06 , C08F110/06 , C08F210/06 , C08F4/61908 , C08F4/61912 , C08F4/61927 , C08F4/63912 , C08F4/63927 , C08F4/65908 , C08F4/65912 , C08F4/65916 , C08F4/65927 , Y10S526/943
摘要： The novel propylene elastomer according to the invention contains (1) units derived from propylene in amounts of 50 to 95% by mol and units derived from 1-butene in amounts of 5 to 50% by mol, and has (2) triad tacticity (mm fraction), determined by the .sup.13 C-NMR spectrum (hexachlorobutadiene solution, based on tetramethylsilane), of not less than 90%, (3) an intrinsic viscosity (in decalin at 135.degree. C.) of 0.1 to 12 dl/g, (4) a molecular weight distribution (Mw/Mn) of not more than 3 and (5) a randomness parameter B value of 1.0 to 1.5, preferably 1.0 to 1.3. In addition, the elastomer desirably has properties that (6) the elastomer has a melting point Tm of 60.degree. to 140.degree. C., and the melting point Tm and a 1-butene constituent unit content M (% by mol) in the elastomer satisfy the relation -2.6M+130.ltoreq.Tm.ltoreq.-2.3M+155, and (7) a crystallinity C of the elastomer measured by X-ray diffractometry and the 1-butene constituent unit content M (% by mol) satisfy the relation C.ltoreq.-1.5M+75. Such propylene elastomer is excellent in rigidity, heat resistance, scratch resistance, transparency, heat sealing properties and blocking resistance. The propylene elastomer can be prepared using a specific transition metal compound catalyst.
摘要翻译： PCT No.PCT / JP94 / 01997 371日期：1995年6月5日 102（e）日期1995年6月5日PCT 1994年11月29日PCT PCT。公开号WO95 / 14717 日期1995年6月1日根据本发明的新型丙烯弹性体含有（1）量为50〜95摩尔％的来自丙烯的单元和5-50摩尔％的来自1-丁烯的单元，并且具有（ 2）通过13 C-NMR光谱（六氯丁二烯溶液，基于四甲基硅烷）测定的三单元组立构规整度（mm分数）不小于90％，（3）特性粘度（在135℃的十氢化萘中）为0.1〜 12dl / g，（4）分子量分布（Mw / Mn）为3以下，（5）无规参数B值为1.0〜1.5，优选为1.0〜1.3。此外，弹性体理想地具有以下性质：（6）弹性体的熔点Tm为60〜140℃，熔点Tm和1-丁烯构成单元含量M（摩尔％）在弹性体中满足-2.6M + 130

2. 发明授权

US5998039A Polypropylene composition and uses thereof 失效
标题翻译：聚丙烯组合物及其用途
公开(公告)号：US5998039A
公开(公告)日：1999-12-07
申请号：US890360
申请日：1997-07-09
申请人： Tatsuya Tanizaki , Mikio Hashimoto , Masahiro Sugi , Toshiyuki Tsutsui , Yasuo Tanaka , Mamoru Kagami
发明人： Tatsuya Tanizaki , Mikio Hashimoto , Masahiro Sugi , Toshiyuki Tsutsui , Yasuo Tanaka , Mamoru Kagami
IPC分类号： C08F210/06 , C08L23/10 , C08L23/12 , C08L23/14 , B32B27/32
CPC分类号： C08L23/12 , C08L23/10 , C08L23/14 , C08L23/142 , C08F210/06 , C08L2205/02 , Y10S428/91 , Y10T428/1328 , Y10T428/31909 , Y10T428/31913
摘要： Disclosed is a polypropylene composition comprising (A) polypropylene and (B) a specific propylene-1-butene random copolymer in a specific amount ratio. The propylene-1-butene random copolymer (B) is characterized in that: (1) the copolymer contains 50 to 95% by mol of constituent units from propylene and 50 to 5% by mol of constituent units from 1-butene, (2) the intrinsic viscosity, as measured in decahydronaphthalene at 135.degree. C., is in the range of 0.1 to 12 dl/g, (3) the molecular weight distribution (Mw/Mn), as determined measured by GPC, is not more than 3, and (4) the parameter B value indicating randomness of the copolymerized monomer sequence distribution is in the range of 1.0 to 1.5. Also disclosed is a polypropylene composite film comprising (I) a crystalline polypropylene layer and (II) a layer formed from the polypropylene composition, which is laminated on at least one surface of the crystalline polypropylene layer (I). The polypropylene composition is excellent in heat resistance and low-temperature heat-sealing properties as well as in flexibility and impact resistance. The polypropylene composite film is excellent in not only heat-sealing properties, particularly low-temperature heat-sealing properties, but also transparency, scratch resistance and blocking resistance.
摘要翻译：公开了包含（A）聚丙烯和（B）特定量比的特定丙烯-1-丁烯无规共聚物的聚丙烯组合物。丙烯-1-丁烯无规共聚物（B）的特征在于：（1）共聚物含有50〜95摩尔％的丙烯构成单元和50〜5摩尔％的来自1-丁烯的构成单元，（2 ），在135℃下在十氢化萘中测得的特性粘度在0.1〜12dl / g的范围内，（3）通过GPC测定的分子量分布（Mw / Mn）不大于 3，（4）表示共聚单体序列分布的随机性的参数B值在1.0〜1.5的范围内。还公开了一种聚丙烯复合膜，其包含（I）结晶聚丙烯层和（II）由聚丙烯组合物形成的层，其层压在结晶聚丙烯层（I）的至少一个表面上。聚丙烯组合物的耐热性和低温热封性以及柔软性和耐冲击性优异。聚丙烯复合膜不仅具有优异的热封性，特别是低温热封性，而且透明性，耐擦伤性和耐粘连性优异。

3. 发明授权

US5610254A Ethylene-.alpha.-olefin-nonconjugated polyene random copolymer, rubber composition, and process for preparing the random copolymer 失效
标题翻译：乙烯-α-烯烃 - 非共轭多烯无规共聚物，橡胶组合物和制备无规共聚物的方法
公开(公告)号：US5610254A
公开(公告)日：1997-03-11
申请号：US574684
申请日：1995-12-19
申请人： Toshihiro Sagane , Toshiyuki Tsutsui , Masaaki Kawasaki , Keiji Okada , Tetsuo Tojo , Tatsuya Tanizaki
发明人： Toshihiro Sagane , Toshiyuki Tsutsui , Masaaki Kawasaki , Keiji Okada , Tetsuo Tojo , Tatsuya Tanizaki
IPC分类号： C08F4/64 , C08F4/642 , C08F4/659 , C08F4/6592 , C08F210/18 , C08L23/16 , C08F236/20 , C08F232/06
CPC分类号： C08F210/18 , C08L23/16 , C08F4/65912 , C08F4/65927 , C08L2312/00 , Y10S526/943
摘要： Disclosed is an ethylene-.alpha.-olefin-nonconjugated polyene random copolymer which is a random copolymer of (a) ethylene, (b) an .alpha.-olefin of 3 or more carbon atoms and (c) a nonconjugated polyene, and has such properties that (i) the copolymer contains (a) units derived from ethylene and (b) units derived from the .alpha.-olefin of 3 or more carbon atoms in a molar ratio of 40/60 to 95/5 ((a)/(b)), (ii) the iodine value is in the range of 1 to 50, (iii) the intrinsic viscosity (.eta.), as measured in decahydronaphthalene at 135.degree. C., is in the range of 0.1 to 8.0 dl/g, and (iv) the ratio g.eta.* of the intrinsic viscosity (.eta.) of the copolymer defined above to the intrinsic viscosity (.eta.).sub.blank of a linear ethylene-propylene copolymer having the same weight-average molecular weight as the ethylene-.alpha.-olefin-nonconjugated polyene random copolymer and having an ethylene content of 70% by mol, (.eta.)/(.eta.).sub.blank, is in the range of 0.2 to 0.9 or the ratio g' of the intrinsic viscosity (.eta.) of said random copolymer defined above to the intrinsic viscosity (.eta.).sub.blank' of a linear ethylene-propylene copolymer having an ethylene content of 70% by mol which is determined by measurement of gel permeation chromatography (GPC) of ethylene-.alpha.-olefin-nonconjugated polyene random copolymer in orthodichlorobenzene at 140.degree. C., (.eta.)/(.eta.).sub.blank', is in the reange of 0.2 to 0.9.
摘要翻译：公开了一种乙烯-α-烯烃 - 非共轭多烯无规共聚物，它是（a）乙烯，（b）3个或更多个碳原子的α-烯烃和（c）非共轭多烯的无规共聚物，（i）共聚物包含（a）衍生自乙烯的单元和（b）衍生自摩尔比为40/60至95/5（（a）/（b）的3个或更多个碳原子的α-烯烃的单元）），（ii）碘值在1〜50的范围内，（iii）在135℃下在十氢化萘中测定的特性粘度（η）为0.1〜8.0dl / g，（iv）上述共聚物的特性粘度（eta）与具有与乙烯-α-烯烃相同的重均分子量的直链乙烯 - 丙烯共聚物的特性粘度（η）空白的比率g eta * 非共轭多烯无规共聚物的乙烯含量为70摩尔％（eta）/（η）空白，在0.2〜0.9的范围内或者int的比例g' 所述上述无规共聚物的特性粘度（η）为乙烯含量为70摩尔％的线性乙烯 - 丙烯共聚物的特性粘度（η）空白'，其通过乙烯的凝胶渗透色谱（GPC） α-烯烃 - 非共轭多烯无规共聚物在140℃，（η）/（η）空白'的邻二氯苯中的摩尔比为0.2-0.9。

4. 发明授权

US06265083B1 Poly (4-methyl-1-pentene) resin laminates and uses thereof 失效
标题翻译：聚（4-甲基-1-戊烯）树脂层合物及其用途
公开(公告)号：US06265083B1
公开(公告)日：2001-07-24
申请号：US09147961
申请日：1999-03-24
申请人： Tatsuya Tanizaki , Takashi Nakahara , Mineo Kubo
发明人： Tatsuya Tanizaki , Takashi Nakahara , Mineo Kubo
IPC分类号： B32B2732
CPC分类号： B32B27/08 , B32B7/12 , B32B27/32 , B32B2323/04 , B32B2323/10 , B32B2439/00 , Y10T428/31909 , Y10T428/31913
摘要： A poly-4-methyl-1-pentene resin laminate excellent in not only heat sealing properties and oxygen gas permeability but also blocking resistance is provided. The poly-4-methyl-1-pentene resin laminate comprises a layer made of a 4-methyl-1-pentene polymer (A), an intermediate layer made of an adhesive resin composition (B) and a layer made of a propylene polymer composition (C) comprising 60 to 90 parts by weight of a propylene polymer (c-1) and 10 to 40 parts by weight of a 1-butene polymer (c-2), the total amount of said components (c-1) and (c-2) being 100 parts by weight. This poly-4-methyl-1-pentene resin laminate can be used as a material of freshness-keeping packaging media and culture containers. Also provided is a poly-4-methyl-1-pentene resin laminate having excellent peel resistance and capable of being easily controlled in the oxygen gas permeability. This poly-4-methyl-1-pentene resin laminate comprises a layer made of a 4-methyl-1-pentene polymer (A′), an intermediate layer made of an adhesive resin composition (B′) and a layer made of an olefin polymer (C′). This poly-4-methyl-1-pentene resin laminate can be used as a material of containers for keeping freshness of vegetables and fruits.
摘要翻译：提供了不仅热封性和氧气渗透性也耐粘连性优异的聚-4-甲基-1-戊烯树脂层压体。聚-4-甲基-1-戊烯树脂层压体包括由4-甲基-1-戊烯聚合物（A）制成的层，由粘合树脂组合物（B）制成的中间层和由丙烯聚合物组合物（C）包含60至90重量份的丙烯聚合物（c-1）和10至40重量份的1-丁烯聚合物（c-2），所述组分（c-1）的总量和（c-2）为100重量份。该聚-4-甲基-1-戊烯树脂层压体可以用作保鲜包装介质和培养容器的材料。还提供了具有优异的耐剥离性并且能够容易地控制氧气渗透性的聚-4-甲基-1-戊烯树脂层压体。该聚-4-甲基-1-戊烯树脂层压体包括由4-甲基-1-戊烯聚合物（A'）制成的层，由粘合树脂组合物（B'）制成的中间层和由烯烃聚合物（C'）。该聚-4-甲基-1-戊烯树脂层压体可以用作保持蔬菜和水果新鲜度的容器的材料。

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