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1. 发明申请

US20050085527A1 Catalysts for the polymerization of unsaturated compounds 有权
标题翻译：用于不饱和化合物聚合的催化剂
公开(公告)号：US20050085527A1
公开(公告)日：2005-04-21
申请号：US10959212
申请日：2004-10-07
申请人： Marc Kristen , Andrei Gonioukh , Dieter Lilge , Stephan Lehmann , Benno Bildstein , Christoph Amort , Michael Malaun
发明人： Marc Kristen , Andrei Gonioukh , Dieter Lilge , Stephan Lehmann , Benno Bildstein , Christoph Amort , Michael Malaun
IPC分类号： C07D401/14 , B01J31/18 , C07B61/00 , C07D213/53 , C07D409/12 , C07F15/02 , C07F15/06 , C08F4/70 , C08F10/00 , C08F10/02 , C08F110/02 , C08F210/16 , C07D333/12 , A61K31/381 , A61K31/382 , A61K31/4025 , C07D333/20
CPC分类号： C07D213/53 , C07F15/025 , C07F15/065 , C08F10/00 , C08F10/02 , C08F110/02 , C08F210/16 , C08F2500/03 , C08F2500/04 , C08F2500/08 , C08F2500/07 , C08F2500/10 , C08F210/14 , C08F4/7042 , C08F4/7047
摘要： Bisimine compounds of the formula (I) where the symbols have the following meanings: A is a nonmetal selected from among N, S, O and P, R1 is a radical of the formula NR5R6, R2 is a radical of the formula NR5R6 or NR7R8, alkyl, aryl or cycloalkyl, R5 and R6 together with the N atom form a 5-, 6- or 7-membered ring in which one or more of the —CH— or —CH2— groups may be replaced by suitable heteroatom groups and which may be saturated or unsaturated and unsubstituted or substituted or be fused with further carbacyclic or heterocarbacyclic 5- or 6-membered rings which may in turn be saturated or unsaturated and substituted or unsubstituted, and R7 and R8 are, independently of one another, alkyl, aryl or cycloalkyl radicals, and R3, R4 are, independently of one another, H or alkyl, aryl or cycloalkyl radicals, and n is 1 or 2, are used to prepare bisimidinato complexes which can be used in the polymerization of unsaturated compounds.
摘要翻译：式（I）的双亚胺化合物，其中符号具有以下含义：A是选自N，S，O和P的非金属，R 1是式NR的基团， 5，R 6，R 2是下式的基团NR 5 R 6或NR 6 烷基，芳基或环烷基，R 5和R 6以及N原子一起形成一个 5-，6-或7-元环，其中一个或多个-CH-或-CH 2 - 亚基可以被合适的杂原子基团取代，并且可以是饱和或不饱和和未取代的或取代或与另外的碳环或杂碳环五或六元环稠合，其又可以是饱和的或不饱和的和取代或未取代的，R 7和R 8是独立地为烷基，芳基或环烷基，R 3，R 4彼此独立地为H或烷基，芳基或环烷基，以及 n为1或2，用于制备可用于不饱和化合物聚合的双嘧啶络合物。

2. 发明授权

US07273940B2 Catalysts for the polymerization of unsaturated compounds 有权
标题翻译：用于不饱和化合物聚合的催化剂
公开(公告)号：US07273940B2
公开(公告)日：2007-09-25
申请号：US10959212
申请日：2004-10-07
申请人： Marc Oliver Kristen , Andrei Gonioukh , Dieter Lilge , Stephan Lehmann , Benno Bildstein , Christoph Amort , Michael Malaun
发明人： Marc Oliver Kristen , Andrei Gonioukh , Dieter Lilge , Stephan Lehmann , Benno Bildstein , Christoph Amort , Michael Malaun
IPC分类号： C07D333/12
CPC分类号： C07D213/53 , C07F15/025 , C07F15/065 , C08F10/00 , C08F10/02 , C08F110/02 , C08F210/16 , C08F2500/03 , C08F2500/04 , C08F2500/08 , C08F2500/07 , C08F2500/10 , C08F210/14 , C08F4/7042 , C08F4/7047
摘要： Bisimine compounds of the formula (I) where the symbols have the following meanings: A is a nonmetal selected from among N, S, O and P, R1 is a radical of the formula NR5R6, R2 is a radical of the formula NR5R6 or NR7R8, alkyl, aryl or cycloalkyl, R5 and R6 together with the N atom form a 5-, 6- or 7-membered ring in which one or more of the —CH— or —CH2— groups may be replaced by suitable heteroatom groups and which may be saturated or unsaturated and unsubstituted or substituted or be fused with further carbacyclic or heterocarbacyclic 5- or 6-membered rings which may in turn be saturated or unsaturated and substituted or unsubstituted, and R7 and R8 are, independently of one another, alkyl, aryl or cycloalkyl radicals, and R3, R4 are, independently of one another, H or alkyl, aryl or cycloalkyl radicals, and n is 1 or 2, are used to prepare bisimidinato complexes which can be used in the polymerization of unsaturated compounds.
摘要翻译：式（I）的双亚胺化合物，其中符号具有以下含义：A是选自N，S，O和P的非金属，R 1是式NR的基团， 5，R 6，R 2是下式的基团NR 5 R 6或NR 6 烷基，芳基或环烷基，R 5和R 6以及N原子一起形成一个 5-，6-或7-元环，其中一个或多个-CH-或-CH 2 - 亚基可以被合适的杂原子基团取代，并且可以是饱和或不饱和和未取代的或取代或与另外的碳环或杂碳环五或六元环稠合，其又可以是饱和的或不饱和的和取代或未取代的，R 7和R 8是独立地为烷基，芳基或环烷基，R 3，R 4彼此独立地为H或烷基，芳基或环烷基，以及 n为1或2，用于制备可用于不饱和化合物聚合的双嘧啶络合物。

3. 发明授权

US06818715B1 Bisimidino compounds and the transitional metal complexes thereof as well as the use thereof as catalysts 有权
标题翻译：双嘧啶系化合物及其过渡金属络合物及其作为催化剂的用途
公开(公告)号：US06818715B1
公开(公告)日：2004-11-16
申请号：US10049861
申请日：2002-02-19
申请人： Marc Oliver Kristen , Andrei Gonioukh , Dieter Lilge , Stephan Lehmann , Benno Bildstein , Christoph Amort , Michael Malaun
发明人： Marc Oliver Kristen , Andrei Gonioukh , Dieter Lilge , Stephan Lehmann , Benno Bildstein , Christoph Amort , Michael Malaun
IPC分类号： C08F406
CPC分类号： C07D213/53 , C07F15/025 , C07F15/065 , C08F10/00 , C08F10/02 , C08F110/02 , C08F210/16 , C08F2500/03 , C08F2500/04 , C08F2500/08 , C08F2500/07 , C08F2500/10 , C08F210/14 , C08F4/7042 , C08F4/7047
摘要： Bisimine compounds of the formula (I) where the symbols are defined in the specification are used to prepare bisimidinato complexes which can be used in the polymerization of unsaturated compounds.
摘要翻译：用于说明书中定义的符号的式（I）的双亚胺化合物用于制备可用于不饱和化合物聚合的双嘧啶络合物。

4. 发明申请

US20050038212A1 Ligands, complexes, and their use for the polymerization of olefins 有权
标题翻译：配体，络合物及其用于烯烃聚合的用途
公开(公告)号：US20050038212A1
公开(公告)日：2005-02-17
申请号：US10932124
申请日：2004-09-02
申请人： Marc Kristen , Benno Bildstein , Christoph Amort , Michael Malaun
发明人： Marc Kristen , Benno Bildstein , Christoph Amort , Michael Malaun
IPC分类号： C07D207/50 , C07D209/08 , C07D209/50 , C07D209/86 , C07F9/50 , C07F15/00 , C07F15/04 , C08F4/06 , C08F4/42 , C08F4/70 , C08F4/80 , C08F10/00 , C08F110/02 , C07F1/00
CPC分类号： C07F15/045 , C07D209/08 , C07D209/50 , C07D209/86 , C07F15/006 , C08F110/02 , C08F4/80 , C08F2500/17 , C08F2500/10 , C08F2500/03 , C08F2500/04
摘要： Ethylene and other 1-olefins and optionally other non-1-olefins are (co)polymerized in the presence of a catalyst which is a complex of formula I, where the variables are defined as follows: M is an element of Groups 6 to 10 of the Periodic Table of the Elements, Nu1 is O, S or Se; Nu2, Nu3 are each N or P, A1 is N or C—R7 or Si—R7, A2 is N or C—R8 or Si—R8, R1 to R5 are hydrogen, R6 to R9 are selected from the group consisting of (i) hydrogen, (ii) substituted or unsubstituted C1-C8-alkyl, (iii) substituted or unsubstituted C2-C8-alkenyl having from one to 4 isolated or conjugated double bonds, (iv) substituted or unsubstituted C3-C12-cycloalkyl, (v) C7-C13-aralkyl, (vi) C6-C14-aryl that is unsubstituted or monosubstituted or polysubstituted by identical or different substituents selected from the group consisting of substituted or unsubstituted C1-C8-alkyl, C3-C12-cycloalkyl, C7-C13-aralkyl, C6-C14-aryl, halogen, substituted or unsubstituted C1-C6-alkoxy, C6-C14-aryloxy, SiR10R11R12 and O—SiR10R11R12; and (vii) five- and six-membered nitrogen-containing heteroaryl radicals, unsubstituted or monosubstituted or polysubstituted by identical or different substituents selected from the group consisting of substituted or unsubstituted C1-C8-alkyl, C3-C12-cycloalkyl, C7-C13-aralkyl, C6-C14-aryl, halogen, C1-C6-alkoxy, C6-C14-aryloxy, SiR10R11R12 and O—SiR10R11R12, where adjacent radicals R1 to R9 optionally joined to one another to form a 5- to 12-membered ring; L1 is an uncharged organic or inorganic ligand, L2 is an organic or inorganic anionic ligand, where L1 and L2 may be joined to one another by one or more covalent bonds, and z is an integer from 1 to 3, and where R10 to R12 are identical or different and are selected from among the group consisting of hydrogen, C1-C8-alkyl, C3-C12-cycloalkyl, C7-C13-aralkyl and C6-C14-aryl.
摘要翻译：乙烯和其它1-烯烃和任选的其它非1-烯烃在式I化合物的催化剂存在下进行（共）聚合，其中变量定义如下：M是第6至10族的元素元素周期表，Nu 1是O，S或Se; Nu 2，Nu 3各自为N或P，A 1为N或CR 7或Si-R 7，A 2为N或CR 8或Si-R 7， R 1至R 5为氢，R 6至R 9选自（i）氢，（ii）取代或未取代的C 1 -C 8 - 烷基，（iii ）取代或未取代的具有1至4个分离或共轭双键的C 2 -C 8 - 烯基，（iv）取代或未取代的C 3 -C 12 - 环烷基，（v）C 7 -C 13 - 芳烷基，（vi）C 6 -C 14 - 芳基，被取代或未取代的C 1 -C 8 - 烷基，C 3 -C 12 - 环烷基，C 7 -C 13 - 芳烷基，C 6 -C 14 - 芳基，卤素，取代或未取代的C1 C 1-6 - 烷氧基，C 6 -C 14 - 芳氧基，SiR 10 R 11和O-SiR 10 R 11; 和（vii）五元和六元含氮杂芳基，其被选自取代或未取代的C 1 -C 8 - 烷基，C 3 -C 12 - 环烷基，C 7 -C 13的相同或不同的取代基未取代或单取代或多取代芳烷基，C 6 -C 14 - 芳基，卤素，C 1 -C 6 - 烷氧基，C 6 -C 14 - 芳氧基，SiR 10 R 11和O-SiR <

5. 发明授权

US06593437B1 Metal organic catalysts for polymerizing unsaturated compounds 有权
标题翻译：用于聚合不饱和化合物的金属有机催化剂
公开(公告)号：US06593437B1
公开(公告)日：2003-07-15
申请号：US09959382
申请日：2001-10-24
申请人： Andrei Gonioukh , Wolfgang Micklitz , Benno Bildstein , Michael Malaun , Andreas Hradsky
发明人： Andrei Gonioukh , Wolfgang Micklitz , Benno Bildstein , Michael Malaun , Andreas Hradsky
IPC分类号： C08F470
CPC分类号： C08G67/02 , C07C249/02 , C07C2603/20 , C07F17/02 , C08F4/00 , C08F4/61908 , C08F4/61912 , C08F4/61925 , C08F10/00 , C08F110/02 , C08F2410/03 , C08F2500/17 , C07C251/08 , C07C251/20 , C07C251/24 , C08F4/7006
摘要： A process for preparing 1,2-diimine compounds of the formula I where R1 and R2 are, independently of one another, alkyl, aryl or metallocenyl radicals, and R3, R4 are, independently of one another, H, alkyl or aryl radicals or R3 and R4 are joined so as to form, with inclusion of the two imine carbon atoms, a 5- to 8-membered ring which may be saturated or unsaturated and may be unsubstituted or substituted by any hydrocarbon radicals. The process involves reacting 1,2-dicarbonyl compounds with primary amines, which have been activated with trialkylaluminum compounds prior to the reaction with the 1,2-dicarbonyl compounds. 1,2-Diimine compounds of the formula I in which R1 and R2 are, independently of one another, metallocenyl radicals can be used to prepare metal complexes which can be used as catalysts in a process for the polymerization of unsaturated compounds.
摘要翻译：制备式I的1,2-二亚胺化合物的方法，其中R 1和R 2彼此独立地为烷基，芳基或金属茂基，且R 3，R 4彼此独立地为H，烷基或芳基或R 3 并且R4连接以形成包含两个亚胺碳原子的5-8元环，其可以是饱和或不饱和的，并且可以是未取代的或被任何烃基取代。该方法包括使1,2-二羰基化合物与伯胺反应，伯胺在与1,2-二羰基化合物反应之前已用三烷基铝化合物活化。其中R 1和R 2彼此独立地为金属茂基的式I的1,2-二亚胺化合物可用于制备可在不饱和化合物的聚合方法中用作催化剂的金属络合物。

6. 发明授权

US07022786B2 Ligands, complexes and their use for the polymerization of olefins 有权
标题翻译：配体，配合物及其用于烯烃聚合的用途
公开(公告)号：US07022786B2
公开(公告)日：2006-04-04
申请号：US10932124
申请日：2004-09-02
申请人： Marc Oliver Kristen , Benno Bildstein , Christoph Amort , Michael Malaun
发明人： Marc Oliver Kristen , Benno Bildstein , Christoph Amort , Michael Malaun
IPC分类号： C08F4/44
CPC分类号： C07F15/045 , C07D209/08 , C07D209/50 , C07D209/86 , C07F15/006 , C08F110/02 , C08F4/80 , C08F2500/17 , C08F2500/10 , C08F2500/03 , C08F2500/04
摘要： Complexes of the formula I, where M is an element of groups 6 to 10 of the Periodic Table of the Elements, preferably Ni, can be used for the polymerization and copolymerization of olefins, for example in suspension polymerisation processes, gas-phase polymerization processes, bulk polymerization processes or emulsion polymerization processes.
摘要翻译：式I的络合物，其中M是元素周期表第6至10族的元素，优选Ni，可用于烯烃的聚合和共聚，例如在悬浮聚合方法中，气相聚合方法，本体聚合方法或乳液聚合方法。

7. 发明授权

US06900278B2 Ligands, complex compounds and their use for polymerising olefins 有权
标题翻译：配体，络合物及其用于聚合烯烃的用途
公开(公告)号：US06900278B2
公开(公告)日：2005-05-31
申请号：US10312587
申请日：2001-07-13
申请人： Marc Oliver Kristen , Benno Bildstein , Christoph Amort , Michael Malaun
发明人： Marc Oliver Kristen , Benno Bildstein , Christoph Amort , Michael Malaun
IPC分类号： C07D207/50 , C07D209/08 , C07D209/50 , C07D209/86 , C07F9/50 , C07F15/00 , C07F15/04 , C08F4/06 , C08F4/42 , C08F4/70 , C08F4/80 , C08F10/00 , C08F110/02 , C08F4/44
CPC分类号： C07F15/045 , C07D209/08 , C07D209/50 , C07D209/86 , C07F15/006 , C08F110/02 , C08F4/80 , C08F2500/17 , C08F2500/10 , C08F2500/03 , C08F2500/04
摘要： Complexes of the formula I, where M is an element of group 6 to 10 of the Period Table of the Elements, preferably Ni, can be used for the polymerization and copolymerization of olefins, for example in suspension polymerisation processes, gas-phase polymerization processes, bulk polymerization processes or emulsion polymerization processes.
摘要翻译：式I的络合物，其中M是元素周期表中第6至10族的元素，优选Ni，可用于烯烃的聚合和共聚，例如在悬浮聚合方法中，气相聚合方法，本体聚合方法或乳液聚合方法。

8. 发明授权

US06743932B2 Polymerization catalyst 失效
标题翻译：聚合催化剂
公开(公告)号：US06743932B2
公开(公告)日：2004-06-01
申请号：US09827099
申请日：2001-04-06
申请人： Marc Oliver Kristen , Benno Bildstein , Michael Malaun , Ulrich Siemeling , Oliver Kuhnert
发明人： Marc Oliver Kristen , Benno Bildstein , Michael Malaun , Ulrich Siemeling , Oliver Kuhnert
IPC分类号： C07F1700
CPC分类号： C07F17/00 , C07F17/02 , Y10S526/943
摘要： An organometallic compound of the formula I where M1 is selected from among Fe, Ru and Os and M2 is selected from among the transition metals of groups IV to VI of the Periodic Table, which can be prepared by reacting an organometallic compound of the formula II with a transition metal compound of the formula III, M2L1L2(L3)x+1 III where the variables are as defined above and the organometallic compound of the formula II can, if desired, be doubly deproteinated beforehand, can be used as part of a catalyst system for the polymerization or copolymerization of olefins. This catalyst system comprises one or more organometallic compounds of the formula I and at least one activator. The compound of the formula I can also be used to produce a solid catalyst comprising at least one organometallic compound of the formula I, at least one activator and a solid support by impregnating a support material with one or more organometallic compounds of the formula I and at least one activator. This solid catalyst can be used in a process for the polymerization or copolymerization of olefins in bulk, in suspension or in the gas phase.
摘要翻译：式I的有机金属化合物，其中M 1选自Fe，Ru和Os，M 2选自周期表IV至VI族的过渡金属，它们可以通过使有机金属式II化合物与式III的过渡金属化合物，其中变量如上所定义，如果需要，可以预先将式II的有机金属化合物双重去蛋白化，可用作催化剂体系的一部分，用于烯烃的聚合或共聚。该催化剂体系包含一种或多种式I的有机金属化合物和至少一种活化剂。式I化合物还可用于制备包含至少一种式I的有机金属化合物，至少一种活化剂和固体载体的固体催化剂，其通过用一种或多种式I的有机金属化合物浸渍载体材料和至少一种活化剂。该固体催化剂可用于本体，悬浮液或气相中烯烃聚合或共聚的方法。

9. 发明申请

US20050085603A1 Metal complexes of iminohydroxamic acids 失效
公开(公告)号：US20050085603A1
公开(公告)日：2005-04-21
申请号：US10961074
申请日：2004-10-12
申请人： Marc Kristen , Peter Preishuber-Pflugl , Benno Bildstein , Alexander Krajete
发明人： Marc Kristen , Peter Preishuber-Pflugl , Benno Bildstein , Alexander Krajete
IPC分类号： C07C259/18 , C07C43/04 , C07C257/22 , C07F15/00 , C07F15/04 , C08F2/00 , C08F4/70 , C08F4/80 , C08F10/00 , C07F15/02 , C07F15/06
CPC分类号： C07F15/0066 , C07F15/045
摘要： Complexes of the formula I where M═Ni, Pd; process for preparing the metal complexes and the use of the complexes obtainable in this way for the polymerization and copolymerization of olefins, for example in suspension polymerization processes, gas-phase polymerization processes and bulk polymerization processes.

10. 发明申请

US20090054609A1 Process for the Preparation of Unsymmetric Bis(Imino) Compounds 有权
标题翻译：制备不对称双（亚氨基）化合物的方法
公开(公告)号：US20090054609A1
公开(公告)日：2009-02-26
申请号：US12087554
申请日：2007-01-08
申请人： Shahram Mihan , Benno Bildstein , Lars Kolling , Alexander Solchinger , Sascha Schlawjinski
发明人： Shahram Mihan , Benno Bildstein , Lars Kolling , Alexander Solchinger , Sascha Schlawjinski
IPC分类号： C08F4/26 , C07D213/50 , C07F15/02
CPC分类号： C07F15/025 , B01J2531/0238 , B01J2531/842 , C07D213/44 , C07D213/53 , C08F10/00 , C08F110/02 , C08F2500/17 , C08F2500/04 , C08F4/7042
摘要： Process for the preparation of monoimine compounds, wherein a dicarbonyl compound is reacted in an aliphatic, non-aromatic solvent with aniline. Monoimine compounds having electron-withdrawing substituents in the ortho position and unsymmetric bis(imino) compounds and unsymmetric iron complexes prepared therefrom and the use thereof in the polymerization of olefins.
摘要翻译：制备单亚胺化合物的方法，其中二羰基化合物在脂族，非芳族溶剂中与苯胺反应。在邻位具有吸电子取代基的单亚胺化合物和由其制备的不对称双（亚氨基）化合物和不对称铁络合物及其在烯烃聚合中的用途。

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