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1. 发明授权

US5426151A Polysiloxane-containing binders, manufacture thereof, coating agents containing them, and use thereof 失效
标题翻译：含有聚硅氧烷的粘合剂，其制造方法，含有它们的涂布剂及其用途
公开(公告)号：US5426151A
公开(公告)日：1995-06-20
申请号：US153938
申请日：1993-11-17
申请人： Lutz Brandt , Carmen Flosbach , Reinhardt Kalus , Walter Schubert
发明人： Lutz Brandt , Carmen Flosbach , Reinhardt Kalus , Walter Schubert
IPC分类号： C08F299/08 , C08F290/00 , C08L83/04 , C08L83/10 , C09D5/00 , C09D151/08 , C09D183/04 , C09D183/10 , C08F30/08
CPC分类号： C09D151/085 , C09D183/10 , Y10S525/903
摘要： A polymeric coating agent which comprises a polymer of from 60 to 97 wt. % of one or more (meth)acrylic monomers the polymerization of which can be initiated by free radicals, from 3 to 40 wt. % of at least one .alpha., .omega.-hydroxy-, carboxy-, and/or epoxy-functional polysiloxanes of the formula (I) ##STR1## wherein R' can be the same or different and is C.sub.1-6 alkyl, and R can be the same or different and is ##STR2## wherein Alk and Alk' are C.sub.1-6 alkylene and the alkylene groups in a molecule can be the same or different, n is a cardinal number from 8 to 40, m is a cardinal number from 2 to 30, and p is a cardinal number from 1 to 20 of solids in the monomers.
摘要翻译：一种聚合物涂层剂，其包含60至97重量％％的一种或多种（甲基）丙烯酸单体，其聚合可以通过自由基引发，为3-40wt。％的至少一种式（I）的α，ω-羟基，羧基和/或环氧官能的聚硅氧烷（I）其中R'可以相同或不同，并且是C 1-6烷基，并且R可以相同或不同，为Alk（OAlk）pOH; 阿尔科其中Alk和Alk'是C1-6亚烷基并且分子中的亚烷基可以相同或不同，n为8至40的基数，m为2至30的基数，p是单体中固体含量为1至20的基数。

2. 发明授权

US06268021B1 Binder vehicle and coating medium composition and the use thereof for multi-layer coating 失效
标题翻译：粘合剂载体和涂料介质组成及其在多层涂料中的应用
公开(公告)号：US06268021B1
公开(公告)日：2001-07-31
申请号：US09208999
申请日：1998-12-11
申请人： Carmen Flosbach , Friedrich Herrmann , Walter Schubert , Dirk Schild
发明人： Carmen Flosbach , Friedrich Herrmann , Walter Schubert , Dirk Schild
IPC分类号： B05D136
CPC分类号： C08G18/631 , C08G18/4063 , C08G18/4241 , C09D175/06
摘要： A binder vehicle composition which is suitable for coating media, containing: A) 20 to 77% by weight of one or more binder vehicles based on oligomeric or polymeric polyol compounds with a hydroxyl number of 80 to 300, an acid number of 0 to 30, a number average molecular weight (Mn) of 500 to 10,000, and a glass transition temperature of −20 to +70° C.; B) 77 to 20% by weight of crosslinking agents based on aliphatic and/or cycloaliphatic polyisocyanates; C) 3 to 20% by weight of oligo- or polyesters, which contain carboxyl groups, as catalyst resins, which have an acid number of 210 to 300 mg KOH/g and a number average molecular weight (Mn) of 420 to 3000; and one or more organic solvents and/or water.
摘要翻译：一种适用于涂布介质的粘合剂载体组合物，其包含：A）20至77重量％的基于羟基数为80至300，酸值为0至30的低聚或多聚多元醇化合物的一种或多种粘合剂载体数均分子量（Mn）为500至10,000，玻璃化转变温度为-20至+ 70℃; B）基于脂族和/或脂环族多异氰酸酯的交联剂为77至20重量％; C ）3〜20重量％的含羧基的低聚或聚酯作为催化剂树脂，其酸值为210〜300mg KOH / g，数均分子量（Mn）为420〜3000;以及一种或多种有机溶剂和/或水。

3. 发明授权

US6063448A Coating media, the use thereof, and a method of producing multilayer coatings 失效
标题翻译：涂布介质及其用途以及多层涂料的制造方法
公开(公告)号：US6063448A
公开(公告)日：2000-05-16
申请号：US981644
申请日：1998-03-09
申请人： Volker Duecoffre , Carmen Flosbach , Hermann Kerber , Walter Schubert , Friedrich Herrmann , Heinz-Walter Reifferscheid , Dirk Schild
发明人： Volker Duecoffre , Carmen Flosbach , Hermann Kerber , Walter Schubert , Friedrich Herrmann , Heinz-Walter Reifferscheid , Dirk Schild
IPC分类号： B05D7/24 , B32B27/30 , C08F220/26 , C08G18/40 , C08G18/42 , C08G18/62 , C08G18/63 , C08G18/80 , C09D133/02 , C09D133/14 , C09D161/26 , C09D175/04 , B05D7/14 , B05D1/36 , B05D3/02
CPC分类号： C08G18/631 , C08G18/4063 , C08G18/4072 , C09D175/04
摘要： A coating medium suitable for multilayer coatings, containing, as a binder vehicle:______________________________________ A) 10 to 90% by weight of one or more hydroxy-functional (meth)acrylic copolymers, obtained from a1) 20 to 40% by weight of hydroxyalkyl esters of (meth)acrylic acid a2) 10 to 30% by weight of non-functionalised (meth) acrylates a3) 0 to 5% by weight of unsaturated carboyxlic acids a4) 10 to 60% by weight of non-functionalised monomers a5) 0 to 15% by weight of amino-functional monomers, and a6) 0 to 5% by weight of multiply-unsaturated monomers B) 90 to 10% by weight of hydroxy-functional polyesters, C) 0 to 40% by weight of hydroxy-functional binder vehicles D) 5 to 50% by weight of blocked polyisocyanates, E) 5 to 40% by weight of components based on triazine which crosslink with the hydroxyl groups of components A), B) and C) with the formation of ether and/or ester groups, ______________________________________ wherein at least 50% by weight of the (meth)acrylic copolymers, with respect to the total amount of component A), has been produced in the presence of the hydroxy-functional polyesters corresponding to at least 20% by weight of the total amount of component B).
摘要翻译： PCT No.PCT / EP96 / 02944 Sec。 371日期1998年3月9日 102（e）1998年3月9日PCT PCT 1996年7月4日PCT公布。公开号WO97 / 03102 日期1997年1月30日适用于多层涂料的涂料介质，其含有作为粘合剂的载体：A）10-90重量％的一种或多种羟基官能 - （甲基）丙烯酸共聚物，其由-a1）20至 40重量％的（甲基）丙烯酸的羟基烷基酯a2）10-30重量％的非官能化（甲基）丙烯酸酯-a3）0-5重量％的不饱和羧酸-a4）10至60重量％的非官能化单体a5）0-15％（重量）的氨基官能单体和-16）0-5％重量的多不饱和单体B）90-10％重量的羟基官能化单体聚酯，-C）0-40％（重量）的羟基官能粘合剂载体-D）5-50％重量的封端多异氰酸酯， - E）5-40％（重量）基于与三羟基交联的三嗪组分组分A），B）和C）与形成醚和/或酯基 - 其中至少50重量％的（甲基）丙烯酸共聚物相对于相对于组分A）的总量已经在对应于组分B）总量的至少20重量％的羟基官能聚酯的存在下生产。

4. 发明授权

US5739216A Binder composition, coating compositions containing this binder composition, production and use thereof 失效
标题翻译：粘合剂组合物，含有该粘合剂组合物的涂料组合物，其生产和使用
公开(公告)号：US5739216A
公开(公告)日：1998-04-14
申请号：US732474
申请日：1997-01-02
申请人： Volker Duecoffre , Carmen Flosbach , Friedrich Herrmann , Heinz-Walter Reifferscheidt , Walter Schubert
发明人： Volker Duecoffre , Carmen Flosbach , Friedrich Herrmann , Heinz-Walter Reifferscheidt , Walter Schubert
IPC分类号： C08L63/00 , C08L75/04 , C09D5/46 , C09D133/06 , C09D163/00 , C09D167/00 , C09D167/06 , C09D175/04 , C09D175/06
CPC分类号： C09D167/00 , C09D133/062 , C09D133/068 , C09D163/00 , C09D175/04 , C08L63/00 , C08L75/04 , Y10T428/31551
摘要： Binder composition, coating compositions produced therefrom and use thereof, in particular for multi-layer lacquer coatings. The binder composition contains: A) 25 to 75 wt. % of the reaction product of one or more carboxy-functionalised (meth) acrylic copolymers containing urethane groups and/or of one or more carboxy-functionalised polyesters containing urethane groups, each having an acid value of 30 to 200 mg of KOH/g, with one or more lactones, B) 25 to 75 wt. % of one or more epoxy-functionalised crosslinking agents having at least two epoxy functions per molecule with a number average molecular weight (Mn) of 200 to 10000 g/mol, C) 0 to 60 wt. % of one or more polyols having at least two hydroxyl functions per molecule, D.sub.1) 0 to 20 wt. % of one or more melamine resins, D.sub.2) 0 to 40 wt. % of one or more free or capped polyisocyanates, wherein the sum of the weight percentages of components A), B), C), D.sub.1) and D.sub.2) amounts to 100 wt. %, together with E) 0 to 10 wt. % of one or more catalysts to catalyse the reaction of carboxyl and epoxy groups, relative to the sum of weights of components A) to D.sub.2).
摘要翻译： PCT No.PCT / EP95 / 01663 Sec。 371日期1997年1月2日 102（e）日期1997年1月2日PCT提交1995年5月3日PCT公布。出版物WO95 / 30719 日期1995年11月16日粘合剂组合物，由其制备的涂料组合物及其用途，特别是多层漆涂料。粘合剂组合物含有：A）25〜75wt。含有氨基甲酸酯基团的一种或多种羧基官能化（甲基）丙烯酸共聚物和/或含有氨基甲酸酯基团的一种或多种羧基官能化聚酯的反应产物的百分比，其酸值为30-200mg KOH / g，与一种或多种内酯，B）25至75wt。％的一种或多种环氧官能化交联剂，每分子具有至少两个环氧官能团，数均分子量（Mn）为200至10000g / mol，C）0至60wt。％的一种或多种每分子具有至少两个羟基官能团的多元醇，D1）0-20重量％％的一种或多种三聚氰胺树脂，D2）0-40重量％％的一种或多种游离或封端的多异氰酸酯，其中组分A），B），C），D1）和D2的重量百分比之和相当于100wt。％，连同E）0〜10wt。％的一种或多种催化剂以催化羧基和环氧基团的反应，相对于组分A）至D2的重量之和）。

5. 发明授权

US6037404A Rheology-influencing composition for coating media 失效
标题翻译：用于涂料介质的流变学影响组合物
公开(公告)号：US6037404A
公开(公告)日：2000-03-14
申请号：US089754
申请日：1998-06-02
申请人： Ralf Dahm , Carmen Flosbach , Hermann Kerber , Sandra Kirchgassler , Dieter Lerch , Frank Schnodewind , Walter Schubert
发明人： Ralf Dahm , Carmen Flosbach , Hermann Kerber , Sandra Kirchgassler , Dieter Lerch , Frank Schnodewind , Walter Schubert
IPC分类号： C09K3/00 , C08G18/40 , C08G18/42 , C08G18/62 , C08G18/63 , C08G18/80 , C09D5/04 , C09D7/12 , C08J3/00 , C08F8/30 , C08G18/08 , C08K3/20 , C08L75/00
CPC分类号： C08G18/631 , C08G18/4072 , C08G18/8074 , C09D5/04
摘要： This invention relates to a composition, and to the preparation and use of thereof said composition being suitable as a rheology influencer for coating media and comprising the reaction product formed by reaction of a mixture of components A, B and C with components D, E and F. Components A, B and C form a mixture wherein component A is one or more (meth)acrylic copolymers and/or one or more polyesters which contain hydroxyl groups. Component B is a copolymer of ethylhexyl (meth)acrylate and one or more hydroxyalkyl (meth)acrylates, as well as .alpha.,.beta.-unsaturated monomers which are different therefrom. Component C is a hydroxy--functional microdispersion which is produced by polymerizing hydroxylalkyl (meth)acrylates in combination with unsaturated monomers in a mixture of polyesters or polyacrylates containing carboxyl and/or hydroxyl groups. Component D is one or more aliphatic polyisocyantes and component E is .epsilon.-caprolactam. The caprolactam partially blocks the polyisocyanate. The component F is one or more primary amines. These ingredients are combined in certain specified amounts. The invention also relates to coating media and to the production of these coating media, which contain said composition as a rheology influencer.
摘要翻译：本发明涉及一种组合物及其制备和用途，所述组合物适合用作涂料介质的流变学影响剂，并且包含通过组分A，B和C的混合物与组分D，E反应形成的反应产物和 F.组分A，B和C形成混合物，其中组分A是一种或多种（甲基）丙烯酸共聚物和/或一种或多种含有羟基的聚酯。组分B是（甲基）丙烯酸乙基己酯和一种或多种（甲基）丙烯酸羟烷基酯以及与其不同的α，β-不饱和单体的共聚物。组分C是通过在含有羧基和/或羟基的聚酯或聚丙烯酸酯的混合物中聚合（甲基）丙烯酸羟烷基酯与不饱和单体组合制备的羟基官能微分散体。组分D是一种或多种脂肪族聚异氰酸酯，组分E是ε-己内酰胺。己内酰胺部分阻断多异氰酸酯。组分F是一种或多种伯胺。这些成分以特定的量组合。本发明还涉及涂料介质和这些包含所述组合物作为流变学影响剂的涂料介质的生产。

6. 发明授权

US5480936A Emulsifier-free coating agent, manufacture and use thereof 失效
标题翻译：无乳化剂涂层剂，其制造和使用
公开(公告)号：US5480936A
公开(公告)日：1996-01-02
申请号：US250449
申请日：1994-05-27
申请人： Volker Duecoffre , Carmen Flosbach , Walter Schubert , Manfred Krumme , Werner Stephan , Fritz Sadowski
发明人： Volker Duecoffre , Carmen Flosbach , Walter Schubert , Manfred Krumme , Werner Stephan , Fritz Sadowski
IPC分类号： C08G18/68 , C08G18/63 , C08G18/79 , C09D5/00 , C09D133/04 , C09D133/06 , C09D151/00 , C09D151/08 , C09D175/14 , C09D175/16 , C09D181/08 , C08L75/06 , C08F3/30 , C08F282/02
CPC分类号： C08G18/631 , C08G18/792 , C09D181/08
摘要： Oligoester acrylate resins having a high content of solids and comparatively low viscosity, and aqueous coating agents with a low content of organic solvents for obtaining coatings with high resistance to chemicals, more particularly high resistance to acids and oily soot, and very low tendency to yellowing.
摘要翻译：具有高固体含量和较低粘度的低聚酯丙烯酸酯树脂以及具有低含量有机溶剂的水性涂料，用于获得对化学品具有高抗性的涂层，更特别是耐酸性和油性烟灰的耐受性以及非常低的黄变倾向。

7. 发明授权

US06743867B1 Coating agents which can be used for multi-layer enameling 失效
标题翻译：可用于多层搪瓷的涂层剂
公开(公告)号：US06743867B1
公开(公告)日：2004-06-01
申请号：US09958993
申请日：2002-03-28
申请人： Carmen Flosbach , Friedrich Herrmann , Claudia Drewin , Walter Schubert , Astrid Tueckmantel
发明人： Carmen Flosbach , Friedrich Herrmann , Claudia Drewin , Walter Schubert , Astrid Tueckmantel
IPC分类号： C08L7100
CPC分类号： C09D133/068 , C08L33/064 , C08L67/00 , C09D167/00 , C08L2666/14 , C08L2666/04 , C08L63/00
摘要： A coating compound comprising a binder/crosslinking agent system that comprises 20 wt. % to 80 wt. % of one or more carboxyl-functional components A) and 80 wt. % to 20 wt. % of one or more epoxy-functional (meth)acrylic copolymers B).
摘要翻译：包含粘合剂/交联剂体系的涂料化合物，其包含20wt。％至80wt。％的一种或多种羧基官能组分A）和80wt。％至20重量％％的一种或多种环氧官能（甲基）丙烯酸共聚物B）。

8. 发明授权

US06555176B1 Sag stabilized coating compositions containing epoxy-functional crosslinking components 失效
标题翻译：含有环氧官能交联组分的凹凸稳定的涂料组合物
公开(公告)号：US06555176B1
公开(公告)日：2003-04-29
申请号：US09914219
申请日：2001-08-22
申请人： Ralf Dahm , Carmen Flosbach , Hans-Jürgen Gawin , Hermann Kerber , Apostolos Manassis , Volker Paschmann , Walter Schubert
发明人： Ralf Dahm , Carmen Flosbach , Hans-Jürgen Gawin , Hermann Kerber , Apostolos Manassis , Volker Paschmann , Walter Schubert
IPC分类号： C08J500
CPC分类号： C09D163/00 , C08L2666/04 , C08L2666/18
摘要： Coating composition containing a binder/crosslinking agent system, organic solvents, optionally together with pigments and/or extenders and conventional lacquer additives, wherein the binder/crosslinking agent system contains A) 20 to 80 wt. % of carboxy-functional (meth)acrylic copolymers and/or polyesters which are dissolved in the continuous phase of the coating composition, with an acid value of 15 to 300 mg of KOH/g, B) 80 to 20 wt. % of epoxy-functional crosslinking agents, wherein the numerical ratio between the component A) carboxyl groups and the component B) epoxy groups is between 1:1 and 1:3, and the epoxy-functional crosslinking agent B) comprises at least one epoxy-functional crosslinking component B1) which is dissolved in the continuous phase of the coating composition and at least one epoxy-functional component B2) dispersed in the continuous phase of the coating composition, wherein the numerical ratio of the epoxy groups of the crosslinking components B1) and B2) is 10:1 to 1:5 and wherein the organic solvents comprise 0 to 35 wt. % of one or more conventional organic lacquer solvents containing oxygen and 65 to 100 wt. % of one or more conventional lacquer hydrocarbons.
摘要翻译：包含粘合剂/交联剂体系的涂料组合物，有机溶剂，任选地与颜料和/或增量剂和常规漆添加剂一起，其中粘合剂/交联剂体系含有A）20至80wt。％的羧酸官能（甲基）丙烯酸共聚物和/或聚酯，其溶解在涂料组合物的连续相中，酸值为15至300mg KOH / g，B）80至20wt。％的环氧官能交联剂，其中组分A）羧基和组分B）环氧基之间的数值比在1:1至1:3之间，并且环氧官能交联剂B）包含至少一种环氧溶解在涂料组合物的连续相中的功能性交联组分B1）和分散在涂料组合物的连续相中的至少一种环氧官能组分B2），其中交联组分B1的环氧基数）和B2）为10:1至1:5，并且其中所述有机溶剂包含0至35重量％％的一种或多种常规有机漆溶剂含有氧和65至100wt。％的一种或多种常规漆油。

9. 发明授权

US6150486A Method for producing glycidyl (meth) acrylate copolymers 失效
标题翻译：（甲基）丙烯酸缩水甘油酯共聚物的制备方法
公开(公告)号：US6150486A
公开(公告)日：2000-11-21
申请号：US355305
申请日：1999-10-18
申请人： Christian Schwede , Walter Schubert , Carmen Flosbach , Friedhelm Bandermann , Aurel Wolf
发明人： Christian Schwede , Walter Schubert , Carmen Flosbach , Friedhelm Bandermann , Aurel Wolf
IPC分类号： C08F2/00 , C08F220/32 , C08F283/02 , C09D133/14 , C09D151/08 , C09D163/10 , C09D167/00
CPC分类号： C08F283/02 , C09D167/00
摘要： Process for the production of glycidyl (meth)acrylate copolymers with a number-average molar mass (Mn) of 1000 to 6000 g/mol by solvent-free, continuous copolymerisation of glycidyl (meth)acrylate with ethylenically unsaturated monomers, in a reaction vessel with feed and discharge means in the presence of a polyester oligomer, wherein polyester oligomer or a mixture of glycidyl (meth)acrylate copolymer and polyester oligomer is initially introduced in a weight ratio of from 95:5 to 50:50 and the glycidyl (meth)acrylates, further monomers, further polyester oligomer and, optionally, free-radical initiators are added, the addition together with discharge of the copolymers formed being effected in such a way that the residence time required for formation of the desired composition is achieved, and wherein, in the event of the initial introduction of the mixture of glycidyl (meth)acrylate copolymer and polyester oligomer, addition is effected in such a way that the ratio between copolymer and oligomer is maintained.
摘要翻译： PCT No.PCT / EP98 / 07646 Sec。 371 1999年10月18日第 102（e）1999年10月18日PCT PCT 1998年11月28日PCT公布。出版物WO99 / 28361 日期1999年6月10日通过（甲基）丙烯酸缩水甘油酯与烯属不饱和单体的无溶剂连续共聚，制备数均摩尔质量（Mn）为1000〜6000g / mol的（甲基）丙烯酸缩水甘油酯共聚物的方法在具有聚酯低聚物存在下的进料和排出装置的反应容器中，其中首先以95:5至50:50的重量比引入聚酯低聚物或（甲基）丙烯酸缩水甘油酯共聚物和聚酯低聚物的混合物和（甲基）丙烯酸缩水甘油酯，另外的单体，另外的聚酯低聚物和任选的自由基引发剂，加入所形成的共聚物的排出，使得形成期望的并且其中，在初始引入（甲基）丙烯酸缩水甘油酯共聚物和聚酯低聚物的混合物的情况下，以这样的方式进行添加：保持共聚物和低聚物之间。

10. 发明授权

US5466860A Process for the preparation of blocked isocyanates 失效
标题翻译：制备封闭的异氰酸酯的方法
公开(公告)号：US5466860A
公开(公告)日：1995-11-14
申请号：US385444
申请日：1995-02-08
申请人： Carmen Flosbach , Dieter Philipp , Walter Schubert
发明人： Carmen Flosbach , Dieter Philipp , Walter Schubert
IPC分类号： C08G18/80 , C08G18/40 , C08G18/62 , C08L61/20 , C08L75/00 , C09D133/06 , C09D175/00 , C09D175/04 , C07C229/24
CPC分类号： C09D133/066 , C08G18/4063 , C08G18/6254 , C08G18/6258 , C09D175/00 , C08L61/20 , C08L75/00
摘要： A process for the preparation of blocked isocyanates by reaction of free isocyanates under water-free conditions with blocking agents containing acid hydrogen in the presence of basic catalysts, these being one or more alkali hydroxides, particularly lithium hydroxide. The process leads to yellowing-free products with a low alkali content which may be used as cross-linking agents for polyols, particularly in the lacquer sector.
摘要翻译：在碱性催化剂存在下，通过游离异氰酸酯在无水条件下与含有酸氢的封闭剂反应来制备封闭的异氰酸酯的方法，这些是一种或多种碱金属氢氧化物，特别是氢氧化锂。该方法导致具有低碱含量的无黄变产物，其可用作多元醇的交联剂，特别是在漆部门中。

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