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1. 发明授权

US5703190A Crosslinkable compositions 失效
标题翻译：可交联组合物
公开(公告)号：US5703190A
公开(公告)日：1997-12-30
申请号：US697359
申请日：1996-08-23
申请人： Jochen Dauth , Christian Herzig , Bernward Deubzer , Klaus Schnitzer , David Huettner
发明人： Jochen Dauth , Christian Herzig , Bernward Deubzer , Klaus Schnitzer , David Huettner
IPC分类号： C08G77/20 , C08G77/22 , C08K5/01 , C08K5/05 , C08L83/04 , C08L83/05 , C08L83/07 , C09D183/04 , C09D183/07 , C08G77/06
CPC分类号： C08L83/04 , C08K5/01 , C08K5/05 , C09D183/04 , C08G77/045 , C08G77/12 , C08G77/20 , C08G77/70 , C08G77/80
摘要： The present invention relates to crosslinkable compositions are described, containing (1) organosilicon compounds which have radicals containing aliphatic carbon-carbon multiple bonds, and (2) organosilicon compounds having Si-bonded hydrogen atoms, or (3) organosilicon compounds where radicals with aliphatic carbon-carbon multiple bonds and Si-bonded hydrogen atoms are present in the same compound, (4) catalysts which promote the addition of Si-bonded hydrogen onto aliphatic multiple bond, and (5) agents which retard the addition of Si-bonded hydrogen onto aliphatic multiple bond at room temperature, of the formula ##STR1## in which R.sup.1, R.sup.2, R.sup.4, R.sup.5 and R.sup.6 are identical or different and are a hydrogen atom or a monovalent, substituted or unsubstituted hydrocarbon radical having 1 to 12 carbon atoms per radical,R.sup.3 is a divalent hydrocarbon radical having 1 to 6 carbon atoms per radical, X is a radical of the formula --OH, --Cl, Br and --CN, and x and y are identical or different and are 0 or 1, with the proviso that there is at least one double bond.
摘要翻译：本发明涉及可交联组合物，其含有（1）具有含有脂族碳 - 碳多键的基团的有机硅化合物，和（2）具有硅键合氢原子的有机硅化合物，或（3）有机硅化合物，碳 - 碳多键和硅键合的氢原子存在于同一化合物中，（4）促进在脂肪族多键上加入Si键的氢的催化剂，和（5）阻止加入Si键的氢在其中R 1，R 2，R 4，R 5和R 6相同或不同且为氢原子或具有1至12个碳原子的单价，取代或未取代的烃基的式（I）每个基团的碳原子，R 3是每个基团具有1至6个碳原子的二价烃基，X是式-OH，-Cl，Br和-CN的基团，x和y相同或不同， 0或1，条件是存在至少一个双键。

2. 发明授权

US6100348A Crosslinkable compositions 失效
标题翻译：可交联组合物
公开(公告)号：US6100348A
公开(公告)日：2000-08-08
申请号：US88518
申请日：1998-06-02
申请人： Jochen Dauth , Bernward Deubzer , Josef Wolferseder , Klaus Schnitzer
发明人： Jochen Dauth , Bernward Deubzer , Josef Wolferseder , Klaus Schnitzer
IPC分类号： C07C49/794 , C07C49/835 , C08K5/07 , C08L83/04 , C08L83/05 , C08L83/07 , C09D183/04 , C09D183/05 , C09D183/07 , C09J183/05 , C09J183/07 , C08F283/00 , B32B9/04 , C08F30/08 , C08G77/12 , C08G77/20
CPC分类号： C07C49/835 , C08K5/07 , C08L83/04 , C09D183/04 , C08G77/12 , C08G77/16 , C08G77/20 , C08G77/24 , C08G77/26
摘要： The invention describes crosslinkable compositions comprising(1) organosilicon compounds which contain radicals having aliphatic carbon-carbon multiple bonds,(2) organosilicon compounds having Si-bonded hydrogen atoms or, in place of or in addition to (1) and (2); said composition further comprising(3) organosilicon compounds which contain radicals having aliphatic carbon-carbon multiple bonds and Si-bonded hydrogen atoms,(4) catalysts which promote the addition of Si-bonded hydrogen to aliphatic multiple bonds, and ##STR1## where R.sup.1 and R.sup.2 are as defined in claim 1, and X is a radical of the formula --OH, --Cl, --Br and --CN, with the radical --OH being particularly preferred.
摘要翻译：本发明描述了可交联组合物，其包含（1）含有具有脂族碳 - 碳多重键的基团的有机硅化合物，（2）具有Si键合的氢原子的有机硅化合物，或代替（1）和（2）或除了（1）和（2）之外。所述组合物还包含（3）含有具有脂肪族碳 - 碳多重键和Si键合氢原子的基团的有机硅化合物，（4）促进与键合氢键合成脂肪族多键的催化剂，其中R1和R2为如权利要求1所定义，X是式-OH，-Cl，-Br和-CN的基团，其中-OH基是特别优选的。

3. 发明授权

US5593787A Organosilicon compounds containing (meth) acryloxy groups, their preparation and their use 失效
标题翻译：含有（甲基）丙烯酰氧基的有机硅化合物，其制备及其应用
公开(公告)号：US5593787A
公开(公告)日：1997-01-14
申请号：US548127
申请日：1995-10-25
申请人： Jochen Dauth , Christian Herzig , Bernward Deubzer , Thomas Hierstetter , Petra Gratzl
发明人： Jochen Dauth , Christian Herzig , Bernward Deubzer , Thomas Hierstetter , Petra Gratzl
IPC分类号： B01J31/22 , C07B61/00 , C07F7/08 , C07F7/18 , C08F30/08 , C08G77/14 , C08G77/20 , C08G77/22 , C08G77/38 , C08L83/07 , C09D137/00 , C09D143/04 , C09D183/06 , C09D183/07 , B32B9/04
CPC分类号： C08G77/38 , C08G77/20 , C09D183/06 , Y10T428/31663
摘要： The present invention relates to organosilicon compounds containing (meth)acryloxy groups which can be prepared in a simple manner with high selectivity using readily accessible starting substances. The organopolysiloxanes containing (meth)acryloxy groups rapidly crosslink in the presence of a photoinitiator and light. The compounds of the present invention may be employed in the production of coatings.
摘要翻译：本发明涉及含有（甲基）丙烯酰氧基的有机硅化合物，其可以使用容易获得的起始物质以高选择性以简单的方式制备。含有（甲基）丙烯酰氧基的有机聚硅氧烷在光引发剂和光的存在下迅速交联。本发明的化合物可用于制备涂料。

4. 发明授权

US5241034A Siloxane copolymers containing alkenyl groups, their preparation and use 失效
标题翻译：含有烯烃基团的硅氧烷共聚物，其制备和使用
公开(公告)号：US5241034A
公开(公告)日：1993-08-31
申请号：US913089
申请日：1992-07-14
申请人： Christian Herzig , Bernward Deubzer , David Huettner
发明人： Christian Herzig , Bernward Deubzer , David Huettner
IPC分类号： C08G77/20 , C08G77/22 , C08G77/38 , C08G77/50 , C08L83/05 , C08L83/07 , C08L83/14 , C09D183/04 , C09D183/05 , C09D183/07 , C09D183/14
CPC分类号： C08L83/14 , C08G77/50 , C09D183/14
摘要： Siloxane copolymers containing alkenyl groups are prepared by reacting an organic compound (1) containing at least two aliphatic double bonds of the general formulaR.sup.2 (CR.sup.3 .dbd.CH.sup.2).sub.xin which R.sup.2 is a divalent, trivalent or tetravalent hydrocarbon radical having from 1 to 25 carbon atoms per radical, R.sup.3 is a hydrogen atom or an alkyl radical having from 1 to 6 carbon atoms per radical and x is 2, 3 or 4, with an organopolysiloxane (2) having an average of more than one Si-bonded hydrogen atom per molecule, in the presence of a catalyst (3) which promotes the addition of Si-bonded hydrogen to an aliphatic double bond, in which the ratio between the aliphatic double bond in the organic compound (1) and the Si-bonded hydrogen in the organopolysiloxane (2) is such that the alkenyl containing siloxane copolymers thus obtained have an average of more than one alkenyl group per molecule of the formula --CR.sup.3 .dbd.CH.sup.2, in which R.sup.3 is the same as above.
摘要翻译：含有烯基的硅氧烷共聚物是通过使含有至少两个通式R 2（CR 3 = CH 2）x的脂肪族双键的有机化合物（1）反应来制备的，其中R 2是具有1至25的二价，三价或四价烃基每个基团的碳原子，R3是氢原子或每个基团具有1至6个碳原子并且x为2,3或4的烷基，与平均具有多于一个Si键合氢原子的有机聚硅氧烷（2）在催化剂（3）的存在下，在有机化合物（1）中的脂族双键与Si键合氢之间的比例促进将Si键合的氢加成到脂族双键中的催化剂（3）有机聚硅氧烷（2）使得由此获得的含烯基的硅氧烷共聚物每分子具有平均多于一个烯基的式-CR 3 = CH 2，其中R 3与上述相同。

5. 发明授权

US5621057A Alkenyl ether-siloxane compositions which can be crosslinked by free radicals 失效
标题翻译：可以通过自由基交联的烯基醚 - 硅氧烷组合物
公开(公告)号：US5621057A
公开(公告)日：1997-04-15
申请号：US455489
申请日：1995-05-31
申请人： Christian Herzig , Bernward Deubzer , Martina Bloechl , David Huettner , Walter Magee
发明人： Christian Herzig , Bernward Deubzer , Martina Bloechl , David Huettner , Walter Magee
IPC分类号： C08F283/12 , C08F290/00 , C08L83/04 , C08L83/07 , C09D4/00 , C08F26/00
CPC分类号： C08F283/124
摘要： Alkenyl ether-siloxane compositions comprising(A) an oligomeric or polymeric organosilicon compound having on average more than one alkenyloxy group of the formulaR.sup.2 --CH.dbd.CH--O-- (VI)(B) a monomeric maleic and/or fumaric acid compound of the formula ##STR1## in which R.sup.2 is a hydrogen atom or the methyl radical,R.sup.3 is identical or different and is a hydrogen atom, a hydrocarbon radical having 1 to 16 carbon atoms, which can be interrupted by oxygen, sulfur or oxygen- or silicon-containing units, a substituted hydrocarbon radical having 1 to 6 carbon atoms, a silyl radical or a siloxanyl radical,R.sup.4 is identical or different and is a hydrogen atom, chlorine, bromine, fluorine or an optionally substituted alkyl radical andZ is an oxygen atom or a radical --NR.sup.5 --, where R.sup.5 has one of the meanings given for R.sup.3,optionally(C) initiators which form free radicals and optionally(D) inhibitors for regulating the pot life.
摘要翻译：烯基醚 - 硅氧烷组合物，其包含（A）具有平均多于一个式R 2 -CH = CH-O-（VI）的烯氧基的低聚或聚合有机硅化合物（B）（B）单体马来酸和/或富马酸化合物该式为氢原子或甲基，R3相同或不同，为氢原子，可被氧，硫或含氧或含硅单元中断的碳原子数为1〜16的烃基，具有1至6个碳原子的取代烃基，甲硅烷基或硅氧烷基，R4相同或不同，为氢原子，氯，溴，氟或任选取代的烷基，Z为氧原子或基团 - NR5-，其中R5具有R3给出的含义之一，任选的（C）引发剂，其形成自由基和任选的（D）抑制剂以调节适用期。

6. 发明授权

US5998562A Permanent organosilicon compounds, their preparation and use 失效
标题翻译：永久性有机硅化合物，其制备和用途
公开(公告)号：US5998562A
公开(公告)日：1999-12-07
申请号：US888934
申请日：1997-07-07
申请人： Guenter Mahr , Jochen Dauth , Bernward Deubzer , Monika Ott , Petra Gratzl , Hans Lautenschlager
发明人： Guenter Mahr , Jochen Dauth , Bernward Deubzer , Monika Ott , Petra Gratzl , Hans Lautenschlager
IPC分类号： C14C11/00 , C07F7/10 , C07F7/18 , C08G77/10 , C08G77/26 , C08G77/388 , C08G77/54 , D06M15/643 , C08G77/08
CPC分类号： C08G77/388 , C08G77/54 , Y10S8/01
摘要： The present invention relates to triazine-containing organosilicon compounds having units of the formulaA.sub.a R.sub.b X.sub.c SiO.sub.(4-a-b-c)/2 (I),whereR is identical or different and denotes a hydrogen atom or a monovalent substituted or unsubstituted hydrocarbon radical, having 1 to 26 carbon atoms, preferably 1 to 18 per radical,X is identical or different and is a halogen atom, a chlorine atom or a radical of the formula --OR.sup.1, where R.sup.1 denotes an alkyl radical, having 1 to 18 carbon atoms, preferably 1 to 8 per radical and which may be substituted by an ether oxygen atom,a is 0 or 1, preferably 0.01-0.5b is 0, 1, 2 or 3, preferably 0.5-3.0c is 0, 1, 2 or 3, preferably 0.0-2.0 and the sum a+b+c.ltoreq.4, preferably 0.1-3.5, andA is a radical of the formula ##STR1## where R.sup.2 is an unbranched or branched, optionally substituted alkylene radical, having 1 to 18, preferably 1 to 12, carbon atoms,Y is identical or different and denotes a hydrogen atom or an unbranched or branched alkyl radical, having 1 to 12, preferably 1 to 8, carbon atoms or denotes a radical of the formula --OR.sup.1, where R.sup.1 has the meaning given above, andZ is identical or different and denotes X, --NR.sub.2, --(O)CR or --SR, where X and R have the meanings given above with the proviso that at least one radical A containing at least one halogen atom, preferably a chlorine atom, is present per polymer molecule.
摘要翻译：本发明涉及具有式AaRbXcSiO（4-abc）/ 2（I）单元的含三嗪的有机硅化合物，其中R相同或不同，表示氢原子或一价取代或未取代的烃基，其具有1至 26个碳原子，优选1至18个基团，X相同或不同，为卤素原子，氯原子或式-OR1基团，其中R1表示具有1至18个碳原子的烷基，优选1 至8个，并且可被醚氧原子取代，a为0或1，优选为0.01-0.5b为0,1,2或3，优选0.5-3.0c为0,1,2或3，优选为总和a + b + c 4，优选0.1-3.5，A是下式的基团，其中R 2是无支链或支链的任选取代的亚烷基，其具有1至18，优选1至 12，碳原子，Y相同或不同，表示氢原子或无支链或支链烷基，具有1至12个，优选为1〜8个碳原子，或表示式-OR1的基团，其中R1具有上述含义，Z相同或不同，表示X，-NR2， - （O）CR或-SR，其中X和 R具有上述含义，条件是每个聚合物分子存在至少一个含有至少一个卤素原子，优选氯原子的基团A.

7. 发明授权

US06251313B1 Process for the preparation of microencapsulated products having organopolysiloxane walls 失效
标题翻译：制备具有有机聚硅氧烷壁的微囊化产品的方法
公开(公告)号：US06251313B1
公开(公告)日：2001-06-26
申请号：US09261401
申请日：1999-03-03
申请人： Bernward Deubzer , Jochen Dauth
发明人： Bernward Deubzer , Jochen Dauth
IPC分类号： B01J1302
CPC分类号： B01J13/18 , B01J13/04 , Y10T428/257 , Y10T428/2982
摘要： In the preparation of microcapsules having shell walls of organopolysiloxane and a core material, the shell walls are produced in situ by hydrolysis and polycondensation of organosilanes and/or their condensates having not more than 4 silicon atoms.
摘要翻译：在制备具有有机聚硅氧烷和核心材料的壳壁的微胶囊时，壳壁通过有机硅烷和/或其具有不超过4个硅原子的缩合物的水解和缩聚而原位制备。

8. 发明授权

US5869726A Process for preparing organosilicon compounds containing (meth)acryloxy groups 失效
标题翻译：制备含有（甲基）丙烯酰氧基的有机硅化合物的方法
公开(公告)号：US5869726A
公开(公告)日：1999-02-09
申请号：US931723
申请日：1997-09-16
申请人： Jochen Dauth , Bernward Deubzer , Petra Gratzl , Josef Wolferseder
发明人： Jochen Dauth , Bernward Deubzer , Petra Gratzl , Josef Wolferseder
IPC分类号： C08G77/12 , C08G77/20 , C08G77/38 , C09D183/06 , C09D183/07 , C07F7/08
CPC分类号： C09D183/06 , C08G77/38
摘要： A novel process for preparing organosilicon compounds containing (meth)acxyloxy groups is described, in which alkoxylated alk-2-yne 1,4-di(meth)acrylates (1) of the formula ##STR1## where R.sup.2 is a hydrogen atom or a methyl radical,R.sup.3 is a linear or branched alkylene radical having from 1 to 6 carbon atoms per radical andR.sub.4 is a linear or branched alkylene radical having from 1 to 6 carbon atoms per radical, andz is an integer from 1 to 12,are reacted with organosilicon compounds (2) comprising units of the formula ##STR2## where R is an identical or different monovalent, optionally halogenated hydrocarbon radical having from 1 to 18 carbon atoms per radical, ande is 0 or 1, on average from 0.01 to 1.0,f is 0, 1, 2 or 3, on average from 0.0 to 3.0, andhaving at least one Si-bonded hydrogen atom per molecule in the presence of catalysts (3) which promote the addition Si-bonded hydrogen onto aliphatic multiple bonds and also in the presence of polymerization inhibitors (4), where alkoxylated alk-2-yne 1,4-di(meth)acrylates (1) are used in amounts of from 1.01 to 1.5 mole per gram atom of Si-bonded hydrogen in organosilicon compound (2).
摘要翻译：描述了制备含有（甲基）丙氧基的有机硅化合物的新方法，其中式（II）的烷氧基化烷基-2-炔基1,4-二（甲基）丙烯酸酯（1）其中R2是氢原子或甲基，R3是每个基团具有1至6个碳原子的直链或支链亚烷基，R4是每个基团具有1至6个碳原子的直链或支链亚烷基，z是1至 12与包含式（III）的单元的有机硅化合物（2）反应，其中R是相对或不同的每个基团具有1至18个碳原子的单价，任选卤代烃基，e是0或1 平均为0.01〜1.0，f为0,1,2或3，平均为0.0〜3.0，在催化剂（3）的存在下，每分子具有至少一个Si键合的氢原子，促进Si的添加键合的氢键到脂族多重键上，并且在聚合抑制剂的存在下（4），其中烷氧基化的烷基-2-炔1,4-二（甲基）丙烯酸酯（1）的用量为有机硅化合物（2）中每克原子的Si键合氢的1.01至1.5摩尔。

9. 发明授权

US5605983A Soluble organopolysiloxane free-radical macroinitators for graft copolymerization 失效
标题翻译：用于接枝共聚的可溶性有机聚硅氧烷自由基大分子
公开(公告)号：US5605983A
公开(公告)日：1997-02-25
申请号：US360102
申请日：1994-12-20
申请人： Jochen Dauth , Catherine Oleggini , Bernward Deubzer
发明人： Jochen Dauth , Catherine Oleggini , Bernward Deubzer
IPC分类号： C08F4/00 , C08F283/12 , C08G77/48 , C08G77/392 , C08G77/388
CPC分类号： C08G77/48 , C08F283/12
摘要： The invention relates to partially crosslinked organopolysiloxanes which contain a radical forming group, a base-catalyzed process for their preparation, graft copolymers produced from these organopolysiloxanes and a process for the preparation of the graft copolymers. The present invention avoids problems related to known methods wherein a considerable portion of the organopolymer chains do not graft to the organopolysiloxane graft back-bone but remain as an unattached homopolymers.
摘要翻译：本发明涉及含有自由基形成基团的部分交联的有机聚硅氧烷，其制备的碱催化方法，由这些有机聚硅氧烷制备的接枝共聚物和制备接枝共聚物的方法。本发明避免了与已知方法相关的问题，其中相当大一部分的有机聚合物链不接枝到有机聚硅氧烷移植物背骨上，而是保留为未附着的均聚物。

10. 发明授权

US5561231A Homogeneous hydrosilylation catalysts 失效
标题翻译：均相氢化硅烷化催化剂
公开(公告)号：US5561231A
公开(公告)日：1996-10-01
申请号：US276922
申请日：1994-07-19
申请人： Jochen Dauth , Bernward Deubzer , Hans Bindl , Udo Peetz
发明人： Jochen Dauth , Bernward Deubzer , Hans Bindl , Udo Peetz
IPC分类号： B01J31/22 , C07B61/00 , C07F7/08 , C07F7/18 , C07F15/00 , C08G77/06 , C08G77/26 , C08G77/38 , C08G77/388 , C08G77/398 , C08K5/00 , C08L83/05 , C08L83/07 , C07F7/02
CPC分类号： C08G77/398 , C07F15/006 , C07F15/0066 , C07F15/0086 , C07F15/0093 , C07F7/0854 , C07F7/1876 , C08G77/26 , C08G77/388 , C08K5/0091
摘要： Transition metal-containing organosiloxanes of at least three organosiloxane units, comprising at least one transition metal complex, chemically bonded via ligands selected from among amino, phosphino or sulfido groups of Pt, Pd, Rh, Ru, Os or Ir, excluding those organosiloxanes which contain exclusively Pt(O) complexes bonded via amino ligands, are used as homogeneous hydrosilylation catalysts.
摘要翻译：至少有三个有机硅氧烷单元的过渡金属的有机硅氧烷包含至少一个过渡金属配合物，通过选自Pt，Pd，Rh，Ru，Os或Ir的氨基，膦基或硫基中的配体化学键合，不包括那些有机硅氧烷仅含有通过氨基配体键合的Pt（O）配合物，被用作均匀的氢化硅烷化催化剂。

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