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1. 发明授权

US07252781B2 Solutions of polymer semiconductors 有权
标题翻译：聚合物半导体解决方案
公开(公告)号：US07252781B2
公开(公告)日：2007-08-07
申请号：US10487665
申请日：2002-08-22
申请人： Hubert Spreitzer , Heinrich Becker , Willi Kreuder , Sybille Berg , Andreas Sauer
发明人： Hubert Spreitzer , Heinrich Becker , Willi Kreuder , Sybille Berg , Andreas Sauer
IPC分类号： C08K5/01
CPC分类号： C08G61/02 , H01L51/0003 , H01L51/0004 , H01L51/0508 , H01L51/42 , H01L51/5012 , Y02E10/549 , Y02P70/521
摘要： The present invention relates to a process for producing particle-free solutions of polymeric semiconductors and to their use for producing layers of polymeric semiconductors in polymeric organic light-emitting diodes (PLEDs), organic integrated circuits (O-ICs), organic field effect transistors (OFETs), organic thin film transistors (OTFTs), organic solar cells (O-SCs) or organic laser diodes (O-lasers).
摘要翻译：本发明涉及一种用于生产聚合物半导体的无颗粒溶液的方法及其在聚合有机发光二极管（PLED），有机集成电路（O-IC），有机场效应晶体管中产生聚合物半导体层的用途（OFET），有机薄膜晶体管（OTFT），有机太阳能电池（O-SC）或有机激光二极管（O激光器）。

2. 发明授权

US06638646B2 Substituted poly(arylenevinylenes), process for their preparation, and their use in electroluminescent elements 有权
标题翻译：取代的聚（亚芳基亚乙烯基），其制备方法及其在电致发光元件中的应用
公开(公告)号：US06638646B2
公开(公告)日：2003-10-28
申请号：US10185061
申请日：2002-06-28
申请人： Hubert Spreitzer , Willi Kreuder , Heinrich Becker , Hermann Schenk , Nu Yu
发明人： Hubert Spreitzer , Willi Kreuder , Heinrich Becker , Hermann Schenk , Nu Yu
IPC分类号： H05B3300
CPC分类号： H01L51/0038 , C08G61/02 , C09K11/06 , H01B1/128 , H01L51/5012 , H05B33/14 , Y10S428/917
摘要： Poly(arylenevinylenes) comprising at least 20% of recurring units of the formula (I), where the symbols and indices have the following meanings: Aryl: is an aryl group having 4 to 14 carbon atoms; R′: is a substituent which is either in the labeled phenylene position 5 or 6 and is CN, F, Cl, N(R1R2) or a straight-chain, branched or cyclic alkyl, alkoxy or thioalkoxy group having 1 to 20 carbon atoms, in which, in addition, one or more H atoms may be replaced by F; R″: are identical or different and are CN, F, Cl or a straight-chain, branched or cyclic alkyl or alkoxy group having 1 to 20 carbon atoms, where one or more non-adjacent CH2 groups may be replaced by —O—, —S—, —CO—, —COO—, —O—CO—, —NR1—, —(NR2R3)+—A− or —CONR4—, and where one or more H atoms may be replaced by F, or an aryl group having 4 to 14 carbon atoms, which may be substituted by one or more non-aromatic radicals R′; R1, R2, R3, R4 are identical or different and are H or an aliphatic or aromatic hydrocarbon radical having 1 to 20 carbon atoms; A−: is a singly charged anion or an equivalent thereof; and n: is 0, 1, 2, 3, 4 or 5, are suitable as electroluminescent material.
摘要翻译：包含至少20％式（I）的重复单元的聚（亚芳基亚乙烯基烯烃），其中符号和指数具有以下含义：芳基：具有4至14个碳原子的芳基; R'是在标记的亚苯基位置5或6中，是CN，F，Cl，N（R 1 R 2）或具有1至20个碳原子的直链，支链或环烷基，烷氧基或硫代烷氧基，其中，另外一个或多个H原子可被F取代; R“：相同或不同，为CN，F，Cl或具有1至20个碳的直链，支链或环状烷基或烷氧基原子，其中一个或多个不相邻的CH 2基团可被-O - ， - S - ， - CO - ， - COO - ， - O-CO - ， - NR 1 - ， - （NR 2） R 3）+ - 或-CONR 4 - ，并且其中一个或多个H原子可以被F取代，或者可以被4〜14个碳原子的芳基取代，可以被一个或多个非芳族基团R'; R 1，R 2，R 3，R 4相同或不同，为H或脂族或芳族氢具有1至20个碳原子的羰基; A 1是单电荷阴离子或其等同物; 和n为0,1,2,3,4或5，适合作为电致发光材料。

3. 发明授权

US06476265B1 Method for producing aryl oligoamines 有权
标题翻译：芳基寡胺的制备方法
公开(公告)号：US06476265B1
公开(公告)日：2002-11-05
申请号：US09486867
申请日：2000-05-10
申请人： Hubert Spreitzer , Willi Kreuder , Heinrich Becker , Ute Neumann
发明人： Hubert Spreitzer , Willi Kreuder , Heinrich Becker , Ute Neumann
IPC分类号： C07C21100
CPC分类号： C07D279/22 , C07C209/10 , C07C213/08 , C07C2603/94 , H01L51/0052 , H01L51/0059 , Y02E10/549 , C07C211/61 , C07C217/92
摘要： In a process for preparing aryl oligoamines, an amine is reacted with an activated aromatic and a base in a temperature range from 0 to 150° C. in the presence of a palladium component and a phosphine ligand. The aryl oligoamines are obtained simply and in good yields.
摘要翻译：在制备芳基低聚胺的方法中，在钯组分和膦配位体的存在下，胺在0至150℃的温度范围内与活化的芳族和碱反应。芳基低聚胺简单地和良好的收益率。

4. 发明授权

US06323373B1 Polymerizable biaryls, method for the production and use thereof 有权
标题翻译：可聚合联芳基，其生产和使用方法
公开(公告)号：US06323373B1
公开(公告)日：2001-11-27
申请号：US09319606
申请日：1999-06-09
申请人： Hubert Spreitzer , Willi Kreuder , Heinrich Becker , Jochen Krause
发明人： Hubert Spreitzer , Willi Kreuder , Heinrich Becker , Jochen Krause
IPC分类号： C07C4752
CPC分类号： C09K11/06 , C07B37/04 , C07C17/12 , C07C17/16 , C07C29/147 , C07C45/29 , C07C67/343 , C07C69/76 , C07C69/94 , C07F9/4056 , C08G61/00 , Y10S428/917 , C07C25/02 , C07C22/04 , C07C47/575 , C07C33/46 , C07C33/26
摘要： A process for preparing polymerizable biaryl derivatives comprises reacting an aromatic comprising a 6-membered ring which bears ester or benzylic OH groups in the 1,4 position with a second aromatic in a palladium-catalyzed cross-coupling reaction to give a biaryl and converting the ester or benzylic OH groups into polymerizable groups in one or more steps. The biaryls obtained are suitable for preparing polymers which are used as electroluminescence materials.
摘要翻译：制备可聚合的联芳基衍生物的方法包括在钯催化的交叉偶联反应中使包含在1,4位上具有酯或苄基OH基团的6元环的芳族化合物与第二芳族化合物反应，得到联芳基并将酯或苄基OH基团在一个或多个步骤中转化成可聚合基团。获得的联芳基适用于制备用作电致发光材料的聚合物。

5. 发明授权

US06458909B1 Aryl-substituted poly (p-arylene-vinylenes), process for their preparation and their use in electroluminescence components 失效
标题翻译：芳基取代的聚（对亚芳基 - 亚乙烯基），其制备方法及其在电致发光组分中的应用
公开(公告)号：US06458909B1
公开(公告)日：2002-10-01
申请号：US08991559
申请日：1997-12-16
申请人： Hubert Spreitzer , Willi Kreuder , Heinrich Becker , Harmannus Schoo , Robert Demandt
发明人： Hubert Spreitzer , Willi Kreuder , Heinrich Becker , Harmannus Schoo , Robert Demandt
IPC分类号： C08F13800
CPC分类号： H01L51/5012 , C08G61/02 , C09B69/105 , C09K11/06 , H01L51/0038
摘要： Poly(p-arylene-vinylenes) comprising repeating units of the formula (I), where the symbols and indices have the following meanings: Y1, Y2, Y3: identical or different, CH, N; Aryl: an aryl group having from 4 to 14 carbon atoms; R′, R″: identical or different, each a straight-chain or branched or cyclic alkyl or alkoxy group having from 1 to 20 carbon atoms, where one or more non-adjacent CH2 groups may be replaced by —O—, —S—, —CO—, —COO—, —O—CO—, —NR1—, —(NR2R3)+—A−, or —CONR4— and one or more H atoms may be replaced by F, or else CN, F, Cl or an aryl group having from 4 to 14 carbon atoms which may be substituted by one or more nonaromatic radicals R′; R1, R2, R3, R4: identical or different, aliphatic or aromatic hydrocarbon radicals having from 1 to 20 carbon atoms or else H; A−: a singly charged anion or its equivalent; m: 0, 1 or 2; n: 1, 2, 3, 4 or 5; are suitable as electroluminescence materials.
摘要翻译：包含式（I）重复单元的聚（对亚芳基 - 烯烃），其中符号和指数具有以下含义：Y1，Y2，Y3：相同或不同，CH，N;芳基：具有4 至14个碳原子; R'，R“：相同或不同，各自为具有1至20个碳原子的直链或支链或环状烷基或烷氧基，其中一个或多个不相邻的CH 2基团可以被 -O-，-S-，-CO-，-COO-，-O-CO-，-NR1-， - （NR2R3）+ -A-或-CONR4-，一个或多个H原子可被F ，或CN，F，Cl或具有4至14个碳原子的芳基，其可以被一个或多个非芳族基团R 1取代; R 1，R 2，R 3，R 4：相同或不同的脂族或芳族烃基，其具有 1至20个碳原子或H; A-：单电荷阴离子或其等价物; m：0,1或2; n：1,2,3,4或5;适合作为电致发光材料。

6. 发明授权

US06541602B1 Conjugated polymers containing 2,7 fluorenyl units with improved properties 有权
标题翻译：含有2,7个芴基单元的共轭聚合物具有改进的性能
公开(公告)号：US06541602B1
公开(公告)日：2003-04-01
申请号：US09806730
申请日：2001-05-02
申请人： Hubert Spreitzer , Heinrich Becker , Willi Kreuder
发明人： Hubert Spreitzer , Heinrich Becker , Willi Kreuder
IPC分类号： C08G7908
CPC分类号： C08G61/02 , C08G61/10 , C09K11/06
摘要： The present invention describes novel polymers, their use as organic semiconductors and/or electroluminescent materials, and electro-luminescent devices containing polymers of this type.
摘要翻译：本发明描述了新颖的聚合物，它们作为有机半导体和/或电致发光材料的用途，以及含有这种聚合物的电致发光器件。

7. 发明授权

US06653438B1 Conjugated polymers containing special fluorene structural elements with improved properties 失效
标题翻译：含有特殊芴结构元素的共轭聚合物具有改进的性能
公开(公告)号：US06653438B1
公开(公告)日：2003-11-25
申请号：US09806707
申请日：2001-04-26
申请人： Hubert Spreitzer , Heinrich Becker Zum , Willi Kreuder
发明人： Hubert Spreitzer , Heinrich Becker Zum , Willi Kreuder
IPC分类号： C08G7908
CPC分类号： C09K11/06 , C07C43/225 , C07C2603/18 , C07F5/025 , C07F7/2208 , C08G61/10 , C09B69/109 , H01L51/0039
摘要： The invention relates to novel polymers containing fluorene structural elements, monomer parent compounds upon which said polymers are based, and the use of said inventive polymers as organic semiconductors and/or as electroluminescent material, in addition to electroluminescent devices containing said polymers.
摘要翻译：本发明涉及除含有所述聚合物的电致发光器件之外，含有芴结构元件的新型聚合物，所述聚合物所基于的单体母体化合物以及所述本发明聚合物作为有机半导体和/或电致发光材料的用途。

8. 发明授权

US06509507B2 Polymerizable biaryls, process for their preparation and their use 有权
公开(公告)号：US06509507B2
公开(公告)日：2003-01-21
申请号：US09981866
申请日：2001-10-16
申请人： Hubert Spreitzer , Willi Kreuder , Heinrich Becker , Jochen Krause
发明人： Hubert Spreitzer , Willi Kreuder , Heinrich Becker , Jochen Krause
IPC分类号： C07C4752
CPC分类号： C09K11/06 , C07B37/04 , C07C17/12 , C07C17/16 , C07C29/147 , C07C45/29 , C07C67/343 , C07C69/76 , C07C69/94 , C07F9/4056 , C08G61/00 , Y10S428/917 , C07C25/02 , C07C22/04 , C07C47/575 , C07C33/46 , C07C33/26
摘要： A process for preparing polymerizable biaryl derivatives comprises reacting an aromatic comprising a 6-membered ring which bears ester or benzylic OH groups in the 1,4 position with a second aromatic in a palladium-catalyzed cross-coupling reaction to give a biaryl and converting the ester or benzylic OH groups into polymerizable groups in one or more steps. The biaryls obtained are suitable for preparing polymers which are used as electroluminescence materials.

9. 发明授权

US06414431B1 Thin film electrode for planar organic light-emitting devices and method for its production 失效
标题翻译：平面有机发光装置用薄膜电极及其制造方法
公开(公告)号：US06414431B1
公开(公告)日：2002-07-02
申请号：US09446744
申请日：2000-03-13
申请人： Nu Yu , Hubert Spreitzer , Hermann Schenk , Willi Kreuder , Heinrich Becker
发明人： Nu Yu , Hubert Spreitzer , Hermann Schenk , Willi Kreuder , Heinrich Becker
IPC分类号： H05B3326
CPC分类号： H05B33/26 , H01L51/5209 , H01L51/5221 , Y10S428/917
摘要： An electroluminescent device, comprising at least one organic light emitting layer (103) sandwiched between two electrode layers (102, 104), wherein the ratio r of the sheet resistances of the bottom electrode layer (102) and the top electrode layer (104) is 0.3
摘要翻译：一种电致发光器件，包括夹在两个电极层（102,104）之间的至少一个有机发光层（103），其中底部电极层（102）和顶部电极层（104）的薄层电阻的比率r 是0.3 <= r <= 3。

10. 发明授权

US06994893B2 Solutions and dispersions of organic semiconductors 失效
标题翻译：有机半导体的解决方案和分散体
公开(公告)号：US06994893B2
公开(公告)日：2006-02-07
申请号：US10469334
申请日：2002-03-07
申请人： Hubert Spreitzer , Heinrich Becker , Kevin Treacher , Susanne Heun , Andreas Sauer
发明人： Hubert Spreitzer , Heinrich Becker , Kevin Treacher , Susanne Heun , Andreas Sauer
IPC分类号： B05D1/26
CPC分类号： C09K11/06 , C09K2211/14 , H01L51/0004 , H01L51/0007
摘要： The present invention relates to solutions and/or dispersions of organic semiconductors in a solvent mixture of at least two different organic solvents, characterized in that A. Each of the solvents on its own has a boiling point of below 200° C. and a melting point of 15° C. or less, B. at least one of the solvents has a boiling point in the range from greater than 140 to less than 200° C., C. the solvents used have no benzylic CH2 or CH groups, D. the solvents used are not benzene derivatives containing tert-butyl substituents or more than two methyl substituents, and their use in printing processes for producing layers of organic semiconductors, especially for the electronics industry.
摘要翻译：本发明涉及有机半导体在至少两种不同有机溶剂的溶剂混合物中的溶液和/或分散体，其特征在于

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