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1. 发明授权

US07951494B2 Solid electrolyte with high ion-conductivity and method for manufacturing the same, and electrochemical system using solid electrolyte 有权
标题翻译：具有高离子电导率的固体电解质及其制造方法，以及使用固体电解质的电化学系统
公开(公告)号：US07951494B2
公开(公告)日：2011-05-31
申请号：US12165860
申请日：2008-07-01
申请人： Haruo Sawa , Haruyuki Nakanishi , Shinichi Matsumoto
发明人： Haruo Sawa , Haruyuki Nakanishi , Shinichi Matsumoto
IPC分类号： H01M6/18 , G01N27/26
CPC分类号： C25B13/08 , C08J5/2256 , C08J5/2268 , C08J2329/04 , C08J2379/04 , H01M6/181 , H01M6/188 , H01M8/0289 , H01M8/1027 , H01M8/103 , H01M8/1046 , H01M8/1072 , H01M10/056 , H01M10/26 , H01M10/347 , H01M2300/0082 , H01M2300/0091 , Y02P70/56
摘要： The present invention provides a solid electrolyte with high ion-conductivity which is cheap and exhibits high conductivity in an alkaline form, and stably keeps high conductivity because of a small amount of the leak of a compound bearing conductivity even in a wet state. The invention is useful in an electrochemical system using the solid electrolyte, such as a fuel cell.The solid electrolyte with high ion-conductivity comprises a hybrid compound which contains at least polyvinyl alcohol and a zirconic acid compound, and also a nitrogen-containing organic compound having a structure of amine, quaternary ammonium compound and/or imine, obtained by hydrolyzing a zirconium salt or an oxyzirconium salt in a solution including water, polyvinyl alcohol, a zirconium salt or an oxyzirconium salt and a nitrogen-containing organic compound having a structure of amine, quaternary ammonium compound and/or imine coexist, removing a solvent and contacting with alkali.
摘要翻译：本发明提供一种廉价且具有高导电性的碱性形式的高离子电导率的固体电解质，并且由于即使在潮湿状态下也具有导电性的化合物的泄漏量少，因而稳定地保持高导电性。本发明在使用诸如燃料电池的固体电解质的电化学系统中是有用的。具有高离子传导性的固体电解质包括至少包含聚乙烯醇和锆酸化合物的杂化化合物，以及具有胺，季铵化合物和/或亚胺结构的含氮有机化合物，其通过水解锆盐或氧锆盐在包括水，聚乙烯醇，锆盐或氧锆盐的溶液中，以及具有胺，季铵化合物和/或亚胺结构的含氮有机化合物共存，除去溶剂并与碱。

2. 发明申请

US20090068531A1 SOLID ELECTROLYTE WITH HIGH ION-CONDUCTIVITY AND METHOD FOR MANUFACTURING THE SAME, AND ELECTROCHEMICAL SYSTEM USING SOLID ELECTROLYTE 有权
标题翻译：具有高导电性的固体电解质及其制造方法，以及使用固体电解质的电化学系统
公开(公告)号：US20090068531A1
公开(公告)日：2009-03-12
申请号：US12165860
申请日：2008-07-01
申请人： Haruo SAWA , Haruyuki Nakanishi , Shinichi Matsumoto
发明人： Haruo SAWA , Haruyuki Nakanishi , Shinichi Matsumoto
IPC分类号： H01M8/10 , H01M6/18 , G01N27/26 , C25B9/00 , C01G25/02 , C01B35/12 , C01B33/20 , C01F7/02
CPC分类号： C25B13/08 , C08J5/2256 , C08J5/2268 , C08J2329/04 , C08J2379/04 , H01M6/181 , H01M6/188 , H01M8/0289 , H01M8/1027 , H01M8/103 , H01M8/1046 , H01M8/1072 , H01M10/056 , H01M10/26 , H01M10/347 , H01M2300/0082 , H01M2300/0091 , Y02P70/56
摘要： The present invention provides a solid electrolyte with high ion-conductivity which is cheap and exhibits high conductivity in an alkaline form, and stably keeps high conductivity because of a small amount of the leak of a compound bearing conductivity even in a wet state. The invention is useful in an electrochemical system using the solid electrolyte, such as a fuel cell.The solid electrolyte with high ion-conductivity comprises a hybrid compound which contains at least polyvinyl alcohol and a zirconic acid compound, and also a nitrogen-containing organic compound having a structure of amine, quaternary ammonium compound and/or imine, obtained by hydrolyzing a zirconium salt or an oxyzirconium salt in a solution including water, polyvinyl alcohol, a zirconium salt or an oxyzirconium salt and a nitrogen-containing organic compound having a structure of amine, quaternary ammonium compound and/or imine coexist, removing a solvent and contacting with alkali.
摘要翻译：本发明提供一种廉价且具有高导电性的碱性形式的高离子电导率的固体电解质，并且由于即使在潮湿状态下也具有导电性的化合物的泄漏量少，因而稳定地保持高导电性。本发明在使用诸如燃料电池的固体电解质的电化学系统中是有用的。具有高离子传导性的固体电解质包括至少包含聚乙烯醇和锆酸化合物的杂化化合物，以及具有胺，季铵化合物和/或亚胺结构的含氮有机化合物，其通过水解锆盐或氧锆盐在包括水，聚乙烯醇，锆盐或氧锆盐的溶液中，以及具有胺，季铵化合物和/或亚胺结构的含氮有机化合物共存，除去溶剂并与碱。

3. 发明申请

US20090098466A1 METHOD FOR MANUFACTURING SOLID ELECTROLYTE WITH HIGH ION-CONDUCTIVITY 审中-公开
标题翻译：具有高电导率的固体电解质的制造方法
公开(公告)号：US20090098466A1
公开(公告)日：2009-04-16
申请号：US12056546
申请日：2008-03-27
申请人： Haruo SAWA , Haruyuki Nakanishi , Yusuke Kuzushima
发明人： Haruo SAWA , Haruyuki Nakanishi , Yusuke Kuzushima
IPC分类号： H01M6/18
CPC分类号： H01M8/1016 , C08K3/10 , H01M2300/0088 , Y02P70/56 , C08L29/04
摘要： A method for manufacturing a solid electrolyte with high ion-conductivity comprising a hybrid compound of polyvinyl alcohol and a zirconic acid compound which can prohibit gelation of the raw material solution with keeping the concentration of the raw material solution of the solid electrolyte desirable for efficient manufacture of membranes, and provides the solid electrolyte which is inexpensive, and even functions in an alkaline form is disclosed.The method comprises the steps of hydrolyzing a zirconium salt or an oxyzirconium salt in a solution including a solvent including water, polyvinyl alcohol, and the zirconium salt or the oxyzirconium salt, removing the solvent, and contacting with alkali. The hydrolysis may be carried out by heating to 50° C. or higher or by heating to 50° C. or higher at a pH of 7 or less.
摘要翻译：一种制造具有高离子电导率的固体电解质的方法，其包括聚乙烯醇和锆酸化合物的混合化合物，其可以防止原料溶液凝胶化，同时保持固体电解质的原料溶液的浓度需要有效制造的膜，并且提供廉价的固体电解质，并且甚至公开了碱性形式的功能。该方法包括在包括水，聚乙烯醇，锆盐或氧锆盐的溶剂的溶液中水解锆盐或氧锆盐，除去溶剂和与碱接触的步骤。水解可以通过加热至50℃以上或通过在pH7以下加热至50℃以上进行。

4. 发明授权

US07951903B2 Hydrazone compound, hydrazone compound for forming complex, ligand for forming metal complex, and monomer for manufacturing polymer compound 有权
标题翻译：腙化合物，用于形成络合物的腙化合物，用于形成金属络合物的配体和用于制备高分子化合物的单体
公开(公告)号：US07951903B2
公开(公告)日：2011-05-31
申请号：US12201469
申请日：2008-08-29
申请人： Haruyuki Nakanishi , Shinichi Matsumoto , Hidekazu Arikawa , Hironobu Kumagai
发明人： Haruyuki Nakanishi , Shinichi Matsumoto , Hidekazu Arikawa , Hironobu Kumagai
IPC分类号： C08G73/06
CPC分类号： C07D213/77 , C08G8/10 , C08G8/28
摘要： A hydrazone compound represented by a General Formula (1) below, a hydrazone compound for forming a metal complex, which is represented by the General Formula (1) below and forms a metal complex by coordination to at least one metal species, a ligand for forming a metal complex including the hydrazone compound, and a monomer for manufacturing a polymer compound including the hydrazone compound: wherein, Py represents a 2-pyridyl group, a 3-pyridyl group, or a 4-pyridyl group.
摘要翻译：由下述通式（1）表示的腙化合物，用于形成金属络合物的腙化合物，其由下述通式（1）表示，并与至少一种金属物质配位形成金属络合物，配体为形成包含腙化合物的金属络合物，和用于制造包含腙化合物的高分子化合物的单体：其中，Py表示2-吡啶基，3-吡啶基或4-吡啶基。

5. 发明申请

US20100092826A1 FUEL CELL AND FUEL CELL SYSTEM 审中-公开
标题翻译：燃料电池和燃料电池系统
公开(公告)号：US20100092826A1
公开(公告)日：2010-04-15
申请号：US12449330
申请日：2008-02-07
申请人： Haruyuki Nakanishi , Yusuke Kuzushima , Norihiko Nakamura , Shinichi Matsumoto , Hidekazu Arikawa , Kazuya Uchisasai
发明人： Haruyuki Nakanishi , Yusuke Kuzushima , Norihiko Nakamura , Shinichi Matsumoto , Hidekazu Arikawa , Kazuya Uchisasai
IPC分类号： H01M8/10 , H01M8/08
CPC分类号： H01M8/222 , H01M8/083 , H01M8/1011 , H01M8/1013 , Y02E60/522 , Y02E60/523
摘要： A fuel cell has an electrolyte, an anode provided on one side of the electrolyte and a cathode provided on the other side of the electrolyte, and a fuel passage which is formed so as to contact the anode and through which fuel flows. A substance having an ion-conducting property is mixed in with the fuel that flows through the fuel passage. For example, fuel is supplied to the fuel passage from a fuel supply apparatus, while a substance having an ion-conducting property is supplied to the fuel passage from an ion-conducting substance supply apparatus.
摘要翻译：燃料电池具有电解质，设置在电解质的一侧上的阳极和设置在电解质的另一侧的阴极以及形成为接触阳极并通过燃料流动的燃料通道。具有离子传导性的物质与流过燃料通道的燃料混合。例如，从燃料供给装置向燃料通路供给燃料，而具有离子传导性的物质从离子传导性物质供给装置供给到燃料通路。

6. 发明申请

US20090200519A1 FINE PARTICLE OF PEROVSKITE OXIDE, PARTICLE HAVING DEPOSITED PEROVSKITE OXIDE, CATALYST MATERIAL, CATALYST MATERIAL FOR OXYGEN REDUCTION, CATALYST MATERIAL FOR FUEL CELL, AND ELECTRODE FOR FUEL CELL 有权
标题翻译：氧化亚铁的细颗粒，具有沉积氧化铝的颗粒，催化材料，氧化还原催化材料，燃料电池催化材料和燃料电极
公开(公告)号：US20090200519A1
公开(公告)日：2009-08-13
申请号：US12304452
申请日：2007-06-12
申请人： Yuko Sawaki , Mikio Kishimoto , Haruyuki Nakanishi , Shigeaki Murata , Masahiro Imanishi , Shinichi Matsumoto
发明人： Yuko Sawaki , Mikio Kishimoto , Haruyuki Nakanishi , Shigeaki Murata , Masahiro Imanishi , Shinichi Matsumoto
IPC分类号： H01B1/08 , B01J23/10 , H01B1/24
CPC分类号： H01M4/925 , C01G49/0018 , C01G49/009 , C01P2002/34 , C01P2002/77 , H01M4/9016 , H01M4/9033 , H01M4/9083 , H01M4/92 , H01M8/1007 , H01M2008/1095
摘要： A catalyst for electrodes in solid-polymer fuel cells which comprises metal oxide particles themselves. It can be used as a substituent for the carbon particles having platinum deposited thereon and platinum metal particles which are presently in general use as, e.g., a catalyst for electrodes in fuel cells, and has a possibility that the amount of platinum to be used can be greatly reduced as compared with the conventional carbon particles having platinum deposited thereon, etc.The catalyst comprises fine transition-metal oxide particles having, in the main phase, a perovskite structure represented by the general formula ABO3 (wherein A represents one or more elements selected among lanthanum, strontium, cerium, calcium, yttrium, erbium, praseodymium, neodymium, samarium, europium, silicon, magnesium, barium, niobium, lead, bismuth, and antimony; and B represents one or more elements selected among iron, cobalt, manganese, copper, titanium, chromium, nickel, and molybdenum), the fine oxide particles having lattice constants satisfying the following relationship (1): 1.402
摘要翻译：固体聚合物燃料电池中用于电极的催化剂，其包含金属氧化物颗粒本身。它可以用作其上沉积有铂的碳颗粒和当前通常用作例如燃料电池中的电极催化剂的铂金属颗粒的取代基，并且具有使用的铂的量可能与其上沉积有铂的常规碳颗粒相比，大大降低。催化剂包括在主相中具有由通式ABO 3表示的钙钛矿结构的细小过渡金属氧化物颗粒（其中A表示一种或多种元素选自镧，锶，铈，钙，钇，铒，镨，钕，钐，铕，硅，镁，钡，铌，铅，铋和锑中的一种或多种; B代表选自铁，钴，锰，铜，钛，铬，镍和钼），具有满足以下关系式（1）的晶格常数的微细氧化物粒子：<β在线式 description =“In-line Formulas”end =“lead”？> 1.402 <2b /（a + c）<1.422（1）<？in-line-formula description =“In-line Formulas”end =“tail”？其中a和c表示钙钛矿型晶格的短轴长度，b表示其长轴长度。

7. 发明申请

US20050147870A1 Fuel cell 有权
标题翻译：燃料电池
公开(公告)号：US20050147870A1
公开(公告)日：2005-07-07
申请号：US11026411
申请日：2005-01-03
申请人： Haruyuki Nakanishi , Shinichi Matsumoto
发明人： Haruyuki Nakanishi , Shinichi Matsumoto
IPC分类号： H01M8/24 , H01M4/94 , H01M8/02 , H01M8/04 , H01M8/10
CPC分类号： H01M4/8605 , H01M8/023 , H01M8/0234 , H01M8/0247 , H01M8/0258 , H01M8/0267 , H01M8/0271 , H01M8/0273 , H01M8/04223 , H01M8/04225 , H01M8/1007 , H01M8/242
摘要： A fuel cell includes a diffusion layer formed in a sheet having a small thickness. The fuel cell is assembled with a tension imposed on the sheet in an in-plane direction of the sheet. The tension is imposed on the diffusion layer from a frame disposed outside the fuel cell. The tension is of such a magnitude as to prevent a portion of the sheet positioned corresponding to a gas passage of a separator from being deformed when the fuel cell is assembled and has a tightening force thereby applied thereto. The tension is adjustable according to a fuel cell operating condition. These structures can prevent a separator rib from pushing into a membrane, maintaining the gas passability of the diffusion layer well.
摘要翻译：燃料电池包括形成在具有小厚度的片材中的扩散层。燃料电池以片材的面内方向施加在片材上的张力组装。从设置在燃料电池外侧的框架施加在扩散层上的张力。张力具有如此大的程度，以防止当燃料电池组装时对应于隔板的气体通道定位的片材的一部分变形并且具有由此施加的紧固力。张力可根据燃料电池工作条件进行调节。这些结构可以防止分隔肋推入膜中，保持扩散层的气体通过性良好。

8. 发明申请

US20080152987A1 Fuel cell system and vehicle with fuel cell system mounted thereon 审中-公开
标题翻译：具有燃料电池系统的燃料电池系统和车辆
公开(公告)号：US20080152987A1
公开(公告)日：2008-06-26
申请号：US10809511
申请日：2004-03-26
申请人： Tomoaki Nakashima , Haruyuki Nakanishi , Shinichi Matsumoto
发明人： Tomoaki Nakashima , Haruyuki Nakanishi , Shinichi Matsumoto
IPC分类号： H01M8/04
CPC分类号： H01M8/249 , H01M8/04089 , H01M8/04126 , H01M8/0432 , H01M8/04492 , H01M8/04559 , H01M8/04589 , H01M8/04619 , H01M8/04649 , H01M8/04761 , H01M8/241 , H01M8/2483
摘要： A fuel cell system of the invention includes a tubular switching member 70 with slits 70a to shift their position and thereby vary an opening area of outlets of oxidizing gas conduits 36 in respective unit fuel cells 30 constituting a fuel cell stack 20. The system further includes a drive roller 74 and a stepping motor 79 that function to change over the position of the slits 70a. An electronic control unit controls rotation of the stepping motor 79 to actuate the tubular switching member 70 first to narrow the opening area of the outlets of the oxidizing gas conduits 36 to or toward 0 and then to widen the opening area of the outlets of the oxidizing gas conduits 36, thereby generating pulsation in the oxidizing gas conduits 36. Water droplets flocculated in the oxidizing gas conduits 36 are thus discharged to the outlets with high efficiency. The structure of the embodiment does not require any bypass in the respective unit fuel cells 30. The characteristic structure of the invention uses the frame of the unit fuel cell 30 equivalent to the existing one and does not substantially increase the size of the fuel cell stack 20.
摘要翻译：本发明的燃料电池系统包括管状切换构件70，其具有狭缝70a以使其位置偏移，从而改变构成燃料电池堆20的各个单位燃料电池30中的氧化气体导管36的出口的开口面积。系统进一步包括用于切换狭缝70a的位置的驱动辊74和步进马达79。电子控制单元控制步进电动机79的旋转，首先致动管状切换构件70，使氧化剂气体导管36的出口的开口面积缩小到0°，然后扩大氧化剂的出口的开口面积气体管道36，从而在氧化气体导管36中产生脉动。因此，氧化气体管道36中絮凝的水滴以高效率排放到出口。本实施例的结构在相应的单元燃料电池30中不需要任何旁路。本发明的特征结构使用与现有燃料电池相当的单元燃料电池30的框架，并且基本上不增加燃料电池堆的尺寸 20。

9. 发明授权

US07175933B2 Fuel cell system and vehicle with fuel cell system mounted thereon 有权
标题翻译：具有燃料电池系统的燃料电池系统和车辆
公开(公告)号：US07175933B2
公开(公告)日：2007-02-13
申请号：US10777659
申请日：2004-02-13
申请人： Haruyuki Nakanishi , Shinichi Matsumoto
发明人： Haruyuki Nakanishi , Shinichi Matsumoto
IPC分类号： H01M2/00
CPC分类号： H01M8/04171 , B60L1/003 , B60L11/1883 , B60L11/1892 , B60L11/1898 , B60L2240/12 , H01M8/0213 , H01M8/0258 , H01M8/026 , H01M8/04119 , H01M8/04141 , H01M8/241 , H01M8/2457 , H01M8/2483 , H01M8/2484 , Y02T90/34
摘要： A fuel cell system of the invention includes outer-conduit water absorbing members that are arranged outside oxidizing gas conduits of respective unit fuel cells, and a changeover mechanism that changes over the status of the outer-conduit water absorbing members between an absorption state in which the outer-conduit water absorbing members absorb moisture in the oxidizing gas conduits and a non-absorption state in which the outer-conduit water absorbing members do not absorb the moisture in the oxidizing gas conduits. Control of this changeover mechanism effectively regulates the moisture level in the oxidizing gas conduits.
摘要翻译：本发明的燃料电池系统包括布置在各单位燃料电池的氧化气体管道外部的外部管道吸水件，以及一个转换机构，其将外部管道吸水件的状态在其中外部导管吸水部件吸收氧化气体导管中的水分和外部导管吸水部件不吸收氧化气体导管内的水分的非吸收状态。该转换机构的控制有效地调节氧化气体管道中的水分含量。

10. 发明授权

US06592741B2 Fuel gas generation system and generation method thereof 失效
公开(公告)号：US06592741B2
公开(公告)日：2003-07-15
申请号：US09893407
申请日：2001-06-29
申请人： Haruyuki Nakanishi , Shinichi Matsumoto
发明人： Haruyuki Nakanishi , Shinichi Matsumoto
IPC分类号： C25B102
CPC分类号： C01B3/065 , C01B3/04 , H01M8/04029 , H01M8/04156 , H01M8/065 , H01M8/0662 , H01M2250/20 , H01M2300/0082 , Y02E60/327 , Y02E60/362 , Y02E60/364 , Y02P20/129 , Y02T90/32
摘要： A metal hydride is supplied into a reactor while being converted into fine particles. By injecting water from an injector, the metal hydride is hydrolyzed to generate hydrogen. The water supplied to the reactor is water generated by a fuel cell. This allows omission or a size reduction of a water tank for the hydrolysis, and therefore allows a size reduction of the system as a whole. It is possible to adopt a construction in which waste heat from the fuel cell is supplied to pyrolyze the metal hydride, a construction in which heat generated by the hydrolysis is used to pyrolyze another metal hydride, etc.

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