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1. 发明授权

US4857171A Hydrocarbon conversion process and catalysts 失效
标题翻译：烃转化过程和催化剂
公开(公告)号：US4857171A
公开(公告)日：1989-08-15
申请号：US55672
申请日：1987-05-29
申请人： Arend Hoek , Tom Huizinga , Ian E. Maxwell
发明人： Arend Hoek , Tom Huizinga , Ian E. Maxwell
IPC分类号： B01J29/08 , B01J29/14 , B01J29/16 , C10G47/16 , C10G47/20
CPC分类号： B01J29/166 , C10G47/16
摘要： A process for converting hydrocarbon oils into products of low average molecular weight and lower average boiling point comprising contacting a hydrocarbon oil at elevated temperature and pressure in the presence of hydrogen with a catalyst comprising a modified Y zeolite having a unit cell size below 24.45 .ANG., a degree of crystallinity which is at least retained at increasing SiO.sub.2 /Al.sub.2 O.sub.3 molar ratios, a water adsorption capacity (at 25.degree. C. and p/p.sub.o value of 0.2) of at least 8% by weight of modified zeolite and a pore volume of at least 0.25 ml/g wherein between 10% and 60% of the total pore volume is made up of pores having a diameter of at least 8 nm, an amorphous cracking component, a binder and at least one hydrogenation component of a Group VI metal and/or at least one hydrogenation component of a Group VIII metal. The invention also relates to catalyst compositions suitable for use in said process.
摘要翻译：一种将烃油转化成低平均分子量和较低平均沸点的产物的方法，包括在氢气存在下在升高的温度和压力下将烃油与包含单元尺寸低于24.45的改性Y沸石的催化剂接触，至少在增加的SiO 2 / Al 2 O 3摩尔比下保持结晶度，水吸附容量（25℃，p / po值为0.2）为至少8重量％的改性沸石，并且孔容积至少0.25ml / g，其中总孔体积的10％至60％由直径至少为8nm的孔组成，无定形裂解组分，粘合剂和至少一种第VI族金属氢化组分和/或至少一种第VIII族金属的氢化组分。本发明还涉及适用于所述方法的催化剂组合物。

2. 发明授权

US4857170A Hydrocarbon conversion catalysts 失效
标题翻译：烃转化催化剂
公开(公告)号：US4857170A
公开(公告)日：1989-08-15
申请号：US55652
申请日：1987-05-29
申请人： Arend Hoek , Tom Huizinga , Ian E. Maxwell
发明人： Arend Hoek , Tom Huizinga , Ian E. Maxwell
IPC分类号： B01J29/08 , B01J29/14 , B01J29/16 , C10G47/02 , C10G47/16 , C10G47/20
CPC分类号： C10G47/16 , B01J29/166
摘要： Composition of matter suitable as a catalyst (base) in hydroprocessing comprising a crystalline aluminosilicate zeolite and a binder wherein the crystalline aluminosilicate comprises a modified Y zeolite having a unit cell size below 24.35 .ANG., a degree of crystallinity which is at least retained at increasing SiO.sub.2 /Al.sub.2 O.sub.3 molar ratios, a water adsorption capacity (at 25.degree. C. and a p/p.sub.o value of 0.2) of at least 8% by weight of modified zeolite and a pore volume of at least 0.25 ml/g wherein between 10% and 60% of the total pore volume is made up of pores having a diameter of at least 8 nm. The invention also relates to hydroconversion catalysts and processes based on said compositions of matter.
摘要翻译：在加氢处理中适合作为催化剂（碱）的物质的组成，其包含结晶硅铝酸盐沸石和粘合剂，其中结晶硅铝酸盐包含单元尺寸低于24.35的改性Y沸石，结晶度至少在增加SiO 2时保持 / Al 2 O 3摩尔比，至少为8重量％的改性沸石的水吸附能力（25℃，ap / po值为0.2），孔体积为至少0.25ml / g，其中10％至60％总孔体积的％由直径至少为8nm的孔组成。本发明还涉及基于所述物质组合物的加氢转化催化剂和方法。

3. 发明授权

US4925820A Hydrocarbon conversion process and catalysts 失效
标题翻译：烃转化过程和催化剂
公开(公告)号：US4925820A
公开(公告)日：1990-05-15
申请号：US344589
申请日：1989-04-28
申请人： Arend Hoek , Tom Huizinga , Ian E. Maxwell
发明人： Arend Hoek , Tom Huizinga , Ian E. Maxwell
IPC分类号： B01J29/08 , B01J29/14 , B01J29/16 , C10G47/16 , C10G47/20
CPC分类号： B01J29/166 , C10G47/16
摘要： A process for converting hydrocarbon oils into products of low average molecular weight and lower average boiling point comprising contacting a hydrocarbon oil at elevated temperature and pressure in the presence of hydrogen with a catalyst comprising a modified Y zeolite having a unit cell size below 24.45 .ANG., a degree of crystallinity which is at least retained at increasing SiO.sub.2 /Al.sub.2 O.sub.3 molar ratios, a water adsorption capacity (at 25.degree. C. and a p/p.sub.o value of 0.2) of at least 8% by weight of modified zeolite and a pore volume of at least 0.25 ml/g wherein between 10% and 60% of the total pore volume is made up of pores having a diameter of at least 8 nm, an amorphous cracking component, a binder and at least one hydrogenation component of a Group VI metal and/or at least one hydrogenation component of a Group VIII metal. The invention also relates to catalyst compositions suitable for use in said process.

4. 发明授权

US4916096A Hydrocarbon conversion catalysts 失效
标题翻译：烃转化催化剂
公开(公告)号：US4916096A
公开(公告)日：1990-04-10
申请号：US344588
申请日：1989-04-28
申请人： Arend Hoek , Tom Huizinga , Ian E. Maxwell
发明人： Arend Hoek , Tom Huizinga , Ian E. Maxwell
IPC分类号： B01J29/08 , B01J29/14 , B01J29/16 , C10G47/02 , C10G47/16 , C10G47/20
CPC分类号： C10G47/16 , B01J29/166
摘要： Composition of matter suitable as a catalyst (base) in hydroprocessing comprising a crystalline aluminosilicate zeolite and a binder wherein the crystalline aluminosilicate comprises a modified Y zeolite having a unit cell size below 24.35 .ANG., a degree of crystallinity which is at least retained at increasing SiO.sub.2 /Al.sub.2 O.sub.3 molar ratios, a water adsorption capacity (at 25.degree. C. and a p/p.sub.o value of 0.2) of at least 8% by weight of modified zeolite and a pore volume of at least 0.25 ml/g wherein between 10% and 60% of the total pore volume is made up of pores having a diameter of at least 8 nm. The invention also relates to hydroconversion catalysts and processes based on said compositions of matter.

5. 发明授权

US4836910A Catalytic dewaxing with zeolite theta-1 失效
标题翻译：用沸石θ-1催化脱蜡
公开(公告)号：US4836910A
公开(公告)日：1989-06-06
申请号：US62971
申请日：1987-06-18
申请人： Jacob A. van de Griend , Arend Hoek , Tom Huizinga
发明人： Jacob A. van de Griend , Arend Hoek , Tom Huizinga
IPC分类号： B01J29/40 , C10G45/64
CPC分类号： B01J29/40 , C10G45/64
摘要： A process is disclosed for the catalytic dewaxing of a hydrocarbon oil by contacting said oil at catalytic dewaxing conditions with a catalyst comprising a crystalline aluminum silicate which has the following composition in terms of the molar ratios of the oxides:(0.9+0.2)Z.sub.p O.sub.q :Al.sub.2 O.sub.3 :xSiO.sub.2 : yH.sub.2 Owherein Z is at least one cation, p and q are each at least one and satisfy the electroneutrality of Z.sub.p O.sub.q, x is at least 10 and y/x is 0-25, and which crystalline aluminum silicate has a defined characteristic X-ray diffraction pattern as set forth in Table A.
摘要翻译：公开了一种用于通过在催化脱蜡条件下使所述油与包含结晶硅酸铝的催化剂接触的方法，所述催化剂具有以下氧化物的摩尔比具有以下组成的结晶硅酸铝：（0.9 + 0.2）ZpOq： Al 2 O 3：xSiO 2：yH 2 O其中Z是至少一个阳离子，p和q各自为至少一个，并且满足ZpOq的电中性，x为至少10，y / x为0-25，并且结晶硅酸铝具有定义的特性X射线衍射图如表A所示。

6. 发明授权

US5006496A Process for the preparation of zeolitic catalysts 失效
标题翻译：沸石催化剂的制备方法
公开(公告)号：US5006496A
公开(公告)日：1991-04-09
申请号：US376277
申请日：1989-06-16
申请人： Tom Huizinga , Arend Hoek , Hennie Schaper , Aan H. Klazinga
发明人： Tom Huizinga , Arend Hoek , Hennie Schaper , Aan H. Klazinga
IPC分类号： B01J37/00 , B01J29/08 , B01J29/10 , B01J29/14 , B01J29/16 , C10G47/18 , C10G47/20
CPC分类号： B01J29/084 , C10G47/20
摘要： Process for the preparation of a zeolitic catalyst which comprises treating a zeolite of the Y-type having an alkali oxide/aluminum oxide molar ratio of at most 0.13 with a solution of a multi-valent metal salt having a cationic radius between 0.6 and 1.0 .ANG. and combining the ion-exchanged zeolite without a calcination step with a hydrogenation component of a Group VIII and/or Group VI(b) metal.

7. 发明授权

US09333492B2 Hydrogenation catalyst and use thereof for hydrogenating fischer-tropsch endproducts 有权
标题翻译：氢化催化剂及其用于氢化费 - 托最终产物的用途
公开(公告)号：US09333492B2
公开(公告)日：2016-05-10
申请号：US12161634
申请日：2006-01-23
申请人： Focco Cornelis Bijlsma , Jan Lodewijk Maria Dierickx , Arend Hoek , Frans Joris Antonius Kellendonk , Anna Elisabeth Maria Oud
发明人： Focco Cornelis Bijlsma , Jan Lodewijk Maria Dierickx , Arend Hoek , Frans Joris Antonius Kellendonk , Anna Elisabeth Maria Oud
IPC分类号： B01J21/00 , B01J23/00 , B01J25/00 , B01J29/00 , B01J23/755 , B01J21/04 , B01J35/10 , B01J37/02 , C10G45/00 , C10G3/00 , C10G45/06 , C10G45/12 , C10G2/00
CPC分类号： B01J23/755 , B01J21/04 , B01J35/10 , B01J35/1061 , B01J35/1085 , B01J37/0205 , C10G2/332 , C10G3/45 , C10G3/50 , C10G45/00 , C10G45/06 , C10G45/12 , C10G2300/1022 , C10G2300/4018 , Y02P30/20
摘要： A hydrogenation catalyst particularly suitable for hydrogenating oxygenates in a hydrogenation unit of a Fischer-Tropsch plant is disclosed. A preferred embodiment comprises more than 5% and less than 20% nickel based on a wide pore alumina support. The catalyst successfully hydrogenates oxygenates which otherwise tend to poison a catalyst in a hydroconversion unit downstream. Moreover, the temperature at which the unwanted hydrogenolysis of long chain paraffins to methane occurs is higher for one catalyst disclosed herein than a comparable known catalyst. This allows the hydrogenation plant to operate at a higher temperature.
摘要翻译：公开了一种特别适用于在费 - 托工厂的氢化单元中氢化含氧化合物的氢化催化剂。优选的实施方案包括基于宽孔氧化铝载体的超过5％且小于20％的镍。催化剂成功地氢化含氧化合物，否则其倾向于在下游的加氢转化单元中毒催化剂。此外，与可比较的已知催化剂相比，长链烷烃对甲烷的不期望的氢解发生的温度比本文公开的一种催化剂更高。这允许氢化装置在较高的温度下运行。

8. 发明授权

US08685231B2 Process for conversion of paraffinic feedstock 有权
标题翻译：石蜡原料转化工艺
公开(公告)号：US08685231B2
公开(公告)日：2014-04-01
申请号：US12952986
申请日：2010-11-23
申请人： Jolinde Machteld Van De Graaf , Arend Hoek , Johannes Petrus De Jonge , Wiebe Sjoerd Kijlstra , Antonius Adrianus Maria Roovers , Jelle Rudolf Anne Sietsma , Johannes Anthonius Robert Van Veen
发明人： Jolinde Machteld Van De Graaf , Arend Hoek , Johannes Petrus De Jonge , Wiebe Sjoerd Kijlstra , Antonius Adrianus Maria Roovers , Jelle Rudolf Anne Sietsma , Johannes Anthonius Robert Van Veen
IPC分类号： C10G47/14 , C07C4/06
CPC分类号： C10G47/16 , C10G47/14 , C10G65/12 , C10G67/04 , C10G2300/202 , C10G2300/301 , C10G2300/44
摘要： The invention provides a process for converting a paraffinic feedstock comprising at least 50 wt % of compounds boiling above 370° C., a paraffin content of at least 60 wt %, an aromatics content below 1 wt %, a naphthenic content below 2 wt %, a nitrogen content below 0.1 wt %, and a sulphur content below 0.1 wt %, comprising: (a) reacting the feedstock with hydrogen at a temperature between 175 and 400° C. and a pressure between 20 and 100 bar using a catalyst comprising 0.005 to 5.0 wt % of a Group VIII noble metal on a carrier comprising 0.1-15 wt % zeolite beta and at least 40 wt % amorphous silica-alumina (b) withdrawing the effluent (c) subjecting the effluent to a fractionation step to form a heavy fraction, an intermediate fraction, and a light fraction; and (d) providing at least part of the heavy fraction to the reaction zone.
摘要翻译：本发明提供了一种转化石蜡原料的方法，该方法包括至少50重量％的沸点高于370℃的化合物，至少60重量％的链烷烃含量，低于1重量％的芳烃含量，低于2重量％的环烷烃含量，，低于0.1重量％的氮含量和低于0.1重量％的硫含量，包括：（a）使原料与氢在175-400℃之间的温度下反应，压力在20-100巴之间，使用的催化剂包括 0.005至5.0重量％的载体上的第VIII族贵金属，其包含0.1-15重量％的沸石β和至少40重量％的无定形二氧化硅 - 氧化铝（b）回收流出物（c）使流出物进行分馏步骤以形成重馏分，中间馏分和轻馏分; 和（d）将至少部分重馏分提供到反应区。

9. 发明授权

US07855234B2 Fischer-tropsch process and reactor assembly 有权
标题翻译：费 - 托法和反应器组装
公开(公告)号：US07855234B2
公开(公告)日：2010-12-21
申请号：US11988970
申请日：2006-07-14
申请人： Arend Hoek , Hans Michiel Huisman
发明人： Arend Hoek , Hans Michiel Huisman
IPC分类号： C07C27/00
CPC分类号： C10G2/32 , B01J8/0278 , B01J8/065 , B01J8/067 , B01J8/22 , B01J2219/00038 , B01J2219/00202 , B01J2219/00211 , B01J2219/00231 , B01J2219/00238 , C10G2/34 , C10G2400/02 , C10G2400/06 , C10G2400/08 , C10G2400/10 , C10G2400/18
摘要： A method of accommodating a reduction in production capacity of one or more reactors in a multi-reactor assembly adapted for the production of hydrocarbon products from syngas, the syngas being provided by a syngas manufacturing facility and provided to an entry stream system providing syngas to each of the reactors, and having an exit stream system taking at least hydrocarbon products from the reactors, wherein the method comprises the steps of: redistributing the syngas from the one or more said reactors to one or more other reactors, and increasing the temperature in the said one or more other reactors to at least partially take over the reduction in production capacity of the one or more reactors.
摘要翻译：一种在适合从合成气生产碳氢化合物产品的多反应器组合中容纳一个或多个反应器的生产能力降低的方法，合成气由合成气制造设施提供并提供给进入流系统，其将合成气提供给每个的反应器，并且具有至少从反应器中取出烃产物的出口流系统，其中所述方法包括以下步骤：将来自所述一个或多个所述反应器的合成气重新分配到一个或多个其它反应器，并且增加所述反应器中的温度所述一个或多个其它反应器至少部分地承担一个或多个反应器的生产能力的降低。

10. 发明授权

US07642294B2 Process to prepare lower olefins from a carbon containing feedstock 有权
标题翻译：从含碳原料制备低级烯烃的方法
公开(公告)号：US07642294B2
公开(公告)日：2010-01-05
申请号：US11664657
申请日：2005-10-06
申请人： Emil Eduard Antonius Cruijsberg , Jan Lodewijk Maria Dierickx , Arend Hoek , Johannes Marie Gemma Van Schijndel , Jeroen Van Westrenen
发明人： Emil Eduard Antonius Cruijsberg , Jan Lodewijk Maria Dierickx , Arend Hoek , Johannes Marie Gemma Van Schijndel , Jeroen Van Westrenen
IPC分类号： C07C27/00 , C10G47/02 , C10G35/00
CPC分类号： C10G9/00 , C10G2/30
摘要： A process is provided to make ethylene and propylene from a carbonaceous feedstock. The process comprises preparing a gaseous mixture of carbon monoxide and hydrogen from a feedstock. A Fischer Tropsch synthesis is then performed on the gaseous mixture to obtain a Fischer Tropsch product along with unconverted carbon monoxide and hydrogen. The Fischer Tropsch product in admixture with the unconverted carbon monoxide and hydrogen from the previous step is then subjected to terminal cracking to form ethylene and propylene.
摘要翻译：提供了从碳质原料制备乙烯和丙烯的方法。该方法包括从原料制备一氧化碳和氢气的气体混合物。然后在气体混合物上进行费 - 托合成，以获得费 - 托产物以及未转化的一氧化碳和氢气。然后将与前一步骤中未转化的一氧化碳和氢气混合的费托产品进行末端裂化以形成乙烯和丙烯。

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