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1. 发明授权

US4613718A Hydroxylated magnesia support 失效
标题翻译：羟基氧化镁载体
公开(公告)号：US4613718A
公开(公告)日：1986-09-23
申请号：US600912
申请日：1984-04-16
申请人： John A. Jaecker , Marvin F. L. Johnson
发明人： John A. Jaecker , Marvin F. L. Johnson
IPC分类号： C07C2/84 , C07C2/00
CPC分类号： C07C2/84 , C07C2521/08 , C07C2521/10 , C07C2523/02 , C07C2523/04 , C07C2523/08 , C07C2523/14 , C07C2523/18 , C07C2523/34 , Y10S585/943
摘要： An improved method for converting methane to higher hydrocarbon products by contacting at a selected temperature at least one reducible oxide of at least one metal, associated with a hydroxylated magnesia support (that is, magnesia derived from magnesium hydroxide or a magnesium-containing component contacted with hydroxyl-containing material).
摘要翻译：一种用于将甲烷转化成较高级烃产物的改进方法，其通过使所选择的温度下接触至少一种与羟基化氧化镁载体相关的至少一种金属的还原氧化物（即来自氢氧化镁的氧化镁或与含羟基材料）。

2. 发明授权

US4464249A Plural stage reforming with catalysts having a skewed distribution of a platinum-group metal and rhenium 失效
标题翻译：用铂族金属和铼倾斜分布的催化剂进行多级重整
公开(公告)号：US4464249A
公开(公告)日：1984-08-07
申请号：US84948
申请日：1979-10-15
申请人： John Mooi , Marvin F. L. Johnson
发明人： John Mooi , Marvin F. L. Johnson
IPC分类号： C10G35/09 , B01J23/656 , C10G59/02 , C10G35/06
CPC分类号： C10G59/02 , B01J23/6567
摘要： A process for reforming naphthene and paraffin-containing hydrocarbon feeds to increase their aromatic content is disclosed which involves the use of a series of reaction zones containing a supported platinum-group metal catalyst and a supported rhenium catalyst, wherein the distribution of catalytically effective platinum-group metal and rhenium among the series of reaction zones is skewed. The ratio of the percent by weight of the supported platinum-group metal in the catalyst in at least one of the earlier reaction zones of the series of reaction zones to that in the catalyst in at least one of the later reaction zones is in the range of about 1.5 to 10, and preferably in the range of about 2 to about 6. The percent by weight of supported rhenium based on the catalyst in the first zone is preferably less than about 10 percent by weight. Broadly, in the skewed distribution of supported platinum-group metal and rhenium, the ratio of the platinum-group metal to rhenium in the earlier zones is greater than about 1.5, and the ratio of platinum-group metal to rhenium in the later zones is less than about 1.
摘要翻译：公开了一种用于重整环烷烃和含链烷烃的烃进料以增加其芳族含量的方法，其涉及使用一系列含有负载的铂族金属催化剂和负载的铼催化剂的反应区，其中催化有效的铂 - 一系列反应区中的金属和铼组合是偏斜的。反应区系列中的至少一个较早的反应区域与催化剂中的至少一个较晚的反应区域中的催化剂中负载的铂族金属的重量百分比的比例在该范围内为约1.5至10，优选在约2至约6的范围内。基于第一区中的催化剂的负载铼的重量百分比优选小于约10重量％。广泛地，在负载的铂族金属和铼的偏斜分布中，较早区域中铂族金属与铼的比例大于约1.5，后区的铂族金属与铼的比例为小于1。

3. 发明授权

US4251350A Hydrocarbon hydrotreating process 失效
标题翻译：烃加氢处理工艺
公开(公告)号：US4251350A
公开(公告)日：1981-02-17
申请号：US93705
申请日：1979-11-13
申请人： Marvin F. L. Johnson , Henry Erickson
发明人： Marvin F. L. Johnson , Henry Erickson
IPC分类号： B01J27/18 , C10G45/08
CPC分类号： C10G45/08 , B01J27/18
摘要： An improved method for preparing a hydrocarbon hydrotreating catalyst containing a major amount of alumina and a minor amount of at least one Group VIB or Group VIII metal comprising:(1) contacting an aqueous mixture of hydrous alumina with at least one phosphorus-containing compound in an amount sufficient to increase the hydrocarbon hydrotreating activity of the final catalyst and forming a phosphorus-containing hydrous alumina;(2) calcining the phosphorus-containing hydrous alumina and forming a calcined alumina;(3) contacting the calcined alumina with at least one metal-containing compound and forming a metal-containing material, the metal being selected from the group consisting of Group VIB metal, Group VIII metal and mixtures thereof; and(4) calcining the metal-containing material and forming a catalyst having increased hydrocarbon hydrotreating activity.Improved hydrocarbon hydrotreating processes and catalysts are also disclosed.
摘要翻译：一种用于制备含有主要量的氧化铝和少量至少一种VIB族或VIII族金属的烃加氢处理催化剂的改进方法，包括：（1）将含水氧化铝的含水混合物与至少一种含磷化合物接触足以提高最终催化剂的烃加氢处理活性并形成含磷水合氧化铝的量; （2）煅烧含磷水合氧化铝并形成煅烧氧化铝; （3）使煅烧的氧化铝与至少一种含金属的化合物接触并形成含金属的材料，该金属选自第VIB族金属，第Ⅷ族金属及其混合物; 和（4）煅烧含金属材料并形成具有提高的烃加氢精制活性的催化剂。还公开了改进的烃加氢处理方法和催化剂。

4. 发明授权

US4311582A Stabilized reforming catalyst 失效
标题翻译：稳定重整催化剂
公开(公告)号：US4311582A
公开(公告)日：1982-01-19
申请号：US193504
申请日：1980-10-02
申请人： Marvin F. L. Johnson , John A. Jaecker
发明人： Marvin F. L. Johnson , John A. Jaecker
IPC分类号： B01J27/10 , C10G35/09
CPC分类号： B01J27/10 , C10G35/09
摘要： Thermal stability of a halide-promoted, supported noble metal reforming catalyst is improved by employing a modified alumina support whose alumina precursor comprises at least about 75 weight percent boehmite, having an average crystallite diameter no greater than about 60 Angstroms. The thermal stability of the support is improved by the inclusion of a minor amount of silica, preferably added as an alkali-metal silicate to a mull of alumina prior to its extrusion and calcination with subsequent washing to remove the alkali metal.
摘要翻译：卤化物促进的负载型贵金属重整催化剂的热稳定性通过使用其氧化铝前体包含至少约75重量百分比的勃姆石，平均微晶直径不大于约60埃的改性氧化铝载体来改善。通过在其挤出和煅烧之前，将少量的二氧化硅作为碱金属硅酸盐添加到氧化铝的母体中，随后进行洗涤以除去碱金属，从而提高了载体的热稳定性。

5. 发明授权

US4305810A Stabilized reforming catalyst 失效
标题翻译：稳定重整催化剂
公开(公告)号：US4305810A
公开(公告)日：1981-12-15
申请号：US193502
申请日：1980-10-02
申请人： Marvin F. L. Johnson , Elmer W. Breder, Jr.
发明人： Marvin F. L. Johnson , Elmer W. Breder, Jr.
IPC分类号： B01J23/656 , C10G35/09
CPC分类号： C10G35/09 , B01J23/6567
摘要： Thermal stability of a halide-promoted, supported noble metal reforming catalyst is improved by employing a modified alumina support whose alumina precusor comprises at least about 75 weight percent boehmite, having an average crystallite diameter no greater than about 60 Angstroms. The thermal stability of the support is improved by the inclusion of a minor amount of silica, preferably added as a low-sodium colloidal silica dispersion to a mull of alumina prior to its extrusion and calcination.
摘要翻译：卤化物促进的负载型贵金属重整催化剂的热稳定性通过使用其氧化铝预处理剂包含至少约75重量百分比的勃姆石，平均微晶直径不大于约60埃的改性氧化铝载体来改进。通过在其挤出和煅烧之前，将少量的二氧化硅（优选作为低钠胶体二氧化硅分散体）加入到氧化铝的母体中来改善载体的热稳定性。

6. 发明授权

US3932270A Method for determining hydrocarbon hydrotreating activity of a catalyst prior to its use in a hydrotreating process 失效
标题翻译：确定催化剂在加氢处理过程中使用前的烃加氢处理活性的方法
公开(公告)号：US3932270A
公开(公告)日：1976-01-13
申请号：US551563
申请日：1975-02-20
申请人： Marvin F. L. Johnson
发明人： Marvin F. L. Johnson
IPC分类号： B01J23/85 , B01J27/188 , B01J35/00 , C10G45/04 , G01N15/08 , C10G23/02
CPC分类号： B01J35/00 , B01J23/85 , B01J27/188 , C10G45/04 , G01N15/088
摘要： An improved method of hydrocarbon hydrotreating is disclosed wherein the activity of a hydrotreating catalyst is determined prior to the catalyst being used to promote hydrocarbon hydrotreating. The catalytic activity of such a catalyst is determined by comparing a parameter involving the relative reflectance of the catalyst relative to the relative reflectance of a standard catalyst having acceptable activity. When it is determined that a given catalyst has catalytic activity at least essentially equal to that of the standard catalyst, the catalyst may be used to promote hydrocarbon hydrotreating thus providing an improved method of hydrocarbon hydrotreating.
摘要翻译：公开了改进的烃加氢处理方法，其中加氢处理催化剂的活性在用于促进烃加氢处理的催化剂之前测定。通过比较涉及催化剂的相对反射率的参数相对于具有可接受活性的标准催化剂的相对反射率来确定这种催化剂的催化活性。当确定给定催化剂具有至少基本上等于标准催化剂的催化活性时，催化剂可用于促进烃加氢处理，从而提供改进的烃加氢处理方法。

7. 发明授权

US4629718A Alkali promoted manganese oxide compositions containing silica and/or alkaline earth oxides 失效
标题翻译：碱促进含有二氧化硅和/或碱土氧化物的氧化锰组合物
公开(公告)号：US4629718A
公开(公告)日：1986-12-16
申请号：US683118
申请日：1984-12-18
申请人： C. Andrew Jones , John J. Leonard , John A. Sofranko , Howard P. Withers , E. William Breder, Jr. , Marvin F. L. Johnson , John A. Jaecker
发明人： C. Andrew Jones , John J. Leonard , John A. Sofranko , Howard P. Withers , E. William Breder, Jr. , Marvin F. L. Johnson , John A. Jaecker
IPC分类号： B01J23/08 , B01J23/14 , B01J23/18 , B01J23/34 , B01J27/18 , C07C2/84 , B01J21/08
CPC分类号： B01J23/14 , B01J23/08 , B01J23/18 , B01J23/34 , B01J27/18 , C07C2/84 , C07C2521/08 , C07C2521/10 , C07C2523/02 , C07C2523/04 , C07C2523/08 , C07C2523/10 , C07C2523/14 , C07C2523/18 , C07C2523/34 , C07C2527/18
摘要： A class of mixed oxide catalysts comprising Mn-containing oxides, alkali metals or compounds thereof, and at least one member of the group consisting of oxides of Si, oxides of alkaline earth metals, and mixed oxides of Si and at least one alkaline earth metal. In the more preferred embodiments, the third component serves as a carrier for the Mn and alkali metal components. The composition preferably comprises a major amount of the carrier material and minor amounts of the other components. The compositions are useful for hydrocarbon coversion, methane conversion, and oxidative dehydrogenation processes characterized by formation of coproduct water.
摘要翻译：一类含有Mn的氧化物，碱金属或其化合物的混合氧化物催化剂，以及由Si的氧化物，碱土金属的氧化物以及Si和至少一种碱土金属的混合氧化物组成的组中的至少一种。在更优选的实施方案中，第三组分用作Mn和碱金属组分的载体。组合物优选包含主要量的载体材料和少量的其它组分。该组合物可用于烃转化，甲烷转化和以特征为副产物水形成的氧化脱氢方法。

8. 发明授权

US4544786A Methane conversion using a magnesia/silica support 失效
标题翻译：使用氧化镁/二氧化硅载体的甲烷转化
公开(公告)号：US4544786A
公开(公告)日：1985-10-01
申请号：US600925
申请日：1984-04-16
申请人： E. William Breder, Jr. , John A. Jaecker , Marvin F. L. Johnson
发明人： E. William Breder, Jr. , John A. Jaecker , Marvin F. L. Johnson
IPC分类号： C07C2/84 , C07C2/00
CPC分类号： C07C2/84 , C07C2521/08 , C07C2521/10 , C07C2523/02 , C07C2523/04 , C07C2523/08 , C07C2523/14 , C07C2523/18 , C07C2523/34 , Y10S585/943
摘要： An improved method for converting methane to higher hydrocarbon products by contacting a gas comprising methane with a contact agent at a selected temperature, the agent comprising a reducibile metal oxide, a support of at least two oxides, and an alkali metal.
摘要翻译：一种通过使包含甲烷的气体与选定温度下的接触剂接触而将甲烷转化为较高级烃产物的改进方法，所述试剂包含还原性金属氧化物，至少两种氧化物的载体和碱金属。

9. 发明授权

US4305811A Stabilized reforming catalyst 失效
标题翻译：稳定重整催化剂
公开(公告)号：US4305811A
公开(公告)日：1981-12-15
申请号：US193503
申请日：1980-10-02
申请人： Marvin F. L. Johnson
发明人： Marvin F. L. Johnson
IPC分类号： B01J21/04 , B01J23/656 , C10G35/09
CPC分类号： B01J21/04 , B01J23/6567 , C10G35/09
摘要： Thermal stability of a halide-promoted, alumina-supported noble metal reforming catalyst is improved by employing an alumina support precursor which comprises at least about 75 weight percent boehmite, having an average crystallite diameter no greater than about 60 Angstroms.
摘要翻译：卤化物促进的氧化铝负载的贵金属重整催化剂的热稳定性通过使用包含至少约75重量％的勃姆石的平均微晶直径不大于约60埃的氧化铝载体前体来改善。

10. 发明授权

US4202798A Phosphorous-containing catalyst and method for preparing and using same 失效
标题翻译：含磷催化剂及其制备和使用方法
公开(公告)号：US4202798A
公开(公告)日：1980-05-13
申请号：US955661
申请日：1978-10-30
申请人： Marvin F. L. Johnson , Henry Erickson
发明人： Marvin F. L. Johnson , Henry Erickson
IPC分类号： B01J23/85 , B01J27/18 , C10G45/04 , C10G45/10
CPC分类号： B01J27/18 , B01J23/85 , C10G45/04 , C10G45/10
摘要： An improved method for preparing a hydrocarbon hydrotreating catalyst containing a major amount of alumina and a minor amount of at least one Group VIB or Group VIII metal comprising:(1) contacting an aqueous mixture of hydrous alumina with at least one phosphorus-containing compound in an amount sufficient to increase the hydrocarbon hydrotreating activity of the final catalyst and forming a phosphorus-containing hydrous alumina;(2) calcining the phosphorus-containing hydrous alumina and forming a calcined alumina;(3) contacting the calcined alumina with at least one metal-containing compound and forming a metal-containing material, the metal being selected from the group consisting of Group VIB metal, Group VIII metal and mixtures thereof; and(4) calcining the metal-containing material and forming a catalyst having increased hydrocarbon hydrotreating activity.Improved hydrocarbon hydrotreating processes and catalysts are also disclosed.
摘要翻译：一种用于制备含有主要量的氧化铝和少量至少一种VIB族或VIII族金属的烃加氢处理催化剂的改进方法，包括：（1）将含水氧化铝的含水混合物与至少一种含磷化合物接触足以提高最终催化剂的烃加氢处理活性并形成含磷水合氧化铝的量; （2）煅烧含磷水合氧化铝并形成煅烧氧化铝; （3）使煅烧的氧化铝与至少一种含金属的化合物接触并形成含金属的材料，所述金属选自第VIB族金属，第Ⅷ族金属及其混合物; 和（4）煅烧含金属材料并形成具有提高的烃加氢精制活性的催化剂。还公开了改进的烃加氢处理方法和催化剂。

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