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1. 发明授权

US4587008A Process comprising reforming, synthesis, and hydrocracking 失效
标题翻译：方法包括重整，合成和加氢裂化
公开(公告)号：US4587008A
公开(公告)日：1986-05-06
申请号：US666527
申请日：1984-10-30
申请人： Johannes K. Minderhoud , Martin F. M. Post , Swan T. Sie , Ernst J. R. Sudholter
发明人： Johannes K. Minderhoud , Martin F. M. Post , Swan T. Sie , Ernst J. R. Sudholter
IPC分类号： B01J23/00 , C07C1/04 , C10G2/00 , C07C27/06 , C10G47/04
CPC分类号： C10G2/332 , C07C1/0435 , C07C1/0485 , C10G2/333 , C07C2521/04 , C07C2521/06 , C07C2521/08 , C07C2521/12 , C07C2523/26 , C07C2523/46 , C07C2523/75 , Y10S208/95
摘要： A two-step process is disclosed wherein C.sub.9.sup.+ hydrocarbons are prepared from C.sub.4.sup.- hydrocarbons by steam reforming followed by Fischer-Tropsch synthesis over a special cobalt-containing catalyst. Yields of C.sub.9.sup.+ hydrocarbons are increased by recycling a gaseous fraction comprising unconverted H.sub.2 and CO as well as C.sub.8.sup.- hydrocarbon by-products and steam to the steam reformer.
摘要翻译：公开了两步法，其中C 9+烃通过蒸汽重整然后在特殊的含钴催化剂上进行费 - 托合成从C4-烃制备。通过将包含未转化的H 2和CO以及C 8 - 烃副产物和蒸汽的气体馏分循环到蒸汽重整器来增加C 9 +烃的产率。

2. 发明授权

US4522938A Process for preparing a catalyst 失效
标题翻译：催化剂的制备方法
公开(公告)号：US4522938A
公开(公告)日：1985-06-11
申请号：US554482
申请日：1983-11-22
申请人： Arend Hoek , Johannes K. Minderhoud , Martin F. M. Post
发明人： Arend Hoek , Johannes K. Minderhoud , Martin F. M. Post
IPC分类号： C07C1/20 , B01J23/80 , B01J23/86 , B01J23/89 , B01J37/00 , B01J37/03 , C07B61/00 , C07C1/00 , C07C27/00 , C07C27/06 , C07C29/15 , C07C29/153 , C07C29/154 , C07C31/04 , C07C67/00 , B01J21/04 , B01J23/06 , B01J23/26 , B01J23/72
CPC分类号： C07C29/153 , B01J23/80 , B01J23/868 , B01J37/0045 , B01J37/03 , Y02P20/52
摘要： Catalysts for the production of methanol from mixtures of carbon monoxide and hydrogen are prepared by dispersing in water a co-precipitate of zinc and at least one of chromium and aluminum together with a co-precipitate of copper, zinc and optionally at least one of chromium and aluminum, followed by spray drying of the dispersion, and calcining the spray dried material.
摘要翻译：用于从一氧化碳和氢气的混合物生产甲醇的催化剂通过在水中分散锌和铬和铝中的至少一种的共沉淀物以及铜，锌的共沉淀物和任选的至少一种铬来制备和铝，然后喷雾干燥分散体，并煅烧喷雾干燥的材料。

3. 发明授权

US4499209A Process for the preparation of a Fischer-Tropsch catalyst and preparation of hydrocarbons from syngas 失效
标题翻译：制备费 - 托催化剂和从合成气制备烃的方法
公开(公告)号：US4499209A
公开(公告)日：1985-02-12
申请号：US546670
申请日：1983-10-28
申请人： Arend Hoek , Martin F. M. Post , Johannes K. Minderhoud , Peter W. Lednor
发明人： Arend Hoek , Martin F. M. Post , Johannes K. Minderhoud , Peter W. Lednor
IPC分类号： B01J23/75 , C07B61/00 , C07C1/00 , C07C1/04 , C07C9/00 , C07C67/00
CPC分类号： B01J23/75 , C07C1/0445 , C07C2521/06 , C07C2521/08 , C07C2523/75
摘要： A Fischer-Tropsch catalyst is prepared by impregnating a silica carrier with a solution of a zirconium or titanium compound, calcining the composition thus obtained, thereafter impregnating the carrier with a cobalt compound-containing solution and calcining and reducing the composition thus obtained. Catalysts so prepared and containing 5-40 pbw of cobalt and 2-150 pbw of zirconium or titanium per 100 pbw of silica, are used in the preparation of hydrocarbons from a H.sub.2 /CO mixture.
摘要翻译：通过用锆或钛化合物的溶液浸渍二氧化硅载体，煅烧所得组合物，然后用含钴化合物的溶液浸渍载体并煅烧并还原由此获得的组合物来制备费 - 托催化剂。如此制备并含有5-40pbw的钴和每100pbw二氧化硅的含有2-150pbw的锆或钛的催化剂用于从H 2 / CO混合物制备烃。

4. 发明授权

US5008094A Crystalline (metallo)silicates and process for preparing such (metallo)silicates 失效
标题翻译：晶体（金属）硅酸盐和制备这种（金属）硅酸盐的方法
公开(公告)号：US5008094A
公开(公告)日：1991-04-16
申请号：US399189
申请日：1989-08-28
申请人： Johannes J. Keijsper , Munro Mackay , Martin F. M. Post
发明人： Johannes J. Keijsper , Munro Mackay , Martin F. M. Post
IPC分类号： C01B39/00 , B01D71/02 , B01J21/18 , B01J29/04 , B01J29/70 , B01J29/86 , B01J29/87 , B01J29/88 , B01J29/89 , B01J32/00 , C01B33/20 , C01B33/32 , C01B35/12 , C01B37/02 , C01B39/02 , C01B39/04 , C01B39/12 , C01B39/48
CPC分类号： C01B33/2892 , B01J29/04 , C01B33/185 , C01B39/48 , C01P2002/72 , C01P2006/80
摘要： Crystalline (metallo)silicates having in the as-synthesized, anhydrous form a molar composition expressed by the formula:(0-9)M.sub.2/n O.(4-9)R.sub.2 O.100SiO.sub.2. (0-2)X.sub.2 O.sub.3,wherein M is an alkali or alkaline earth metal ion having a valency n, R represents a tetramethylammonium cation or a precursor thereof, X represents at least one of Al, Fe, B or Ga, and having a specific X-ray diffraction pattern.The silicates can be prepared from an aqueous mixture comprising a source of silicon, optionally a source of at least one of aluminium, iron boron or gallium, and a source of tetramethylammonium cations or precursors thereof, which mixture is kept at a temperature of between 140.degree.-240.degree. C. whereby the following requirement is fulfilled: T.gtoreq.244.5-18.2 ln t, wherein T is the temperature (in .degree.C.) and t is the period of time (in hours) during which the mixture is kept at temperature T, until a crystalline silicate is formed which is subsequently separated from the mother liquor and dried, and which may subsequently be calcined.

5. 发明授权

US4443561A Process for the preparation of organic compounds 失效
标题翻译：制备有机化合物的方法
公开(公告)号：US4443561A
公开(公告)日：1984-04-17
申请号：US381619
申请日：1982-05-24
申请人： Sikko J. A. Boelema , Martin F. M. Post , Swan T. Sie
发明人： Sikko J. A. Boelema , Martin F. M. Post , Swan T. Sie
IPC分类号： B01J23/00 , B01J23/26 , B01J23/75 , B01J23/78 , B01J23/86 , B01J29/00 , B01J29/70 , B01J29/87 , B01J29/88 , B01J29/89 , C07B61/00 , C07C1/00 , C07C1/04 , C07C9/00 , C07C11/02 , C07C15/00 , C07C27/00 , C07C27/06 , C07C29/158 , C07C67/00 , C10G2/00
CPC分类号： C10G2/332 , C07C1/044 , C07C1/0445 , C07C1/0485 , C10G2/32 , C10G2/344 , C07C2521/04 , C07C2521/08 , C07C2521/10 , C07C2523/06 , C07C2523/26 , C07C2523/46 , C07C2523/745 , C07C2523/75 , C07C2523/755 , C07C2529/06
摘要： In a two-stage process for the conversion of H.sub.2 -poor syngas into hydrocarbons and oxygenates in which uncoverted syngas from the first stage product is converted in a second stage into paraffins over a Ni, Co or Ru catalyst, the H.sub.2 /CO molar ratio of the feed for the second stage is adjusted to the required value of 1.75-2.25 by blending this feed with an H.sub.2 -rich syngas with an H.sub.2 /CO molar ratio of at least above 1.75 which latter gas has been obtained by subjecting a small portion of the feed for the first stage to a high temperature (above 325.degree. C.) CO-shift.
摘要翻译：在将H2贫的合成气转化为烃和含氧化合物的两阶段方法中，其中来自第一阶段产物的未转化合成气在第二阶段中通过Ni，Co或Ru催化剂转化成链烷烃，H2 / CO摩尔比通过将该进料与H 2 / CO摩尔比至少为1.75以上的富H 2的合成气混合，将第二阶段的进料调节至所需值1.75-2.25，后者气体是通过将小部分的第一阶段的进料到高温（高于325℃）CO转移。

6. 发明授权

US4331774A Process for the preparation of hydrocarbons 失效
标题翻译：烃类制备方法
公开(公告)号：US4331774A
公开(公告)日：1982-05-25
申请号：US169550
申请日：1980-07-17
申请人： Michael A. M. Boersma , Martin F. M. Post , Lambert Schaper
发明人： Michael A. M. Boersma , Martin F. M. Post , Lambert Schaper
IPC分类号： B01J23/00 , B01J29/00 , B01J29/87 , C07B61/00 , C07C1/00 , C07C1/04 , C07C15/00 , C07C67/00 , C10G2/00
CPC分类号： B01J29/87 , C07C1/043 , C07C2523/06 , C07C2523/26 , C07C2529/87
摘要： A process is disclosed for the preparation of aromatic hydrocarbon mixtures from a feed mixture of carbon monoxide and hydrogen by contacting said feed at elevated temperature and pressure with a mixture of two catalysts; one capable of converting said feed into acyclic oxygen containing hydrocarbons and the other certain crystalline gallium silicates.
摘要翻译：公开了一种从一氧化碳和氢气的进料混合物制备芳族烃混合物的方法，该方法是将升温和高压的所述进料与两种催化剂的混合物接触; 能够将所述进料转化为无环氧的烃和其它某些晶体硅酸镓的一种。

7. 发明授权

US4318802A Process for the purification of hydrocarbons 失效
标题翻译：烃类净化方法
公开(公告)号：US4318802A
公开(公告)日：1982-03-09
申请号：US200175
申请日：1980-10-24
申请人： Petrus F. A. Van Grinsven , Martin F. M. Post
发明人： Petrus F. A. Van Grinsven , Martin F. M. Post
IPC分类号： C10G25/05
CPC分类号： C10G25/05
摘要： A process is disclosed for removal of mercaptans from mercaptan-containing low boiling hydrocarbon mixture wherein said mixtures are fed to a contact zone containing a crystalline metal silicate which in dehydrated form has a composition in terms of moles of the oxides:(1.0.+-.0.3)(R).sub.2/n 0.[aFe.sub.2 O.sub.3.bAl.sub.2 O.sub.3.cGa.sub.2 O.sub.3. y(dSiO.sub.2.eGeO.sub.2)],where R is one or more mono- or bivalent cations and a, b, c, d, e, y and n are defined as hereinafter disclosed. The disclosed silicate crystalline metal silicate is (a) thermally stable up to a temperature above 600.degree. C.; (b) exhibits a specified X-ray powder diffraction pattern showing the reflections set out in Table A of the specification; (c) in the formula which represents the composition of the silicate expressed in terms of moles of the oxides, the (Al.sub.2 O.sub.3 +Fe.sub.2 O.sub.3)/SiO.sub.2 molar ratio is lower than 0.1; and separating from said crystalline silicate a hydrocarbon mixture product having a lower mercaptan content than the feed.
摘要翻译：公开了一种从含硫醇的低沸点烃混合物中除去硫醇的方法，其中将所述混合物进料到含有结晶金属硅酸盐的接触区，其中脱水形式具有以氧化物摩尔数计的组成：（1.0 +/- 0.3）（R）2 / n0。[aFe2O3.bAl2O3.cGa2O3。 y（dSiO2.eGeO2）]，其中R是一个或多个一价或二价阳离子，a，b，c，d，e，y和n如下文所述。公开的硅酸盐结晶金属硅酸盐是（a）在高于600℃的温度下热稳定; （b）表示说明书的表A所示的反射的规定的X射线粉末衍射图。（c）在表示以氧化物的摩尔数表示的硅酸盐的组成的式中，（Al 2 O 3 + Fe 2 O 3）/ SiO 2摩尔比低于0.1; 并且与所述结晶硅酸盐分离出具有比所述进料低的硫醇含量的烃混合物产物。

8. 发明授权

US4857497A Supported metal catalysts and use thereof 失效
标题翻译：负载金属催化剂及其用途
公开(公告)号：US4857497A
公开(公告)日：1989-08-15
申请号：US186782
申请日：1988-04-25
申请人： Krijn P. De Jong , Johannes H. E. Glezer , Martin F. M. Post
发明人： Krijn P. De Jong , Johannes H. E. Glezer , Martin F. M. Post
IPC分类号： B01J23/89 , C07B61/00 , C07C1/00 , C07C1/04 , C07C67/00
CPC分类号： C07C1/0435 , B01J23/89 , C07C1/0485 , C07C2521/04 , C07C2521/06 , C07C2521/08 , C07C2521/12 , C07C2523/42 , C07C2523/745 , C07C2523/75 , C07C2523/755 , C07C2523/89
摘要： A catalyst comprising a silica-containing carrier on which a metal component iron, nickel, or cobalt promoted by zirconium is supported snd, in addition, as promoter a noble metal from Group VIII of the Periodic Table; the promoter cobalt/zirconium catalyst is suitable for the preparation of hydrocarbons from carbon monoxide and hydrogen.
摘要翻译：包含含有二氧化硅的载体的催化剂，其上由锆负载的金属组分铁，镍或钴还原起来，另外作为助催化剂作为元素周期表第VIII族的贵金属; 助催化剂钴/锆催化剂适用于从一氧化碳和氢气制备烃。

9. 发明授权

US4637993A Process for preparation of catalyst 失效
标题翻译：催化剂的制备方法
公开(公告)号：US4637993A
公开(公告)日：1987-01-20
申请号：US780066
申请日：1985-09-25
申请人： Willibrord A. van Erp , Johannes M. Nanne , Martin F. M. Post
发明人： Willibrord A. van Erp , Johannes M. Nanne , Martin F. M. Post
IPC分类号： B01J23/74 , B01J23/75 , B01J23/86 , B01J23/89 , B01J37/02 , C07B61/00 , C07C1/00 , C07C1/04 , C07C67/00 , B01J21/06 , B01J21/08
CPC分类号： B01J23/75 , B01J23/864 , B01J23/8913 , C07C1/0435 , C07C2521/04 , C07C2521/06 , C07C2521/08 , C07C2521/12 , C07C2523/26 , C07C2523/46 , C07C2523/75 , C07C2523/86 , C07C2523/89
摘要： Supported cobalt catalysts with specified inhomogeneous cobalt distribution over the catalyst particles (expressed as a ratio (.SIGMA.V.sub.p /.SIGMA.V.sub.c).ltoreq.0.55 are prepared by immersion of a porous carrier into a solution of a cobalt compound in such a way that a given relation between the viscosity (in cS) and Temperature (degrees K.) of the solution and the immersion time (in sec) is met. For each immersion, this relation is (log v/t.times.T).times.10.sup.4 .gtoreq.1.
摘要翻译：通过将多孔载体浸入钴化合物的溶液中，以使得给定的钴化合物的溶液浸渍在催化剂颗粒上（具有比率（SIGMA Vp / SIGMA Vc））表示的具有规定的不均匀钴分布的负载型钴催化剂满足溶液的粘度（cS）和温度（度K）与浸渍时间（秒）之间的关系，对于每次浸渍，该关系为（log v / txT）×104> / = 1。

10. 发明授权

US4628133A Process for the preparation of hydrocarbons from a mixture of CO and H.sub. 2 失效
标题翻译：从CO和H2的混合物制备烃的方法
公开(公告)号：US4628133A
公开(公告)日：1986-12-09
申请号：US779328
申请日：1985-09-23
申请人： Johannes K. Minderhoud , Martin F. M. Post , Swan T. Sie , Ernst J. R. Sudholter
发明人： Johannes K. Minderhoud , Martin F. M. Post , Swan T. Sie , Ernst J. R. Sudholter
IPC分类号： B01J23/00 , C07C1/04 , C10G2/00 , C07C27/08
CPC分类号： C10G2/332 , C07C1/0435 , C07C1/0485 , C10G2/333 , C07C2521/04 , C07C2521/06 , C07C2521/08 , C07C2521/12 , C07C2523/26 , C07C2523/46 , C07C2523/75 , Y10S208/95
摘要： A two-step process is disclosed wherein C.sub.9.sup.+ hydrocarbons are prepared from C.sub.4.sup.- hydrocarbons by steam reforming followed by Fischer-Tropsch synthesis over a special cobalt-containing catalyst. Yields of C.sub.9.sup.+ hydrocarbons are increased by recycling a gaseous fraction comprising unconverted H.sub.2 and CO as well as C.sub.8.sup.- hydrocarbon by-products and steam to the steam reformer.

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