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31. 发明授权

US06316679B1 Treatment of a composition comprising a trimethylolalkane bis-monolinear formal 有权
标题翻译：包含三羟甲基烷烃双 - 单变体形式的组合物的处理
公开(公告)号：US06316679B1
公开(公告)日：2001-11-13
申请号：US09579743
申请日：2000-05-26
申请人： Carolyn Supplee , Jerry A. Broussard , Tobin J. Marks , William E. Slinkard , Edwards G. Zey
发明人： Carolyn Supplee , Jerry A. Broussard , Tobin J. Marks , William E. Slinkard , Edwards G. Zey
IPC分类号： C07C2726
CPC分类号： C07D319/06
摘要： A process for treating a composition containing a substantial proportion of trimethyflolpropane bis-monolinear formal (TMP-BMLF) or trimethylolethane bis-monolinear formal (TME-BMLF), e.g., a heavy ends residue obtained from the purification of a crude trimethylolpropane (TMP) or trimethylolethane (TME) product, wherein the composition is contacted at an elevated temperature with a strong acid catalyst, e.g., methanesulfonic acid, to produce a composition containing significantly increased amounts of TMP and trimethylolpropane monocyclic formal (TMP-MCF) or TME and trimethylolethane monocyclic formal (TME-MCF) respectively. Also disclosed is a process for reacting TMP-MCF or TME-MCF, either in substantially pure form or as present in the light ends overhead stream obtained in a finishing treatment of crude TMP or TME, with a monohydric or dihydric alcohol, e.g., ethylene glycol, in the presence of a strong acid catalyst to obtain additional TMP or TME and an acetal by-product, e.g., 1,3-dioxolane; and a process for directly reacting the TMP-BMLF or TME-BMLF present in a composition, e.g., the heavy ends residue obtained in the purification of TMP or TME, with a monohydric or dihydric alcohol, e.g., ethylene glycol, in the presence of a strong acid to obtain additional TMP or TME and an acetal by-product, e.g., 1,3-dioxolane.
摘要翻译：一种用于处理含有大量比例的三甲基十四烷丙基双 - 单体形式（TMP-BMLF）或三羟甲基乙烷双 - 单体形式（TME-BMLF）的组合物的方法，例如从纯化三羟甲基丙烷（TMP）得到的重馏分残余物，或三羟甲基乙烷（TME）产物，其中组合物在高温下与强酸催化剂（例如甲磺酸）接触以产生含有显着增加量的TMP和三羟甲基丙烷单环形式（TMP-MCF）或TME和三羟甲基乙烷的组合物单体形式（TME-MCF）。还公开了一种使TMP-MCF或TME-MCF以基本纯的形式或存在于在粗TMP或TME的整理处理中获得的轻馏分塔顶馏出物与一元或二元醇（例如乙烯乙二醇，在强酸催化剂存在下，得到另外的TMP或TME和缩醛副产物，例如1,3-二氧戊环; 以及将组合物中存在的TMP-BMLF或TME-BMLF直接反应的方法，例如在TMP或TME纯化中获得的重馏分残基与一元或二元醇（例如乙二醇）在存在下强酸以获得额外的TMP或TME和缩醛副产物，例如1,3-二氧戊环。

32. 发明授权

US6156692A Ruthenium-containing catalyst composition for olefin metathesis 失效
标题翻译：用于烯烃复分解的含钌催化剂组合物
公开(公告)号：US6156692A
公开(公告)日：2000-12-05
申请号：US842251
申请日：1997-04-24
申请人： Philip O. Nubel , Craig Lane Hunt , David S. Choi , Tobin J. Marks
发明人： Philip O. Nubel , Craig Lane Hunt , David S. Choi , Tobin J. Marks
IPC分类号： B01J31/18 , B01J31/22 , B01J31/24 , C07C6/04 , C07C6/06 , C07F15/00 , C08G61/08 , B01J31/00
CPC分类号： C08G61/08 , B01J31/185 , B01J31/2286 , B01J31/2295 , B01J31/24 , C07C6/04 , C07C6/06 , B01J2231/14 , B01J2231/543 , B01J2531/821 , C07C2531/02 , C07C2531/24
摘要： A ruthenium-containing metathesis catalyst system which contains a ruthenium compound (A), a phosphorus compound (B), and a compound (C) containing a carbon-to-carbon triple bond. The mole ratio of compounds A:B:C is typically in the range of about 1.0:0.01-100:0.01-100. The ruthenium compound (A) is a Ru(II), Ru(III), or Ru(IV) compound containing an anionic ligand (X) and optionally an arene ligand and optionally a phosphorus compound ligand. The phosphorus compound (B) is optional if the ruthenium compound (A) contains a phosphorus-containing ligand. The catalyst system is employed in processes to metathesize olefins, including ring-opening metathesis polymerization of cyclic olefins, metathesis of acyclic olefins, acyclic diene metathesis oligomerization or polymerization, cross-metathesis of cyclic and acyclic olefins, ring-closing metathesis, metathesis depolymerization of unsaturated polymers, and metathesis of functionalized olefins.
摘要翻译：含有钌化合物（A），磷化合物（B）和含有碳 - 碳三键的化合物（C）的含钌复分解催化剂体系。化合物A：B：C的摩尔比通常在约1.0：0.01-100：0.01-100的范围内。钌化合物（A）是含有阴离子配体（X）的Ru（II），Ru（III）或Ru（IV）化合物以及任选的芳族配体和任选的磷化合物配体。如果钌化合物（A）含有含磷配体，磷化合物（B）是任选的。催化剂体系用于将烯烃分离的方法，包括环烯烃的开环易位聚合，无环烯烃的复分解，无环二烯复分解低聚或聚合，环状和非环烯烃的交叉复分解，闭环复分解，复分解解聚不饱和聚合物和官能化烯烃的复分解。

33. 发明授权

US6153776A Bimetallic complexes and polymerization catalysts therefrom 有权
标题翻译：双金属络合物和聚合催化剂
公开(公告)号：US6153776A
公开(公告)日：2000-11-28
申请号：US141659
申请日：1998-08-28
申请人： Jasson T. Patton , Tobin J. Marks , Liting Li
发明人： Jasson T. Patton , Tobin J. Marks , Liting Li
IPC分类号： C07F17/00 , C08F4/64 , C08F4/659 , C08F4/6592 , C08F10/00 , C07F7/00 , C08F4/44
CPC分类号： C07F17/00 , C08F10/00 , C08F210/16 , C08F2410/03 , C08F4/65908 , C08F4/65912 , Y10S526/943
摘要： Group 3-6 or Lanthanide metal complexes possessing two metal centers, catalysts derived therefrom by combining the same with strong Lewis acids, Bronsted acid salts, salts containing a cationic oxidizing agent or subjected to bulk electrolysis in the presence of compatible, inert non-coordinating anions and the use of such catalysts for polymerizing olefins, diolefins and/or acetylenically unsaturated monomers are disclosed.
摘要翻译：具有两个金属中心的第3-6族或镧系元素金属络合物，由其衍生的催化剂通过与强路易斯酸，布朗斯台德酸盐，含有阳离子氧化剂的盐或在相容惰性非配位的存在下进行大量电解公开了阴离子和使用这种用于聚合烯烃，二烯烃和/或炔属不饱和单体的催化剂。

34. 发明授权

US6077919A Silyl-terminated polymer and method for preparing silyl-terminated polyolefins 失效
标题翻译：甲硅烷基封端的聚合物和制备甲硅烷基封端的聚烯烃的方法
公开(公告)号：US6077919A
公开(公告)日：2000-06-20
申请号：US96918
申请日：1998-06-12
申请人： Tobin J. Marks , Kwangmo Koo
发明人： Tobin J. Marks , Kwangmo Koo
IPC分类号： C08F2/38 , C08F4/606 , C08F4/646 , C08F4/659 , C08F10/00 , C08F110/06 , C08F110/14 , C08F210/16
CPC分类号： C08F10/00 , C08F110/06 , C08F110/14 , C08F210/16 , C08F4/65908
摘要： There is disclosed a method for synthesizing polyolefins having a silyl group at one terminus, the method comprising reacting a monomer of an a-olefin (C.ltoreq.3.ltoreq.10) and a tetrasubstituted silyl radical in the presence of a metallocene catalyst.
摘要翻译：公开了一种在一个末端具有甲硅烷基的聚烯烃的合成方法，该方法包括在茂金属催化剂存在下使α-烯烃（C 3 = 10）和四取代甲硅烷基的单体反应。

35. 发明授权

US5834100A Organic light-emitting dioddes and methods for assembly and emission control 失效
标题翻译：有机发光二极管及组装和排放控制方法
公开(公告)号：US5834100A
公开(公告)日：1998-11-10
申请号：US673600
申请日：1996-06-25
申请人： Tobin J. Marks , Wuping Ma , Homer Chou
发明人： Tobin J. Marks , Wuping Ma , Homer Chou
IPC分类号： C08G77/04 , C08G77/26 , H01L51/00 , H01L51/30 , H01L51/40 , H01L51/50 , H05B33/12 , B32B9/00 , H01J63/04
CPC分类号： H01L51/5012 , B82Y10/00 , B82Y30/00 , H01L51/0012 , H01L51/0059 , H01L51/0069 , H01L51/007 , H01L51/0094 , H01L51/0595 , H01L51/0034 , H01L51/0035 , H01L51/0036 , H01L51/0078 , H01L51/0081 , Y10S428/917 , Y10T428/24917 , Y10T428/31612 , Y10T428/31663
摘要： New organic light-emitting diodes and related electroluminescent devices and methods for fabrication, using siloxane self-assembly techniques.
摘要翻译：新的有机发光二极管和相关的电致发光器件及其制造方法，使用硅氧烷自组装技术。

36. 发明授权

US5371173A Poled polymeric nonlinear optical materials 失效
标题翻译：极化聚合物非线性光学材料
公开(公告)号：US5371173A
公开(公告)日：1994-12-06
申请号：US981342
申请日：1992-11-25
申请人： Tobin J. Marks , Michael A. Hubbard , Jiann T. Lin
发明人： Tobin J. Marks , Michael A. Hubbard , Jiann T. Lin
IPC分类号： C08G73/12 , G02F1/361 , C08G73/10
CPC分类号： G02F1/3617 , C08G73/124
摘要： The synthesis of a nonlinear chromophoric co-monomer 3,5-diamino-4'-nitrodiphenylamine and use as a reactive component in combination with a bismaleimide monomer in a NLO-active polyimide matrix is disclosed. After concurrent corona or contact poling and thermal polymerization, thin films of these chromophoric polyimides exhibit high second harmonic generation efficiencies and high DSC-determined glass transition temperatures. These poled polyimides also exhibit excellent SHG temporal stability, retaining 85-90% of the initial second harmonic efficiency after more than one month in air at 85.degree. C.
摘要翻译：公开了非线性发色共聚单体3,5-二氨基-4'-硝基二苯胺的合成，并将其用作与Nlo-活性聚酰亚胺基体中的双马来酰亚胺单体组合的反应性组分。在共同电晕或接触极化和热聚合之后，这些发色聚酰亚胺的薄膜表现出高的二次谐波产生效率和高DSC测定的玻璃化转变温度。这些极化的聚酰亚胺也具有优异的SHG时效性，在85℃的空气中保持一个月以上的初始二次谐波效率的85-90％。

37. 发明授权

US5330948A Homogeneous catalysts for stereoregular olefin polymerization 失效
标题翻译：用于立体规则烯烃聚合的均相催化剂
公开(公告)号：US5330948A
公开(公告)日：1994-07-19
申请号：US860784
申请日：1992-03-31
申请人： Tobin J. Marks , Moris S. Eisen , Michael A. Giardello
发明人： Tobin J. Marks , Moris S. Eisen , Michael A. Giardello
IPC分类号： C08F4/16 , C08F4/52 , C08F4/64 , C08F4/76 , C08F20/12 , C08F4/62 , C08F4/622 , C08F4/642 , C08F4/68
CPC分类号： C08F20/12 , C08F4/52 , C08F4/76 , Y10S526/943
摘要： The synthesis, and use as precatalysts of chiral organozirconium complexes for olefin polymerization are disclosed, having the structure (C.sub.5 R'.sub.4-x R*.sub.x) A (C.sub.5 R".sub.4-y R'".sub.y) M Q.sub.p, where x and y represent the number of unsubstituted locations on the cyclopentadienyl ring; R', R", R'", and R* represent substituted and unsubstituted alkyl groups having 1-30 carbon atoms and R* is a chiral ligand; A is a fragment containing a Group 13, 14, 15, or 16 element of the Periodic Table; M is a Group 3, 4, or 5 metal of the Periodic Table; and Q is a hydrocarbyl radical, or halogen radical, with 3.ltoreq.p.ltoreq.o. Related complexes may be prepared by alkylation of the corresponding dichorides. In the presence of methylalumoxane or triarylborane cocatalysts, these complexes form "cation-like" species which are highly active for olefin polymerization. In combination with a Lewis acid cocatalyst, propylene or other .alpha.-olefin polymerization can be effected with very high efficiency and isospecificity.
摘要翻译：公开了具有结构（C5R'4-xR * x）A（C5R''4-yR“'y）M Qp的合成和用作烯烃聚合的手性有机锆络合物的预催化剂，其中x和y表示环戊二烯基环上未取代位置的数目; R'，R“，R”'和R *表示取代和未取代的具有1-30个碳原子的烷基，R *是手性配体; A是含有元素周期表第13,14,15或16族元素的片段; M是元素周期表的第3,4或5族金属; 且Q为烃基或卤素基团，其中3≤n≤0。相关络合物可以通过相应的二氯化碳的烷基化来制备。在甲基铝氧烷或三芳基硼烷助催化剂存在下，这些络合物形成对于烯烃聚合具有高活性的“阳离子”物质。与路易斯酸助催化剂组合，丙烯或其它α-烯烃聚合可以以非常高的效率和特异性实现。

38. 发明授权

US4097384A Process for uranium isotope separation 失效
标题翻译：铀同位素分离方法
公开(公告)号：US4097384A
公开(公告)日：1978-06-27
申请号：US668829
申请日：1976-03-22
申请人： John H. Coleman , Tobin J. Marks
发明人： John H. Coleman , Tobin J. Marks
IPC分类号： B01D59/34 , B01J19/12 , C07F5/00 , B01J1/10 , B01K1/00
CPC分类号： B01D59/34 , B01J19/121 , C07F5/003
摘要： Separation of U.sup.235 and U.sup.238 isotopes by converting a mixture of these isotopes to organic compounds or to silicon compounds and then irradiating the isotope compounds selectively to change their chemical (and/or physical) properties, thereby to facilitate separation. In a preferred embodiment of the invention the uranium compounds are selected from the group having a chemical moiety R bonded directly to the U atom, the U-R bond having a fundamental, overtone, or combination virbational absorption frequency between 900 and 1100 cm.sup.-1. The selected U mixture is then irradiated with a frequency-selective CO.sub.2 laser.
摘要翻译：通过将这些同位素的混合物转化为有机化合物或硅化合物，然后选择性地照射同位素化合物来改变其化学（和/或物理）性质，从而便于分离，从而分离U235和U238同位素。在本发明的一个优选实施方案中，铀化合物选自具有与U原子直接键合的化学部分R的基团，U-R键具有基本的，泛音，或者在900和1100cm -1之间的组合防晒吸收频率。然后将所选的U混合物用频率选择性CO 2激光器照射。

39. 发明申请

US20160035855A1 Organic-Inorganic Hybrid Multilayer Gate Dielectrics for Thin-Film Transistors 有权
标题翻译：用于薄膜晶体管的有机 - 无机混合多层栅极电介质
公开(公告)号：US20160035855A1
公开(公告)日：2016-02-04
申请号：US13111699
申请日：2011-05-19
申请人： Tobin J. Marks , Young-geun Ha , Antonio Facchetti
发明人： Tobin J. Marks , Young-geun Ha , Antonio Facchetti
IPC分类号： H01L29/51 , H01L51/05 , H01L29/786
CPC分类号： H01L51/0533 , H01L21/441 , H01L29/24 , H01L29/4908 , H01L29/513 , H01L29/517 , H01L29/66969 , H01L51/0053 , H01L51/0055 , H01L51/0529 , H01L51/0537 , H01L51/0545 , H01L2251/301
摘要： Disclosed are organic-inorganic hybrid self-assembled multilayers that can be used as electrically insulating (or dielectric) materials. These multilayers generally include an inorganic primer layer and one or more bilayers deposited thereon. Each bilayer includes a chromophore or “π-polarizable” layer and an inorganic capping layer composed of zirconia. Because of the regularity of the bilayer structure and the aligned orientation of the chromophore resulting from the self-assembly process, the present multilayers have applications in electronic devices such as thin film transistors, as well as in nonlinear optics and nonvolatile memories.
摘要翻译：公开了可用作电绝缘（或电介质）材料的有机 - 无机混合自组装多层膜。这些多层通常包括无机底漆层和沉积在其上的一个或多个双层。每个双层包括发色团或“＆pgr可极化”层和由氧化锆组成的无机覆盖层。由于双层结构的规则性和由自组装过程产生的发色团的排列取向，所以本发明的多层膜可用于诸如薄膜晶体管的电子器件，以及非线性光学和非易失性存储器中。

40. 发明授权

US08859714B1 Polymeric semiconductors and related devices 有权
标题翻译：聚合物半导体及相关器件
公开(公告)号：US08859714B1
公开(公告)日：2014-10-14
申请号：US12827146
申请日：2010-06-30
申请人： Tobin J. Marks , Antonio Facchetti
发明人： Tobin J. Marks , Antonio Facchetti
IPC分类号： C08G69/08
CPC分类号： C08G61/126 , C08G73/06 , C08G2261/3223 , C08G2261/3229 , C08G2261/3246 , C08G2261/3327 , C08G2261/344 , C08G2261/51 , C08G2261/91 , C08G2261/92 , C08G2261/95
摘要： Disclosed are new organic semiconductor materials prepared from polymers based on N-alkyl-2,2′-bithiophene-3,3′-dicarboximide (BTI) repeating units. Such polymers can exhibit desirable electronic properties and can possess processing advantages including solution-processability and/or good stability at ambient conditions.
摘要翻译：公开了由基于N-烷基-2,2'-二噻吩-3,3'-二甲酰亚胺（BTI）重复单元的聚合物制备的新的有机半导体材料。这样的聚合物可以表现出所需的电子性质，并且可以具有包括溶液加工性和/或在环境条件下的良好稳定性的加工优点。

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