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1. 发明专利

JP2015016420A 水素分離体及び水素分離体を用いた水素製造装置审中-公开
标题翻译：氢分离体和氢生产装置使用氢分离体
公开(公告)号：JP2015016420A
公开(公告)日：2015-01-29
申请号：JP2013144694
申请日：2013-07-10
申请人：日本特殊陶業株式会社 , Ngk Spark Plug Co Ltd , 東京瓦斯株式会社 , Tokyo Gas Co Ltd
发明人： HIKOSAKA HIDEAKI , YOKOYAMA TAKAHIRO , KAWASE HIROKI , KAJITANI MASAHIRO , TANAKA HIROYUKI , TAKAGI YASUHIRO , KUME TAKAO , IKEDA YOICHI
IPC分类号： B01D71/02 , B01D53/22 , C01B3/56
摘要：【課題】高い水素透過性能と耐剥離性とを両立できる水素分離体及び水素分離体を用いた水素製造装置を提供すること。【解決手段】多孔質体(20)と、多孔質体(20)の細孔内に水素を含む気体のうち水素のみを選択して透過させる水素分離金属が充填された水素分離層(17)と、を有する水素分離体(1)に関するものである。この水素分離体(1)は、水素分離層(17)における水素分離金属の充填の割合を示す指標である充填率&egr;と、水素分離層(17)の厚み方向における水素の透過経路の長さの程度を示す指標である屈曲度τとの比(&egr;/τ)が、0.2〜0.6の範囲である。【選択図】図2
摘要翻译：要解决的问题：提供能够建立高透氢性和耐剥离性之间的相容性的氢分离体和使用氢分离体的氢制造装置。解决方案：在具有多孔体（20）的氢分离体（1）和填充有多孔体（20）的孔中的含氢气体中仅选择性渗透氢的氢分离金属的氢分离层（17），填充率（egr /τ）的比率作为表示氢分离层（17）中的氢分离金属的填充率的指标，作为表示氢在氢分离层（17）的厚度方向上的渗透路径长度的程度的折射率τ的折射率，在0.2-0.6的范围内。

2. 发明专利

JP2014156362A Hydrogen production apparatus 有权
标题翻译：氢生产设备
公开(公告)号：JP2014156362A
公开(公告)日：2014-08-28
申请号：JP2013026894
申请日：2013-02-14
申请人： Tokyo Gas Co Ltd , 東京瓦斯株式会社 , Ngk Spark Plug Co Ltd , 日本特殊陶業株式会社
发明人： IZEKI KOYA , KUME TAKAO , IKEDA YOICHI , ITO MASAYA , TAKAGI YASUHIRO , HIKOSAKA HIDEAKI , TANAKA HIROYUKI
IPC分类号： C01B3/38 , B01D53/22 , B01D63/06 , B01J33/00 , C01B3/56
CPC分类号： Y02P20/52
摘要： PROBLEM TO BE SOLVED: To provide a hydrogen production apparatus having a catalyst housing body in which an air permeable case is packed with pellet type catalyst of a quota evenly, being superior in hydrogen production efficiency, and preventing deterioration of a hydrogen separation body.SOLUTION: A hydrogen production apparatus 1 has a device shell 2, a hydrogen separation body 3, and a catalyst housing body 4. The catalyst housing body 4 is a unit in which a double tubular air permeable case 10 having a permeable inner peripheral wall 11 and outer peripheral wall 12 is packed with granular reforming catalyst 15. A plurality of catalyst housing bodies 4 is put on the hydrogen separation body 3 from outside and is arranged to be piled up within the device shell 2 by multistage. Reformed gas containing hydrogen gas is provided by source gas contacting with the reforming catalyst 15, and the hydrogen having passed through the hydrogen separation body 3 selectively is taken out from an extraction opening 6.
摘要翻译：要解决的问题：提供一种具有催化剂壳体的氢制造装置，其中透气性壳体均匀地填充有配量的颗粒状催化剂，氢生产效率优异，并且防止氢分离体的劣化。氢制造装置1具有装置壳体2，氢分离体3和催化剂壳体4.催化剂壳体4是具有透气性内周壁11和双层管状透气性壳体10的单体，外周壁12填充有粒状重整催化剂15.多个催化剂壳体4从外部放置在氢分离体3上，并且被布置成通过多段堆积在装置壳体2内。含有氢气的改性气体由与重整催化剂15接触的原料气提供，选择性地通过氢分离体3的氢从抽出口6取出。

3. 发明专利

JP2011195352A Apparatus for producing hydrogen 有权
标题翻译：生产氢气的装置
公开(公告)号：JP2011195352A
公开(公告)日：2011-10-06
申请号：JP2010061679
申请日：2010-03-17
申请人： Ngk Spark Plug Co Ltd , Tokyo Gas Co Ltd , 日本特殊陶業株式会社 , 東京瓦斯株式会社
发明人： NISHII TAKUMI , NAKAGAWA TOMOKI , TOMINAGA RYUICHI , IZEKI KOYA , SHIRASAKI YOSHINORI , YASUDA ISAMU , ITO MASAYA , TAKAGI YASUHIRO , SHIGAKI HIDEKAZU , HIKOSAKA HIDEAKI , TANAKA HIROYUKI
IPC分类号： C01B3/38 , B01D53/22 , B01D69/04 , B01D69/10 , C01B3/56
摘要： PROBLEM TO BE SOLVED: To obtain an apparatus for producing hydrogen capable of reducing pressure drop of gas to suppress an energy loss by shortening the gas passage in a reforming catalyst serving also as a support that has comparatively large resistance in a unified reforming catalyst module.SOLUTION: The apparatus for producing hydrogen is composed of an inserted tube having a hollow part through which each of a feed gas and an offgas flows, the reforming catalyst serving also as a support installed on the outer peripheral surface of the inserted tube, and a hydrogen separation membrane on the outer peripheral surface of the reforming catalyst serving also as a support. A partition for dividing the hollow part of the inserted tube in the longitudinal direction is installed at the center of the cross section of the hollow part to form two hollow parts in the longitudinal direction. Feed gas blowing holes are disposed on the wall opposite to the partition in the longitudinal direction of one hollow part of the inserted tube, while offgas discharge holes are disposed on the wall opposite to the partition in the longitudinal direction of the other hollow part of the inserted tube.
摘要翻译：要解决的问题：为了获得能够减少气体压降的氢气的装置，通过缩短在统一的重整催化剂组件中作为同时具有较大阻力的载体的重整催化剂中的气体通道来抑制能量损失。解决方案：用于生产氢的装置由具有中空部分的插入管组成，每个进料气体和废气流过该中空部分，重整催化剂也用作安装在插入管的外周表面上的载体，在还用作载体的重整催化剂的外周表面上的氢分离膜。插入管的中空部分沿纵向方向分隔的隔板安装在中空部分的横截面的中心处，以沿长度方向形成两个中空部分。进料气体吹入孔设置在与插入管的一个中空部分的纵向方向上的分隔壁相对的壁上，而废气排放孔设置在与隔板相对的壁上，插管。

4. 发明专利

JP2005314163A Reaction cylinder for and reaction plate for manufacturing hydrogen 有权
标题翻译：用于制造氢的反应釜和反应板
公开(公告)号：JP2005314163A
公开(公告)日：2005-11-10
申请号：JP2004133906
申请日：2004-04-28
申请人： Ngk Spark Plug Co Ltd , Tokyo Gas Co Ltd , 日本特殊陶業株式会社 , 東京瓦斯株式会社
发明人： YASUDA ISAMU , SHIRASAKI YOSHINORI , TSUNEKI TATSUYA , SHIMAMORI TORU , ISHIKAWA HIROYA , TANAKA HIROYUKI
IPC分类号： B01D53/22 , B01D63/06 , B01D63/08 , B01D69/10 , B01D71/02 , C01B3/38 , C01B3/56 , H01M8/06
CPC分类号： Y02E60/50
摘要： PROBLEM TO BE SOLVED: To provide such a reaction cylinder and a reaction plate each for use in an apparatus for manufacturing a hydrogen as is capable of solving that deterioration of a hydrogen permeability performance in a hydrogen permeable membrane which is caused by the interdiffusion of the components between a modified catalyst-cum-supporter material and the hydrogen-permeable membrane. SOLUTION: The reaction cylinder for use in an apparatus for manufacturing a hydrogen, comprising a cylindrical reforming catalyst-cum-supporter material and the hydrogen-permeable membrane arranged on the external circumferential surface of or the internal circumferential surface of the above reforming catalyst-cum-supporter material, is provided between the external circumferential surface of or the internal circumferential surface of the cylindrical reforming catalyst-cum-supporter material and the hydrogen-permeable membrane with a barrier layer for preventing the interdiffusion between the supporter component and the hydrogen-permeable membrane. Similarly, the reaction plate for use in an apparatus for manufacturing a hydrogen by using a plate-formed reforming catalyst-cum-supporter material, is also provided between this and the hydrogen-permeable membrane with a barrier layer for preventing the interdiffusion between the supporter component and the hydrogen-permeable membrane. COPYRIGHT: (C)2006,JPO&NCIPI
摘要翻译：要解决的问题：提供这样的反应缸和反应板，各自用于氢气制造装置，其能够解决由氢气渗透膜引起的氢渗透性能的劣化改性的催化剂 - 辅助材料与氢渗透膜之间的组分的相互扩散。解决方案：用于制造氢气的装置中的反应气缸，包括圆柱形重整催化剂 - 辅助材料和布置在上述重整单元的外圆周表面或内圆周表面上的氢透膜催化剂载体材料设置在圆筒形重整催化剂 - 载体材料的外圆周表面或内圆周表面和具有阻挡层的氢透过膜之间，用于防止支撑构件和支撑构件之间的相互扩散透氢膜。类似地，也可以使用用于通过使用板状重整催化剂 - 辅助材料的氢气制造装置的反应板，其与透氢膜之间设置有用于防止支撑体之间相互扩散的阻挡层组分和氢渗透膜。版权所有（C）2006，JPO＆NCIPI

5. 发明专利

JP2013071849A Hydrogen production apparatus 审中-公开
标题翻译：氢生产设备
公开(公告)号：JP2013071849A
公开(公告)日：2013-04-22
申请号：JP2011209604
申请日：2011-09-26
申请人： Ngk Spark Plug Co Ltd , 日本特殊陶業株式会社 , Tokyo Gas Co Ltd , 東京瓦斯株式会社
发明人： TANAKA HIROYUKI , TAKAGI YASUHIRO , HIKOSAKA HIDEAKI , IZEKI KOYA , KUME TAKAO , IKEDA YOICHI
IPC分类号： C01B3/38 , C01B3/56
摘要： PROBLEM TO BE SOLVED: To provide a hydrogen production apparatus preventing damage of a hydrogen separation layer, and having high capability for separating hydrogen from raw material gas.SOLUTION: A hydrogen separation cylinder 3 used in this hydrogen production apparatus 1 is constituted by combining a first molding 23 (for separating hydrogen) and a second molding 25 (for reforming raw material gas) which are different members, and at least a part of the surface of the second molding 25 has a contact with the surface of a porous ceramic protection layer 31 of the first molding 25. When the first molding 23 and the second molding 25 are arranged in contact with each other in this way, hydrogen can be separated and produced efficiently. Further, even when the first molding 23 and the second molding 25 which are different bodies are arranged in contact with each other, since there is a slight clearance 33 therebetween, even if stress is applied onto the first molding 23 and the second molding 25, there is such an advantage that a hydrogen separation layer 29 is hardly damaged.
摘要翻译：解决的问题：提供一种防止氢分离层损坏的氢制造装置，并且具有从原料气体分离氢的高能力。解决方案：在该氢气制备装置1中使用的氢气分离筒3通过组合作为不同构件的第一模制件23（用于分离氢气）和第二模制件25（用于重整原料气体），并且至少第二模制件25的表面的一部分与第一模制件25的多孔陶瓷保护层31的表面接触。当第一模塑件23和第二模塑件25以这种方式彼此接触时，可以有效地分离和生产氢。此外，即使不同体的第一模塑件23和第二模塑件25彼此接触，由于它们之间存在轻微的间隙33，即使在第一模塑件23和第二模塑件25上施加应力，存在氢分离层29几乎不被损坏的优点。版权所有（C）2013，JPO＆INPIT

6. 发明专利

JP2008246315A Hydrogen separation device and fuel cell 审中-公开
标题翻译：氢分离装置和燃料电池
公开(公告)号：JP2008246315A
公开(公告)日：2008-10-16
申请号：JP2007088670
申请日：2007-03-29
申请人： Ngk Spark Plug Co Ltd , Tokyo Gas Co Ltd , 日本特殊陶業株式会社 , 東京瓦斯株式会社
发明人： SHIGAKI HIDEKAZU , SHIMAMORI TORU , TANAKA HIROYUKI , MITSUYA KOHEI , NISHI MASARU , TSUNEKI TATSUYA , SHIRASAKI YOSHINORI , YASUDA ISAMU
IPC分类号： B01D53/22 , B01D63/00 , B01D71/02 , C01B3/38 , C01B3/56 , H01M8/06
CPC分类号： Y02E60/50
摘要： PROBLEM TO BE SOLVED: To provide a hydrogen separation device which has excellent sealability, and is unnecessary for performing brazing or the like for gas sealing.
SOLUTION: The hydrogen separation device includes: a porous support tube having both ends or one end opened; a dense ceramic molding bonded to one end side of the porous support tube with a bonding agent; a hydrogen-permeable membrane covering an exposure part of the bonding agent for bonding the porous support tube and the ceramic molding, and a part uncovered by the ceramic molding of the porous support tube, to make hydrogen gas selectively permeate; and a seal member provided on the outer peripheral surface of the ceramic molding.
COPYRIGHT: (C)2009,JPO&INPIT
摘要翻译：要解决的问题：提供一种具有优异的密封性的氢分离装置，并且不需要进行用于气体密封的钎焊等。解决方案：氢分离装置包括：具有两端或一端打开的多孔支撑管; 用粘结剂粘结在多孔支撑管的一端侧的致密陶瓷模制件; 覆盖多孔支撑管和陶瓷成型体的接合剂的曝光部的透氢性膜，以及多孔支撑管的陶瓷成形体未覆盖的部分，使氢气选择性渗透; 以及设置在陶瓷成型体的外周面上的密封部件。版权所有（C）2009，JPO＆INPIT

7. 发明专利

JP2007269595A Hydrogen production system 有权
标题翻译：氢生产系统
公开(公告)号：JP2007269595A
公开(公告)日：2007-10-18
申请号：JP2006099686
申请日：2006-03-31
申请人： Ngk Spark Plug Co Ltd , Tokyo Gas Co Ltd , 日本特殊陶業株式会社 , 東京瓦斯株式会社
发明人： MITSUYA KOHEI , SHIMAMORI TORU , SHIGAKI HIDEKAZU , TANAKA HIROYUKI , YASUDA ISAMU , SHIRASAKI YOSHINORI , TSUNEKI TATSUYA
IPC分类号： C01B3/56 , B01D53/22 , B01D69/10 , B01D71/02 , C01B3/38 , H01M8/06
CPC分类号： Y02E60/50
摘要： PROBLEM TO BE SOLVED: To provide a hydrogen production system which, while preventing the releasing or cracking of a porous support and a hydrogen-permeable membrane, prevents the diffusion and reaction between a metal component in the hydrogen-permeable membrane and a metal component in the porous substrate, and thus exhibits a long life even when used at a high temperature. SOLUTION: There is provided the hydrogen production system 1 having the following characteristics: an adhesion layer 3, a barrier layer 4, and the hydrogen-permeable membrane 5 are formed sequentially on the surface of the porous substrate 2; the porous substrate 2 contains a catalyst metal component; the hydrogen-permeable membrane 5 contains a hydrogen-permeable metal; the barrier layer 4 is a porous layer having a layer not containing the catalyst metal component; and the adhesion layer 3 is a porous layer having a thermal expansion coefficient between that of the porous substrate 2 and that of the barrier layer 4. There is also provided the hydrogen production system 1 having the following characteristics: an adhesion layer 3, a barrier layer 4, and a hydrogen-permeable membrane 5 are formed sequentially on the surface of the porous substrate 2; the porous substrate 2, the hydrogen-permeable membrane 5, and the barrier layer 4 are each the same as those described above; and the adhesion layer 3 is a porous layer containing the catalyst metal component in a quantity smaller than that contained in the porous substrate 2. COPYRIGHT: (C)2008,JPO&INPIT
摘要翻译：要解决的问题：提供一种氢制造系统，其在防止多孔载体和氢渗透膜的释放或破裂的同时，防止氢渗透膜中的金属成分与多孔基材中的金属成分，即使在高温下使用也显示出长寿命。解决方案：提供具有以下特征的氢气制备系统1：在多孔基材2的表面上依次形成粘合层3，阻挡层4和氢渗透膜5; 多孔基材2含有催化剂金属成分; 透氢膜5含有透氢性金属; 阻挡层4是具有不含催化剂金属成分的层的多孔层，并且粘合层3是具有在多孔基材2和阻挡层4的热膨胀系数之间的热膨胀系数的多孔层。还提供具有以下特征的氢气生产系统1：粘附层3，阻挡层层4和透氢膜5依次形成在多孔基材2的表面上; 多孔质基材2，透氢膜5和阻挡层4分别与上述相同; 粘合层3是含有比多孔质基材2中所含的催化剂金属成分少的多孔层。（C）2008，JPO＆INPIT

8. 发明专利

JP2007253066A Hydrogen-permeable membrane module and its manufacturing method 审中-公开
标题翻译：氢渗透膜模块及其制造方法
公开(公告)号：JP2007253066A
公开(公告)日：2007-10-04
申请号：JP2006080943
申请日：2006-03-23
申请人： Ngk Spark Plug Co Ltd , Tokyo Gas Co Ltd , 日本特殊陶業株式会社 , 東京瓦斯株式会社
发明人： YASUDA ISAMU , SHIRASAKI YOSHINORI , TSUNEKI TATSUYA , SHIMAMORI TORU , SHIGAKI HIDEKAZU , TANAKA HIROYUKI , MITSUYA KOHEI
IPC分类号： B01D63/00 , B01D53/22 , B01D63/06 , B01D69/10 , C01B3/38
摘要： PROBLEM TO BE SOLVED: To obtain a hydrogen-permeable membrane module, which is characterized in that the anxiety of a gas leak at its bonded part is eliminated, without using an inorganic adhesive, without exposing the hydrogen-permeable membrane module to a soldering temperature and requiring twice labor apprehended in preceding technique, and its manufacturing method.
SOLUTION: The hydrogen-permeable membrane module is constituted by joining a metal cap member to the outer peripheral surface of a cylindrical porous support or a cylindrical porous reforming catalyst and support and manufactured by a process (a) for joining the outer peripheral surface of the end part of the cylindrical porous support or the cylindrical porous reforming catalyst and support and the metal cap member by soldering using a metal solder material and a process (b) for forming a hydrogen-permeable membrane on the outer peripheral surface of the cylindrical porous support or the cylindrical porous reforming catalyst and support.
COPYRIGHT: (C)2008,JPO&INPIT
摘要翻译：要解决的问题：为了获得一种氢渗透膜组件，其特征在于消除了在其接合部分处的气体泄漏的焦虑，而不使用无机粘合剂，而不将氢渗透膜组件暴露于焊接温度及其前期技术要求两次劳动及其制造方法。解决方案：透氢膜组件通过将金属盖构件连接到圆柱形多孔载体的外周表面或圆柱形多孔重整催化剂和支撑体构成，并通过用于连接外周的方法（a）制造圆柱形多孔载体的端部表面或圆柱形多孔重整催化剂和支撑体和金属盖构件通过使用金属焊料材料进行焊接和用于在其外周表面上形成氢渗透膜的方法（b）圆柱形多孔载体或圆柱形多孔重整催化剂和载体。版权所有（C）2008，JPO＆INPIT

9. 发明专利

JP2006314876A Hydrogen separator 审中-公开
标题翻译：氢分离器
公开(公告)号：JP2006314876A
公开(公告)日：2006-11-24
申请号：JP2005138195
申请日：2005-05-11
申请人： Ngk Spark Plug Co Ltd , Tokyo Gas Co Ltd , 日本特殊陶業株式会社 , 東京瓦斯株式会社
发明人： TANAKA HIROYUKI , SHIMAMORI TORU , SHIGAKI HIDEKAZU , YASUDA ISAMU , SHIRASAKI YOSHINORI , TSUNEKI TATSUYA
IPC分类号： B01D53/22 , B01D69/10 , C01B3/56
摘要： PROBLEM TO BE SOLVED: To provide a hydrogen separator capable of separating a high-purity hydrogen gas.
SOLUTION: The hydrogen separator 1 comprises a porous support 10 and a hydrogen permeable membrane 20 supported by the porous support 10, wherein the hydrogen permeable membrane 20 has a membrane thickness of 1 to 30 μm and 0.010 pieces/cm
2 or smaller of surface defects.
COPYRIGHT: (C)2007,JPO&INPIT

10. 发明专利

JP2015033656A 水素分離体及びその製造方法有权
标题翻译：氢分离体及其生产方法
公开(公告)号：JP2015033656A
公开(公告)日：2015-02-19
申请号：JP2013164273
申请日：2013-08-07
申请人：日本特殊陶業株式会社 , Ngk Spark Plug Co Ltd , 東京瓦斯株式会社 , Tokyo Gas Co Ltd
发明人： KAWASE HIROKI , KAJITANI MASAHIRO , TANAKA HIROYUKI , HIKOSAKA HIDEAKI , TAKAGI YASUHIRO , ITO MASAYA , IKEDA YOICHI , KUME TAKAO
IPC分类号： B01D71/02 , B01D69/10 , B01D69/12
摘要：【課題】水素透過性能が高い水素分離体及びその製造方法を提供すること。【解決手段】多孔質層(19)と、多孔質層(19)の内部に設けられ、水素を含む気体のうち水素のみを選択して透過させる水素分離金属が充填された水素分離層(17)と、を備えた水素分離体(1)であり、多孔質層(19)のうち、水素分離層(17)に隣接する水素を含む気体が供給される側の厚み5μm以内の範囲では、多孔質層(19)の構成材料及び水素分離金属以外の無機の元素の濃度の平均が0.30atm%以下である。【選択図】図3
摘要翻译：要解决的问题：提供具有高透氢性的氢分离体及其制造方法。氢分离体（1）包括：多孔层（19）; 以及设置在所述多孔层（19）内并且填充有氢分离金属的氢分离层（17），所述氢分离金属在含氢气体中仅选择性渗透氢气。在与氢分离层（17）相邻的一侧的厚度范围内，多孔层（19）的构成材料和氢分离金属以外的无机元素的平均浓度为0.30atm％以下，并且在多孔层（19）中供给含氢气体。

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