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1. 发明授权

US07094841B2 Primer composition and bonding method 有权
公开(公告)号：US07094841B2
公开(公告)日：2006-08-22
申请号：US10865938
申请日：2004-06-14
申请人： Yoshimichi Yamanaka
发明人： Yoshimichi Yamanaka
IPC分类号： C08L83/16 , C08G77/38
CPC分类号： C08K5/541 , C08K5/0091 , C08L83/04 , C09D123/22 , Y10T428/31663 , C08L23/22 , C08L2666/28 , C08L83/00
摘要： This invention provides a primer composition comprising the following (A), (B), (C) and (D) components: (A) a saturated hydrocarbon polymer having at least one alkenyl group per molecule, (B) a silane coupling agent, (C) a polyvalent alkoxysilane and/or a condensation product thereof, and (D) an organoaluminum compound and/or an organotitanium compound.

2. 发明授权

US06303728B1 Hydrosilylation process and polymers produced by the process 失效
标题翻译：通过该方法制备的氢化硅烷化方法和聚合物
公开(公告)号：US06303728B1
公开(公告)日：2001-10-16
申请号：US09462467
申请日：2000-03-03
申请人： Shigeru Hagimori , Koji Tsuneishi , Yoshimichi Yamanaka , Syun Wachi , Kazuya Yonezawa
发明人： Shigeru Hagimori , Koji Tsuneishi , Yoshimichi Yamanaka , Syun Wachi , Kazuya Yonezawa
IPC分类号： C08G7708
CPC分类号： C08F8/42
摘要： The present invention has its object to provide an effective method of accelerating a hydrosilylation reaction. This invention is related to a hydrosilylation reaction method which comprises carrying out the hydrosilylation reaction between a silicon compound (A) represented by the following general formula (1) and an alkenyl group-containing compound (B) in the presence of a Group VIII metal-containing catalyst (C) and a sulfur compound (D); RaXbHcSi (1).
摘要翻译：本发明的目的是提供一种加氢氢化反应的有效方法。本发明涉及一种氢化硅烷化反应方法，包括进行下述通式（1）表示的硅化合物（A）和含有烯基的化合物（B）在含Ⅷ族金属催化剂（C）和硫化合物（D）的存在下反应;

3. 发明授权

US5777037A Process for producing isobutylene polymer 失效
标题翻译：制备异丁烯聚合物的方法
公开(公告)号：US5777037A
公开(公告)日：1998-07-07
申请号：US585515
申请日：1996-01-16
申请人： Yoshimichi Yamanaka , Hiroshi Fujisawa , Takeshi Chiba , Yoshikuni Deguchi , Kazuya Yonezawa
发明人： Yoshimichi Yamanaka , Hiroshi Fujisawa , Takeshi Chiba , Yoshikuni Deguchi , Kazuya Yonezawa
IPC分类号： C08F2/06 , C08F2/38 , C08F4/06 , C08F4/14 , C08F8/00 , C08F10/00 , C08F10/10 , C08F110/10 , C08F290/00 , C08F299/00 , C08F4/16
CPC分类号： C08F10/00 , C08F10/10 , C08F110/10 , Y10S525/918
摘要： The present invention provides a novel solvent which is capable of providing an excellent isobutylene polymer, little affects the environment, has a lower solubility in water than those of halogenated hydrocarbons having 1 or 2 carbon atoms and can be decomposed relatively easily. Namely, the present invention relates to: a process for producing an isobutylene polymer, which comprises performing a cationic polymerization reaction in a solvent containing primary and/or secondary monohalogenated hydrocarbon(s) having 3 to 8 carbon atoms, and an isobutylene polymer thus obtained; and a process for producing an isobutylene polymer having a vinyl group introduced into the terminal thereof, which comprises reacting the isobutylene polymer produced above with 1,9-decadiene or allyltrimethylsilane, and an isobutylene polymer thus obtained.
摘要翻译：本发明提供能够提供优异的异丁烯聚合物的新型溶剂，对环境影响小，在水中的溶解度低于具有1或2个碳原子的卤代烃的溶解度，并且可以相对容易地分解。即，本发明涉及：异丁烯系聚合物的制造方法，其包括在含有碳原子数为3〜8的一次和/或仲一卤化烃的溶剂中进行阳离子聚合反应，得到异丁烯系聚合物 ; 以及制造其末端具有乙烯基的异丁烯聚合物的方法，其包括使上述制备的异丁烯聚合物与1,9-癸二烯或烯丙基三甲基硅烷和由此获得的异丁烯聚合物反应。

4. 发明授权

US06320010B1 Curable composition 失效
标题翻译：可固化组合物
公开(公告)号：US06320010B1
公开(公告)日：2001-11-20
申请号：US09462904
申请日：2000-03-27
申请人： Masashi Sakaguchi , Yoshimichi Yamanaka , Hidenari Tsunemi
发明人： Masashi Sakaguchi , Yoshimichi Yamanaka , Hidenari Tsunemi
IPC分类号： C08G7720
CPC分类号： C08L23/02 , C08K5/5419 , C08L23/22 , C08L83/04 , C08L2666/02 , C08L83/00
摘要： By incorporating (A) a saturated hydrocarbon polymer having more than one alkenyl group capable of being hydrosilylated in each molecule and having a molecular weight of 2,000 to 50,000, (B) a component comprising a compound containing more than two silicon atom-bound hydrogen atoms, on average, in each molecule, (C) a compound having, within the molecule, one alkenyl group capable of being hydrosilylated, (D) a compound having, within the molecule, at least two alkenyl groups capable of being hydrosilylated and having a molecular weight less than 2,000, and (E) a hydrosilylation catalyst, a composition having good mechanical characteristics, a high gel fraction and a small heating loss can be obtained. As a result, the invention can provide a composition to secure the uniformity within a wide range of selection not depending on its viscosity, because it is markedly relaxed the restriction on SiH-containing compounds that are curing agents possibly becoming a cause of said insufficient curing.
摘要翻译：通过并入（A）具有多于一个能够在每个分子中进行氢化硅烷化的链烯基并且分子量为2,000至50,000的饱和烃聚合物，（B）包含含有多于两个硅原子键合的氢原子的化合物平均来说，在每个分子中，（C）在分子内具有一个能够被氢化硅烷基化的烯基的化合物，（D）在分子内具有至少两个能够被氢化硅烷化并且具有分子量小于2,000，和（E）氢化硅烷化催化剂，可以获得具有良好机械特性，高凝胶分数和小的加热损失的组合物。结果，本发明可以提供一种组合物，以确保在宽范围的选择范围内的均匀性，而不依赖于其粘度，因为显着地松弛了对含有SiH的化合物的限制，这些化合物是可能成为固化不足的原因的固化剂。

5. 发明授权

US5811501A Process for producing unsaturated group-terminated isobutylene polymer 失效
标题翻译：制备不饱和基团的异丁烯聚合物的方法
公开(公告)号：US5811501A
公开(公告)日：1998-09-22
申请号：US671198
申请日：1996-06-27
申请人： Takeshi Chiba , Hiroshi Fujisawa , Yoshimichi Yamanaka , Yoshikuni Deguchi , Kazuya Yonezawa
发明人： Takeshi Chiba , Hiroshi Fujisawa , Yoshimichi Yamanaka , Yoshikuni Deguchi , Kazuya Yonezawa
IPC分类号： C08F2/06 , C08F10/10
CPC分类号： C08F10/10 , Y10S525/918
摘要： The present invention provides a novel halogen-free solvent system which can produce a good isobutylene polymer and can be easily reused. A novel process for the production of an isobutylene polymer is provided which comprises using a hydrocarbon solvent having a boiling point of not lower than 105.degree. C. and a melting point of not higher than -90.degree. C. Heretofore, a solvent system containing a halogenated hydrocarbon such as methylene chloride has been used for the production of an isobutylene polymer. However, such a solvent system has a great adverse effect on the environment. Therefore, a non-halogenated solvent is desirable. The present invention is characterized by the use of a hydrocarbon solvent as a reaction solvent. The resulting polymer has good properties. Further, compounds which are produced as by-products during the reaction can be easily removed, enabling the recycling of the solvent used. Thus, the production cost can be reduced.
摘要翻译：本发明提供了一种新型的无卤素溶剂体系，其可以产生良好的异丁烯聚合物并且可以容易地重复使用。提供了一种生产异丁烯聚合物的新方法，其包括使用沸点不低于105℃，熔点不高于-90℃的烃溶剂。迄今为止，含有卤代烃如二氯甲烷已被用于生产异丁烯聚合物。然而，这种溶剂体系对环境有很大的不利影响。因此，非卤化溶剂是理想的。本发明的特征在于使用烃溶剂作为反应溶剂。所得聚合物具有良好的性能。此外，可以容易地除去在反应期间作为副产物生成的化合物，使得所用溶剂的再循环。因此，可以降低生产成本。

6. 发明授权

US06773758B2 Primer composition and bonding method 失效
标题翻译：底漆组成和粘合方法
公开(公告)号：US06773758B2
公开(公告)日：2004-08-10
申请号：US09854474
申请日：2001-05-15
申请人： Yoshimichi Yamanaka
发明人： Yoshimichi Yamanaka
IPC分类号： B05D136
CPC分类号： C08K5/541 , C08K5/0091 , C08L83/04 , C09D123/22 , Y10T428/31663 , C08L23/22 , C08L2666/28 , C08L83/00
摘要： This invention provides a primer composition comprising the following (A), (B), (C) and (D) components: (A) a saturated hydrocarbon polymer having at least one alkenyl group per molecule, (B) a silane coupling agent, (C) a polyvalent alkoxysilane and/or a condensation product thereof, and (D) an organoaluminum compound and/or an organotitanium compound.
摘要翻译：本发明提供了包含以下（A），（B），（C）和（D）成分的底漆组合物：（A）每分子具有至少一个烯基的饱和烃聚合物，（B）硅烷偶联剂，（C）多价烷氧基硅烷和/或其缩合产物，和（D）有机铝化合物和/或有机钛化合物。

7. 发明授权

US6121379A Processes for producing polymers having functional groups 失效
标题翻译：制备具有官能团的聚合物的方法
公开(公告)号：US6121379A
公开(公告)日：2000-09-19
申请号：US77374
申请日：1998-08-06
申请人： Yoshimichi Yamanaka , Yoshikuni Deguchi , Naoki Furukawa , Shigeru Hagimori , Shun Wachi
发明人： Yoshimichi Yamanaka , Yoshikuni Deguchi , Naoki Furukawa , Shigeru Hagimori , Shun Wachi
IPC分类号： C08F8/42 , C08L23/22
CPC分类号： C08F8/42
摘要： A process for producing organic polymers having silicon containing groups in high yields comprises hydrosilylating a polymer having unsaturated groups with a hydrosilicon compound. This process includes keeping the polymer and a solvent in an inert gas environment and introducing oxygen into the reactor just before starting the hydrosilylation reaction.
摘要翻译： PCT No.PCT / JP96 / 03461 Sec。 371日期1998年8月6日 102（e）1998年8月6日PCT PCT 1996年11月27日PCT公布。公开号WO97 / 19962 日期：1997年6月5日以高产率制备含硅基团的有机聚合物的方法包括使具有不饱和基团的聚合物与氢硅烷化合物进行氢化硅烷基化。该方法包括将聚合物和溶剂保持在惰性气体环境中，并在开始氢化硅烷化反应之前将氧气引入反应器。

8. 发明授权

US6087456A Curable composition 失效
标题翻译：可固化组合物
公开(公告)号：US6087456A
公开(公告)日：2000-07-11
申请号：US977741
申请日：1997-11-25
申请人： Masashi Sakaguchi , Yoshimichi Yamanaka , Makoto Chiba , Toshihiko Okamoto , Yuriko Asai , Jyunji Takase
发明人： Masashi Sakaguchi , Yoshimichi Yamanaka , Makoto Chiba , Toshihiko Okamoto , Yuriko Asai , Jyunji Takase
IPC分类号： C08F8/42 , C08L43/04 , C08L25/02
CPC分类号： C08F8/42
摘要： A curable composition comprising the components (A), (B), (C) and (D), viz.(A) an isobutylene polymer which contains in a molecule, at least one alkenyl group capable of hydrosilylation reaction;(B) a curing agent which contains at least two hydrosilyl groups in a molecule;(C) a hydrosilylation catalyst; and(D) an organic compound which contains in a molecule, at least one alkenyl or alkynyl group capable of hydrosilylation reaction.This composition is excellent in workability because of its low viscosity, and has such advantages that the cured product thereof has large strength and further that the weight loss by heating is small. Since a large amount of an inorganic filler can be blended with this composition, it is possible to obtain a composition having high thixotropy and little sagging.
摘要翻译：包含组分（A），（B），（C）和（D）的可固化组合物，（A）在分子中含有至少一个能够进行氢化硅烷化反应的链烯基的异丁烯聚合物; （B）在分子中含有至少两个氢化硅烷基的固化剂; （C）氢化硅烷化催化剂; 和（D）在分子中含有至少一个能够进行氢化硅烷化反应的烯基或炔基的有机化合物。该组合物由于其低粘度而具有优异的可加工性，并且具有这样的优点，即其固化产物具有较大的强度，进一步减少加热失重。由于可以将大量的无机填料与该组合物共混，所以可以获得具有高触变性和低流挂性的组合物。

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