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1. 发明授权

US06303728B1 Hydrosilylation process and polymers produced by the process 失效
标题翻译：通过该方法制备的氢化硅烷化方法和聚合物
公开(公告)号：US06303728B1
公开(公告)日：2001-10-16
申请号：US09462467
申请日：2000-03-03
申请人： Shigeru Hagimori , Koji Tsuneishi , Yoshimichi Yamanaka , Syun Wachi , Kazuya Yonezawa
发明人： Shigeru Hagimori , Koji Tsuneishi , Yoshimichi Yamanaka , Syun Wachi , Kazuya Yonezawa
IPC分类号： C08G7708
CPC分类号： C08F8/42
摘要： The present invention has its object to provide an effective method of accelerating a hydrosilylation reaction. This invention is related to a hydrosilylation reaction method which comprises carrying out the hydrosilylation reaction between a silicon compound (A) represented by the following general formula (1) and an alkenyl group-containing compound (B) in the presence of a Group VIII metal-containing catalyst (C) and a sulfur compound (D); RaXbHcSi (1).
摘要翻译：本发明的目的是提供一种加氢氢化反应的有效方法。本发明涉及一种氢化硅烷化反应方法，包括进行下述通式（1）表示的硅化合物（A）和含有烯基的化合物（B）在含Ⅷ族金属催化剂（C）和硫化合物（D）的存在下反应;

2. 发明授权

US5777037A Process for producing isobutylene polymer 失效
标题翻译：制备异丁烯聚合物的方法
公开(公告)号：US5777037A
公开(公告)日：1998-07-07
申请号：US585515
申请日：1996-01-16
申请人： Yoshimichi Yamanaka , Hiroshi Fujisawa , Takeshi Chiba , Yoshikuni Deguchi , Kazuya Yonezawa
发明人： Yoshimichi Yamanaka , Hiroshi Fujisawa , Takeshi Chiba , Yoshikuni Deguchi , Kazuya Yonezawa
IPC分类号： C08F2/06 , C08F2/38 , C08F4/06 , C08F4/14 , C08F8/00 , C08F10/00 , C08F10/10 , C08F110/10 , C08F290/00 , C08F299/00 , C08F4/16
CPC分类号： C08F10/00 , C08F10/10 , C08F110/10 , Y10S525/918
摘要： The present invention provides a novel solvent which is capable of providing an excellent isobutylene polymer, little affects the environment, has a lower solubility in water than those of halogenated hydrocarbons having 1 or 2 carbon atoms and can be decomposed relatively easily. Namely, the present invention relates to: a process for producing an isobutylene polymer, which comprises performing a cationic polymerization reaction in a solvent containing primary and/or secondary monohalogenated hydrocarbon(s) having 3 to 8 carbon atoms, and an isobutylene polymer thus obtained; and a process for producing an isobutylene polymer having a vinyl group introduced into the terminal thereof, which comprises reacting the isobutylene polymer produced above with 1,9-decadiene or allyltrimethylsilane, and an isobutylene polymer thus obtained.
摘要翻译：本发明提供能够提供优异的异丁烯聚合物的新型溶剂，对环境影响小，在水中的溶解度低于具有1或2个碳原子的卤代烃的溶解度，并且可以相对容易地分解。即，本发明涉及：异丁烯系聚合物的制造方法，其包括在含有碳原子数为3〜8的一次和/或仲一卤化烃的溶剂中进行阳离子聚合反应，得到异丁烯系聚合物 ; 以及制造其末端具有乙烯基的异丁烯聚合物的方法，其包括使上述制备的异丁烯聚合物与1,9-癸二烯或烯丙基三甲基硅烷和由此获得的异丁烯聚合物反应。

3. 发明授权

US5811501A Process for producing unsaturated group-terminated isobutylene polymer 失效
标题翻译：制备不饱和基团的异丁烯聚合物的方法
公开(公告)号：US5811501A
公开(公告)日：1998-09-22
申请号：US671198
申请日：1996-06-27
申请人： Takeshi Chiba , Hiroshi Fujisawa , Yoshimichi Yamanaka , Yoshikuni Deguchi , Kazuya Yonezawa
发明人： Takeshi Chiba , Hiroshi Fujisawa , Yoshimichi Yamanaka , Yoshikuni Deguchi , Kazuya Yonezawa
IPC分类号： C08F2/06 , C08F10/10
CPC分类号： C08F10/10 , Y10S525/918
摘要： The present invention provides a novel halogen-free solvent system which can produce a good isobutylene polymer and can be easily reused. A novel process for the production of an isobutylene polymer is provided which comprises using a hydrocarbon solvent having a boiling point of not lower than 105.degree. C. and a melting point of not higher than -90.degree. C. Heretofore, a solvent system containing a halogenated hydrocarbon such as methylene chloride has been used for the production of an isobutylene polymer. However, such a solvent system has a great adverse effect on the environment. Therefore, a non-halogenated solvent is desirable. The present invention is characterized by the use of a hydrocarbon solvent as a reaction solvent. The resulting polymer has good properties. Further, compounds which are produced as by-products during the reaction can be easily removed, enabling the recycling of the solvent used. Thus, the production cost can be reduced.
摘要翻译：本发明提供了一种新型的无卤素溶剂体系，其可以产生良好的异丁烯聚合物并且可以容易地重复使用。提供了一种生产异丁烯聚合物的新方法，其包括使用沸点不低于105℃，熔点不高于-90℃的烃溶剂。迄今为止，含有卤代烃如二氯甲烷已被用于生产异丁烯聚合物。然而，这种溶剂体系对环境有很大的不利影响。因此，非卤化溶剂是理想的。本发明的特征在于使用烃溶剂作为反应溶剂。所得聚合物具有良好的性能。此外，可以容易地除去在反应期间作为副产物生成的化合物，使得所用溶剂的再循环。因此，可以降低生产成本。

4. 发明授权

US5652276A Foaming resin composition, plastic foam formed from the composition, and method for forming the plastic foam 失效
标题翻译：发泡树脂组合物，由组合物形成的塑料泡沫以及形成塑料泡沫的方法
公开(公告)号：US5652276A
公开(公告)日：1997-07-29
申请号：US669301
申请日：1996-09-05
申请人： Hiroshi Ando , Kensuke Kondo , Naoaki Nakanishi , Hiroshi Ito , Shigeki Hamaguchi , Kazuya Yonezawa
发明人： Hiroshi Ando , Kensuke Kondo , Naoaki Nakanishi , Hiroshi Ito , Shigeki Hamaguchi , Kazuya Yonezawa
IPC分类号： C08J9/00 , C08J9/02 , C08J9/06
CPC分类号： C08J9/02 , C08J9/0061 , C08J2383/04
摘要： A foaming resin composition consisting essentially of (A) an organic compound having a carbon-carbon double bond, (B) a compound having an SiH group, and (C) a compound having an OH group is foamed and cured at room temperature or under heat at relatively low temperatures, to obtain hard, semi-hard or soft plastic foam having good weather resistance and good compatibility with coating compositions and adhesives.
摘要翻译： PCT No.PCT / JP95 / 02335 Sec。 371日期：1996年9月5日 102（e）日期1996年9月5日PCT 1995年11月15日PCT PCT。出版物WO96 / 15194 日期1996年5月23日发泡树脂组合物主要由（A）具有碳 - 碳双键的有机化合物，（B）具有SiH基团的化合物和（C）具有OH基团的化合物组成的发泡树脂组合物发泡固化室温或在相对低的温度下加热，以获得具有良好耐候性和与涂料组合物和粘合剂的良好相容性的硬质，半硬或软塑料泡沫。

5. 发明授权

US5177173A Heat-resting aromatic polyestersulfone and process for preparing the same 失效
标题翻译：热稳定性芳族聚酯和其制备方法
公开(公告)号：US5177173A
公开(公告)日：1993-01-05
申请号：US583820
申请日：1984-02-27
申请人： Hiroshi Iwakiri , Masahiro Asada , Kazuya Yonezawa
发明人： Hiroshi Iwakiri , Masahiro Asada , Kazuya Yonezawa
IPC分类号： C08G63/00 , B32B27/36 , C08G63/18 , C08G63/19 , C08G63/68 , C08G63/688 , C08G63/82
CPC分类号： C08G63/6886
摘要： An aromatic polyestersulfone having improved heat resistance, film-forming property, hydrolysis resistance and mechanical strength which comprises 1 to 100% by mole of recurring units of the general formula: ##STR1## and 99 to 0% by mole of recurring units of the general formula: ##STR2## wherein R and R' are the same or different and each is an alkyl or alkoxyl group having 1 to 4 carbon atoms, Ar is a bivalent aromatic group, and x and y are 0 or an integer of 1 to 4 provided that the sum of x and y is from 1 to 8.
摘要翻译：具有改善的耐热性，成膜性，耐水解性和机械强度的芳族聚酯砜，其包含1至100摩尔％的通式为：IMAGE的重复单元和99至0摩尔％的一般重复单元式：其中R和R'相同或不同，并且各自为具有1至4个碳原子的烷基或烷氧基，Ar为二价芳族基团，x和y为0或1至4的整数条件是x和y的和为1至8。

6. 发明授权

US4334036A Process for producing curable vinyl polymer having silyl group 失效
标题翻译：制备具有甲硅烷基的可固化乙烯基聚合物的方法
公开(公告)号：US4334036A
公开(公告)日：1982-06-08
申请号：US167657
申请日：1980-07-11
申请人： Kazuya Yonezawa , Hisao Furukawa , Masaaki Azuma
发明人： Kazuya Yonezawa , Hisao Furukawa , Masaaki Azuma
IPC分类号： C08F8/42 , C08F8/34 , C08F236/02
CPC分类号： C08F8/42
摘要： A curable vinyl polymer having at least one silyl group of the formula: ##STR1## wherein R.sub.1 and R.sub.2 are each a hydrogen or a monovalent hydrocarbon radical having 1 to 10 carbon atoms, X is a group selected from halogen, alkoxy, acryloxy, aminoxy, phenoxy, thioalkoxy and amino groups; and "a" is a whole number equal to 0, 1 or 2, and having molecular weight of between 200 and 30,000, preferably between 1,500 and 25,000; and method for producing same, and products comprised of same; and wherein said method comprises reacting hydrosilane represented by the formula: ##STR2## wherein the same designations as above apply, with a polymer having carbon-carbon double bonds in the terminal or side chains of the polymer in which the main chain is a vinyl polymer having a molecular weight of between 200 and 30,000, and at a temperature of between 50.degree. and 150.degree. C.
摘要翻译：一种具有至少一个具有下式的甲硅烷基的可固化乙烯基聚合物：其中R 1和R 2各自为氢或具有1-10个碳原子的一价烃基，X为选自卤素，烷氧基，丙烯酰氧基，氨基，苯氧基，硫代烷氧基和氨基; 和“a”是等于0,1或2的整数，分子量在200至30,000之间，优选在1,500至25,000之间; 及其制造方法及其制造方法。并且其中所述方法包括使由下式表示的氢硅烷：其中与上述相同的名称适用于具有碳 - 碳双键的聚合物的聚合物的末端或侧链中的聚合物，其中主链是乙烯基聚合物分子量为200至30,000，温度为50至150℃。

7. 发明授权

US4191714A Curable polyester oligomer and a process for producing same 失效
标题翻译：可固化聚酯低聚物及其制备方法
公开(公告)号：US4191714A
公开(公告)日：1980-03-04
申请号：US973889
申请日：1978-12-28
申请人： Kazuya Yonezawa , Yasushi Kato , Hisao Furukawa , Masaaki Azuma
发明人： Kazuya Yonezawa , Yasushi Kato , Hisao Furukawa , Masaaki Azuma
IPC分类号： C08G63/695 , C08L83/12 , C08L43/04
CPC分类号： C08G63/695
摘要： A curable polyester oligomer having a molecular weight of between 300 and 10,000 and at least one silyl radical at the side chain or at the end of the molecule, with the silyl radical being represented by the formula: ##STR1## wherein R, R.sub.1 and R.sub.2 represent hydrogen or any monovalent hydrocarbon radical with 1 to 10 carbon atoms, selected from the group consisting of alkyl radical, aryl radical and aralkyl radical; R.sub.3 represents divalent hydrocarbon radical with 0 to 10 carbon atoms, "X" represents any radical selected from the group consisting of halogen, alkoxy, acyloxy, aminoxy, phenoxy, thioalkoxy, and amino radicals; "a" is an integer 0, 1 or 2; and "b" is an integer 0 or 1.
摘要翻译：分子量为300至10,000的可固化的聚酯低聚物和分子侧链或末端的至少一个甲硅烷基，其中甲硅烷基由下式表示：其中R，R 1和R 2 表示氢或具有1至10个碳原子的任何一价烃基，其选自烷基，芳基和芳烷基; R3表示具有0至10个碳原子的二价烃基，“X”表示选自卤素，烷氧基，酰氧基，氨氧基，苯氧基，硫代烷氧基和氨基的任何基团; “a”是整数0,1或2; “b”为整数0或1。

8. 发明授权

US4161572A Curable diallyl phthalate compounds and process for producing same 失效
标题翻译：可固化邻苯二甲酸二烯丙酯化合物及其制备方法
公开(公告)号：US4161572A
公开(公告)日：1979-07-17
申请号：US936378
申请日：1978-08-24
申请人： Kazuya Yonezawa , Hisao Furukawa , Masaaki Azuma
发明人： Kazuya Yonezawa , Hisao Furukawa , Masaaki Azuma
IPC分类号： C08F8/00 , C08F8/42 , C08F30/00 , C08F30/08 , C09D4/00 , C09J131/00 , C09J137/00 , C08F8/18 , C08F8/32 , C08F8/34
CPC分类号： C08F8/42
摘要： Diallyl Phthalate compounds having a molecular weight of 250 to 20,000 and having at least one silyl group represented by the formula: ##STR1## wherein R.sub.1, R.sub.2 and R.sub.3 are each a hydrogen or a monovalent hydrocarbon radicals having 1 to 10 carbon atoms, such as alkyl, aryl or aralkyl radicals; X is a group selected from halogen, alkoxy, acryloxy, aminoxy, phenoxy, thioalkoxy and amino groups, and "a" is an integer 0, 1 or 2, in the molecule; and process for producing same wherein a diallyl phthalate monomer or prepolymer having molecular weight of 20,000 or less is reacted with a hydrosilane compound having the formula: ##STR2## WHEREIN THE DESIGNATIONS ARE THE SAME AS ABOVE, AND AT A TEMPERATURE WITHIN THE RANGE OF 50.degree. TO 150.degree. C.
摘要翻译：具有250至20,000分子量的具有至少一个由下式表示的甲硅烷基的邻苯二甲酸二烯丙酯化合物：其中R 1，R 2和R 3各自为氢或具有1至10个碳原子的一价烃基，例如烷基，芳基或芳烷基; X是选自卤素，烷氧基，丙烯酰氧基，氨氧基，苯氧基，硫代烷氧基和氨基的基团，“a”是分子中0,1或2的整数; 和其制备方法，其中分子量为20,000以下的邻苯二甲酸二烯丙酯单体或预聚物与具有下列结构式的氢化硅烷化合物反应：其中指定为上述，在50℃范围内的温度下 ℃至150℃

9. 发明授权

US5728791A Polyvinyl graft-polymers and manufacturing method thereof 失效
标题翻译：聚乙烯基接枝聚合物及其制备方法
公开(公告)号：US5728791A
公开(公告)日：1998-03-17
申请号：US557329
申请日：1995-11-14
申请人： Kazuhiko Tamai , Kazuya Yonezawa
发明人： Kazuhiko Tamai , Kazuya Yonezawa
IPC分类号： C08F291/00 , C08F24/00 , C08F12/08 , C08F16/14 , C08F20/18 , C08F20/42 , C08F269/00
CPC分类号： C08F291/00
摘要： The present invention provides a polyvinyl graft-polymer having one structural unit having a glycidyloxy group represented by the following general formula (I) at side chains of the polyvinyl polymer per 2-1,000 repeating units of vinyl: ##STR1## wherein Ar represents an aromatic hydrocarbon group 6-23 in carbon number having at least one glycidyloxy group, and R represents hydrogen atom or methyl group, and its manufacturing method. The polyvinyl graft-polymer of the present invention is excellent not only in mechanical properties and heat resistance, but also in adhesiveness, paintability dyeability and antistatic property.
摘要翻译：本发明提供一种具有一个结构单元的聚乙烯基接枝聚合物，每个2-1,000个乙烯基重复单元在聚乙烯基聚合物的侧链上具有由以下通式（I）表示的缩水甘油氧基：其中Ar 表示具有至少一个缩水甘油基氧基的碳数为6-23的芳族烃基，R表示氢原子或甲基，及其制造方法。本发明的聚乙烯基接枝聚合物不仅具有机械性能和耐热性，而且在粘合性，可着色性和抗静电性方面也是优异的。

10. 发明授权

US5567833A Curing agent, preparation thereof and curable composition comprising the same 失效
公开(公告)号：US5567833A
公开(公告)日：1996-10-22
申请号：US313923
申请日：1994-09-26
申请人： Takahisa Iwahara , Makoto Chiba , Tomoko Takahara , Kazuya Yonezawa
发明人： Takahisa Iwahara , Makoto Chiba , Tomoko Takahara , Kazuya Yonezawa
IPC分类号： C07F7/08 , C07F7/21 , C08G65/336 , C08G77/48 , C08G77/50 , C08K5/54 , C08L43/04 , C08L71/00 , C08L101/10
CPC分类号： C08L71/00 , C07F7/0896 , C07F7/21 , C08G65/336 , C08G77/48 , C08G77/50 , C08K5/54 , C08L101/10 , C08L43/04
摘要： A curable composition which comprises(C) a non-polymeric organic curing agent having at least two hydrosilyl groups in a molecule,(D) an organic polymer having at least one alkenyl group in a molecule, and(E) a hydrosilylation catalysthas rapid curability and good depth curability, and gives a homogeneous cured material having good mechanical properties.

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